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1. 发明公开

EP2070910A1 Functionalized monomers and functionalized rubbery polymers made therewith 审中-公开
标题翻译： Funktionalisierte Monomere und damit hergestellte funktionalisierte gummiartige Polymere
公开(公告)号：EP2070910A1
公开(公告)日：2009-06-17
申请号：EP08170779.6
申请日：2008-12-05
申请人： The Goodyear Tire & Rubber Company
发明人： Halasa, Adel, Farhan , Hsu, Wen-Liang , Futamura, Shingo , Zhou, Joe , Jasiunas, Chad, Aaron
IPC分类号： C07C323/29 , C08F2/00
CPC分类号： C08F236/14 , C07C323/25 , C07F7/1836 , C07F9/5004 , C07F9/5031 , C08L19/006
摘要： A functionalized monomer is formed having the general formula:

R 1 R 2 N-(CH 2 ) n -X-CH 2 -CHR 3 R 4

wherein R 1 and R 2 are independently selected from a group consisting of alkyls, cycloalkyls, alkenyls, cycloalkenyls, aryls, phenyls, heterocycles, acyls, and silanes, or R 1 in combination with R 2 forms a heterocyclic ring; n is an integer from 1 to 20; X is selected from a group consisting of sulfur, a phosphorus moiety, and a silicon moiety; R 3 and R 4 are one of hydrogen, alkyls, alkenyls, and at least one of which includes reactive unsaturation such as an alkenyl group. The invention also discloses a process of making functionalized rubbery polymers from the functionalized monomers.
摘要翻译：形成具有以下通式的官能化单体：ƒ€ƒ€ƒ€ƒ€ƒ€ƒR 1 R 2 N-（CH 2）n -X-CH 2 -CHR 3 R 4其中R 1 R 2独立地选自烷基，环烷基，烯基，环烯基，芳基，苯基，杂环，酰基和硅烷，或R 1与R 2结合形成杂环; n为1〜20的整数， X选自硫，磷部分和硅部分; R 3和R 4是氢，烷基，链烯基之一，并且其中至少一个包括反应性不饱和键如烯基。本发明还公开了由官能化单体制备官能化橡胶聚合物的方法。

2. 发明公开

EP1900548A1 Carbon black-rich rubber composition containing particulate hydrophylic water absorbing polymer and tire with tread thereof 审中-公开
标题翻译：负载较重的橡胶组合物具有亲水性，吸水性聚合物和轮胎胎面与它们的
公开(公告)号：EP1900548A1
公开(公告)日：2008-03-19
申请号：EP07115834.9
申请日：2007-09-06
申请人： THE GOODYEAR TIRE & RUBBER COMPANY
发明人： Zhang, Ping , Sandstrom, Paul Harry , Kulig, Joseph John , Futamura, Shingo , Bates, Kenneth Allen , Hsu, Wen-Liang , Hua, Kuo-Chih
IPC分类号： B60C1/00 , C08K3/04 , C08K3/36 , C08K9/12 , C08L9/00 , C08L21/00
CPC分类号： B60C1/0016 , C08K3/013 , C08K7/02 , C08L21/00 , C08L29/04 , C08L33/02 , C08L33/26 , C08L2666/04
摘要： This invention relates to a rubber composition which contains a dispersion of a particulate hydrophilic water absorbing polymer and tire with a tread thereof.
The water-absorbing polymer has the capability of absorbing water in an amount of at least 1 g/g and is preferably present at the surface of the rubber composition.
摘要翻译：本发明涉及一种含有微粒的亲水性吸水聚合物和轮胎用胎面它们的分散体的橡胶组合物。吸水性聚合物具有至少1g / g的量的吸水的能力，并且优选存在于所述橡胶组合物的表面上。

3. 发明公开

EP1714984A1 Rubber composition containing an alkoxysilane coupled in-chain functionalized elastomer and tire with component thereof 审中-公开
标题翻译：其中包含一个加上烷氧基硅烷和在由此制得的聚合物链和弹性轮胎组分改性的橡胶组合物
公开(公告)号：EP1714984A1
公开(公告)日：2006-10-25
申请号：EP06112726.2
申请日：2006-04-18
申请人： THE GOODYEAR TIRE & RUBBER COMPANY
发明人： Halasa, Adel Farhan , Hsu, Wen-Liang , Bates, Kenneth Allan , Benko, David Andrew , Futamura, Shingo , Hua, Kuo-Chih
IPC分类号： C08C19/44 , C08L21/00 , B60C1/00
CPC分类号： B60C1/0016 , C08C19/25 , C08C19/44 , C08L15/00 , C08L19/006 , C08L21/00 , C08L2666/08
摘要： A precipitated silica reinforced conjugated diene-based elastomer composition is disclosed containing an alkoxysilane coupled, in-chain functionalized, conjugated diene-based elastomer. Said elastomer is a conjugated diene-based elastomer which contains a plurality of at least one of in-chain p- and m-(2-pyrrolidinoethyl) styrene (PES) and m-(2-pyrrolidino-1-methylethyl) alpha-methylstyrene (PAMS) groups.
摘要翻译：的沉淀二氧化硅增强的共轭二烯类弹性体组合物是游离缺失盘在耦合含烷氧基硅烷，在链官能化，共轭二烯基弹性体。所述弹性体是共轭二烯基弹性体其中包含在链对 - 和间 - （2-吡咯烷基乙基）苯乙烯（PES）和间 - （2-吡咯烷子基-1-甲基乙基）α-甲基苯乙烯中的至少一种的多元（PAMS）基团。

4. 发明公开

EP1593529A1 Natural rubber-rich composition and tire with tread thereof 有权
标题翻译： Naturkautschukreiche Zusammensetzung und Reifen mit daraus hergestellterLauffläche
公开(公告)号：EP1593529A1
公开(公告)日：2005-11-09
申请号：EP05103530.1
申请日：2005-04-28
申请人： THE GOODYEAR TIRE & RUBBER COMPANY
发明人： Sandstrom, Paul Harry , Halasa, Adel Farhan , Hsu, Wen-Liang , Verthe, John Joseph Andre , Jasiunas, Chad Aaron
IPC分类号： B60C1/00 , C08L9/06 , C08L7/00
CPC分类号： B60C1/0016 , C08K3/013 , C08K5/548 , C08L7/00 , C08L9/00 , C08L9/06 , C08L21/00 , C08L2666/02 , C08L2666/08
摘要： This invention relates to a natural rubber-rich rubber composition and tire with a tread thereof. A partial replacement of the natural rubber in the natural rubber-rich tire tread is accomplished by an inclusion of a specialized trans 1,4-styrene/butadiene copolymer rubber characterized by having a combination of bound styrene content and microstructure limitations. The tire tread rubber composition is comprised of a blend of the specialized trans 1,4-styrene/butadiene rubber and cis 1,4-polyisoprene natural rubber optionally together with at least one additional diene-based elastomer in which the natural rubber remains a major portion of the elastomers in the tread rubber composition. The specialized trans 1,4-styrene/butadiene rubber has a bound styrene content in a range of from 15 to 35 percent and a microstructure of its polybutadiene portion composed of from 50 to 80 percent trans 1,4-isomeric units, from 10 to 20 percent cis 1,4- isomeric units and from 2 to 10 percent vinyl 1,2- isomeric units.
摘要翻译：本发明涉及一种具有天然橡胶的橡胶组合物和具有胎面的轮胎。天然橡胶丰富的轮胎胎面中天然橡胶的部分替代是通过包含特征在于具有结合苯乙烯含量和微结构限制的组合的专用反式1,4-苯乙烯/丁二烯共聚物橡胶来实现的。轮胎胎面橡胶组合物由专门的反式1,4-苯乙烯/丁二烯橡胶和顺式1,4-聚异戊二烯天然橡胶的混合物组成，任选地与至少一种另外的二烯基弹性体共混，其中天然橡胶保持主要橡胶组合物中的部分弹性体。专用的反式1,4-苯乙烯/丁二烯橡胶具有15至35％的结合苯乙烯含量，其聚丁二烯部分的显微组织由50至80％的反式1,4-异构体单元组成，10至 20％的顺式1,4-异构体单元和2至10％的乙烯基1,2-异构体单元。

5. 发明公开

EP1514899A1 Tire with at least one of sidewall insert and/or apex of a rubber composition which contains a high vinyl polybutadiene 审中-公开
标题翻译：具有至少一个侧壁插入件和/或聚丁二烯的顶点与含有高乙烯基含量的轮胎橡胶组合物
公开(公告)号：EP1514899A1
公开(公告)日：2005-03-16
申请号：EP04104059.3
申请日：2004-08-24
申请人： THE GOODYEAR TIRE & RUBBER COMPANY
发明人： D'Sidocky, Richard Michael , Bezilla, Bernard Matthew, Jr , Benko, David Andrew , Halasa, Adel Farhan , Hsu, Wen-Liang , Deevers, Susan Lynn , Puhala, Aaron Scott , Burlett, Donald James
IPC分类号： C08L9/00
CPC分类号： C08L9/00 , B60C1/0025 , B60C15/06 , B60C17/0009 , C08K3/013 , C08K5/548 , C08L21/00 , C08L2666/08
摘要： This invention relates to a tire with a sidewall insert and/or apex of a rubber composition which contains a high vinyl polybutadiene elastomer.
摘要翻译：本发明涉及与含有高乙烯基聚丁二烯弹性体的橡胶组合物的侧壁插入件和/或顶点的轮胎。

6. 发明公开

EP0990670A1 Calcium-based catalyst system 有权
标题翻译： Katalysatorsystem auf Kalziumbasis
公开(公告)号：EP0990670A1
公开(公告)日：2000-04-05
申请号：EP99118676.8
申请日：1999-09-22
申请人： THE GOODYEAR TIRE & RUBBER COMPANY
发明人： Halasa, Adel Farhan , Hsu, Wen-Liang , Zuppo III, John Robert
IPC分类号： C08F236/10 , C08F136/08 , C08F4/54
CPC分类号： C08F136/08 , C08F236/10 , C08F4/54
摘要： The process and catalyst system of this invention can be utilized to synthesize a highly random styrene-butadiene rubber having a high trans content by solution polymerization. The styrene-butadiene rubber made by the process of this invention can be utilized in tire tread rubbers that exhibit improved wear characteristics. This invention more specifically reveals a catalyst system for use in isothermal polymerizations which consists essentially of (a) an organolithium compound, (b) a calcium alkoxide and (c) a lithium alkoxide. The subject invention further discloses a process for synthesizing a random styrene-butadiene rubber having a low vinyl content by a process which comprises copolymerizing styrene and 1,3-butadiene under isothermal conditions in an organic solvent in the presence of a catalyst system which consists essentially of (a) an organolithium compound, (b) a calcium alkoxide and (c) a lithium alkoxide. An amine can also be added to the catalyst system to increase the molecular weight (Mooney viscosity) of the rubber.
摘要翻译：本发明的方法和催化剂体系可用于通过溶液聚合合成具有高反式含量的高度无规的丁苯橡胶。通过本发明方法制备的苯乙烯 - 丁二烯橡胶可以用于表现出改进的磨损特性的轮胎胎面橡胶中。本发明更具体地揭示了用于等温聚合的催化剂体系，其基本上由（a）有机锂化合物，（b）醇盐和（c）醇锂组成。本发明进一步公开了一种合成具有低乙烯基含量的无规苯乙烯 - 丁二烯橡胶的方法，该方法包括在等温条件下在有机溶剂中，在催化剂体系存在下共聚苯乙烯和1,3-丁二烯，催化剂体系基本上组成（a）有机锂化合物，（b）醇盐和（c）醇锂。也可以向催化剂体系中加入胺以提高橡胶的分子量（门尼粘度）。

7. 发明公开

EP0796869A1 Rubbers having improved interaction with silica 失效
标题翻译：与硅石增强的交互橡胶
公开(公告)号：EP0796869A1
公开(公告)日：1997-09-24
申请号：EP97104323.7
申请日：1997-03-13
申请人： THE GOODYEAR TIRE & RUBBER COMPANY
发明人： Hsu, Wen-Liang , Halasa, Adel Farhan
IPC分类号： C08C19/26 , C08C19/42
CPC分类号： C08C19/26 , C08C19/42
摘要： The subject invention discloses a process for modifying a rubbery polymer to improve silica interaction which comprises the steps of: (1) metallating the rubbery polymer with lithium by reacting the rubbery polymer with an organo lithium compound in the presence of a member selected from the group consisting of alkali metal alkoxides, alkali metal phenoxides and chelating tertiary alkyl 1,2-ethylene diamines to produce a metallated rubbery polymer; and (2) reacting the metallated rubbery polymer with a silicon containing compound to produce the modified rubbery polymer having improved silica interaction, wherein the silicon containing compound is selected from the group consisting of silanes and siloxanes, wherein said silanes and siloxanes contain at least two functional groups which can be the same or different and which are selected from the group consisting of alkoxy groups, tertiary amino groups, cyano groups, sulfonyl groups, epoxy groups and halogen atoms; and wherein the reaction between the metallated rubbery polymer and the silicon containing compound is conducted in the presence of a member selected from the group consisting of alkali metal alkoxides, alkali metal phenoxides and chelating tertiary alkyl 1,2-ethylene diamines.

8. 发明公开

EP0764688A1 High performance blend for tire treads 失效
标题翻译： HochleistungsmischungfürReifenlaufflächen
公开(公告)号：EP0764688A1
公开(公告)日：1997-03-26
申请号：EP96114679.2
申请日：1996-09-13
申请人： THE GOODYEAR TIRE & RUBBER COMPANY
发明人： Halasa, Adel Farhan , Hsu, Wen-Liang , Zanzig, David John , Sandstrom, Paul Harry , Henning, Steven Kristofer , Lucas, Danielle
IPC分类号： C08L9/00 , B60C1/00 , C08F136/06
CPC分类号： C08F36/04 , C08F136/06 , C08K5/06 , C08K5/17 , C08L9/00 , Y02T10/862 , Y10S152/905 , C08F4/565 , C08L2666/08
摘要： This invention reveals a high performance polybutadiene rubber blend comprised of (a) a first polybutadiene rubber, (b) a second polybutadiene rubber, and (c) a third polybutadiene rubber; wherein the first polybutadiene rubber, the second polybutadiene rubber, and the third polybutadiene rubber are selected from the group of consisting of super-high vinyl polybutadiene rubbers having a vinyl content which is within the range of 80 percent to 100 percent, high vinyl polybutadiene rubbers having a vinyl content which is within the range of 60 percent to 79 percent, medium vinyl polybutadiene rubbers having a vinyl content which is within the range of 35 percent to 59 percent, and low vinyl polybutadiene rubbers having a vinyl content which is within the range of 8 percent to 34 percent; wherein at least three members selected from the group consisting of super-high vinyl polybutadiene rubbers, high vinyl polybutadiene rubbers, medium vinyl polybutadiene rubbers, and low vinyl polybutadiene rubbers are included in the blend, wherein at least one of the polybutadiene rubbers in the blend has a vinyl content which is within 35 percentage points of the vinyl content of at least one other polybutadiene rubber in the blend, wherein the blend as a whole has a vinyl content of at least 40 percent, and wherein the blend contains at least 10 parts of the first polybutadiene rubber, at least 10 parts of the second polybutadiene rubber and at least 10 parts of the third polybutadiene rubber, based upon a total of 100 parts of rubber in the blend.
摘要翻译：用于制造的高性能聚丁二烯橡胶混合物。轮胎胎面cpds。包括：（a）第一聚丁二烯橡胶（I），（b）第二聚丁二烯橡胶（II）和（c）第三聚丁二烯橡胶（III）; （I），（II）和（III）是乙烯基含量为80-100％的超高乙烯基聚丁二烯橡胶，乙烯基含量为60-79％的高乙烯基聚丁二烯橡胶，具有乙烯基含量为35-59％，乙烯基含量为8-34％的低乙烯基聚丁二烯橡胶; 在共混物中包括来自超乙烯基聚丁二烯橡胶，高乙烯基聚丁二烯橡胶，中乙烯基聚丁二烯橡胶，低乙烯基聚丁二烯橡胶的3个或更多个成员，其中共混物中的一种或多种聚丁二烯橡胶具有在其中（I）的乙烯基含量与（II）和（III）的乙烯基含量不同于（II）和（III）的其他聚丁二烯橡胶的乙烯基含量的35％不同于（III）的乙烯基含量为5％以上，其中共混物作为整体的总乙烯基含量为40％以上，共混物含有10个。或更多（I），10点。或更多（II）和10点。以上（III），w.r.t. 共计100个的混合物中的橡胶。

9. 发明授权

EP0438967B1 Segmented elastomer 失效
标题翻译：细分弹性体
公开(公告)号：EP0438967B1
公开(公告)日：1996-05-01
申请号：EP90630215.3
申请日：1990-12-05
申请人： THE GOODYEAR TIRE & RUBBER COMPANY
发明人： Hsu, Wen-Liang , Halasa, Adel Farhan
IPC分类号： C08F297/04 , B60C1/00
CPC分类号： C08F297/046 , B60C1/0016 , Y02T10/862

10. 发明授权

EP0483572B1 Process for the synthesis of a high vinyl isoprene-butadiene copolymer 失效
标题翻译：一种用于异戊二烯 - 丁二烯共聚物的具有高乙烯基含量的合成过程。
公开(公告)号：EP0483572B1
公开(公告)日：1995-04-26
申请号：EP91117427.4
申请日：1991-10-12
申请人： THE GOODYEAR TIRE & RUBBER COMPANY
发明人： Hsu, Wen-Liang , Halasa, Adel Farhan
IPC分类号： C08F236/04 , C08F4/70
CPC分类号： C08F236/04 , C08F2410/01 , C08F4/7027

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