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41. 发明授权

US4717782A Catalytic process for oligomerizing ethene 失效
标题翻译：催化乙烯齐聚的方法
公开(公告)号：US4717782A
公开(公告)日：1988-01-05
申请号：US893522
申请日：1986-08-05
申请人： William E. Garwood , John D. Kushnerick , Samuel A. Tabak
发明人： William E. Garwood , John D. Kushnerick , Samuel A. Tabak
IPC分类号： C07C2/12 , C07C2/02
CPC分类号： C07C2/12 , C07C2529/46 , Y02P20/52
摘要： A continuous catalytic process for converting ethene-rich olefinic feedstock containing reducing gas to heavier liquid hydrocarbon product, comprising the steps ofcontacting the ethene-rich feedstock at elevated temperature in a catalytic reaction zone with a zeolite catalyst comprising a nickel-ethene oligomerization component and a shape-selective medium pore acid zeolite oligomerization component to convert at least a portion of the lower olefinic components to heavier olefinic hydrocarbons; andfeeding water with the feedstock in sufficient amount to prevent substantial reduction of the nickel component.
摘要翻译：一种用于将含有还原气体的富含烯烃的烯烃原料转化为较重液体烃产物的连续催化方法，包括以下步骤：使催化反应区中升温的富含乙烯的原料与包含镍 - 乙烯低聚组分的沸石催化剂和形状选择性中孔酸性沸石低聚组分，将至少一部分较低级烯烃组分转化成较重的烯烃; 并用足够量的原料给予原料以防止镍组分的显着减少。

42. 发明授权

US4549396A Conversion of coal to electricity 失效
标题翻译：煤转电
公开(公告)号：US4549396A
公开(公告)日：1985-10-29
申请号：US339962
申请日：1982-01-18
申请人： William E. Garwood , James C. Kuo , Solomon M. Jacob , John J. Wise
发明人： William E. Garwood , James C. Kuo , Solomon M. Jacob , John J. Wise
IPC分类号： F02B43/08
CPC分类号： F02B43/08 , Y02T10/32 , Y10S48/06
摘要： Utilizing air, rather than oxygen, to convert coal to synthesis gas containing very high proportions of inert nitrogen; subjecting this entire gas, possibly with intermediate cleanup, e.g., sulfur removal, to conversion over a special metal-zeolite catalyst to produce a product comprising C.sub.5 to C.sub.11 normally liquid hydrocarbons, a gas containing C.sub.1 to C.sub.4 hydrocarbons, carbon dioxide and large proportions of nitrogen, and an aqueous product comprising water; utilizing the gas product to run electric power generation equipment, such as a direct fired turbine, at base load levels; storing and accumulating the liquid product; and intermittently using the liquid product for electric power generation to meet higher than base loads, including peak load situations.
摘要翻译：利用空气而不是氧将煤转化成含有非常高比例惰性氮的合成气; 对整个气体进行处理，可能进行中间清洗，例如除硫，通过特殊的金属 - 沸石催化剂进行转化，生产出包含C 1到C 11通常为液态烃的产物，含有C1至C4烃的气体，二氧化碳和大比例氮气和包含水的含水产物; 利用气体产品以基本负载水平运行诸如直接燃烧的涡轮机的发电设备; 储存和积聚液体产品; 并间歇地使用液体产品进行发电，以满足高于基本负载，包括峰值负载情况。

43. 发明授权

US4413153A Integrated process for making transportation fuels and lubes from wet natural gas 失效
标题翻译：从湿天然气制造运输燃料和润滑油的综合过程
公开(公告)号：US4413153A
公开(公告)日：1983-11-01
申请号：US436158
申请日：1982-10-22
申请人： William E. Garwood , Wooyoung Lee
发明人： William E. Garwood , Wooyoung Lee
IPC分类号： C10G3/00 , C10G50/00 , C10G57/02 , F02B3/06 , C07C1/04
CPC分类号： C10G50/00 , C10G2400/02 , C10G2400/04 , C10G2400/08 , C10G2400/10 , F02B3/06 , Y02P30/20
摘要： The synthetic fuel slate of products derived from wet natural gas is expanded to include both aromatic gasoline from the methane rich dry gas portion via steam reforming to synthesis gas, the production of methanol from synthesis gas and the conversion of methanol to gasoline over a ZSM-5 type catalyst, plus high quality jet fuel, diesel fuel and lubricating oils from the C.sub.3.sup.+ paraffin rich fraction of wet natural gas via thermal cracking of the paraffin rich fraction to olefins and the conversion of the olefins to gasoline and distillate boiling range hydrocarbons over a ZSM-5 type catalyst. Methane separated from the thermal cracked product can be mixed with the dry gas fraction for synthesis gas production and a portion of the hydrogen from the synthesis gas may be used to hydrogenate the distillate fraction from the catalytic conversion of the thermal cracked product.
摘要翻译：来自湿天然气的产品的合成燃料石板膨胀，包括从富甲烷干燥部分通过蒸汽重整到合成气的芳香族汽油，从合成气生产甲醇，通过ZSM- 5型催化剂，加上高品质的喷气燃料，柴油燃料和润滑油，通过富含馏分的烯烃的热裂解将烯烃转化为汽油和馏出物沸点烃，来自富含天然气的C3 +石蜡馏分 ZSM-5型催化剂。与热裂解产物分离的甲烷可以与用于合成气生产的干燥气体馏分混合，并且可以使用来自合成气的一部分氢气从热裂化产物的催化转化中氢化馏出物馏分。

44. 发明授权

US4376036A Production of high V. I. lubricating oil stock 失效
标题翻译：生产高V. I.润滑油原料
公开(公告)号：US4376036A
公开(公告)日：1983-03-08
申请号：US241319
申请日：1981-03-06
申请人： William E. Garwood , Paul G. Rodewald , Nai Y. Chen
发明人： William E. Garwood , Paul G. Rodewald , Nai Y. Chen
IPC分类号： B01J21/08 , B01J29/40 , B01J29/70 , C10G45/64 , C10G47/16
CPC分类号： B01J29/40 , B01J21/08 , B01J2229/26 , B01J2229/42 , B01J29/70 , C10G2400/10
摘要： A process for the manufacture of high quality lubricating oils having a high viscosity index and low pour point is disclosed which comprises catalytically dewaxing a lubricating oil stock by contacting the same in the presence of hydrogen over a zeolite such as ZSM-5 which has been silica-modified.
摘要翻译：公开了一种用于制造具有高粘度指数和低倾点的高品质润滑油的方法，其包括通过在氢气存在下使其与沸石如ZSM-5（其已经是二氧化硅）接触来催化脱蜡润滑油原料 -改性。

45. 发明授权

US4304871A Conversion of synthesis gas to hydrocarbon mixtures utilizing a dual catalyst bed 失效
标题翻译：使用双催化剂床将合成气转化为烃混合物
公开(公告)号：US4304871A
公开(公告)日：1981-12-08
申请号：US825875
申请日：1977-08-19
申请人： James A. Brennan , Philip D. Caesar , Julius Ciric , William E. Garwood
发明人： James A. Brennan , Philip D. Caesar , Julius Ciric , William E. Garwood
IPC分类号： C07C1/04
CPC分类号： C07C1/044 , C07C1/0435 , C07C1/0485 , C07C2529/46
摘要： A gaseous mixture of carbon monoxide and hydrogen is passed in contact over a first catalyst bed comprising an iron or cobalt containing Fischer-Tropsch catalyst in combination with a crystalline aluminosilicate of the class of crystalline zeolite represented by ZSM-5 so as to obtain a liquid hydrocarbon product having a boiling range of less than 400.degree. F. at a 90% overhead and being a predominantly olefinic product. The total products from said contact including said liquid hydrocarbon product are then converted over a second catalyst bed containing HZSM-5 to obtain a highly aromatic product, i.e., greater than 20 weight percent.
摘要翻译：将一氧化碳和氢气的气体混合物在包含含铁或钴的费 - 托催化剂的第一催化剂床上与由ZSM-5表示的结晶沸石类的结晶硅铝酸盐组合使其接触，以获得液体烃产物在90％塔顶馏出物下沸点低于400°F，主要是烯烃产物。来自包括所述液体烃产物的所述接触的总产物然后在含有HZSM-5的第二催化剂床上转化，以获得高度芳族的产物，即大于20重量％。

46. 发明授权

US4283272A Manufacture of hydrocracked low pour lubricating oils 失效
标题翻译：加氢裂化低润滑油的制造
公开(公告)号：US4283272A
公开(公告)日：1981-08-11
申请号：US159011
申请日：1980-06-12
申请人： William E. Garwood , Murray R. Silk
发明人： William E. Garwood , Murray R. Silk
IPC分类号： C10G47/16 , C10G49/22 , C10G65/12 , C10G67/00 , C10G67/06
CPC分类号： C10G65/12 , C10G2400/10
摘要： Hydrocracked, low pour lubricating oils of good stability are manufactured by passing a suitable hydrocarbon feed and hydrogen sequentially through a hydrocracking zone, a catalytic dewaxing zone, and a hydrotreating zone, all at high pressure and in that order, with purification of the hydrogen gas prior to passage to the dewaxing zone. By maintaining all zones at high pressure, the efficiency of the process is augmented.
摘要翻译：通过使合适的烃进料和氢气依次通过加氢裂化区，催化脱蜡区和加氢处理区，全部以高压和顺序通过氢气净化来制备加氢裂化的低倾点润滑油在通过脱蜡区之前。通过将所有区域保持在高压状态，增加了处理效率。

47. 发明授权

US4269783A Conversion of syngas to high octane olefinic naphtha 失效
标题翻译：合成气转化为高辛烷值的烯烃石脑油
公开(公告)号：US4269783A
公开(公告)日：1981-05-26
申请号：US775129
申请日：1977-03-07
申请人： James A. Brennan , Philip D. Caesar , Julius Ciric , William E. Garwood , Robert E. Holland
发明人： James A. Brennan , Philip D. Caesar , Julius Ciric , William E. Garwood , Robert E. Holland
IPC分类号： C07C1/02 , C07C27/06
CPC分类号： C07C1/02 , C07C2521/12 , C07C2521/14 , C07C2523/745 , C07C2529/14 , C07C2529/24 , C07C2529/56 , C07C2529/76
摘要： A method is disclosed for the conversion of a syngas to a liquid hydrocarbon product having a boiling range of less than 400.degree. F. at a 90% overhead and being a predominantly olefinic product, wherein the olefins have substantially internal double bonds. The method for accomplishing this stated result involves an improvement in the method for the conversion of synthesis gas by contacting the same with a catalyst composite comprising a mixture of a Fischer-Tropsch catalyst and a volume excess of an acidic catalyst, e.g., silica-alumina or a crystalline aluminosilicate zeolite and wherein the activity of the acidic component is balanced with the activity of the Fischer-Tropsch component so as to maximize the yield of desired olefinic product.
摘要翻译：公开了一种在90％塔顶馏分将合成气转化为沸点低于400°F的液体烃产物并且主要是烯烃产物的方法，其中烯烃具有基本上内部的双键。实现所述结果的方法涉及通过使合成气与包含费 - 托催化剂和体积过量的酸性催化剂的混合物的催化剂复合物接触来改进合成气的方法，例如二氧化硅 - 氧化铝或结晶硅铝酸盐沸石，并且其中酸性组分的活性与费 - 托组分的活性相平衡，以使所需烯属产物的产率最大化。

48. 发明授权

US4227992A Process for separating ethylene from light olefin mixtures while producing both gasoline and fuel oil 失效
标题翻译：在轻质烯烃混合物中分离乙烯同时生产汽油和燃油的方法
公开(公告)号：US4227992A
公开(公告)日：1980-10-14
申请号：US41843
申请日：1979-05-24
申请人： William E. Garwood , Wooyoung Lee
发明人： William E. Garwood , Wooyoung Lee
IPC分类号： B01J29/40 , C07C7/148 , C10G29/16 , C10G35/095 , C10G35/06
CPC分类号： C10G35/095 , B01J29/40 , C07C7/148 , C10G29/16 , Y02P20/52
摘要： A process is disclosed for separating ethylene in admixture with light olefins by contacting said olefinic mixture under very critical reaction conditions over a special catalyst, such as a zeolite of the ZSM-5 type so as to selectively react the C.sub.3 and higher olefins and convert the same to both gasoline and fuel oil.
摘要翻译：公开了一种用于通过在非常临界的反应条件下使所述烯烃混合物在特殊催化剂如ZSM-5型沸石上接触来分离乙烯与轻质烯烃混合的方法，以选择性地使C3和更高级烯烃反应，并将与汽油和燃油相同。

49. 发明授权

US4149960A Gas oil processing 失效
标题翻译：瓦斯油加工
公开(公告)号：US4149960A
公开(公告)日：1979-04-17
申请号：US889483
申请日：1978-03-23
申请人： William E. Garwood , Philip D. Caesar , James A. Brennan
发明人： William E. Garwood , Philip D. Caesar , James A. Brennan
IPC分类号： B01J29/00 , B01J29/40 , B01J29/65 , B01J29/70 , C10G11/05 , C10G29/16 , C10G45/64 , C10G73/02 , C10G13/04 , B01J29/28 , C10G11/04
CPC分类号： C10G29/16 , B01J29/40 , C10G11/05 , B01J2229/26 , B01J2229/42 , B01J29/65 , B01J29/70 , C10G2400/06
摘要： An improved processing technique is provided for gas oil pour point reduction and dewaxing. The improved technique comprises contacting an appropriate gas oil feedstock with a catalyst comprising a crystalline aluminosilicate zeolite characterized by a silica/alumina mole ratio of at least 12 and a constraint index, hereinafter defined, within the approximate range of 1 to 12 in the presence of a relatively large amount of co-fed water. The amount of co-fed water is maintained at from about 0.5 to about 15 moles of water/mole of gas oil feedstock.
摘要翻译：提供了一种改进的加工技术，用于瓦斯油倾点降低和脱蜡。改进的技术包括使合适的瓦斯油原料与包含结晶硅铝酸盐沸石的催化剂接触，其结晶硅铝酸盐沸石的特征在于二氧化硅/氧化铝摩尔比为至少12，约束指数（下文中定义）在大约1至12的范围内，相对大量的共同供水。共同供水的量保持在约0.5至约15摩尔的水/摩尔瓦斯油原料。

50. 发明授权

US3950241A Method for upgrading a wide cut naphtha to full range gasoline 失效
标题翻译：一种将切割片段切割成全范围汽油的方法
公开(公告)号：US3950241A
公开(公告)日：1976-04-13
申请号：US482537
申请日：1974-06-24
申请人： John C. Bonacci , William E. Garwood
发明人： John C. Bonacci , William E. Garwood
IPC分类号： C10G59/02 , C10G37/00
CPC分类号： C10G59/02
摘要： Upgrading a full boiling range naphtha by the combination of reforming only a low boiling portion of the naphtha followed by contacting the reformate product thereof combined with the high boiling portion of the naphtha over a ZSM-5 type catalyst conversion operation is described.

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