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1. 发明申请

US20060074267A1 Aluminophosphate molecular sieve, its synthesis and use 有权
公开(公告)号：US20060074267A1
公开(公告)日：2006-04-06
申请号：US11231677
申请日：2005-09-21
申请人： Guang Cao , Matu Shah , John Brody , Douglas Dorset , Karl Strohmaier
发明人： Guang Cao , Matu Shah , John Brody , Douglas Dorset , Karl Strohmaier
IPC分类号： C07C1/00 , C01B37/04 , C01B37/06
CPC分类号： C07C1/20 , B01J29/83 , B01J29/85 , C01B37/04 , C01B37/08 , C01B39/54 , C10G3/00 , C10G3/49 , C10G2400/20 , C07C11/02
摘要： A large pore (metallo)aluminophosphate molecular sieve is disclosed The material has an X-ray diffraction pattern including the lines listed in Table 4 and is synthesized in the presence of 4-dimethylaminopyridine as structure directing agent.

2. 发明申请

US20070286799A1 Aluminophosphate Molecular Sieve, Its Synthesis and Use 失效
标题翻译：磷酸铝分子筛，其合成与应用
公开(公告)号：US20070286799A1
公开(公告)日：2007-12-13
申请号：US11663716
申请日：2005-09-12
申请人： Guang Cao , Matu Shah
发明人： Guang Cao , Matu Shah
IPC分类号： C01B39/00 , C01B33/36
CPC分类号： C01B39/54 , B01J29/83 , B01J29/85 , C01B37/04 , C01B37/08 , C07C1/20 , C10G3/49 , C10G3/56 , C10G3/62 , C10G2400/20 , C10G2400/22 , C07C11/02
摘要： A novel small pore (metallo)aluminophosphate molecular sieve is disclosed. The as-synthesized material has an X-ray diffraction pattern including the lines listed in Table 1 and is produced in the presence of fluoride ions and 4-dimethylaminopyridine as structure directing agent. The silicoaluminophosphate material has methanol conversion activity and n-hexane cracking activity.
摘要翻译：公开了一种新型的小孔（金属）磷酸铝分子筛。合成原料具有包括表1中列出的线的X射线衍射图，并且在氟离子和4-二甲基氨基吡啶作为结构导向剂存在下制备。硅铝磷酸盐材料具有甲醇转化活性和正己烷裂解活性。

3. 发明申请

US20070100185A1 Synthesis of chabazite-containing molecular sieves and their use in the conversion of oxygenates to olefins 有权
标题翻译：含有菱沸石的分子筛的合成及其在含氧化合物转化为烯烃的用途
公开(公告)号：US20070100185A1
公开(公告)日：2007-05-03
申请号：US11521155
申请日：2006-09-14
申请人： Guang Cao , Machteld Mertens , Matu Shah , Marc Anthonis , Hailian Li , Anil Guram , Robert Saxton , Mark Muraoka , Jeffrey Yoder , Anthony Volpe
发明人： Guang Cao , Machteld Mertens , Matu Shah , Marc Anthonis , Hailian Li , Anil Guram , Robert Saxton , Mark Muraoka , Jeffrey Yoder , Anthony Volpe
IPC分类号： C07C1/00 , C01B39/00 , C01B39/48
CPC分类号： C01B39/48 , B01J29/70 , B01J29/7015 , B01J29/80 , C01B37/02 , C01B39/023 , C07C1/20 , C10G3/49 , C10G3/62 , C10G2300/1011 , C10G2400/20 , Y02P30/20 , C07C11/02
摘要： The synthesis of a crystalline material, in particular, a high silica zeolite, comprising a chabazite-type framework molecular sieve is conducted in the presence of an organic directing agent having the formula: [R1R2R3N—R4]+Q− wherein R1 and R2 are independently selected from hydrocarbyl groups and hydroxy-substituted hydrocarbyl groups having from 1 to 3 carbon atoms, provided that R1 and R2 may be joined to form a nitrogen-containing heterocyclic structure, R3 is an alkyl group having 2 to 4 carbon atoms and R4 is selected from a 4- to 8-membered cycloalkyl group, optionally, substituted by 1 to 3 alkyl groups each having from 1 to 3 carbon atoms; and a 4- to 8-membered heterocyclic group having from 1 to 3 heteroatoms, said heterocyclic group being, optionally, substituted by 1 to 3 alkyl groups each having from 1 to 3 carbon atoms and the or each heteroatom in said heterocyclic group being selected from the group consisting of O, N, and S, or R3 and R4 are hydrocarbyl groups having from 1 to 3 carbon atoms joined to form a nitrogen-containing heterocyclic structure; and Q− is a anion.
摘要翻译：包含菱沸石型框架分子筛的结晶材料，特别是高二氧化硅沸石的合成在有机导向剂的存在下进行，所述有机导向剂具有以下结构式：<？in-line-formula description =“In-line 公式“end =”lead“？> [R 1] 2 3 <？in-line-formula description =“In-line Formulas”end =“tail”？>其中R 1和R 2 > 2个独立地选自烃基和具有1至3个碳原子的羟基取代的烃基，条件是R 1和R 2可以连接形成含氮杂环结构，R 3是具有2至4个碳原子的烷基，R 4选自4-至8-元环烷基任选被1至3个具有1至3个碳原子的烷基取代; 和具有1至3个杂原子的4至8元杂环基，所述杂环基任选被1至3个具有1至3个碳原子的烷基取代，并且所述杂环基中的每个杂原子被选定由O，N和S组成的组，或R 3和R 4是具有1至3个碳原子的烃基，连接形成含氮杂环结构体; 而Q ^{是阴离子。}

4. 发明申请

US20070043249A1 Synthesis of molecular sieves having the chabazite framework type and their use in the conversion of oxygenates to olefins 有权
标题翻译：具有菱沸石骨架类型的分子筛的合成及其在将含氧化合物转化为烯烃的用途
公开(公告)号：US20070043249A1
公开(公告)日：2007-02-22
申请号：US11206444
申请日：2005-08-18
申请人： Guang Cao , Matu Shah
发明人： Guang Cao , Matu Shah
IPC分类号： C07C1/00 , C01B37/04 , C01B37/08
CPC分类号： C01B39/54 , B01J29/83 , B01J29/85 , C01B37/04 , C01B37/08 , C10G3/49 , C10G3/62 , C10G2300/708 , C10G2400/20 , Y02P30/42
摘要： The synthesis of a crystalline aluminophosphate or silicoaluminophosphate molecular sieve having a chabazite-type framework type is conducted in the presence of an organic directing agent having the formula (I) [R1R2R3N—R4]+X− (I) wherein R1, R2 and R3 are independently selected from the group consisting of alkyl groups having from 1 to 3 carbon atoms and hydroxyalkyl groups having from 1 to 3 carbon atoms; R4 is selected from the group consisting of 4- to 8-membered cycloalkyl groups, optionally substituted by 1 to 3 alkyl groups having from 1 to 3 carbon atoms; 4- to 8-membered heterocyclic groups having from 1 to 3 heteroatoms, said heterocyclic groups being optionally substituted by 1 to 3 alkyl groups having from 1 to 3 carbon atoms and the heteroatoms in said heterocyclic groups being selected from the group consisting of O, N, and S; and aromatic groups optionally substituted by 1 to 3 alkyl groups, said alkyl groups having from 1 to 3 carbon atoms; and X− is an anion.
摘要翻译：在具有式（I）的有机导向剂的存在下进行具有菱沸石型骨架型的结晶铝磷酸盐或硅铝磷酸盐分子筛的合成<？in-line-formula description =“In-Line Formulas”end = “铅”？> [R 1] 2 3 3 4 （I）<？in-line-formula description =“In-line Formulas”end =“tail”？>其中R 1，R 2， 2和R 3独立地选自具有1至3个碳原子的烷基和具有1至3个碳原子的羟基烷基; R 4选自4-8元环烷基，任选被1至3个具有1至3个碳原子的烷基取代; 具有1至3个杂原子的4-至8-元杂环基，所述杂环基团任选被1至3个具有1至3个碳原子的烷基取代，所述杂环基中的杂原子选自O， N和S; 和任选被1至3个烷基取代的芳族基团，所述烷基具有1至3个碳原子; 而X - 是阴离子。

5. 发明申请

US20050009691A1 Synthesis of silicoaluminophosphates 有权
公开(公告)号：US20050009691A1
公开(公告)日：2005-01-13
申请号：US10617852
申请日：2003-07-11
申请人： Guang Cao , Matu Shah , John Brody
发明人： Guang Cao , Matu Shah , John Brody
IPC分类号： B01J29/85 , B01J35/02 , B01J37/00 , C01B37/08 , C01B39/54 , B01J27/182
CPC分类号： B01J29/85 , B01J35/023 , B01J37/0045 , B01J2229/42 , C01B37/08 , C01B39/54 , Y10S423/30
摘要： The invention is directed to a method of synthesising silicoaluminophosphate molecular sieves and in particular those of framework type CHA and AEL. The method uses synthesis templates that comprise one or more tertiary dialkylbutylamines, wherein the alkyl groups are not butyl. The use of such templates. especially N,N-dimethylbutylamine, results in SAPO-11 of a desirable platelet morphology.

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