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21. 发明授权

US06825310B2 Halogenated aromatic compound, polymer thereof, and proton-conductive membrane comprising same 有权
标题翻译：卤化芳族化合物，其聚合物和包含其的质子传导膜
公开(公告)号：US06825310B2
公开(公告)日：2004-11-30
申请号：US10105213
申请日：2002-03-26
申请人： Kohei Goto , Masayuki Takahashi , Yoshitaka Yamakawa , Makoto Higami
发明人： Kohei Goto , Masayuki Takahashi , Yoshitaka Yamakawa , Makoto Higami
IPC分类号： C08G6538
CPC分类号： H01B1/122 , C07C45/71 , C07C49/84 , C07C317/22 , C08G61/12 , C08G65/40 , C08G65/4018 , C08G65/4025 , C08G75/23 , C08J5/2256 , C08J2381/06 , H01M6/181 , H01M2300/0082
摘要： A polymer which has a flexible structure in its main chain and thus exhibits a high toughness and can difficultly be deteriorated in its mechanical properties and thermal properties even when sulfonated, a sulfonic acid group-containing polymer obtained by the sulfonation of the polymer, and a proton-conductive membrane having an excellent mechanical strength and durability made of the sulfonic acid group-containing polymer. A novel halogenated aromatic compound represented by the following general formula (1m) is provided: wherein A independently represents an electron-withdrawing group; B independently represents an electron-donating atom or group; X represents a chlorine atom, iodine atom or bromine atom; R1 to R8 may be the same or different and each represent a hydrogen atom, fluorine atom or alkyl group; and n represents an integer of 2 or more.
摘要翻译：一种聚合物，其主链具有柔性结构，因此即使在磺化时也显示出高的韧性并且难以在其机械性能和热性能上劣化，通过聚合物磺化得到的含磺酸基的聚合物和质子传导膜具有优异的机械强度和耐久性，由含磺酸基的聚合物制成。提供由以下通式（1m）表示的新型卤代芳族化合物：其中A独立地表示吸电子基团; B独立地表示给电子原子或基团; X表示氯原子，碘原子或溴原子; R 1至R 8可以相同或不同，各自表示氢原子，氟原子或烷基; n表示2以上的整数。

22. 发明授权

US06812290B2 Polyarylene copolymers and proton-conductive membrane 有权
标题翻译：聚亚芳基共聚物和质子传导膜
公开(公告)号：US06812290B2
公开(公告)日：2004-11-02
申请号：US10303821
申请日：2002-11-26
申请人： Kohei Goto , Yoshitaka Yamakawa , Mayumi Kakuta , Igor Rozhanskii
发明人： Kohei Goto , Yoshitaka Yamakawa , Mayumi Kakuta , Igor Rozhanskii
IPC分类号： C08F836
CPC分类号： C08G61/12 , C07C45/46 , C07C49/84
摘要： A polyarylene copolymer which comprises (A) aromatic compound units having a main chain containing one or more electron-withdrawing groups therein and (B) aromatic compound units having a main chain containing no electron-withdrawing groups therein, and a proton-conductive membrane comprising the polyarylene copolymer having sulfonic acid groups.
摘要翻译：一种聚亚芳基共聚物，其包含（A）具有含有一个或多个吸电子基团的主链的芳香族化合物单元和（B）具有不含吸电子基团的主链的芳香族化合物单元，以及质子传导性膜，所述聚亚芳基共聚物具有磺酸基。

23. 发明申请

US20090149625A1 AROMATIC COMPOUND HAVING FLUORENE SKELETON AND POLYARYLENE HAVING SULFONIC ACID GROUP 审中-公开
标题翻译：具有荧光素的芳香族化合物和具有亚磺酸的聚合物
公开(公告)号：US20090149625A1
公开(公告)日：2009-06-11
申请号：US12298443
申请日：2007-04-24
申请人： Yoshitaka Yamakawa , Yousuke Konno , Kohei Goto
发明人： Yoshitaka Yamakawa , Yousuke Konno , Kohei Goto
IPC分类号： C08G14/00 , C07C317/14
CPC分类号： H01B1/122 , C08G65/4012 , H01M8/1025 , H01M8/1027 , H01M8/103 , H01M8/1032 , H01M8/1039
摘要： Sulfonated polyarylenes have excellent processability and methanol resistance.The polyarylene includes a structural unit (S) represented by Formula (2-2) below and a structural unit (T) represented by Formula (2-3) below, the structural unit (S) accounting for a proportion “s” of 95 to 50 mol %, the structural unit (T) accounting for a proportion “t” of 5 to 50 mol % (“s”+“t”=100 mol %): wherein each A independently represents a divalent linking group represented by —CO— or —SO2—; and R1 to R4 each independently represent a hydrogen atom, a fluorine atom, an alkyl group or an aryl group.
摘要翻译：磺化聚亚芳基具有优异的加工性和耐甲醇性。聚亚芳基包括由下式（2-2）表示的结构单元（S）和由下式（2-3）表示的结构单元（T），结构单元（S）占比例“s”为95 至50摩尔％，结构单元（T）的比例“t”为5-50摩尔％（“s”+“t”= 100摩尔％））：其中每个A独立地表示由 - CO-或-SO 2 - ; R 1〜R 4各自独立地表示氢原子，氟原子，烷基或芳基。

24. 发明授权

US06555626B2 Polyarylene copolymers and proton-conductive membrane 有权
标题翻译：聚亚芳基共聚物和质子传导膜
公开(公告)号：US06555626B2
公开(公告)日：2003-04-29
申请号：US09818847
申请日：2001-03-28
申请人： Kohei Goto , Yoshitaka Yamakawa , Mayumi Kakuta , Igor Rozhanskii
发明人： Kohei Goto , Yoshitaka Yamakawa , Mayumi Kakuta , Igor Rozhanskii
IPC分类号： C08F836
CPC分类号： C08G61/12 , C07C45/46 , C07C49/84
摘要： A polyarylene copolymer which comprises (A) from 60 to 3 mol % aromatic compound units having a main chain containing one or more electron-withdrawing groups therein and (B) from 40 to 97 mol % aromatic compound units having a main chain containing no electron-withdrawing groups therein (provided that (A)+(B)=100 mol %), and a proton-conductive membrane comprising the polyarylene copolymer having sulfonic acid groups.
摘要翻译：一种聚亚芳基共聚物，其包含（A）60〜3摩尔％的含有一个或多个吸电子基团的主链的芳族化合物单元和（B）40〜97摩尔％的不含电子的主链的芳族化合物单元（A）+（B）= 100摩尔％）和包含具有磺酸基的聚亚芳基共聚物的质子传导膜。

25. 发明授权

US5527860A Process for producing a diolefin polymer or copolymer and a rubber composition containing such a diolefin polymer or copolymer 失效
标题翻译：制备二烯烃聚合物或共聚物的方法和含有这种二烯烃聚合物或共聚物的橡胶组合物
公开(公告)号：US5527860A
公开(公告)日：1996-06-18
申请号：US184217
申请日：1994-01-21
申请人： Yoshitaka Yamakawa , Kyouyuu Yasuda , Iwakazu Hattori , Hideaki Yokoyama , Tatsuro Hamada
发明人： Yoshitaka Yamakawa , Kyouyuu Yasuda , Iwakazu Hattori , Hideaki Yokoyama , Tatsuro Hamada
IPC分类号： C08F4/08 , C08F4/48 , C08F36/04 , C08F8/42
CPC分类号： C08F36/04
摘要： A process for producing a diolefin polymer or copolymer, comprising the steps of polymerizing 55-100 wt % of a conjugated diolefin with 0-45 wt % of an aromatic vinyl compound as monomers in a hydrocarbon as a solvent, by using initiators: a reaction product [a1] between at least one secondary amine compound (A) and an organic lithium compound and/or a lithium amide compound [a2] of the at least one secondary amine compound (A) as well as a reaction product [b1] between at least one alcohol (B) and an organic lithium compound and/or a lithium alkoxide compound of the at least one alcohol (B). A rubber composition containing not less than 30 wt % of such a diolefin polymer or copolymer with respect to an entire rubber component is also disclosed. This rubber composition exhibits excellent abrasion resistance, high tensile strength, steering stability and low rolling resistance, and is suitable for tires, particularly, as treads of low fuel consumption tires.
摘要翻译：一种制备二烯烃聚合物或共聚物的方法，包括以下步骤：通过使用引发剂将55-100重量％的共轭二烯烃与0-45重量％的芳族乙烯基化合物作为单体在烃中作为溶剂聚合：反应至少一种仲胺化合物（A）的至少一种仲胺化合物（A）和有机锂化合物和/或氨化锂化合物[a2]之间的产物[a1]以及至少一种仲胺化合物（A）的反应产物[b1] 至少一种醇（B）和至少一种醇（B）的有机锂化合物和/或醇锂化合物。还公开了相对于整个橡胶组分含有不少于30重量％的这种二烯烃聚合物或共聚物的橡胶组合物。该橡胶组合物表现出优异的耐磨性，高拉伸强度，操纵稳定性和低滚动阻力，并且适用于轮胎，特别是作为低燃料轮胎的胎面。

26. 发明授权

US07893303B2 Polyarylene, process for producing the same, solid polyelectrolyte, and proton-conductive film 有权
标题翻译：聚亚芳基，其制备方法，固体聚电解质和质子传导膜
公开(公告)号：US07893303B2
公开(公告)日：2011-02-22
申请号：US11815370
申请日：2005-02-04
申请人： Yoshitaka Yamakawa , Makoto Higami
发明人： Yoshitaka Yamakawa , Makoto Higami
IPC分类号： C07C315/00
CPC分类号： C08G61/02 , C08G61/12 , C08J5/18 , C08J2365/02 , H01B1/122
摘要： A polyarylene having a structural unit shown by the following formula (1) is disclosed. wherein X and Y indicate a divalent organic group or a single bond, Z shows an oxygen atom or a sulfur atom, R represents at least one atom or group selected from the group consisting of a hydrogen atom, a fluorine atom, an alkyl group, and a fluorine-substituted alkyl group, a is an integer of 1 to 20, n is an integer of 1 to 5, and p is an integer of 0 to 10.
摘要翻译：公开了具有下述通式（1）所示的结构单元的聚亚芳基。其中X和Y表示二价有机基团或单键，Z表示氧原子或硫原子，R表示至少一个选自氢原子，氟原子，烷基，氟取代烷基，a为1〜20的整数，n为1〜5的整数，p为0〜10的整数。

27. 发明申请

US20090149623A1 NITROGENATED AROMATIC COMPOUND, PROCESS FOR PRODUCTION OF THE SAME, POLYMER, AND PROTON CONDUCTIVE MEMBRANE 有权
标题翻译：硝基芳族化合物，其制备方法，聚合物和导电膜
公开(公告)号：US20090149623A1
公开(公告)日：2009-06-11
申请号：US11995793
申请日：2006-06-30
申请人： Makoto Higami , Igor Rozhanskii , Yoshitaka Yamakawa
发明人： Makoto Higami , Igor Rozhanskii , Yoshitaka Yamakawa
IPC分类号： C08G8/02 , C07D233/64 , C07D277/74
CPC分类号： H01M10/0565 , C07C49/84 , C07D207/325 , C07D209/08 , C07D209/86 , C07D213/643 , C07D213/65 , C07D213/68 , C07D215/233 , C07D231/12 , C07D233/60 , C07D235/18 , C07D239/32 , C07D239/34 , C07D249/08 , C07D257/04 , C07D263/57 , C07D277/36 , C07D277/66 , C07D277/74 , C08G61/02 , C08G61/10 , C08G61/12 , C08G73/028 , C08G2261/126 , C08G2261/1424 , C08G2261/1428 , C08G2261/143 , C08G2261/1452 , C08G2261/148 , C08G2261/149 , C08G2261/3442 , C08G2261/3444 , C08G2261/354 , C08G2261/516 , C08J5/2256 , C08J2371/12 , H01B1/122 , H01M8/1027 , H01M8/103 , H01M8/1032 , H01M8/1039 , H01M2300/0082 , Y02P70/56
摘要： A nitrogen-containing aromatic compound is represented by Formula (1). A polymer is obtained by polymerizing the compound. wherein X is an atom or a group selected from halogen atoms other than fluorine and —OSO2Rb (wherein Rb is an alkyl group, a fluorine-substituted alkyl group or an aryl group); Y is at least one structure selected from the group consisting of —CO—, —SO2—, —SO—, —CONH—, —COO—, —(CF2)l— (wherein l is an integer of 1 to 10) and —C(CF3)2—; Z is at least one structure selected from the group consisting of a direct bond, —O— and —S—; R20 is a nitrogen-containing heterocyclic group; q is an integer of 1 to 5; and p is an integer of 0 to 4.
摘要翻译：含氮芳香族化合物由式（1）表示。通过聚合化合物获得聚合物。其中X是选自除氟和-OSO 2 R b之外的卤素原子的原子或基团（其中R b是烷基，氟取代的烷基或芳基）。 Y是选自-CO - ， - SO 2 - ， - SO - ， - CONH - ， - COO - ， - （CF 2）1 - （其中l是1-10的整数）和 -C（CF 3）2 - ; Z是选自直接键，-O-和-S-的至少一种结构; R20是含氮杂环基; q为1〜5的整数， p为0〜4的整数。

28. 发明授权

US5854384A Process for preparing poly-.alpha.-amino acid particles 失效
标题翻译：制备聚-α-氨基酸颗粒的方法
公开(公告)号：US5854384A
公开(公告)日：1998-12-29
申请号：US719544
申请日：1996-09-25
申请人： Kyoko Kuroda , Masayuki Hattori , Yoshitaka Yamakawa , Kenya Makino , Toshio Hayashi
发明人： Kyoko Kuroda , Masayuki Hattori , Yoshitaka Yamakawa , Kenya Makino , Toshio Hayashi
IPC分类号： A61K9/16 , C08G69/10 , C08G69/00
CPC分类号： A61K9/1641 , C08G69/10
摘要： A process for preparing poly-.alpha.-amino acid particles comprising polymerizing an .alpha.-amino acid-N-carboxy anhydride using a polymerization initiator in an organic solvent in which both the solubility of the .alpha.-amino acid-N-carboxy anhydride and the solubility of the produced poly-.alpha.-amino acid are 0.1 g/100 ml or less at 25.degree. C. Polyamino acid particles having a high molecular weight and a small bulk specific gravity can be manufactured very easily without requiring specific procedures. The polyamino acid particles can be used as a coating material for papers, resins, rubbers, and fibers; particles for cosmetics; particles for diagnostic drugs; fillers for chromatography; and an encapsulating material for drugs, fertilizers, and perfumes.
摘要翻译：一种制备聚-α-氨基酸颗粒的方法，包括在有机溶剂中使用聚合引发剂聚合α-氨基酸-N-羧酸酐，其中α-氨基酸-N-羧酸酐的溶解度和溶解度的制备的聚-α-氨基酸在25℃下为0.1g / 100ml或更少。具有高分子量和小堆积比重的聚氨基酸颗粒可以非常容易地制造，而不需要特定的程序。聚氨基酸颗粒可用作纸，树脂，橡胶和纤维的涂料; 化妆品颗粒用于诊断药物的颗粒; 色谱填料; 以及用于药物，肥料和香水的包封材料。

29. 发明授权

US5593639A Blood-sampling vessel 失效
标题翻译：血液取样容器
公开(公告)号：US5593639A
公开(公告)日：1997-01-14
申请号：US450144
申请日：1995-05-26
申请人： Kenya Makino , Yoshitaka Yamakawa , Mitsuhiro Murata , Toshio Hayashi
发明人： Kenya Makino , Yoshitaka Yamakawa , Mitsuhiro Murata , Toshio Hayashi
IPC分类号： B01L3/14 , A61B5/14
CPC分类号： B01L3/5082
摘要： A blood-sampling vessel containing therein a conjugated diene (co)polymer with a weight average molecular weight, reduced to sodium polystyrene sulfonate, of at least 3,000 and containing 2 mmol/g or more of at least one sulfonic acid group or a salt thereof. The vessel can be easily manufactured and constantly exhibits high anticoagulant and fibrinogen-removing capability to the blood contained therein, with no adverse effects on a variety of inspections and tests.
摘要翻译：一种血液取样容器，其中含有重均分子量为至少3,000并且含有2mmol / g或更多的至少一种磺酸基或其盐的共聚二烯（共）聚合物，其重量平均分子量降低至聚苯乙烯磺酸钠。该容器可以容易地制造，并且对其中所含的血液持续显示高抗凝和纤维蛋白原去除能力，对各种检查和试验没有不利影响。

30. 发明授权

US07906608B2 Nitrogenated aromatic compound, process for production of the same, polymer, and proton conductive membrane 有权
标题翻译：氮化芳族化合物，其制备方法，聚合物和质子传导膜
公开(公告)号：US07906608B2
公开(公告)日：2011-03-15
申请号：US11995793
申请日：2006-06-30
申请人： Makoto Higami , Igor Rozhanskii , Yoshitaka Yamakawa
发明人： Makoto Higami , Igor Rozhanskii , Yoshitaka Yamakawa
IPC分类号： C08G8/02
CPC分类号： H01M10/0565 , C07C49/84 , C07D207/325 , C07D209/08 , C07D209/86 , C07D213/643 , C07D213/65 , C07D213/68 , C07D215/233 , C07D231/12 , C07D233/60 , C07D235/18 , C07D239/32 , C07D239/34 , C07D249/08 , C07D257/04 , C07D263/57 , C07D277/36 , C07D277/66 , C07D277/74 , C08G61/02 , C08G61/10 , C08G61/12 , C08G73/028 , C08G2261/126 , C08G2261/1424 , C08G2261/1428 , C08G2261/143 , C08G2261/1452 , C08G2261/148 , C08G2261/149 , C08G2261/3442 , C08G2261/3444 , C08G2261/354 , C08G2261/516 , C08J5/2256 , C08J2371/12 , H01B1/122 , H01M8/1027 , H01M8/103 , H01M8/1032 , H01M8/1039 , H01M2300/0082 , Y02P70/56
摘要： A nitrogen-containing aromatic compound is represented by Formula (1). A polymer is obtained by polymerizing the compound. wherein X is an atom or a group selected from halogen atoms other than fluorine and —OSO2Rb (wherein Rb is an alkyl group, a fluorine-substituted alkyl group or an aryl group); Y is at least one structure selected from the group consisting of —CO—, —SO2—, —SO—, —CONH—, —COO—, —(CF2)1— (wherein l is an integer of 1 to 10) and —C(CF3)2—; Z is at least one structure selected from the group consisting of a direct bond, —O— and —S—; R20 is a nitrogen-containing heterocyclic group; q is an integer of 1 to 5; and p is an integer of 0 to 4.
摘要翻译：含氮芳香族化合物由式（1）表示。通过聚合化合物获得聚合物。其中X是选自除氟和-OSO 2 R b之外的卤素原子的原子或基团（其中R b是烷基，氟取代的烷基或芳基）。 Y是选自-CO - ， - SO 2 - ， - SO - ， - CONH - ， - COO - ， - （CF 2）1 - （其中l是1-10的整数）和 -C（CF 3）2 - ; Z是选自直接键，-O-和-S-的至少一种结构; R20是含氮杂环基; q为1〜5的整数， p为0〜4的整数。

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