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1. 发明授权

US5927063A High efficiency reformed methanol gas turbine power plants 失效
标题翻译：高效改造甲醇燃气轮机发电厂
公开(公告)号：US5927063A
公开(公告)日：1999-07-27
申请号：US914920
申请日：1997-08-19
申请人： Gary F. Janda , Keith H. Kuechler , John J. Guide , Frank F. Mittricker , Frank Roberto
发明人： Gary F. Janda , Keith H. Kuechler , John J. Guide , Frank F. Mittricker , Frank Roberto
IPC分类号： F01K21/04 , F02C3/28 , F02C3/30
CPC分类号： F01K21/042 , Y02E20/14 , Y02E20/16
摘要： The present invention is a high efficiency reformed methanol (syngas) gas turbine power plant. The invention utilizes a Back Pressure steam Turbine (BPT) to maximize the thermal efficiency and the power output of a reformed methanol gas turbine power generation system. Methanol feed is reformed to syngas (H.sub.2 and CO.sub.2) prior to combustion in the BPT turbine. The endothermic reforming reaction, and the generation of the significant amount of process steam essential for reforming, recovers most of the useful heat in the gas turbine exhaust gas. The process steam pressure is set by the gas turbine inlet requirements, and can be referred to as low pressure steam. Additional heat in the gas turbine exhaust gas is recovered by generating the system's process steam at an elevated pressure, rather than the required low pressure. This high pressure steam is used to drive a BPT, generating additional power and the discharged low pressure steam from the BPT is used as the process steam for the methanol reformer.
摘要翻译：本发明是高效改性甲醇（合成气）燃气轮机发电厂。本发明利用背压式蒸汽轮机（BPT）来最大化改造甲醇燃气轮机发电系统的热效率和功率输出。在BPT涡轮机燃烧之前，将甲醇进料重整成合成气（H 2和CO 2）。吸热重整反应和重整所需的大量工艺蒸汽的产生可以回收燃气轮机废气中大部分有用的热量。过程蒸汽压力由燃气轮机入口要求设定，可称为低压蒸汽。通过在升高的压力下产生系统的过程蒸汽而不是所需的低压来回收燃气涡轮废气中的额外的热量。这种高压蒸汽用于驱动BPT，产生额外的功率，并且将来自BPT的排出的低压蒸汽用作甲醇重整器的工艺蒸汽。

2. 发明授权

US06660812B2 Production of olefin derivatives 有权
公开(公告)号：US06660812B2
公开(公告)日：2003-12-09
申请号：US09882713
申请日：2001-06-15
申请人： Keith H. Kuechler , Minquan Cheng , Marc L. DeChellis , David R. Lumgair, Jr. , Russell D. Sellen , Gary F. Janda
发明人： Keith H. Kuechler , Minquan Cheng , Marc L. DeChellis , David R. Lumgair, Jr. , Russell D. Sellen , Gary F. Janda
IPC分类号： C08F200
CPC分类号： B01J8/1809 , B01J2208/00256 , B01J2208/00274 , B01J2208/00336 , B01J2219/00006 , B01J2219/00247 , C07C1/20 , C07C2529/85 , C07D301/10 , C08F10/00 , Y02P30/42 , Y10S585/903 , C07C11/02 , C08F2/00
摘要： Disclosed is a system of making an olefin derivative from a dilute olefin feed. Dilute olefin is sent to an olefin reaction unit to form an olefin derivative product. The olefin derivative product is recovered from the reaction unit while a vent stream is also removed. Olefin is separated from the vent stream, and the olefin is sent to the olefin reaction unit for additional processing.

3. 发明授权

US06441261B1 High pressure oxygenate conversion process via diluent co-feed 失效
标题翻译：通过稀释剂共进料的高压含氧化合物转化过程
公开(公告)号：US06441261B1
公开(公告)日：2002-08-27
申请号：US09627634
申请日：2000-07-28
申请人： Keith H. Kuechler , Stephen N. Vaughn , Gary F. Janda , Russell D. Sellen
发明人： Keith H. Kuechler , Stephen N. Vaughn , Gary F. Janda , Russell D. Sellen
IPC分类号： C07C100
CPC分类号： C07C1/20 , C07C2529/85 , Y02P30/42 , C07C11/02
摘要： This invention relates to a method for converting an oxygenate feedstock to an olefin product. In particular, this invention relates to a method for converting an oxygenate feedstock, including a diluent co-feed, to an olefin product, by contacting the feedstock with a silicoaluminophosphate catalyst at a high total pressure of the feedstock while maintaining a low partial pressure of the oxygenates undergoing reaction.
摘要翻译：本发明涉及将含氧化合物原料转化成烯烃产物的方法。特别地，本发明涉及通过在原料的高总压力下使原料与硅铝磷酸盐催化剂接触而将包含稀释剂共进料的含氧化合物原料转化为烯烃产物的方法，同时保持低氧化物进行反应。

4. 发明授权

US06049011A Hydroformylation process 失效
标题翻译：加氢甲酰化过程
公开(公告)号：US06049011A
公开(公告)日：2000-04-11
申请号：US875157
申请日：1997-10-15
申请人： Gabor Kiss , Michael G Matturro , Harry William Deckman , Frank Hershkowitz , David R. Lumgair, Jr. , Gary F Janda , Daniel N King
发明人： Gabor Kiss , Michael G Matturro , Harry William Deckman , Frank Hershkowitz , David R. Lumgair, Jr. , Gary F Janda , Daniel N King
IPC分类号： B01J21/06 , B01J23/04 , B01J23/44 , B01J23/74 , B01J27/232 , B01J31/24 , C07B61/00 , C07C29/141 , C07C29/17 , C07C31/125 , C07C45/50 , C07C45/62 , C07C45/73 , C07C45/74 , C07C47/02 , C07C47/21 , C07C51/235 , C07C53/126 , C07C53/128 , C07C67/08 , C07C69/14 , C07C69/24 , C07C69/44 , C07C69/76 , C07C69/80 , C08K5/10 , C10M105/38 , C11B9/00 , C07C45/00
CPC分类号： C07C45/74 , C07C29/141 , C07C45/50 , C07C45/62
摘要： A dilute ethylene stream, e.g., one produced by steam cracking, is oxonated to yield propanal, without the need to separate other lower hydrocarbons.
摘要翻译： PCT No.PCT / EP96 / 00163 Sec。 371日期：1997年10月15日 102（e）日期1997年10月15日PCT 1996年1月17日PCT PCT。 WO96 / 22265 PCT出版物日期1996年7月25日稀释的乙烯流，例如通过蒸汽裂化产生的乙烯流被氧化以产生丙醛，而不需要分离其它低级烃。

5. 发明授权

US06486219B1 Methanol, olefin, and hydrocarbon synthesis process 失效
标题翻译：甲醇，烯烃和烃的合成过程
公开(公告)号：US06486219B1
公开(公告)日：2002-11-26
申请号：US09670755
申请日：2000-09-27
申请人： Gary F. Janda , Keith H. Kuechler
发明人： Gary F. Janda , Keith H. Kuechler
IPC分类号： C07C2700
CPC分类号： C10G2/30 , C01B3/382 , C01B3/386 , C01B2203/0233 , C01B2203/0238 , C01B2203/0244 , C01B2203/025 , C01B2203/0405 , C01B2203/0415 , C01B2203/043 , C01B2203/046 , C01B2203/0475 , C01B2203/06 , C01B2203/061 , C01B2203/062 , C01B2203/063 , C01B2203/065 , C01B2203/0805 , C01B2203/0811 , C01B2203/0816 , C01B2203/0827 , C01B2203/0844 , C01B2203/0866 , C01B2203/1052 , C01B2203/1082 , C01B2203/1241 , C01B2203/127 , C01B2203/141 , C01B2203/142 , C01B2203/143 , C01B2203/145 , C01B2203/148 , C01B2203/82 , C07C29/1518 , C10G3/49 , C10G3/52 , C10G3/62 , C10G2300/1022 , C10G2300/1025 , C10G2300/4043 , C10G2300/42 , C10G2400/20 , Y02P30/20 , Y02P30/40 , Y02P30/446 , C07C31/04
摘要： An improved method for the production of methanol and hydrocarbons from a methane-containing gas, such as natural gas. The improved method integrates a hydrocarbon synthesis unit with a methanol synthesis unit. The invention combines a syngas stream from a steam reformer, a syngas stream from an oxidation reformer and additional carbon dioxide to form an optimal syngas composition that is directed to a methanol synthesis reactor. The invention also integrates other process parameters and process components of a methanol and hydrocarbon synthesis process plant to effectively convert most of the carbon in the natural gas to commercial-value products. The invention is also directed to a method of making olefin from the methanol produced by the process of the invention.
摘要翻译：一种用于从含瓦斯气体如天然气生产甲醇和烃的改进方法。改进的方法将烃合成单元与甲醇合成单元结合。本发明结合了来自蒸汽重整器的合成气流，来自氧化重整器的合成气流和另外的二氧化碳，以形成被引导至甲醇合成反应器的最佳合成气组合物。本发明还集成了甲醇和烃合成工艺装置的其它工艺参数和工艺组件，以有效地将天然气中的大部分碳转化为商业价值产品。本发明还涉及由本发明方法生产的甲醇制备烯烃的方法。

6. 发明授权

US06444712B1 Methanol, olefin, and hydrocarbon synthesis process 失效
标题翻译：甲醇，烯烃和烃的合成过程
公开(公告)号：US06444712B1
公开(公告)日：2002-09-03
申请号：US09672470
申请日：2000-09-28
申请人： Gary F. Janda
发明人： Gary F. Janda
IPC分类号： C07C2700
CPC分类号： C10G2/30 , C01B3/382 , C01B3/386 , C01B2203/0233 , C01B2203/0238 , C01B2203/0244 , C01B2203/025 , C01B2203/0405 , C01B2203/0415 , C01B2203/043 , C01B2203/046 , C01B2203/0475 , C01B2203/06 , C01B2203/061 , C01B2203/062 , C01B2203/063 , C01B2203/065 , C01B2203/0811 , C01B2203/0816 , C01B2203/0838 , C01B2203/0844 , C01B2203/0866 , C01B2203/1052 , C01B2203/1082 , C01B2203/1241 , C01B2203/127 , C01B2203/141 , C01B2203/142 , C01B2203/143 , C01B2203/145 , C01B2203/148 , C01B2203/82 , C07C29/1518 , C10G3/49 , C10G2300/1022 , C10G2300/1025 , C10G2400/20 , Y02P30/20 , Y02P30/40 , C07C31/04
摘要： An improved method for the production of methanol and hydrocarbons from a methane-containing gas, such as natural gas. The improved method integrates a hydrocarbon synthesis unit with a methanol synthesis unit without the need to recycle unreacted syngas exiting the methanol synthesis reactor. The invention combines a syngas stream and additional carbon dioxide from the hydrocarbon synthesis unit to form an optimal syngas composition for methanol and hydrocarbon synthesis. The invention also integrates other process parameters and process components of a methanol and hydrocarbon synthesis process plant to effectively convert most of the carbon in the natural gas to commercial-value products. The invention is also directed to a method of making olefin from the methanol produced by the process of the invention.
摘要翻译：一种用于从含瓦斯气体如天然气生产甲醇和烃的改进方法。改进的方法将烃合成单元与甲醇合成装置整合，而不需要循环离开甲醇合成反应器的未反应的合成气。本发明将合成气流和来自烃合成单元的另外的二氧化碳组合以形成用于甲醇和烃合成的最佳合成气组合物。本发明还集成了甲醇和烃合成工艺装置的其它工艺参数和工艺组件，以有效地将天然气中的大部分碳转化为商业价值产品。本发明还涉及由本发明方法生产的甲醇制备烯烃的方法。

7. 发明授权

US06388156B1 Direct selective synthesis of para-xylene by reacting an aromatic compound with a methylating agent formed from CO, Co2 and H2 有权
标题翻译：通过使芳族化合物与由CO，CO 2和H 2形成的甲基化剂反应直接选择性合成对二甲苯
公开(公告)号：US06388156B1
公开(公告)日：2002-05-14
申请号：US09312104
申请日：1999-05-14
申请人： John D. Y. Ou , Gary F. Janda , Zongxuan Hong , Russell D. Sellen
发明人： John D. Y. Ou , Gary F. Janda , Zongxuan Hong , Russell D. Sellen
IPC分类号： C07C120
CPC分类号： C07C2/862 , B01J23/002 , B01J29/061 , B01J29/40 , B01J29/85 , B01J35/0006 , B01J37/0203 , B01J37/086 , B01J2229/12 , B01J2229/32 , B01J2229/34 , B01J2523/00 , Y02P20/52 , C07C15/08 , B01J2523/3712 , B01J2523/48
摘要： It has been discovered that para-xylene (PX) can be synthesized with improved selectivity by reacting an aromatic compound such as toluene and/or benzene with a reactant(s) such as a combination of hydrogen and carbon monoxide and/or carbon dioxide and/or methanol or methylating agents produced therefrom. Catalytic reaction systems are employed, such as crystalline or amorphous aluminosilicates having one-dimensional channel structure, para-alkyl selectivated crystalline or amorphous aluminosilicates, para-alkyl selectivated substituted aluminosilicates, crystalline or amorphous substituted silicates having one-dimensional channel structure, para-alkyl selectivated substituted silicates, crystalline or amorphous aluminophosphates, para-alkyl selectivated crystalline or amorphous aluminophosphates, para-alkyl selectivated zeolite-bound zeolite and para-alkyl selectivated substituted aluminophosphates, and mixtures thereof. The catalytic reaction systems may be selectivated with organometallic compounds, compounds of elements selected from Groups 1 through 16, coke, and mixtures thereof. Using this process, catalyst stability and life is improved.
摘要翻译：已经发现，通过使芳族化合物如甲苯和/或苯与诸如氢和一氧化碳和/或二氧化碳的组合的反应物反应，可以通过使诸如甲苯和/或苯等芳族化合物与/或二氧化碳的组合反应而使提高的选择性合成对二甲苯（PX） /或由其制备的甲醇或甲基化剂。使用催化反应体系，例如具有一维通道结构的结晶或无定形硅铝酸盐，对位烷基选择性结晶或无定形硅铝酸盐，对烷基选择取代的硅铝酸盐，具有一维通道结构的结晶或无定形取代的硅酸盐，对 - 烷基选择性取代的硅酸盐，结晶或无定形磷酸铝，对烷基选择性晶体或无定形磷酸铝，对位烷基选择性沸石键合沸石和对位烷基选择取代的铝磷酸盐，及其混合物。可以用有机金属化合物，选自第1至16组的元素的化合物，焦炭及其混合物选择催化反应体系。使用该方法，提高了催化剂的稳定性和寿命。

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