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11. 发明授权

US07563743B2 Doped catalyst and improved process for treatment of hydrocarbon feedstocks 有权
标题翻译：掺杂催化剂和用于处理烃原料的改进方法
公开(公告)号：US07563743B2
公开(公告)日：2009-07-21
申请号：US11221416
申请日：2005-09-08
申请人： Patrick Euzen , Alexandra Chaumonnot , Carole Bobin , Patrick Bourges , Christophe Gueret , Hugues Dulot
发明人： Patrick Euzen , Alexandra Chaumonnot , Carole Bobin , Patrick Bourges , Christophe Gueret , Hugues Dulot
IPC分类号： B01J27/00 , B01J21/00 , B01J23/00 , B01J23/10 , B01J23/40 , B01J23/42 , B01J23/44 , B01J23/56 , B01J20/00 , C07C4/02 , C10G11/00 , C10G11/02
CPC分类号： B01J37/28 , B01J21/02 , B01J21/12 , B01J23/74 , B01J23/85 , B01J23/883 , B01J23/8877 , B01J23/888 , B01J23/8885 , B01J23/8993 , B01J27/188 , B01J35/0006 , B01J35/002 , B01J35/10 , B01J35/1019 , B01J35/1038 , B01J35/1061 , B01J35/108 , B01J37/0201 , B01J37/03 , B01J37/10 , B01J37/20 , B01J37/30 , C10G49/04 , C10G2300/107 , C10G2300/1074 , C10G2300/1077 , C10G2300/4018
摘要： This invention relates to doped catalysts on an aluminosilicate substrate with a low content of macropores and the hydrocracking/hydroconversion and hydrotreatment processes that use them. The catalyst comprises at least one hydro-dehydrogenating element that is selected from the group that is formed by the elements of group VIB and group VIII of the periodic table and a dopant in a controlled quantity that is selected from among phosphorus, boron, and silicon and a non-zeolitic substrate with a silica-alumina base that contains a quantity of more than 15% by weight and of less than or equal to 95% by weight of silica (SiO2).
摘要翻译：本发明涉及具有低含量大孔的铝硅酸盐底物上的掺杂催化剂和使用它们的加氢裂化/加氢转化和加氢处理方法。催化剂包含至少一种选自由元素周期表VIB族和VIII族的元素形成的基团和选自磷，硼和硅中的受控量的掺杂剂的氢脱氢元素和具有二氧化硅 - 氧化铝基底的非沸石基材，其含有大于15重量％且小于或等于95重量％的二氧化硅（SiO 2）的量。

12. 发明申请

US20090118556A1 ZEOLITIC CATALYST WITH A CONTROLLED DOPING ELEMENT CONTENT, AND IMPROVED PROCESS FOR PROCESSING HYDROCARBON FEEDS 有权
标题翻译：具有控制元素含量的新兴催化剂，以及加工油料进料的改进方法
公开(公告)号：US20090118556A1
公开(公告)日：2009-05-07
申请号：US11722610
申请日：2005-12-13
申请人： Patrick Euzen , Patrick Bourges , Christophe Gueret , Carole Bobin , Alexandra Chaumonnot , Hugues Dulot
发明人： Patrick Euzen , Patrick Bourges , Christophe Gueret , Carole Bobin , Alexandra Chaumonnot , Hugues Dulot
IPC分类号： B01J29/14 , B01J29/08 , C07C5/10
CPC分类号： B01J37/0009 , B01J21/12 , B01J29/146 , B01J29/166 , B01J35/1019 , B01J35/1023 , B01J35/1038 , B01J35/1061 , B01J35/108 , B01J2229/20 , B01J2229/42 , C10G47/14 , C10G47/20 , C10G65/12 , C10G2300/107 , C10G2300/1074 , C10G2300/1077 , C10G2300/4018
摘要： The present invention concerns doped catalysts on a mixed zeolite/alumino-silicate support with a low macropore content, and hydrocracking/hydroconversion and hydrotreatment processes employing them. The catalyst comprises at least one hydrodehydrogenating element selected from the group formed by elements from group VIB and group VIII of the periodic table and a doping element in a controlled quantity selected from phosphorus, boron and silicon, and a support based on zeolite Y defined by a lattice parameter a of the unit cell in the range 24.40×10−10 m to 24.15×10−10 m and silica-alumina containing a quantity of more than 5% by weight and 95% by weight or less of silica (SiO2).
摘要翻译：本发明涉及具有低大孔含量的混合沸石/铝硅酸盐载体上的掺杂催化剂，以及使用它们的加氢裂化/加氢转化和加氢处理方法。该催化剂包含至少一种选自由元素周期表第ⅥB族和第Ⅷ族元素形成的基团和选自磷，硼和硅的受控量的掺杂元素和基于沸石Y的载体的脱氢元素，在24.40×10 -10 m至24.15×10 -10 m范围内的晶胞的晶格参数a和含有多于5重量％和95重量％以下的二氧化硅（SiO 2）的二氧化硅 - 氧化铝。

13. 发明授权

US07404890B2 Process for the production of middle distillates by hydroisomerisation and hydrocracking feeds from the Fischer-Tropsch process 有权
标题翻译：通过费 - 托工艺的加氢异构化和加氢裂化原料生产中间馏分的方法
公开(公告)号：US07404890B2
公开(公告)日：2008-07-29
申请号：US10189738
申请日：2002-07-08
申请人： Eric Benazzi , Christophe Gueret
发明人： Eric Benazzi , Christophe Gueret
IPC分类号： C10G47/00 , C10G45/58
CPC分类号： C10G65/12 , C10G45/62 , C10G47/14 , C10G2300/1022 , C10G2300/301 , C10G2300/4081 , C10G2400/06 , C10G2400/08
摘要： The invention concerns a process and apparatus wherein the paraffin effluent from the Fischer-Tropsch process is separated into a heavy fraction with an initial boiling point of 120-200° C., said heavy fraction then optionally being hydrotreated then brought into contact with an amorphous hydroisomerization/hydrocracking catalyst that converts at least 80% by weight of the 370° C.+ products into products with a boiling point of less than 370° C. After distilling the hydrocracked fraction obtained to separate middle distillates, the residual heavy fraction is recycled.
摘要翻译：本发明涉及一种方法和设备，其中将来自费 - 托法的石蜡流出物分离成初馏点为120-200℃的重馏分，然后任选加氢处理然后使其与非晶态物质接触加氢异构化/加氢裂化催化剂，其将370℃+产物的至少80重量％转化成沸点小于370℃的产物。蒸馏得到的加氢裂化馏分分离中间馏分后，将残余重馏分循环。

14. 发明授权

US07381321B2 Process for improving aromatic and naphtheno-aromatic gas oil fractions 有权
$Process for improving aromatic and naphtheno-aromatic gas oil fractions$
标题翻译：用于改进芳族和环烷 - 芳烃瓦斯油馏分的方法
公开(公告)号：US07381321B2
公开(公告)日：2008-06-03
申请号：US10367965
申请日：2003-02-19
申请人： Eric Benazzi , Patrick Bourges , Christophe Gueret , Pierre Marion
发明人： Eric Benazzi , Patrick Bourges , Christophe Gueret , Pierre Marion
IPC分类号： C10G65/12
CPC分类号： C10G65/12
摘要： Process for transforming a gas-oil fraction that makes it possible to produce a fuel that has a quality according to stringent requirements in terms of sulfur content, aromatic compound content, cetane number, boiling point, T95, of 95% of the compounds and density, d15/4, at 15° C. This process comprises a hydrorefining stage and a hydrocracking stage, whereby the latter uses a catalyst that contains at least one zeolite. The conversion of products that have a boiling point of less than 150° C. is, throughout the two stages of hydrocracking and hydrorefining, less than 40% by weight and, for the hydrorefining stage, between 1 and 15% by weight. The temperature, TR2, of the hydrocracking stage is less than the temperature, TR1, of the hydrorefining stage, and the variation between temperatures TR1 and TR2 is between 0 and 80° C.
摘要翻译：用于转化瓦斯油馏分的方法，其使得可以生产具有根据硫含量，芳香族化合物含量，十六烷值，沸点，T95的严格要求的质量为95％的化合物和密度的燃料，d15 / 4，在15℃。该方法包括加氢精制阶段和加氢裂化阶段，由此后者使用含有至少一种沸石的催化剂。在加氢裂化和加氢精制两个阶段，沸点低于150℃的产物的转化率小于40重量％，加氢精制阶段为1至15重量％。加氢裂化阶段的温度TR2小于加氢精制阶段的温度TR1，温度TR1和TR2之间的变化在0和80℃之间。

15. 发明授权

US07371315B2 Flexible method for producing oil bases and distillates by hydroisomerization-conversion on a weakly dispersed catalyst followed by a catalyctic dewaxing 失效
标题翻译：通过在弱分散催化剂上进行加氢异构化转化生产油基和馏出物的灵活方法，然后进行催化脱蜡
公开(公告)号：US07371315B2
公开(公告)日：2008-05-13
申请号：US10450400
申请日：2001-12-13
申请人： Eric Benazzi , Nathalie Marchal-George , Tivadar Cseri , Pierre Marion , Christophe Gueret , Slavik Kasztelan
发明人： Eric Benazzi , Nathalie Marchal-George , Tivadar Cseri , Pierre Marion , Christophe Gueret , Slavik Kasztelan
IPC分类号： C10G69/02
CPC分类号： C10G65/12 , C10G65/043
摘要： A process for production of very high-quality base oils, and simultaneous production of high-quality middle distillates, comprises the successive stages of hydroisomerization and catalytic dewaxing. The hydroisomerization takes place in the presence of a catalyst containing at least one noble metal deposited on an amorphous acid support, the metal dispersion being less than 20%. The support is preferably an amorphous silica-alumina. The catalytic dewaxing takes place in the presence of a catalyst containing at least one hydrodehydrogenating element (Group VIII) and at least one molecular sieve chosen from ZBM-30, EU-2, and EU-11.
摘要翻译：用于生产非常优质基础油的方法，以及同时生产高品质中间馏分，包括加氢异构化和催化脱蜡的连续阶段。加氢异构化在含有沉积在无定形酸载体上的至少一种贵金属的催化剂存在下进行，金属分散体小于20％。载体优选为无定形二氧化硅 - 氧化铝。催化脱蜡在含有至少一种氢化脱氢元素（VIII族）和至少一种选自ZBM-30，EU-2和EU-11的分子筛的催化剂存在下进行。

16. 发明授权

US06602402B1 Flexible process for producing base stock and distillates by conversion-hydroisomerisation using a catalyst with low dispersion followed by catalytic dewaxing 失效
标题翻译：通过使用低分散体催化脱蜡的催化剂通过转化 - 加氢异构化生产基础油料和馏出物的柔性方法
公开(公告)号：US06602402B1
公开(公告)日：2003-08-05
申请号：US09562286
申请日：2000-05-01
申请人： Eric Benazzi , Nathalie Marchal-George , Tivadar Cseri , Pierre Marion , Christophe Gueret , Slavik Kasztelan
发明人： Eric Benazzi , Nathalie Marchal-George , Tivadar Cseri , Pierre Marion , Christophe Gueret , Slavik Kasztelan
IPC分类号： C10G6512
CPC分类号： C10G65/12 , B01J21/12 , B01J23/40 , B01J23/42 , B01J23/44 , B01J29/064 , B01J29/076 , B01J29/67 , B01J29/7446 , B01J29/7484 , B01J35/006 , B01J35/0066 , B01J35/023 , C10G45/62 , C10G65/043
摘要： An improved process for producing very high quality base stock and for simultaneous production of high quality middle distallates, comprising successive hydroisomerisation and catalystic dewaxing steps wherein hydroisomerisation is carried out in the presence of a catalyst containing at least one noble metal deposited on an amorphous acidic support, the dispersion of the metal being less than 20%. The support is preferably an amorphous silica-alumina. Catalytic dewaxing is carried out in the presence of a catalyst containing at least one hydrodehydrogenating element (group VIII) and at least one molecular sieve (preferably zeolite). The sieve is preferable selected from NU-10, EU-1, EU-13, zeolite and ferrierite.
摘要翻译：一种用于生产非常高质量的基础油料和用于同时生产高质量中间蒸馏物的改进方法，其包括连续加氢异构化和催化脱蜡步骤，其中加氢异构化在含有至少一种沉积在无定形酸性载体上的贵金属的催化剂存在下进行，金属的分散度小于20％。载体优选为无定形二氧化硅 - 氧化铝。催化脱蜡在含有至少一种氢化脱氢元素（VIII族）和至少一种分子筛（优选沸石）的催化剂存在下进行。筛子优选选自NU-10，EU-1，EU-13，沸石和镁碱沸石。

17. 发明授权

US5989410A Process for improving the pour point of paraffin feedstocks with a catalyst containing an IM-5 zeolite base 有权
标题翻译：用含有IM-5沸石基质的催化剂改进石蜡原料倾点的方法
公开(公告)号：US5989410A
公开(公告)日：1999-11-23
申请号：US172757
申请日：1998-10-15
申请人： Eric Benazzi , Nathalie George-Marchal , Christophe Gueret , Patrick Briot , Alain Billon , Pierre Marion
发明人： Eric Benazzi , Nathalie George-Marchal , Christophe Gueret , Patrick Briot , Alain Billon , Pierre Marion
IPC分类号： B01J29/72 , B01J29/44 , B01J29/74 , C01B39/08 , C08L91/06 , C09K3/00 , C10G35/06 , C10G45/04 , C10G45/20 , C10G45/64 , C10G35/085 , C10G35/095 , C10G47/12
CPC分类号： C10G45/64 , B01J29/74 , B01J2229/16 , B01J2229/26 , B01J2229/42
摘要： The invention relates to a process for improving the pour point of a feedstock that comprises paraffins of more than 10 carbon atoms, in which the feedstock that is to be treated is brought into contact with a catalyst that comprises the IM-5 zeolite and at least one hydro-dehydrogenating element, at a temperature of between 170 and 500.degree. C., a pressure of between 1 and 250 bar, and an hourly volume velocity of between 0.05 and 100 h.sup.-1, in the presence of hydrogen at a ratio of 50 to 2000 l/l of feedstock. The oils that are obtained have good pour points and high viscosity indices (VI). The process can also be applied to gas-oils and other feedstocks whose pour points need to be lowered.
摘要翻译：本发明涉及一种改进原料倾点的方法，该方法包括超过10个碳原子的链烷烃，其中待处理的原料与包含IM-5沸石的催化剂接触，并且至少一个加氢脱氢元件，在170-500℃的温度下，压力为1-250巴，小时体积速度为0.05-100小时-1，在氢存在下，比例为 50至2000升/原料。获得的油具有良好的倾点和高粘度指数（VI）。该方法也可应用于需要降低其倾点的瓦斯油和其他原料。

18. 发明授权

US07790019B2 Zeolitic catalyst, substrate based on a silica-alumina matrix and zeolite, and hydrocracking process for hydrocarbon feedstocks 有权
标题翻译：沸石催化剂，基于二氧化硅 - 氧化铝基质和沸石的底物，以及烃原料的加氢裂化方法
公开(公告)号：US07790019B2
公开(公告)日：2010-09-07
申请号：US10584144
申请日：2004-12-16
申请人： Patrick Euzen , Patrick Bourges , Hugues Dulot , Christophe Gueret
发明人： Patrick Euzen , Patrick Bourges , Hugues Dulot , Christophe Gueret
IPC分类号： C10G47/24 , C10G47/02 , B01J29/06
CPC分类号： B01J29/70 , B01J21/12 , B01J23/883 , B01J27/1853 , B01J27/19 , B01J29/064 , B01J29/076 , B01J29/084 , B01J29/74 , B01J29/78 , B01J35/1019 , B01J35/1023 , B01J35/1038 , B01J35/1042 , B01J35/1061 , B01J35/108 , B01J2229/42 , C10G45/64 , C10G47/12 , C10G65/12
摘要： The invention relates to a catalyst including at least one hydro-dehydrogenating element chosen from the group formed by the group VIB and group VIII elements of the periodic table and a substrate based on a silica-alumina matrix with a reduced content of macropores containing a quantity greater than 5% by weight and less than or equal to 95% by weight of silica (SiO2) and based on at least one zeolite.The invention also relates to a substrate based on a silica-alumina matrix with a reduced content of macropores containing a quantity greater than 5% by weight and less than or equal to 95% by weight of silica (SiO2) and based on at least one zeolite.The invention also relates to hydrocracking and/or hydroconversion processes and hydrotreating processes utilizing a catalyst according to the invention.
摘要翻译：本发明涉及一种催化剂，其包括至少一种选自由元素周期表VIB族和VIII族元素形成的加氢脱氢元素，以及基于二氧化硅 - 氧化铝基质的底物，其中含有大量的大孔大于5重量％且小于或等于95重量％的二氧化硅（SiO 2）并且基于至少一种沸石。本发明还涉及一种基于二氧化硅 - 氧化铝基质的底物，其具有含量大于5重量％且小于或等于95重量％的二氧化硅（SiO 2）的量的大孔含量，并基于至少一种沸石。本发明还涉及利用根据本发明的催化剂的加氢裂化和/或加氢转化方法和加氢处理方法。

19. 发明授权

US07582204B2 Method for treating a hydrocarbon feedstock including resin removal 有权
标题翻译：用于处理包括树脂去除的烃原料的方法
公开(公告)号：US07582204B2
公开(公告)日：2009-09-01
申请号：US10584048
申请日：2004-12-13
申请人： Christophe Gueret , Raphaël Huyghe , Hugues Dulot , Patrick Euzen
发明人： Christophe Gueret , Raphaël Huyghe , Hugues Dulot , Patrick Euzen
IPC分类号： C10G7/00 , C10G21/00 , B01D3/00
CPC分类号： C10G21/14 , C10G47/00 , C10G67/049 , C10G2300/107 , C10G2300/1077 , C10G2300/301 , C10G2300/44
摘要： The invention relates to a process, including removal of resins, for the treatment of a hydrocarbon charge, at least 80% of the compounds of which have a boiling point which is above or equal to 340° C., in which process: the charge is sent to a fractionation stage during which the recovery takes place of at least one heavy fraction and at least one light fraction, at least some of the heavy fraction is sent to an extraction stage during which resins contained in said heavy fraction are extracted, and a purified fraction is recovered, a mixture is made which comprises at least part of the purified fraction which was obtained in the extraction stage and at least one light fraction which was obtained in the fractionation stage, and the mixture thus obtained is sent to a cracking stage.
摘要翻译：本发明涉及一种方法，包括除去树脂，用于处理烃装料，其中至少80％的化合物具有高于或等于340℃的沸点，其中所述装料送入分馏阶段，在此阶段，回收发生至少一个重馏分和至少一个轻馏分，至少部分重馏分被送至萃取阶段，在此阶段萃取所述重馏分中所含的树脂，以及回收纯化的馏分，制备包含在萃取阶段获得的至少一部分纯化级分和在分馏阶段获得的至少一种轻馏分的混合物，将得到的混合物送入裂化阶段。

20. 发明授权

US07507325B2 Process for converting heavy petroleum fractions for producing a catalytic cracking feedstock and middle distillates with a low sulfur content 有权
$Process for converting heavy petroleum fractions for producing a catalytic cracking feedstock and middle distillates with a low sulfur content$
标题翻译：用于转化重质石油馏分以生产催化裂化原料的方法和具有低硫含量的中间馏分
公开(公告)号：US07507325B2
公开(公告)日：2009-03-24
申请号：US10152987
申请日：2002-05-23
申请人： Christophe Gueret , Pierre Marion , Cecile Plain , Jerome Bonnardot , Eric Benazzi , Olivier Martin
发明人： Christophe Gueret , Pierre Marion , Cecile Plain , Jerome Bonnardot , Eric Benazzi , Olivier Martin
IPC分类号： C10G45/04 , C10G47/02
CPC分类号： C10G69/02 , C10G2400/04
摘要： The invention relates to a process and installation for treating heavy petroleum feedstocks for producing a gas oil fraction that has a sulfur content of less than 50 ppm and most often 10 ppm that includes the following stages: a) mild hydrocracking in a fixed catalyst bed, b) separation from hydrogen sulfide of a distillate fraction that includes a gas oil fraction and a heavier fraction than the gas oil, c) hydrotreatment (including desulfurization) of said distillate fraction, and d) separation of a gas oil fraction with less than 50 ppm of sulfur. Advantageously, the heavy fraction is sent into catalytic cracking. The process preferably operates with make-up hydrogen that is brought to stage c), and very advantageously all of the make-up hydrogen of the process in introduced in stage c).
摘要翻译：本发明涉及用于处理重质石油原料的方法和装置，用于生产硫含量小于50ppm，最常为10ppm的瓦斯油馏分，其包括以下阶段：a）固定催化剂床中的轻度加氢裂化， b）与包含粗柴油馏分和比瓦斯油更重馏分的馏出物馏分的硫化氢分离，c）所述馏出馏分的加氢处理（包括脱硫），和d）分馏小于50的粗柴油馏分 ppm的硫。有利地，重馏分被送入催化裂化。该方法优选以使阶段c）中的补充氢运行，非常有利地在阶段c）中引入的所有方法的补充氢。

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