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1. 发明申请

US20100004383A1 MODIFIED POLYOLEFIN RESIN AND USES THEREOF 有权
标题翻译：改性聚烯烃树脂及其用途
公开(公告)号：US20100004383A1
公开(公告)日：2010-01-07
申请号：US12375032
申请日：2007-07-18
申请人： Yasutaka Watanabe , Kenichi Fujino , Hidetoshi Yoshioka , Naoshi Nagai , Sadahiko Matsuura
发明人： Yasutaka Watanabe , Kenichi Fujino , Hidetoshi Yoshioka , Naoshi Nagai , Sadahiko Matsuura
IPC分类号： C08L23/12 , C08F210/00 , C08F210/06 , C08L23/00
CPC分类号： C08L23/0815 , C08F8/00 , C08F255/00 , C08F255/02 , C08F299/00 , C08L23/10 , C08L51/06 , C08L2205/02 , C08L2666/02 , C08L2666/04 , C09J151/06 , C09J155/005 , C08F10/00 , C08L2666/24 , C08L2666/06
摘要： It is an object of the present invention to provide a modified polyolefin resin adhesive agent which is excellent in adhesiveness to a nonpolar substrate, particularly a poorly adhesive polyolefin substrate to which no surface treatment has been given and to a polar substrate, develops the excellent adhesiveness by drying or thermal compression bonding at relatively low temperature, and exhibits a low tack. That is, the present invention provides the modified polyolefin resin obtained by modifying a polyolefin resin with (A) a polarity imparting agent which is at least one selected from chlorine, unsaturated carboxylic acid, derivatives and anhydrides of unsaturated carboxylic acid and radical polymerizable monomers; and (B) an ethylene-α-olefin copolymer having an unsaturated bond at one end, and use of said modified polyolefin resin as an aqueous resin composition or an organic solvent resin composition.
摘要翻译：本发明的目的是提供一种与非极性基材，特别是不进行表面处理的粘合性差的聚烯烃基材和极性基材粘合性优异的改性聚烯烃树脂粘合剂，具有优异的粘合性通过在相对低的温度下进行干燥或热压接，并且具有低的粘性。也就是说，本发明提供了通过（A）极性赋予剂（其为选自氯，不饱和羧酸，不饱和羧酸的衍生物和酸酐以及可自由基聚合的单体）中的至少一种来改性聚烯烃树脂而获得的改性聚烯烃树脂; 和（B）在一端具有不饱和键的乙烯-α-烯烃共聚物，使用所述改性聚烯烃树脂作为水性树脂组合物或有机溶剂树脂组合物。

2. 发明授权

US6028030A Thermal sensitive recording medium 失效
标题翻译：热敏记录介质
公开(公告)号：US6028030A
公开(公告)日：2000-02-22
申请号：US34402
申请日：1998-03-04
申请人： Tomoyuki Nakano , Koichi Yanai , Junko Seki , Reiji Ohashi , Hidetoshi Yoshioka
发明人： Tomoyuki Nakano , Koichi Yanai , Junko Seki , Reiji Ohashi , Hidetoshi Yoshioka
IPC分类号： B41M5/333 , B41M5/337 , B41M5/30
CPC分类号： B41M5/3331 , B41M5/3372
摘要： A thermal sensitive recording medium which further contains poly urea compound in the thermal color developing layer containing dye precursor and color developer, which displays an excellent image preservative stability. Said poly urea compound contains units of a structure represented by general formula (1), and further contains a repeating unit represented by general formulae (2).about.(7). ##STR1## In these formulae A.sup.1 .about.A.sup.7 are a divalent group, R.sup.1 .about.R.sup.5 are an alkyl group, an alkoxy group or an electron accepting group, o, p, and q are an integer from 0 to 4, r is an integer from 2 to 12 and s and t are an integer from 0 to 8.
摘要翻译：在含有染料前体和显色剂的热显色层中还含有聚脲化合物的热敏记录介质，显示出优异的图像保存稳定性。所述聚脲化合物含有由通式（1）表示的结构的单元，并且还含有由通式（2）DIFFERENCE（7）表示的重复单元。在这些式中，A1差A7是二价基团，R1不同的R5是烷基，烷氧基或电子接受基，o，p和q是0-4的整数，r是2到12的整数 s和t为0〜8的整数。

3. 发明授权

US5053499A 2',3'-dideoxy purine nucleoside 失效
标题翻译： 2'，3'-DIDEOXY PURINE NUCLEOSIDE
公开(公告)号：US5053499A
公开(公告)日：1991-10-01
申请号：US388806
申请日：1989-08-03
申请人： Eiji Kojima , Hidetoshi Yoshioka , Hidenori Fukinbara , Kunichika Murakami
发明人： Eiji Kojima , Hidetoshi Yoshioka , Hidenori Fukinbara , Kunichika Murakami
IPC分类号： C12P17/18 , A61K31/52 , A61P31/12 , C07D473/00 , C07D473/24 , C07D473/38 , C07D473/40 , C07D487/04 , C07H19/06 , C07H19/12 , C07H19/14 , C07H19/16 , C07H19/173 , C12N15/09 , C12R1/01 , C12R1/19 , C12R1/22
CPC分类号： C07H19/06 , C07H19/12 , C07H19/14 , C07H19/16 , Y10S435/847 , Y10S435/849 , Y10S435/852
摘要： 2', 3'-Dideoxy purine nucleosides represented by following general formulae [I] and/or [II] ##STR1## (wherein X and Y indicate nitrogen atoms or carbon atoms and R.sub.1, R.sub.2, R.sub.3, R.sub.4 and R.sub.5 indicate each independently any of hydrogen atom, hydroxyl group, amino group, alkyl group, halogen atom, alkoxy group and mercapto group), process for the preparation thereof and applications thereof to the antiviral agent, antiretroviral agent, therapeutic drug and preventive drug for acquired immunodeficiency syndrome (AIDS), and experimental medicine and experimental reagent to be used in genetic engineering are claimed.
摘要翻译： 2'，3'-二脱氧嘌呤核苷由以下通式[I]和/或[II]表示：其中X和Y表示氮原子或碳原子，R1，R2 ，R3，R4和R5各自独立地表示氢原子，羟基，氨基，烷基，卤原子，烷氧基和巯基中的任一个），其制备方法及其在抗病毒剂，抗逆转录病毒剂，治疗剂要求用于获得性免疫缺陷综合征（AIDS）的药物和预防药物，以及用于基因工程的实验药物和实验试剂。

4. 发明授权

US08236900B2 Modified polyolefin resin and uses thereof 有权
标题翻译：改性聚烯烃树脂及其用途
公开(公告)号：US08236900B2
公开(公告)日：2012-08-07
申请号：US12375032
申请日：2007-07-18
申请人： Yasutaka Watanabe , Kenichi Fujino , Hidetoshi Yoshioka , Naoshi Nagai , Sadahiko Matsuura
发明人： Yasutaka Watanabe , Kenichi Fujino , Hidetoshi Yoshioka , Naoshi Nagai , Sadahiko Matsuura
IPC分类号： C08F8/18 , C08F8/46 , C08F8/02
CPC分类号： C08L23/0815 , C08F8/00 , C08F255/00 , C08F255/02 , C08F299/00 , C08L23/10 , C08L51/06 , C08L2205/02 , C08L2666/02 , C08L2666/04 , C09J151/06 , C09J155/005 , C08F10/00 , C08L2666/24 , C08L2666/06
摘要： It is an object of the present invention to provide a modified polyolefin resin adhesive agent which is excellent in adhesiveness to a nonpolar substrate, particularly a poorly adhesive polyolefin substrate to which no surface treatment has been given and to a polar substrate, develops the excellent adhesiveness by drying or thermal compression bonding at relatively low temperature, and exhibits a low tack. That is, the present invention provides the modified polyolefin resin obtained by modifying a polyolefin resin with (A) a polarity imparting agent which is at least one selected from chlorine, unsaturated carboxylic acid, derivatives and anhydrides of unsaturated carboxylic acid and radical polymerizable monomers; and (B) an ethylene-α-olefin copolymer having an unsaturated bond at one end, and use of said modified polyolefin resin as an aqueous resin composition or an organic solvent resin composition.
摘要翻译：本发明的目的是提供一种与非极性基材，特别是不进行表面处理的粘合性差的聚烯烃基材和极性基材粘合性优异的改性聚烯烃树脂粘合剂，具有优异的粘合性通过在相对低的温度下进行干燥或热压接，并且具有低的粘性。也就是说，本发明提供了通过（A）极性赋予剂（其为选自氯，不饱和羧酸，不饱和羧酸的衍生物和酸酐和自由基聚合性单体）中的至少一种来改性聚烯烃树脂而获得的改性聚烯烃树脂; 和（B）一端具有不饱和键的乙烯-α-烯烃共聚物，使用所述改性聚烯烃树脂作为水性树脂组合物或有机溶剂树脂组合物。

5. 发明申请

US20060025533A1 Binder resin compositions, production process and use thereof 有权
标题翻译：粘合剂树脂组合物，生产工艺及其用途
公开(公告)号：US20060025533A1
公开(公告)日：2006-02-02
申请号：US10500111
申请日：2002-12-20
申请人： Naosuke Komoto , Hidetoshi Yoshioka
发明人： Naosuke Komoto , Hidetoshi Yoshioka
IPC分类号： C08F251/00 , C08F10/00
CPC分类号： C08F8/22 , C08F8/50 , C08F255/02 , C08F255/023 , C08L51/06 , C08F10/06 , C08F220/08
摘要： The invention provides a novel binder resin composition with good adherence onto prime materials of polyolefin, poly (vinyl chloride), polycarbonate, PET, ABS and nylon, and also with excellent solvent solubility. A binder resin composition characterized by being chlorinated propylenic random copolymer with weight average molecular weight of 3000 to 250000, wherein propylenic random copolymer with melting point (Tm) measured by differential scanning calorimeter (DSC) of 115 to 165° C. obtained by copolymerizing propylene with other α-olefin in the coexistence of metallocene type catalyst is chlorinated to chlorine content of 10 to 40% by weight, after thermal degradation or directly without thermal degradation, and/or a binder resin composition characterized by containing carboxyl group-containing chlorinated propylenic random copolymer with weight average molecular weight of 30000 to 220000, wherein propylenic random copolymer with melting point (Tm) measured by differential scanning calorimeter (DSC) of 115 to 165° C. obtained by copolymerizing propylene with other α-olefin in the coexistence of metallocene type catalyst is grafted with α,β-unsaturated carboxylic acid or its anhydride in amounts of 0.1 to 20% by weight, after thermal degradation or directly without thermal degradation, and then chlorinated to chlorine content of 10 to 40% by weight, stabilizer and organic solvent.
摘要翻译：本发明提供了对聚烯烃，聚（氯乙烯），聚碳酸酯，PET，ABS和尼龙的主要材料具有良好粘附性的新型粘合剂树脂组合物，并且还具有优异的溶剂溶解性。一种粘合剂树脂组合物，其特征在于重均分子量为3000〜250000的氯化丙烯酸无规共聚物，其中通过差示扫描量热计（DSC）测定的熔点（Tm）为115〜165℃的丙烯无规共聚物，其通过使丙烯与茂金属型催化剂共存的其它α-烯烃氯化成氯含量为10〜40重量％，热降解后或直接不进行热降解，和/或以含羧基的氯化丙烯酸为特征的粘合剂树脂组合物重均分子量为30000至220000的无规共聚物，其中通过差示扫描量热计（DSC）测量的熔点（Tm）为115至165℃的丙烯无规共聚物通过共聚丙烯与其它α-烯烃共聚获得茂金属型催化剂用α，β-不饱和羧酸或其a 二氢化钠的量为0.1〜20重量％，经热降解后直接进行无热降解，氯化至氯含量为10〜40重量％的稳定剂和有机溶剂。

6. 发明授权

US06426388B1 Modified polyolefin composition and uses thereof 有权
标题翻译：改性聚烯烃组合物及其用途
公开(公告)号：US06426388B1
公开(公告)日：2002-07-30
申请号：US09709329
申请日：2000-11-13
申请人： Kenichi Fujino , Terumasa Fujitaka , Kazuhiro Usui , Kouji Masumoto , Hidetoshi Yoshioka
发明人： Kenichi Fujino , Terumasa Fujitaka , Kazuhiro Usui , Kouji Masumoto , Hidetoshi Yoshioka
IPC分类号： C08F25500
CPC分类号： C09D151/06 , C08F255/00 , C08F255/02 , C08F255/04 , C08L51/06 , C08L2666/02 , C09J151/06
摘要： Disclosed is a novel chlorine-free modified polyolefin composition with excellent adherence to polyolefin substrates, with excellent solventresistance, oil resistance and weather resistance, with no tack, and also with excellentcohesion, obtainable by using 0.5 to 15% (by weight) of maleic anhydride and 0.1 to 7.5% (by weight) of styrenic monomer to polypropylene, eyhylene-propylene copolymer or ethylene-propylene-buten copolymer, and by graft polymerizing so as the weight ratio of maleic anhydride to styrenic monomer to become not less than 2 to not more than 5.
摘要翻译：公开了一种新型的无氯改性聚烯烃组合物，其具有优异的耐聚烯烃基材的粘合性，耐油性，耐油性和耐候性，无粘性，并且还具有优异的粘合性，可通过使用0.5〜15重量％的马来酸酐和0.1〜7.5％（重量）的苯乙烯类单体与聚丙烯，叶烯 - 丙烯共聚物或乙烯 - 丙烯 - 丁烯共聚物，并通过接枝聚合使马来酸酐与苯乙烯类单体的重量比变为不小于2 超过5。

7. 发明授权

US07235610B2 Aqueous dispersion, process for producing the same, and use 有权
标题翻译：水分散体，其制造方法和用途
公开(公告)号：US07235610B2
公开(公告)日：2007-06-26
申请号：US10505458
申请日：2003-02-28
申请人： Kenichi Fujino , Hidetoshi Yoshioka
发明人： Kenichi Fujino , Hidetoshi Yoshioka
IPC分类号： C08F8/18
CPC分类号： C08F8/22 , C08F8/50 , C08F255/02 , C08F255/023 , C08J3/05 , C08J2323/14 , C08J2351/06 , C08L51/06 , C08L2666/02 , C09D5/002 , C09D11/106 , C09D151/06 , C09J151/06 , C08F10/06 , C08F220/08
摘要： The purpose of the invention is to provide a novel aqueous dispersion that allows high solidification and that has good adherence and gasohol resistance to polyolefin substrates even on low-temperature baking.An aqueous dispersion characterized by dispersedly containing carboxyl group-containing chlorinated propylenic random copolymer with chlorine content of 5 to 40% by weight, grafting level of α,β-unsaturated carboxylic acid or its anhydride of 0.1 to 20% by weight and weight average molecular weight of 10,000 to 300,000, and stabilizer, a method for the production and the uses thereof.
摘要翻译：本发明的目的是提供一种新颖的水性分散体，其即使在低温烘烤下也能够高度固化，并且对聚烯烃基材具有良好的粘附性和耐醇性。一种水分散体，其特征在于分散含有含氯量为5-40重量％的含羧基的氯化丙烯酸无规共聚物，α，β-不饱和羧酸或其酸酐的接枝量为0.1-20重量％，重均分子量重量为10,000至300,000，以及稳定剂，其制备方法及其用途。

8. 发明申请

US20050171271A1 Aqueous dispersion, process for producing the same, and use 有权
标题翻译：水分散体，其制造方法和用途
公开(公告)号：US20050171271A1
公开(公告)日：2005-08-04
申请号：US10505458
申请日：2003-02-28
申请人： Kenichi Fujino , Hidetoshi Yoshioka
发明人： Kenichi Fujino , Hidetoshi Yoshioka
IPC分类号： C08F8/20 , C08F8/22 , C08F8/50 , C08F255/02 , C08L51/06 , C09D5/00 , C09D11/10 , C09D151/06 , C09J151/06 , C08K3/00
CPC分类号： C08F8/22 , C08F8/50 , C08F255/02 , C08F255/023 , C08J3/05 , C08J2323/14 , C08J2351/06 , C08L51/06 , C08L2666/02 , C09D5/002 , C09D11/106 , C09D151/06 , C09J151/06 , C08F10/06 , C08F220/08
摘要： The purpose of the invention is to provide a novel aqueous dispersion that allows high solidification and that has good adherence and gasohol resistance to polyolefin substrates even on low-temperature baking. An aqueous dispersion characterized by dispersedly containing carboxyl group-containing chlorinated propylenic random copolymer with chlorine content of 5 to 40% by weight, grafting level of α,β-unsaturated carboxylic acid or its anhydride of 0.1 to 20% by weight and weight average molecular weight of 10,000 to 300,000, and stabilizer, a method for the production and the uses thereof.
摘要翻译：本发明的目的是提供一种新颖的水性分散体，其即使在低温烘烤下也能够高度固化，并且对聚烯烃基材具有良好的粘附性和耐醇性。一种水分散体，其特征在于分散含有含氯量为5-40重量％的含羧基的氯化丙烯酸无规共聚物，α，β-不饱和羧酸或其酸酐的接枝量为0.1-20重量％，重均分子量重量为10,000至300,000，以及稳定剂，其制备方法及其用途。

9. 发明授权

US06800688B2 Modified polyolefin resin, modified polyolefin resin composition, and uses thereof 有权
标题翻译：改性聚烯烃树脂，改性聚烯烃树脂组合物及其应用
公开(公告)号：US06800688B2
公开(公告)日：2004-10-05
申请号：US10168521
申请日：2002-08-06
申请人： Kazuhiro Usui , Kenichi Fujino , Terumasa Fujitaka , Tadashi Matsui , Hidetoshi Yoshioka , Shunji Sekiguchi
发明人： Kazuhiro Usui , Kenichi Fujino , Terumasa Fujitaka , Tadashi Matsui , Hidetoshi Yoshioka , Shunji Sekiguchi
IPC分类号： C08F25500
CPC分类号： C09D151/06 , C08F255/00 , C08F255/02 , C08F255/04 , C08F255/08 , C08L51/06 , C08L2666/02 , C09D5/002 , C09D7/65 , C09D11/03 , C09D11/106 , C09J151/06
摘要： A resin which has excellent adhesion to nonpolar substrates, is nontacky, and has satisfactory solubility in aromatic or nonaromatic solvents and satisfactory compatibility with other resins. The resin is a modified polyolefin resin having a weight-average molecular weight of 15,000 to 150,000 obtained by modifying a polyolefin resin by grafting thereto (A) an unsaturated polycarboxylic acid or a derivative thereof and (B) a (meth)acrylic ester represented by a specific general formula, the contents of (A) and (B) in the modified polyolefin resin being 0.1 to 20 wt. % and 0.1 to 30 wt. %, respectively.
摘要翻译：对非极性基材具有优异的粘合性的树脂是非粘性的，并且在芳族或非芳族溶剂中具有令人满意的溶解性和与其它树脂的令人满意的相容性。树脂是通过接枝聚烯烃树脂（A）不饱和多元羧酸或其衍生物而得到的重均分子量为15,000〜150,000的改性聚烯烃树脂和（B）由（甲基）丙烯酸酯表示的（甲基）丙烯酸酯具体的通式中，改性聚烯烃树脂中的（A）和（B）的含量为0.1〜20重量％。％和0.1〜30wt。％，分别。

10. 发明授权

US06495629B2 Modified polyolefin resin composition and uses thereof 有权
标题翻译：改性聚烯烃树脂组合物及其用途
公开(公告)号：US06495629B2
公开(公告)日：2002-12-17
申请号：US09805999
申请日：2001-03-15
申请人： Kazuhiro Usui , Kenichi Fujino , Terumasa Fujitaka , Koji Masumoto , Hidetoshi Yoshioka
发明人： Kazuhiro Usui , Kenichi Fujino , Terumasa Fujitaka , Koji Masumoto , Hidetoshi Yoshioka
IPC分类号： C08F25500
CPC分类号： C09J151/04 , C08F255/00 , C09D11/10 , C09D151/04 , C08F220/06
摘要： A novel chlorine-free modified polyolefin resin composition with excellent adherence to nonpolar substrates, excellent solubility in solvents, excellent compatibility with other resins, and without tack after painting and drying is obtainable by graft modifying a mixed resin having 40 to 99 parts by weight of polyolefin resin (A) and 1 to 60 parts by weight of ethylenic compound-unsaturated carboxylic acid copolymer (B) that contains 0.1 to 50% by weight of unsaturated carboxylic acid derivative, with unsaturated carboxylic acid derivative and/or its anhydride (C), the modified polyolefin resin composition having weight average molecular weight of 20,000 to 150 000 and the grafting weight of (C) being 0.1 to 20% by weight.
摘要翻译：通过将具有40〜99重量份的混合树脂进行接枝改性，可获得对非极性基材具有优异粘附性的无氯改性聚烯烃树脂组合物，在溶剂中的溶解性优异，与其它树脂的相容性优异，聚烯烃树脂（A）和1〜60重量份含有0.1〜50重量％不饱和羧酸衍生物的不饱和羧酸衍生物和/或其酸酐（C）的烯属化合物 - 不饱和羧酸共聚物（B），重均分子量为20,000〜150000，（C）的接枝重量为0.1〜20重量％的改性聚烯烃树脂组合物。

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