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1. 发明申请

US20090192342A1 Process for Oligomerizing Olefins Using a Catalyst Based On Silica-Alumina 有权
标题翻译：使用基于二氧化硅 - 氧化铝的催化剂低聚烯烃的方法
公开(公告)号：US20090192342A1
公开(公告)日：2009-07-30
申请号：US12360231
申请日：2009-01-27
申请人： Vincent COUPARD , Alexandra Chaumonnot , Laurent Simon
发明人： Vincent COUPARD , Alexandra Chaumonnot , Laurent Simon
IPC分类号： C07C2/02 , B01J21/12
CPC分类号： C07C2/10 , C10G50/00 , C10G2300/1081 , C10G2300/1088 , C10G2300/1092 , C10G2400/22
摘要： A process for oligomerizing an olefinic hydrocarbon feed is described which consists of bringing said feed into contact with a catalyst comprising a silica-alumina, the silica content of said catalyst being in the range 5% to 95% by weight, said catalyst being prepared using a process comprising at least: a) mixing at least one alumina compound which is partially soluble in an acid medium with either at least one silica compound which is completely soluble in the reaction mixture or a combination formed by at least one silica compound and at least one alumina compound, said silica and alumina compounds being completely soluble in the reaction mixture, in order to form a solid precursor of said catalyst; b) hydrothermal treatment of the solid derived from step a) by calcining in moist air for a period in the range 4 to 7 hours.
摘要翻译：描述了一种使烯烃进料低聚的方法，其包括使所述进料与包含二氧化硅 - 氧化铝的催化剂接触，所述催化剂的二氧化硅含量在5重量％至95重量％的范围内，所述催化剂使用一种方法至少包括：a）将至少一种部分可溶于酸性介质的氧化铝化合物与至少一种完全可溶于反应混合物的二氧化硅化合物或由至少一种二氧化硅化合物形成的组合物和至少一种氧化铝化合物，所述二氧化硅和氧化铝化合物完全溶于反应混合物中，以形成所述催化剂的固体前体; b）通过在潮湿空气中煅烧4至7小时的时间段对来自步骤a）的固体进行水热处理。

2. 发明授权

US08222470B2 Process for oligomerizing olefins using a catalyst based on silica-alumina 有权
标题翻译：使用基于二氧化硅 - 氧化铝的催化剂使烯烃低聚的方法
公开(公告)号：US08222470B2
公开(公告)日：2012-07-17
申请号：US12360231
申请日：2009-01-27
申请人： Vincent Coupard , Alexandra Chaumonnot , Laurent Simon
发明人： Vincent Coupard , Alexandra Chaumonnot , Laurent Simon
IPC分类号： C07C2/10 , B01J21/12
CPC分类号： C07C2/10 , C10G50/00 , C10G2300/1081 , C10G2300/1088 , C10G2300/1092 , C10G2400/22
摘要： A process for oligomerizing an olefinic hydrocarbon feed is described which consists of bringing said feed into contact with a catalyst comprising a silica-alumina, the silica content of said catalyst being in the range 5% to 95% by weight, said catalyst being prepared using a process comprising at least: a) mixing at least one alumina compound which is partially soluble in an acid medium with either at least one silica compound which is completely soluble in the reaction mixture or a combination formed by at least one silica compound and at least one alumina compound, said silica and alumina compounds being completely soluble in the reaction mixture, in order to form a solid precursor of said catalyst; b) hydrothermal treatment of the solid derived from step a) by calcining in moist air for a period in the range 4 to 7 hours.
摘要翻译：描述了一种使烯烃进料低聚的方法，其包括使所述进料与包含二氧化硅 - 氧化铝的催化剂接触，所述催化剂的二氧化硅含量在5重量％至95重量％的范围内，所述催化剂使用一种方法至少包括：a）将至少一种部分可溶于酸性介质的氧化铝化合物与至少一种完全可溶于反应混合物的二氧化硅化合物或由至少一种二氧化硅化合物形成的组合物和至少一种氧化铝化合物，所述二氧化硅和氧化铝化合物完全溶于反应混合物中，以形成所述催化剂的固体前体; b）通过在潮湿空气中煅烧4至7小时的时间段对来自步骤a）的固体进行水热处理。

3. 发明申请

US20110172482A1 CATALYST BASED ON A CRYSTALLIZED MATERIAL WITH HIERARCHIZED AND ORGANIZED POROSITY AND ITS USE IN OLIGOMERIZATION OF LIGHT OLEFINS 失效
标题翻译：基于结晶化材料的催化剂，具有分层和组织的孔隙度，并且用于轻质烯烃的低分子化
公开(公告)号：US20110172482A1
公开(公告)日：2011-07-14
申请号：US12994194
申请日：2009-04-28
申请人： Amandine Cabiac , Alexandra Chaumonnot , Laurent Simon
发明人： Amandine Cabiac , Alexandra Chaumonnot , Laurent Simon
IPC分类号： C07C2/02 , B01J21/06 , B01J35/10 , B01J29/04 , B01J29/18 , B01J29/65 , B01J29/70 , B01J21/02 , B01J21/04 , B01J21/16 , B01J21/14 , B01J27/182 , B01J21/18
CPC分类号： C07C2/12 , B01J29/041 , B01J29/06 , B01J29/40 , B01J29/7007 , B01J35/023 , B01J37/0009 , B01J37/0045 , B01J2229/42 , C07C2529/40 , C07C2529/70 , C10G50/00
摘要： A catalyst that comprises at least one binder and at least one crystallized material with hierarchized and organized porosity in the fields of microporosity and mesoporosity is described, whereby said crystallized material consists of at least two elementary spherical particles, each of said particles comprising a mesostructured silicon-oxide-based matrix that has a mesopore diameter of between 1.5 and 30 nm and that has microporous and crystallized walls with a thickness of between 1 and 60 nm, whereby said elementary spherical particles have a maximum diameter of 200 microns. Said catalyst is used in a process for oligomerization of an olefinic feedstock that contains hydrocarbon molecules that have 2 to 12 carbon atoms per molecule.
摘要翻译：描述了一种催化剂，其包含至少一种粘合剂和至少一种在微孔和中孔性的领域中具有分级和有组织的孔隙率的结晶材料，由此所述结晶材料由至少两个基本球形颗粒组成，每个所述颗粒包含介孔结构的硅基于氧化物的基质，其中孔直径在1.5至30nm之间，并且具有厚度在1至60nm之间的微孔和结晶壁，由此所述基本球形颗粒的最大直径为200微米。所述催化剂用于含有每分子具有2至12个碳原子的烃分子的烯烃原料低聚的方法。

4. 发明申请

US20110124936A1 PROCEDE DOLIGOMERISATION DES OLEFINS USING LEGERES UTILISANT UN CATALYSEUR A BASE D'UN MATERIAU AMORPHE A POROSITE HIERARCHISEE 失效
标题翻译：使用LEGERES过程加工过程使用说明书联合国催化剂基地D'UN MATERIAU AMORPHE A多孔分子
公开(公告)号：US20110124936A1
公开(公告)日：2011-05-26
申请号：US12994213
申请日：2009-04-28
申请人： Amandine Cabiac , Alexandra Chaumonnot , Laurent Simon
发明人： Amandine Cabiac , Alexandra Chaumonnot , Laurent Simon
IPC分类号： C07C2/24 , C07C2/08
CPC分类号： B01J29/40 , B01J29/06 , B01J35/023 , B01J35/08 , B01J35/108 , B01J37/0009 , B01J37/0045 , B01J2229/62 , C07C2/12 , C07C2529/40 , C07C2529/70 , C10G50/00 , C10G2300/1088 , C10G2300/1092 , C10G2300/4018 , C10G2400/22
摘要： A process for oligomerization of an olefinic feedstock that contains olefinic hydrocarbon molecules that have 2 to 10 carbon atoms per molecule is described, whereby said process comprises bringing said feedstock into contact with a catalyst that comprises at least one amorphous material with hierarchized and organized porosity and consists of at least two elementary spherical particles, each of said particles comprising a mesostructured silicon-oxide-based matrix that has a mesopore diameter of between 1.5 and 30 nm and that exhibits amorphous and microporous walls with a thickness of between 1 and 50 nm, whereby said elementary spherical particles have a maximum diameter of 200 microns.
摘要翻译：描述了含有每分子具有2-10个碳原子的烯属烃分子的烯烃原料的低聚方法，其中所述方法包括使所述原料与包含至少一种具有分级和组织的孔隙率的至少一种无定形材料的催化剂接触，由至少两个基本球形颗粒组成，每个所述颗粒包含介孔结构的基于氧化硅的基质，其中孔直径在1.5至30nm之间，并且具有介于1和50nm之间的无定形和微孔壁，由此所述基本球形颗粒的最大直径为200微米。

5. 发明授权

US08742193B2 Process for oligomerization of light olefins using a catalyst based on an amorphous material with hierarchized and organized porosity 失效
标题翻译：使用基于无定形材料的催化剂轻质烯烃的低聚方法，其具有分级和有组织的孔隙率
公开(公告)号：US08742193B2
公开(公告)日：2014-06-03
申请号：US12994213
申请日：2009-04-28
申请人： Amandine Cabias , Alexandra Chaumonnot , Laurent Simon
发明人： Amandine Cabias , Alexandra Chaumonnot , Laurent Simon
IPC分类号： C07C2/10 , C07C2/12
CPC分类号： B01J29/40 , B01J29/06 , B01J35/023 , B01J35/08 , B01J35/108 , B01J37/0009 , B01J37/0045 , B01J2229/62 , C07C2/12 , C07C2529/40 , C07C2529/70 , C10G50/00 , C10G2300/1088 , C10G2300/1092 , C10G2300/4018 , C10G2400/22
摘要： A process for oligomerization of an olefinic feedstock that contains olefinic hydrocarbon molecules that have 2 to 10 carbon atoms per molecule is described, whereby said process comprises bringing said feedstock into contact with a catalyst that comprises at least one amorphous material with hierarchized and organized porosity and consists of at least two elementary spherical particles, each of said particles comprising a mesostructured silicon-oxide-based matrix that has a mesopore diameter of between 1.5 and 30 nm and that exhibits amorphous and microporous walls with a thickness of between 1 and 50 nm, whereby said elementary spherical particles have a maximum diameter of 200 microns.
摘要翻译：描述了含有每分子具有2-10个碳原子的烯属烃分子的烯烃原料的低聚方法，其中所述方法包括使所述原料与包含至少一种具有分级和组织的孔隙率的至少一种无定形材料的催化剂接触，由至少两个基本球形颗粒组成，每个所述颗粒包含介孔结构的基于氧化硅的基质，其中孔直径在1.5至30nm之间，并且具有介于1和50nm之间的无定形和微孔壁，由此所述基本球形颗粒的最大直径为200微米。

6. 发明授权

US08785707B2 Catalyst based on a crystallized material with hierarchized and organized porosity and its use in oligomerization of light olefins 失效
标题翻译：基于具有分级和有组织孔隙率的结晶材料的催化剂及其在轻烯烃低聚中的应用
公开(公告)号：US08785707B2
公开(公告)日：2014-07-22
申请号：US12994194
申请日：2009-04-28
申请人： Amandine Cabiac , Alexandra Chaumonnot , Laurent Simon
发明人： Amandine Cabiac , Alexandra Chaumonnot , Laurent Simon
IPC分类号： C07C2/12 , B01J29/04 , C10G50/00 , B01J29/40 , B01J35/02 , B01J29/70 , B01J29/06 , B01J37/00
CPC分类号： C07C2/12 , B01J29/041 , B01J29/06 , B01J29/40 , B01J29/7007 , B01J35/023 , B01J37/0009 , B01J37/0045 , B01J2229/42 , C07C2529/40 , C07C2529/70 , C10G50/00
摘要： A catalyst that comprises at least one binder and at least one crystallized material with hierarchized and organized porosity in the fields of microporosity and mesoporosity is described, whereby said crystallized material consists of at least two elementary spherical particles, each of said particles comprising a mesostructured silicon-oxide-based matrix that has a mesopore diameter of between 1.5 and 30 nm and that has microporous and crystallized walls with a thickness of between 1 and 60 nm, whereby said elementary spherical particles have a maximum diameter of 200 microns. Said catalyst is used in a process for oligomerization of an olefinic feedstock that contains hydrocarbon molecules that have 2 to 12 carbon atoms per molecule.
摘要翻译：描述了一种催化剂，其包含至少一种粘合剂和至少一种在微孔和中孔性的领域中具有分级和有组织的孔隙率的结晶材料，由此所述结晶材料由至少两个基本球形颗粒组成，每个所述颗粒包含介孔结构的硅基于氧化物的基质，其中孔直径在1.5至30nm之间，并且具有厚度在1至60nm之间的微孔和结晶壁，由此所述基本球形颗粒的最大直径为200微米。所述催化剂用于含有每分子具有2至12个碳原子的烃分子的烯烃原料低聚的方法。

7. 发明授权

US07476773B2 Process for preparing a gas oil by oligomerization 有权
标题翻译：通过低聚制备瓦斯油的方法
公开(公告)号：US07476773B2
公开(公告)日：2009-01-13
申请号：US11476203
申请日：2006-06-28
申请人： Sylvain Louret , Vincent Coupard , Laurent Simon
发明人： Sylvain Louret , Vincent Coupard , Laurent Simon
IPC分类号： C07C2/00
CPC分类号： C10G50/00
摘要： A process for preparing a gas oil cut comprises the following steps in succession: 1) oligomerizing an olefinic C2-C12 hydrocarbon cut, preferably C3-C7 and more preferably C3-C5; 2) separating the mixture of products obtained in step 1) into three cuts: a light cut containing unreacted C4 and/or C5 olefinic hydrocarbons, an intermediate cut having a T95 in the range 200-220° C. and a heavy cut comprising the complement; T95 being the temperature at which 95% by weight of product has evaporated, as determined in accordance with standard method ASTM D2887; 3) oligomerizing the intermediate cut obtained in the separation step; characterized in that in step 3), oligomerization is carried out in the presence of an olefinic C4 and/or C5 hydrocarbon cut in a weight ratio of intermediate cut to olefinic C4 and/or C5 cut in the range of 60/40 to 80/20.
摘要翻译：一种制备瓦斯油切割的方法包括以下步骤：1）使烯烃C2-C12烃馏分低聚，优选C3-C7，更优选C3-C5; 2）将步骤1）中获得的产物的混合物分成三个切口：含有未反应的C 4和/或C 5烯烃的轻馏分，T95在200-220℃范围内的中间切口，以及包含补充; T95是按照标准方法ASTM D2887测定的95重量％的产品蒸发的温度; 3）使分离步骤中获得的中间切片低聚; 其特征在于在步骤3）中，在中间切割的烯烃C4和/或C5切割重量比为60/40至80 /℃的烯烃C4和/或C5烃切割的存在下进行低聚， 20。

8. 发明申请

US20070015945A1 Process for preparing a gas oil by oligomerization 有权
标题翻译：通过低聚制备瓦斯油的方法
公开(公告)号：US20070015945A1
公开(公告)日：2007-01-18
申请号：US11476203
申请日：2006-06-28
申请人： Sylvain Louret , Vincent Coupard , Laurent Simon
发明人： Sylvain Louret , Vincent Coupard , Laurent Simon
IPC分类号： C07C2/00
CPC分类号： C10G50/00
摘要： The present invention concerns a process for preparing a gas oil cut, which comprises the following steps in succession: 1) oligomerizing an olefinic C2-C12 hydrocarbon cut, preferably C3-C7 and more preferably C3-C5; 2) separating the mixture of products obtained in step 1) into three cuts: a light cut containing unreacted C4 and/or C5 olefinic hydrocarbons, an intermediate cut having a T95 in the range 200-220° C. and a heavy cut comprising the complement; T95 being the temperature at which 95% by weight of product has evaporated, as determined in accordance with standard method ASTM D2887; 3) oligomerizing the intermediate cut obtained in the separation step; characterized in that in step 3), oligomerization is carried out in the presence of an olefinic C4 and/or C5 hydrocarbon cut.
摘要翻译：本发明涉及一种制备瓦斯油切割的方法，其包括以下步骤：1）使烯烃C2-C12烃馏分低聚，优选C 3 -C 7烃馏分，并且更优选C 3 -C 5; 2）将步骤1）中获得的产物的混合物分成三个切口：含有未反应的C 4和/或C 5烯烃的轻馏分，T95在200-220℃范围内的中间切口，以及包含补充; T95是按照标准方法ASTM D2887测定的95重量％的产品蒸发的温度; 3）使分离步骤中获得的中间切片低聚; 其特征在于在步骤3）中，在烯烃C4和/或C5烃馏分存在下进行低聚。

9. 发明授权

US08258071B2 Catalyst in the form of grains comprising an acidic porous core surrounded by a uniform outer layer 失效
标题翻译：包含由均匀外层包围的酸性多孔核的颗粒形式的催化剂
公开(公告)号：US08258071B2
公开(公告)日：2012-09-04
申请号：US10587854
申请日：2005-01-13
申请人： Younes Bouizi , Valentin Valtchev , Loiec Rouleau , Nicolas Bats , Laurent Simon
发明人： Younes Bouizi , Valentin Valtchev , Loiec Rouleau , Nicolas Bats , Laurent Simon
IPC分类号： B01J29/06
CPC分类号： B01J37/0246 , B01J29/035 , B01J29/084 , B01J29/7007 , B01J29/80 , B01J35/023 , B01J2229/62
摘要： The invention relates to a catalyst that comes in the form of grains, each grain consisting of a core covered by at least one external layer, the core consisting of an acidic porous solid and having a size of between 0.1 micron and 0.4 millimeter, in which the external layer has a uniform thickness with a uniformity criterion C, which is less than 0.30, whereby said uniformity criterion C is defined as being equal to an average, on a number N of catalyst grain samples, of the ratio of the difference between the maximum thickness, Eimax, of the external layer and the minimum thickness, Eimin, of this same layer to the average of these two thicknesses Eimax and Eimin.
摘要翻译：本发明涉及一种呈颗粒形式的催化剂，每个颗粒由至少一层外层覆盖的芯组成，芯由酸性多孔固体组成，尺寸为0.1微米至0.4毫米，其中外层具有均匀的厚度，其均匀性标准C小于0.30，其中所述均匀性标准C被定义为等于催化剂颗粒样品数目N上的平均值最大厚度，Eimax以及最小厚度Eimin，与该两个厚度Eimax和Eimin的平均值相同。

10. 发明申请

US20120205286A1 HYDROCRACKING PROCESS USING A ZEOLITE CATALYST CONTAINING TWO DISTINCT HYDROGENATING FUNCTIONS 有权
标题翻译：使用含有两个异步氢化功能的沸石催化剂的水解工艺
公开(公告)号：US20120205286A1
公开(公告)日：2012-08-16
申请号：US13345041
申请日：2012-01-06
申请人： Jeremy FRANCIS , Laurent Simon , Emmanuelle Guillon , Nicolas Bats , Avelino Corma , Christophe Pichon
发明人： Jeremy FRANCIS , Laurent Simon , Emmanuelle Guillon , Nicolas Bats , Avelino Corma , Christophe Pichon
IPC分类号： C10G65/12 , B01J29/04 , C10G47/06
CPC分类号： B01J29/146 , B01J29/166 , B01J35/002 , B01J35/0066 , B01J35/109 , B01J37/0009 , B01J37/0205 , B01J37/20 , B01J2229/14 , B01J2229/16 , B01J2229/186 , B01J2229/20 , B01J2229/36 , B01J2229/37 , B01J2229/38 , B01J2229/42 , C10G49/08 , C10G2300/301 , C10G2300/4018
摘要： Process for hydrocracking and/or hydrotreatment of hydrocarbon feeds utilizing a catalyst comprising at least one hydro-dehydrogenating element of group VIB and of non-precious group VIII used alone or mixed, and a support comprising at least one porous mineral matrix and at least one dealuminated USY zeolite having an overall silicon-to-aluminium atomic ratio comprised between 2.5 and 10, a fraction by weight of extra-network aluminium atom greater than 10% relative to the total mass of the aluminium present in the zeolite, a mesopore volume measured by nitrogen porosimetry greater than 0.07 ml.g−1, and a crystal parameter a0 of the elemental mesh greater than 24.28 Å, in which a quantity of the element nickel comprised between 0.5 and 3% by weight relative to the total mass of the zeolite is deposited on said USY zeolite and in which said catalyst is in the sulphide form.
摘要翻译：使用包含至少一种单独或混合使用的VIB族和非贵重族VIII的加氢脱氢元素的催化剂，以及包含至少一种多孔矿物基质和至少一种多孔矿物基质的载体来加氢裂化和/或加氢处理烃进料的方法具有2.5至10的整体硅 - 铝原子比的脱铝USY沸石，相对于存在于沸石中的铝的总质量大于10％的网络外铝原子的重量百分比，测量的中孔体积通过氮气孔隙度法大于0.07ml.g-1，并且元素网的晶体参数a0大于24.28，其中元素镍的量相对于沸石的总质量为0.5-3重量％沉积在所述USY沸石上，其中所述催化剂为硫化物形式。

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