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31. 发明申请

US20080293859A1 CURABLE FLUOROPOLYETHER COMPOSITION AND INTEGRAL MOLDED RESIN/RUBBER ARTICLES 有权
标题翻译：可固化氟聚乙烯组合物和一体成型树脂/橡胶制品
公开(公告)号：US20080293859A1
公开(公告)日：2008-11-27
申请号：US12124436
申请日：2008-05-21
申请人： Hiromasa Yamaguchi , Mikio Shiono
发明人： Hiromasa Yamaguchi , Mikio Shiono
IPC分类号： C08K5/541
CPC分类号： C08G65/007 , C08G65/336 , C08G77/12 , C08G77/24 , C08G2650/48 , C08L71/02 , C08L83/04 , C08L2205/02 , Y10T428/31663 , Y10T428/31786 , C08L83/00
摘要： Curable fluoropolyether compositions comprising (a) a polyfluorodialkenyl compound, (b) a fluorinated organohydrogenpolysiloxane, (c) a platinum catalyst, (d) hydrophobic silica powder, (e) a tackifier in the form of a specific silicon compound, and (f) an organosiloxane having a SiH group, an epoxy and/or trialkoxysilyl group, and a perfluoroalkyl or perfluoropolyether group cure to thermoplastic resins to form a durable tight bond at a low temperature within a short time and are readily releasable from metal molds.
摘要翻译：固化氟聚醚组合物，其包含（a）多氟二烯基化合物，（b）氟化有机氢聚硅氧烷，（c）铂催化剂，（d）疏水性二氧化硅粉末，（e）特定硅化合物形式的增粘剂，和（f）具有SiH基团，环氧基和/或三烷氧基甲硅烷基的有机硅氧烷和全氟烷基或全氟聚醚基固化成热塑性树脂，以在短时间内在低温下形成耐久的紧密结合，并且容易从金属模上释放。

32. 发明授权

US06624231B2 Fluorinated hydrosilylation-curable elastomer composition 失效
标题翻译：氟化氢化硅烷化固化弹性体组合物
公开(公告)号：US06624231B2
公开(公告)日：2003-09-23
申请号：US10046173
申请日：2002-01-16
申请人： Mikio Shiono
发明人： Mikio Shiono
IPC分类号： C08G7712
CPC分类号： C08L83/04 , C08G65/007 , C08G65/336 , C08G77/12 , C08G77/16 , C08G77/18 , C08G77/20 , C08G77/24 , C08K3/36 , C08K5/5406 , C08L83/14 , Y10T428/2995 , C08L83/08 , C08L2666/14 , C08L83/00
摘要： A curable composition comprising (A) a fluorinated amide compound having alkenyl radicals, (B) a fluorinated organohydrogensiloxane having SiH radicals, (C) a platinum group compound, (D) a silica powder, (E) an organosilane or organosiloxane having a monovalent perfluorooxyalkyl or perfluoroalkyl, divalent perfluorooxyalkylene or perfluoroalkylene radical and a hydroxy and/or alkoxy radical, and (F) an organosilane or organosiloxane having an alkenyl radical, a monovalent perfluorooxyalkyl or perfluoroalkyl, divalent perfluorooxyalkylene or perfluoroalkylene radical, and a hydroxy and/or alkoxy radical cures into a fluorinated elastomer that has good solvent resistance, chemical resistance, heat resistance, low-temperature properties, mold release, water and oil repellency and weather resistance as well as significantly improved mechanical strength and compression set.
摘要翻译：一种可固化组合物，其包含（A）具有烯基的氟化酰胺化合物，（B）具有SiH基团的氟化有机氢硅氧烷，（C）铂族化合物，（D）二氧化硅粉末，（E）有机硅烷或具有一价全氟氧烷基或全氟烷基，二价全氟氧化烯或全氟亚烷基和羟基和/或烷氧基，和（F）具有烯基，一价全氟氧烷基或全氟烷基，二价全氟氧化烯或全氟亚烷基的有机硅烷或有机硅氧烷，以及羟基和/或烷氧基自由基固化成耐溶剂性，耐化学性，耐热性，低温性，脱模性，拒水拒油性和耐候性以及显着改善的机械强度和压缩永久变形性的氟化弹性体。

33. 发明授权

US06576737B2 Curable compositions of fluorinated amide compounds 失效
标题翻译：氟化酰胺化合物的可固化组合物
公开(公告)号：US06576737B2
公开(公告)日：2003-06-10
申请号：US09969829
申请日：2001-10-04
申请人： Mikio Shiono , Takashi Matsuda , Masatoshi Arai
发明人： Mikio Shiono , Takashi Matsuda , Masatoshi Arai
IPC分类号： C08G7724
CPC分类号： C08L71/02 , C08G65/007 , C08L83/08 , C08L83/14 , C08L83/00
摘要： A curable composition comprising (A) a fluorinated amide compound having at least one alkenyl radical, (B) a fluorinated organohydrogensiloxane, (C) a platinum group compound, (D) a first organosiloxane having at least one SiH radical and at least one epoxy and/or trialkoxysilyl radical, and (E) a second organosiloxane having at least one SiH radical, at least one cyclic carboxylic anhydride residue, and at least one monovalent perfluorooxyalkyl or perfluoroalkyl radical cures into a fluorinated elastomer that not only has good solvent resistance, chemical resistance, heat resistance, low-temperature properties, low moisture permeability and electrical properties, but also firmly bonds to a variety of substrates including PPS, polyamide and polyimide resins.
摘要翻译：一种可固化组合物，其包含（A）具有至少一个烯基的氟化酰胺化合物，（B）氟化有机氢硅氧烷，（C）铂族化合物，（D）具有至少一个SiH基团和至少一个环氧基的第一有机硅氧烷和/或三烷氧基甲硅烷基，和（E）具有至少一个SiH基，至少一个环状羧酸酐残基和至少一个一价全氟氧烷基或全氟烷基的第二有机硅氧烷固化成不仅耐溶剂性良好的氟化弹性体，耐化学性，耐热性，低温性，低透湿性和电性能，而且牢固地粘合到各种基材，包括PPS，聚酰胺和聚酰亚胺树脂。

34. 发明授权

US5506302A Organopolysiloxane composition and rubber substrate having a coating thereof 失效
标题翻译：有机聚硅氧烷组合物和具有其涂层的橡胶基材
公开(公告)号：US5506302A
公开(公告)日：1996-04-09
申请号：US493154
申请日：1995-06-21
申请人： Mikio Shiono , Kazumi Okada , Hironao Fujiki
发明人： Mikio Shiono , Kazumi Okada , Hironao Fujiki
IPC分类号： C08K7/16 , C08K13/02 , C09D183/04 , C08K5/54
CPC分类号： C08K13/02 , C08K7/16 , C09D183/04
摘要： An organopolysiloxane composition contains (A) a both end hydroxyl-blocked diorganopoly-siloxane, (B) a hydroxyl-free diorganopoly-siloxane having a degree of polymerization equal to or greater than that of (A), (C) an organo-hydrogenpolysiloxane having at least three hydrogen atoms in a molecule, (D) an organosilane containing at least two alkoxy groups and an amino group attached to a silicon atom through an alkylene group in a molecule and/or a partial hydrolyzate thereof, (E) a fatty acid metal salt, (F) polycarbonate powder having a mean particle size of up to 50 .mu.m, and optionally (G) an organo-silane containing at least two alkoxy groups and a mercapto group attached to a silicon atom through an alkylene group in a molecule and/or a partial hydrolyzate thereof. It is applied to a rubber substrate to form a wear resistance coating thereon.
摘要翻译：有机聚硅氧烷组合物含有（A）双端羟基封端的二有机硅氧烷，（B）聚合度等于或大于（A）的聚合度的无羟基的二有机聚硅氧烷，（C）有机氢聚硅氧烷在分子中具有至少三个氢原子，（D）含有至少两个烷氧基的有机硅烷和通过分子中的亚烷基与硅原子连接的氨基和/或其部分水解产物，（E）脂肪酸性金属盐，（F）平均粒径达50μm的聚碳酸酯粉末，以及任选地（G）含有至少两个烷氧基的有机硅烷和通过亚烷基连接到硅原子上的巯基，分子和/或部分水解产物。将其施加到橡胶基材上以在其上形成耐磨性涂层。

35. 发明授权

US5064891A Curable silicone compositions 失效
标题翻译：可固化硅胶组合物
公开(公告)号：US5064891A
公开(公告)日：1991-11-12
申请号：US525047
申请日：1990-05-18
申请人： Hironao Fujiki , Mikio Shiono , Toshiaki Takahashi
发明人： Hironao Fujiki , Mikio Shiono , Toshiaki Takahashi
IPC分类号： A61K6/10 , C08L83/04 , C08L83/07 , G02B1/04
CPC分类号： A61K6/10 , C08L83/04 , G02B1/043 , C08G77/12 , C08G77/20 , C08G77/46 , Y10S524/912
摘要： A curable silicone composition comprising:(A) an organopolysiloxane having at least two silicon-bonded aliphatic unsaturated hydrocarbon radicals in its molecule;(B) an organohydrogenpolysiloxane having at least three silicon-bonded hydrogen atoms in its molecule;(C) a platinum family metal catalyst; and(D) a nonionic surface active agent having a hydrophobic silicone portion and at least one hydrophilic polyol portion in its molecule. The curable silicone composition gives cured products having good hydrophilic properties and dimensional stability, and are especially suitable for use as a dental impression material.

36. 发明授权

US08440777B2 Addition-cure fluoropolyether adhesive composition 有权
标题翻译：加成固化氟聚醚粘合剂组合物
公开(公告)号：US08440777B2
公开(公告)日：2013-05-14
申请号：US13007134
申请日：2011-01-14
申请人： Hidenori Koshikawa , Mikio Shiono
发明人： Hidenori Koshikawa , Mikio Shiono
IPC分类号： C08G77/42
CPC分类号： C09J171/02 , C08G65/007 , C08G77/12 , C08G77/14 , C08G77/18 , C08G77/24 , C08G2650/48 , C08K5/56 , C08L83/04
摘要： A fluoropolyether adhesive composition comprising (A) a linear polyfluoro compound having at least two alkenyl groups and a perfluoropolyether structure in its main chain, (B) a fluorinated organohydrogensiloxane containing at least two SiH groups, but not alkoxy and epoxy groups, (C) a platinum group metal-based catalyst, (D) an organosilicon compound having at least one silicon-bonded alkoxy group, and (E) a hydrolytic catalyst can be cured to metal and plastic substrates through addition reaction.
摘要翻译：一种氟聚醚粘合剂组合物，其包含（A）在其主链中具有至少两个烯基和全氟聚醚结构的线性多氟化合物，（B）含有至少两个SiH基但不包括烷氧基和环氧基的氟化有机氢硅氧烷，（C）铂族金属类催化剂，（D）具有至少一个与硅键合的烷氧基的有机硅化合物，（E）水解催化剂可以通过加成反应固化成金属和塑料基材。

37. 发明授权

US08314190B2 RT curable fluoropolyether base rubber composition and cured product 有权
标题翻译： RT固化氟聚醚基橡胶组合物和固化产物
公开(公告)号：US08314190B2
公开(公告)日：2012-11-20
申请号：US12874768
申请日：2010-09-02
申请人： Mitsuo Muto , Takashi Matsuda , Mikio Shiono
发明人： Mitsuo Muto , Takashi Matsuda , Mikio Shiono
IPC分类号： C08G77/00 , C08L83/00
CPC分类号： C08G65/007 , C08G2650/48 , C08L71/02 , C08L83/00
摘要： A fluoropolyether base rubber composition comprising (a) a linear fluoropolyether compound containing at least two ester groups in a molecule and a divalent perfluoroalkyl ether structure in its backbone, and having a Mn of 3,000-100,000, and (b) a siloxane polymer containing at least three amino groups in a molecule cures at room temperature into a product having heat resistance, low-temperature performance, chemical resistance, solvent resistance and oil resistance.
摘要翻译：一种含氟聚醚基橡胶组合物，其包含（a）在分子中含有至少两个酯基的直链含氟聚醚化合物和其主链中的二价全氟烷基醚结构，并且具有3,000-100,000的Mn，和（b）含有分子中至少三个氨基在室温下固化成具有耐热性，低温性能，耐化学性，耐溶剂性和耐油性的产品。

38. 发明申请

US20110257315A1 ADHESIVE COMPOSITION 有权
标题翻译：粘合剂组合物
公开(公告)号：US20110257315A1
公开(公告)日：2011-10-20
申请号：US13085510
申请日：2011-04-13
申请人： Mikio Shiono , Noriyuki Koike
发明人： Mikio Shiono , Noriyuki Koike
IPC分类号： C09J183/07 , C09J185/00 , C09J11/06
CPC分类号： C09D183/08 , C08G77/24 , C08L71/02
摘要： An adhesive composition is provided comprising (A) a fluorinated amide compound containing at least two vinyl groups and having a polyfluoro structure, (B) a fluorinated organosilicon compound containing a fluorinated organic group, at least two SiH groups, and an alkyl, aryl or aralkyl group, and (C) a platinum catalyst, and (D) an organosiloxane containing a SiH group and an epoxy and/or trialkoxysilyl group. The composition is cured on brief heating into a product which achieves adhesion to various substrates and has solvent resistance, chemical resistance, heat resistance, low-temperature properties, low moisture permeability, electric insulation, and acid resistance.
摘要翻译：提供一种粘合剂组合物，其包含（A）含有至少两个乙烯基并具有多氟结构的氟化酰胺化合物，（B）含氟化有机基团的氟化有机硅化合物，至少两个SiH基团和烷基，芳基或芳族烷基，（C）铂催化剂，（D）含有SiH基和环氧基和/或三烷氧基甲硅烷基的有机硅氧烷。该组合物在短暂加热下固化成实现对各种基材的粘合性的产品，并具有耐溶剂性，耐化学性，耐热性，低温性，低透湿性，电绝缘性和耐酸性。

39. 发明申请

US20080269389A1 Fluoropolyether adhesive composition 有权
标题翻译：氟聚醚粘合剂组合物
公开(公告)号：US20080269389A1
公开(公告)日：2008-10-30
申请号：US12081076
申请日：2008-04-10
申请人： Mikio Shiono
发明人： Mikio Shiono
IPC分类号： C08K3/36
CPC分类号： C09J171/02 , C08G65/007 , C08G65/336 , C08K5/541 , C08K5/5419 , C08L71/02 , C08L83/00 , C08L83/08 , C08L2666/14 , C09J183/08
摘要： An adhesive composition comprising the following components: (A) a linear polyfluoro compound having at least two SiH bonds per molecule and a perfluoropolyether residue in a main chain of the linear polyfluoro compound (A); (B) an organohydrogensiloxane having a fluorinated group and at least two hydrogen atoms each bonded to a silicon atom per molecule; (C) a compound of a platinum group metal; (D) hydrophobic silica powder; (E) an alkoxysilane represented by the following formula (1) (RO)3—Si-T (1) wherein R is a monovalent hydrocarbon group, T is a group represented by the formula, —OR1 or —CHR2—COOR3, wherein R1 is a monovalent hydrocarbon group, which may be the same with or different from R, R2 is a hydrogen atom or a methyl group and R3 is a monovalent hydrocarbon group; and (F) an organosiloxane having at least one SiH bond and at least one group selected from the group consisting of an epoxy group and a trialkoxysilyl group. The composition has no quality variation from lot to lot and gives a cured product having good resistance to solvents and heat, and durability.
摘要翻译：一种粘合剂组合物，其包含以下组分：（A）每分子具有至少两个SiH键的直链多氟化合物和所述直链多氟化合物（A）的主链中的全氟聚醚残基; （B）具有氟化基团和至少两个氢原子的有机氢硅氧烷，每个分子与硅原子键合; （C）铂族金属的化合物; （D）疏水性二氧化硅粉末; （E）由下式（1）表示的烷氧基硅烷<？in-line-formula description =“In-line Formulas”end =“lead”？>（RO）3 -Si-T （1）<？in-line-formula description =“In-line formula”end =“tail”？>其中R是一价烃基，T是由下式表示的基团：-OR 1 其中R 1是一价烃基，其可以与R相同或不同，R 1，R 2，R 3， R 2是氢原子或甲基，R 3是一价烃基; 和（F）具有至少一个SiH键的有机硅氧烷和至少一种选自环氧基和三烷氧基甲硅烷基的基团。该组合物从批次到批次之间没有质量差异，并且得到具有良好的耐溶剂性和耐热性和耐久性的固化产品。

40. 发明授权

US06846896B2 Curable compositions 失效
标题翻译：可固化组合物
公开(公告)号：US06846896B2
公开(公告)日：2005-01-25
申请号：US10690526
申请日：2003-10-23
申请人： Hiromasa Yamaguchi , Mikio Shiono
发明人： Hiromasa Yamaguchi , Mikio Shiono
IPC分类号： C08L71/00 , C08G65/336 , C08K5/541 , C08K9/06 , C08L23/28 , C08L43/04 , C08L71/02 , C08L83/05 , C08L83/08 , C09D143/04 , C09J4/06 , C09J143/00 , C08G77/24
CPC分类号： C08G65/336 , C08L23/28 , C08L43/04 , C08L71/02 , C08L83/08 , C08L2666/02 , C09D143/04 , C09J143/00
摘要： A curable composition comprising (A) a polyfluorodialkenyl compound having at least two alkenyl radicals, (B) a fluorinated organohydrogensiloxane having at least two Si—H radicals, (C) a platinum group compound, (D) a hydrophobic silica powder, and (E) an organosiloxane having a Si—H radical and a trialkyl or trialkoxy-containing organic radical attached to a silicon atom cures into a product having improved solvent resistance, chemical resistance, heat resistance, low-temperature properties, low moisture permeability and electric properties and exhibiting good adhesion to a variety of substrates including metals and plastics by brief heating at relatively low temperatures.
摘要翻译：一种可固化组合物，其包含（A）具有至少两个烯基的多氟二烯基化合物，（B）具有至少两个Si-H基团的氟化有机氢硅氧烷，（C）铂族化合物，（D）疏水性二氧化硅粉末和（ E）具有Si-H基团和连接到硅原子上的三烷基或三烷氧基的有机基团的有机硅氧烷固化成具有改善的耐溶剂性，耐化学性，耐热性，低温性能，低透湿性和电性能的产品并且通过在较低温度下的短时间加热对包括金属和塑料在内的各种基材表现出良好的粘合性。

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