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1. 发明专利

JP2003225567A CERAMIC COMPOSITE MATERIAL CONVERTED INTO CATALYST, PRODUCTION METHOD THEREFOR, AND CERAMIC FILM TYPE REACTOR 审中-公开
公开(公告)号：JP2003225567A
公开(公告)日：2003-08-12
申请号：JP2002299228
申请日：2002-10-11
申请人： TEIKOKU OIL , NIPPON STEEL CORP
发明人： KURIMURA HIDEKI , KAGANOI SHOICHI , SUZUKI YOHEI , ITO TAKASHI , SAKON TADASHI , ITO WATARU , DONOMAE HITOSHI , NAGAI TORU , HIRANO KENJI
IPC分类号： B01D53/22 , B01D71/02 , B01J23/656 , B01J23/755 , B01J23/847 , B01J23/89 , B01J37/02 , B32B18/00 , C01B3/40 , C01G49/00 , C01G51/00 , C04B35/00
摘要： PROBLEM TO BE SOLVED: To obtain a ceramic composite material converted into a catalyst which is applicable to a film type reactor for producing synthesis gas using an oxygen-containing gas and hydrocarbons as raw materials and can stably obtain a high oxygen transmission velocity. SOLUTION: The ceramic composite material converted into the catalyst has a multi-layer structure in which a porous catalyst layer comprising a mixed conductive oxide adjoins the first surface of a selectively oxygen-permeable compact continuous layer comprising the mixed conductive oxide, a porous intermediate catalyst layer comprising the mixed conductive oxide and/or a catalytic oxide having a combustion catalyst function adjoins the second surface of the continuous layer, and a porous reaction catalyst layer comprising a metal catalyst and a carrier adjoins the porous intermediate catalyst layer. COPYRIGHT: (C)2003,JPO

2. 发明专利

JP2003055671A Treating method of crude coke-oven gas and treatment system 有权
标题翻译：焦油焦炉和处理系统的处理方法
公开(公告)号：JP2003055671A
公开(公告)日：2003-02-26
申请号：JP2001248921
申请日：2001-08-20
申请人： Nippon Steel Corp , Teikoku Oil Co Ltd , 帝国石油株式会社 , 新日本製鐵株式会社
发明人： JITSUHARA IKUO , FUJIMOTO KENICHIRO , KURIMURA HIDEKI , KAGANOI SHOICHI , SUZUKI YOHEI
IPC分类号： C01B3/38 , B01J23/755 , C10K3/02
CPC分类号： Y02P20/124 , Y02P20/52
摘要： PROBLEM TO BE SOLVED: To provide a new recovery technique and energy saving system of heat energy, and a new energy creative system that in view of the present state that sensible heat is not effectively used due to a quenching treatment by spraying ammonia water, in spite of a coke-oven gas comprising a coal volatile matter as a principal component, generated by dry distilling coal to produce coke, and retaining high temperature sensible heat near at 800 deg.C at a nascent time, comprises introducing a catalytic cracking reaction into a heavy hydrocarbon accompanied with the high temperature gas to convert the heavy hydrocarbon into light-duty chemical energy as an effectively utilizing technique of the sensible heat. SOLUTION: The converting method of the heat energy and heavy chemical energy into highly efficient clean light-duty chemical energy and its system comprise passing the crude COG accompanied with the heavy hydrocarbon through a heavy hydrocarbon cracking catalytic reactor, thereby effectively utilizing the sensible heat and converting the heavy hydrocarbon into light-duty hydrocarbon, demanding ion circumstances, continuously pas the resultant product through an oxide ion and electron mixing conductive solid electrolyte membrane type reactor, and practically using oxygen permselective performance of the solid electrolyte membrane to convert into a synthesis gas due to partial oxidation modification.
摘要翻译：要解决的问题：提供一种新的热能回收技术和节能系统，以及一种新能源创新系统，鉴于目前的状况，由于通过喷洒氨水进行淬火处理，不能有效地使用显热，尽管焦炭炉气体包括煤挥发物质作为主要成分，通过干蒸馏生成焦炭产生，并在新生时在800摄氏度附近保持高温显热，包括将催化裂化反应引入伴随着高温气体的重质烃将有效利用显热技术将重质烃转化成轻负荷的化学能。解决方案：将热能和重化学能转换为高效清洁轻型化学能及其系统，包括使重质烃伴随着重质烃通过重质烃裂化催化反应器，有效利用显热和将重质烃转化为轻质烃，要求离子环境，通过氧化物离子和电子混合导电固体电解质膜型反应器连续吸收所得产物，实际使用固体电解质膜的氧选择性转化为合成气由于部分氧化改性。

3. 发明专利

JP2006298664A Solid electrolyte membrane-type reactor 有权
标题翻译：固体电解膜型反应器
公开(公告)号：JP2006298664A
公开(公告)日：2006-11-02
申请号：JP2005118794
申请日：2005-04-15
申请人： Nippon Steel Corp , Teikoku Oil Co Ltd , 帝国石油株式会社 , 新日本製鐵株式会社
发明人： ITO WATARU , SAKON TADASHI , HIRANO KENJI , NAGAI TORU , KURIMURA HIDEKI , YAMAZAKI TOSHINORI
IPC分类号： C01B3/38 , B01D53/22 , B01D69/10
CPC分类号： Y02P20/52
摘要： PROBLEM TO BE SOLVED: To provide a supporting membrane-type membrane-type reactor having a new structure which provides gas species having high utilization value, such as synthesis gases, by a high efficiency chemical conversion reaction by employing a structure for eliminating the influence of the gas diffusion in a porous support. SOLUTION: The solid electrolyte membrane-type reactor has reaction structure of a three layer structure comprising a porous support 1, a dense layer 2 comprising an oxygen ion-electron mixed conductive solid electrolyte formed on the support 1, and a catalyst layer 3 formed on the dense layer 2, wherein a gas 4 to be treated containing a hydrocarbon as main component is supplied onto the surface of the catalyst layer 3 and a high purity oxygen gas 5 is supplied onto the surface of the porous support 1 side, respectively. COPYRIGHT: (C)2007,JPO&INPIT
摘要翻译：要解决的问题：提供一种具有新结构的支撑膜型膜型反应器，其通过采用消除结构的方式通过高效率化学转化反应提供诸如合成气体的具有高利用价值的气体种类多孔载体中气体扩散的影响。解决方案：固体电解质膜型反应器具有包括多孔载体1的三层结构的反应结构，包含形成在载体1上的氧离子电子混合导电固体电解质的致密层2和催化剂层 3，其中将含有烃作为主要成分的待处理气体4供应到催化剂层3的表面上，并将高纯度氧气5供应到多孔载体1侧的表面上，分别。版权所有（C）2007，JPO＆INPIT

4. 发明专利

JP2004277256A Ceramic composition, composite material, oxygen separation apparatus, and chemical reaction apparatus 有权
标题翻译：陶瓷组合物，复合材料，氧分离装置和化学反应装置
公开(公告)号：JP2004277256A
公开(公告)日：2004-10-07
申请号：JP2003074090
申请日：2003-03-18
申请人： Nippon Steel Corp , Teikoku Oil Co Ltd , 帝国石油株式会社 , 新日本製鐵株式会社
发明人： NAGAI TORU , ITO WATARU , HIRANO KENJI , SAKON TADASHI , KURIMURA HIDEKI , KAGANOI SHOICHI , SUZUKI YOHEI , ITO TAKASHI
IPC分类号： C04B35/00 , C04B35/495 , H01B1/06
摘要： PROBLEM TO BE SOLVED: To provide a ceramic composition having excellent oxygen permeability, a composite material of a mixed conductor dense continuous layer and a porous supporting body using the ceramic composition and an oxygen separation apparatus and a chemical reaction apparatus in an industrial selective permeation/separation process for oxygen by an oxide ion mixed conductor and a partial oxidation process of hydrocarbon. SOLUTION: The ceramic composition is the oxide ion mixed conductor substantially having perovskite type crystalline structure and expressed by a composition formula, [(Ba x Sr 1-x )α(Co 1-y Fe y )O 3- δ]. There 0.5≤x≤0.65, 0.9≤α≤1.1, 0.075≤y≤0.125 and (δ) is a value fixed to satisfy an electric charge neutralization condition. The composite material contains the porous supporting part and/or the dense continuous layer using the ceramic composition. The oxygen separation apparatus and the chemical reaction apparatus have the ceramic composition and/or the composite material. COPYRIGHT: (C)2005,JPO&NCIPI
摘要翻译：要解决的问题：提供一种具有优异的氧气渗透性的陶瓷组合物，混合导体致密连续层的复合材料和使用该陶瓷组合物的多孔支撑体以及工业上的氧分离装置和化学反应装置通过氧化物离子混合导体对氧的选择性渗透/分离方法和烃的部分氧化方法。解决方案：陶瓷组合物是基本上具有钙钛矿型结晶结构并由组成式表示的氧化物离子混合导体[（Ba x Sr 1-x ） α（共 1-Y 铁ý）O 3 - δ。 0.5≤x≤0.65,0.9≤α≤1.1,0.075≤y≤0.125，（δ）为满足电荷中和条件的固定值。复合材料包含使用陶瓷组合物的多孔支撑部分和/或致密的连续层。氧分离装置和化学反应装置具有陶瓷组合物和/或复合材料。版权所有（C）2005，JPO＆NCIPI

5. 发明专利

JP2003190792A CATALYZED CERAMIC COMPOSITE MATERIAL AND METHOD FOR PRODUCING SYNTHESIS GAS USING THE SAME 审中-公开
公开(公告)号：JP2003190792A
公开(公告)日：2003-07-08
申请号：JP2002299229
申请日：2002-10-11
申请人： TEIKOKU OIL , NIPPON STEEL CORP
发明人： KURIMURA HIDEKI , KAGANOI SHOICHI , SUZUKI YOHEI , ITO TAKASHI , SAKON TADASHI , ITO WATARU , DONOMAE HITOSHI , NAGAI TORU , HIRANO KENJI
IPC分类号： B01D53/22 , B01D71/02 , B01J23/78 , B01J23/89 , C01B3/40 , C01G49/00 , C01G51/00
摘要： PROBLEM TO BE SOLVED: To provide a catalyzed ceramic composite material preferable for a diaphragm which is utilized for inexpensively and stably producing synthesis gas with a high energy efficiency for a long time using gas containing air and methane as a raw material and has a structure in which a dense oxygen permselective ceramic film is integrally formed with a methane reforming catalytic layer. SOLUTION: The catalyzed ceramic composite material is characterized by the structure in which a catalytic part containing Ni and having a catalyst carrier composed mainly of magnesium is adjacent to the first surface of a dense ceramic film having a composition represented by formula (1) [Ln 1-a-b A a B ab ] [B x B' y B" z ]O 3-δ and a perovskite crystalline structure of an oxide ion-electron mixed conductive oxide. COPYRIGHT: (C)2003,JPO

6. 发明专利

JP2000054852A GAS TURBINE COMBINED CYCLE POWER GENERATION SYSTEM 失效
公开(公告)号：JP2000054852A
公开(公告)日：2000-02-22
申请号：JP7751699
申请日：1999-03-23
申请人： NIPPON STEEL CORP , TEIKOKU OIL
发明人： JITSUHARA IKUO , KUBO YUJI , KANEDA YOSHIHIRO , FUJIMOTO KENICHIRO , KURIMURA HIDEKI , KAGANOI SHOICHI
IPC分类号： F01K23/10 , F02C3/22 , F02C6/18
摘要： PROBLEM TO BE SOLVED: To amplify both enthalpy and exergy and reduce the exergy loss in combustion process by connecting a steam reforming system of fuel to a combustor. SOLUTION: A combustor is connected to an air compressor, and a gas turbine is connected to the combustor to connect a methanol steam reforming reactor to the combustor through the gas turbine. A part of the exhaust steam 12 of a high-pressure steam turbine is supplied to the steam reforming reactor together with methanol, and a reaction heat is also supplied by use of the heat of the exhaust gas 6 of the gas turbine. The steam reforming reactor converts all the methanol is converted to hydrogen and carbon dioxide at about 250 deg.C in the steam reforming reactor, and the methanol steam reformed gas is mixed with natural gas in a mixer and then supplied to the combustor to provide a combustion gas of 1450 deg.C or higher.

7. 发明专利

JPH11350972A GAS TURBINE COMBINED CYCLE POWER GENERATION SYSTEM 失效
公开(公告)号：JPH11350972A
公开(公告)日：1999-12-21
申请号：JP15790598
申请日：1998-06-05
申请人： NIPPON STEEL CORP , TEIKOKU OIL
发明人： JITSUHARA IKUO , KANEDA YOSHIHIRO , KUBO YUJI , KURIMURA HIDEKI , KAGANOI SHOICHI
IPC分类号： F01K23/10 , F02C3/20 , F02C6/14 , F02C6/18 , F02C9/40
摘要： PROBLEM TO BE SOLVED: To reduce the amount of fuel used as compared to when natural gas is used as fuel and enable the reduction of carbon dioxide emissions by converting natural gas into synthesis gas through partial oxidation to produce liquid fuel from the synthesis gas and further reforming the liquid fuel with steam to obtain a gas containing mainly hydrogen, and supplying this gas. SOLUTION: A solid electrolyte film is used as a natural gas partial oxidation reactor. Natural gas is passed 8 to a low pressure side of a solid electrolyte film type reactor, and synthesis gas is generated by reaction of methane, which is a major component of natural gas, and permeated oxygen. The generated synthesis gas is introduced 9 into a methanol reaction tower after heat exchange and pressure rise. Methanol is mixed 11, 12 with exhaust steam of a steam turbine, and then introduced into a steam reformer to be converted into hydrogen. The hydrogen-rich gas is introduced 13 to a burner as fuel. The fuel gas is then used for driving a gas turbine, or the like.

8. 发明专利

JP2005288259A Catalyst for reforming methane-containing gas and method for manufacturing synthetic gas 审中-公开
标题翻译：用于改造含甲烷气体的催化剂和制造合成气的方法
公开(公告)号：JP2005288259A
公开(公告)日：2005-10-20
申请号：JP2004105009
申请日：2004-03-31
申请人： National Institute Of Advanced Industrial & Technology , Teikoku Oil Co Ltd , 帝国石油株式会社 , 独立行政法人産業技術総合研究所
发明人： KURIMURA HIDEKI , KAGANOI SHOICHI , YAMAZAKI TOSHINORI , ITO TAKASHI , HAYAKAWA TAKASHI , INABA MIEKO , ANDREI TSUIGANOKU
IPC分类号： B01J23/46
摘要： PROBLEM TO BE SOLVED: To produce an inexpensive and high-performance catalyst used in a reforming reaction of a methane-containing gas, and to provide a method for manufacturing a synthetic gas using the same.
SOLUTION: The method comprises manufacturing the synthetic gas using the catalyst for reforming of the methane-containing gas produced by sintering a hydrotalcite-like layered compound represented by the formula (I); [(M(II)
2+ )
1-x (M(III)
3+ )
x (OH
- )
2 ]
x+ [(A
n- )
x/n ].mH
2 O (I) (wherein M(II)
2+ is Mg
2+ alone or a combination of Mg
2+ with Ni
2+ , Co
2+ , Zn
2+ , Cr
2+ or Fe
2+ ; M(III)
3+ is Al
3+ alone or a combination of Al
3+ with Co
3+ , Cr
3+ or Fe
3+ ; the sum of ions other than Mg
2+ and Al
3+ is 30.0 mol% or lower based on the total of the metal cations; (x) is ≥0.24 and ≤0.33; A
n- are n-valent anions present between layers and on surfaces of the layered compound; and at least a part of A
n- ions is anions derived from an organic metal complex of Ru, Pt, Pd, Rh or Ir).
COPYRIGHT: (C)2006,JPO&NCIPI
摘要翻译：要解决的问题：为了生产用于含甲烷气体的重整反应中使用的便宜且高性能的催化剂，并提供使用该催化剂制造合成气体的方法。解决方案：该方法包括使用通过烧结由式（I）表示的类水滑石层状化合物制备的含甲烷气体的重整用催化剂来制造合成气体; [（M（II） 2 + ） 1-x （M（III） 3 + ） X （ OH - ） 2 ] X + [（A N - ） X / N ]其中M（II） 2 + 单独使用Mg或SP + 2 + ，具有Ni 2 + ，Co 2 + ，Zn 2 + ，Cr 2 + 或Fe 2 + ; M（III） 3 + 是单独的A1 3 + 或Al 3 + > Co 3 + ，Cr 3 + 或Fe 3 + ; Mg以外的离子之和 2 + 并且Al 3 + 基于金属阳离子的总量为30.0mol％或更低;（x）≥0.24和≤0.33; A n - 存在于层之间和层状化合物的表面上的价阴离子;并且至少一部分A n - / SP>离子是衍生自Ru，Pt，Pd，Rh或Ir的有机金属络合物的阴离子）。版权所有（C）2006，JPO＆NCIPI

9. 发明专利

JP2003117395A CATALYST FOR REFORMING AND PRODUCTION METHOD OF SYNTHETIC GAS USING THE SAME 审中-公开
公开(公告)号：JP2003117395A
公开(公告)日：2003-04-22
申请号：JP2001316662
申请日：2001-10-15
申请人： TEIKOKU OIL , NAT INST OF ADV IND & TECHNOL
发明人： KURIMURA HIDEKI , KAGANOI SHOICHI , SUZUKI YOHEI , ITO TAKASHI , HAYAKAWA TAKASHI , HAMAKAWA SATOSHI
IPC分类号： C01B3/40 , B01J23/889
摘要： PROBLEM TO BE SOLVED: To provide a catalyst material for reforming hydrocarbon which enables not only the suppression of carbon deposition for minimizing a amount of a reformer changed but also catalytic reductive control and reaction control for a compound contacting with the catalyst, and a production method of synthetic gas using the same. SOLUTION: This catalyst for reforming consists of a multiplex oxide of which the composition is represented by the following formula and the crystalline structure is a perovskite type and, therein, B, B' and Co are highly dispersed in the multiple oxide: XYa Cob Zc Z'd O3-δ , wherein, 0

10. 发明专利

JP2002085946A CERAMIC MEMBRANE-TYPE REACTOR AND METHOD OF PRODUCING HYDROGEN AT LOW PRESSURE USING THE SAME 失效
公开(公告)号：JP2002085946A
公开(公告)日：2002-03-26
申请号：JP2000284648
申请日：2000-09-20
申请人： TEIKOKU OIL , DALIAN CHEMICAL PHYSICS INST
发明人： KURIMURA HIDEKI , KAGANOI SHOICHI , SUZUKI YOHEI , YO ISHIN
IPC分类号： B01D71/02 , B01D53/22 , B01J19/00 , B01J23/78 , C01B3/38 , C01B3/48 , C04B35/00 , H01M8/06
摘要： PROBLEM TO BE SOLVED: To provide a technique related to an oxygen-permeable ceramic membrane-type reactor, by which a gas containing hydrogen as a main component is stably, efficiently and inexpensively produced under low pressure conditions using gaseous light hydrocarbons and air as raw materials. SOLUTION: A perovskite-type oxide, BaxSr1-xCoyFe1-yO3-δ(wherein, x=0.3 to 0.7 and y=0.6 to 1.0) having a high permeability to oxygen and being highly stable is used as a dense ceramic membrane material selectively permeable to oxygen. As a catalyst for partially oxidizing light hydrocarbons, a catalyst having a composition expressed by formula: Nix/CaySr1-yTiO3 (wherein, x=0.1 to 0.3 and y=0.8 or 0.0) or Nix/BaTiO3 (wherein, x=0.1 to 0.3) or a catalyst obtained by loading rhodium, platinum or ruthenium to the catalyst mentioned above in an amount of 0.1 to 1,000 ppm by weight, based on the weight of the catalyst, is used. At the upstream region of the stream of gaseous raw materials, the catalyst is arranged flatly against the ceramic membrane, and at the downstream region, the catalyst is arranged stereoscopically against the ceramic membrane.

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