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1. 发明申请

US20100239950A1 CATALYST LAYER-SUPPORTING SUBSTRATE, METHOD OF PRODUCING THE SAME AND FUEL CELL 有权
标题翻译：催化层支撑基板，其制造方法和燃料电池
公开(公告)号：US20100239950A1
公开(公告)日：2010-09-23
申请号：US12726638
申请日：2010-03-18
申请人： Wu MEI , Jun Tamura , Mutsuki Yamazaki , Yoshihiko Nakano
发明人： Wu MEI , Jun Tamura , Mutsuki Yamazaki , Yoshihiko Nakano
IPC分类号： H01M4/92 , B01J32/00 , B01J21/18 , B01J23/46
CPC分类号： H01M4/8871 , H01M4/8807 , H01M4/8878 , H01M2008/1095
摘要： A catalyst layer-supporting substrate includes a substrate and a catalyst layer. The catalyst layer includes a catalyst material and pores. The catalyst layer is formed on the substrate. The catalyst material has a layer or wire shape. A half-value width of a main peak of the catalyst material, as determined from X-ray diffraction spectrum of the catalyst layer, is 1.5° or more. A porosity of the catalyst layer is 30% or more.
摘要翻译：催化剂层支撑基板包括基板和催化剂层。催化剂层包括催化剂材料和孔。催化剂层形成在基板上。催化剂材料具有层或线形。由催化剂层的X射线衍射光谱确定的催化剂材料的主峰的半值宽度为1.5°以上。催化剂层的孔隙率为30％以上。

2. 发明授权

US08334233B2 Catalyst layer-supporting substrate, method of producing the same and fuel cell 有权
标题翻译：催化剂层支撑基板，其制造方法和燃料电池
公开(公告)号：US08334233B2
公开(公告)日：2012-12-18
申请号：US12726638
申请日：2010-03-18
申请人： Wu Mei , Jun Tamura , Mutsuki Yamazaki , Yoshihiko Nakano
发明人： Wu Mei , Jun Tamura , Mutsuki Yamazaki , Yoshihiko Nakano
IPC分类号： B01J21/04
CPC分类号： H01M4/8871 , H01M4/8807 , H01M4/8878 , H01M2008/1095
摘要： A catalyst layer-supporting substrate includes a substrate and a catalyst layer. The catalyst layer includes a catalyst material and pores. The catalyst layer is formed on the substrate. The catalyst material has a layer or wire shape. A half-value width of a main peak of the catalyst material, as determined from X-ray diffraction spectrum of the catalyst layer, is 1.5° or more. A porosity of the catalyst layer is 30% or more.
摘要翻译：催化剂层支撑基板包括基板和催化剂层。催化剂层包括催化剂材料和孔。催化剂层形成在基板上。催化剂材料具有层或线形。由催化剂层的X射线衍射光谱确定的催化剂材料的主峰的半值宽度为1.5°以上。催化剂层的孔隙率为30％以上。

3. 发明申请

US20090257931A1 METHOD OF RECOVERING NOBLE METALS AND RECOVERING SYSTEM FOR NOBLE METALS 审中-公开
标题翻译：回收金属的方法和用于金属的回收系统
公开(公告)号：US20090257931A1
公开(公告)日：2009-10-15
申请号：US12490563
申请日：2009-06-24
申请人： Yoshihiko Nakano , Jun Tamura , Kazuhiro Yasuda , Mutsuki Yamazaki , Itsuko Mizutani , Yoshiko Hiraoka
发明人： Yoshihiko Nakano , Jun Tamura , Kazuhiro Yasuda , Mutsuki Yamazaki , Itsuko Mizutani , Yoshiko Hiraoka
IPC分类号： C01G55/00
CPC分类号： C22B11/048 , C22B3/08 , C22B3/165 , C22B3/22 , C22B3/44 , C22B7/006 , C22B7/007 , Y02P10/214 , Y02P10/234
摘要： A recovering method is provided, which includes contacting a solid component containing Ru with an aqueous solution to create a Ru compound, and causing the Ru compound to selectively elute in the aqueous solution. The aqueous solution is formed of at least one selected from the group consisting of aqueous solutions A, B, C, D, and E. The aqueous solution A comprises an acid and formic acid, alcohols, aldehydes, a compound having a hemiacetal structure or a compound having an acetal structure. The aqueous solution B comprises an acid and a compound which creates, in the coexistence thereof with the acid, formic acid, alcohols, aldehydes, a compound having a hemiacetal structure or a compound having an acetal structure. The aqueous solution C comprises an acid and sugars. The aqueous solution D comprises formic acid, and the aqueous solution E comprises oxalic acid.
摘要翻译：提供一种回收方法，其包括将含有Ru的固体组分与水溶液接触以产生Ru化合物，并使Ru化合物在水溶液中选择性洗脱。水溶液由选自水溶液A，B，C，D和E中的至少一种形成。水溶液A包含酸和甲酸，醇，醛，具有半缩醛结构的化合物或具有缩醛结构的化合物。水溶液B包含与酸，甲酸，醇，醛，具有半缩醛结构的化合物或具有缩醛结构的化合物共存的酸和化合物。水溶液C包含酸和糖。水溶液D含有甲酸，水溶液E含有草酸。

4. 发明申请

US20090081528A1 SUPPORTED CATALYST FOR FUEL CELL, AND ELECTRODE AND FUEL CELL USING THE SAME 审中-公开
标题翻译：用于燃料电池，电极和燃料电池的支持催化剂
公开(公告)号：US20090081528A1
公开(公告)日：2009-03-26
申请号：US12207851
申请日：2008-09-10
申请人： Yoshihiko Nakano , Jun Tamura , Mutsuki Yamazaki
发明人： Yoshihiko Nakano , Jun Tamura , Mutsuki Yamazaki
IPC分类号： H01M4/48 , B01J21/18
CPC分类号： H01M4/9008 , H01M4/9083 , H01M4/926 , H01M2008/1095
摘要： The present invention provides a supported catalyst excellent both in catalytic performance and in stability against concentrated methanol. The supported catalyst is used for an electrode of a fuel cell, and comprises catalytic metal particles supported on supports. The supports have hydrophilicity. On at least one part of the surface of the hydrophilic supports, particles of metal oxide super-strong acid are also supported. The metal oxide super-strong acid particles promote proton conduction.
摘要翻译：本发明提供催化性能和对浓缩甲醇稳定性优异的负载型催化剂。负载催化剂用于燃料电池的电极，并且包括负载在载体上的催化金属颗粒。支持物具有亲水性。在亲水载体表面的至少一部分上，也支持金属氧化物超强酸的颗粒。金属氧化物超强酸颗粒促进质子传导。

5. 发明授权

US08318382B2 Fuel cell electrode containing proton conductive inorganic oxide 失效
标题翻译：含有质子传导性无机氧化物的燃料电池电极
公开(公告)号：US08318382B2
公开(公告)日：2012-11-27
申请号：US11537219
申请日：2006-09-29
申请人： Jun Tamura , Yoshihiko Nakano , Wu Mei
发明人： Jun Tamura , Yoshihiko Nakano , Wu Mei
IPC分类号： H01M4/36 , H01M4/90
CPC分类号： H01M4/90 , H01M4/8657 , H01M4/8803 , H01M4/8828 , H01M4/8882 , H01M4/9016 , H01M8/1004 , Y02P70/56
摘要： According to one embodiment, a catalyst layer of an electrode for a fuel cell has a proton conductive inorganic oxide containing an oxide superacid compound. The compound contains an element X (Titanium, Zirconium, Silicon, Tin, Hafnium, Germanium, Gallium, Indium, Cerium, Niobium or Aluminum) and an element Y (Tungsten, Molybdenum, Chromium, Boron or Vanadium). The catalyst layer also contains a reduction-oxidation metal catalyst or a carrier carrying a reduction-oxidation metal catalyst.
摘要翻译：根据一个实施例，用于燃料电池的电极的催化剂层具有含有氧化物超强酸化合物的质子传导性无机氧化物。化合物含有元素X（钛，锆，硅，锡，铪，锗，镓，铟，铈，铌或铝）和元素Y（钨，钼，铬，硼或钒）。催化剂层还含有还原氧化金属催化剂或载有还原氧化金属催化剂的载体。

6. 发明授权

US07759019B2 Liquid fuel cell, membrane electrode assembly and cathode 有权
标题翻译：液体燃料电池，膜电极组件和阴极
公开(公告)号：US07759019B2
公开(公告)日：2010-07-20
申请号：US11370852
申请日：2006-03-09
申请人： Wu Mei , Miho Maruyama , Jun Tamura , Yoshihiro Akasaka , Yoshihiko Nakano
发明人： Wu Mei , Miho Maruyama , Jun Tamura , Yoshihiro Akasaka , Yoshihiko Nakano
IPC分类号： H01M4/00
CPC分类号： H01M4/8605 , H01M4/90 , H01M4/9083 , H01M4/923 , H01M4/926 , H01M8/1011 , Y02E60/523
摘要： A cathode includes a diffusion layer, and a porous catalyst layer provided on the diffusion layer. The porous catalyst layer has a thickness not greater than 60 μm, a porosity of 30 to 70% and a pore diameter distribution including a peak in a range of 20 to 200 nm of a pore diameter. A volume of pores having a diameter of 20 to 200 nm is not less than 50% of a pore volume of the porous catalyst layer. The porous catalyst layer contains a supported catalyst comprising 10 to 30% by weight of a fibrous supported catalyst and 70 to 90% by weight of a granular supported catalyst. The fibrous supported catalyst includes a carbon nanofiber having a herringbone structure or a platelet structure. The granular supported catalyst includes a carbon black having 200 to 600 mL/100 g of a dibutyl phthalate (DBP) absorption value.
摘要翻译：阴极包括扩散层和设置在扩散层上的多孔催化剂层。多孔催化剂层的厚度不大于60μm，孔隙率为30-70％，孔径分布包括孔径在20至200nm范围内的峰。一直径为20〜200nm的孔体积不小于多孔催化剂层的孔体积的50％。多孔催化剂层包含载体催化剂，其包含10至30重量％的纤维负载催化剂和70至90重量％的颗粒负载型催化剂。纤维状载体催化剂包括具有人字形结构或血小板结构的碳纳米纤维。颗粒状载体催化剂包括具有200至600mL / 100g邻苯二甲酸二丁酯（DBP）吸收值的炭黑。

7. 发明授权

US07572543B2 Supported catalyst and fuel cell 有权
标题翻译：负载催化剂和燃料电池
公开(公告)号：US07572543B2
公开(公告)日：2009-08-11
申请号：US11512207
申请日：2006-08-30
申请人： Wu Mei , Jun Tamura , Yoshihiko Nakano
发明人： Wu Mei , Jun Tamura , Yoshihiko Nakano
IPC分类号： H01M4/00
CPC分类号： H01M4/925 , H01M4/9016 , H01M4/92
摘要： A supported catalyst includes an oxide carrier, catalyst particles supported on the oxide carrier, and catalyst layers which locate among the catalyst particles, with interface portions among the oxide carrier, the catalyst particles and the catalyst layers. The catalyst layers have a melting point lower than 1,500° C. and contain an oxide or a composite oxide which includes at least one element selected from the group consisting of Mo, W, Sn and Ru.
摘要翻译：载体催化剂包括氧化物载体，负载在氧化物载体上的催化剂颗粒和位于催化剂颗粒之间的催化剂层，其中氧化物载体，催化剂颗粒和催化剂层中的界面部分。催化剂层的熔点低于1500℃，并含有包含选自Mo，W，Sn和Ru中的至少一种元素的氧化物或复合氧化物。

8. 发明申请

US20070207360A1 ELECTROLYTE MEMBRANE, MEMBRANE ELECTRODE ASSEMBLY, AND FUEL CELL 审中-公开
标题翻译：电解质膜，膜电极组件和燃料电池
公开(公告)号：US20070207360A1
公开(公告)日：2007-09-06
申请号：US11744267
申请日：2007-05-04
申请人： Jun Tamura , Yoshihiko Nakano , Wu Mei , Kazuhiro Yasuda
发明人： Jun Tamura , Yoshihiko Nakano , Wu Mei , Kazuhiro Yasuda
IPC分类号： H01M8/10
CPC分类号： H01M8/1004 , H01M8/1016 , H01M2300/0071 , H01M2300/0091
摘要： An electrolyte membrane includes a porous membrane and a proton conductive inorganic material loaded in the porous membrane. The proton conductive inorganic material has a super strong acidity. The proton conductive inorganic material contains a first oxide and a second oxide bonded to the first oxide. The first oxide contains an element X formed of at least one element selected from the group consisting of Ti, Zr, Hf, Nb, Al, Ga, In, Si, Ge, Sn and Ce. The second oxide contains an element Y formed of at least one element selected from the group consisting of V, Cr, Me, W and B.
摘要翻译：电解质膜包括多孔膜和负载在多孔膜中的质子传导性无机材料。质子传导性无机材料具有超强的酸性。质子传导性无机材料含有与第一氧化物结合的第一氧化物和第二氧化物。第一氧化物含有由选自Ti，Zr，Hf，Nb，Al，Ga，In，Si，Ge，Sn和Ce中的至少一种元素形成的元素X。第二氧化物含有由选自V，Cr，Me，W和B的至少一种元素形成的元素Y。

9. 发明申请

US20070003823A1 Supported catalyst and fuel cell 有权
标题翻译：负载催化剂和燃料电池
公开(公告)号：US20070003823A1
公开(公告)日：2007-01-04
申请号：US11512207
申请日：2006-08-30
申请人： Wu Mei , Jun Tamura , Yoshihiko Nakano
发明人： Wu Mei , Jun Tamura , Yoshihiko Nakano
IPC分类号： H01M4/86 , B01J21/00 , B01J23/00
CPC分类号： H01M4/925 , H01M4/9016 , H01M4/92
摘要： A supported catalyst includes an oxide carrier, catalyst particles supported on the oxide carrier, and catalyst layers which locate among the catalyst particles, with interface portions among the oxide carrier, the catalyst particles and the catalyst layers. The catalyst layers have a melting point lower than 1,500° C. and contain an oxide or a composite oxide which includes at least one element selected from the group consisting of Mo, W, Sn and Ru.
摘要翻译：载体催化剂包括氧化物载体，负载在氧化物载体上的催化剂颗粒和位于催化剂颗粒之间的催化剂层，其中氧化物载体，催化剂颗粒和催化剂层中的界面部分。催化剂层的熔点低于1500℃，并含有包含选自Mo，W，Sn和Ru中的至少一种元素的氧化物或复合氧化物。

10. 发明授权

US08197965B2 Anode for fuel cell and fuel cell using the same 有权
标题翻译：燃料电池阳极和使用其的燃料电池
公开(公告)号：US08197965B2
公开(公告)日：2012-06-12
申请号：US12201332
申请日：2008-08-29
申请人： Jun Tamura , Yoshihiko Nakano , Wu Mei , Taishi Fukazawa
发明人： Jun Tamura , Yoshihiko Nakano , Wu Mei , Taishi Fukazawa
IPC分类号： H01M4/02 , H01M4/90 , H01M4/92
CPC分类号： H01M4/8605 , H01M4/925 , H01M4/926 , H01M2004/8684 , H01M2008/1095
摘要： This invention provides an anode for a fuel cell which can realize stable output for a long period of time, and a fuel cell using the anode for a fuel cell. The anode for a fuel cell comprises an electrode catalyst layer, the electrode catalyst layer comprising a supported catalyst comprising an electroconductive carrier material and catalyst fine particles supported on the electroconductive carrier material, a proton conductive inorganic oxide, and a proton conductive organic polymer binder, the weight ratio between the supported catalyst (C) and the proton conductive inorganic oxide (SA), WSA/WC, being 0.06 to 0.38, the weight ratio between the proton conductive inorganic oxide (SA) and the proton conductive organic polymer binder (P), WP/WSA, being 0.125 to 0.5.
摘要翻译：本发明提供一种能够长时间实现稳定输出的燃料电池用阳极和使用燃料电池用阳极的燃料电池。用于燃料电池的阳极包括电极催化剂层，该电极催化剂层包含负载的催化剂，其包含导电载体材料和负载在导电载体材料上的催化剂细颗粒，质子传导性无机氧化物和质子传导性有机聚合物粘合剂，载体催化剂（C）和质子传导性无机氧化物（SA）之间的重量比WSA / WC为0.06〜0.38，质子传导性无机氧化物（SA）与质子传导性有机聚合物粘合剂（P ），WP / WSA为0.125〜0.5。

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