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1. 发明专利

JP2004261771A Unsupported catalyst for directly decomposing hydrocarbon, production method thereof and production method of hydrogen and carbon by directly decomposing hydrocarbon 有权
公开(公告)号：JP2004261771A
公开(公告)日：2004-09-24
申请号：JP2003057240
申请日：2003-03-04
申请人： Japan Steel Works Ltd:The , Kajima Corp , Asao Tada , 旭男多田 , 株式会社日本製鋼所 , 鹿島建設株式会社
发明人： NAKAMURA SATOSHI , TADA ASAO , TOGO YOSHITAKA , KOSEKI KIKUO
IPC分类号： C01B3/26 , B01J23/755 , C01B31/02
摘要： PROBLEM TO BE SOLVED: To provide a catalyst maintaining stable performance with respect to the decomposition of hydrocarbons for a long period of time without requiring a carrier. SOLUTION: The catalyst is prepared by activating a catalyst metal precursor in a non-oxidizing atmosphere, preferably in the atmosphere of inert gas or a hydrocarbon gas by heating in a range of temperature of 200-1,000°C. The catalyst is interposed by carbon particles between catalyst metal particles without being carried by the carrier. The hydrocarbons are directly decomposed by bringing the catalyst prepared by the activation into contact with the catalyst at 200-1,000°C. The prevention of aggregation of the catalyst metal particles by generation of carbon between them enables the catalyst performance to maintain for a long period of time to obtain high purity carbon not-containing the catalyst carrier. The catalyst is prepared without requiring the carrier to be produced at a low cost. COPYRIGHT: (C)2004,JPO&NCIPI

2. 发明专利

JP2005058908A Catalyst, reactor and reaction apparatus for directly cracking lower hydrocarbon 有权
标题翻译：催化剂，反应器和反应装置直接破碎下层烃
公开(公告)号：JP2005058908A
公开(公告)日：2005-03-10
申请号：JP2003292342
申请日：2003-08-12
申请人： Japan Steel Works Ltd:The , Kajima Corp , Noritake Co Ltd , Asao Tada , 旭男多田 , 株式会社ノリタケカンパニーリミテド , 株式会社日本製鋼所 , 鹿島建設株式会社
发明人： NAKAMURA SATOSHI , ITO HIDEAKI , TADA ASAO , TOGO YOSHITAKA , IWATA MISAO , KATO SHINJI , TAKASAGO HIROYUKI
IPC分类号： C01B3/26 , B01J23/755 , B01J35/04 , C01B31/02 , H01M8/06
CPC分类号： Y02E60/50
摘要： PROBLEM TO BE SOLVED: To eliminate such a weak point that carbon is made to grow by a porous catalyst and the grown carbon increases pressure loss or a gas passage is blocked by a vessel when a lower hydrocarbon such as methane is directly cracked by using the porous catalyst to produce hydrogen and carbon. SOLUTION: The catalyst is obtained by depositing a catalytic material on a porous carrier and used for producing high-purity hydrogen and nano-size functional carbon by directly cracking the lower hydrocarbon. The carrier has such a function that the carrier is expanded/deformed analogously by the accumulation of the carbon produced by the direct cracking reaction to restrain the increase of the pressure loss and the clogging. When this catalyst is used, methane, or the like, can be reformed stably for a long time and a small-sized domestic fuel cell system from the process of which CO 2 is not discharged can be manufactured. COPYRIGHT: (C)2005,JPO&NCIPI
摘要翻译：要解决的问题：为了消除碳被多孔催化剂生长的这样的弱点，并且当甲烷等低级烃直接破裂时，生长的碳增加压力损失或气体通道被容器阻塞通过使用多孔催化剂来产生氢和碳。解决方案：通过在多孔载体上沉积催化材料并通过直接裂解低级烃来生产高纯度氢和纳米尺寸的功能性碳来获得催化剂。载体具有通过由直接裂化反应产生的碳的积累类似地使载体膨胀/变形的功能，以抑制压力损失和堵塞的增加。当使用这种催化剂时，可以长时间稳定地重整甲烷等，并且可以制造从不排放CO 2的过程的小型家用燃料电池系统。版权所有（C）2005，JPO＆NCIPI

3. 发明专利

JP2008183560A Carrier-free hydrocarbon direct decomposition catalyst 有权
标题翻译：无载体碳氢化合物直接分解催化剂
公开(公告)号：JP2008183560A
公开(公告)日：2008-08-14
申请号：JP2008104049
申请日：2008-04-11
申请人： Japan Steel Works Ltd:The , Kajima Corp , Asao Tada , 旭男多田 , 株式会社日本製鋼所 , 鹿島建設株式会社
发明人： NAKAMURA SATOSHI , TADA ASAO , TOGO YOSHITAKA , KOSEKI KIKUO
IPC分类号： B01J23/70
摘要： PROBLEM TO BE SOLVED: To provide a catalyst that maintains a stable performance with regard to the decomposition of hydrocarbons over a long time without a carrier. SOLUTION: A catalytic metal precursor is heated in the temperature range of 200 to 1,000°C to be activated under a non-oxidizing atmosphere and preferably, under an inert gas or hydrocarbon gas to obtain a catalyst. The catalyst is not supported by a carrier and carbon particles are interposed between catalytic metal particles. The hydrocarbon is allowed to contact the catalyst obtained by the activation at 200 to 1,000°C to perform direct decomposition on the hydrocarbon. Carbons are produced between the catalytic metal particles to prevent the flocculation of the catalytic metal particles and this allows a catalyst performance to be maintained for a long time, thereby enabling the system to obtain a high purity-carbon containing no catalyst carrier. The catalyst can be obtained without any carrier, thereby enabling the system to manufacture the catalyst at a low cost. COPYRIGHT: (C)2008,JPO&INPIT
摘要翻译：待解决的问题：提供一种在没有载体的情况下长时间保持烃的分解的稳定性能的催化剂。解决方案：将催化金属前体在200-1000℃的温度范围内加热，以在非氧化性气氛下，优选在惰性气体或烃气体下活化，得到催化剂。催化剂不被载体负载，碳颗粒介于催化金属颗粒之间。允许烃在200至1000℃下与通过活化获得的催化剂接触以对烃进行直接分解。在催化金属颗粒之间产生碳以防止催化金属颗粒的絮凝，并且这允许长时间保持催化剂性能，从而使得该体系可以获得不含催化剂载体的高纯度碳。可以在没有任何载体的情况下获得催化剂，从而能够以低成本制造催化剂。版权所有（C）2008，JPO＆INPIT

4. 发明专利

JP2006043645A Catalyst for direct decomposition of lower hydrocarbon 有权
标题翻译：催化剂用于低碳氢化合物的直接分解
公开(公告)号：JP2006043645A
公开(公告)日：2006-02-16
申请号：JP2004231736
申请日：2004-08-06
申请人： Japan Steel Works Ltd:The , Kajima Corp , Asao Tada , 旭男多田 , 株式会社日本製鋼所 , 鹿島建設株式会社
发明人： TADA ASAO , TOGO YOSHITAKA , TAKASAGO HIROYUKI , NAKAMURA SATOSHI , ITO HIDEAKI
IPC分类号： B01J23/745 , C01B3/26 , C01B31/02 , H01M8/06
CPC分类号： Y02E60/50
摘要： PROBLEM TO BE SOLVED: To provide a catalyst for direct decomposition of lower hydrocarbon which is friendly to environment and is economical. SOLUTION: The catalyst for direct decomposition of lower hydrocarbon is prepared by depositing iron on a surface of a carrier consisting essentially of silica (SiO 2 ) via covering of non-ferrous metal oxide. For example, after the carrier consisting essentially of silica is impregnated with a non-ferrous metal salt solution and then is dried and calcined, the carrier is impregnated with the mixed solution of the non-ferrous metal salt and an iron salt and then is dried and calcined. Preferably the non-ferrous metal oxide is alumina (Al 2 O 3 ). More preferably foamed glass is used as the carrier consisting essentially of silica. The foamed glass can be obtained as a bulk phase porous body, for example, by adding a foaming agent to pulverized matter of waste glass and performing melting and foaming. The foamed glass having higher ratio of continuous air pores compared to closed cells is desirable. COPYRIGHT: (C)2006,JPO&NCIPI
摘要翻译：要解决的问题：提供一种直接分解对环境友好且经济的低级烃的催化剂。解决方案：通过覆盖有色金属氧化物，通过在基本上由二氧化硅（SiO 2 SB 2）组成的载体的表面上沉积铁来制备用于直接分解低级烃的催化剂。例如，在基本上由二氧化硅组成的载体用非铁金属盐溶液浸渍之后，将其干燥和煅烧，用非铁金属盐和铁盐的混合溶液浸渍载体，然后干燥并煅烧。优选地，有色金属氧化物是氧化铝（Al 2 SB 3 O 3 / SB 3）。更优选使用泡沫玻璃作为主要由二氧化硅组成的载体。作为体相多孔体，例如可以通过在废玻璃的粉碎物中添加发泡剂，进行熔融发泡而得到发泡玻璃。与闭孔相比，具有较高连续空气孔率的泡沫玻璃是理想的。版权所有（C）2006，JPO＆NCIPI

5. 发明专利

JP2006096590A Apparatus for directly cracking lower hydrocarbon 有权
标题翻译：直接破碎下层油料的装置
公开(公告)号：JP2006096590A
公开(公告)日：2006-04-13
申请号：JP2004282763
申请日：2004-09-28
申请人： Japan Steel Works Ltd:The , Kajima Corp , Asao Tada , 旭男多田 , 株式会社日本製鋼所 , 鹿島建設株式会社
发明人： TADA ASAO , TOGO YOSHITAKA , TAKASAGO HIROYUKI , NAKAMURA SATOSHI , ITO HIDEAKI
IPC分类号： C01B3/26 , B01J23/94 , B01J38/00 , C01B3/02
CPC分类号： Y02P20/584
摘要： PROBLEM TO BE SOLVED: To provide an apparatus for directly cracking lower hydrocarbons capable of continuously removing hydrogen and solid carbon. SOLUTION: A heat resistant coil-shaped reaction tube 2 is heated by a heating means 10 to a cracking reaction temperature. A lower hydrocarbon gas M (for example, methane gas) and a catalyst powder T for direct cracking reaction of the hydrocarbon are concurrently delivered from a delivery apparatus 20 to one end 3 of the reaction tube 2. A generated cracking gas (for example, hydrogen) and the catalyst powder T discharged from the other end 5 of the reaction tube 2 are separated in a separating apparatus 30. The delivery apparatus 20 comprises a blower 21 for injecting the lower hydrocarbon gas flow M and a catalyst charging device 22 for mixing the catalyst powder T into the gas flow M from the blower 21. The catalyst powder T separated in the separating apparatus 30 is returned back to the catalyst charging device 22. The separating apparatus 30 comprises an unreacted gas-separating apparatus 34 for separating the generated cracking gas from the unreacted low hydrocarbon gas M. The unreacted gas M separated in the unreacted gas-separating apparatus 34 is returned back to the blower 21 or to the gas flow M. The heating means 10 is mounted so that it is aligned with the central axis of the coil-shaped reaction tube 2. COPYRIGHT: (C)2006,JPO&NCIPI
摘要翻译：要解决的问题：提供一种用于直接裂解能够连续除去氢和固体碳的低级烃的装置。解决方案：将耐热线圈形反应管2通过加热装置10加热到裂化反应温度。烃的直接裂解反应的低级烃气体M（例如甲烷气体）和催化剂粉末T从输送装置20同时输送到反应管2的一端。产生的裂解气体（例如，氢），从反应管2的另一端5排出的催化剂粉末T在分离装置30中分离。输送装置20包括用于喷射下部烃类气体流M的鼓风机21和用于混合的催化剂填充装置22 催化剂粉末T进入来自鼓风机21的气流M.在分离装置30中分离的催化剂粉末T返回到催化剂装料装置22.分离装置30包括未反应气体分离装置34，用于将产生的从未反应的低碳氢化合物气体M中裂解气体。未反应气体分离装置34中分离的未反应气体M返回到鼓风机21或气流加热装置10安装成使其与线圈形反应管2的中心轴线对准。版权所有（C）2006，JPO＆NCIPI

6. 发明专利

JP2006290682A Method and catalyst reactor for producing nano-carbon 有权
标题翻译：用于生产纳米碳的方法和催化剂反应器
公开(公告)号：JP2006290682A
公开(公告)日：2006-10-26
申请号：JP2005114302
申请日：2005-04-12
申请人： Japan Steel Works Ltd:The , Kajima Corp , Kitami Institute Of Technology , 国立大学法人北見工業大学 , 株式会社日本製鋼所 , 鹿島建設株式会社
发明人： TADA ASAO , NAKAMURA SATOSHI , NAKAMURA TETSUSHIGE , KAKIHARA HAJIME , TOGO YOSHITAKA , KOSEKI KIKUO , TAKASAGO HIROYUKI
IPC分类号： C01B31/02 , B01J8/08
CPC分类号： C01B31/02 , B01J6/008 , B01J8/10 , B01J19/20 , B01J35/02 , B01J2208/00867 , B82Y30/00 , C01B3/26 , C01B32/05 , C01B32/15 , C01B32/164 , C01B2203/04 , C01B2203/1047 , C01B2203/1058 , Y10S977/842 , Y10S977/843
摘要： PROBLEM TO BE SOLVED: To continuously and stably produce nano-carbon by a catalytic reaction using lower hydrocarbons as raw materials.
SOLUTION: The catalyst reactor has a screw feeder body 1a being a pressure reactor, a catalyst feeding parts 5,6,7 for introducing a catalyst 20 into the feeder body 1a, a lower hydrocarbon feeding parts 3, 4 for introducing the lower hydrocarbons into the feeder body 1a, a screw 1b for transporting the catalyst and the nano-carbon formed by the thermal decomposition of the lower hydrocarbons in the feeder body 1a, a solid sending-out part 10 for sending out the catalyst and the nano-carbon transported by the screw 1b to the outside of the feeder body 1a, and a gas sending-out part 11 for sending out unreacted lower hydrocarbons and hydrogen formed by the thermal decomposition to the outside of the feeder body 1a. The continuous reaction is performed efficiently at a constant conversion ratio by continuously discharging the nano-carbon growing with the elapse of time and used catalyst to the outside of the reactor and feeding the same amount of a virgin catalyst as that of the used catalyst.
COPYRIGHT: (C)2007,JPO&INPIT
摘要翻译：要解决的问题：通过使用低级烃作为原料的催化反应来连续稳定地制造纳米碳。解决方案：催化剂反应器具有作为压力反应器的螺旋进料器主体1a，用于将催化剂20引入进料器主体1a的催化剂供给部5,6,7，用于引入低级烃进入给料体1a，用于输送催化剂的螺杆1b和通过进料器主体1a中的低级烃的热分解形成的纳米碳，用于送出催化剂和纳米级的固体发出部分10 通过螺杆1b输送到供给体1a的外部的气体输送部11和用于将未反应的低级烃和通过热分解形成的氢排出到供给体1a的外部的气体输出部11。通过将经过时间的纳米碳生长和使用的催化剂连续排出到反应器的外部并进料与使用的催化剂相同量的原始催化剂，以恒定的转化率进行连续反应。版权所有（C）2007，JPO＆INPIT

7. 发明专利

JP2006315891A Method of manufacturing functional nanocarbon and hydrogen by direct decomposition of lower hydrocarbon 有权
标题翻译：低碳氢化合物直接分解制备功能纳米碳和氢的方法
公开(公告)号：JP2006315891A
公开(公告)日：2006-11-24
申请号：JP2005138675
申请日：2005-05-11
申请人： Japan Steel Works Ltd:The , Kajima Corp , Kitami Institute Of Technology , 国立大学法人北見工業大学 , 株式会社日本製鋼所 , 鹿島建設株式会社
发明人： TADA ASAO , NAKAMURA SATOSHI , ITO HIDEAKI , TOGO YOSHITAKA , KOSEKI KIKUO , TAKASAGO HIROYUKI
IPC分类号： C01B31/02 , B01J23/745 , B01J23/755 , C01B3/26
CPC分类号： D01F9/127 , B01J23/745 , B01J23/75 , B01J23/755 , B01J23/8906 , B01J23/892 , B82Y30/00 , C01B3/26 , C01B32/15 , C01B2203/06 , C01B2203/1047 , Y10S977/891
摘要： PROBLEM TO BE SOLVED: To prevent reduction in conversion rate with time in the manufacture of hydrogen and nanocarbon by the direct decomposition of a lower hydrocarbon using a catalyst. SOLUTION: In a reaction of obtaining the functional nanocarbon and hydrogen by the direct decomposition of the lower hydrocarbon 4 using the catalyst 1, a gas 9 obtained by allowing a low concentration oxidizing gas, reducing gas or the mixture thereof to coexist with the lower hydrocarbon is used. A precursor of the functional nanocarbon or amorphous carbon of a by-product produced on the catalyst by the reaction reacts with the coexisting gas to be removed from the catalyst and then, the inhibition of the reaction and the reduction in conversion rate with time due to the precursor or the by-product are prevented. When the raw material of the lower hydrocarbon is a bio-gas, the coexisting gas is easily mixed in the methane by lowering the refining degree of the methane and hydrogen is obtained as one of decomposition products of the lower hydrocarbon and is added in the re-reaction. COPYRIGHT: (C)2007,JPO&INPIT
摘要翻译：要解决的问题：为了防止通过使用催化剂直接分解低级烃来制造氢气和纳米碳的转化率随时间的降低。解决方案：在通过使用催化剂1直接分解低级烃4获得功能性纳米碳和氢的反应中，通过使低浓度氧化气体，还原性气体或其混合物与使用低级烃。通过反应在催化剂上产生的副产物的功能性纳米碳或无定形碳的前体与从催化剂除去的共存气体反应，然后由于由于催化剂而导致的反应的抑制和随时间的转化率的降低可以防止前体或副产物。当低碳氢化合物的原料是生物气体时，通过降低甲烷的精炼度，可以将共存气体容易地混合在甲烷中，并将氢气作为下层烃的分解产物得到，并加入 -反应。版权所有（C）2007，JPO＆INPIT

8. 发明专利

JP2011189347A Method for producing catalyst for directly cracking lower hydrocarbon 有权
标题翻译：生产用于直接破碎下层烃的催化剂的方法
公开(公告)号：JP2011189347A
公开(公告)日：2011-09-29
申请号：JP2011140416
申请日：2011-06-24
申请人： Japan Steel Works Ltd:The , Kajima Corp , Kitami Institute Of Technology , 国立大学法人北見工業大学 , 株式会社日本製鋼所 , 鹿島建設株式会社
发明人： TADA ASAO , NAKAMURA SATOSHI , KOSEKI KIKUO , TOGO YOSHITAKA
IPC分类号： B01J23/745
摘要： PROBLEM TO BE SOLVED: To provide a method for producing a catalyst for directly cracking lower hydrocarbons which can efficiently crack lower hydrocarbons using scrap materials. SOLUTION: An aqueous solution of aluminum chloride that is obtained by dissolving a material of waste aluminum in an aqueous solution of hydrochloric acid is used as a raw material of the catalyst carrier. An aqueous solution of iron chloride or an aqueous solution of iron nitrate that is obtained by dissolving a material of waste iron in an aqueous solution of hydrochloric acid or nitric acid is used as a catalyst raw material. In order to precipitate the aqueous solution of aluminum chloride as aluminum hydroxide by neutralization, an aqueous solution of sodium hydroxide or ammonia is used for filtration. Aluminum hydroxide is separated from an aqueous solution of sodium chloride or an aqueous solution of ammonium chloride. Iron-carrying alumina is obtained by impregnating the separated aluminum hydroxide with the aqueous solution of iron chloride or the aqueous solution of iron nitrate and evaporating the same to dryness. COPYRIGHT: (C)2011,JPO&INPIT
摘要翻译：要解决的问题：提供一种用于直接裂化低级烃的催化剂的方法，其可以使用废料有效地裂解低级烃。溶液：将废铝的材料溶解在盐酸水溶液中而得到的氯化铝水溶液用作催化剂载体的原料。使用通过将废铁的材料溶解在盐酸或硝酸的水溶液中而获得的氯化铁水溶液或硝酸铁水溶液作为催化剂原料。为了通过中和将氢氧化铝中的氯化铝水溶液中和，使用氢氧化钠或氨水溶液进行过滤。将氢氧化铝与氯化钠水溶液或氯化铵水溶液分离。通过用氯化铁水溶液或硝酸铁水溶液浸渍分离的氢氧化铝，并将其蒸发至干，得到载铁氧化铝。版权所有（C）2011，JPO＆INPIT

9. 发明专利

JP2011116656A Method and catalytic reactor for producing nano-carbon 有权
标题翻译：用于生产纳米碳的方法和催化反应器
公开(公告)号：JP2011116656A
公开(公告)日：2011-06-16
申请号：JP2011055448
申请日：2011-03-14
申请人： Japan Steel Works Ltd:The , Kajima Corp , Kitami Institute Of Technology , 国立大学法人北見工業大学 , 株式会社日本製鋼所 , 鹿島建設株式会社
发明人： TADA ASAO , NAKAMURA SATOSHI , NAKAMURA TETSUSHIGE , KAKIHARA HAJIME , TOGO YOSHITAKA , KOSEKI KIKUO , TAKASAGO HIROYUKI
IPC分类号： C01B31/02
摘要： PROBLEM TO BE SOLVED: To make it possible to continuously and stably produce nano-carbon by catalytic reaction using lower hydrocarbons as raw materials.
SOLUTION: A catalytic reactor has a screw feeder 1a as a pressure reactor, catalyst feeding parts 5, 6, 7 for introducing a catalyst 20 into the feeder 1a, lower hydrocarbon feeding parts 3, 4 for introducing the lower hydrocarbons into the feeder 1a, a screw 1b for transporting the catalyst and the nano-carbon formed by the thermal decomposition of the lower hydrocarbons in the feeder 1a only by its rotation, a solid sending-out part 10 for sending out the catalyst and the nano-carbon transported by the screw 1b to the outside of the feeder 1a, and a gas sending-out part 11 for sending out unreacted lower hydrocarbons and hydrogen formed by the thermal decomposition to the outside of the feeder 1a. The continuous reaction is performed efficiently at a constant conversion ratio by continuously discharging the nano-carbon growing with the elapse of time and used catalyst to the outside of the reactor and feeding the same amount of a virgin catalyst as that of the used catalyst.
COPYRIGHT: (C)2011,JPO&INPIT
摘要翻译：要解决的问题：通过使用低级烃作为原料的催化反应，可以连续稳定地制造纳米碳。解决方案：催化反应器具有作为压力反应器的螺旋进料器1a，用于将催化剂20引入进料器1a的催化剂进料部分5,6,7，用于将低级烃引入到下部烃进料部分3,4中进料器1a，用于输送催化剂的螺杆1b和通过其进给器1a中的低级烃的热分解形成的纳米碳;固体送出部分10，用于将催化剂和纳米碳通过螺杆1b输送到进料器1a的外部，以及气体输出部11，用于将未反应的低级烃和由热分解形成的氢气送出到进料器1a的外部。通过将经过时间的纳米碳生长和使用的催化剂连续排出到反应器的外部并进料与使用的催化剂相同量的原始催化剂，以恒定的转化率进行连续反应。版权所有（C）2011，JPO＆INPIT

10. 发明专利

JP2012236727A Method and apparatus for producing nanocarbon 有权
标题翻译：用于生产纳米碳的方法和装置
公开(公告)号：JP2012236727A
公开(公告)日：2012-12-06
申请号：JP2011105267
申请日：2011-05-10
申请人： Japan Steel Works Ltd:The , 株式会社日本製鋼所 , Kitami Institute Of Technology , 国立大学法人北見工業大学
发明人： NAKAMURA SATOSHI , TADA ASAO
IPC分类号： C01B31/02 , C01B3/40 , C01B3/56
CPC分类号： B01J8/24 , B01J8/0045 , B01J8/0055 , B01J8/1818 , B01J8/1827 , B01J8/26 , B01J2208/00504 , B01J2208/00752 , B01J2208/00893 , B82Y30/00 , B82Y40/00 , C01B3/44 , C01B32/15 , C01B32/16 , C01B32/18 , C01B2203/0261 , C01B2203/0405 , C01B2203/0415 , C01B2203/043 , C01B2203/0475 , C01B2203/1047 , C01B2203/1058 , C01B2203/1241 , C01B2203/1247 , C01B2203/142 , D01F9/127 , D01F9/133
摘要： PROBLEM TO BE SOLVED: To provide a method and apparatus for producing a nanocarbon which can mass-produces a nanocarbon while the energy necessary for production is suppressed low, and can suppress the generation amount of carbon dioxide.SOLUTION: By using an apparatus for producing a nanocarbon having a fluid layer reactor 2 in which a fluid catalyst or a fluid catalyst 1 concurrently using a fluid medium is accommodated, and a lower hydrocarbon and oxygen are fed and can be auto-burned, a gas feed part 5 connected to the fluid layer reactor 2 and feeding the lower hydrocarbon and oxygen in the fluid layer rector 2, an exhaust gas path 8 connected to the fluid layer reactor 2 and discharging an exhaust gas in the fluid layer reactor 2 outside, and a replenishing part 2a connected to the fluid layer reactor 2 and replenishing the fluid catalyst or the fluid catalyst 1 concurrently using the fluid medium in the fluid layer reactor 2, and by feeding the lower hydrocarbon and oxygen to the fluid catalyst or the fluid catalyst 1 concurrently using the fluid medium, a fluid layer is formed and the nanocarbon and hydrogen are formed by the decomposition reaction of the lower hydrocarbon accompanied by auto-combustion of the lower hydrocarbon and oxygen.
摘要翻译：解决的问题：提供一种能够大量生产纳米碳的纳米碳的制造方法和装置，同时将生产所需的能量抑制得较低，并且可以抑制二氧化碳的产生量。解决方案：通过使用具有流体层反应器2的纳米碳制造装置，其中容纳有同时使用流体介质的流体催化剂或流体催化剂1，并且进料下部烃和氧，燃烧，连接到流体层反应器2并供给流体层反应器2中的下部烃和氧的气体进料部分5，连接到流体层反应器2并排出流体层反应器中的废气的废气通道8 2和连接到流体层反应器2的补充部分2a并且使用流体层反应器2中的流体介质同时补充流体催化剂或流体催化剂1，并且通过将下部烃和氧气供给流体催化剂或流体催化剂1同时使用流体介质，形成流体层，并且通过下层烃的分解反应形成纳米碳和氢，伴随着t的自燃他降低了碳氢化合物和氧气。版权所有（C）2013，JPO＆INPIT

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