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1. 发明授权

US5768910A Adsorption heat pump 失效
标题翻译：吸附热泵
公开(公告)号：US5768910A
公开(公告)日：1998-06-23
申请号：US738113
申请日：1996-10-25
申请人： Shinji Inagaki , Yuri Yamada , Yoshiaki Fukushima , Masanobu Hasatani , Fujio Watanabe
发明人： Shinji Inagaki , Yuri Yamada , Yoshiaki Fukushima , Masanobu Hasatani , Fujio Watanabe
IPC分类号： B01J20/10 , C09K5/04 , F25B17/08
CPC分类号： F25B17/08 , C09K5/047 , Y02P20/123 , Y02P20/124
摘要： An adsorption heat pump includes a working fluid, an adsorption-desorption unit, and an evaporation-condensation unit connected with the adsorption-desorption unit. The adsorption-desorption unit adsorbs and desorbs vapor resulting from the working fluid, and includes an adsorbent being a porous substance. The porous substance has pores, and exhibits a pore diameter distribution curve having a maximum peak falling in a pore diameter range of from 1 to 10 nm. The pores in the diameter range of .+-.40% of pore diameter at the maximum peak have pore volume not less than 60% of a whole volume of the porous substance. The evaporation-condensation unit evaporates and condenses the working fluid. The adsorption heat pump can be operated by a low-temperature heat source, and can exhibit a large pumping temperature difference regardless of its small size.
摘要翻译：吸附热泵包括工作流体，吸附解吸单元和与吸附 - 解吸单元连接的蒸发 - 冷凝单元。吸附 - 解吸装置吸附和解吸由工作流体产生的蒸气，并且包括作为多孔物质的吸附剂。多孔物质具有孔，表现出孔径分布曲线，孔径范围为1〜10nm。在最大峰的孔径的+/- 40％的直径范围内的孔具有不小于整个体积的多孔物质的60％的孔体积。蒸发冷凝单元蒸发和冷凝工作流体。吸附式热泵可以通过低温热源进行操作，无论体积小，均可显示较大的泵送温度差。

2. 发明授权

US5599759A Process for producing porous silicon oxide material 失效
标题翻译：多孔氧化硅材料的制造方法
公开(公告)号：US5599759A
公开(公告)日：1997-02-04
申请号：US493042
申请日：1995-06-21
申请人： Shinji Inagaki , Yoshiaki Fukushima , Yuri Yamada
发明人： Shinji Inagaki , Yoshiaki Fukushima , Yuri Yamada
IPC分类号： B01J21/16
CPC分类号： B01J21/16
摘要： A process for producing a heat-resistant and high-purity porous silicon oxide material having excellent crystallinity and uniformity in pore size. The process includes: a first step of dispersing a substance containing silicon in an aqueous solution of a surfactant and adjusting the pH of the dispersion to a value of 10 or higher; a second step of adjusting the pH thereof to a value lower than 10 and forming a composite of a silicon oxide and a surfactant; and a third step of removing the surfactant from the composite. A water-soluble component is preferably removed from the dispersion between the first and second steps.
摘要翻译：一种具有优异的结晶度和孔径均匀性的耐热和高纯度多孔氧化硅材料的制造方法。该方法包括：将含硅物质分散在表面活性剂的水溶液中并将分散体的pH调节至10以上的第一步骤; 将pH调节至低于10的值并形成氧化硅和表面活性剂的复合物的第二步骤; 以及从复合材料中除去表面活性剂的第三步骤。优选从第一和第二步骤之间的分散体中除去水溶性组分。

3. 发明授权

US5750085A Process for manufacturing a silica porous material 失效
标题翻译：二氧化硅多孔材料的制造方法
公开(公告)号：US5750085A
公开(公告)日：1998-05-12
申请号：US598352
申请日：1996-02-08
申请人： Yuri Yamada , Shinji Inagaki , Yoshiaki Fukushima
发明人： Yuri Yamada , Shinji Inagaki , Yoshiaki Fukushima
IPC分类号： C04B38/04 , B01J20/10 , B01J21/08 , B01J29/035 , C01B33/12 , C01B33/18 , C01B33/20 , C01B33/26 , C04B38/06
CPC分类号： B01J21/08 , B01J20/103 , C01B33/20 , C01B33/26
摘要： A process for manufacturing a silica porous material with high solid acidity, catalytic activity and adsorption ability as well as excellent crystallinity and heat resistance has the steps of adding a compound of metallic element such as Al to a waterglass, aging the resultant mixture, calcining the aged mixture to form a layered crystal, incorporating an organic substance between layers of the layered crystal, calcining the resultant layered crystal for crosslinking the layered crystal. By this process, a plurality of layers formed of SiO.sub.4 tetrahedral and metallic oxide constitute a silica porous material, and the gap between adjacent layers of the layered crystal is reduced at a crosslinking site, while the gap of the other portion is expanded to form a micro pore.
摘要翻译：制备具有高固体酸度，催化活性和吸附能力以及优异的结晶度和耐热性的二氧化硅多孔材料的方法具有以下步骤：向水玻璃中加入诸如Al的金属元素化合物，使所得混合物老化，煅烧形成层状结晶，在层状结晶层之间并入有机物质，煅烧所得到的层状结晶以交联层状结晶。通过该工艺，由SiO 4四面体和金属氧化物形成的多个层构成二氧化硅多孔材料，层状结晶的相邻层之间的间隙在交联部位减少，而另一部分的间隙扩大形成微孔。

4. 发明授权

US08034509B2 Polymer electrolyte membrane with an inorganic backbone 有权
标题翻译：具有无机骨架的聚合物电解质膜
公开(公告)号：US08034509B2
公开(公告)日：2011-10-11
申请号：US10379812
申请日：2003-03-06
申请人： Shinji Inagaki , Yoshiaki Fukushima , Masaya Kawasumi , Naoki Hasegawa , Yu Morimoto , Kyoko Tsusaka
发明人： Shinji Inagaki , Yoshiaki Fukushima , Masaya Kawasumi , Naoki Hasegawa , Yu Morimoto , Kyoko Tsusaka
IPC分类号： H01M8/10 , C01B33/20 , C08J5/20
CPC分类号： C25B9/10 , H01M4/861 , H01M4/926 , H01M8/1004 , H01M8/1037 , H01M8/1051 , H01M8/1067 , H01M8/1074 , H01M2300/0082 , H01M2300/0094 , Y02P70/56
摘要： The membrane electrode assembly 1 has an anode 10, a cathode 20, and an electrolyte membrane 30 disposed between the anode and cathode; the anode and cathode are gas diffusion electrodes; the electrolyte membrane contains a solid electrolyte in which a plurality of pores with mean pore diameters of 1 to 30 nm are formed; and the solid electrolyte has a backbone comprising organic groups having one or more metal atoms, oxygen atoms bonded to the metal atoms, and carbon atoms bonded to the metal atoms or oxygen atoms, and also has functional groups with ion-exchange capabilities that are bonded to the organic groups in the pores.
摘要翻译：膜电极组件1具有阳极10，阴极20和设置在阳极和阴极之间的电解质膜30; 阳极和阴极是气体扩散电极; 电解质膜含有固体电解质，其中形成平均孔径为1〜30nm的多个孔; 并且所述固体电解质具有包含具有一个或多个金属原子的有机基团，与所述金属原子键合的氧原子和与所述金属原子或氧原子键合的碳原子的骨架，并且还具有键合的离子交换能力的官能团到毛孔中的有机基团。

5. 再颁专利

USRE37385E1 Composite material and process for manufacturing same 有权
标题翻译：复合材料及其制造方法相同
公开(公告)号：USRE37385E1
公开(公告)日：2001-09-18
申请号：US09396871
申请日：1999-09-15
申请人： Akane Okada , Yoshiaki Fukushima , Masaya Kawasumi , Shinji Inagaki , Arimitsu Usuki , Shigetoshi Sugiyama , Toshio Kurauchi , Osami Kamigaito
发明人： Akane Okada , Yoshiaki Fukushima , Masaya Kawasumi , Shinji Inagaki , Arimitsu Usuki , Shigetoshi Sugiyama , Toshio Kurauchi , Osami Kamigaito
IPC分类号： C08K302
CPC分类号： B82Y30/00 , C08J5/005 , C08J2377/00 , C08K3/346 , C08L77/02 , C08L77/00
摘要： Composite material with high mechanical strength and excellent high-temperature characteristics comprising a polymer matrix containing polyamide and layers of a silicate uniformly dispersed in the order of molecules in the polymer matrix, each of said silicate layers being 7 to 12 Å thick and the interlayer distance being at least 20 Å; and a process for manufacturing such composite material.
摘要翻译：具有高机械强度和优异的高温特性的复合材料包括含有聚酰胺的聚合物基体和以聚合物基质中的分子顺序均匀分散的硅酸盐层，每个所述硅酸盐层的厚度为7至12埃，层间距离至少20Å; 以及这种复合材料的制造方法。

6. 发明授权

US6107243A Cluster-included material 失效
标题翻译：集群包含的材料
公开(公告)号：US6107243A
公开(公告)日：2000-08-22
申请号：US925769
申请日：1997-09-09
申请人： Shinji Inagaki , Noriaki Sugimoto , Tatsumi Hioki , Yoshiaki Fukushima , Masaru Ichikawa
发明人： Shinji Inagaki , Noriaki Sugimoto , Tatsumi Hioki , Yoshiaki Fukushima , Masaru Ichikawa
IPC分类号： B01J20/28 , B01J20/10
CPC分类号： B01J20/28083 , B01J20/28004 , B01J20/28009 , B01J20/2803 , B01J20/28069 , B01J20/28097 , Y10T428/24149
摘要： The present cluster-included material characterized by utilizing a porous host material for clusters having a pore larger in size than that of zeolite. The cluster-included material is obtained by forming a cluster in a pore of a mesoporous material having a pore size of 1.3 to 10 nm. When the mesoporous material is particularly a mesoporous material having a pore volume of not less than 60% of a total pore volume within a pore size range of -40 to +40% of a pore size which shows a maximum peak in a pore size distribution curve, a granular cluster having a uniform particle size or a fine-linear cluster having a uniform diameter is obtained. The cluster-included material performs the various quantum effects.
摘要翻译：本发明的包含簇的材料的特征在于利用多孔主体材料用于具有比沸石尺寸更大的孔的簇。通过在孔径为1.3〜10nm的介孔材料的孔中形成簇而获得含有簇的材料。当介孔材料特别是孔体积为孔体积的孔体积的最大峰值在孔径的-40〜+ 40％的孔径范围内的孔体积的60％以上的中孔材料时，得到具有均匀粒径的粒状团簇或具有均匀直径的微细线粒团。包含簇的材料执行各种量子效应。

7. 发明授权

US5508081A Porous material composed of layered silica and metal oxide and a process for manufacturing the same 失效
标题翻译：由层状二氧化硅和金属氧化物构成的多孔材料及其制造方法
公开(公告)号：US5508081A
公开(公告)日：1996-04-16
申请号：US192933
申请日：1994-02-07
申请人： Shinji Inagaki , Yoshiaki Fukushima , Akane Okata , Chuzo Kato , Kazuyuki Kuroda
发明人： Shinji Inagaki , Yoshiaki Fukushima , Akane Okata , Chuzo Kato , Kazuyuki Kuroda
IPC分类号： C01B33/12 , B01J20/10 , B01J21/08 , B01J23/04 , B01J29/00 , B01J29/04 , B01J35/04 , C01B33/20 , C01B33/32 , C01B33/44 , B32B3/12
CPC分类号： B01J20/10 , B01J21/08 , B01J23/04 , B01J29/049 , B01J35/04 , Y10T428/24149 , Y10T428/249969 , Y10T428/24997
摘要： A porous material composed of many SiO.sub.4 tetrahedra sheets having interlayer bridges of SiO.sub.2. It has pores having a diameter of 10 .ANG. or above, and possesses the properties of a solid acid formed by the isomorphous substitution of metal atoms for Si of SiO.sub.4 frameworks. It is made by a process including introducing an organic substance into interlayer space of crystals of layered silicates to expand the spacing between crystal layers, as well as forming bridges of SiO.sub.2 therebetween, bringing the intercalated compounds into contact with a metal salt to link metal atoms to the SiO.sub.4 frameworks, and firing the products. The material can withstand a temperature of 800.degree. C., has a pore diameter larger than that of zeolites, etc., and is useful in making an adsorbent or catalyst for molecules having a high molecular weight, such as a catalyst for the catalytic cracking of petroleum.
摘要翻译：由具有SiO 2层间桥的许多SiO 4四面体片组成的多孔材料。它具有直径为10或更大的孔，并且具有通过金属原子对SiO 4骨架的Si的同晶取代而形成的固体酸的性质。它是通过包括将有机物质引入到层状硅酸盐晶体的层间空间中以扩大晶体层之间的间距，以及在其间形成二氧化硅之间的过程，使插入的化合物与金属盐接触以连接金属原子到SiO4框架，并烧制产品。该材料可以承受800℃的温度，孔径大于沸石等的孔径，并且可用于制备具有高分子量的分子的吸附剂或催化剂，例如用于催化裂化的催化剂的石油。

8. 发明授权

US5462905A Exhaust gas purifying catalyst 失效
标题翻译：废气净化催化剂
公开(公告)号：US5462905A
公开(公告)日：1995-10-31
申请号：US105932
申请日：1993-08-13
申请人： Tetsuo Nagami , Yoshitsugu Ogura , Masahiko Ogai , Yoshiaki Fukushima , Shinji Inagaki , Kazuhiro Fukumoto , Kouji Banno , Yuji Sakakibara , Yasuo Takada , Takashi Ohta , Akane Okada , Yukimura Yamada , Kiyotaka Hayashi , Shinji Matsuura , Kazuyuki Kuroda
发明人： Tetsuo Nagami , Yoshitsugu Ogura , Masahiko Ogai , Yoshiaki Fukushima , Shinji Inagaki , Kazuhiro Fukumoto , Kouji Banno , Yuji Sakakibara , Yasuo Takada , Takashi Ohta , Akane Okada , Yukimura Yamada , Kiyotaka Hayashi , Shinji Matsuura , Kazuyuki Kuroda
IPC分类号： B01D53/86 , B01D53/94 , B01J21/08 , B01J29/03
CPC分类号： B01J29/0308 , B01D53/9418 , B01D53/9445 , B01D53/945 , B01D53/9481 , B01J21/08 , B01J29/0325 , B01J35/1061 , B01D2255/1021 , B01D2255/912 , B01D2255/9202 , Y02T10/22
摘要： An exhaust gas purifying catalyst is characterized in that at least one kind of catalyst metal is loaded on a layered porous silica or a layered porous silica-metal oxide. The exhaust gas purifying catalyst is used as an oxidation catalyst for purifying hydrocarbon and carbon monoxide, or a reduction catalyst for purifying nitrogen oxides (NO.sub.x), which is suitable for purifying exhaust gases in automobiles. An exhaust gas purifying apparatus includes the above exhaust gas purifying catalyst and an absorbent for trapping hydrocarbon components, in which aromatic HC such as trimethylbenzene and the like are effectively trapped.
摘要翻译：废气净化催化剂的特征在于，在层状多孔质二氧化硅或层状多孔二氧化硅 - 金属氧化物上载持至少一种催化剂金属。废气净化催化剂用作净化烃和一氧化碳的氧化催化剂，或者用于净化汽车中的废气的氮氧化物（NOx）的还原催化剂。废气净化装置包括上述废气净化催化剂和用于捕获烃成分的吸收剂，其中芳族HC如三甲基苯等被有效地捕获。

9. 发明授权

US07488559B2 Solid electrolyte 有权
标题翻译：固体电解质
公开(公告)号：US07488559B2
公开(公告)日：2009-02-10
申请号：US10415353
申请日：2001-10-31
申请人： Shinji Inagaki , Shiyou Guan , Yoshiaki Fukushima
发明人： Shinji Inagaki , Shiyou Guan , Yoshiaki Fukushima
IPC分类号： H01M10/40 , H01M6/18 , H01M8/10
CPC分类号： H01M8/124 , H01B1/122 , H01M6/18 , H01M8/1027 , H01M8/1037 , H01M8/1044 , H01M8/1067 , H01M10/05 , Y02P70/56
摘要： The solid electrolyte of the present invention is composed of an organic/inorganic composite material having pores with a mean pore diameter of 1 to 30 nm and having a skeleton comprising a metal atom, an oxygen atom bonded to the metal atom, and an organic group having at least one carbon atom bonded to the metal atom or the oxygen atom, and a functional group having an ion exchange function and bonded to the organic group inside the pores. As a result, even if the relative pressure of the water vapor in the atmosphere is less than 1.0, it is still possible to achieve a solid electrolyte with a sufficiently high ion conductivity at a lower temperature than with a conventional solid electrolyte such as stabilized zirconia.
摘要翻译：本发明的固体电解质由平均孔径为1〜30nm，具有金属原子，与金属原子键合的氧原子和有机基团的骨架的有机/无机复合材料构成具有与金属原子或氧原子键合的至少一个碳原子，和具有离子交换功能的官能团，并与孔内的有机基团结合。结果，即使气氛中的水蒸气的相对压力小于1.0，仍然可以在比常规固体电解质如稳定的氧化锆更低的温度下获得具有足够高的离子传导性的固体电解质。

10. 发明授权

US06248686B1 Organic/inorganic complex porous materials 有权
标题翻译：有机/无机复合多孔材料
公开(公告)号：US06248686B1
公开(公告)日：2001-06-19
申请号：US09347005
申请日：1999-07-02
申请人： Shinji Inagaki , Shiyou Guan , Yoshiaki Fukushima
发明人： Shinji Inagaki , Shiyou Guan , Yoshiaki Fukushima
IPC分类号： B01J2100
CPC分类号： C08G77/58 , B01J20/103 , B01J20/262 , B01J20/28083 , C08G77/22 , C08G83/001
摘要： Organic/inorganic complex porous materials are disclosed having a main skeletal chain containing metal atoms, oxygen atoms, and organic groups. Preferably, the metal atoms, oxygen atoms and organic groups are bound by ionic bonds and/or covalent bonds, and the organic group is bound to at least two metal atoms in the main chain of the skeleton of the porous material. More preferably, 60% or more of the total pore volume in the porous material has a pore diameter in a range of ±40% of the pore diameter, as determined from the maximum peak in a pore size distribution curve. Alternatively, at least one peak is present at a diffraction angle that preferably corresponds to a d value of at least 1 nm in an x-ray diffraction pattern. Method of making such organic/inorganic complex materials are also disclosed.
摘要翻译：公开了具有含有金属原子，氧原子和有机基团的主骨架链的有机/无机复合多孔材料。优选地，金属原子，氧原子和有机基团通过离子键和/或共价键结合，并且有机基团结合到多孔材料的骨架的主链中的至少两个金属原子。更优选地，多孔材料中的总孔体积的60％以上具有从孔径分布曲线中的最大峰值确定的孔径在±40％范围内的孔径。或者，在x射线衍射图中优选对应于至少1nm的d值的衍射角处存在至少一个峰。还公开了制备这种有机/无机复合材料的方法。

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