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1. 发明授权

US4810599A Structure suitable for solid electrochemical elements 失效
标题翻译：结构适用于固体电化学元素
公开(公告)号：US4810599A
公开(公告)日：1989-03-07
申请号：US172166
申请日：1988-03-23
申请人： Shigeo Kondo , Naoshi Yasuda , Masaki Nagata , Tadashi Sotomura
发明人： Shigeo Kondo , Naoshi Yasuda , Masaki Nagata , Tadashi Sotomura
IPC分类号： G02F1/15 , H01G9/02 , H01G11/56 , H01M4/62 , H01M6/18
CPC分类号： H01G9/038 , G02F1/1525 , H01G11/56 , H01M4/621 , H01M6/18 , H01M6/181 , Y02E60/13
摘要： A structure comprising a pair of electrode sheets and an electrolyte sheet, the latter being sandwiched in between the former, wherein each of the pair of electrode sheets comprises a mixture comprising an insulating elastomer and an electrode active substance powder and/or an inorganic solid electrolyte powder, in which mixture the electrode active substance powder and/or the inorganic solid electrolyte powder are dispersed in a volume fraction of 75-95% in the insulating elastomer, and said electrolyte sheet comprises a mixture of an inorganic solid electrolyte powder and an insulating elastomer and optionally an electrode active substance powder, in which mixture the inorganic solid electrolyte powder and optionally the electrode active substance powder are dispersed in a volume fraction of 55-95% in the insulating elastomer. Each of said electrode sheet and said electrolyte sheet may further comprise a reticulate material sheet, the openions of which are filled with the mixture. The structure is excellent in ion-conductivity, processability, productivity, storage stability and flexibility and enables one to make solid electrolyte cells, solid electric double layer capacitors and solid electrochromic display thinner and larger in area.
摘要翻译：一种结构，包括一对电极片和电解质片，后者被夹在前者之间，其中每对电极片包括包含绝缘弹性体和电极活性物质粉末和/或无机固体电解质的混合物粉末，其中电极活性物质粉末和/或无机固体电解质粉末在绝缘弹性体中以75-95％的体积分数分散，并且所述电解质片材包含无机固体电解质粉末和绝缘体的混合物弹性体和任选的电极活性物质粉末，其中无机固体电解质粉末和任选的电极活性物质粉末在绝缘弹性体中以55-95％的体积分数分散。所述电极片和所述电解质片中的每一个可以进一步包括网状材料片，其开口填充有混合物。该结构具有优异的离子传导性，加工性，生产率，储存稳定性和柔韧性，使得固体电解质电池，固体双电层电容器和固体电致变色显示器的面积更薄更大。

2. 发明授权

US4977007A Solid electrochemical element and production process therefor 失效
标题翻译：固体电化学元件及其生产工艺
公开(公告)号：US4977007A
公开(公告)日：1990-12-11
申请号：US097367
申请日：1987-09-08
申请人： Shigeo Kondo , Tadashi Sotomura
发明人： Shigeo Kondo , Tadashi Sotomura
IPC分类号： H01M12/00 , G02F1/15 , H01G9/00 , H01G9/155 , H01M4/02 , H01M6/18
CPC分类号： H01G9/155 , G02F1/1525 , H01M4/02 , H01M6/18 , H01M6/188 , Y02E60/13 , Y10T428/239 , Y10T428/24917 , Y10T428/25 , Y10T428/2933 , Y10T428/30 , Y10T428/31786 , Y10T428/31913 , Y10T428/31935
摘要： A solid electrochemical element which is flexible and has improved resistance to environmental exposure includes at least one solid electrolyte sheet which is flexible, has a pair of opposing surfaces, and is comprised of solid electrolyte particles and a plastic resin, which plastic resin was coated on each particle of the solid electrolyte particles prior to formation of the at least one solid electrolyte; and at least two electrode sheets comprised of an electrode material, one of the at least two electrode sheets being provided on each of the pair of opposing surfaces of the at least one solid electrolyte sheet, wherein an ion conductive path is formed between the pair of opposing surfaces of the at least one solid electrolyte sheet by virtual contact of the solid electrolyte particles and the electrode material. A process for producing the solid electrochemical element uses, as starting materials, (a) solid electrolyte particles coated with a thin layer of a plastic resin and (b) electrode material particles coated with a thin layer of a plastic resin, and preferably includes a step of crushing the solid electrolyte particles by pressing.
摘要翻译：柔性并且具有改善的耐环境暴露性的固体电化学元件包括至少一种柔性的固体电解质片，具有一对相对表面，并且由固体电解质颗粒和塑料树脂构成，该塑料树脂被涂覆在所述固体电解质颗粒的每个颗粒在形成所述至少一种固体电解质之前; 以及至少两个由电极材料组成的电极片，所述至少两个电极片中的至少一个电极片中的一个设置在所述至少一个固体电解质片的所述一对相对表面中的每一个上，其中在所述一对电极片之间形成离子传导路径通过固体电解质颗粒和电极材料的虚拟接触，至少一个固体电解质片的相对表面。固体电化学元件的制造方法使用（a）涂覆有塑料树脂薄层的固体电解质颗粒和（b）涂覆有塑料树脂薄层的电极材料颗粒，优选包括通过压制粉碎固体电解质颗粒的步骤。

3. 发明授权

US4828945A Solid electrolyte sheet and process for producing the same 失效
标题翻译：固体电解质片及其制造方法
公开(公告)号：US4828945A
公开(公告)日：1989-05-09
申请号：US172165
申请日：1988-03-23
申请人： Masaki Nagata , Naoshi Yasuda , Shigeo Kondo , Tadashi Sotomura
发明人： Masaki Nagata , Naoshi Yasuda , Shigeo Kondo , Tadashi Sotomura
IPC分类号： C08K3/16 , H01G9/02 , H01G11/56 , H01M6/18 , H01M6/22
CPC分类号： H01G9/038 , C08K3/16 , H01G11/56 , H01M6/18 , H01M6/181 , H01M6/22 , Y02E60/13
摘要： A solid electrolyte sheet comprising an ion-conductive inorganic solid electrolyte and an insulating elastomer, wherein the inorganic solid electrolyte powder is uniformly dispersed in the insulating elastomer in a volume fraction of 55-95% and which sheet has a hardness (ASTM A) of 65-96 and a thickness of 10-250 .mu.m, or a solid electrolyte sheet comprising a non-conductive reticulate material and a mixture of an ion-conductive inorganic solid electrolyte powder and an insulating elastomer, in which mixture the solid electrolyte powder is uniformly dispersed in the insulating elastomer in a volume fraction of 55-95%, at least the openings of the reticulate material being filled with said mixture. Said solid electrolyte sheets are superior in ion-conductivity, processability, productivity, storage stability and flexibility and are suitable for use in thin and large electrochemical elements.
摘要翻译：一种固体电解质片，包括离子传导性无机固体电解质和绝缘弹性体，其中所述无机固体电解质粉末以55-95％的体积分数均匀地分散在所述绝缘弹性体中，并且所述片的硬度（ASTM A）为 65-96和10-250μm的厚度，或包含非导电网状材料和离子传导无机固体电解质粉末和绝缘弹性体的混合物的固体电解质片，其中固体电解质粉末是均匀地分散在绝缘弹性体中，体积分数为55-95％，网状材料的至少开口填充有所述混合物。所述固体电解质片材的离子传导性，加工性，生产率，储存稳定性和柔软性都优异，适用于薄型和大型电化学元件。

4. 发明授权

US4789610A Solid-electrolyte secondary cell 失效
标题翻译：固体电解质二次电池
公开(公告)号：US4789610A
公开(公告)日：1988-12-06
申请号：US95146
申请日：1987-09-11
申请人： Shigeo Kondo , Tadashi Sotomura , Teruhisa Kanbara , Satoshi Sekido
发明人： Shigeo Kondo , Tadashi Sotomura , Teruhisa Kanbara , Satoshi Sekido
IPC分类号： H01M4/136 , H01M4/58 , H01M10/054 , H01M10/0562 , H01M6/18
CPC分类号： H01M10/0562 , H01M4/581
摘要： A solid-electrolyte secondary cell comprising a positive and a negative electrode composed of a copper chevrel compound (Cu.sub.x Mo.sub.6 S.sub.8), and copper ion conductive solid electrolyte is provided. This secondary cell is capable of charging with a current as high as about 1 mA/cm.sup.2, can stand high temperatures of up to 100.degree. C. and maintains its initial performance even after long-time charging and discharging. A cell small in voltage drop during dicharge is also provided by using a heat treated mixture of a copper chevrel compound and a copper ion conductive solid electrolyte represented by the formula K.sub.q Rb.sub.1-q Cu.sub.4 I.sub.2-p Cl.sub.3+3 (0.ltoreq.q.ltoreq.0.5, 0.25.ltoreq.p.ltoreq.1.0) for both positive and negative electrodes.
摘要翻译：提供了由铜螯合物（CuxMo6S8）和铜离子导电性固体电解质构成的正极和负极的固体电解质二次电池。该二次电池能够以高达约1mA / cm 2的电流充电，可以承受高达100℃的高温，并且即使在长时间充电和放电之后也保持其初始性能。通过使用铜螯合物和由KqRb1-qCu4I2-pCl3 + 3（0≤q≤0.5）表示的铜离子导电固体电解质的热处理混合物，也提供了在二次加注期间电压降小的电池，0.25

5. 发明授权

US07115338B2 Battery and method for generating electricity 有权
标题翻译：电池和发电方法
公开(公告)号：US07115338B2
公开(公告)日：2006-10-03
申请号：US11135283
申请日：2005-05-24
申请人： Tadashi Sotomura
发明人： Tadashi Sotomura
IPC分类号： H01M6/30 , H01M4/60
CPC分类号： H01M6/30 , H01M2/38 , H01M4/38 , H01M4/42 , H01M4/48 , H01M4/50 , H01M4/583 , H01M4/60 , H01M4/661 , H01M8/04082 , H01M8/04276 , H01M12/04 , H01M2004/027 , H01M2004/028 , Y02P70/56
摘要： A positive electrode, a negative electrode, and an electrolyte intervening between the positive electrode and the negative electrode are employed, and a molecule capable of being excited due to absorption of light and electrochemically oxidizing carbohydrate is provided at at least either the negative electrode or the electrolyte, with production of electromotive force occurring between the positive electrode and the negative electrode as a result of supply of carbohydrate while the molecule is irradiated with light and oxidization of carbohydrate by the molecule at the negative electrode. This method makes it possible for the chemical energy which carbohydrates possess to be directly utilized as electrical energy.
摘要翻译：采用在正极和负极之间插入的正极，负极和电解质，能够在负极或负极的至少一方具有由于吸收光而被激发而进行电化学氧化的碳分子电解质，由于供给碳水化合物而在正极和负极之间产生电动势，而分子被光照射并且在负极处被分子氧化碳水化合物。这种方法使碳水化合物所具有的化学能直接用作电能。

6. 发明授权

US06596431B1 Battery and method for generating an electric power 有权
标题翻译：用于产生电力的电池和方法
公开(公告)号：US06596431B1
公开(公告)日：2003-07-22
申请号：US09759317
申请日：2001-01-16
申请人： Tadashi Sotomura , Isao Taniguchi
发明人： Tadashi Sotomura , Isao Taniguchi
IPC分类号： H01M460
CPC分类号： H01M6/04 , H01M6/16 , H01M6/181 , H01M8/08 , H01M8/1009 , H01M12/04
摘要： For utilizing the chemical energy of a sugar directly as electric energy, electrolytic oxidation of a sugar on the negative electrode associated with cleavage of a carbon-carbon bond thereof is employed, thereby generating an electromotive force between the positive electrode and the negative electrode having an electrolyte therebetween. For an efficient oxidation of a sugar, it is effective for the negative electrode to have a component capable of forming a coordination compound with a sugar via a hydroxyl group thereof. Such a component may comprise a metal element capable of forming an amphoteric hydroxide. Use of an oxygen electrode as the positive electrode gives a battery capable of efficiently converting the chemical energy of a sugar into electric energy.
摘要翻译：为了将糖的化学能直接用作电能，使用与其碳 - 碳键相切的负极上的糖的电解氧化，从而在具有碳 - 碳键的正极和负极之间产生电动势，具有电解液。为了有效地氧化糖，对于负极具有能够通过其羟基与糖形成配位化合物的成分是有效的。这种组分可以包含能够形成两性氢氧化物的金属元素。使用氧电极作为正极，能够提供能够将糖的化学能有效地转化为电能的电池。

7. 发明授权

US06245458B1 Composite electrode, method of producing the same, and lithium secondary battery using the same 有权
标题翻译：复合电极及其制造方法以及使用该电极的锂二次电池
公开(公告)号：US06245458B1
公开(公告)日：2001-06-12
申请号：US09211779
申请日：1998-12-15
申请人： Tadashi Sotomura
发明人： Tadashi Sotomura
IPC分类号： H01M460
CPC分类号： H01M4/604 , H01M4/02 , H01M4/364 , H01M4/38 , H01M4/60 , H01M4/608 , H01M10/052
摘要： To provide a composite electrode, which does not lose large capacity and high energy density of sulfur and proceeds oxidation-reduction reaction rapidly even at room temperature. There is disclosed in the specification that a composite electrode comprising a composition containing an organic sulfide compound having at least a thiol or thiolate group in the molecule, polyaniline, and sulfur.
摘要翻译：为了提供即使在室温下也不会失去大容量和高能量密度的硫并迅速进行氧化还原反应的复合电极。在说明书中公开了一种复合电极，其包含含有分子中至少具有硫醇或硫醇基的有机硫化物的组合物，聚苯胺和硫。

8. 发明授权

US5869206A Electrode including organic disulfide compound and method of producing the same 失效
标题翻译：含有有机二硫化物的电极及其制造方法
公开(公告)号：US5869206A
公开(公告)日：1999-02-09
申请号：US820210
申请日：1997-03-18
申请人： Tadashi Sotomura
发明人： Tadashi Sotomura
IPC分类号： G01N27/333 , G02F1/155 , H01M4/13 , H01M4/137 , H01M4/139 , H01M4/1399 , H01M4/36 , H01M4/60
CPC分类号： H01M4/137 , H01M4/02 , G02F2001/1555 , H01M4/60
摘要： An electrode of the present invention comprises a complex of at least one organic disulfide compound and at least one copper ion. The electrode maintains a high charging and discharging efficiency and has favorable charge and discharge cycle characteristic without losing a high energy density that is characteristic of the organic disulfide compound.
摘要翻译：本发明的电极包含至少一种有机二硫化物和至少一种铜离子的络合物。该电极保持高的充放电效率并且具有良好的充放电循环特性，而不会失去有机二硫化物化合物特征的高能量密度。

9. 发明授权

US5190695A Methods to produce solid electrolyte and solid electrode composites 失效
标题翻译：生产固体电解质和固体电极复合材料的方法
公开(公告)号：US5190695A
公开(公告)日：1993-03-02
申请号：US706234
申请日：1991-05-28
申请人： Tadashi Sotomura
发明人： Tadashi Sotomura
IPC分类号： H01B1/20 , H01G9/02 , H01G9/025 , H01M4/62 , H01M6/18 , H01M10/36
CPC分类号： H01G9/025 , H01B1/20 , H01M10/0562 , H01M6/188 , H01M4/621 , H01M6/181 , H01M6/182 , H01M6/185 , Y02E60/13
摘要： This invention relates to methods to produce solid electroyte composites and solid electrode composites employed extensively to fabricate various solid electrochemical devices such as batteries, capacitors, sensors, display devices, recording devices, etc., and also to offer methods to produce solid electrolyte composites of high mechanical strength and large area electrode composites wherein fine powders of said solid electrolyte are uniformly dispersed.The methods to produce said solid electrolyte composites and solid electrode composites of the invention include a process to produce slurry by dispersing said solid electrolyte powders in a solvent in which plastic resin in dissolved, a process to remove said solvent from said slurry, and a process to add to the solvent one of the compounds selected from (a) to (e): (a) is a catonic surfactant having ethylene-oxide chains and/or propylene-oxide chains; (b) is a cationic surfactant having ethylene-oxide chains and butyleneoxide chains; (c) is a polyether compound produced by adding ethylene-oxide and/or propylene-oxide to a polyamine compound; (d) is a polyether compound produced by adding both ethylene-oxide and butylene-oxide chains to a polyamine compound; and (e) is an amide compound which is a dehydro-condensation product of polyalkyleneimine and fatty acid.
摘要翻译：本发明涉及广泛用于制造诸如电池，电容器，传感器，显示装置，记录装置等各种固体电化学装置的固体电解质复合材料和固体电极复合材料的制备方法，并提供生产固体电解质复合材料的方法，高机械强度和大面积电极复合材料，其中所述固体电解质的细粉末均匀分散。制备本发明的固体电解质复合材料和固体电极复合材料的方法包括通过将所述固体电解质粉末分散在其中溶解有塑料树脂的溶剂中，将所述溶剂从所述浆料中除去的方法，以及工艺为了向溶剂中添加选自（a）至（e）的化合物之一：（a）是具有环氧乙烷链和/或环氧丙烷链的结合表面活性剂; （b）是具有环氧乙烷链和环氧丁烷链的阳离子表面活性剂; （c）是通过向多胺化合物中加入环氧乙烷和/或环氧丙烷而制备的聚醚化合物; （d）是通过向多胺化合物中加入环氧乙烷和环氧丁烷链而制备的聚醚化合物; 和（e）是聚亚烷基亚胺和脂肪酸的脱氢缩合产物的酰胺化合物。

10. 发明申请

US20070243449A1 Electrode for use in oxygen reduction 有权
标题翻译：用于氧还原的电极
公开(公告)号：US20070243449A1
公开(公告)日：2007-10-18
申请号：US11808811
申请日：2007-06-13
申请人： Tadashi Sotomura , Mitsuru Hashimoto , Yuka Yamada
发明人： Tadashi Sotomura , Mitsuru Hashimoto , Yuka Yamada
IPC分类号： H01M4/90
CPC分类号： C07D487/22 , H01M4/90 , H01M4/92 , H01M8/16 , H01M12/06 , H01M2004/8689 , Y02E60/527
摘要： The present invention is usable in oxygen electrodes and air electrodes for air cells, fuel cells, electrochemical sensors and like electrochemical devices. The present invention provides a very stable oxygen-reducing electrode that can achieve electrochemical reduction of oxygen at a noble potential. The oxygen-reducing electrode of the present invention contains a cobalt tetrapyrazinoporphyrazine derivative represented by the following Structural Formula (1) as a catalytic component.
摘要翻译：本发明可用于空气电池，燃料电池，电化学传感器和类似电化学装置的氧电极和空气电极。本发明提供了一种非常稳定的氧还原电极，其能够实现在高电位下氧化的电化学还原。本发明的氧还原电极含有作为催化成分的由以下结构式（1）表示的钴四吡唑并吡喃衍生物。

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