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1. 发明授权

US06133183A Process for regenerating a catalyst for the production of aromatic compounds or for reforming, with improved oxychlorination 失效
标题翻译：用于再生用于生产芳族化合物的催化剂或用于重整的方法，用改进的氧氯化
公开(公告)号：US06133183A
公开(公告)日：2000-10-17
申请号：US59293
申请日：1998-04-14
申请人： Marianne Capelle , Jean-Marie Deves , Frede ricfmann , Michel Thery
发明人： Marianne Capelle , Jean-Marie Deves , Frede ricfmann , Michel Thery
IPC分类号： B01J38/14 , B01J23/96 , B01J38/22 , B01J38/44 , C07B61/00 , C10G35/12 , B01J38/12 , B01J38/28 , B01J38/34
CPC分类号： B01J8/12 , B01J23/96 , B01J38/44 , C10G35/12
摘要： The invention concerns a process for regenerating a catalyst for the production of aromatic compounds, in particular for reforming, comprising combustion (A), oxychlorination (B) and calcining (C) steps, in which at least one chlorinating agent (conduit 19), at least one oxygen-containing gas (conduit 18), and water (conduit 20) are introduced into the oxychlorination step such that the H.sub.2 O/HCl molar ratio is 3 to 50, the oxychlorination step being carried out in the presence of an oxychlorination gas containing less than 21% of oxygen and at least 50 ppm by weight of chlorine (based on HCl), and at a temperature of 350-600.degree. C.
摘要翻译：本发明涉及用于再生用于生产芳族化合物，特别是用于重整的催化剂的方法，其包括燃烧（A），氧氯化（B）和煅烧（C）步骤，其中至少一种氯化剂（导管19）将至少一种含氧气体（导管18）和水（导管20）引入氧氯化步骤，使得H 2 O / HCl摩尔比为3至50，氧氯化步骤在氧氯化气体存在下进行含有少于21％的氧和至少50重量ppm的氯（基于HCl），并且在350-600℃的温度下

2. 发明授权

US06048814A Process and unit for regeneration of a catalyst for the production of aromatic compounds or for reforming 失效
标题翻译：用于生产芳香族化合物或重整用催化剂再生的方法和单元
公开(公告)号：US06048814A
公开(公告)日：2000-04-11
申请号：US59294
申请日：1998-04-14
申请人： Marianne Capelle , Jean-Marie Deves , Frederic Hoffmann , Michel Thery , Fran.cedilla.ois-Xavier Brunet , Emmanuelle Bromet
发明人： Marianne Capelle , Jean-Marie Deves , Frederic Hoffmann , Michel Thery , Fran.cedilla.ois-Xavier Brunet , Emmanuelle Bromet
IPC分类号： B01J38/14 , B01J23/96 , B01J38/22 , B01J38/44 , C07B61/00 , C07C17/152 , C10G35/12 , B01J38/00
CPC分类号： B01J8/12 , B01J23/96 , B01J38/44 , C10G35/12
摘要： The invention concerns a process and unit for regenerating a catalyst for the production of aromatic compounds, in particular for reforming, the catalyst being in a moving bed, comprising combustion, oxychlorination and calcining steps, in which at least one chlorinating agent, at least one oxygen-containing gas, and water are introduced into the oxychlorination step such that the H.sub.2 O/HCl molar ratio is 1 to 50, the oxychlorination step being carried out in the presence of an oxychlorination gas containing less than 21% of oxygen and at least 50 ppm by weight of chlorine (based on HCl), and at a temperature of 350-600.degree. C., and in which the combustion step is carried out in at least two combustion zones, each zone being separated from the adjacent zones, and at least one gas charged with oxygen is introduced into each zone, the gases produced being extracted from each zone, and in which the severity of the operating conditions increases in the direction of flow of the catalyst.
摘要翻译：本发明涉及用于再生催化剂的方法和单元，所述催化剂用于生产芳族化合物，特别是重整催化剂在移动床中，包括燃烧，氧氯化和煅烧步骤，其中至少一种氯化剂，至少一种将含氧气体和水引入到氧氯化步骤中，使得H 2 O / HCl摩尔比为1至50，氧氯化步骤在含有小于21％氧气和至少50％的氧氯化气体存在下进行氯化氢（基于HCl），并且在350-600℃的温度下，并且其中燃烧步骤在至少两个燃烧区域中进行，每个区域与相邻区域分离，并且在将至少一个带有氧气的气体引入每个区域，所产生的气体从每个区域提取，并且其中操作条件的严重性在催化剂流动方向上增加。

3. 发明授权

US06277335B1 Process and unit for regeneration of a catalyst for the production of aromatic compounds or for reforming 有权
标题翻译：用于生产芳香族化合物或重整用催化剂再生的方法和单元
公开(公告)号：US06277335B1
公开(公告)日：2001-08-21
申请号：US09503731
申请日：2000-02-15
申请人： Marianne Capelle , Jean-Marie Deves , Frédéric Hoffmann , Michel Thery , François-Xavier Brunet , Emmanuelle Bromet
发明人： Marianne Capelle , Jean-Marie Deves , Frédéric Hoffmann , Michel Thery , François-Xavier Brunet , Emmanuelle Bromet
IPC分类号： B01J3800
CPC分类号： B01J8/12 , B01J23/96 , B01J38/44 , C10G35/12
摘要： The invention concerns a process and unit for regenerating a catalyst for the production of aromatic compounds, in particular for reforming, the catalyst being in a moving bed, comprising combustion, oxychlorination and calcining steps, in which at least one chlorinating agent, at least one oxygen-containing gas, and water are introduced into the oxychlorination step such that the H2O/HCl molar ratio is 1 to 50, the oxychlorination step being carried out in the presence of an oxychlorination gas containing less than 21% of oxygen and at least 50 ppm by weight of chlorine (based on HCl), and at a temperature of 350-600° C., and in which the combustion step is carried out in at least two combustion zones, each zone being separated from the adjacent zones, and at least one gas charged with oxygen is introduced into each zone, the gases produced being extracted from each zone, and in which the severity of the operating conditions increases in the direction of flow of the catalyst.
摘要翻译：本发明涉及用于再生催化剂的方法和单元，所述催化剂用于生产芳族化合物，特别是重整催化剂在移动床中，包括燃烧，氧氯化和煅烧步骤，其中至少一种氯化剂，至少一种将含氧气体和水引入到氧氯化步骤中，使得H 2 O / HCl摩尔比为1至50，氧氯化步骤在含有小于21％氧气和至少50％的氧氯化气体存在下进行 ppm（基于HCl），并且在350-600℃的温度下，并且其中燃烧步骤在至少两个燃烧区域中进行，每个区域与相邻区域分离，并且在将至少一个带有氧气的气体引入每个区域，所产生的气体从每个区域提取，并且其中操作条件的严重性在催化剂流动方向上增加。

4. 发明授权

US06426052B1 Vessel for regenerating a catalyst for the production of aromatic compounds or for reforming, with improved oxychlorination 有权
标题翻译：用于再生用于生产芳族化合物或重整的催化剂的容器，具有改进的氧氯化
公开(公告)号：US06426052B1
公开(公告)日：2002-07-30
申请号：US09627075
申请日：2000-07-27
申请人： Marianne Capelle , Jean-Marie Deves , Frédéric Hoffmann , Michel Thery
发明人： Marianne Capelle , Jean-Marie Deves , Frédéric Hoffmann , Michel Thery
IPC分类号： B01J3844
CPC分类号： B01J8/12 , B01J23/96 , B01J38/44 , C10G35/12
摘要： A vessel for regenerating a catalyst for reforming or for aromatic compound production comprising a support, at least one noble metal and chlorine, the catalyst being in the form of a moving bed, said vessel comprising at least one combustion zone (A) provided with at least one conduit (9) for introducing oxygen gas and at least one conduit (5) for evacuating gasses from the combustion step, at least one oxychlorination zone (B) and at least one calcining zone (C) provided with at least one conduit (18) for introducing an oxygen-containing gas, said vessel also comprising at least one conduit (1) for introducing catalyst into the vessel, at least one conduit (3) for introducing catalyst from the combustion zone into the following oxychlorination zone (B), and at least one conduit (21) for evacuating gases from the oxychlorination zone comprising at least one means (20) for introducing least one chlorinating agent and at least one means (19) for introducing water and at least one means (17) for introducing an oxygen containing gas.
摘要翻译：一种用于再生用于重整或芳族化合物生产的催化剂的容器，包括载体，至少一种贵金属和氯，催化剂为移动床的形式，所述容器包括至少一个燃烧区（A），其设置在用于引入氧气的至少一个导管（9）和用于从燃烧步骤抽空气体的至少一个导管（5），至少一个氧氯化区（B）和至少一个设置有至少一个导管的煅烧区（C） 18，用于引入含氧气体，所述容器还包括用于将催化剂引入容器的至少一个导管（1），用于将催化剂从燃烧区引入到以下氧氯化区（B）中的至少一个导管（3），以及用于从氧氯化区排出气体的至少一个导管（21），包括用于引入最少一个氯化剂的至少一个装置（20）和用于引入水的至少一个装置（19）和至少一个装置（17），用于引入含氧气体。

5. 发明授权

US06548305B1 Automatic multi-reactor catalyst evaluation method an device with in-line analysis without liquid-gas separation 有权
标题翻译：自动多反应器催化剂评价方法一种无液气分离的在线分析装置
公开(公告)号：US06548305B1
公开(公告)日：2003-04-15
申请号：US09604736
申请日：2000-06-28
申请人： Jean-Marie Deves , Jean-Yves Bernhard , Bernard Chatelain , Pierre Toutant , José Brandely , Corinne Guitton
发明人： Jean-Marie Deves , Jean-Yves Bernhard , Bernard Chatelain , Pierre Toutant , José Brandely , Corinne Guitton
IPC分类号： G01N3110
CPC分类号： G01N31/10 , Y10T436/24
摘要： A method and an equipment carry out measurements on an effluent resulting from a chemical reaction taking place in a reactor containing a catalyst. The method includes, in combination, injecting at least one feedstock into at least two reactors, sending the effluent coming from one of the reactors for analysis and measuring controlling the pressure and the temperature of the effluent in the circuit contained between downstream from the reactors and upstream from the analysis device, and allowing automatic monitoring and control of the chemical reaction in the reactors and of the analysis and measurement cycle performed on the effluent produced by the reaction.
摘要翻译：一种方法和设备对在含有催化剂的反应器中发生的化学反应产生的流出物进行测量。该方法包括组合地将至少一种原料注入至少两个反应器中，送出来自反应器之一的流出物进行分析和测量，以控制在反应器下游包含的回路中的流出物的压力和温度，以及并且允许对反应器中的化学反应的自动监测和控制以及对由反应产生的流出物进行的分析和测量循环进行。

6. 发明授权

US06387246B1 Catalyst that comprises a partially amorphous Y zeolite and its use in hydroconversion of hydrocarbon petroleum feedstocks 有权
标题翻译：包含部分无定形Y沸石的催化剂及其在烃类石油原料加氢转化中的用途
公开(公告)号：US06387246B1
公开(公告)日：2002-05-14
申请号：US09572970
申请日：2000-05-18
申请人： Eric Benazzi , Jean-Marie Deves , Bernadette Rebours , Frédéric Chaigne , Tivadar Cseri , Slavik Kasztelan
发明人： Eric Benazzi , Jean-Marie Deves , Bernadette Rebours , Frédéric Chaigne , Tivadar Cseri , Slavik Kasztelan
IPC分类号： C01G4718
CPC分类号： B01J29/084 , B01J29/166 , B01J2229/20 , B01J2229/22 , B01J2229/36 , B01J2229/37 , B01J2229/42 , C10G45/12 , C10G47/16
摘要： The invention relates to a catalyst that contains at least one matrix, a partially amorphous Y zeolite, optionally at least one metal that is selected from the group that is formed by the metals of group VIB and group VIII of the periodic table, optionally at least one element that is selected from the group that is formed by phosphorus, boron and silicon, optionally at least one element of group VIIA, and optionally at least one element of group VIIB. The partially amorphous Y zeolite has a peak rate that is less than 0.4, and a crystalline fraction that is expressed relative to a reference zeolite in sodium form and that is less than 60%. The invention also relates to the use of this catalyst in hydroconversion, in particular hydrocracking and hydrorefining of hydrocarbon feedstocks.
摘要翻译：本发明涉及一种催化剂，其含有至少一种基质，部分无定形Y沸石，任选至少一种金属，其选自由元素周期表第ⅥB族和Ⅷ族金属形成的基团，任选至少选自由磷，硼和硅形成的基团，任选的ⅦA族的至少一种元素和任选的至少一种ⅦB族元素的一种元素。部分无定形的Y沸石具有小于0.4的峰值速率和相对于钠形式的参考沸石表达并且小于60％的结晶部分。本发明还涉及该催化剂在加氢转化中的用途，特别是烃原料的加氢裂化和加氢精制。

7. 发明授权

US6103652A Staged combustion process and apparatus for regenerating a reforming or aromatic compound production catalyst in a moving bed 失效
标题翻译：用于在移动床中再生重整或芳族化合物生产催化剂的分段燃烧方法和装置
公开(公告)号：US6103652A
公开(公告)日：2000-08-15
申请号：US59292
申请日：1998-04-14
申请人： Fran.cedilla.ois-Xavier Brunet , Emmanuelle Bromet , Jean-Marie Deves
发明人： Fran.cedilla.ois-Xavier Brunet , Emmanuelle Bromet , Jean-Marie Deves
IPC分类号： B01J27/32 , B01J23/96 , B01J38/14 , B01J38/20 , B01J38/24 , B01J38/34 , B01J38/44 , C07B61/00 , C10G35/12 , B01J20/34 , B01J38/12 , B01J38/22
CPC分类号： B01J8/12 , B01J23/96 , B01J38/20 , B01J38/24 , B01J38/44 , C10G35/12
摘要： The invention concerns a process for moving bed regeneration of a reforming or aromatic hydrocarbon production catalyst. The catalyst includes a support, at least one noble metal and at least one halogen. The process includes a combustion step in which the catalyst is treated in at least two successive combustion zones. Also, the process includes each combustion zone separated from adjacent combustion zones allowing catalyst to pass and preventing passage of gas, at least one oxygen-containing gas introduced into each zone and produced gases extracted from each zone, and the severity of the operating conditions in each zone increasing in the direction of catalyst flow. Advantageously, the combustion step ends in a zone for monitoring and controlling combustion completion characterized by a low or zero oxygen consumption.
摘要翻译：本发明涉及一种用于移动重整或芳族烃生产催化剂的床再生的方法。催化剂包括载体，至少一种贵金属和至少一种卤素。该方法包括燃烧步骤，其中在至少两个连续的燃烧区域中处理催化剂。此外，该方法还包括从相邻燃烧区分离的每个燃烧区，使得催化剂通过并防止气体的通过，至少一个引入每个区域的含氧气体和从每个区域提取的产生的气体，以及操作条件的严重性每个区域在催化剂流动方向上增加。有利地，燃烧步骤终止于用于监测和控制燃烧完成的区域，其特征在于低或零氧气消耗。

8. 发明授权

US06007700A Process for the catalyst conversion of hydrocarbons into aromatics using a catalyst containing at least one doping metal chosen from the group consisting of titanium, zirconium, hafnium, cobalt, nickel, zinc, and/or the lanthanides 失效
标题翻译：使用含有选自钛，锆，铪，钴，镍，锌和/或镧系元素中的至少一种掺杂金属的催化剂将烃转化成芳族化合物的方法
公开(公告)号：US06007700A
公开(公告)日：1999-12-28
申请号：US973404
申请日：1997-12-15
申请人： Fabio Alario , Jean-Marie Deves , Patrick Euzen
发明人： Fabio Alario , Jean-Marie Deves , Patrick Euzen
IPC分类号： B01J21/04 , B01J21/06 , B01J23/56 , B01J23/63 , B01J23/656 , B01J27/13 , B01J37/02 , B01J37/24 , C10G35/06 , C10G35/09 , C10G35/095 , C10G45/68 , C10G35/085
CPC分类号： C10G45/68 , B01J21/04 , B01J23/56 , B01J23/63 , B01J23/6567 , B01J27/13 , C10G35/06 , C10G35/065 , C10G35/09 , C10G35/095 , B01J21/06 , B01J21/063 , B01J21/066 , B01J37/0209 , B01J37/24
摘要： Gasolines are reformed and parafin and naphthene hydrocarbons are converted to aromatic compounds by contacting the hydrocarbons with a catalyst comprising a matrix of .eta. transition alumina and .gamma. transition alumina. The catalyst contains at least one doping metal, at least one halogen, at least one noble metal and at least one promoter metal. The doping metals are selected from titanium, zirconium, hafnium, cobalt, nickel, zinc, and the lanthanides and the promoter metals are selected from tin, germanium, indium, gallium, thallium, antimony, lead, rhenium, manganese, chromium, molybdenum and tungsten.
摘要翻译： PCT No.PCT / FR96 / 00917 Sec。 371 1997年12月15日第 102（e）日期1997年12月15日PCT Filted 1996年6月14日PCT公布。公开号WO97 / 00305 PCT 日期1997年1月3日通过使烃与包含等离子体氧化铝和γ过渡氧化铝的基质的催化剂接触来改变石脑油并将石蜡和环烷烃转化为芳族化合物。催化剂含有至少一种掺杂金属，至少一种卤素，至少一种贵金属和至少一种助催化剂金属。掺杂金属选自钛，锆，铪，钴，镍，锌和镧系元素，助催化剂金属选自锡，锗，铟，镓，铊，锑，铅，铼，锰，铬，钼和钨。

9. 发明授权

US08728404B1 Vessel for regeneration of a catalyst including monitoring and monitoring and control of combustion completion 有权
标题翻译：用于再生催化剂的容器，包括监测和监测和控制燃烧完成
公开(公告)号：US08728404B1
公开(公告)日：2014-05-20
申请号：US09551831
申请日：2000-04-18
申请人： François-Xavier Brunet , Emmanuelle Bromet , Jean-Marie Deves , Dominique Humeau , Eric Sanchez
发明人： François-Xavier Brunet , Emmanuelle Bromet , Jean-Marie Deves , Dominique Humeau , Eric Sanchez
IPC分类号： B01J38/14 , B01J38/20 , B01J38/22
CPC分类号： B01J8/12 , B01J38/12 , B01J38/14 , B01J38/20 , B01J38/24 , C10G35/12
摘要： A vessel for regenerating used catalyst comprising at least one combustion zone provided with at least two walls (5a, 5b) between which the catalyst circulates as a moving bed, and provided with at least one conduit (4) for introducing at least one oxygen-containing gas entering the moving bed via one of the walls and leaving via another wall, characterized in that it also comprises a zone (FC) for monitoring and controlling the end of combustion located after the end of the flame front of the last combustion zone (Z2), provided with a conduit (11) for introducing an oxygen-containing monitoring and control gas and at least one means for measuring the temperature and/or the oxygen content in the gas and/or the catalyst leaving the monitoring and control zone.A separator (29) is located between the monitoring and control zone and the last combustion zone for preventing the passage of gas while allowing for the passage of the catalyst.
摘要翻译：一种用于再生所用催化剂的容器，包括至少一个燃烧区，该燃烧区设置有至少两个壁（5a，5b），催化剂在其之间作为移动床循环，并且设置有至少一个导管（4），用于引入至少一个氧 - 包含气体通过一个壁进入移动床并通过另一个壁离开，其特征在于，其还包括用于监测和控制位于最后燃烧区域的火焰前端的末端之后的燃烧端的区域（FC） Z2），其具有用于引入含氧监测和控制气体的导管（11）和用于测量离开监测和控制区的气体和/或催化剂中的温度和/或氧含量的至少一种装置。分离器（29）位于监测和控制区域与最后一个燃烧区之间，用于防止气体通过，同时允许催化剂通过。

10. 发明申请

US20050214176A1 Process and device for the production of aromatic compounds including a reduction of the catalyst 审中-公开
标题翻译：用于生产芳族化合物的方法和装置，包括催化剂的还原
公开(公告)号：US20050214176A1
公开(公告)日：2005-09-29
申请号：US10703546
申请日：2003-11-10
申请人： Francois-Xavier Brunet , Olivier Clause , Jean-Marie Deves , Eric Sanchez , Frederic Hoffmann
发明人： Francois-Xavier Brunet , Olivier Clause , Jean-Marie Deves , Eric Sanchez , Frederic Hoffmann
IPC分类号： B01J38/04 , C07B61/00 , C07C5/42 , C07C15/04 , C07C15/06 , C07C15/08 , C10G35/09 , C10G35/12 , C10G35/22 , B01J8/18
CPC分类号： B01J8/12 , C10G35/12
摘要： The invention relates to a process for the production of aromatic compounds from a hydrocarbon fraction with a catalyst that preferably circulates in a moving bed, a process that comprises at least the following successive stages that take place in at least one zone: treatment of the fraction in the presence of hydrogen and implementing at least one reaction for dehydrogenation of naphthenes; separation of the gas effluent that contains hydrogen, the liquid product and the catalyst; regeneration of the catalyst; reduction of the catalyst; and reintroduction of the catalyst for the treatment stage; recycling in the treatment stage of at least a portion of the gas effluent that contains the hydrogen that is called recycling gas; process in which the reduction stage is carried out in the presence of recycling gas that is introduced in an amount such that the amount of pure hydrogen that is provided is between 1-10 kg/kg of catalyst, whereby the effluent that is obtained from the reduction is then separated from the catalytic bed. The invention also pertains to the related device.
摘要翻译：本发明涉及一种由具有优选在移动床中循环的催化剂的烃馏分生产芳族化合物的方法，该方法至少包括在至少一个区域中发生的以下连续阶段：处理馏分在氢的存在下，并且实施至少一个用于环烷酸脱氢的反应; 分离含有氢气，液体产物和催化剂的气体流出物; 催化剂再生; 还原催化剂; 并重新引入用于治疗阶段的催化剂; 在处理阶段回收至少一部分含有称为再循环气体的氢气的气体流出物; 在再循环气体的存在下进行还原阶段的方法，该再循环气体的导入量使得提供的纯氢的量在1-10kg / kg的催化剂之间，由此得到的流出物然后将还原与催化床分离。本发明也涉及相关设备。

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