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31. 发明授权

US4340685A Process for preparing polybutadiene having a 1,2-configuration content of 5-40% and a cis-1,4-configuration content of 60% or more 失效
标题翻译：制备1,2-构型含量为5-40％，顺式-1,4-构型含量为60％以上的聚丁二烯的方法
公开(公告)号：US4340685A
公开(公告)日：1982-07-20
申请号：US228625
申请日：1981-01-26
申请人： Yasumasa Takeuchi , Yutaka Obata , Noboru Ohshima , Tooru Shibata , Kaoru Nakako
发明人： Yasumasa Takeuchi , Yutaka Obata , Noboru Ohshima , Tooru Shibata , Kaoru Nakako
IPC分类号： C08F2/00 , C08F2/04 , C08F2/06 , C08F2/44 , C08F4/00 , C08F4/26 , C08F4/60 , C08F4/70 , C08F36/00 , C08F36/06 , C08F136/06
CPC分类号： C08F136/06
摘要： A process for preparing polybutadiene having a 1,2-configuration content of 5-40% and a cis-1,4-configuration content of 60% or more, which comprises polymerizing 1,3-butadiene in the presence of a catalyst consisting of:(A) a cobalt compound,(B) at least one member selected from the group consisting of:(i) a trialkylaluminum,(ii) a reaction product of a trialkylaluminum and an alcohol or water,(iii) a mixture of a trialkylaluminum and a dialkylaluminum halide,(iv) a dialkylaluminum hydride, and(v) an organolithium compound, and(C) at least one compound selected from the group consisting of phenyl isothiocyanate and carbon disulfide, in a hydrocarbon or halogenated hydrocarbon solution of a high cis-1,4-polybutadiene obtained by polymerizing 1,3-butadiene with a catalyst consisting of:(D) at least one compound selected from the group consisting of the organocarboxylates of nickel and organic complex compounds of nickel,(E) at least one compound selected from the group consisting of boron trifluoride, boron trifluoride complex compounds and hydrogen fluoride, and(F) at least one compound selected from the group consisting of the organometallic compounds of the alkali metals of the Group II or III metals of the Periodic Table. The polybutadiene produced by this process has an improved tear strength and improved flexural fatigue properties.
摘要翻译：一种制备1,2-构型含量为5-40％，顺式-1,4-构型含量为60％以上的聚丁二烯的方法，其包括在催化剂存在下将1,3-丁二烯聚合，所述催化剂由：（A）钴化合物，（B）选自由以下组成的组中的至少一种：（i）三烷基铝，（ii）三烷基铝与醇或水的反应产物，（iii）三烷基铝和二烷基卤化铝，（iv）氢化二烷基铝，和（v）有机锂化合物，和（C）至少一种选自异硫氰酸苯酯和二硫化碳的化合物在烃或卤代烃溶液中通过由以下组成的催化剂聚合1,3-丁二烯获得的高顺式-1,4-聚丁二烯：（D）至少一种选自镍的有机羧酸盐和镍的有机络合物的化合物，（E）在选自组中的至少一种化合物三氟化硼配位化合物和氟化氢，和（F）选自元素周期表第二或第三族金属的碱金属的有机金属化合物中的至少一种化合物。通过该方法制备的聚丁二烯具有改进的撕裂强度和改善的弯曲疲劳性能。

32. 发明授权

US08870976B2 Method for manufacturing a secondary battery 有权
标题翻译：二次电池的制造方法
公开(公告)号：US08870976B2
公开(公告)日：2014-10-28
申请号：US11896068
申请日：2007-08-29
申请人： Shigeo Kondo , Yasumasa Takeuchi
发明人： Shigeo Kondo , Yasumasa Takeuchi
IPC分类号： H01M4/82 , H01M4/13 , H01M10/44
CPC分类号： H01M10/44 , Y02E60/12 , Y10T29/49108 , Y10T29/4911 , Y10T29/49112 , Y10T29/49115
摘要： A secondary battery that can avoid reduction in battery capacity over the lapse of charge-discharge cycles and can exhibit high performance is provided. A method for manufacturing a secondary battery, the secondary battery including a laminated body having a pair of electrodes and an electrolyte layer provided between the pair of electrodes, the laminated body having an end portion, and a restrictor provided so as to cover at least the end portion of the laminated body for restricting expansion of the electrolyte layer in the plane direction thereof, the method includes preparing a mold, the pair of electrodes and electrolyte particles for forming the electrolyte layer, joining the pair of electrodes and the electrolyte layer together by pressing the electrodes and the electrolyte particles within the mold to form the laminated body, and providing the restrictor so as to cover at least the end portion of the laminated body removed from the mold.
摘要翻译：提供了能够避免在充放电循环过程中电池容量下降并且可以表现出高性能的二次电池。一种二次电池的制造方法，所述二次电池包括具有一对电极的层叠体和设置在所述一对电极之间的电解质层，所述层叠体具有端部，所述限制器设置成至少覆盖所述电极层叠体的端部，用于限制电解质层在其平面方向上的膨胀，该方法包括制备模具，用于形成电解质层的一对电极和电解质颗粒，将一对电极和电解质层一起接合在一起，由将模具内的电极和电解质颗粒按压以形成层叠体，并且设置限制器以至少覆盖从模具移除的层压体的至少端部。

33. 发明授权

US08614020B2 Electrochemical device 有权
公开(公告)号：US08614020B2
公开(公告)日：2013-12-24
申请号：US12232794
申请日：2008-09-24
申请人： Shigeo Kondo , Yasumasa Takeuchi , Yuji Shinohara , Takeo Kawase
发明人： Shigeo Kondo , Yasumasa Takeuchi , Yuji Shinohara , Takeo Kawase
IPC分类号： H01M6/18
CPC分类号： H01M4/62 , H01M2/021 , H01M2/0217 , H01M2/0222 , H01M4/0435 , H01M4/13 , H01M4/139 , H01M4/621 , H01M4/622 , H01M6/18 , H01M10/052 , H01M10/056 , H01M10/0562 , H01M10/0565 , H01M10/36 , H01M10/4235 , H01M10/4285 , H01M2220/30
摘要： An electrochemical device manufactured using an electrode layer in which severe increase of electrode resistance is prevented and/or a solid electrolyte layer in which severe decrease of ion conductivity of a solid electrolyte is prevented is provided. The electrochemical device includes a pair of electrode layers, and a solid electrolyte layer provided between the pair of electrode layers, wherein at least one layer of the electrode layers and the solid electrolyte layer is composed of first particles each providing a function of the at least one layer, second particles and a binder which is composed of an organic polymer and binds the first and second particles, and wherein the at least one layer is formed from a mixture material containing the first particles and binder particles, each of the binder particles including the second particle and the binder carried on at least a part of a surface thereof.

34. 发明申请

US20090087751A1 Solid electrolyte material of conducting lithium ion, battery device using the solid electrolyte material and all-solid lithium secondary battery provided with the battery device 有权
标题翻译：导电锂离子的固体电解质材料，使用固体电解质材料的电池装置和配有电池装置的全固态锂二次电池
公开(公告)号：US20090087751A1
公开(公告)日：2009-04-02
申请号：US12230767
申请日：2008-09-04
申请人： Shigeo Kondo , Yasumasa Takeuchi , Yuji Shinohara , Takeo Kawase
发明人： Shigeo Kondo , Yasumasa Takeuchi , Yuji Shinohara , Takeo Kawase
IPC分类号： H01M10/40 , H01M6/18
CPC分类号： H01M10/0562 , H01M6/18 , Y02E60/12 , Y02E60/122
摘要： A solid electrolyte material of conducting a lithium ion comprises a sulfide-based lithium-ion conductor and α-alumina. Such a solid electrolyte material exhibits superior lithium-ion conductivity. Further, a battery device provided with such a solid electrolyte material is also provided. Furthermore, an all-solid lithium-ion secondary battery provided with such a battery device is also provided.
摘要翻译：导电锂离子的固体电解质材料包括硫化物基锂离子导体和α-氧化铝。这种固体电解质材料表现出优异的锂离子传导性。此外，还提供了设置有这种固体电解质材料的电池装置。此外，还提供了具有这种电池装置的全固体锂离子二次电池。

35. 发明申请

US20080070113A1 Secondary battery and a method for manufacturing the secondary battery 有权
标题翻译：二次电池和二次电池的制造方法
公开(公告)号：US20080070113A1
公开(公告)日：2008-03-20
申请号：US11896054
申请日：2007-08-29
申请人： Shigeo Kondo , Yasumasa Takeuchi , Yoshiharu Ajiki
发明人： Shigeo Kondo , Yasumasa Takeuchi , Yoshiharu Ajiki
IPC分类号： H01M10/36 , B32B37/10
CPC分类号： H01M4/139 , B32B37/10 , B32B2457/10 , H01M4/0404 , H01M4/0414 , H01M4/13 , H01M4/70 , H01M4/78 , H01M10/0427 , H01M10/0436 , H01M10/052 , H01M10/0562 , H01M10/0585 , H01M2010/0495 , H01M2220/30 , H01M2300/0071 , H01M2300/0091 , Y02E60/122 , Y02P70/54
摘要： A secondary battery that can avoid reduction in battery capacity over the lapse of charge-discharge cycles and can exhibit high performance is provided. The secondary battery includes a first electrode layer, a second electrode layer, and an electrolyte layer provided between the first and second electrode layers, the electrolyte layer including electrolyte particles, wherein at least one of the first and second electrode layers includes a base member having a major surface on which a plurality of concave portions are formed and an electrode material filled in at least the concave portions, the major surface facing to the electrolyte layer.
摘要翻译：提供了能够避免在充放电循环过程中电池容量下降并且可以表现出高性能的二次电池。二次电池包括第一电极层，第二电极层和设置在第一和第二电极层之间的电解质层，电解质层包括电解质颗粒，其中第一和第二电极层中的至少一个包括具有其上形成有多个凹部的主表面和填充在至少凹部中的电极材料，主表面面向电解质层。

36. 发明授权

US5682261A Protonic conductor and electrochemical element using the same 失效
标题翻译：质子导体和电化学元素使用相同
公开(公告)号：US5682261A
公开(公告)日：1997-10-28
申请号：US583254
申请日：1996-01-05
申请人： Kazunori Takada , Shigeo Kondo , Tsutomu Minami , Masahiro Tatsumisago , Yasumasa Takeuchi
发明人： Kazunori Takada , Shigeo Kondo , Tsutomu Minami , Masahiro Tatsumisago , Yasumasa Takeuchi
IPC分类号： G02F1/15 , H01B1/06 , H01M6/18 , H01M8/02 , H01M8/10 , G02F1/00
CPC分类号： H01M8/1016 , G02F1/1523 , H01M6/185
摘要： A protonic conductor comprises a silicon oxide doped with a Br.o slashed.nsted acid and a thermoplastic elastomer. It has excellent protonic conductivity, which is not substantially lowered even in a dry atmosphere and thereby ensures excellent working properties.
摘要翻译：质子导体包括掺杂有Br + 526 nsted酸和热塑性弹性体的氧化硅。它具有优异的质子传导性，即使在干燥气氛中也不显着降低，从而确保优异的加工性能。

37. 发明授权

US4461883A Process for producing conjugated diene polymer using a solubilized lanthanum carboxylate catalyst 失效
标题翻译：使用溶解的镧羧酸盐催化剂制备共轭二烯聚合物的方法
公开(公告)号：US4461883A
公开(公告)日：1984-07-24
申请号：US387780
申请日：1982-06-14
申请人： Yasumasa Takeuchi , Mitsuhiko Sakakibara , Tooru Shibata
发明人： Yasumasa Takeuchi , Mitsuhiko Sakakibara , Tooru Shibata
IPC分类号： C08F2/06 , C08F4/12 , C08F4/14 , C08F4/44 , C08F36/04 , C08F4/52
CPC分类号： C08F36/04
摘要： A process for producing a conjugated diene polymer, characterized by polymerizing at least one conjugated diene with a catalyst consisting of (A) a reaction product of a Lewis base and a carboxylate of a rare earth element of the lanthanum series represented by Ln(R.sup.1 CO.sub.2).sub.3 wherein Ln is a rare earth element of the lanthanum series having an atomic number of 57 to 71 and R.sup.1 is a hydrocarbon substituent having 1 to 20 carbon atoms, (B) an organic aluminum compound represented by AlR.sup.2 R.sup.3 R.sup.4 wherein R.sup.2, R.sup.3 and R.sup.4, which may be identical or different, represent hydrogen atoms or hydrocarbon substituents having 1 to 8 carbon atoms, excluding the case where all of R.sup.2, R.sup.3 and R.sup.4 are hydrogen atoms at the same time, and (C) an (alkyl)aluminum halide represented by AlX.sub.n R.sup.5.sub.3-n wherein X is Cl, Br, F or I; R.sup.5 is a hydrocarbon substituent having 1 to 8 carbon atoms; and n has a value of 1, 1.5, 2 or 3, or consisting of these (A), (B) and (C) components and (D) a conjugated diene. A polymer obtained by said process has a high cis-1,4-configuration content and is excellent in physical properties of vulcanizate.
摘要翻译：一种共轭二烯聚合物的制备方法，其特征在于，将由（L）（R 1 CO 2）表示的镧系稀土元素的路易斯碱与羧酸酯的反应产物与（A） 3其中Ln是原子序数为57〜71的镧系稀土元素，R1为碳原子数1〜20的烃取代基，（B）由AlR2R3R4表示的有机铝化合物，其中R2，R3和R4，可以相同或不同，表示氢原子或具有1至8个碳原子的烃取代基，不包括所有R 2，R 3和R 4同时为氢原子的情况，（C）（烷基）卤化铝代表通过AlXnR53-n，其中X是Cl，Br，F或I; R5是具有1-8个碳原子的烃取代基; 并且n具有1,1.5,2或3的值，或由这些（A），（B）和（C）组分组成，和（D）共轭二烯。通过所述方法获得的聚合物具有高顺式-1,4-构型含量，并且硫化橡胶的物理性能优异。

38. 发明授权

US4182813A Process for the preparation of 1,2-polybutadiene 失效
标题翻译： 1,2-聚丁二烯的制备方法
公开(公告)号：US4182813A
公开(公告)日：1980-01-08
申请号：US905951
申请日：1978-05-15
申请人： Kenya Makino , Koei Komatsu , Yasumasa Takeuchi , Masayuki Endo
发明人： Kenya Makino , Koei Komatsu , Yasumasa Takeuchi , Masayuki Endo
IPC分类号： C08F4/00 , C08F4/30 , C08F4/60 , C08F4/70 , C08F36/00 , C08F136/06 , C08F4/80
CPC分类号： C08F136/06
摘要： A process for preparing crystalline 1,2-polybutadiene by contacting 1,3-butadiene with a catalyst consisting of (A) a cobalt compound, (B) an organoaluminum compound, (C) water in an amount of 0.25 to 1.5 mole per mol of said organoaluminum compound, and (D) an organic phosphorus compound in a halogenated hydrocarbon solvent to polymerize the butadiene, characterized in that as said organic phosphorus compound there is used a compound represented by the formula: ##STR1## wherein R.sup.1 is an alkyl or aryl group, and R.sup.2 and R.sup.3 represent independently hydrogen, or alkyl or aryl groups. This process can produce 1,2-polybutadiene having a degree of crystallization of 25 to 50% in a high yield at a temperature of from 0.degree. to 30.degree. C.
摘要翻译：通过使1,3-丁二烯与（A）钴化合物，（B）有机铝化合物，（C）每摩尔0.25至1.5摩尔的量的水组成的催化剂接触来制备结晶1,2-聚丁二烯的方法的所述有机铝化合物，和（D）在卤代烃溶剂中的有机磷化合物以使所述丁二烯聚合，其特征在于，作为所述有机磷化合物，使用由下式表示的化合物：其中R 1是烷基或芳基，R2和R3独立地表示氢或烷基或芳基。该方法可以在0〜30℃的温度下以高收率生产结晶度为25〜50％的1,2-聚丁二烯。

39. 发明授权

US3948667A Photosensitive compositions 失效
标题翻译：感光组合物
公开(公告)号：US3948667A
公开(公告)日：1976-04-06
申请号：US484982
申请日：1974-07-01
申请人： Mitsuo Ichikawa , Yasumasa Takeuchi , Takao Miura , Yoshiyuki Harita , Mitsuru Tashiro , Takahiro Tsunoda
发明人： Mitsuo Ichikawa , Yasumasa Takeuchi , Takao Miura , Yoshiyuki Harita , Mitsuru Tashiro , Takahiro Tsunoda
IPC分类号： C08C19/10 , G03F7/038 , G03C1/68
CPC分类号： G03F7/038 , C08C19/10 , Y10S430/12 , Y10S430/122 , Y10S430/126
摘要： Solvent-developed type photosensitive compositions containing as an essential ingredient at least one selected from the group of the cyclization product of butadiene polymer or copolymer and organic solvent, with or without at least one member selected from the group consisting of photosensitizer and photosensitive crosslinking agent, both soluble in an organic solvent.
摘要翻译：含有选自丁二烯聚合物或共聚物和有机溶剂的环化产物的组中的至少一种的溶剂显影型感光性组合物，含有或不含有选自光敏剂和光敏交联剂中的至少一种，均溶于有机溶剂。

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