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1. 发明专利

JP2007112687A Metallic silicon based cementing material, bonded product and its manufacturing method 有权
标题翻译：金属硅基烧结材料，粘结产品及其制造方法
公开(公告)号：JP2007112687A
公开(公告)日：2007-05-10
申请号：JP2005308549
申请日：2005-10-24
申请人： Chubu Electric Power Co Inc , Noritake Co Ltd , 中部電力株式会社 , 株式会社ノリタケカンパニーリミテド
发明人： YOKOYAMA MAKIKO , ANDO TAISUKE , TAGUCHI HISATOMI , TSUNODA KOSUKE , NAGAYA SHIGEO , SEO TAKUSHI
IPC分类号： C04B37/00
摘要： PROBLEM TO BE SOLVED: To provide a cementing material which can mutually bond silicon-based ceramics with high heat resistance; and also to provide a bonded product of a silicon-based ceramic having high heat resistance and its manufacturing method. SOLUTION: A sealing agent 56 comprises silicon, as a major component, which is a major constituting element of silicon nitride. When the sealing agent 56 is used for mutually bonding a porous cylinder 12 and an end cap 18, both of which comprise boron nitride, the silicon and nitrogen atoms of the interposing sealing agent 56 disperse with each other to form an integrated part of the object. Further, silicon has a high boiling point and cannot be used as a sealing material all alone. However, when silicon is used with germanium which is solid soluble with silicon and has a boiling point lower than that of silicon, the mixed product such as the sealing agent 56 has a boiling point lowered corresponding to the proportion of the constituents of the mixture. Consequently, both parts comprising boron nitride can be highly air-tightly bonded. COPYRIGHT: (C)2007,JPO&INPIT
摘要翻译：要解决的问题：提供可以将硅基陶瓷相互粘合的高耐热性的固井材料; 并且还提供具有高耐热性的硅基陶瓷的粘结产品及其制造方法。解决方案：密封剂56包括作为主要组分的硅，其是氮化硅的主要组成元素。当密封剂56用于相互粘合多孔圆筒12和端盖18（两者都包括氮化硼）时，中间密封剂56的硅和氮原子彼此分散以形成物体的一体化部分。此外，硅具有高沸点，并且不能单独用作密封材料。然而，当硅与硅固溶并且沸点低于硅的锗一起使用时，诸如密封剂56的混合产物的沸点相应于混合物组分的比例降低。因此，包含氮化硼的两部分可以高度气密地结合。版权所有（C）2007，JPO＆INPIT

2. 发明专利

JP2005199211A Membrane reactor 有权
标题翻译：膜反应器
公开(公告)号：JP2005199211A
公开(公告)日：2005-07-28
申请号：JP2004009799
申请日：2004-01-16
申请人： Chubu Electric Power Co Inc , Noritake Co Ltd , 中部電力株式会社 , 株式会社ノリタケカンパニーリミテド
发明人： ANDO TAISUKE , NAGAYA SHIGEO , FURUMURA SEIJI , WATANABE AKIZO
IPC分类号： C01B3/38 , B01J19/24
摘要： PROBLEM TO BE SOLVED: To provide a membrane reactor in which a porous ceramic membrane is used as a separation membrane, the loss of a raw material is restrained, and consequently, the yield of a product is made high.
SOLUTION: A permeability-controlled portion 52 the gas permeability of which is made lower than that of an ordinary portion 54 on the downstream side by thickening the separation membrane 48 is arranged on the upstream side so that a gas in a first gas passage 42 is restrained from flowing out to a second gas passage 40 on the upstream side where the concentration of a generated gas is comparatively low and the gas in the first gas passage 42 flows out easily to the second gas passage 40 on the downstream side where the concentration of the generated gas becomes higher since the gas permeability on the downstream side is higher than that on the upstream side. As a result, the generated gas can be recovered satisfactorily on the downstream side and the loss of the gaseous raw material can be restrained since the gaseous raw material permeates through the separation membrane on the upstream side so that hydrogen gas can be obtained in high yield.
COPYRIGHT: (C)2005,JPO&NCIPI
摘要翻译：要解决的问题：为了提供使用多孔陶瓷膜作为分离膜的膜反应器，可以抑制原料的损失，从而使产品的收率高。解决方案：通过使分离膜48变厚，使其透气度比下游侧的普通部分54低的渗透率控制部分52设置在上游侧，使得第一气体中的气体通道42被阻止流出到产生气体的浓度相对较低的上游侧的第二气体通道40，并且第一气体通道42中的气体容易地流出到下游侧的第二气体通道40，由于下游侧的气体渗透性高于上游侧的气体渗透性，所以产生的气体的浓度变高。结果，能够在下游侧令人满意地回收产生的气体，并且由于气态原料渗透到上游侧的分离膜，因此能够抑制气体原料的损失，能够高收率地获得氢气。版权所有（C）2005，JPO＆NCIPI

3. 发明专利

JP2005145776A Porous ceramic material, method of manufacturing the same and gas separation module provided with the same 有权
标题翻译：多孔陶瓷材料及其制造方法及其分离模块
公开(公告)号：JP2005145776A
公开(公告)日：2005-06-09
申请号：JP2003387633
申请日：2003-11-18
申请人： Chubu Electric Power Co Inc , Noritake Co Ltd , 中部電力株式会社 , 株式会社ノリタケカンパニーリミテド
发明人： BARAGOPARU N NAIR , ANDO TAISUKE , NAGAYA SHIGEO , FURUMURA SEIJI , WATANABE AKIZO
IPC分类号： B01D71/02 , C04B38/00
摘要： PROBLEM TO BE SOLVED: To provide a porous ceramic material stable at a high temperature particularly exceeding 600°C.
SOLUTION: The porous ceramic material is obtained by thermally decomposing a ceramic precursor polymer having a number average molecular weight of ≥80 and 2 /g, particularly 150 m
2 /g surface area. It is preferable that a film of the porous ceramic material is formed particularly on at least a part of a surface of a supporting body.
COPYRIGHT: (C)2005,JPO&NCIPI
摘要翻译：要解决的问题：提供在特别高于600℃的高温下稳定的多孔陶瓷材料。解决方案：通过将数均分子量为≥80且<1,000，特别是≥500和<1,000的陶瓷前体聚合物热分解并基本上由惰性气体气氛中的Si和C组成而获得多孔陶瓷材料。多孔陶瓷材料基本上由Si和C组成，并且即使在700℃的高温和至少100m 2 SP SP 2下，也具有至少4，特别是至少10的小的氢/氮分离因子。 / g，特别是150m 2 / SP / g表面积。优选地，多孔陶瓷材料的膜特别地形成在支撑体的表面的至少一部分上。版权所有（C）2005，JPO＆NCIPI

4. 发明专利

JP2003010658A Gas separation material, method for producing the same, and reactor 有权
标题翻译：气体分离材料，其制造方法和反应器
公开(公告)号：JP2003010658A
公开(公告)日：2003-01-14
申请号：JP2001201330
申请日：2001-07-02
申请人： Chubu Electric Power Co Inc , Noritake Co Ltd , 中部電力株式会社 , 株式会社ノリタケカンパニーリミテド
发明人： MASE SHIGEKAZU , SUZUKI TAKEHIRO , ANDO TAISUKE , NAGAYA SHIGEO , FURUMURA SEIJI
IPC分类号： B01D71/02 , B01D53/22 , B01D67/00 , B01D69/04 , B01D69/10
摘要： PROBLEM TO BE SOLVED: To provide a reactor that realizes improvement in a gas formation reaction efficiency and to provide a gas separation membrane with which the reactor is provided.
SOLUTION: A gas separation material (36) is the one mainly consisting of a porous support (35) and a ceramic membrane (34) formed on the surface, wherein the ceramic membrane (34) has two parts (34A and 34B) differing from each other in both gas permeability and gas permselectivity, the two parts (34A and 34B) are arranged in such a direction that the gas permeability is decreasing and the gas permselectivity of each part is increasing along a specified direction on the surface of the porous support. The reactor (32) is provided with such a gas separation material as a gas separation module.
COPYRIGHT: (C)2003,JPO
摘要翻译：要解决的问题：提供实现气体形成反应效率提高的反应器，并提供设置反应器的气体分离膜。解决方案：气体分离材料（36）是主要由形成在表面上的多孔载体（35）和陶瓷膜（34）组成的气体分离材料（36），其中陶瓷膜（34）具有两部分（34A和34B）气体渗透性和气体选择性两者中，两部分（34A和34B）沿着气体渗透性降低的方向排列，并且每个部分的气体选择性沿着多孔载体表面上的指定方向增加。反应器（32）设置有气体分离材料作为气体分离模块。

5. 发明专利

JP2007131528A Method for manufacturing non-oxide porous ceramic material 有权
标题翻译：制造非氧化物多孔陶瓷材料的方法
公开(公告)号：JP2007131528A
公开(公告)日：2007-05-31
申请号：JP2006347393
申请日：2006-12-25
申请人： Chubu Electric Power Co Inc , Noritake Co Ltd , 中部電力株式会社 , 株式会社ノリタケカンパニーリミテド
发明人： ANDO TAISUKE , YAMADA SEIJI , TAKAHASHI YOSUKE , TAGUCHI HISATOMI , NAGAYA SHIGEO , FURUMURA SEIJI
IPC分类号： C04B35/591 , B01D39/20 , B01D71/02 , C04B35/565 , C04B35/584 , C04B38/00
摘要： PROBLEM TO BE SOLVED: To provide a method for manufacturing a non-oxide porous ceramic material suitable for being used as a substrate for a ceramic separation membrane or the like at a comparatively low cost. SOLUTION: The method comprises: a process for preparing a shaping material containing a silicon carbide powder and/or a silicon nitride powder, a metallic silicon powder, and an yttrium oxide powder and/or an aluminum oxide powder, where 10-100 pts.mass of the metallic silicon powder to 100 pts.mass of the total of the silicon carbide powder and the silicon nitride powder is added and the yttrium oxide powder and/or the aluminum oxide powder of a quantity corresponding to 2-250 mass% of the content of the metallic silicon powder and not exceeding 20 mass% of the total of the shaping material is added; a process for shaping the shaping material into a specified shape; and a process for reaction-sintering the shaped body comprising the shaping material in a nitriding atmosphere. COPYRIGHT: (C)2007,JPO&INPIT
摘要翻译：待解决的问题：提供一种制造适合用作陶瓷分离膜等的基材的非氧化多孔陶瓷材料的方法，成本较低。解决方案：该方法包括：制备含有碳化硅粉末和/或氮化硅粉末，金属硅粉末和氧化钇粉末和/或氧化铝粉末的成形材料的方法，其中10- 将100质量度的金属硅粉末加入到总共的碳化硅粉末和氮化硅粉末的100个质量份中，加入相当于2-250质量份的氧化钇粉末和/或氧化铝粉末加入金属硅粉的含量％，不超过成形材料总量的20质量％; 将成形材料成形为规定形状的工序; 以及在氮化气氛中将包含成形材料的成形体反应烧结的方法。版权所有（C）2007，JPO＆INPIT

6. 发明专利

JP2006182597A Silicon-based ceramic joining material, joined body and its manufacturing method 审中-公开
标题翻译：硅基陶瓷接合材料，接合体及其制造方法
公开(公告)号：JP2006182597A
公开(公告)日：2006-07-13
申请号：JP2004377466
申请日：2004-12-27
申请人： Chubu Electric Power Co Inc , Noritake Co Ltd , 中部電力株式会社 , 株式会社ノリタケカンパニーリミテド
发明人： YOKOYAMA MAKIKO , TAGUCHI HISATOMI , ANDO TAISUKE , MIYAJIMA KEITA , NAGAYA SHIGEO , WATANABE AKIZO , SEO TAKUSHI
IPC分类号： C04B37/00
摘要： PROBLEM TO BE SOLVED: To provide joining materials where silicon-based ceramics can be mutually joined with high heat resistance, a silicon-based ceramic joined body having high heat resistance and its manufacturing method.
SOLUTION: As the main components of a sealing material 56 are Si and Al which are the main constituent elements of silicon carbide and sintering auxiliary agents, the sealing material 56 intervening between a porous cylinder 12 consisting of silicon carbide and an end cap 18 is unified with a body to be joined by the mutual diffusion of Si, Al and N. Si is difficult to be used independently as the joining material because of its high melting point. When Si is used with Al having lower melting point and making a eutectic with Si, the melting point of the sealing material 56 is lowered corresponding to their mixing rate and then respective members consisting of silicon carbide are joined with high joining strength. As the rate of Si in the sealing material 56 is 90 wt% which is sufficiently high, its melting point is high and almost 1,375°C.
COPYRIGHT: (C)2006,JPO&NCIPI
摘要翻译：要解决的问题：提供具有高耐热性的硅基陶瓷可以相互接合的接合材料，具有高耐热性的硅基陶瓷接合体及其制造方法。解决方案：由于密封材料56的主要成分是作为碳化硅和烧结辅助剂的主要构成元素的Si和Al，所以密封材料56介于由碳化硅组成的多孔圆筒12和端盖 18与由Si，Al和N的相互扩散连接的主体统一。由于其高熔点，Si难以独立地用作接合材料。当Si与具有较低熔点的Al并与Si共晶时，密封材料56的熔点相应于其混合速率降低，然后由碳化硅组成的各个部件以高接合强度接合。由于密封材料56中的Si的比率为足够高的90重量％，所以其熔点高且接近1375℃。版权所有（C）2006，JPO＆NCIPI

7. 发明专利

JP2005081246A Oxygen separation membrane element and production method therefor 有权
标题翻译：氧分离膜元件及其生产方法
公开(公告)号：JP2005081246A
公开(公告)日：2005-03-31
申请号：JP2003316219
申请日：2003-09-09
申请人： Chubu Electric Power Co Inc , Noritake Co Ltd , 中部電力株式会社 , 株式会社ノリタケカンパニーリミテド
发明人： TAKAHASHI YOSUKE , ANDO TAISUKE , NAGAYA SHIGEO , FURUMURA SEIJI , WATANABE AKIZO
IPC分类号： B01D53/22 , B01D69/10 , B01D69/12 , B01D71/02 , C01B13/02 , C04B35/00 , C04B35/495 , C04B35/50 , C04B38/00
摘要： PROBLEM TO BE SOLVED: To provide an oxygen separation membrane element with superior mechanical strengths and oxygen separation performance, and a production method therefor. SOLUTION: In the oxygen separation membrane element, a porous support body is composed of at least two stacked porous layers of different porosities, with the porosity of the stacked porous layers gradually decreasing toward an oxygen separation membrane. Preferably, the difference of the porosities between the adjacent porous layers is within 20%, and the difference of the porosities between the oxygen separation membrane and the porous layer adjacent to the membrane is within 5%. Such layers with different porosities can be produced by controlling the average particle size of raw material powder. COPYRIGHT: (C)2005,JPO&NCIPI
摘要翻译：要解决的问题：提供具有优异的机械强度和氧分离性能的氧分离膜元件及其制备方法。解决方案：在氧分离膜元件中，多孔支撑体由至少两层不同孔隙度的堆叠多孔层组成，堆叠的多孔层的孔隙率朝向氧分离膜逐渐减小。优选地，相邻多孔层之间的孔隙率差在20％以内，氧分离膜与邻近膜的多孔层之间的孔隙度差在5％以内。可以通过控制原料粉末的平均粒径来制造具有不同孔隙率的这些层。版权所有（C）2005，JPO＆NCIPI

8. 发明专利

JP2005041720A Porous ceramic film and method for producing the same 审中-公开
标题翻译：多孔陶瓷膜及其制造方法
公开(公告)号：JP2005041720A
公开(公告)日：2005-02-17
申请号：JP2003201233
申请日：2003-07-24
申请人： Chubu Electric Power Co Inc , Noritake Co Ltd , 中部電力株式会社 , 株式会社ノリタケカンパニーリミテド
发明人： MIYAJIMA KEITA , ANDO TAISUKE , BARAGOPARU N NAIR , NAGAYA SHIGEO , FURUMURA SEIJI , WATANABE AKIZO
IPC分类号： C04B38/00 , C04B41/87
摘要： PROBLEM TO BE SOLVED: To provide a method for stably producing a porous ceramic film substantially free from cracks and defects and to provide a porous ceramic film obtained thereby.
SOLUTION: The method for producing the porous ceramic film comprises a step of applying a ceramic film forming material to the surface of a porous support (14), a step of placing the support (14) to which the material is applied in a specific gaseous atmosphere, and a step of forming the porous ceramic film from the material while permeating the specified gas in the direction of thickness of the support in at least that area of the support (14) to which the material is applied.
COPYRIGHT: (C)2005,JPO&NCIPI
摘要翻译：要解决的问题：提供一种稳定地制造基本上没有裂缝和缺陷的多孔陶瓷膜的方法，并提供由此获得的多孔陶瓷膜。＆lt; P＆gt;解决方案：多孔陶瓷膜的制造方法包括将陶瓷膜形成材料涂布在多孔质体（14）的表面的步骤，将涂布有材料的载体（14）特定的气体气氛，以及至少在所述材料的所述支撑体（14）的所述区域中沿着所述支撑体的厚度方向渗透所述特定气体的同时从所述材料形成所述多孔陶瓷膜的步骤。版权所有（C）2005，JPO＆NCIPI

9. 发明专利

JP2004123416A Method for manufacturing non-oxide-based porous ceramic material consisting essentially of silicon 有权
标题翻译：制造基于非氧化物的多孔陶瓷材料的方法
公开(公告)号：JP2004123416A
公开(公告)日：2004-04-22
申请号：JP2002286830
申请日：2002-09-30
申请人： Chubu Electric Power Co Inc , Noritake Co Ltd , 中部電力株式会社 , 株式会社ノリタケカンパニーリミテド
发明人： ANDO TAISUKE , YAMADA SEIJI , TAKAHASHI YOSUKE , TAGUCHI HISATOMI , NAGAYA SHIGEO , FURUMURA SEIJI
IPC分类号： B01D69/10 , B01D39/00 , B01D39/20 , B01D71/02 , C04B35/565 , C04B35/573 , C04B35/584 , C04B35/591
摘要： PROBLEM TO BE SOLVED: To provide a method for manufacturing a non-oxide-based porous ceramic material suitable for being used as a base material of a ceramic separation membrane or the like relatively at a low cost. SOLUTION: The manufacturing method includes a process of preparing a molding material which contains silicon carbide powder and/or silicon nitride powder, metallic silicon powder and yttrium oxide powder and/or aluminum oxide powder and in which 10-100 pts.mass metallic silicon powder is added to 100 pts.mass in total of silicon carbide powder and silicon nitride powder, and yttrium oxide powder and/or aluminum oxide powder is added in a quantity equivalent to 2-250 mass% of the content of metallic silicon powder and not exceeding 20 mass% of total of the molding material, a process of molding the molding material into a prescribed shape and a process of reacting and sintering the molding composed of the molding material under an atmosphere where nitriding can be carried out. COPYRIGHT: (C)2004,JPO
摘要翻译：要解决的问题：提供一种制造适合用作陶瓷分离膜等的基材的非氧化物基多孔陶瓷材料的方法，其成本相对较低。解决方案：该制造方法包括制备包含碳化硅粉末和/或氮化硅粉末，金属硅粉末和氧化钇粉末和/或氧化铝粉末的成型材料的方法，其中10-100个质点将金属硅粉末加入到总计为100质量份的碳化硅粉末和氮化硅粉末中，并且加入相当于金属硅粉末含量的2-250质量％的氧化钇粉末和/或氧化铝粉末不超过模塑材料总量的20质量％，将成型材料成型为规定形状的工序以及在可进行氮化的气氛下使成型材料成型的成形体进行反应烧结的工序。版权所有（C）2004，JPO

10. 发明专利

JP2009022902A Porous material, method for manufacturing the same, and gas separating device 审中-公开
标题翻译：多孔材料，其制造方法和气体分离装置
公开(公告)号：JP2009022902A
公开(公告)日：2009-02-05
申请号：JP2007189888
申请日：2007-07-20
申请人： Chisso Corp , Chubu Electric Power Co Inc , Noritake Co Ltd , チッソ株式会社 , 中部電力株式会社 , 株式会社ノリタケカンパニーリミテド
发明人： MIYAJIMA KEITA , ANDO TAISUKE , NAGAYA SHIGEO , SEO TAKUSHI , OBA TOMOYUKI
IPC分类号： B01D69/12 , B01D53/22 , B01D71/02 , C01B3/56 , C04B38/00 , C04B41/85
摘要： PROBLEM TO BE SOLVED: To provide a porus material having high and stable characteristics preferably used as a gas separating film, a method for manufacturing the same, and a gas separating device.
SOLUTION: A solution containing polysilazane is coated on the circumferential surface of a porus base material composed of silicon nitride, and a porus film 16 comprising a porus ceramics of amorphous state having bondings such as Si-C, Si-N, Si-O-N and Si-O-C having a pore diameter of about 0.62 nm and a thickness of 100 to 200 nm is subsequently produced by performing calcining treatment. Because a solution with a number average molecular weight within a range of 2,000 to 5,000 g/mol and a viscosity within a range of 20 to 200 mPa s is used as a solution containing poly silazane, the solution can be coated on the surface of an intermediate layer 14 in a proper thickness, to thereby form a porous ceramic film produced by the calcining treatment with a thin thickness of 100 to 200 nm and with a micro pore diameter of about 0.5 to 1.0 nm.
COPYRIGHT: (C)2009,JPO&INPIT
摘要翻译：要解决的问题：提供优选用作气体分离膜的具有高且稳定特性的孔隙材料，其制造方法和气体分离装置。解决方案：将含有聚硅氮烷的溶液涂覆在由氮化硅构成的孔基材的圆周表面上，以及包含非晶状态的具有诸如Si-C，Si-N，Si 通过进行煅烧处理，随后制造孔径为约0.62nm，厚度为100〜200nm的-ON和Si-OC。由于使用数均分子量在2,000〜5,000g / mol范围内且粘度在20〜200mPa·s范围内的溶液作为含有聚硅氮烷的溶液，所以可以将溶液涂布在中间层14以适当的厚度形成多孔陶瓷膜，通过100-200nm厚的微孔直径约0.5-1.0nm的煅烧处理形成多孔陶瓷膜。版权所有（C）2009，JPO＆INPIT

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