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1. 发明专利

JP2007117810A Hydrogen permeable membrane and fuel cell using the same 审中-公开
标题翻译：氢化透明膜和燃料电池使用相同
公开(公告)号：JP2007117810A
公开(公告)日：2007-05-17
申请号：JP2005310225
申请日：2005-10-25
申请人： Sumitomo Electric Ind Ltd , Toyota Motor Corp , トヨタ自動車株式会社 , 住友電気工業株式会社
发明人： MIZUNO OSAMU , IIJIMA MASAHIKO
IPC分类号： B01D71/02 , B01D69/12 , C01B3/56 , H01M8/02 , H01M8/12
CPC分类号： Y02E60/525
摘要： PROBLEM TO BE SOLVED: To provide a hydrogen permeable membrane which is composed of a Pd membrane, a hydrogen permeable base material using V or a V alloy and an intermediate layer containing other elements of the group V, and can suppress the degradation of hydrogen permeability with time by oxidation, and to provide a fuel cell which uses the hydrogen permeable membrane and is improved the problem that the hydrogen permeability is degraded with time. SOLUTION: The hydrogen permeable membraneis composed of the hydrogen permeable base material using V or a V alloy, hydrogen permeable Pd membrane containing Pd, and the intermediate layer provided between the hydrogen permeable base material and Pd membrane. The intermediate layer contains elements of the group V other than V, and has a dense structure. The fuel cell uses the hydrogen permeable membrane. COPYRIGHT: (C)2007,JPO&INPIT
摘要翻译：要解决的问题：提供由Pd膜，使用V或V合金的氢渗透性基材和含有V族其他元素的中间层构成的氢透过膜，并且可以抑制劣化通过氧化时的氢渗透性随时间变化，并且提供使用氢可渗透膜的燃料电池，并且改善了氢渗透性随时间劣化的问题。解决方案：使用V或V合金的氢渗透性基材，含有Pd的氢可渗透Pd膜，以及设置在氢透过性基材与Pd膜之间的中间层构成的氢透过膜。中间层包含V以外的V族元素，具有致密结构。燃料电池使用氢可渗透膜。版权所有（C）2007，JPO＆INPIT

2. 发明专利

JP2007141669A Hydrogen permeation structure, manufacturing method of the same, and fuel cell using the same 有权
标题翻译：氢气渗透结构及其制造方法及使用其的燃料电池
公开(公告)号：JP2007141669A
公开(公告)日：2007-06-07
申请号：JP2005334382
申请日：2005-11-18
申请人： Sumitomo Electric Ind Ltd , Toyota Motor Corp , トヨタ自動車株式会社 , 住友電気工業株式会社
发明人： KAMIMURA TAKU , BOKU TATSUTAMA , IIJIMA MASAHIKO
IPC分类号： H01M8/02
CPC分类号： Y02E60/50
摘要： PROBLEM TO BE SOLVED: To provide a hydrogen permeation structure having a hydrogen permeative base material and an oxide proton conductive film, excellent in tight adhering property between the hydrogen permeative base material and the oxide proton conductive film, hardly generating exfoliation of the oxide proton conductive film, and to provide a manufacturing method of the same and a fuel cell using the same. SOLUTION: The hydrogen permeation structure is composed of the hydrogen permeative base material, an oxide proton conductive film, and an intermediate layer on both surfaces of which the hydrogen permeative base material and the oxide proton conductive film are adhered respectively. The intermediate layer contains a main element A constituting an intermediate layer side surface part of the hydrogen permeative base material, and a main metallic element B contained in constituent element of the oxide proton conductive film. The ratio of the number of atoms A/B of the A and B is not less than 0.1. The manufacturing method of the same and the fuel cell using the same are provided. COPYRIGHT: (C)2007,JPO&INPIT
摘要翻译：要解决的问题：为了提供具有氢渗透性基材和氧化物质子传导膜的氢透过结构，在透氢性基材与氧化物质子传导膜之间的紧密附着性优异，几乎不产生剥离氧化物质子传导膜，并提供其制造方法和使用其的燃料电池。解决方案：氢渗透结构由氢渗透性基材，氧化物质子传导膜和两个表面上分别粘附有氢渗透性基材和氧化物质子传导膜的中间层构成。中间层包含构成氢渗透性基材的中间层侧表面部分的主要元素A和包含在氧化物质子传导膜的构成元素中的主要金属元素B. A和B的原子数A / B的比例不小于0.1。提供其制造方法和使用其的燃料电池。版权所有（C）2007，JPO＆INPIT

3. 发明专利

JP2007090132A Hydrogen permeable membrane and fuel cell using it 审中-公开
标题翻译：氢气渗透膜和燃料电池使用它
公开(公告)号：JP2007090132A
公开(公告)日：2007-04-12
申请号：JP2005279140
申请日：2005-09-27
申请人： Sumitomo Electric Ind Ltd , Toyota Motor Corp , トヨタ自動車株式会社 , 住友電気工業株式会社
发明人： MIZUNO OSAMU , IIJIMA MASAHIKO
IPC分类号： B01D71/02 , B01D53/22 , B01D69/10 , B01D69/12 , H01M8/02 , H01M8/12
CPC分类号： H01M4/8657 , B01D67/0069 , B01D67/0072 , B01D69/12 , B01D71/022 , B01D2325/04 , B01D2325/28 , C01B3/505 , H01M4/8807 , H01M4/8867 , H01M4/8871 , H01M4/92 , H01M4/94 , H01M8/0232 , H01M8/0245 , Y10T428/12493
摘要： PROBLEM TO BE SOLVED: To provide a hydrogen permeable membrane comprising a hydrogen permeable base material using V or a V alloy, an intermediate layer containing other elements of the group V and a Pd membrane, in which mutual diffusion among the hydrogen permeable base material, intermediate layer and Pd membrane is suppressed, and a problem of lowering of hydrogen permeability with time is resolved, and to provide a fuel cell in which a problem of deterioration with time is improved by using the hydrogen permeable membrane. SOLUTION: This hydrogen permeable membrane comprises the hydrogen permeable base material using V or a V alloy, the hydrogen permeable Pd membrane containing Pd, and the intermediate layer provided between the hydrogen permeable base material and the Pd membrane. The intermediate layer has a layer of the group V containing elements selected from the group V, different from the element in the hydrogen permeable base material, in contact with the hydrogen permeable base material, and has an iron group layer containing elements selected from the group VIII, IX or X, with a thickness from 1nm to 100nm in contact with the Pd membrane. The fuel cell uses the hydrogen permeable membrane. COPYRIGHT: (C)2007,JPO&INPIT
摘要翻译：要解决的问题：提供一种使用V或V合金的含氢透过性基材的氢透过膜，含有V族其他元素的中间层和Pd膜，其中透氢性基材，中间层和Pd膜被抑制，并且解决了渗透性随时间降低的问题，并且提供了通过使用氢可渗透膜来提高劣化问题的燃料电池。解决方案：该氢可渗透膜包括使用V或V合金的氢可渗透基材，含Pd的氢可渗透Pd膜，以及设置在氢透过性基材和Pd膜之间的中间层。中间层具有含有选自V组的V族元素，V族不同于氢可渗透性基材中的元素，与氢可渗透性基材接触，并且具有含有选自基团 VIII，IX或X，与Pd膜接触，厚度为1nm至100nm。燃料电池使用氢可渗透膜。版权所有（C）2007，JPO＆INPIT

4. 发明专利

JP2007048569A Oxide proton-conductive film, hydrogen permeation structure, and its manufacturing method 有权
标题翻译：氧化物导电膜，氢气渗透结构及其制造方法
公开(公告)号：JP2007048569A
公开(公告)日：2007-02-22
申请号：JP2005231125
申请日：2005-08-09
申请人： Sumitomo Electric Ind Ltd , Toyota Motor Corp , トヨタ自動車株式会社 , 住友電気工業株式会社
发明人： YAMAKAWA AKIRA , KAMIMURA TAKU , MIZUNO OSAMU , IIJIMA MASAHIKO
IPC分类号： H01B1/08 , C01B3/56 , C01F17/00 , C01G23/00 , C01G25/00 , C01G27/00 , C23C16/40 , G01N27/406 , H01M8/02 , H01M8/12
CPC分类号： Y02E60/525
摘要： PROBLEM TO BE SOLVED: To provide an oxide proton-conductive film having little faults such as pinholes, a high reliability and a high proton conductivity, to provide a hydrogen permeation structure using the oxide proton-conductive film, and to provide a manufacturing method of the hydrogen permeation structure. SOLUTION: The oxide proton-conductive film is composed of a perovskite structure oxide represented by the general formula A a L b(1-x) M bx O 3 (A represents an element selected from Ba, Mg, Ca and Sr; L represents an element selected from Ce, Zr, Ti and Hf; M represents an element selected from elements of group 3 and group 13; and 0.5 COPYRIGHT: (C)2007,JPO&INPIT
摘要翻译：解决问题：为了提供使用该氧化物质子传导膜的氢透过结构，能够提供具有小针孔，高可靠性，高质子传导性的故障的氧化物质子传导膜，氢渗透结构的制造方法。解决方案：氧化物质子传导膜由通式A表示的钙钛矿结构氧化物组成.B（1-x） M （A表示选自Ba，Mg，Ca和Sr的元素; L表示选自Ce，Zr，Ti和Hf的元素; M表示选自元素中的元素的组3和组13;和0.5

5. 发明专利

JP2007021416A Oxide proton conductive film and hydrogen permeable structure containing the same 有权
标题翻译：氧化物导电膜和含有其的氢渗透结构
公开(公告)号：JP2007021416A
公开(公告)日：2007-02-01
申请号：JP2005209083
申请日：2005-07-19
申请人： Sumitomo Electric Ind Ltd , Toyota Motor Corp , トヨタ自動車株式会社 , 住友電気工業株式会社
发明人： YAMAKAWA AKIRA , KAMIMURA TAKU , MIZUNO OSAMU , IIJIMA MASAHIKO
IPC分类号： B01D71/02 , B01D69/12 , C23C14/08 , G01N27/406 , H01B1/06 , H01M8/02
CPC分类号： Y02E60/50
摘要： PROBLEM TO BE SOLVED: To provide an oxide proton conductive film which contains metals such as alkali earth metals, Ce and Zr, and is composed of an oxide having a perovskite type crystal structure, and has high proton conductivity, and has strong adhesion strength to a hydrogen permeable substrate, and to provide a hydrogen permeable structure comprising the oxide proton conductive film and the hydrogen permeable substrate, and in which the exfoliation of the oxide proton conductive film from the hydrogen permeable substrate is hard to occur. SOLUTION: The oxide proton conductive film comprises the oxide represented by a formula: Ba x M y L z O 3 , (wherein M is Ce or Zr; L is a group III element in the short period type periodic table; and 0 COPYRIGHT: (C)2007,JPO&INPIT
摘要翻译：要解决的问题：提供含有碱土金属，Ce和Zr等金属的氧化物质子传导膜，由具有钙钛矿型晶体结构的氧化物构成，具有高质子传导性，并且具有强的并且提供包含氧化物质子传导膜和氢可渗透基底的氢可渗透结构，并且其中难以发生氧化物质子传导膜从氢可渗透基底的剥离。＆lt; P＆gt;解决方案：氧化物质子传导膜包含由下式表示的氧化物：Ba X Y （其中M是Ce或Zr; L是短周期型周期表中的III族元素; 0

6. 发明专利

JP2013089569A Electrolyte membrane, and method for manufacturing the same 审中-公开
标题翻译：电解质膜及其制造方法
公开(公告)号：JP2013089569A
公开(公告)日：2013-05-13
申请号：JP2011232014
申请日：2011-10-21
申请人： Toyota Motor Corp , トヨタ自動車株式会社
发明人： OKADA YOSHIO , IZAWA YASUHIRO , ITO NAOKI , IIJIMA MASAHIKO
IPC分类号： H01M8/02 , H01B1/06 , H01B13/00 , H01M8/12
CPC分类号： Y02P70/56
摘要： PROBLEM TO BE SOLVED: To provide an electrolyte membrane in which the formation of a solid solution of a zirconia-based electrolyte and a ceria-based electrolyte is suppressed, and to provide a method for manufacturing the same.SOLUTION: A method for manufacturing an electrolyte membrane (30) comprises: a preparing step of preparing a laminate formed by laminating a ceria-based electrolyte green layer (32) and a zirconia-based electrolyte green layer (31); and calcining step of calcining the ceria-based electrolyte green layer and the zirconia-based electrolyte green layer. The laminate includes: a sintering-resistant layer with sintering resistant property at the interface between the ceria-based electrolyte green layer and the zirconia-based electrolyte green layer; and a readily sinterable layer with sinterable property at a position other than the interface.
摘要翻译：要解决的问题：提供抑制氧化锆系电解质和氧化铈电解质的固溶体的形成的电解质膜，并提供其制造方法。电解质膜（30）的制造方法包括：准备层叠氧化铈系电解质生层（32）和氧化锆系电解质绿层（31）而形成的层叠体的准备工序。以及煅烧二氧化铈基电解质绿层和氧化锆基电解质绿层的煅烧步骤。层压体包括：在二氧化铈基电解质绿层和氧化锆基电解质绿层之间的界面处具有耐烧结性的耐烧结层; 以及在界面以外的位置具有可烧结性的易烧结层。版权所有（C）2013，JPO＆INPIT

7. 发明专利

JP2011096420A Method for manufacturing electrode-electrolyte membrane assembly and fuel cell 审中-公开
标题翻译：制造电极 - 电解质膜组件和燃料电池的方法
公开(公告)号：JP2011096420A
公开(公告)日：2011-05-12
申请号：JP2009247293
申请日：2009-10-28
申请人： Toyota Motor Corp , トヨタ自動車株式会社
发明人： OKADA YOSHIO , IIJIMA MASAHIKO
IPC分类号： H01M8/02 , H01M8/12
CPC分类号： Y02P70/56
摘要： PROBLEM TO BE SOLVED: To provide a method for manufacturing an electrode-electrolyte membrane assembly, which can restrain separation of gallium from an electrolyte material at the time of a calcining process, and to provide a fuel cell. SOLUTION: The method for manufacturing an electrode-electrolyte membrane assembly includes a deposition step of depositing an electrolyte material (20) including lanthanum gallate oxide on either of a fuel electrode (10) and an air electrode (30) (step S10); and a calcination step of calcining the electrolyte material in a space where gallium or a gallium compound is arranged (step S20). Gallium in the electrolyte material can be restrained from desorption caused by reduction at the time of the calcination process according to this manufacturing method. COPYRIGHT: (C)2011,JPO&INPIT
摘要翻译：要解决的问题：提供一种用于制造电极 - 电解质膜组件的方法，其可以在煅烧过程中抑制镓与电解质材料的分离并提供燃料电池。解决方案：电极 - 电解质膜组件的制造方法包括沉积步骤，在燃料电极（10）和空气电极（30）中的任一个上沉积包含没有没有的镧镓的氧化镧的电解质材料（步骤S10））; 以及在布置镓或镓化合物的空间中煅烧电解质材料的煅烧步骤（步骤S20）。根据该制造方法，电解质材料中的镓可以被抑制在煅烧过程时的还原引起的解吸附。版权所有（C）2011，JPO＆INPIT

8. 发明专利

JP2009252418A Manufacturing method of proton conductor, and manufacturing method of fuel cell 审中-公开
标题翻译：原子导体的制造方法和燃料电池的制造方法
公开(公告)号：JP2009252418A
公开(公告)日：2009-10-29
申请号：JP2008096555
申请日：2008-04-02
申请人： Toyota Motor Corp , トヨタ自動車株式会社
发明人： IIJIMA MASAHIKO
IPC分类号： H01B13/00 , C01B25/45 , C23C14/24 , H01M4/94 , H01M8/02 , H01M8/12
CPC分类号： Y02P70/56
摘要： PROBLEM TO BE SOLVED: To provide a manufacturing method of a proton conductor which suppresses deliquescence, and a manufacturing method of a fuel cell. SOLUTION: The manufacturing method of the proton conductor 30 includes a process for forming the proton conductor formed of AB 2 O 7 type electrolyte in which an A site contains Sn and a B site contains P by using a physical vapor deposition method. The manufacturing method of the fuel cell 100 includes a film forming process for forming the proton conductor 130 formed of the AB 2 O 7 type electrolyte, in which the A site contains Sn and the B side contains P, on a first electrode 110 by using the physical vapor deposition method, and a process for arranging a second electrode 140 on an opposite surface to an anode of the proton conductor after the film forming process. COPYRIGHT: (C)2010,JPO&INPIT
摘要翻译：要解决的问题：提供抑制潮解的质子导体的制造方法以及燃料电池的制造方法。＆lt; P＆gt;解决方案：质子导体30的制造方法包括形成由AB单元形成的质子导体的方法，其中A位含有Sn 并且B位置通过使用物理气相沉积法包含P。燃料电池100的制造方法包括用于形成由AB SB> 7 型电解质形成的质子导体130的成膜工艺，其中A部位含有Sn 并且B侧通过使用物理气相沉积法在第一电极110上包含P，以及在成膜处理之后在与质子导体的阳极相反的表面上布置第二电极140的工艺。版权所有（C）2010，JPO＆INPIT

9. 发明专利

JP2008282570A Method and device for membrane deposition 审中-公开
标题翻译：膜沉积的方法和装置
公开(公告)号：JP2008282570A
公开(公告)日：2008-11-20
申请号：JP2007123417
申请日：2007-05-08
申请人： Toyota Motor Corp , トヨタ自動車株式会社
发明人： ITO NAOKI , IIJIMA MASAHIKO , IZAWA YASUHIRO
IPC分类号： H01M8/02 , H01M8/04
CPC分类号： Y02E60/50
摘要： PROBLEM TO BE SOLVED: To provide a method and device for depositing an electrolyte membrane in which the occurrence of penetrating defects in the electrolyte membrane can be controlled.
SOLUTION: The method of depositing a membrane includes a membrane-depositing process, in which electrolyte membranes (25, 26) having a proton conductivity are deposited by a gas phase depositing method on a hydrogen-separation membrane (21) with hydrogen permeability and the depositing process includes a changing process for changing a depositing condition during depositing the electrolyte membranes (25, 26). The depositing device (100) is provided with a depositing means (24) for depositing the electrolyte membranes (25, 26) with the proton conductivity, on the hydrogen separation membrane with hydrogen permeability by the gas phase depositing method and a changing means (23) for changing the depositing conditions during depositing of the electrolyte membrane.
COPYRIGHT: (C)2009,JPO&INPIT
摘要翻译：解决的问题：提供一种沉积电解质膜的方法和装置，其中可以控制电解质膜中的穿透缺陷的发生。解决方案：沉积膜的方法包括膜沉积工艺，其中具有质子传导性的电解质膜（25,26）通过气相沉积方法沉积在氢分离膜（21）上，氢气渗透性和沉积过程包括在沉积电解质膜（25,26）期间改变沉积条件的变化过程。沉积装置（100）具有沉积装置（24），用于通过气相沉积方法在具有氢渗透性的氢分离膜上沉积具有质子传导性的电解质膜（25,26）和改变装置（23）），用于在沉积电解质膜期间改变沉积条件。版权所有（C）2009，JPO＆INPIT

10. 发明专利

JP2007106642A Hydrogen generator and fuel cell system 审中-公开
标题翻译：氢发生器和燃料电池系统
公开(公告)号：JP2007106642A
公开(公告)日：2007-04-26
申请号：JP2005300728
申请日：2005-10-14
申请人： Toyota Motor Corp , トヨタ自動車株式会社
发明人： IIJIMA MASAHIKO , ITO NAOKI
IPC分类号： C01B3/38 , H01M8/04 , H01M8/06
CPC分类号： Y02E60/50
摘要： PROBLEM TO BE SOLVED: To provide a hydrogen generator which can suppress degradation of catalyst by a thermal shock; and also to provide a fuel cell system using the same. SOLUTION: A PSR type reforming device 100 and a PSR reforming device 200 are disposed in positions that make a catalyst supporting part 130 and a catalyst supporting part 230 situate close to each other and that enable thermal exchange between these parts. COPYRIGHT: (C)2007,JPO&INPIT

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