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21. 发明授权

US09051519B2 Diene-selective hydrogenation of metathesis derived olefins and unsaturated esters 有权
标题翻译：复分解衍生烯烃和不饱和酯的二烯选择性氢化
公开(公告)号：US09051519B2
公开(公告)日：2015-06-09
申请号：US13827153
申请日：2013-03-14
申请人： ELEVANCE RENEWABLE SCIENCES, INC.
发明人： Linda A. Kunz , Tessa M. Pals , Steven A. Cohen , Melvin L. Luetkens, Jr. , Chander Balakrishnan , Robert B. Snyder
IPC分类号： C07C1/00 , C07C6/02 , C07C5/05 , C10G3/00 , C11C3/12 , C10G29/20 , C10G45/00 , C10G45/58 , C10G50/00 , C10G65/04 , C10G69/12 , C11B3/00 , C10L1/02 , C10L1/08 , C11C3/00 , C11C3/10 , C07C6/04 , C07C1/213 , C07C5/03 , C07C7/13
CPC分类号： C11C3/126 , C07C1/213 , C07C5/03 , C07C5/05 , C07C6/04 , C07C7/13 , C07C2523/28 , C07C2523/42 , C07C2523/44 , C07C2523/46 , C07C2523/72 , C07C2523/745 , C07C2523/755 , C10G3/42 , C10G3/44 , C10G3/50 , C10G29/205 , C10G45/00 , C10G45/58 , C10G50/00 , C10G65/043 , C10G69/123 , C10G2300/1014 , C10G2300/1018 , C10G2300/1088 , C10G2300/30 , C10G2400/02 , C10G2400/04 , C10G2400/08 , C10G2400/20 , C10G2400/22 , C10L1/00 , C10L1/026 , C10L1/08 , C10L2200/0469 , C10L2200/0476 , C11B3/00 , C11C3/003 , C11C3/10 , C11C3/12 , C11C3/123 , Y02P20/582 , Y02P30/20 , C07C11/02 , C07C11/12 , C07C9/14 , C07C9/22 , C07C11/21
摘要： Methods are provided for refining natural oil feedstocks and partially hydrogenating polyunsaturated olefins and polyunsaturated esters. The methods comprise reacting the feedstock in the presence of a metathesis catalyst under conditions sufficient to form a metathesized product comprising olefins and esters. In certain embodiments, the methods further comprise separating the polyunsaturated olefins from the polyunsaturated esters in the metathesized product. In certain embodiments, the methods further comprise partially hydrogenating the polyunsaturated olefins in the presence of a hydrogenation catalyst, wherein at least a portion of the polyunsaturated olefins are converted to monounsaturated olefins. In other embodiments, the methods further comprise partially hydrogenating the polyunsaturated esters in the presence of a hydrogenation catalyst, wherein at least a portion of the polyunsaturated esters are converted to monounsaturated esters.
摘要翻译：提供了用于澄清天然油原料和部分氢化多不饱和烯烃和多不饱和酯的方法。所述方法包括在复分解催化剂存在下，在足以形成包含烯烃和酯的复分解产物的条件下使原料反应。在某些实施方案中，所述方法还包括从所述多元不饱和酯中分离所述多不饱和烯烃。在某些实施方案中，所述方法还包括在氢化催化剂存在下部分氢化多不饱和烯烃，其中至少一部分多不饱和烯烃转化为单不饱和烯烃。在其它实施方案中，所述方法还包括在氢化催化剂存在下部分氢化多不饱和酯，其中至少一部分多不饱和酯转化为单不饱和酯。

22. 发明授权

US08729283B2 Chain-selective synthesis of fuel components and chemical feedstocks 有权
标题翻译：燃料组分和化学原料的链选择性合成
公开(公告)号：US08729283B2
公开(公告)日：2014-05-20
申请号：US13741965
申请日：2013-01-15
申请人： Energy & Environmental Research Center Foundation
发明人： Edwin S. Olson
IPC分类号： C07C51/36 , C07C6/02
CPC分类号： C07C2/862 , C07C6/04 , C07C29/145 , C07C67/03 , C07C2601/14 , C11C3/00 , C12P7/6445 , Y02E50/13 , Y02T50/678 , C07C13/23 , C07C31/276 , C07C69/533
摘要： A method comprising providing a starting composition comprising a polyunsaturated fatty acid, a polyunsaturated fatty ester, a carboxylate salt of a polyunsaturated fatty acid, a polyunsaturated triglyceride, or a mixture thereof; self-metathesizing the starting composition or cross-metathesizing the starting composition with at least one short-chain olefin in the presence of a metathesis catalyst to form self-/cross-metathesis products comprising: cyclohexadiene; at least one olefin; and one or more acid-, ester-, or salt-functionalized alkene; and reacting cyclohexadiene to produce at least one cycloalkane or cycloalkane derivatives. A method for producing cycloalkanes for jet fuel by providing a starting composition comprising at least one selected from the group consisting of algal and polyunsaturated vegetable oils, subjecting the starting composition to metathesis to produce metathesis product comprising at least one olefin, cyclohexadiene, and at least one acid-, ester-, or salt-functionalized alkene, and reacting the at least one olefin and cyclohexadiene to form cycloalkane(s).
摘要翻译：一种包括提供包含多不饱和脂肪酸，多不饱和脂肪酯，多不饱和脂肪酸的羧酸盐，多不饱和甘油三酸酯或其混合物的起始组合物的方法; 在复分解催化剂的存在下，使起始组合物自分化或用至少一种短链烯烃交联混合以形成自交联/交叉复分解产物，其包含：环己二烯; 至少一种烯烃; 和一种或多种酸，酯或盐官能化的烯烃; 并使环己二烯反应生成至少一种环烷烃或环烷烃衍生物。一种通过提供包含选自藻类和多不饱和植物油中的至少一种的起始组合物来制备用于喷气燃料的环烷烃的方法，使起始组合物进行复分解以产生包含至少一种烯烃，环己二烯和至少包含至少一种烯烃的复分解产物一种酸，酯或盐官能化的烯烃，并使所述至少一种烯烃和环己二烯反应形成环烷烃。

23. 发明授权

US08552242B2 Efficient methods for Z- or cis-selective cross-metathesis 有权
公开(公告)号：US08552242B2
公开(公告)日：2013-10-08
申请号：US13023400
申请日：2011-02-08
申请人： Amir H. Hoveyda , Simon J. Meek , Robert V. O'Brien , Josep Llaveria Cros , Richard R. Schrock
发明人： Amir H. Hoveyda , Simon J. Meek , Robert V. O'Brien , Josep Llaveria Cros , Richard R. Schrock
IPC分类号： C07C6/04 , C07C6/02
摘要： The present invention generally relates to methods for performing metathesis reactions, including cross-metathesis reactions. Methods described herein exhibit enhanced activity and stereoselectivity, relative to known methods, and are useful in the synthesis of a large assortment of biologically and therapeutically significant agents.

24. 发明申请

US20100145126A1 Process of Producing Olefins 失效
标题翻译：生产烯烃的工艺
公开(公告)号：US20100145126A1
公开(公告)日：2010-06-10
申请号：US11883540
申请日：2006-02-24
申请人： Toshihiro Takai , Takeshi Kubota
发明人： Toshihiro Takai , Takeshi Kubota
IPC分类号： C07C6/02
CPC分类号： C07C6/04 , C07C2523/30 , Y02P20/52 , C07C11/06 , C07C11/02
摘要： A process of producing olefins by a metathesis reaction in a practical low temperature range by improving the reactivity of the catalyst is provided.The process of producing olefins according to the present invention allows a metathesis reaction of olefins, which uses a catalyst containing metal elements such as tungsten, molybdenum, rhenium or the like, to proceed at an industrially sufficient reaction rate in a practical low temperature range, by using a compound containing at least one metal element selected from the metals of Group Ia (alkali metals), Group IIa (alkaline earth metals), Group IIb and Group IIIa as co-catalyst and allowing hydrogen gas to co-exist with the reaction raw material.
摘要翻译：提供了通过提高催化剂的反应性在实际的低温范围内通过复分解反应制备烯烃的方法。根据本发明的烯烃的制造方法允许使用含有金属元素如钨，钼，铼等的催化剂在实际的低温范围内以工业上足够的反应速率进行的烯烃的复分解反应，通过使用含有选自Ia族金属（碱金属），IIa族（碱土金属），IIb族和IIIa族金属中的至少一种金属元素作为助催化剂并使氢气与反应共存的化合物原材料。

25. 发明授权

US07525007B2 Production of propylene from steam cracking of hydrocarbons, particularly ethane 有权
标题翻译：从烃类特别是乙烷的蒸汽裂解生产丙烯
公开(公告)号：US07525007B2
公开(公告)日：2009-04-28
申请号：US11703498
申请日：2007-02-07
申请人： Charles Sumner
发明人： Charles Sumner
IPC分类号： C07C6/02
CPC分类号： C10G9/06 , C07C6/04 , C07C11/06 , Y02P30/44
摘要： An ethane or other hydrocarbon feedstock is steam cracked to produce an ethylene stream which is processed in an ethylene plant recovery section to separate an ethane recycle and a polymer grade or chemical grade ethylene product stream. A portion of the ethylene product stream may then be reacted by dimerization to produce a butene stream. These formed butenes and/or butenes recovered from other sources and another portion of the ethylene product stream are reacted by metathesis to produce a propylene stream which is deethanized and separated from heavier hydrocarbons to produce the propylene product. The butene product stream may also be deethanized and is separated from heavier hydrocarbons. The overhead from the metathesis section deethanizer may be recycled to the ethylene plant recovery section. The reflux for the metathesis section deethanizer may be generated from the overhead or may be a portion of the ethylene product stream.
摘要翻译：乙烷或其他烃原料蒸汽裂化以产生乙烯料流，其在乙烯装置回收段中加工以分离乙烷再循环和聚合物级或化学级乙烯产物流。然后可以通过二聚反应将一部分乙烯产物流反应以产生丁烯流。从其他来源回收的这些形成的丁烯和/或丁烯和乙烯产物流的另一部分通过复分解反应以产生丙烯料流，该丙烯料流与较重的烃脱乙基化并分离以产生丙烯产物。丁烯产物流也可以脱乙烷并与较重的烃分离。来自复分解段脱乙烷器的塔顶馏出物可以再循环到乙烯装置回收部分。复分解段脱乙烷器的回流可以从塔顶产生，也可以是乙烯产物流的一部分。

26. 发明授权

US07371917B2 Preparation of olefins by metathesis over a carbide or oxycarbide of a transition metal 失效
标题翻译：通过在过渡金属的碳化物或碳氧化物上复分解制备烯烃
公开(公告)号：US07371917B2
公开(公告)日：2008-05-13
申请号：US10811940
申请日：2004-03-30
申请人： Markus Schubert , Till Gerlach , Michael Hesse , Juergen Stephan , Volker Boehm , Andreas Brodhagen , Frank Poplow
发明人： Markus Schubert , Till Gerlach , Michael Hesse , Juergen Stephan , Volker Boehm , Andreas Brodhagen , Frank Poplow
IPC分类号： C07C6/02
CPC分类号： C07C6/04 , B01J21/08 , B01J23/30 , B01J27/22 , C07C2521/04 , C07C2521/06 , C07C2521/08 , C07C2521/12 , C07C2523/08 , C07C2523/14 , C07C2527/22
摘要： Process for preparing a compound having a nonaromatic C—C double or triple bond (compound A) from another compound or a mixture of other compounds having a nonaromatic C—C double or triple bond (compound B), which comprises bringing the compound (B) into contact with a heterogeneous catalyst comprising carbides or oxycarbides of a transition element at from 50 to 500° C.
摘要翻译：制备具有非芳族CC双键或三键（化合物B）的其它化合物或其它化合物的混合物的具有非芳族CC双键或三键的化合物（化合物A）的方法（化合物B），其包括使化合物（B）与包含50-500℃的过渡元素的碳化物或碳氧化物的多相催化剂

27. 发明授权

US07041861B2 Olefin metathesis 有权
标题翻译：烯烃复分解
公开(公告)号：US07041861B2
公开(公告)日：2006-05-09
申请号：US10431186
申请日：2003-05-07
申请人： Gary G. Podrebarac
发明人： Gary G. Podrebarac
IPC分类号： C07C6/04 , C07C6/02
CPC分类号： C07C11/107 , C07C6/04 , C07C11/02 , C07C11/06 , C07C11/10 , C07C2523/28 , C07C2523/36 , C07C2523/75 , Y02P20/127 , Y10S203/06
摘要： A process in which neohexene is produced by starting with butene in a distillation column reactor to produce a product containing ethylene, diisobutene, heavier oligomers. After separating these components, the separated diisobutene is further reacted with ethylene produced from the first step to produce neohexene.
摘要翻译：通过在蒸馏塔反应器中由丁烯开始生产新己烯的方法，以制备含有乙烯，二异丁烯，较重的低聚物的产物。在分离这些组分后，分离的二异丁烯进一步与由第一步产生的乙烯反应以产生新己烯。

28. 发明授权

US6166279A Preparation of olefins 失效
标题翻译：烯烃的制备
公开(公告)号：US6166279A
公开(公告)日：2000-12-26
申请号：US275784
申请日：1999-03-25
申请人： Peter Schwab , Ralf Schulz , Michael Schulz , Boris Breitscheidel , Gerald Meyer
发明人： Peter Schwab , Ralf Schulz , Michael Schulz , Boris Breitscheidel , Gerald Meyer
IPC分类号： B01J23/36 , C07B61/00 , C07C6/02 , C07C7/163 , C07C11/06 , C07C41/06 , C10G35/06 , C07C1/00 , C07C6/00
CPC分类号： B01D3/141 , C07C7/163 , C07C11/06 , C07C41/06 , C07C2521/04 , C07C2523/36 , C07C2523/42 , C07C2523/44 , C07C2523/755 , Y02P20/52 , C07C43/04
摘要： The preparation of olefins from steam cracker or refinery C.sub.4 streams is carried out by selective hydrogenation of butadienes and acetylenic impurities in the steam cracker or refinery C.sub.4 stream, with simultaneous or subsequent, at least partial isomerization of 1-butene to 2-butene, followed by removal of i-butene from the C.sub.4 stream by reaction with an alcohol to form an ether, followed by removal of oxygen-containing impurities from the C.sub.4 stream using adsorber materials, followed by two-stage metathesis of the butenes in the C.sub.4 stream by conversion of 1-butene and 2-butene present in the C.sub.4 stream into propene and 2-pentene and subsequent reaction of the 2-pentene with ethene in the presence of a metathesis catalyst to form propene and 1-butene. Optionally, butadiene may be removed from the C.sub.4 stream by extractive distillation in a preliminary step.
摘要翻译：通过蒸汽裂解装置或炼油厂C4流中的丁二烯和炔属杂质的选择性氢化来进行来自蒸汽裂解装置或炼油厂C4流的烯烃的制备，其中1-丁烯与2-丁烯的同时或随后至少部分异构化，随后通过与醇反应从C4流中除去1-丁烯以形成醚，然后使用吸附材料从C4流中除去含氧杂质，随后通过C4流中的丁烯的两步复分解将C4流中存在的1-丁烯和2-丁烯转化为丙烯和2-戊烯，随后在复分解催化剂存在下2-戊烯与乙烯的反应形成丙烯和1-丁烯。任选地，可以在预备步骤中通过萃取蒸馏从C4流中除去丁二烯。

29. 发明授权

US5932777A Hydrocarbon conversion 失效
标题翻译：烃转化
公开(公告)号：US5932777A
公开(公告)日：1999-08-03
申请号：US899219
申请日：1997-07-23
申请人： Edward L. Sughrue, II , Charles A. Drake , Scott D. Love
发明人： Edward L. Sughrue, II , Charles A. Drake , Scott D. Love
IPC分类号： C07C6/02 , C07C6/08 , C10G9/00 , C10G35/095 , C10G59/00 , C10G61/00 , C10G61/02 , C10G61/04 , C10G63/00 , C10G63/02 , C10G63/04 , C10G67/00 , C10L1/06 , C07C1/00
CPC分类号： C10G67/00 , C10G61/00 , C10G61/02 , C10G61/04 , C10G63/00 , C10G63/02
摘要： A hydrocarbon conversion process comprises: (1) contacting a hydrocarbon feed such as, for example, gasoline, with a catalyst under a sufficient condition to effect the conversion of the hydrocarbon to a product stream comprising aromatic hydrocarbons and olefins; (2) separating the product stream into a lights fraction comprising primarily hydrocarbons less than 6 carbon atoms per molecule, a middle fraction comprising C.sub.6 -C.sub.8 aromatic hydrocarbons and non-aromatic hydrocarbons, and a C.sub.9 + fraction comprising aromatic compounds; (3) separating the C.sub.6 -C.sub.8 aromatic hydrocarbons from the middle fraction; and (4) separating hydrocarbons containing 5 or more carbons per molecule (C.sub.5 + hydrocarbons) from the lights fraction. The C.sub.5 + hydrocarbons can be combined with the hydrocarbon feed. The non-aromatic hydrocarbons can also be converted to olefins by a thermal cracking process. Furthermore, the middle fraction can also be obtained by reforming naphtha.
摘要翻译：烃转化方法包括：（1）在足够的条件下使烃进料例如汽油与催化剂接触，以使烃转化为包含芳族烃和烯烃的产物流; （2）将产物流分离成每分子主要包含少于6个碳原子的烃的轻馏分，包含C 6 -C 8芳族烃和非芳族烃的中间馏分和包含芳族化合物的C 9+馏分; （3）从中间馏分中分离C6-C8芳烃; 和（4）从轻馏分中分离每分子含有5个或更多个碳的碳（C5 +烃）。 C5 +烃可与烃进料组合。非芳族烃也可以通过热裂解过程转化为烯烃。此外，也可以通过重整石脑油获得中间馏分。

30. 发明授权

US4522936A Metathesis catalyst 失效
标题翻译：复分解催化剂
公开(公告)号：US4522936A
公开(公告)日：1985-06-11
申请号：US611785
申请日：1984-05-18
申请人： Simon G. Kukes , Robert L. Banks
发明人： Simon G. Kukes , Robert L. Banks
IPC分类号： B01J23/24 , C07C6/02 , C07C6/04 , B01J23/18
CPC分类号： C07C6/02 , B01J23/24 , C07C6/04
摘要： A supported tungsten oxide or supported molybdenum oxide is treated with elemental tungsten, silicon or antimony. The composition is useful as a metathesis catalyst.
摘要翻译：用元素钨，硅或锑处理负载的氧化钨或负载的氧化钼。该组合物可用作复分解催化剂。

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