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71. 发明授权

US4851109A Integrated hydroprocessing scheme for production of premium quality distillates and lubricants 失效
标题翻译：一体化加氢处理方案，用于生产优质馏出物和润滑剂
公开(公告)号：US4851109A
公开(公告)日：1989-07-25
申请号：US192072
申请日：1988-05-09
申请人： Nai Y. Chen , Rene B. LaPierre , Randall D. Partridge , Stephen S. Wong
发明人： Nai Y. Chen , Rene B. LaPierre , Randall D. Partridge , Stephen S. Wong
IPC分类号： C10G65/12 , F02B3/06
CPC分类号： C10G65/12 , C10G2300/1074 , C10G2400/02 , C10G2400/04 , C10G2400/08 , F02B3/06
摘要： An integrated refining scheme for hydroprocessing high boiling fractions such as gas oil and catalytically cracked cycle oils to produce premium quality distillates, especially jet fuels and naphthas suitable for reforming into high octane gasoline. In addition, unconverted, high boiling fractions suitable for processing by conventional refining techniques into high quality, low pour point lube base stocks are obtained. The integrated hydroprocessing comprises a first stage hydrocracking step employing an aromatic selective hydrocracking catalyst based on a large pore size acidic component such as amorphous alumina or silica alumina or a large pore size zeolite such as zeolite X or zeolite Y. The hydrocracking may be operated either in a naphtha directing mode under conditions of moderate to high severity or under conditions of low to moderate severity to produce a relatively higher proportion of product boiling in the middle distillate range. The unconverted fraction from the hydrocracking step is passed to a second step in which it is hydroprocessed over a zeolite beta catalyst with additional hydrogenation-dehydrogenation functionality. In this stage, the paraffins remaining in the feed are attacked by the zeolite beta to form isoparaffins and conditions may be controlled to favor hydroisomerization over hydrocracking so as to increase the yield of middle distillate product, especially of highly isoparaffinic jet fuels and diesel fuel.
摘要翻译：一种用于加氢处理高沸点馏分（如瓦斯油和催化裂解循环油）的综合精炼方案，以生产优质馏出物，特别是适用于重整为高辛烷值汽油的喷气燃料和石脑油。此外，获得了适用于通过常规精制技术加工成高质量低倾点润滑油基础油料的未转化的高沸点馏分。一体化加氢处理包括使用基于大孔径酸性组分如无定形氧化铝或二氧化硅氧化铝或大孔径沸石如沸石X或沸石Y的芳族选择性加氢裂化催化剂的第一阶段加氢裂化步骤。加氢裂化可以在中等至高严重度的条件下或在低至中等严重度的条件下以石脑油引导模式在中间馏分范围内产生相对较高比例的沸点产物。来自加氢裂化步骤的未转化的级分被传递到第二步骤，其中其在具有另外的氢化 - 脱氢官能团的沸石β催化剂上进行加氢处理。在这个阶段，剩余在饲料中的链烷烃被沸石β攻击以形成异链烷烃，并且可以控制条件以有利于加氢裂化加氢异构化，从而提高中间馏分产物，特别是高度异链烷烃喷气燃料和柴油燃料的产率。

72. 发明授权

US4803186A Shape selective crystalline silicate zeolite containing intermetallic component and use as catalyst in hydrocarbon conversions 失效
标题翻译：含有金属间化合物的形状选择性结晶硅酸盐沸石，并用作烃转化中的催化剂
公开(公告)号：US4803186A
公开(公告)日：1989-02-07
申请号：US938095
申请日：1986-12-04
申请人： Nai Y. Chen , Thomas F. Degnan , Paul B. Weisz
发明人： Nai Y. Chen , Thomas F. Degnan , Paul B. Weisz
IPC分类号： B01J20060101 , B01J29/06 , B01J29/40 , B01J29/74 , C10G20060101 , C10G45/64 , B01J29/10 , B01J29/28
CPC分类号： C10G45/64 , B01J29/06 , B01J29/7415 , B01J2229/32 , B01J2229/36 , B01J29/40
摘要： The catalytic properties of a metal-containing shape selective crystalline silicate zeolite are significantly improved by converting said metal to an intermetallic compound. Thus, for example, zeolite beta containing the intermetallic component platinum zeolite demonstrates improved catalytic properties for dewaxing a hydrocarbon feedstock compared to zeolite beta containing platinum metal alone.

73. 发明授权

US4788169A Low acidity alumina-bound zeolites containing tetrahedral boron, gallium, indium and/or thallium 失效
标题翻译：含有四面体硼，镓，铟和/或铊的低酸性氧化铝键合沸石
公开(公告)号：US4788169A
公开(公告)日：1988-11-29
申请号：US112342
申请日：1987-10-26
申请人： Thomas F. Degman, Jr. , John D. Lutner , Nai Y. Chen
发明人： Thomas F. Degman, Jr. , John D. Lutner , Nai Y. Chen
IPC分类号： B01J29/04 , B01J29/87 , C10G11/05 , B01J29/06 , B01J29/28
CPC分类号： B01J29/04 , B01J29/87 , C10G11/05
摘要： A method for preparing low acidity alumina bound zeolites containing tetrahedral boron, gallium, indium and/or thallium which comprises ammonium-exchanging an organic-sorbed zeolite followed by calcination.
摘要翻译：一种制备含有四面体硼，镓，铟和/或铊的低酸性氧化铝结合沸石的方法，其包括将有机 - 吸附的沸石铵交换并进行煅烧。

74. 发明授权

US4737263A Process and apparatus for catalytic dewaxing of paraffinic stocks and the simultaneous removal of cracked products 失效
标题翻译：用于石蜡原料的催化脱蜡的方法和装置以及同时除去裂化产物
公开(公告)号：US4737263A
公开(公告)日：1988-04-12
申请号：US884466
申请日：1986-07-11
申请人： Nai Y. Chen , Thomas F. Degnan, Jr. , Bruce P. Pelrine , Richard F. Socha
发明人： Nai Y. Chen , Thomas F. Degnan, Jr. , Bruce P. Pelrine , Richard F. Socha
IPC分类号： C10G45/58 , C10G45/64 , C10G23/00
CPC分类号： C10G45/64 , C10G45/58
摘要： Dewaxing a waxy feedstock is achieved by submerging the dewaxing catalyst bed in the waxy feedstock and removing gaseous products out of contact with the catalyst by agitating the bed to prevent further cracking or polymerization. Catalyst aging during dewaxing is significantly reduced by operating the dewaxing reactor within a narrow low temperature range.
摘要翻译：脱蜡蜡质原料通过将脱蜡催化剂床浸没在蜡质原料中并通过搅拌床除去与催化剂接触的气态产物以防止进一步的开裂或聚合来实现。脱蜡过程中的催化剂老化通过在较低的低温范围内操作脱蜡反应器而显着降低。

75. 发明授权

US4668377A Catalytic process for dewaxing 失效
标题翻译：催化脱蜡工艺
公开(公告)号：US4668377A
公开(公告)日：1987-05-26
申请号：US789608
申请日：1985-10-21
申请人： Nai Y. Chen , Bruce P. Pelrine
发明人： Nai Y. Chen , Bruce P. Pelrine
IPC分类号： C10G45/64 , C10G11/05 , C10G47/16
CPC分类号： C10G45/64
摘要： A process for dewaxing lube basestocks over low acidity dewaxing catalysts can be undertaken at steady state temperature. In a preferred embodiment, the feedstock is subjected to catalytic dewaxing with concommident removal of gaseous product. When high boiling feed with end points above 1000.degree. F., such as heavy neutrals and bright stocks, and waxy feeds containing more than 20 wt % wax are subject of the process, it is preferred to use continuously stirred tank reactors.
摘要翻译：在低酸度脱蜡催化剂上脱蜡润滑油基础油的方法可以在稳态温度下进行。在优选的实施方案中，原料经过催化脱蜡，同时除去气体产物。当终点高于1000°F的高沸点饲料（如重质中性粒子和光亮的油料）和含有20％（重量）以上蜡的蜡质进料时，最好使用连续搅拌釜式反应器。

76. 发明授权

US4583993A Process for the production of carbon monoxide and hydrogen from carbonaceous material 失效
标题翻译：从碳质材料生产一氧化碳和氢气的方法
公开(公告)号：US4583993A
公开(公告)日：1986-04-22
申请号：US305675
申请日：1981-09-25
申请人： Nai Y. Chen
发明人： Nai Y. Chen
IPC分类号： C10J3/54
CPC分类号： C10J3/54 , C10J3/48 , C10J3/78 , C10J2300/093 , C10J2300/0959 , C10J2300/0976 , C10J2300/0986 , C10J2300/1815 , C10J2300/1846 , C10J2300/1884 , C10J2300/1892
摘要： Hydrogen and carbon monoxide are produced from coal, char or other carbonaceous material in a processing combination comprising a catalytic CO generator employing as reactant materials, fluid carbon material and CO.sub.2 product of the reaction of steam with CO to produce hydrogen and CO.sub.2. CO.sub.2 produced in the process is relied upon as the primary endothermic heat source in the fluid CO generator.
摘要翻译：氢和一氧化碳是由煤，炭或其他含碳材料在加工组合中生产的，该加工组合包括使用作为反应物材料的催化CO发生器，流体碳材料和蒸汽与CO的反应产生氢气和CO 2的CO 2产物。在该过程中产生的二氧化碳作为流体CO发生器中的主要吸热热源。

77. 发明授权

US4522703A Thermal treatment of heavy hydrocarbon oil 失效
标题翻译：重质烃油的热处理
公开(公告)号：US4522703A
公开(公告)日：1985-06-11
申请号：US554013
申请日：1983-11-21
申请人： Tsoung Y. Yan , Nai Y. Chen
发明人： Tsoung Y. Yan , Nai Y. Chen
IPC分类号： C10C3/00 , C10G9/00 , C10G9/14
CPC分类号： C10C3/002 , C10G9/00
摘要： This invention provides a process for upgrading heavy hydrocarbon oil by thermal treatment which in one preferred embodiment involves heating a petroleum residuum type of heavy oil feedstock at a temperature of 450.degree.-550.degree. C. and a pressure of 10-200 psi for a period of about 0.1-1 hour to convert at least 60 weight percent of the heavy oil to gasoline and gas oil range products, and additionally providing a residual tar fraction which has a fusion temperature below about 160.degree. C.About 1-10 weight percent of solid carbonaceous fines are incorporated in the feedstock to suppress the deposition of coke in the thermal treatment zone.
摘要翻译：本发明提供了一种通过热处理改质重质烃油的方法，在一个优选实施方案中，该方法包括在450-550℃的温度和10-200psi的压力下加热石油渣油类型的重油原料一段时间约0.1-1小时以将至少60重量％的重油转化为汽油和瓦斯油产品，并且另外提供熔点低于约160℃的残余焦油馏分。约1-10重量％将固体碳质细粉掺入原料中以抑制焦炭在热处理区中的沉积。

78. 发明授权

US4420561A Fermentation process 失效
标题翻译：发酵过程
公开(公告)号：US4420561A
公开(公告)日：1983-12-13
申请号：US230461
申请日：1981-02-02
申请人： Nai Y. Chen , Joseph N. Miale
发明人： Nai Y. Chen , Joseph N. Miale
IPC分类号： C07C29/76 , C12P7/06
CPC分类号： C12P7/06 , C07C29/76 , Y02E50/17 , Y10S435/942
摘要： In an ethanol fermentation process in which an aqueous solution of fermentable sugar is converted by an ethanol-producing microorganism such as a yeast to a dilute aqueous solution of ethanol with the ethanol being present in the solution at a concentration which does not exceed a predetermined maximum level, an improvement is provided which comprises selectively sorbing ethanol present in the solution within a hydrophilic crystalline aluminosilicate ZSM-5 or HZSM-5 zeolite so that the non-sorbed ethanol present in the solution does not exceed the predetermined maximum level of concentration therein, and thereafter removing sorbed ethanol from the zeolite.
摘要翻译：在乙醇发酵过程中，其中可发酵糖的水溶液由产乙醇的微生物如酵母转化为稀乙醇水溶液，乙醇以不超过预定最大值的浓度存在于溶液中水平，提供了一种改进，其包括选择性吸附在亲水结晶硅铝酸盐ZSM-5或HZSM-5沸石中的溶液中存在的乙醇，使得溶液中存在的未吸附的乙醇不超过其中预定的最大浓度水平，然后从沸石中除去吸附的乙醇。

79. 发明授权

US4419220A Catalytic dewaxing process 失效
标题翻译：催化脱蜡工艺
公开(公告)号：US4419220A
公开(公告)日：1983-12-06
申请号：US379422
申请日：1982-05-18
申请人： Rene B. LaPierre , Randall D. Partridge , Nai Y. Chen , Steven S. Wong
发明人： Rene B. LaPierre , Randall D. Partridge , Nai Y. Chen , Steven S. Wong
IPC分类号： C10G47/12 , B01J29/00 , B01J29/06 , C10G29/06 , C10G45/64 , C10G73/02 , C10G47/16
CPC分类号： C10G45/64 , C10G29/06 , Y10S208/02
摘要： Hydrocarbon feedstocks such as distillate fuel oils and gas oils are dewaxed by isomerizing the waxy components over a zeolite beta catalyst. The process may be carried out in the presence or absence of added hydrogen. Preferred catalysts have a zeolite silica:alumina ratio over 100:1.
摘要翻译：诸如馏出燃料油和瓦斯油之类的烃原料通过在沸石β催化剂上使蜡状组分异构化来脱蜡。该方法可以在存在或不加入氢气的情况下进行。优选的催化剂具有100:1以上的沸石二氧化硅：氧化铝比。

80. 发明授权

US4259174A Catalytic dewaxing of hydrocarbon oils 失效
标题翻译：烃油的催化脱蜡
公开(公告)号：US4259174A
公开(公告)日：1981-03-31
申请号：US21735
申请日：1979-03-19
申请人： Nai Y. Chen , William E. Garwood
发明人： Nai Y. Chen , William E. Garwood
IPC分类号： C10G73/02 , B01J29/50 , B01J29/54 , C10G45/64 , C10G1/04 , C10G11/05 , C10G21/00 , C10G47/16
CPC分类号： B01J29/505 , B01J29/54 , C10G45/64
摘要： Hydrocarbon oils, especially waxy distillate lubricating oil stocks suitable for the preparation, by conventional unit processes, of high V.I., low pour point lubricating oils, are advantageously catalytically dewaxed with synthetic offretite catalyst preferably associated with a hydrogenation metal such as platinum or palladium.
摘要翻译：烃类油，特别是适用于通过常规单元方法制备高含量低倾点润滑油的蜡状馏出物润滑油，有利地用合成的漂白剂催化剂进行催化脱蜡，优选与氢化金属如铂或钯缔合。

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