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1. 发明申请

US20090240006A1 NOVEL NAPHTHOXAZINE COMPOSITION 有权
标题翻译：新型萘普生组合物
公开(公告)号：US20090240006A1
公开(公告)日：2009-09-24
申请号：US12054182
申请日：2008-03-24
申请人： Hatsuo ISHIDA , Masanori Nakamura
发明人： Hatsuo ISHIDA , Masanori Nakamura
IPC分类号： C08L63/00
CPC分类号： C08G59/621 , C08L63/00
摘要： The present invention is intended to provide a novel naphthoxazine composition having a smaller amount of volatile components (weight reduction) upon curing, and is to provide a naphthoxazine composition characterized in that a naphthoxazine compound having a phenolic hydroxyl group in the same molecule is further added with an epoxy resin, and a molded product obtained by molding the naphthoxazine composition.
摘要翻译：本发明旨在提供一种在固化时具有较少挥发组分量（重量减少）的新型萘并恶组合物，并提供一种萘并恶嗪组合物，其特征在于进一步添加同一分子中具有酚羟基的萘并恶嗪化合物和通过模塑萘并恶嗪组合物得到的成型体。

2. 发明申请

US20090187003A1 THERMOSETTING RESIN, THERMOSETTING COMPOSITION CONTAINING SAME, AND MOLDED PRODUCT OBTAINED FROM SAME 审中-公开
标题翻译：热固性树脂，含有该组合物的热固化组合物和从其获得的成型产品
公开(公告)号：US20090187003A1
公开(公告)日：2009-07-23
申请号：US12088681
申请日：2006-09-25
申请人： Yuji Eguchi , Kazuo Doyama , Hatsuo Ishida
发明人： Yuji Eguchi , Kazuo Doyama , Hatsuo Ishida
IPC分类号： C08G65/00
CPC分类号： C08G73/06 , C07D265/14 , C08L79/04
摘要： An object of the invention is to provide a thermosetting resin excellent in dielectric characteristics and heat resistance, and to provide a thermosetting composition comprising the thermosetting resin, as well as a molded product, substrate material for electronic devices and so forth obtained from the thermosetting resin. The present invention provides a thermosetting resin having a dihydrobenzoxazine ring structure represented by formula (I) in a main chain thereof, a thermosetting composition comprising the thermosetting resin, as well as a molded product, substrate material for electronic devices and so forth obtained from the thermosetting resin. (in formula (I), Ar1 represents a tetravalent aromatic group, R1 is a hydrocarbon group having a fused alicyclic structure, and n represents an integer from 2 to 500).
摘要翻译：本发明的目的是提供一种介电特性和耐热性优异的热固性树脂，并且提供一种包含热固性树脂的热固性组合物，以及由热固性树脂获得的模塑产品，电子器件等的基材。本发明提供一种热固性树脂，其主链具有由式（I）表示的二氢苯并恶嗪环结构，包含热固性树脂的热固性组合物，以及模塑产品，电子器件用基材等热固性树脂。（式（I）中，Ar 1表示四价芳香族基，R 1表示稠合脂环式结构的烃基，n表示2〜500的整数）。

3. 发明申请

US20090069533A1 Benzoxazine monomers, polymers and compositions 有权
标题翻译：苯并恶嗪单体，聚合物和组合物
公开(公告)号：US20090069533A1
公开(公告)日：2009-03-12
申请号：US11899438
申请日：2007-09-06
申请人： Hatsuo Ishida , Pedro Velez-Herrera
发明人： Hatsuo Ishida , Pedro Velez-Herrera
IPC分类号： C08G63/00 , C07D265/06 , C07D265/14 , C07D413/04 , C07D498/04
CPC分类号： C07D265/16 , C07D498/04 , C08G73/02 , C08G73/026
摘要： Benzoxazine monomers comprising at least one pendant group are described. (Co)Polymers comprising at least one benzoxazine monomer having at least one pendant group are also described. In a preferred embodiment, the pendant group is located in a side chain of the benzoxazine monomer or polymer. Methods for preparing the benzoxazine monomers and polymers are described. Compositions comprising the benzoxazine monomers and polymers have numerous uses including optical materials, and in electronic materials as electrically insulating materials, and as fireproof materials.
摘要翻译：描述包含至少一个侧基的苯并恶嗪单体。（Co）还描述了包含至少一种具有至少一个侧基的苯并恶嗪单体的聚合物。在优选的实施方案中，侧基位于苯并恶嗪单体或聚合物的侧链中。描述了制备苯并恶嗪单体和聚合物的方法。包含苯并恶嗪单体和聚合物的组合物具有许多用途，包括光学材料，以及作为电绝缘材料的电子材料和耐火材料。

4. 发明申请

US20070191555A1 Thermosetting resin composition and its article 审中-公开
标题翻译：热固性树脂组合物及其制品
公开(公告)号：US20070191555A1
公开(公告)日：2007-08-16
申请号：US10811952
申请日：2004-03-30
申请人： Hatsuo Ishida , Koichi Shibayama , Hiroshi Abe
发明人： Hatsuo Ishida , Koichi Shibayama , Hiroshi Abe
IPC分类号： C08L63/02 , C08L63/04
CPC分类号： C08G59/027 , C08G59/4014 , H05K1/0346
摘要： The invention provides a thermosetting resin composition comprising a bifunctional dihydrobenzoxazine compound and an epoxy compound, and provides a thermosetting resin molding obtained by thermally curing the thermosetting resin composition. The molding has excellent electric properties of low dielectric constant and low dielectric loss tangent. The resin composition comprises an epoxy compound and a bifunctional dihydrobenzoxazine compound of the following general formula (1), wherein the equivalent ratio of the epoxy compound to the bifunctional dihydrobenzoxazine compound is 1/(0.1 to 20): wherein R represents a linear alkylene group having at least 2 carbon atoms, or a branched alkylene group derived from it by substituting the hydrogen atom therein with an alkyl group, and the hydrogen atom of the benzene ring may be substituted with an alkyl group or an alkoxy group.
摘要翻译：本发明提供一种包含双官能二氢苯并恶嗪化合物和环氧化合物的热固性树脂组合物，并提供通过热固化热固性树脂组合物获得的热固性树脂模制品。该模制品具有优异的低介电常数和低介电损耗角正切的电性能。树脂组合物包含下述通式（1）的环氧化合物和双官能二氢苯并恶嗪化合物，其中环氧化合物与双官能二氢苯并恶嗪化合物的当量比为1 /（0.1〜20）：其中R表示直链亚烷基具有至少2个碳原子，或者由烷基衍生自其中的氢原子衍生的支链亚烷基，苯环的氢原子可以被烷基或烷氧基取代。

5. 发明授权

US5543516A Process for preparation of benzoxazine compounds in solventless systems 失效
标题翻译：在无溶剂体系中制备苯并恶嗪化合物的方法
公开(公告)号：US5543516A
公开(公告)日：1996-08-06
申请号：US245478
申请日：1994-05-18
申请人： Hatsuo Ishida
发明人： Hatsuo Ishida
IPC分类号： C07D265/12 , C07D265/16 , C07D498/04 , C07F7/10 , C08F12/00 , C08F212/00 , C08F212/14 , C08F212/32 , C08G14/06 , C08G77/38 , C08G77/382 , C08G77/388 , C07D265/14
CPC分类号： C08G77/382 , C07D265/16
摘要： A method for preparing a desired benzoxazine compound comprises preparing a substantially homogeneous reaction mixture that includes a phenolic compound; a primary amine; and an aldehyde, but no solvent other than for the solvency which the reactants may have for each other. Following its preparation, the reaction mixture is maintained at a temperature, and for a period sufficient to cause the reactants to combine chemically to form the desired compound.
摘要翻译：制备所需苯并恶嗪化合物的方法包括制备包含酚类化合物的基本均匀的反应混合物; 伯胺; 和醛，但不包括反应物可能彼此具有的溶解能力之外的溶剂。在其制备之后，将反应混合物保持在一定温度下，并持续足以使反应物化学结合形成所需化合物的时间。

6. 发明授权

US07834099B2 Imide-naphthoxazine copolymer 有权
标题翻译：酰肼 - 萘恶嗪共聚物
公开(公告)号：US07834099B2
公开(公告)日：2010-11-16
申请号：US11896841
申请日：2007-09-06
申请人： Hatsuo Ishida , Masanori Nakamura
发明人： Hatsuo Ishida , Masanori Nakamura
IPC分类号： C08G73/16
CPC分类号： C08G73/06 , C08G73/1085
摘要： An imide-naphthoxazine copolymer comprising a repeating unit represented by General Formula (1) below: (wherein X and Y independently represent a single bond, an oxygen atom, a carbonyl group, or an organic group which may be substituted by a heteroatom; R represents CH3 or H, n represents an integer from 1 to 10; and m represents an integer from 1 to 20).
摘要翻译：包含由以下通式（1）表示的重复单元的酰亚胺 - 萘并恶嗪共聚物：其中X和Y独立地表示单键，氧原子，羰基或可被杂原子取代的有机基团; R 表示CH3或H，n表示1〜10的整数，m表示1〜20的整数。

7. 发明申请

US20090076229A1 Imide-naphthoxazine copolymer 有权
标题翻译：酰肼 - 萘恶嗪共聚物
公开(公告)号：US20090076229A1
公开(公告)日：2009-03-19
申请号：US11896841
申请日：2007-09-06
申请人： Hatsuo Ishida , Masanori Nakamura
发明人： Hatsuo Ishida , Masanori Nakamura
IPC分类号： C08G73/12
CPC分类号： C08G73/06 , C08G73/1085
摘要： An imide-naphthoxazine copolymer comprising a repeating unit represented by General Formula (1) below: (wherein X and Y independently represent a single bond, an oxygen atom, a carbonyl group, or an organic group which may be substituted by a heteroatom; R represents CH3 or H, n represents an integer from 1 to 10; and m represents an integer from 1 to 20).
摘要翻译：包含由以下通式（1）表示的重复单元的酰亚胺 - 萘并恶嗪共聚物：其中X和Y独立地表示单键，氧原子，羰基或可被杂原子取代的有机基团; R 表示CH3或H，n表示1〜10的整数，m表示1〜20的整数。

8. 发明申请

US20090054614A1 METHOD FOR PRODUCING THERMOSETTING RESIN, THERMOSETTING RESIN, THERMOSETTING COMPOSITION CONTAINING SAME, MOLDED BODY, CURED BODY, AND ELECTRONIC DEVICE CONTAINING THOSE 审中-公开
标题翻译：生产热固性树脂，热固性树脂，含有其的热成型组合物，模制体，固化体和包含这些组合物的电子装置的方法
公开(公告)号：US20090054614A1
公开(公告)日：2009-02-26
申请号：US12280029
申请日：2007-02-20
申请人： Yuji Eguchi , Kazuo Doyama , Hatsuo Ishida
发明人： Yuji Eguchi , Kazuo Doyama , Hatsuo Ishida
IPC分类号： C08G14/073
CPC分类号： C08G14/06
摘要： The present invention provides a method for producing a thermosetting resin having a dihydrobenzoxazine ring structure, characterized by heating and reacting a) a multi-functional phenolic compound represented by the following general formula (I), b) a diamine compound represented by the following general formula (II) and c) an aldehyde compound: wherein X is an organic group containing an aromatic ring and having 6 or more carbon atoms, Y is an organic group having 5 or more carbon atoms, while both X and Y optionally have N, O, F as a heteroatom, and the benzene rings of both sides of X and Y are bonded to different atoms in X and Y.
摘要翻译：本发明提供一种具有二氢苯并恶嗪环结构的热固性树脂的制造方法，其特征在于加热和反应a）由以下通式（I）表示的多官能酚类化合物，b）由以下通式式（II）和c）醛化合物：其中X是含有芳环并且具有6个或更多个碳原子的有机基团，Y是具有5个或更多个碳原子的有机基团，而X和Y任选具有N， O，F为杂原子，X和Y两面的苯环与X和Y中的不同原子结合。

9. 发明授权

US6160079A Activated arylamine-based polybenzoxazines 失效
标题翻译：活性芳胺基聚苯并恶嗪
公开(公告)号：US6160079A
公开(公告)日：2000-12-12
申请号：US291466
申请日：1999-04-14
申请人： Hatsuo Ishida , Daniel Sanders
发明人： Hatsuo Ishida , Daniel Sanders
IPC分类号： C07D265/16 , C08G14/06 , C08G61/12 , C08G8/04
CPC分类号： C08G61/12 , C07D265/16 , C08G14/06
摘要： Arylamines with electron donating groups such as alkyl and alkoxy groups in the meta position on the aromatic ring change the polymerization temperature of the benzoxazine prepared therefrom and offer an opportunity for an additional crosslinking site (the para position on the aromatic amine can couple to a Mannich base generated by the opening of the oxazine ring of the benzoxazine or a methylene bridge generated by a degradation reaction). Naphthenic amines with an alkyl or alkoxy substituent on the 5.sup.th through the 8.sup.th carbon atom on the naphthalene ring can function similarly. The polymers for benzoxazines prepared from at least 10% substituted aromatic or naphthenic amines are useful due to low polymerization temperatures and higher Tg (glass transition temperature).
摘要翻译：在芳环上的间位的具有供体基团如烷基和烷氧基的芳胺改变由其制备的苯并恶嗪的聚合温度，并提供另外的交联位点的机会（芳胺上的对位可以连接到曼尼希通过苯并恶嗪的恶嗪环的开放产生的碱或由降解反应产生的亚甲基桥）。在萘环上的第5个到第8个碳原子上具有烷基或烷氧基取代基的环烷胺类似地起作用。由至少10％取代的芳族或环烷胺制备的苯并恶嗪的聚合物是有用的，因为低聚合温度和较高的Tg（玻璃化转变温度）。

10. 发明授权

US5900447A Composition for forming high thermal conductivity polybenzoxazine-based material and method 失效
标题翻译：用于形成高导热性聚苯并恶嗪的材料和方法的组合物
公开(公告)号：US5900447A
公开(公告)日：1999-05-04
申请号：US846457
申请日：1997-05-01
申请人： Hatsuo Ishida
发明人： Hatsuo Ishida
IPC分类号： C08K3/22 , C08G14/073 , C08G59/40 , C08K3/28 , C08K3/36 , C08K3/38 , C08L61/34
CPC分类号： C08K3/38 , C08K2003/382
摘要： The present invention relates to a composition and method for forming a high thermal conductivity polybenzoxazine-based material. The composition comprises at least one benzoxazine resin and a filler material which includes particles of boron nitride in an amount sufficient to establish a thermal conductivity of between about 3 W/mK and 37 W/mK in the polybenzoxazine-based material.
摘要翻译：本发明涉及形成高导热性聚苯并恶嗪类材料的组合物和方法。所述组合物包含至少一种苯并恶嗪树脂和填料，其包含足以在聚苯并恶嗪类材料中建立约3W / mK至37W / mK之间的热导率的氮化硼颗粒。

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