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11. 发明申请

US20090318651A1 HETEROCYCLIC COMPOUND AND HETEROCYCLIC POLYMERS 审中-公开
标题翻译：杂环化合物和杂环聚合物
公开(公告)号：US20090318651A1
公开(公告)日：2009-12-24
申请号：US12515436
申请日：2007-11-19
申请人： Kenta Tanaka , Hideyuki Higashimura , Kazuei Ohuchi , Akio Tanaka , Masato Ueda
发明人： Kenta Tanaka , Hideyuki Higashimura , Kazuei Ohuchi , Akio Tanaka , Masato Ueda
IPC分类号： C08F28/06 , C07D277/20
CPC分类号： C08G75/32 , C07D263/34 , C07D277/20 , C07D277/32 , C07F7/0816 , C07F9/6564 , C08G61/123 , C08G2261/1412 , C08G2261/212 , C08G2261/3229 , C08G2261/417 , H01B1/127 , H01L51/0036 , H01L51/0094
摘要： The present invention provides a heterocyclic compound of the following general formula (I): wherein X and Y are different from each other and represent a halogen atom selected from among a chlorine atom, bromine atom and iodine atom, or CF3SO3−, CH3SO3−, C6H5SO3− or CH3C6H4SO3−; R1 represents an optionally substituted monovalent aliphatic hydrocarbon group having two or more carbon atoms; one of A1 and A2 represents —S—, —O—, —Se— or Te—, while the other represents —N═, —P═ or —Si(R2)═, wherein R2 represents a hydrogen atom, an optionally substituted monovalent hydrocarbon group, a halogen atom, an amino group or a carbonyl group; and one of two linkages each represented by a solid line and a dashed line is a single bond, while the other is a double bond.
摘要翻译：本发明提供以下通式（I）的杂环化合物：其中X和Y彼此不同，表示选自氯原子，溴原子和碘原子的卤原子，或CF 3 SO 3 - ，CH 3 SO 3 - ， C6H5SO3-或CH3C6H4SO3-; R1表示具有两个或更多个碳原子的任选取代的一价脂族烃基; A 1和A 2中的一个表示-S-，-O-，-Se-或Te-，而另一个表示-N-，-P-或-Si（R 2） - ，其中R 2表示氢原子，一价烃基，卤素原子，氨基或羰基; 并且每个由实线和虚线表示的两个键之一是单键，而另一个是双键。

12. 发明授权

US09455408B2 Layered structure, polymer, electroluminescent device, and photoelectric conversion device 有权
标题翻译：分层结构，聚合物，电致发光器件和光电转换器件
公开(公告)号：US09455408B2
公开(公告)日：2016-09-27
申请号：US13499631
申请日：2010-09-28
申请人： Masanobu Tanaka , Kenta Tanaka , Ken Sakakibara , Hideyuki Higashimura , Rui Ishikawa
发明人： Masanobu Tanaka , Kenta Tanaka , Ken Sakakibara , Hideyuki Higashimura , Rui Ishikawa
IPC分类号： H01L51/54 , C08G63/685 , C08G63/66 , H01L51/00 , C08G61/02 , C08G61/12 , H01L51/50
CPC分类号： H01L51/0039 , C08G61/02 , C08G61/12 , C08G61/122 , C08G2261/1424 , C08G2261/1426 , C08G2261/146 , C08G2261/312 , C08G2261/3142 , C08G2261/3162 , C08G2261/344 , C08G2261/91 , C08G2261/95 , H01L51/0038 , H01L51/0043 , H01L51/5056 , H01L51/5072 , Y02E10/549
摘要： Provided is a layered structure having a first electrode, a second electrode, a light emitting layer or a charge separation layer located between the first electrode and the second electrode, and a layer located between the light emitting layer or the charge separation layer and the first electrode and containing a polymer having a repeating unit containing one or more ionic groups selected from two specific groups and one or more specific polar groups. Also provided is a polymer having, as the repeating unit containing one or more ionic groups selected from two specific groups and one or more specific polar groups, one or more repeating units selected from four specific repeating units containing an aromatic group. The layered structure of the present invention provides an electroluminescent device capable of emitting light at a high luminance and a photoelectric conversion device having a high photoelectric conversion efficiency.
摘要翻译：提供一种分层结构，其具有位于第一电极和第二电极之间的第一电极，第二电极，发光层或电荷分离层，以及位于发光层或电荷分离层之间的层和第一并且含有具有重复单元的聚合物，所述重复单元含有选自两个特定基团和一个或多个特定极性基团的一个或多个离子基团。还提供了作为含有选自两个特定基团和一个或多个特定极性基团的一个或多个离子基团的重复单元的聚合物，一个或多个选自含有芳族基团的四个特定重复单元的重复单元。本发明的分层结构提供了能够以高亮度发光的电致发光器件和具有高光电转换效率的光电转换器件。

13. 发明授权

US09318706B2 Laminated structure, method for producing same, and electronic element comprising same 有权
标题翻译：叠层结构体及其制造方法以及包含其的电子元件
公开(公告)号：US09318706B2
公开(公告)日：2016-04-19
申请号：US13056475
申请日：2009-07-29
申请人： Kenta Tanaka , Rui Ishikawa , Tomohisa Temma , Hideyuki Higashimura
发明人： Kenta Tanaka , Rui Ishikawa , Tomohisa Temma , Hideyuki Higashimura
IPC分类号： B32B15/08 , B05D5/12 , H01L51/00 , H01M4/137 , H01M4/1399 , H01M4/60 , H05B33/26 , H01L51/50 , H01L51/52
CPC分类号： H01L51/0039 , H01L51/0035 , H01L51/0067 , H01L51/5048 , H01L51/5088 , H01L51/5203 , H01M4/137 , H01M4/1399 , H01M4/60 , H01M4/606 , H05B33/26 , Y02E60/122 , Y02P70/54 , Y10T428/24975 , Y10T428/31692 , Y10T428/31855
摘要： A laminated structure comprising an electrode, a polymer binding layer arranged on the electrode, and an electrically conductive organic material layer arranged on the polymer binding layer, wherein the polymer binding layer comprises an aromatic polymeric compound which has a structure represented by formula (I) [wherein Ar represents a conjugated divalent group which may have a substituent, provided that when there are multiple Ar's, the Ar's may be the same as or different from each other; and n represents an integer of 1 or greater] and has a number average molecular weight of 1×103 to 1×108 inclusive in terms of polystyrene content, the polymer binding layer is bonded to the electrode via a chemical bond between the aromatic polymeric compound and the surface of the electrode, and an electrically conductive organic material that composes a layer included in the electrically conductive organic material layer and arranged adjacent to the polymer binding layer has a number average molecular weight of 3×102 to 1×108 inclusive in terms of polystyrene content.
摘要翻译：一种叠层结构，包括电极，布置在电极上的聚合物结合层和布置在聚合物结合层上的导电有机材料层，其中聚合物结合层包含具有由式（I）表示的结构的芳族聚合物， [其中Ar表示可以具有取代基的共轭二价基团，条件是当存在多个Ar时，Ar可以彼此相同或不同; n表示1以上的整数]，以聚苯乙烯含量换算的数均分子量为1×10 3〜1×10 8，聚合物结合层通过芳香族聚合物之间的化学键与电极结合并且电极表面和构成导电有机材料层中包含的并且邻近聚合物结合层布置的层的导电有机材料的数均分子量为3×102〜1×108，包括在内的聚苯乙烯含量。

14. 发明申请

US20120181529A1 LAYERED STRUCTURE, POLYMER, ELECTROLUMINESCENT DEVICE, AND PHOTOELECTRIC CONVERSION DEVICE 有权
标题翻译：层状结构，聚合物，电致发光器件和光电转换器件
公开(公告)号：US20120181529A1
公开(公告)日：2012-07-19
申请号：US13499631
申请日：2010-09-28
申请人： Masanobu Tanaka , Kenta Tanaka , Ken Sakakibara , Hideyuki Higashimura , Rui Ishikawa
发明人： Masanobu Tanaka , Kenta Tanaka , Ken Sakakibara , Hideyuki Higashimura , Rui Ishikawa
IPC分类号： H01L51/54 , C08G63/685 , C08G63/66
CPC分类号： H01L51/0039 , C08G61/02 , C08G61/12 , C08G61/122 , C08G2261/1424 , C08G2261/1426 , C08G2261/146 , C08G2261/312 , C08G2261/3142 , C08G2261/3162 , C08G2261/344 , C08G2261/91 , C08G2261/95 , H01L51/0038 , H01L51/0043 , H01L51/5056 , H01L51/5072 , Y02E10/549
摘要： Provided is a layered structure having a first electrode, a second electrode, a light emitting layer or a charge separation layer located between the first electrode and the second electrode, and a layer located between the light emitting layer or the charge separation layer and the first electrode and containing a polymer having a repeating unit containing one or more ionic groups selected from two specific groups and one or more specific polar groups. Also provided is a polymer having, as the repeating unit containing one or more ionic groups selected from two specific groups and one or more specific polar groups, one or more repeating units selected from four specific repeating units containing an aromatic group. The layered structure of the present invention provides an electroluminescent device capable of emitting light at a high luminance and a photoelectric conversion device having a high photoelectric conversion efficiency.
摘要翻译：提供一种分层结构，其具有位于第一电极和第二电极之间的第一电极，第二电极，发光层或电荷分离层，以及位于发光层或电荷分离层之间的层和第一并且含有具有重复单元的聚合物，所述重复单元含有选自两个特定基团和一个或多个特定极性基团的一个或多个离子基团。还提供了作为含有选自两个特定基团和一个或多个特定极性基团的一个或多个离子基团的重复单元的聚合物，一个或多个选自含有芳族基团的四个特定重复单元的重复单元。本发明的分层结构提供了能够以高亮度发光的电致发光器件和具有高光电转换效率的光电转换器件。

15. 发明申请

US20110006294A1 LAYERED STRUCTURE 有权
标题翻译：层状结构
公开(公告)号：US20110006294A1
公开(公告)日：2011-01-13
申请号：US12921108
申请日：2009-03-05
申请人： Masanobu Tanaka , Kenta Tanaka , Shohgo Yamauchi , Hideyuki Higashimura
发明人： Masanobu Tanaka , Kenta Tanaka , Shohgo Yamauchi , Hideyuki Higashimura
IPC分类号： H01L51/54 , C08G63/00
CPC分类号： H01L51/0039 , C08G61/02 , C08G61/12 , C08G61/122 , C08G2261/124 , C08G2261/1426 , C08G2261/3142 , C08G2261/316 , C08G2261/3221 , C08G2261/5222 , C08G2261/80 , H01L51/5048 , Y02E10/549 , Y10S428/917
摘要： Disclosed is a layered structure including a first electrode and a second electrode, a light-emitting layer or a charge separation layer between the first electrode and the second electrode, and a layer containing a conjugated polymer compound between the light-emitting layer or the charge separation layer and the first electrode, wherein the conjugated polymer compound contains a repeating unit selected from the group consisting of a repeating unit represented by formula (1): wherein Ar1 represents a divalent aromatic group, R1 represents a substituent group having a group represented by formula (2), Ar1 may have a substituent group other than R1, and n1 represents an integer of 1 or more; -(R2)c1-(Q1)n2-Y1(M1)a1(Z1)b1 (2) wherein R2 represents a divalent aromatic group which may have a substituent group, Q1 represents a divalent organic group which may have a substituent group, Y1 represents a carbocation, an ammonium cation, a phosphonyl cation or a sulfonyl cation, M1 represents F−, Cl−, Br−, I−, OH−, RaSO3−, RaCOO−, ClO−, ClO2−, ClO3−, ClO4−, SCN−, CN−, NO3−, SO42−, HSO4−, PO43−, HPO42−, H2PO4−, BF4− or PF6−, Z1 represents a metal ion or an ammonium ion which may have a substituent group, c1 represents 0 or 1, n2 represents an integer of 0 or more, provided that n2 is 0 when c1 is 0, a1 represents an integer of 1 or more, b1 represents an integer of 0 or more, a1 and b1 are selected so that the charge of the substituent group represented by formula (2) is 0, Ra represents an alkyl group having 1 to 30 carbon atoms, which may have a substituent group, or an aryl group having 6 to 50 carbon atoms, which may have a substituent group.
摘要翻译：公开了一种层状结构，其包括第一电极和第二电极，在第一电极和第二电极之间的发光层或电荷分离层，以及在发光层或电荷之间含有共轭高分子化合物的层分离层和第一电极，其中共轭高分子化合物含有选自由式（1）表示的重复单元的重复单元：其中Ar1表示二价芳族基团，R1表示具有由式（2）中，Ar 1可以具有除了R1以外的取代基，n1表示1以上的整数。 - （R2）c1-（Q1）n2-Y1（M1）a1（Z1）b1（2）其中R2表示可以具有取代基的二价芳族基团，Q1表示可以具有取代基的二价有机基团， Y1表示碳阳离子，铵阳离子，膦酰基阳离子或磺酰基阳离子，M1表示F-，Cl-，Br-，I-，OH-，RaSO 3 - ，RaCOO-，ClO-，ClO 2 - ，ClO 3 - ，ClO 4 - ，SCN-，CN-，NO3-，SO42-，HSO4-，PO43-，HPO42-，H2PO4-，BF4-或PF6-，Z1表示可具有取代基的金属离子或铵离子，c1表示 0或1，n2表示0以上的整数，条件是当c1为0时，n2为0，a1表示1以上的整数，b1表示0以上的整数，a1和b1选择为电荷由式（2）表示的取代基为0，R a表示可以具有取代基的碳原子数1〜30的烷基或碳原子数6〜50的芳基，可以具有取代基 ent组。

16. 发明申请

US20100133476A1 POLYMERIC ADSORPTION FILMS AND PROCESSES FOR PRODUCING THESE 审中-公开
标题翻译：聚合吸附膜及其生产工艺
公开(公告)号：US20100133476A1
公开(公告)日：2010-06-03
申请号：US12411599
申请日：2009-03-26
申请人： Kenta TANAKA , Hideyuki Higashimura , Toshihiko Tanaka , Tomohisa Temma , Daisuke Fukushima
发明人： Kenta TANAKA , Hideyuki Higashimura , Toshihiko Tanaka , Tomohisa Temma , Daisuke Fukushima
IPC分类号： H01B1/12
CPC分类号： C08G61/00 , C08G61/12 , C08G2261/126 , C08G2261/3142 , C08G2261/3162 , C08L65/00 , H01L51/0036 , H01L51/0039 , H01L51/0043 , H01L51/4253
摘要： The present invention provides a polymeric adsorption film comprising a polymer containing two or more charge-transport blocks and a substrate, wherein any of the charge-transport blocks is preferentially adhered to a surface of the substrate; a polymeric adsorption film comprising a polymer containing two or more charge-transport blocks and a substrate, wherein any of the charge-transport blocks different from the charge-transport block preferentially adhered to a surface of the substrate is preferentially exposed; or a polymeric adsorption film comprising a polymer and a substrate, wherein the polymer contains two or more charge-transport blocks and any charge-transport block selected from the charge-transport blocks is adhered to a surface of the substrate more preferentially than the other charge-transport blocks.
摘要翻译：本发明提供一种聚合物吸附膜，其包含含有两个或更多个电荷输送嵌段和基材的聚合物，其中任何电荷传输嵌段优先粘附于基材的表面; 包含含有两个或更多个电荷输送嵌段的聚合物和基材的聚合物吸附膜，其中与电荷传输嵌段不同的电荷传输嵌段优先粘附到基材表面的任何电荷传输嵌段优先暴露; 或包含聚合物和基底的聚合物吸附膜，其中所述聚合物含有两个或更多个电荷输送嵌段，并且从所述电荷传输嵌段中选择的任何电荷传输嵌段比其它电荷更优先地粘附到所述衬底的表面运输块。

17. 发明申请

US20100069603A1 METHOD FOR PRODUCING STRUCTURE WHEREIN AROMATIC POLYMER IS BONDED TO BASE, STRUCTURE HAVING AROMATIC POLYMER CHAIN BONDED TO CONDUCTIVE BASE, AND ELECTRONIC DEVICE COMPRISING THE STRUCTURE 审中-公开
标题翻译：用于生产结构的方法，其中芳族聚合物结合到基底，具有结合到导电基底的芳族聚合物链的结构，以及包含结构的电子装置
公开(公告)号：US20100069603A1
公开(公告)日：2010-03-18
申请号：US12525132
申请日：2008-02-01
申请人： Kenta Tanaka , Hideyuki Higashimura , Tsutomu Yokozawa , Rui Ishiyama
发明人： Kenta Tanaka , Hideyuki Higashimura , Tsutomu Yokozawa , Rui Ishiyama
IPC分类号： C08G75/04
CPC分类号： C08G61/02 , C08G61/10 , C08G61/12 , C08G61/122 , C08G61/126 , C08G2261/411 , C08G2261/5222 , C08G2261/77 , C08G2261/91
摘要： Disclosed is a method for efficiently producing a structure wherein an aromatic polymer is bonded to a base. Also disclosed is such a structure wherein the base is electrically conductive. Specifically disclosed is a method for producing a structure, which comprises a step for polycondensing an aromatic compound represented by the formula (I) below in the presence of a polymerization catalyst and a base having a group represented by the formula (II) below. MYnAr—X (I) (In the formula (I), Ar represents a divalent group composed of an aromatic ring; X represents a halogen atom or the like; Y represents an oxygen atom, a sulfur atom, an imino group or the like; n represents 0 or 1; and M represents a hydrogen atom, —B(OQ1)2 (wherein Q1 represents a hydrogen atom, a hydrocarbon group or the like) or the like.) —Ara—(Xa)p (II) (In the formula (II), Ara represents a group having a valence of (p+1) and composed of an aromatic ring; Xa represents a halogen atom or a monovalent group expressed as —SO3Qa (wherein Qa represents a substituted or unsubstituted hydrocarbon group); p represents an integer not less than 1, and when p is an integer not less than 2, the plurality of Xa's may be the same as or different from each other.)
摘要翻译：公开了一种有效地制备其中芳族聚合物与碱结合的结构的方法。还公开了这样的结构，其中基底是导电的。具体公开的是一种结构的制造方法，该方法包括在聚合催化剂和具有下述通式（II）所示基团的基团的存在下使由下式（I）表示的芳族化合物缩聚的步骤。（I）（式（I）中，Ar表示由芳香环构成的二价基团，X表示卤素原子等，Y表示氧原子，硫原子，亚氨基基团等; n表示0或1; M表示氢原子，-B（OQ1）2（其中Q1表示氢原子，烃基等）等。）-Ara-（Xa） p（II）（式（II）中，Ara表示具有（p + 1）价并且由芳香环构成的基团; Xa表示卤素原子或表示为-SO 3 Q a的一价基团（其中Qa表示取代或未取代的烃基）; p表示1以上的整数，当p为2以上的整数时，多个X a可以相同也可以不同。

18. 发明授权

US09704612B2 Composition of silver-conjugated compound composite 有权
公开(公告)号：US09704612B2
公开(公告)日：2017-07-11
申请号：US14005099
申请日：2012-03-15
申请人： Takayuki Iijima , Hideyuki Higashimura
发明人： Takayuki Iijima , Hideyuki Higashimura
IPC分类号： H01B1/00 , H01B1/12 , B22F1/00 , B22F1/02 , C22C5/06 , H01B1/22 , C08K3/08 , H01B1/02 , H01L51/00 , H01L51/50
CPC分类号： H01B1/121 , B22F1/0003 , B22F1/02 , C08G2261/91 , C08G2261/95 , C08K3/08 , C22C5/06 , H01B1/02 , H01B1/22 , H01L51/0035 , H01L51/0039 , H01L51/0043 , H01L51/5076 , C08K5/098 , C08L65/00
摘要： A composition of a silver-conjugated compound composite containing (1) a silver-conjugated compound composite containing a silver particle with a Feret diameter of 1,000 nm or less and a conjugated compound having a weight average molecular weight of 3.0×102 or more being adsorbed to the silver particles and (2) an ionic compound. The ionic compound may be a compound having a structure represented by the following Formula (hh-1): [Chem. 1] Mm′+aX′n′−b (hh-1) wherein Mm′+ represents a metal cation, X′n′− represents an anion, a and b each independently represent an integer of 1 or more, and when Mm′+ and X′n′− are each plurally present, they may be the same as or different from each other.

19. 发明授权

US09184388B2 Layered structure, electronic device using same, aromatic compound, and method for manufacturing said compound 有权
标题翻译：层状结构，使用其的电子器件，芳族化合物，以及所述化合物的制造方法
公开(公告)号：US09184388B2
公开(公告)日：2015-11-10
申请号：US13812678
申请日：2011-07-29
申请人： Arihiro Yashiro , Hideyuki Higashimura , Rui Ishikawa , Masanobu Tanaka
发明人： Arihiro Yashiro , Hideyuki Higashimura , Rui Ishikawa , Masanobu Tanaka
IPC分类号： H01L51/50 , H01L51/00 , C07C211/56 , C07C211/63 , C07F9/54 , C07F9/572 , C08G61/12 , C07D209/86 , C07F5/02
CPC分类号： H01L51/0035 , C07C211/56 , C07C211/63 , C07D209/86 , C07F5/025 , C07F9/5407 , C07F9/5442 , C07F9/5456 , C07F9/5728 , C08G61/12 , C08G2261/1424 , C08G2261/312 , C08G2261/3162 , C08G2261/411 , C08G2261/512 , C08G2261/91 , C08G2261/92 , C08G2261/95 , H01L51/5056 , Y02E10/549 , Y02P70/521
摘要： The present invention provides: a layered structure having a substrate and a hole injection and/or hole transport layer comprising an aromatic compound having, on a side chain, at least one type of group having a cationic center; an electronic device having the layered structure; an aromatic compound having, on a hydrocarbon side chain, at least one type of group having a cationic center; an aromatic compound having a leaving group on a hydrocarbon side chain; and a method for manufacturing the aromatic compound having, on a hydrocarbon side chain, at least one type of group having a cationic center, the method comprising reacting the aromatic compound having a leaving group on a hydrocarbon side chain with a specific nitrogen compound, phosphorus compound, sulfur compound, or a combination of two or more of these compounds, thereby converting the aromatic compound into an onium salt thereof. When used as an electronic device material, and particularly as a hole transport and/or hole injection material, the aromatic compound can achieve a higher current density at a given voltage.
摘要翻译：本发明提供：具有基材和空穴注入和/或空穴传输层的层状结构，所述空穴注入和/或空穴传输层包含芳族化合物，所述芳族化合物在侧链上具有至少一种具有阳离子中心的基团; 具有层状结构的电子设备; 在烃侧链上具有至少一种具有阳离子中心的基团的芳族化合物; 在烃侧链上具有离去基团的芳族化合物; 以及在烃侧链具有至少一种具有阳离子中心的基团的芳香族化合物的制造方法，其特征在于，使烃侧链上具有离去基团的芳香族化合物与特定的氮化合物反应，化合物，硫化合物或两种或更多种这些化合物的组合，从而将芳族化合物转化成其鎓盐。当用作电子器件材料，特别是用作空穴传输和/或空穴注入材料时，芳族化合物可以在给定电压下实现更高的电流密度。

20. 发明申请

US20120168693A1 SILVER-(CONJUGATED COMPOUND) COMPOSITE 有权
标题翻译：银（复合）复合材料
公开(公告)号：US20120168693A1
公开(公告)日：2012-07-05
申请号：US13496611
申请日：2010-09-17
申请人： Takayuki Iijima , Masahiro Fujioka , Hideyuki Higashimura
发明人： Takayuki Iijima , Masahiro Fujioka , Hideyuki Higashimura
IPC分类号： H01B1/02 , C08G79/00 , C08G73/06
CPC分类号： H01B1/22 , B22F1/00 , B22F1/0062 , B22F1/02 , B22F9/00 , B22F9/24 , B22F2001/0092 , B82Y30/00 , C08G73/06 , C08G79/00 , C08G2261/1424 , C08G2261/1432 , C08G2261/148 , C08G2261/3142 , C08G2261/3162 , C08G2261/514 , C08G2261/95 , C08K3/08 , C08L65/00 , H01B1/00
摘要： A silver-(conjugated compound) composite comprising silver particles having a number-average Feret diameter of not more than 1,000 nm, and a conjugated compound having a weight-average molecular weight of not less than 3.0×102 adsorbed to the silver particles. The composite exhibits excellent conductivity and charge injection properties, and excellent dispersibility within non-polar solvents.
摘要翻译：包含平均Feret直径不大于1000nm的银颗粒的银 - （共轭化合物）复合物和吸附在银颗粒上的重均分子量不小于3.0×102的共轭化合物。该复合材料具有优异的导电性和电荷注入性能，并且在非极性溶剂中具有优异的分散性。

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