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31. 发明申请

US20090005497A1 METHOD FOR PRODUCING CONJUGATED DIENE POLYMER, CONJUGATED DIENE POLYMER, AND POLYMER COMPOSITION 有权
标题翻译：生产聚合二烯聚合物，共轭二烯聚合物和聚合物组合物的方法
公开(公告)号：US20090005497A1
公开(公告)日：2009-01-01
申请号：US12140304
申请日：2008-06-17
申请人： Naoaki MAEDA , Mayumi Oshima , Katsunari Inagaki
发明人： Naoaki MAEDA , Mayumi Oshima , Katsunari Inagaki
IPC分类号： C08F36/14 , C08F2/60 , C08K3/36 , C08K3/04
CPC分类号： C08F36/04 , C08C19/44 , C08K3/013 , C08F4/48 , C08L15/00
摘要： A method for producing a conjugated diene polymer is provided that includes a step of polymerizing a conjugated diene-containing monomer in a hydrocarbon solvent in the presence of an alkali metal catalyst, thus giving a polymer having a catalyst-derived alkali metal at one terminus of a polymer chain comprising a conjugated diene-based monomer unit, and a step of reacting the polymer obtained in the step of polymerizing and a trialkoxysilane compound represented by the formula below. (In the formula, Y and Z independently denote an oxygen atom or a sulfur atom, R1, R2, and R3 independently denote an alkyl group having 1 to 4 carbon atoms, m denotes an integer of 1 to 5, and n denotes an integer of 0 to 5.) There are also provided a conjugated diene polymer produced by the production method, and a polymer composition containing a rubber component that includes the conjugated diene polymer and carbon black and/or silica, the total content of the carbon black and the silica being 5 to 200 parts by weight relative to 100 parts by weight of the rubber component.
摘要翻译：提供一种共轭二烯聚合物的制造方法，其包括在碱金属催化剂的存在下，在烃溶剂中使含共轭二烯的单体聚合的步骤，由此得到在一端具有催化剂衍生的碱金属的聚合物包含共轭二烯基单体单元的聚合物链和使聚合步骤中获得的聚合物与由下式表示的三烷氧基硅烷化合物反应的步骤。（式中，Y和Z分别独立地表示氧原子或硫原子，R1，R2，R3分别表示碳原子数1〜4的烷基，m表示1〜5的整数，n表示整数 0〜5）。还提供了通过制造方法制造的共轭二烯聚合物和含有包含共轭二烯聚合物和炭黑和/或二氧化硅的橡胶成分的聚合物组合物，二氧化硅相对于100重量份的橡胶组分为5〜200重量份。

32. 发明申请

US20090005496A1 METHOD FOR PRODUCING CONJUGATED DIENE POLYMER, CONJUGATED DIENE POLYMER, AND POLYMER COMPOSITION 有权
标题翻译：生产聚合二烯聚合物，共轭二烯聚合物和聚合物组合物的方法
公开(公告)号：US20090005496A1
公开(公告)日：2009-01-01
申请号：US12140301
申请日：2008-06-17
申请人： Naoaki MAEDA , Mayumi Oshima , Katsunari Inagaki
发明人： Naoaki MAEDA , Mayumi Oshima , Katsunari Inagaki
IPC分类号： C08F136/04 , C08F8/42 , C08K3/36 , C08K3/04
CPC分类号： C08F36/04 , C08C19/44 , C08K3/013 , C08F4/48 , C08L15/00
摘要： A method for producing a conjugated diene polymer is provided that includes a step of polymerizing a conjugated diene-containing monomer in a hydrocarbon solvent in the presence of an alkali metal catalyst, thus giving a polymer having a catalyst-derived alkali metal at one terminus of a polymer chain comprising a conjugated diene-based monomer unit, and a step of reacting the polymer obtained in the step of polymerizing and a trialkoxysilane compound represented by the formula below. (In the formula, M denotes an oxygen atom or a sulfur atom, R1, R2, and R3 independently denote an alkyl group having 1 to 4 carbon atoms, m denotes an integer of 1 to 5, and n denotes an integer of 0 to 5.) There are also provided a conjugated diene polymer produced by the production method, and a polymer composition containing a rubber component that includes the conjugated diene polymer and carbon black and/or silica, the total content of the carbon black and the silica being 5 to 200 parts by weight relative to 100 parts by weight of the rubber component.
摘要翻译：提供一种共轭二烯聚合物的制造方法，其包括在碱金属催化剂的存在下，在烃溶剂中使含共轭二烯的单体聚合的步骤，由此得到在一端具有催化剂衍生的碱金属的聚合物包含共轭二烯基单体单元的聚合物链和使聚合步骤中获得的聚合物与由下式表示的三烷氧基硅烷化合物反应的步骤。（式中，M表示氧原子或硫原子，R1，R2，R3分别表示碳原子数1〜4的烷基，m表示1〜5的整数，n表示0〜 5）还提供了通过制造方法制造的共轭二烯聚合物和含有共轭二烯聚合物和炭黑和/或二氧化硅的橡胶成分的聚合物组合物，炭黑和二氧化硅的总含量为相对于100重量份的橡胶组分为5〜200重量份。

33. 发明授权

US07339005B2 Process for producing modified diene polymer rubber 有权
标题翻译：生产改性二烯聚合物橡胶的方法
公开(公告)号：US07339005B2
公开(公告)日：2008-03-04
申请号：US10740670
申请日：2003-12-22
申请人： Mayumi Oshima , Seiichi Mabe , Katsunari Inagaki
发明人： Mayumi Oshima , Seiichi Mabe , Katsunari Inagaki
IPC分类号： C08C19/22 , C08C19/25 , C08F136/04 , C08F236/04
CPC分类号： C08C19/44 , C08F36/04 , C08F4/48
摘要： There is provided a process for producing a both end-modified diene polymer rubber comprising the steps of: (1) polymerizing a conjugated diene monomer or a combination thereof with an aromatic vinyl monomer in the presence of a compound represented by the following formula (1) to produce an alkali metal end-carrying active polymer, and (2) reacting the alkali metal end-carrying active polymer with an amine compound, a ketone compound, an acrylamide compound, a heterocyclic compound or a silyl compound represented by specific formulas, respectively: R—(CH2)n—X-M (1) wherein R is a functional group containing a substituent group-carrying nitrogen atom, X is a saturated or unsaturated hydrocarbon group comprising from 0 to 10 conjugated diene monomer units or aromatic vinyl monomer units, n is an integer of from 1 to 10, and M is an alkali metal.
摘要翻译：提供了两端改性二烯聚合物橡胶的制造方法，包括以下步骤：（1）在下式（1）表示的化合物存在下，将共轭二烯单体或其与芳族乙烯基单体的组合聚合）以制备碱金属末端活性聚合物，和（2）使碱金属末端活性聚合物与胺化合物，酮化合物，丙烯酰胺化合物，杂环化合物或由具体式表示的甲硅烷基化合物反应，分别为：<？in-line-formula description =“In-line Formulas”end =“lead”？> R-（CH 2）

34. 发明授权

US06469106B2 Process for producing modified diene polymer rubber 失效
标题翻译：生产改性二烯聚合物橡胶的方法
公开(公告)号：US06469106B2
公开(公告)日：2002-10-22
申请号：US09931770
申请日：2001-08-20
申请人： Katsunari Inagaki , Seiichi Mabe , Yoshihiro Nakatsuji
发明人： Katsunari Inagaki , Seiichi Mabe , Yoshihiro Nakatsuji
IPC分类号： C08F832
CPC分类号： C08C19/44
摘要： There is provided a process for producing a modified diene polymer rubber, which comprises the steps of: (i) polymerizing a conjugated diene compound, or a combination of a conjugated diene compound and an aromatic vinyl compound in a hydrocarbon solvent in the presence of an alkali metal catalyst, thereby obtaining an active conjugated diene polymer having an alkali metal at the end thereof, and (ii) reacting the active conjugated diene polymer having an alkali metal at the end thereof with an amine compound represented by the specific formula (1), thereby obtaining the modified diene polymer rubber.
摘要翻译：提供了一种制备改性二烯聚合物橡胶的方法，其包括以下步骤：（ⅰ）在烃溶剂中，在共聚二烯化合物或共轭二烯化合物碱金属催化剂，从而得到末端具有碱金属的活性共轭二烯聚合物，和（ii）使末端具有碱金属的活性共轭二烯聚合物与由具体式（1）表示的胺化合物反应，，得到改性二烯聚合物橡胶。

35. 发明授权

US5539050A Polyphenylene ether thermoplastic resin composition 失效
标题翻译：聚苯醚热塑性树脂组合物
公开(公告)号：US5539050A
公开(公告)日：1996-07-23
申请号：US328327
申请日：1994-10-24
申请人： Takeshi Fujii , Yuji Saga , Mitsuyoshi Odashima , Katsunari Inagaki
发明人： Takeshi Fujii , Yuji Saga , Mitsuyoshi Odashima , Katsunari Inagaki
IPC分类号： C08L25/04 , C08L51/00 , C08L51/06 , C08L51/08 , C08L59/00 , C08L61/00 , C08L67/00 , C08L69/00 , C08L71/00 , C08L71/12 , C08L77/00 , C08L81/02 , C08L85/00 , C08L23/16
CPC分类号： C08L51/06 , C08L71/123 , C08L59/00 , C08L61/00 , C08L67/00 , C08L69/00 , C08L77/00 , C08L81/02 , C08L85/00
摘要： A polyphenylene ether thermoplastic resin composition excellent in impact resistance, particularly surface impact strength, which comprises a blend of: 95 to 5 parts by weight of a mixture of:(A) 1 to 100% by weight of a polyphenylene ether resin and(B) 0 to 99% by weight of an alkenyl aromatic resin, with(C) 5 to 95 parts by weight of a graft copolymer obtained by graft-copolymerizing (a) an alkenyl aromatic compound and, if necessary, (b) other unsaturated monomer onto (c) an ethylene-.alpha.-olefin copolymer rubber having a ratio (Q value) of weight average molecular weight/number average molecular weight as measured by GPC of 4.0 or less and having a Mooney viscosity at 121.degree. C. of 40 or more, in which graft copolymer the weight ratio of (a) the alkenyl aromatic compound/(b) the other unsaturated monomer/(c) the ethylene-.alpha.-olefin copolymer rubber is 20-80/0-18.4/80-20 (the total of the component (a) and the component (c) is 100 parts by weight) and the weight ratio of the component (b)/(the component (a)+the component (b)) is 0.23 or less.
摘要翻译：一种抗冲击性，特别是表面冲击强度优异的聚苯醚热塑性树脂组合物，其包含以下混合物：95〜5重量份的：（A）1〜100重量％的聚苯醚树脂和（B ）0〜99重量％的烯基芳香族树脂，（C）5〜95重量份的接枝共聚物，其通过将（a）链烯基芳族化合物和（b）其它不饱和单体（c）通过GPC测定的重均分子量/数均分子量的比值（Q值）为4.0以下并且在121℃具有门尼粘度为40的乙烯-α-烯烃共聚橡胶或更多地，其中（a）烯基芳族化合物/（b）其它不饱和单体/（c）乙烯-α-烯烃共聚物橡胶的重量比为20-80 / 0-18.4 / 80-20（组分（a）和组分（c）的总量为100重量份）和重量比 e成分（b）/（成分（a）+成分（b））为0.23以下。

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