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1. 发明授权

US07652183B2 Method for producing alkyl aromatic compounds 失效
标题翻译：烷基芳族化合物的制备方法
公开(公告)号：US07652183B2
公开(公告)日：2010-01-26
申请号：US10552434
申请日：2004-04-14
申请人： Ulrich Steinbrenner , Thomas Narbeshuber , Joerg Unger , Peter Zehner , Soeren Zimdahl , Regina Benfer
发明人： Ulrich Steinbrenner , Thomas Narbeshuber , Joerg Unger , Peter Zehner , Soeren Zimdahl , Regina Benfer
IPC分类号： C07C2/66
CPC分类号： C07C303/08 , C07C2/66 , C07C15/107 , C07C303/06 , C07C309/31
摘要： In a process for the preparation of alkylaromatic compounds by reacting C3-30-olefins, or alcohols from which C3-30-olefins are formed under the reaction conditions, with an aromatic hydrocarbon in the presence of an alkylation catalyst, the reaction is carried out in a reactor cascade of at least two reactors, where each of the reactors comprises the alkylation catalyst, at least 80% of the aromatic hydrocarbon are fed into the first reactor of the reactor cascade, and at least 40% of the olefins are intermediately fed in after the first reactor.
摘要翻译：在烷基芳族化合物的制备方法中，在烷基化催化剂的存在下，使C3-30-烯烃或在反应条件下由C 3-30-烯烃形成的醇与芳烃反应，进行反应在至少两个反应器的反应器级联中，其中每个反应器包含烷基化催化剂，至少80％的芳族烃进料到反应器级联的第一反应器中，并且至少40％的烯烃被中间进料在第一反应堆之后。

2. 发明申请

US20060241328A1 Method for producing alkyl aromatic compounds 失效
标题翻译：烷基芳族化合物的制备方法
公开(公告)号：US20060241328A1
公开(公告)日：2006-10-26
申请号：US10552434
申请日：2004-04-14
申请人： Ulrich Steinbrenner , Thomas Narbeshuber , Jörg Unger , Peter Zehner , Soeren Zimdahl , Regina Benfer
发明人： Ulrich Steinbrenner , Thomas Narbeshuber , Jörg Unger , Peter Zehner , Soeren Zimdahl , Regina Benfer
IPC分类号： C07C2/64
CPC分类号： C07C303/08 , C07C2/66 , C07C15/107 , C07C303/06 , C07C309/31
摘要： In a process for the preparation of alkylaromatic compounds by reacting C3-30-olefins, or alcohols from which C3-30-olefins are formed under the reaction conditions, with an aromatic hydrocarbon in the presence of an alkylation catalyst, the reaction is carried out in a reactor cascade of at least two reactors, where each of the reactors comprises the alkylation catalyst, at least 80% of the aromatic hydrocarbon are fed into the first reactor of the reactor cascade, and at least 40% of the olefins are intermediately fed in after the first reactor.
摘要翻译：在制备烷基芳族化合物的方法中，通过使C 3-30 - 烯烃或在反应条件下形成C 3-30 - α-烯烃的醇与式在烷基化催化剂存在下的芳族烃，反应在至少两个反应器的反应器级联中进行，其中每个反应器包含烷基化催化剂，将至少80％的芳烃加入第一反应器的反应器级联，并且至少40％的烯烃在第一反应器之后中间进料。

3. 发明授权

US07601861B2 Method for producing alkylaryl compounds and alkylaryl sulphonates 失效
标题翻译：烷基芳基化合物和烷基芳基磺酸盐的制备方法
公开(公告)号：US07601861B2
公开(公告)日：2009-10-13
申请号：US10577321
申请日：2004-10-29
申请人： Nils Bottke , Regina Benfer , Marco Bosch , Thomas Narbeshuber , Ulrich Steinbrenner , Juergen Stephan
发明人： Nils Bottke , Regina Benfer , Marco Bosch , Thomas Narbeshuber , Ulrich Steinbrenner , Juergen Stephan
IPC分类号： C07C309/31
CPC分类号： C11D1/22 , C07C2/66 , C07C2529/18 , C07C2529/70 , C07C15/107
摘要： In a process for preparing alkylaryl compounds by reacting a C10-14-monoolefin mixture with an aromatic hydrocarbon in the presence of an alkylation catalyst to form alkyl aromatic compounds and if appropriate subsequently sulfonating and neutralizing the resulting alkylaryl compounds, in the C10-14-monoolefins, on average, more than 0% and up to 100% of methyl branches are present in the longest carbon chain and fewer than 50% of the methyl branches are in the 2-, 3- and 4-position, calculated starting from the chain ends of the longest carbon chain.
摘要翻译：在烷基芳基化合物存在下，通过使C10-14-单烯烃混合物与芳族烃反应制备烷基芳基化合物的方法形成烷基芳香族化合物，如果合适，则随后磺化和中和得到的烷基芳基化合物，在C10-14- 平均来说，最长碳链中存在大于0％和高达100％的甲基支链的单烯烃，并且少于50％的甲基支链位于2-，3-和4-位，从最长碳链的链端。

4. 发明申请

US20070142258A1 Method for producing alkylaryl compounds 审中-公开
标题翻译：烷基芳基化合物的制备方法
公开(公告)号：US20070142258A1
公开(公告)日：2007-06-21
申请号：US10583140
申请日：2004-12-17
申请人： Ulrich Steinbrenner , Thomas Heidemann , Michael Roper , Jurgen Stephan , Thomas Narbeshuber , Jurgen Tropsch , Nils Bottke , Regina Benfer
发明人： Ulrich Steinbrenner , Thomas Heidemann , Michael Roper , Jurgen Stephan , Thomas Narbeshuber , Jurgen Tropsch , Nils Bottke , Regina Benfer
IPC分类号： C09D9/00
CPC分类号： C07C6/04 , C07C2/08 , C07C2/66 , C07C5/2506 , C07C303/06 , C11D1/22 , C11D11/04 , C07C309/31 , C07C11/02 , C07C11/10 , C07C15/107
摘要： The preparation of alkylaryl compounds takes place by a) reaction of a C4/C5-olefin mixture over a metathesis catalyst to prepare a C4-8-olefin mixture comprising 2-pentene, and optional removal of the C4-8-olefin mixture, b) removal of from 5 to 100% of the 2-pentene present in stage a) and subsequent reaction over an isomerization catalyst to give a mixture of 2-pentene and 1-pentene which is returned to stage a), c) dimerization of the C4-8-olefin mixture obtained in stage b) following removal in the presence of a dimerization catalyst to give a mixture containing C8-16-olefins, removal of these C8-16-olefins and optional removal of a partial stream thereof, d) reaction of the c8-16-olefin mixtures obtained in stage c) or of the partial stream with an aromatic hydrocarbon in the presence of an alkylation catalyst to form alkyl aromatic compounds where, prior to the reaction, 0 to 60% by weight, based on the c8-16-olefin mixtures obtained in stage c), of linear olefins may additionally be added, e) optional sulfonation of the alkyl aromatic compounds obtained in stage d) and neutralization to give alkylarylsulfonates, where, prior to the sulfonation, 0 to 60% by weight, based on the alkyl aromatic compounds obtained in stage d), of linear alkylbenzenes may additionally be added if no admixing has taken place in stage d), f) optional mixing of the alkylarylsulfonates obtained in stage e) with 0 to 60% by weight, based on the alkylarylsulfonates obtained in stage e), of linear alkylarylsulfonate, if no admixing has taken place in stages d) and e).
摘要翻译：烷基芳基化合物的制备通过以下步骤进行：a）在复分解催化剂上使C 4-14 C 5 -C 5 - 烯烃混合物反应以制备C 4-8 - 其包含2-戊烯，任选地除去C 4-18α-烯烃混合物，b）除去在步骤a）中存在的5-100％的2-戊烯，并随后在异构化催化剂上反应，得到2-戊烯和1-戊烯的混合物，将其返回到a）步骤，c）在步骤b中获得的C 4-18α-烯烃混合物的二聚反应），在二聚催化剂存在下除去，得到含有C 8-16 - 烯烃的混合物，除去这些C 8-16 - 烯烃并任选地除去其部分流，d）在烷基化催化剂存在下，将阶段c）或部分流中获得的C 8-16 - α-烯烃混合物与芳族烃反应，形成烷基芳族化合物，其中在反应之前，0至60重量％，b 在阶段c）中得到的C 8-16α-烯烃混合物中，可以另外加入线性烯烃，e）任选的在步骤d）中获得的烷基芳族化合物磺化，中和得到烷基芳基磺酸盐，其中在磺化之前，如果在步骤d）中没有混合，则可以另外加入基于直链烷基苯中得到的直链烷基苯0至60重量％，f）任选混合如果在阶段d）和e）中没有混合，则在阶段e）中获得的烷基芳基磺酸盐以0至60重量％的量计，基于阶段e）中得到的烷基芳基磺酸盐，为直链烷基芳基磺酸盐。

5. 发明申请

US20070078075A1 Method for producing alkylaryl compounds and alklaryl sulphonates 失效
标题翻译：烷基芳基化合物和烷芳基磺酸盐的制备方法
公开(公告)号：US20070078075A1
公开(公告)日：2007-04-05
申请号：US10577321
申请日：2004-10-29
申请人： Nils Bottke , Regina Benfer , Marco Bosch , Thomas Narbeshuber , Ulrich Steinbrenner , Jurgen Stephan
发明人： Nils Bottke , Regina Benfer , Marco Bosch , Thomas Narbeshuber , Ulrich Steinbrenner , Jurgen Stephan
IPC分类号： C11D17/08 , C07C309/24
CPC分类号： C11D1/22 , C07C2/66 , C07C2529/18 , C07C2529/70 , C07C15/107
摘要： In a process for preparing alkylaryl compounds by reacting a C10-14-monoolefin mixture with an aromatic hydrocarbon in the presence of an alkylation catalyst to form alkyl aromatic compounds and if appropriate subsequently sulfonating and neutralizing the resulting alkylaryl compounds, in the C10-14-monoolefins, on average, more than 0% and up to 100% of methyl branches are present in the longest carbon chain and fewer than 50% of the methyl branches are in the 2-, 3- and 4-position, calculated starting from the chain ends of the longest carbon chain.
摘要翻译：在烷基芳基化合物的存在下通过使C 10-14 - 单烯烃混合物与芳族烃反应制备烷基芳基化合物的方法，以形成烷基芳族化合物，并且如果合适，则随后磺化和中和所得的烷基芳基在最长的碳链中存在C 10-14 - 单烯烃中的平均超过0％和高达100％的甲基支链的化合物，少于50％的甲基支链是在2-，3-和4-位，从最长碳链的链端开始计算。

6. 发明申请

US20070225189A1 Surfactant Composition And Method Of Forming 有权
标题翻译：表面活性剂组合物和形成方法
公开(公告)号：US20070225189A1
公开(公告)日：2007-09-27
申请号：US11677824
申请日：2007-02-22
申请人： James Dailey , Ernst Lippert , Sridhar Iyer , Ulrich Steinbrenner , Christoffer Kieburg , Jurgen Tropsch , Richard Baur , Soeren Zimdahl
发明人： James Dailey , Ernst Lippert , Sridhar Iyer , Ulrich Steinbrenner , Christoffer Kieburg , Jurgen Tropsch , Richard Baur , Soeren Zimdahl
IPC分类号： C11D3/00
CPC分类号： C11D1/8255 , A01N25/30 , C11D1/29 , C11D1/345 , C11D1/37 , C11D1/72 , C11D1/8305 , C11D3/0026 , D06M13/17 , D06M15/53
摘要： A surfactant composition includes a first surfactant, a second surfactant, and a polyalkylene glycol. The first surfactant is of the general formula R1—O-(A)mH, wherein R1 is an aliphatic hydrocarbon having 10 carbon atoms, A is an alkyleneoxy group having from 2 to 5 carbon atoms, and m is a positive number. The second surfactant is of the general formula R2—O—(B)nH, wherein R2 is an aliphatic hydrocarbon having from 12 to 14 carbon atoms, B is an alkyleneoxy group having from 2 to 5 carbon atoms, and n is a positive number. The polyalkylene glycol is present in the surfactant composition in an amount of from 3 to 20 parts by weight per 100 parts by weight of the surfactant composition.
摘要翻译：表面活性剂组合物包括第一表面活性剂，第二表面活性剂和聚亚烷基二醇。第一表面活性剂具有通式R 1 -O -O-（A）m H，其中R 1是具有10个碳原子的脂族烃原子，A是具有2至5个碳原子的亚烷氧基，m是正数。第二表面活性剂具有通式R 2 -O-（B）n H，其中R 2是具有12个碳原子的脂族烃，至14个碳原子，B为具有2至5个碳原子的亚烷基氧基，n为正数。表面活性剂组合物中存在的聚亚烷基二醇的量为每100重量份表面活性剂组合物3至20重量份。

7. 发明授权

US07504373B2 Surfactant composition and method of forming 有权
标题翻译：表面活性剂组成和形成方法
公开(公告)号：US07504373B2
公开(公告)日：2009-03-17
申请号：US11677824
申请日：2007-02-22
申请人： James S. Dailey , Ernst Lippert , Sridhar Iyer , Ulrich Steinbrenner , Christoffer Kieburg , Juergen Tropsch , Richard Baur , Soeren Zimdahl
发明人： James S. Dailey , Ernst Lippert , Sridhar Iyer , Ulrich Steinbrenner , Christoffer Kieburg , Juergen Tropsch , Richard Baur , Soeren Zimdahl
IPC分类号： C11D1/72 , C11D1/825 , C11D3/20 , C11D11/04
CPC分类号： C11D1/8255 , A01N25/30 , C11D1/29 , C11D1/345 , C11D1/37 , C11D1/72 , C11D1/8305 , C11D3/0026 , D06M13/17 , D06M15/53
摘要： A surfactant composition includes a first surfactant, a second surfactant, and a polyalkylene glycol. The first surfactant is of the general formula R1—O—(A)mH, wherein R1 is an aliphatic hydrocarbon having 10 carbon atoms, A is an alkyleneoxy group having from 2 to 5 carbon atoms, and m is a positive number. The second surfactant is of the general formula R2—O—(B)nH, wherein R2 is an aliphatic hydrocarbon having from 12 to 14 carbon atoms, B is an alkyleneoxy group having from 2 to 5 carbon atoms, and n is a positive number. The polyalkylene glycol is present in the surfactant composition in an amount of from 3 to 20 parts by weight per 100 parts by weight of the surfactant composition.
摘要翻译：表面活性剂组合物包括第一表面活性剂，第二表面活性剂和聚亚烷基二醇。第一表面活性剂具有通式R 1 -O-（A）m H，其中R 1是具有10个碳原子的脂族烃，A是具有2至5个碳原子的亚烷基氧基，m是正数。第二表面活性剂为通式R 2 -O-（B）n H，其中R 2为具有12至14个碳原子的脂族烃，B为具有2至5个碳原子的亚烷氧基，n为正数。表面活性剂组合物中存在的聚亚烷基二醇的量为每100重量份表面活性剂组合物3至20重量份。

8. 发明申请

US20090023820A1 SURFACTANT MIXTURE CONTAINING SHORT-CHAIN AND ALSO LONG-CHAIN COMPONENTS 审中-公开
标题翻译：含短链和长链组分的表面活性剂混合物
公开(公告)号：US20090023820A1
公开(公告)日：2009-01-22
申请号：US12280114
申请日：2007-02-15
申请人： James S. Dailey , Ernst Lippert , Sridhar G. Iyer , Ulrich Steinbrenner , Christoffer Kieburg , Jurgen Tropsch , Richard Baur , Soeren Zimdahl
发明人： James S. Dailey , Ernst Lippert , Sridhar G. Iyer , Ulrich Steinbrenner , Christoffer Kieburg , Jurgen Tropsch , Richard Baur , Soeren Zimdahl
IPC分类号： B01F17/38
CPC分类号： C11D1/8255 , A01N25/30 , C11D1/29 , C11D1/345 , C11D1/37 , C11D1/72 , C11D1/8305 , C11D3/0026 , D06M13/17 , D06M15/53
摘要： The present invention relates to a surfactant mixture comprising (A) a short-chain component comprising the alkoxylation product of alkanols, where the alkanols have 8 to 12 carbon atoms and the average number of alkoxy groups per alkanol group in the alkoxylation product assumes a value from 3 to 30 and the alkoxy groups are chosen from the group consisting of ethoxy, propoxy, butoxy and pentoxy groups and the alkanols have an average degree of branching of at least 1; and (B) a long-chain component comprising the alkoxylation product of alkanols where the alkanols have 13 to 20 carbon atoms and the average number of alkoxy groups per alkanol group in the alkoxylation product assumes a value from 3 to 30 and the alkoxy groups are chosen from the group consisting of ethoxy, propoxy, butoxy and pentoxy groups and the alkanols have an average degree of branching of from 0.0 to 0.3; and phosphate esters, sulfate esters and ether carboxylates thereof. In addition, the present invention relates to a formulation comprising such surfactant mixtures, and to the use of these, for example for the cleaning of hard surfaces.
摘要翻译：本发明涉及一种表面活性剂混合物，其包含（A）包含烷醇的烷氧基化产物的短链组分，其中烷醇具有8至12个碳原子，并且烷氧基化产物中每个烷醇基团的烷氧基的平均数呈现值 3至30，并且烷氧基选自乙氧基，丙氧基，丁氧基和戊氧基，并且所述链烷醇具有至少1的平均支化度; 和（B）包含烷醇的烷氧基化产物的长链组分，其中链烷醇具有13-20个碳原子，烷氧基化产物中每个烷醇基团的烷氧基的平均数为3-30，烷氧基为选自乙氧基，丙氧基，丁氧基和戊氧基，并且所述链烷醇的平均支化度为0.0至0.3; 和磷酸酯，硫酸酯和醚羧酸盐。此外，本发明涉及包含这种表面活性剂混合物的制剂，以及这些用于清洁硬表面的用途。

9. 发明授权

US06262325B1 Basic catalyst based on titanates, zirconates and hafnates 失效
标题翻译：基于钛酸盐，锆酸盐和铪的基本催化剂
公开(公告)号：US06262325B1
公开(公告)日：2001-07-17
申请号：US09412604
申请日：1999-10-06
申请人： Thomas Narbeshuber , Ulrich Steinbrenner
发明人： Thomas Narbeshuber , Ulrich Steinbrenner
IPC分类号： C07C266
CPC分类号： B01J21/06 , B01J21/063 , B01J21/066 , B01J23/002 , B01J23/02 , B01J23/04 , B01J2523/00 , C07C2/72 , C07C2521/06 , C07C2521/10 , C07C2523/02 , C07C2523/04 , C07C2523/06 , C07C2523/14 , C07C2523/745 , C07C2523/75 , C07C2523/755 , Y10S502/525 , C07C15/00 , B01J2523/23 , B01J2523/48 , B01J2523/47 , B01J2523/22 , B01J2523/25
摘要： The catalyst comprises at least one alkali metal on a support which has the general formula (I) An′Tim′Zrp′Hfq′On′+2(m′+p′+q′) (I) where A is a divalent metal, 20·(m′+p′+q′)>n′>0.05·(m′+p′+q′), and which may be doped with at least one compound of an alkali metal and/or alkaline earth metal, where the alkali metal/support ratio by weight is 0.01-5:1 and, when a dopant is present, the dopant/support ratio by weight is 0.01-5:1, and where the proportion of support phase corresponding to the ZrO2 structure or an alkaline earth metal oxide structure or consisting of ZrO2 or alkaline earth metal oxide is less than 10% by weight. The catalyst is used for the side-chain alkylation or alkenylation of alkylaromatic compounds with olefins or diolefins, for the double-bond isomerization of olefins, for the dimerization of olefins, for the coupling of aromatic nuclei and for the amination of olefins and conjugated diolefins.
摘要翻译：催化剂包含至少一种碱金属，其具有通式（I），其中A是二价金属，20（m'+ p'+ q'）> n'> 0.05（m'+ p'+ q'），并且其可以掺杂有至少一种碱金属和/或碱土金属的化合物，其中碱金属/载体重量比为0.01-5:1，并且当存在掺杂剂时，掺杂剂 /载体重量比为0.01-5:1，其中对应于ZrO 2结构或碱土金属氧化物结构或由ZrO 2或碱土金属氧化物组成的支撑相的比例小于10重量％。催化剂用于烷基芳基化合物与烯烃或二烯烃的侧链烷基化或链烯基化，用于烯烃的双键异构化，用于烯烃的二聚，芳族核的偶联和用于烯烃和共轭二烯烃的胺化。

10. 发明授权

US06870014B2 Catalyst and method for producing polytetrahydrofurane 失效
标题翻译：催化剂和生产聚四氢呋喃的方法
公开(公告)号：US06870014B2
公开(公告)日：2005-03-22
申请号：US10312860
申请日：2001-07-02
申请人： Ulrich Steinbrenner , Thomas Narbeshuber , Martin Haubner , Christoph Sigwart , Gerd Linden , Gerhard Cox , Rolf-Hartmuth Fischer , Michael Hesse , Gerd Bohner , Hartmut Hibst , Ekkehard Schwab , Andreas Tenten
发明人： Ulrich Steinbrenner , Thomas Narbeshuber , Martin Haubner , Christoph Sigwart , Gerd Linden , Gerhard Cox , Rolf-Hartmuth Fischer , Michael Hesse , Gerd Bohner , Hartmut Hibst , Ekkehard Schwab , Andreas Tenten
IPC分类号： C08G65/10 , B01J21/06 , B01J23/28 , B01J23/30 , B01J27/188 , B01J35/00 , B01J35/10 , B01J37/00 , C08G65/20 , C08G65/26 , C08F4/06 , B01J23/00 , C08F4/40 , C08F4/42 , C08F124/00
CPC分类号： B01J37/0018 , B01J21/063 , B01J21/066 , B01J23/28 , B01J23/30 , B01J27/188 , B01J35/1019 , B01J35/1038 , B01J35/1042 , B01J35/1061 , C08G65/20 , C08G65/266 , C08G65/2666 , C08G65/2693
摘要： The invention relates to a catalyst which contains a catalytically active quantity of at least one oxygen-containing molybdenum and/or wolfram compound on an oxidic support material and which has been calcinated at temperatures of 400 to 900° C. after the precursor compound of the catalytically active compounds have been applied to the support material or to a support material precursor. The transport pores for this catalyst each have a diameter of >25 nm and a volume of at least 50 mm3/g. The catalyst contains x μmol (wolfram and/or molybdenum)/m2 molybdenum and/or wolfram, with 10.1
摘要翻译：本发明涉及一种催化剂，其在氧化载体材料上含有至少一种含氧钼和/或钨化合物的催化活性量，并且在400-900℃的温度下煅烧之后，催化活性化合物已经施加到载体材料或载体材料前体上。该催化剂的输送孔各自具有> 25nm的直径和至少50mm 3 / g的体积。该催化剂含有xmumol（钨和/或钼）/ m 2钼和/或钨，相对于成品催化剂为10.1

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