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1. 发明授权

US08043762B2 Polyphenylene-containing electrode paste 有权
标题翻译：含聚苯撑的电极糊
公开(公告)号：US08043762B2
公开(公告)日：2011-10-25
申请号：US11995701
申请日：2006-06-30
申请人： Makoto Higami , Igor Rozhanskii , Yoshitaka Yamakawa , Nagayuki Kanaoka , Kaoru Fukuda , Ryoichiro Takahashi , Hiroshi Shinkai
发明人： Makoto Higami , Igor Rozhanskii , Yoshitaka Yamakawa , Nagayuki Kanaoka , Kaoru Fukuda , Ryoichiro Takahashi , Hiroshi Shinkai
IPC分类号： H01M8/10
CPC分类号： C08G61/02 , C08G73/028 , C08J5/2256 , C08J2371/12 , H01M4/8652 , H01M4/8807 , H01M4/92 , H01M4/926 , H01M8/0239 , H01M8/1023 , H01M8/1025 , H01M8/1027 , H01M8/103 , H01M8/1032 , H01M8/1048 , H01M8/106
摘要： The present invention provides an electrode paste which comprises catalyst particles, a solvent and an varnish which comprises a solvent and an electrode electrolyte for a solid polymer fuel cell electrolyte, wherein the electrode electrolyte comprises a polymer with a structure having a main chain including a polyphenylene, a side chain including a sulfonic acid group and a repeating structural unit represented by formula (C) as a side chain including a nitrogen-containing heterocyclic group; wherein the structural variables are defined herein.
摘要翻译：本发明提供一种电极糊料，其包含催化剂颗粒，溶剂和清漆，其包含溶剂和用于固体聚合物燃料电池电解质的电极电解质，其中所述电极电解质包含具有主链的聚合物，所述主链包含聚亚苯基，包含磺酸基的侧链和由式（C）表示的重复结构单元作为包含含氮杂环基的侧链; 其中结构变量在本文中定义。

2. 发明申请

US20090149623A1 NITROGENATED AROMATIC COMPOUND, PROCESS FOR PRODUCTION OF THE SAME, POLYMER, AND PROTON CONDUCTIVE MEMBRANE 有权
标题翻译：硝基芳族化合物，其制备方法，聚合物和导电膜
公开(公告)号：US20090149623A1
公开(公告)日：2009-06-11
申请号：US11995793
申请日：2006-06-30
申请人： Makoto Higami , Igor Rozhanskii , Yoshitaka Yamakawa
发明人： Makoto Higami , Igor Rozhanskii , Yoshitaka Yamakawa
IPC分类号： C08G8/02 , C07D233/64 , C07D277/74
CPC分类号： H01M10/0565 , C07C49/84 , C07D207/325 , C07D209/08 , C07D209/86 , C07D213/643 , C07D213/65 , C07D213/68 , C07D215/233 , C07D231/12 , C07D233/60 , C07D235/18 , C07D239/32 , C07D239/34 , C07D249/08 , C07D257/04 , C07D263/57 , C07D277/36 , C07D277/66 , C07D277/74 , C08G61/02 , C08G61/10 , C08G61/12 , C08G73/028 , C08G2261/126 , C08G2261/1424 , C08G2261/1428 , C08G2261/143 , C08G2261/1452 , C08G2261/148 , C08G2261/149 , C08G2261/3442 , C08G2261/3444 , C08G2261/354 , C08G2261/516 , C08J5/2256 , C08J2371/12 , H01B1/122 , H01M8/1027 , H01M8/103 , H01M8/1032 , H01M8/1039 , H01M2300/0082 , Y02P70/56
摘要： A nitrogen-containing aromatic compound is represented by Formula (1). A polymer is obtained by polymerizing the compound. wherein X is an atom or a group selected from halogen atoms other than fluorine and —OSO2Rb (wherein Rb is an alkyl group, a fluorine-substituted alkyl group or an aryl group); Y is at least one structure selected from the group consisting of —CO—, —SO2—, —SO—, —CONH—, —COO—, —(CF2)l— (wherein l is an integer of 1 to 10) and —C(CF3)2—; Z is at least one structure selected from the group consisting of a direct bond, —O— and —S—; R20 is a nitrogen-containing heterocyclic group; q is an integer of 1 to 5; and p is an integer of 0 to 4.
摘要翻译：含氮芳香族化合物由式（1）表示。通过聚合化合物获得聚合物。其中X是选自除氟和-OSO 2 R b之外的卤素原子的原子或基团（其中R b是烷基，氟取代的烷基或芳基）。 Y是选自-CO - ， - SO 2 - ， - SO - ， - CONH - ， - COO - ， - （CF 2）1 - （其中l是1-10的整数）和 -C（CF 3）2 - ; Z是选自直接键，-O-和-S-的至少一种结构; R20是含氮杂环基; q为1〜5的整数， p为0〜4的整数。

3. 发明授权

US08399148B2 Varnish for a solid polymer fuel cell 有权
标题翻译：固体聚合物燃料电池的清漆
公开(公告)号：US08399148B2
公开(公告)日：2013-03-19
申请号：US13205177
申请日：2011-08-08
申请人： Makoto Higami , Igor Rozhanskii , Yoshitaka Yamakawa , Nagayuki Kanaoka , Kaoru Fukuda , Ryoichiro Takahashi , Hiroshi Shinkai
发明人： Makoto Higami , Igor Rozhanskii , Yoshitaka Yamakawa , Nagayuki Kanaoka , Kaoru Fukuda , Ryoichiro Takahashi , Hiroshi Shinkai
IPC分类号： H01M8/10
CPC分类号： C08G61/02 , C08G73/028 , C08J5/2256 , C08J2371/12 , H01M4/8652 , H01M4/8807 , H01M4/92 , H01M4/926 , H01M8/0239 , H01M8/1023 , H01M8/1025 , H01M8/1027 , H01M8/103 , H01M8/1032 , H01M8/1048 , H01M8/106
摘要： Provided is a varnish which contains a solvent and an electrode electrolyte for a solid polymer fuel cell electrolyte, which contains a polymer with a structure having a main chain including a polyphenylene, a side chain including a sulfonic acid group and a repeating structural unit as a side chain including a nitrogen-containing heterocyclic group.
摘要翻译：提供一种清漆，其含有固体高分子型燃料电池用电解质的溶剂和电极电解质，其含有具有主链的聚合物，所述主链包含聚亚苯基，包含磺酸基的侧链和重复结构单元作为侧链包括含氮杂环基。

4. 发明申请

US20120040271A1 ELECTRODE ELECTROLYTE FOR SOLID POLYMER-TYPE FUEL CELL 有权
标题翻译：用于固体聚合物型燃料电池的电极电解质
公开(公告)号：US20120040271A1
公开(公告)日：2012-02-16
申请号：US13205177
申请日：2011-08-08
申请人： Makoto Higami , Igor Rozhanskii , Yoshitaka Yamakawa , Nagayuki Kanaoka , Kaoru Fukuda , Ryoichiro Takahashi , Hiroshi Shinkai
发明人： Makoto Higami , Igor Rozhanskii , Yoshitaka Yamakawa , Nagayuki Kanaoka , Kaoru Fukuda , Ryoichiro Takahashi , Hiroshi Shinkai
IPC分类号： H01M8/10
CPC分类号： C08G61/02 , C08G73/028 , C08J5/2256 , C08J2371/12 , H01M4/8652 , H01M4/8807 , H01M4/92 , H01M4/926 , H01M8/0239 , H01M8/1023 , H01M8/1025 , H01M8/1027 , H01M8/103 , H01M8/1032 , H01M8/1048 , H01M8/106
摘要： An electrode electrolyte for a solid polymer electrolyte-type fuel cell contains a polymer, which has a polyphenylene structure as a main chain and both a sulfonic acid group and a nitrogen-containing heterocyclic group as a side chain. A side chain having the nitrogen-containing heterocyclic group has a structure represented by the following general formula (D). where Z represents at least one kind of structures selected from a group consisting of a direct bond, —O— and —S—, Y represents at least one member selected from a group consisting of —CO—, —SO2—, —SO—, —CONH—, —COO—, —(CF2)1— (1 is an integer of 1 to 10) and —C(CF3)2, R20 represents a specified nitrogen-containing heterocyclic group, q represents an integer of 1 to 5 and p represents an integer of 0 to 4.
摘要翻译：固体高分子电解质型燃料电池用电极电解质含有作为主链的聚亚苯基结构和磺酸基和含氮杂环基作为侧链的聚合物。具有含氮杂环基的侧链具有由以下通式（D）表示的结构。其中Z表示选自由直接键，-O-和-S-组成的组中的至少一种结构，Y表示选自-CO - ， - SO 2 - ， - SO 2 - 的至少一种，，-CONH-，-COO - ， - （CF 2）1 - （1为1〜10的整数）和-C（CF 3）2，R 20表示规定的含氮杂环基，q表示1〜 5，p表示0〜4的整数。

5. 发明授权

US07906608B2 Nitrogenated aromatic compound, process for production of the same, polymer, and proton conductive membrane 有权
标题翻译：氮化芳族化合物，其制备方法，聚合物和质子传导膜
公开(公告)号：US07906608B2
公开(公告)日：2011-03-15
申请号：US11995793
申请日：2006-06-30
申请人： Makoto Higami , Igor Rozhanskii , Yoshitaka Yamakawa
发明人： Makoto Higami , Igor Rozhanskii , Yoshitaka Yamakawa
IPC分类号： C08G8/02
CPC分类号： H01M10/0565 , C07C49/84 , C07D207/325 , C07D209/08 , C07D209/86 , C07D213/643 , C07D213/65 , C07D213/68 , C07D215/233 , C07D231/12 , C07D233/60 , C07D235/18 , C07D239/32 , C07D239/34 , C07D249/08 , C07D257/04 , C07D263/57 , C07D277/36 , C07D277/66 , C07D277/74 , C08G61/02 , C08G61/10 , C08G61/12 , C08G73/028 , C08G2261/126 , C08G2261/1424 , C08G2261/1428 , C08G2261/143 , C08G2261/1452 , C08G2261/148 , C08G2261/149 , C08G2261/3442 , C08G2261/3444 , C08G2261/354 , C08G2261/516 , C08J5/2256 , C08J2371/12 , H01B1/122 , H01M8/1027 , H01M8/103 , H01M8/1032 , H01M8/1039 , H01M2300/0082 , Y02P70/56
摘要： A nitrogen-containing aromatic compound is represented by Formula (1). A polymer is obtained by polymerizing the compound. wherein X is an atom or a group selected from halogen atoms other than fluorine and —OSO2Rb (wherein Rb is an alkyl group, a fluorine-substituted alkyl group or an aryl group); Y is at least one structure selected from the group consisting of —CO—, —SO2—, —SO—, —CONH—, —COO—, —(CF2)1— (wherein l is an integer of 1 to 10) and —C(CF3)2—; Z is at least one structure selected from the group consisting of a direct bond, —O— and —S—; R20 is a nitrogen-containing heterocyclic group; q is an integer of 1 to 5; and p is an integer of 0 to 4.
摘要翻译：含氮芳香族化合物由式（1）表示。通过聚合化合物获得聚合物。其中X是选自除氟和-OSO 2 R b之外的卤素原子的原子或基团（其中R b是烷基，氟取代的烷基或芳基）。 Y是选自-CO - ， - SO 2 - ， - SO - ， - CONH - ， - COO - ， - （CF 2）1 - （其中l是1-10的整数）和 -C（CF 3）2 - ; Z是选自直接键，-O-和-S-的至少一种结构; R20是含氮杂环基; q为1〜5的整数， p为0〜4的整数。

6. 发明申请

US20090130526A1 ELECTRODE ELECTROLYTE FOR USE IN SOLID POLYMER FUEL CELL 有权
标题翻译：用于固体聚合物燃料电池的电极电解质
公开(公告)号：US20090130526A1
公开(公告)日：2009-05-21
申请号：US11995701
申请日：2006-06-30
申请人： Makoto Higami , Igor Rozhanskii , Yoshitaka Yamakawa , Nagayuki Kanaoka , Kaoru Fukuda , Ryoichiro Takahashi , Hiroshi Shinkai
发明人： Makoto Higami , Igor Rozhanskii , Yoshitaka Yamakawa , Nagayuki Kanaoka , Kaoru Fukuda , Ryoichiro Takahashi , Hiroshi Shinkai
IPC分类号： H01M8/10
CPC分类号： C08G61/02 , C08G73/028 , C08J5/2256 , C08J2371/12 , H01M4/8652 , H01M4/8807 , H01M4/92 , H01M4/926 , H01M8/0239 , H01M8/1023 , H01M8/1025 , H01M8/1027 , H01M8/103 , H01M8/1032 , H01M8/1048 , H01M8/106
摘要： This invention provides an electrode electrolyte for a solid polymer-type fuel cell, in which a cost problem and a problem related to recovery of catalyst metals are solved, having excellent proton conductivity, dimensional stability and heat resistance.An electrode electrolyte for a solid polymer electrolyte-type fuel cell contains a polymer, which has a polyphenylene structure as a main chain and both a sulfonic acid group and a nitrogen-containing heterocyclic group as a side chain. A side chain having the nitrogen-containing heterocyclic group has a structure represented by the following general formula (D). (In formula, Z represents at least one kind of structures selected from a group consisting of a direct bond, —O— and —S—, Y represents at least one kind of structures selected from a group consisting of —CO—, —SO2—, —SO—, —CONH—, —COO—, —(CF2)1— (1 is an integer of 1 to 10) and —C(CF3)2— and R20 represents a nitrogen-containing heterocyclic group. q represents an integer of 1 to 5 and p represents an integer of 0 to 4.)The above nitrogen-containing heterocyclic group is at least one kind of group derived from a compound selected from the group consisting of nitrogen-containing heterocyclic compounds including pyrrole, thiazole, isothiazole, oxazole, isoxazole, pyridine, imidazole, imidazoline, pyrazole, 1,3,5-triazine, pyrimidine, pyridazine, pyrazine, indole, quinoline, isoquinoline, purine, benzimidazole, benzoxazole, benzothiazole, tetrazole, tetrazine, triazole, carbazole, acridine, quinoxaline and quinazoline and derivatives thereof.
摘要翻译：本发明提供一种固体聚合物型燃料电池用电极电解质，其中解决了成本问题和与催化剂金属的回收相关的问题，具有优异的质子传导性，尺寸稳定性和耐热性。固体高分子电解质型燃料电池用电极电解质含有作为主链的聚亚苯基结构和磺酸基和含氮杂环基作为侧链的聚合物。具有含氮杂环基的侧链具有由以下通式（D）表示的结构。（式中，Z表示选自由直链，-O-和-S-组成的组中的至少一种结构，Y表示选自-CO - ， - SO 2的至少一种结构 - ， - SO - ， - CONH - ， - COO - ， - （CF 2）1 - （1为1〜10的整数）和-C（CF 3）2 - ，R 20为含氮杂环基 1〜5的整数，p表示0〜4的整数。）上述含氮杂环基是选自包含吡咯，噻唑等含氮杂环化合物的化合物中的至少一种异噻唑，恶唑，异恶唑，吡啶，咪唑，咪唑啉，吡唑，1,3,5-三嗪，嘧啶，哒嗪，吡嗪，吲哚，喹啉，异喹啉，嘌呤，苯并咪唑，苯并恶唑，苯并噻唑四唑，四嗪，三唑，，吖啶，喹喔啉和喹唑啉及其衍生物。

7. 发明授权

US06812290B2 Polyarylene copolymers and proton-conductive membrane 有权
标题翻译：聚亚芳基共聚物和质子传导膜
公开(公告)号：US06812290B2
公开(公告)日：2004-11-02
申请号：US10303821
申请日：2002-11-26
申请人： Kohei Goto , Yoshitaka Yamakawa , Mayumi Kakuta , Igor Rozhanskii
发明人： Kohei Goto , Yoshitaka Yamakawa , Mayumi Kakuta , Igor Rozhanskii
IPC分类号： C08F836
CPC分类号： C08G61/12 , C07C45/46 , C07C49/84
摘要： A polyarylene copolymer which comprises (A) aromatic compound units having a main chain containing one or more electron-withdrawing groups therein and (B) aromatic compound units having a main chain containing no electron-withdrawing groups therein, and a proton-conductive membrane comprising the polyarylene copolymer having sulfonic acid groups.
摘要翻译：一种聚亚芳基共聚物，其包含（A）具有含有一个或多个吸电子基团的主链的芳香族化合物单元和（B）具有不含吸电子基团的主链的芳香族化合物单元，以及质子传导性膜，所述聚亚芳基共聚物具有磺酸基。

8. 发明授权

US07163988B2 Aromatic sulfonic acid ester derivative, polyarylene, polyarylene having sulfonic acid group and process for producing the same, and polymer solid electrolyte and proton-conductive membrane 有权
标题翻译：芳族磺酸酯衍生物，聚亚芳基，具有磺酸基的聚亚芳基及其制备方法，以及聚合物固体电解质和质子传导膜
公开(公告)号：US07163988B2
公开(公告)日：2007-01-16
申请号：US10642694
申请日：2003-08-19
申请人： Igor Rozhanskii , Masayuki Takahashi , Kohei Goto , Yousuke Konno , Toshihiro Ohtsuki , Yoshitaka Yamakawa , Toshiaki Kadota
发明人： Igor Rozhanskii , Masayuki Takahashi , Kohei Goto , Yousuke Konno , Toshihiro Ohtsuki , Yoshitaka Yamakawa , Toshiaki Kadota
IPC分类号： C08F283/08 , C08G61/10
CPC分类号： C08G61/12 , C07C309/73 , C07C309/75
摘要： Disclosed is an aromatic sulfonic acid ester derivative represented by the formula (1); in the formula, X is an atom or a group selected from a halogen atom excluding fluorine, —OSO3CH3 and —OSO3CF3, A is a divalent electron attractive group, B is a divalent electron donating group or a direct bonding, Ra is a hydrocarbon group of 1 to 20 carbon atoms, Ar is an aromatic group having a substituent of —SO3Rb (wherein Rb is a hydrocarbon group of 1 to 20 carbon atoms), m is an integer of 0 to 10, n is an integer of 0 to 10 and k is an integer of 1 to 4. Also disclosed is a process for producing a polyarylene having a sulfonic acid group, which process comprises the steps of coupling polymerization of an aromatic compound containing the derivative of the formula (1), to prepare a polyarylene and hydrolysis of the polyarylene, and which process has high safety and is easily capable of controlling the amount of sulfonoc acid group introduced into a polymer and the introducing position thereof.
摘要翻译：公开了由式（1）表示的芳族磺酸酯衍生物; 在该式中，X是选自除氟以外的卤素原子的原子或基团，-OSO 3 CH 3和-OSO 3 CF A是二价吸电子基团，B是二价给电子基团或直接键合，R a是1-20个碳原子的烃基，Ar 是具有-SO 3 R b的取代基的芳香族基团（其中R b为1〜20个碳原子的烃基）， m为0〜10的整数，n为0〜10的整数，k为1〜4的整数。还公开了具有磺酸基的聚亚芳基的制造方法，该方法包括使聚合的含有式（1）的衍生物的芳族化合物，以制备聚亚芳基并且聚亚芳基的水解，并且该方法具有高安全性并且易于控制引入聚合物的磺酸基团的量和引入位置那里 F。

9. 发明授权

US06555626B2 Polyarylene copolymers and proton-conductive membrane 有权
标题翻译：聚亚芳基共聚物和质子传导膜
公开(公告)号：US06555626B2
公开(公告)日：2003-04-29
申请号：US09818847
申请日：2001-03-28
申请人： Kohei Goto , Yoshitaka Yamakawa , Mayumi Kakuta , Igor Rozhanskii
发明人： Kohei Goto , Yoshitaka Yamakawa , Mayumi Kakuta , Igor Rozhanskii
IPC分类号： C08F836
CPC分类号： C08G61/12 , C07C45/46 , C07C49/84
摘要： A polyarylene copolymer which comprises (A) from 60 to 3 mol % aromatic compound units having a main chain containing one or more electron-withdrawing groups therein and (B) from 40 to 97 mol % aromatic compound units having a main chain containing no electron-withdrawing groups therein (provided that (A)+(B)=100 mol %), and a proton-conductive membrane comprising the polyarylene copolymer having sulfonic acid groups.
摘要翻译：一种聚亚芳基共聚物，其包含（A）60〜3摩尔％的含有一个或多个吸电子基团的主链的芳族化合物单元和（B）40〜97摩尔％的不含电子的主链的芳族化合物单元（A）+（B）= 100摩尔％）和包含具有磺酸基的聚亚芳基共聚物的质子传导膜。

10. 发明授权

US6084053A Electronic part and process for manufacturing the same 失效
标题翻译：电子零件和制造过程相同
公开(公告)号：US6084053A
公开(公告)日：2000-07-04
申请号：US60105
申请日：1998-04-15
申请人： Minoru Matsubara , Yasutake Inoue , Mayumi Kakuta , Igor Rozhanskii , Kohei Goto
发明人： Minoru Matsubara , Yasutake Inoue , Mayumi Kakuta , Igor Rozhanskii , Kohei Goto
IPC分类号： C08G73/10 , H01B3/30 , H05K1/03 , B32B27/00
CPC分类号： H01B3/306 , C08G73/10 , C08G73/1039 , H05K1/0346 , Y10S428/901
摘要： Electronic parts and a process for manufacturing the electronic parts are provided. The electronic parts comprise an electric insulating material exhibiting a high heat resistance and low dielectric constant as a structural component. The electric insulating material is formed of a polyimide containing a recurring unit represented by the following general formula (1). ##STR1##
摘要翻译：提供了电子部件和用于制造电子部件的工艺。电子部件包括表现出高耐热性和低介电常数作为结构部件的电绝缘材料。电绝缘材料由含有由以下通式（1）表示的重复单元的聚酰亚胺形成。

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