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1. 发明授权

EP0128851B1 Poly-diisopropenyl benzene synthesis 有权
标题翻译：聚对二苯乙烯合成
公开(公告)号：EP0128851B1
公开(公告)日：1989-08-23
申请号：EP84630074.7
申请日：1984-05-04
申请人： THE GOODYEAR TIRE & RUBBER COMPANY
发明人： Jalics, George
IPC分类号： C08F12/34 , C08F2/06
CPC分类号： C08F12/34

2. 发明授权

EP0824133B1 Silica-filled rubber compositions and the processing thereof 失效
标题翻译：二氧化硅填充的橡胶组合物以及它们的制备
公开(公告)号：EP0824133B1
公开(公告)日：2003-04-23
申请号：EP97113559.5
申请日：1997-08-06
申请人： THE GOODYEAR TIRE & RUBBER COMPANY
发明人： Jalics, George , Halasa, Adel Farhan , Zanzig, David John
IPC分类号： C08K9/08 , C08L21/00 , C08G83/00 , C08K3/36
CPC分类号： C08C19/44 , C08K9/08 , Y10S152/905 , C08L21/00

3. 发明授权

EP0448902B1 Comb polymers having a halobutyl rubber backbone 失效
标题翻译：具有卤代丁基橡胶主链的梳形聚合物
公开(公告)号：EP0448902B1
公开(公告)日：1996-05-29
申请号：EP90630239.3
申请日：1990-12-18
申请人： THE GOODYEAR TIRE & RUBBER COMPANY
发明人： Jalics, George , Bauer, Richard George
IPC分类号： C08G81/02
CPC分类号： C08G81/021

4. 发明公开

EP0128851A3 Poly-diisopropenyl benzene synthesis 有权
标题翻译：聚对二苯乙烯合成
公开(公告)号：EP0128851A3
公开(公告)日：1986-07-02
申请号：EP84630074
申请日：1984-05-04
申请人： THE GOODYEAR TIRE & RUBBER COMPANY
发明人： Jalics, George
IPC分类号： C08F12/34 , C08F02/06
CPC分类号： C08F12/34
摘要： It has been unexpectedly found that meta-diisopropenyl benzene can be polymerized into poly-m-diisopropenyl benzene with a relatively narrow molecular weight distribution and with only a small degree of crosslinking (gel formation) if done in the presence of at least one alpha-olefin containing from 2 to 12 carbon atoms in tetrahydrofuran (solvent) at low temperatures employing an alkyl lithium initiator. The poly-m-diisopropenyl benzene produced by employing this technique has an isopropenyl moiety on almost every diisopropenyl benzene repeat unit in the polymer. This polymer is particularly useful since its pendant isopropenyl groups can be further reacted with other compounds leading to polymers with various functionalities. This technique can also be employed in the synthesis of copolymers containing repeat units derived from meta-diisopropenyl benzene and one or more other monomers. The copolymers synthesized using the process of this invention contain an essentially quantitative number of unreacted isopropenyl groups on the meta-diisopropenyl benzene repeat units in the polymer chain.

5. 发明公开

EP0824133A1 Silica-filled rubber compositions and the processing thereof 失效
标题翻译：二氧化硅填充的橡胶组合物以及它们的制备
公开(公告)号：EP0824133A1
公开(公告)日：1998-02-18
申请号：EP97113559.5
申请日：1997-08-06
申请人： THE GOODYEAR TIRE & RUBBER COMPANY
发明人： Jalics, George , Halasa, Adel Farhan , Zanzig, David John
IPC分类号： C08K9/08 , C08L21/00 , C08G83/00 , C08K3/36
CPC分类号： C08C19/44 , C08K9/08 , Y10S152/905 , C08L21/00
摘要： The present invention relates to silica-filled rubber compositions and their method of processing. The rubber compositions contain a mixture of 10 to 150 phr of a particulate precipitated silica having dispersed thereon, from 1 to 20 percent by weight based upon the weight of the silica, of a silane-modified elastomer.

6. 发明公开

EP0128851A2 Poly-diisopropenyl benzene synthesis 有权
标题翻译：聚二异丙烯基苯的合成
公开(公告)号：EP0128851A2
公开(公告)日：1984-12-19
申请号：EP84630074.7
申请日：1984-05-04
申请人： THE GOODYEAR TIRE & RUBBER COMPANY
发明人： Jalics, George
IPC分类号： C08F12/34 , C08F2/06
CPC分类号： C08F12/34
摘要： It has been unexpectedly found that meta-diisopropenyl benzene can be polymerized into poly-m-diisopropenyl benzene with a relatively narrow molecular weight distribution and with only a small degree of crosslinking (gel formation) if done in the presence of at least one alpha-olefin containing from 2 to 12 carbon atoms in tetrahydrofuran (solvent) at low temperatures employing an alkyl lithium initiator. The poly-m-diisopropenyl benzene produced by employing this technique has an isopropenyl moiety on almost every diisopropenyl benzene repeat unit in the polymer. This polymer is particularly useful since its pendant isopropenyl groups can be further reacted with other compounds leading to polymers with various functionalities.
This technique can also be employed in the synthesis of copolymers containing repeat units derived from meta-diisopropenyl benzene and one or more other monomers. The copolymers synthesized using the process of this invention contain an essentially quantitative number of unreacted isopropenyl groups on the meta-diisopropenyl benzene repeat units in the polymer chain.
摘要翻译：出乎意料地发现，如果在至少一种α-烯烃存在下进行，则间二异丙烯基苯可聚合成具有相对窄的分子量分布且仅具有小程度的交联（凝胶形成）的聚间二异丙烯基苯，使用烷基锂引发剂在低温下在四氢呋喃（溶剂）中含有2至12个碳原子的烯烃。采用该技术生产的聚间二异丙烯基苯在聚合物中的几乎每个二异丙烯基苯重复单元上都具有异丙烯基部分。这种聚合物是特别有用的，因为其悬挂的异丙烯基可以进一步与其他化合物反应，产生具有各种官能度的聚合物。该技术也可用于合成含有衍生自间二异丙烯基苯和一种或多种其它单体的重复单元的共聚物。使用本发明方法合成的共聚物在聚合物链中的间二异丙烯基苯重复单元上含有基本定量数量的未反应的异丙烯基。

7. 发明公开

EP0095996A2 High green strength emulsion rubbers by the use of half esters of unsaturated dicarboxylic acids 有权
标题翻译：乳液橡胶与由使用的不饱和二羧酸的半酯的高Rohzugfestigkeit。
公开(公告)号：EP0095996A2
公开(公告)日：1983-12-07
申请号：EP83630090.5
申请日：1983-05-20
申请人： THE GOODYEAR TIRE & RUBBER COMPANY
发明人： Jalics, George
IPC分类号： C08F236/04 , C07C69/593
CPC分类号： C08F236/04 , C08F222/00
摘要： The green strength of polymers produced by emulsion polymerization processes is improved through the use of carboxyl containing compounds.
Specifically, the compounds are half esters of unsaturated dicarboxylic acids wherein the half ester moiety renders the carboxyl containing compound hydrophobic. As a result, carboxylic copolymers can be produced in emulsion polymerizations having a basic (pH > 7.0) aqueous medium. Heretofore, use of carboxylic acids in emulsion polymerizations have been limited to acidic mediums.

8. 发明公开

EP0448902A3 Comb polymers having a halobutyl rubber backbone 失效
标题翻译：具有HOBOBUTYL橡胶背面的聚乙烯聚合物
公开(公告)号：EP0448902A3
公开(公告)日：1992-08-12
申请号：EP90630239.3
申请日：1990-12-18
申请人： THE GOODYEAR TIRE & RUBBER COMPANY
发明人： Jalics, George , Bauer, Richard George
IPC分类号： C08G81/02
CPC分类号： C08G81/021
摘要： The subject invention relates to comb polymers having a halobutyl rubber backbone and to techniques for synthesizing such polymers. The comb polymers of this invention can be thermoplastic elastomers. For instance, halobutyl rubbers having sidechains which are derived from vinyl aromatic monomers are thermoplastic elastomers which can be made by a technique of the subject invention. Such thermoplastic elastomers typically have a chlorobutyl rubber backbone and side chains which are comprised of polystyrene. The subject invention more specifically discloses a process for grafting a lithium terminated vinyl aromatic polymer onto a halobutyl rubber which comprises: (1) capping the lithium terminated vinyl aromatic polymer with a diene monomer to produce a lithium terminated diene capped vinyl aromatic polymer, and (2) reacting the lithium terminated diene capped vinyl aromatic polymer with the halobutyl rubber to produce a halobutyl rubber having vinyl aromatic sidechains grafted thereto.

9. 发明公开

EP0217723A3 Siloxane containing network polymer 失效
标题翻译：含硅氧烷的聚合物
公开(公告)号：EP0217723A3
公开(公告)日：1988-08-24
申请号：EP86630136
申请日：1986-09-03
申请人： THE GOODYEAR TIRE & RUBBER COMPANY
发明人： Halasa, Adel Farhan , Jalics, George
IPC分类号： C08C19/44 , C08G77/42
CPC分类号： C08C19/44 , C08F8/42
摘要： Metals from groups I and II are commonly used to catalyze the polymerization of monomers into polymers. The polymers formed in such polymerizations are terminated with the metal used to catalyze the polymerization and are sometimes referred to as living polymers. Such polymers can be crosslinked to produce a polymeric network by utilizing the process of the present invention. More specifically, the present invention discloses a process for endlinking a living polymer comprising reacting the living polymer which is metal terminated with a halogenated silicon containing compound to produce a polymer which is terminated with halogenated silicon moieties; followed by reacting that polymer with a tertiary alcohol to produce a polymer which is terminated with hydroxy silyl moieties. The polymer which is terminated with hydroxy silyl moieties can then be endlinked into a network polymer that contains siloxane linkages by simply heating it.

10. 发明公开

EP0217723A2 Siloxane containing network polymer 失效
标题翻译：含硅氧烷的聚合物网络。
公开(公告)号：EP0217723A2
公开(公告)日：1987-04-08
申请号：EP86630136.9
申请日：1986-09-03
申请人： THE GOODYEAR TIRE & RUBBER COMPANY
发明人： Halasa, Adel Farhan , Jalics, George
IPC分类号： C08C19/44 , C08G77/42
CPC分类号： C08C19/44 , C08F8/42
摘要： Metals from groups I and II are commonly used to catalyze the polymerization of monomers into polymers. The polymers formed in such polymerizations are terminated with the metal used to catalyze the polymerization and are sometimes referred to as living polymers. Such polymers can be crosslinked to produce a polymeric network by utilizing the process of the present invention. More specifically, the present invention discloses a process for endlinking a living polymer comprising reacting the living polymer which is metal terminated with a halogenated silicon containing compound to produce a polymer which is terminated with halogenated silicon moieties; followed by reacting that polymer with a tertiary alcohol to produce a polymer which is terminated with hydroxy silyl moieties. The polymer which is terminated with hydroxy silyl moieties can then be endlinked into a network polymer that contains siloxane linkages by simply heating it.

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