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61. 发明授权

US06525228B2 Process of telomerizing conjugated dienes 失效
公开(公告)号：US06525228B2
公开(公告)日：2003-02-25
申请号：US10036265
申请日：2001-10-22
申请人： Yves Chauvin , Lionel Magna , Gerald Peter Niccolai , Jean-Marie Basset
发明人： Yves Chauvin , Lionel Magna , Gerald Peter Niccolai , Jean-Marie Basset
IPC分类号： C07C4101
CPC分类号： B01J31/0284 , B01J31/2239 , B01J31/2404 , B01J2231/20 , B01J2531/824 , B01J2531/96 , B01J2540/32 , C07C29/36 , C07C41/06 , Y02P20/584 , C07C43/15 , C07C33/02
摘要： The present invention is related to a process for telomerizing a conjugated diene which comprises reacting said conjugated diene with a compound containing active hydrogen in the presence of a catalyst system comprising at least one transition metal compound, at least one phosphorus-containing compound, and at least one salt which forms a liquid under the conditions of the telomerization process.

62. 发明授权

US6040263A Catalytic composition based on transition metal complexes, and a process for the hydrogenation of unsaturated compounds 有权
标题翻译：基于过渡金属络合物的催化组合物，以及不饱和化合物氢化的方法
公开(公告)号：US6040263A
公开(公告)日：2000-03-21
申请号：US154402
申请日：1998-09-15
申请人： Lothar Mussmann , Yves Chauvin , Helene Olivier
发明人： Lothar Mussmann , Yves Chauvin , Helene Olivier
IPC分类号： B01J31/22 , B01J23/46 , B01J31/02 , B01J31/16 , B01J31/24 , C07B61/00 , C07C5/03 , C07C5/11 , C07C9/00 , C07C13/20 , C07C13/58 , B01J31/00 , C07C5/02 , C07C5/05 , C07C5/10
CPC分类号： B01J31/16 , B01J31/0278 , B01J31/0284 , B01J31/0288 , B01J31/20 , B01J31/2291 , B01J31/2404 , B01J31/2409 , B01J2231/645 , B01J23/462 , B01J23/464 , B01J2531/821 , B01J2531/822 , B01J2531/824 , B01J2531/827 , B01J2531/828 , B01J2531/845
摘要： A novel non-aqueous catalytic composition comprises at least one quaternary ammonium and/or phosphonium salt in which the anion is selected from the group consisting of tetrafluoroborate, tetrachloroborate, hexafluorophosphate, hexafluoroantimonate, hexafluoroarsenate, trifluorosulphonate, fluorosulphonate, trifluoromethylsulphonate, trifluoroarsenate, dichlorocuprate, trichlorocuprate, tetrachlorocuprate, and trichlorozincate, and at least one complex of a transition metal from groups 8, 9 or 10, i.e., iron, ruthenium, colbalt, rhodium iridium, nickel, palladium and platinum. The catalyst can be used in a process of total or selective hydrogenation of unsaturated compounds such as monoolefins, diolefins, acetylene compounds, aromatic compounds, or polynuclear aromatic compounds. Hydrogenation may be accompanied by isomerisation.
摘要翻译：一种新型非水催化剂组合物包含至少一种季铵盐和/或鏻盐，其中阴离子选自四氟硼酸盐，四氯硼酸盐，六氟磷酸盐，六氟锑酸盐，六氟砷酸盐，三氟磺酸盐，氟磺酸盐，三氟甲基磺酸盐，三氟砷酸盐，二氯磷酸盐，三氯代磷酸盐四氯蔗糖和三氯酸锌，以及至少一种来自组8,9或10的过渡金属络合物，即铁，钌，钴，铑，铱，镍，钯和铂。催化剂可用于不饱和化合物如单烯烃，二烯烃，乙炔化合物，芳香族化合物或多核芳族化合物的全部或选择性氢化的方法。氢化可伴随异构化。

63. 发明授权

US5780702A Process for displacing the double bond in olefins using a catalytic composition based on transition metal complexes 失效
标题翻译：使用基于过渡金属络合物的催化组合物来置换烯烃中的双键的方法
公开(公告)号：US5780702A
公开(公告)日：1998-07-14
申请号：US664561
申请日：1996-06-17
申请人： Yves Chauvin , Lothar Mussmann , Helene Olivier
发明人： Yves Chauvin , Lothar Mussmann , Helene Olivier
IPC分类号： B01J31/24 , C07B61/00 , C07C5/25 , C07C11/02 , C07C11/10 , C07C5/23
CPC分类号： C07C5/2562
摘要： A catalytic composition comprises at least one quaternary ammonium and/or phosphonium salt in which the anion is preferably selected from the group formed by tetrafluoroborate, tetrachloroborate, hexafluorophosphate, hexafluoroantimonate, hexafluoroarsenate, trifluorosulphonate, fluorosulphonate, tetrachloroaluminate, dichlorocuprate, and trichlorozincate, and at least one complex of a transition metal from groups 8, 9 and 10, i.e., iron, ruthenium, cobalt, rhodium, iridium, nickel, palladium and platinum, is for the displacement of the double bond in olefins.
摘要翻译：催化剂组合物包含至少一种季铵盐和/或鏻盐，其中阴离子优选选自四氟硼酸盐，四氯硼酸盐，六氟磷酸盐，六氟锑酸盐，六氟砷酸盐，三氟磺酸盐，氟磺酸盐，四氯铝酸盐，二氯磷酸盐和三氯酸锌形成的基团，来自组8,9和10的过渡金属的一个复合物，即铁，钌，钴，铑，铱，镍，钯和铂，用于在烯烃中置换双键。

64. 发明授权

US5750455A Catalytic composition and process for the alkylation of aliphatic hydrocarbons 失效
标题翻译：用于烷基化脂族烃的催化组合物和方法
公开(公告)号：US5750455A
公开(公告)日：1998-05-12
申请号：US547205
申请日：1995-10-24
申请人： Yves Chauvin , Andre Hirschauer , Helene Olivier
发明人： Yves Chauvin , Andre Hirschauer , Helene Olivier
IPC分类号： B01J31/22 , B01J27/122 , B01J31/02 , B01J31/30 , C07B61/00 , C07C2/60 , C07C9/16 , B01J31/00 , B01J23/70 , C07C2/58
CPC分类号： C07C2/60 , B01J27/122 , B01J31/0284 , B01J31/26 , B01J31/30 , B01J2231/321 , C07C2527/08 , C07C2527/10 , C07C2527/122 , C07C2527/125 , C07C2531/02 , C07C2531/26
摘要： The invention concerns a catalytic composition resulting from mixing at least one aluminum halide, at least one quaternary ammonium halide and/or at least one amine halohydrate and at least one cuprous compound, preferable a halide. The invention also concerns a process for the alkylation of isoparaffins by olefins with that composition.
摘要翻译：本发明涉及通过混合至少一种卤化铝，至少一种季铵卤化物和/或至少一种胺卤化水合物和至少一种亚铜化合物，优选卤化物而得到的催化组合物。本发明还涉及用该组合物用烯烃烷基化异链烷烃的方法。

65. 发明授权

US5675051A Catalytic composition and olefin disproportion process 失效
标题翻译：催化组分和烯烃不成比例过程
公开(公告)号：US5675051A
公开(公告)日：1997-10-07
申请号：US551338
申请日：1995-11-01
申请人： Yves Chauvin , Francoise Di Marco-Van Tiggelen
发明人： Yves Chauvin , Francoise Di Marco-Van Tiggelen
IPC分类号： B01J31/22 , B01J31/02 , B01J31/12 , B01J31/14 , C07B61/00 , C07C6/04 , C07C11/02 , C07C6/00
CPC分类号： C07C6/04 , B01J31/0239 , B01J31/0268 , B01J31/0278 , B01J31/0284 , B01J31/0288 , B01J31/143 , B01J31/2226 , B01J2231/543 , B01J2531/64 , B01J2531/66 , C07C2531/12
摘要： The invention concerns a catalytic olefin disproportion (also known as metathesis) process wherein the catalyst produced by dissolving a tungsten and/or molybdenum compound, more particularly a tungsten and/or molybdenum halide substituted with one or more phenoxo groups containing at least two hydrocarbon substituents in the ortho, ortho' positions, in a medium produced by mixing at least one quaternary ammonium halide and/or at least one quaternary phosphonium halide, at least one aluminium halide, and an organometallic aluminium compound.
摘要翻译：本发明涉及催化烯烃不成比例（也称为复分解）方法，其中通过溶解钨和/或钼化合物，更特别是被含有至少两个烃取代基的一个或多个苯氧基取代的钨和/或卤化钼产生的催化剂在通过混合至少一种季铵卤化物和/或至少一种季鏻卤化物，至少一种卤化铝和有机金属铝化合物制备的介质中的邻位，邻位。

66. 发明授权

US5525567A Catalytic composition and olefin disproportion process 失效
标题翻译：催化组分和烯烃不成比例过程
公开(公告)号：US5525567A
公开(公告)日：1996-06-11
申请号：US377705
申请日：1995-01-25
申请人： Yves Chauvin , Francoise Di Marco-Van Tiggelen
发明人： Yves Chauvin , Francoise Di Marco-Van Tiggelen
IPC分类号： B01J31/22 , B01J31/02 , B01J31/12 , B01J31/14 , C07B61/00 , C07C6/04 , C07C11/02 , B01J31/00 , B01J31/18 , B01J31/34
CPC分类号： C07C6/04 , B01J31/0239 , B01J31/0268 , B01J31/0278 , B01J31/0284 , B01J31/0288 , B01J31/143 , B01J31/2226 , B01J2231/543 , B01J2531/64 , B01J2531/66 , C07C2531/12
摘要： The invention concerns a catalytic composition for olefin disproportion (also known as metathesis) produced by dissolving a tungsten and/or molybdenum compound, more particularly a tungsten and/or molybdenum halide substituted with one or more phenoxo groups containing at least two hydrocarbon substituents in the ortho, ortho' positions, in a medium produced by mixing at least one quaternary ammonium halide and/or at least one quaternary phosphonium halide, at least one aluminum halide, and an organometallic aluminum compound.The invention also concerns an olefin disproportion process using this composition.
摘要翻译：本发明涉及通过将钨和/或钼化合物，更特别是被一个或多个含有至少两个烃取代基的苯氧基取代的钨和/或钼卤化物溶解在所述烯烃不成比例（也称为复分解）在通过混合至少一种季铵卤化物和/或至少一种季鏻卤化物，至少一种卤化铝和有机金属铝化合物产生的介质中的邻位，邻位。本发明还涉及使用该组合物的烯烃不成比例的方法。

67. 发明授权

US5476956A Process for codimerization of dienes and olefins 失效
标题翻译：二烯和烯烃的同分异构化方法
公开(公告)号：US5476956A
公开(公告)日：1995-12-19
申请号：US232984
申请日：1994-04-25
申请人： Gerard Hillion , Robert Stern , Abakar Kotoko , Yves Chauvin
发明人： Gerard Hillion , Robert Stern , Abakar Kotoko , Yves Chauvin
IPC分类号： B01J27/13 , B01J31/16 , C07B37/02 , C07B61/00 , C07C2/04 , C07C2/38 , C07C11/12 , C07C67/347 , C07C69/65 , C09F7/06
CPC分类号： C07C2/04 , C07B37/02 , C07C67/347 , C07C2531/22
摘要： Co dimerization is conducted of at least one monoolefin, for example a monoolefinic hydrocarbon such as ethylene, propylene or 1-butene, a halogenated monoolefin such as vinyl chloride, or an olefinic functional compound such as methyl acrylate, acrylonitrile, allyl acetate or vinyl acetate, with at least one polyolefin containing at least two conjugated or unconjugated ethylene bonds, for example a diene hydrocarbon such as 1,3-butadiene, piperylene, or isoprene or a polyolefin containing a carboxylic function, such as a fatty acid or a fatty acid ester having 14 to 24 carbon atoms in the fatty chain derived, for example, from a natural oil. The reaction is carried out in the presence of a catalytic system having general formula [RhX.sub.4 ][YR.sub.4 ] where X represents a halogen ion or a SO.sub.4.sup.--, SO.sub.3.sup.-, OH.sup.-, OR.sup.- or R.sup.- group, at least one X being a halogen ion, Y represents a nitrogen atom or a phosphorous atom, and R represents an alkyl, cycloalkyl, alkenyl, aryl, alkylaryl, polystyryl, alkyl polystyryl or acyl radical.
摘要翻译： Co二聚化由至少一种单烯烃，例如单烯烃如乙烯，丙烯或1-丁烯，卤代单烯烃如氯乙烯或烯属官能化合物如丙烯酸甲酯，丙烯腈，乙酸烯丙酯或乙酸乙烯酯与至少一种含有至少两个共轭或非共轭的乙烯键的聚烯烃，例如二烯烃如1,3-丁二烯，戊间二烯或异戊二烯或含有羧酸官能团的聚烯烃如脂肪酸或脂肪酸在脂肪链中具有14至24个碳原子的酯衍生自例如天然油。该反应在具有通式[RhX4] [YR4]的催化体系存在下进行，其中X表示卤素离子或SO 4 - ，SO 3 - ，OH-，OR-或R-基团，至少一个X 作为卤素离子，Y表示氮原子或磷原子，R表示烷基，环烷基，烯基，芳基，烷基芳基，聚苯乙烯基，烷基聚苯乙烯基或酰基。

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