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1. 发明授权

US08763364B2 Treatment of cold start engine exhaust 有权
标题翻译：冷启动发动机排气处理
公开(公告)号：US08763364B2
公开(公告)日：2014-07-01
申请号：US13088885
申请日：2011-04-18
申请人： Shanmugam Palani Elangovan , Tatsuya Okubo , Stacey I. Zones , Cong-Yan Chen , Allen W. Burton, Jr.
发明人： Shanmugam Palani Elangovan , Tatsuya Okubo , Stacey I. Zones , Cong-Yan Chen , Allen W. Burton, Jr.
IPC分类号： F01N3/00 , B01D53/02 , B01D53/94 , F01N3/10 , F01N9/00
CPC分类号： F01N3/101 , B01D53/02 , B01D53/9486 , B01D2253/108 , B01D2253/1122 , F01N3/106 , F01N9/00 , F01N2370/02 , Y02A50/2324 , Y02T10/22 , Y02T10/47
摘要： A method of treating a cold-start engine exhaust gas stream comprising hydrocarbons and other pollutants, the method comprising: flowing the exhaust gas stream over a molecular sieve bed, the molecular sieve bed comprising an alkali metal cation-exchanged molecular sieve having intersecting 10- and 12-membered ring pore channels, to provide a first exhaust stream; flowing the first exhaust gas stream over a catalyst to convert any residual hydrocarbons and other pollutants contained in the first exhaust gas stream to innocuous products to provide a treated exhaust stream; and discharging the treated exhaust stream into the atmosphere.
摘要翻译：一种处理包含碳氢化合物和其他污染物的冷启动发动机排气流的方法，所述方法包括：使排气流在分子筛床上流动，所述分子筛床包含碱金属阳离子交换的分子筛，和12元环孔通道，以提供第一排气流; 使第一废气流流过催化剂以将包含在第一废气流中的任何残留烃和其它污染物转化为无害产物以提供经处理的废气流; 并将经处理的废气流排放到大气中。

2. 发明申请

US20120260628A1 TREATMENT OF COLD START ENGINE EXHAUST 有权
标题翻译：冷起动发动机排气的处理
公开(公告)号：US20120260628A1
公开(公告)日：2012-10-18
申请号：US13088885
申请日：2011-04-18
申请人： Shanmugam Palani Elangovan , Tatsuya Okubo , Stacey I. Zones , Cong-Yan Chen , Allen W. Burton
发明人： Shanmugam Palani Elangovan , Tatsuya Okubo , Stacey I. Zones , Cong-Yan Chen , Allen W. Burton
IPC分类号： F01N3/10
CPC分类号： F01N3/101 , B01D53/02 , B01D53/9486 , B01D2253/108 , B01D2253/1122 , F01N3/106 , F01N9/00 , F01N2370/02 , Y02A50/2324 , Y02T10/22 , Y02T10/47
摘要： A method of treating a cold-start engine exhaust gas stream comprising hydrocarbons and other pollutants, the method comprising: flowing the exhaust gas stream over a molecular sieve bed, the molecular sieve bed comprising an alkali metal cation-exchanged molecular sieve having intersecting 10- and 12-membered ring pore channels, to provide a first exhaust stream; flowing the first exhaust gas stream over a catalyst to convert any residual hydrocarbons and other pollutants contained in the first exhaust gas stream to innocuous products to provide a treated exhaust stream; and discharging the treated exhaust stream into the atmosphere.
摘要翻译：一种处理包含碳氢化合物和其他污染物的冷启动发动机排气流的方法，所述方法包括：使排气流在分子筛床上流动，所述分子筛床包含碱金属阳离子交换分子筛，和12元环孔通道，以提供第一排气流; 使第一废气流流过催化剂，以将包含在第一废气流中的任何残留烃和其它污染物转化为无害产物以提供经处理的废气流; 并将经处理的废气流排放到大气中。

3. 发明授权

US08282908B2 Zeolite beta and process for producing the same 有权
标题翻译：沸石β及其生产方法
公开(公告)号：US08282908B2
公开(公告)日：2012-10-09
申请号：US13387631
申请日：2010-07-21
申请人： Keiji Itabashi , Tatsuya Okubo , Yoshihiro Kamimura , Watcharop Chaikittisilp , Shanmugam Palani Elangovan
发明人： Keiji Itabashi , Tatsuya Okubo , Yoshihiro Kamimura , Watcharop Chaikittisilp , Shanmugam Palani Elangovan
IPC分类号： C01B39/46
CPC分类号： C01B39/46 , B01D53/945 , B01D2255/502 , B01D2255/912 , B01D2255/9205 , B01D2255/9207 , B01D2258/012 , B01D2258/014 , B01J29/7007 , B01J2229/36 , Y02T10/22
摘要： A zeolite beta according to the present invention has a SiO2/Al2O3 ratio of 10 to 16 and is aluminum-rich. The zeolite beta has a BET specific surface area measured in the state of a sodium type of 500 to 700 m2/g, a micropore specific surface area of 350 to 500 m2/g, and a micropore volume of 0.15 to 0.25 cm3/g.
摘要翻译：本发明的沸石β的SiO 2 / Al 2 O 3比为10〜16，富铝。沸石β具有在500〜700m 2 / g的钠型，微孔比表面积为350〜500m 2 / g，微孔体积为0.15〜0.25cm 3 / g的状态下测定的BET比表面积。

4. 发明申请

US20120190534A1 ZEOLITE BETA AND PROCESS FOR PRODUCING THE SAME 有权
标题翻译：沸石BETA及其生产方法
公开(公告)号：US20120190534A1
公开(公告)日：2012-07-26
申请号：US13387631
申请日：2010-07-21
申请人： Keiji Itabashi , Tatsuya Okubo , Yoshihiro Kamimura , Watcharop Chaikittisilp , Shanmugam Palani Elangovan
发明人： Keiji Itabashi , Tatsuya Okubo , Yoshihiro Kamimura , Watcharop Chaikittisilp , Shanmugam Palani Elangovan
IPC分类号： B01J29/70 , C01B39/02 , B82Y30/00 , B82Y40/00
CPC分类号： C01B39/46 , B01D53/945 , B01D2255/502 , B01D2255/912 , B01D2255/9205 , B01D2255/9207 , B01D2258/012 , B01D2258/014 , B01J29/7007 , B01J2229/36 , Y02T10/22
摘要： A zeolite beta according to the present invention has a SiO2/Al2O3 ratio of 10 to 16 and is aluminum-rich. The zeolite beta has a BET specific surface area measured in the state of a sodium type of 500 to 700 m2/g, a micropore specific surface area of 350 to 500 m2/g, and a micropore volume of 0.15 to 0.25 cm3/g.
摘要翻译：本发明的沸石β的SiO 2 / Al 2 O 3比为10〜16，富铝。沸石β具有在500至700m 2 / g的钠类型，微孔比表面积为350至500m 2 / g，微孔体积为0.15至0.25cm 3 / g的状态下测量的BET比表面积。

5. 发明授权

US09108187B2 Fe(II)-substituted beta type zeolite, gas adsorbent containing same and method for producing same, and method for removing nitrogen monoxide and hydrocarbon 有权
标题翻译： Fe（II）取代的β型沸石，含有它的气体吸附剂及其制备方法，以及除去一氧化氮和烃的方法
公开(公告)号：US09108187B2
公开(公告)日：2015-08-18
申请号：US13979670
申请日：2012-01-17
申请人： Masaru Ogura , Keiji Itabashi , Tatsuya Okubo , Shanmugam Palani Elangovan
发明人： Masaru Ogura , Keiji Itabashi , Tatsuya Okubo , Shanmugam Palani Elangovan
IPC分类号： C01B39/46 , F01N3/08 , B01J20/30 , B01J20/28 , C01B39/06 , B01D53/02
CPC分类号： B01J20/3085 , B01D53/02 , B01D2253/108 , B01D2253/1085 , B01D2253/306 , B01D2253/311 , B01D2257/404 , B01D2257/702 , B01D2258/01 , B01J20/28061 , B01J20/28071 , C01B39/065 , C01B39/46 , C01P2006/12 , C01P2006/14 , F01N3/0835 , F01N3/0842
摘要： To provide an Fe(II)-substituted beta type zeolite which has been ion-exchanged with Fe(II) ions and can effectively adsorb and remove nitrogen monoxide or hydrocarbon contained in gas to be cleaned, even if oxygen is present in the gas at a high concentration or the temperature of the gas is low. In the Fe(II)-substituted beta type zeolite, a ratio of SiO2/Al2O3 is preferably 10 to 18, a BET specific surface area is preferably 400 m2/g to 700 m2/g, a micropore specific surface area is preferably 290 m2/g to 500 m2/g, and a micropore volume is preferably 0.15 cm3/g to 0.25 cm3/g. The amount of Fe(II) supported is preferably 0.01% by mass to 6.5% by mass based on the Fe(II)-substituted beta type zeolite.
摘要翻译：为了提供与Fe（II）离子进行离子交换的Fe（II） - 取代的β型沸石，并且即使在气体中存在氧气也可以有效地吸附和去除待清洁的气体中所含的一氧化氮或烃。高浓度或气体的温度低。在Fe（II）取代的β型沸石中，SiO 2 / Al 2 O 3的比例优选为10〜18，BET比表面积优选为400m 2 / g〜700m 2 / g，微孔比表面积优选为290m 2 g〜500m 2 / g，微孔体积优选为0.15cm 3 / g〜0.25cm 3 / g。相对于Fe（II）取代的β型沸石，Fe（II）的量优选为0.01质量％〜6.5质量％。

6. 发明申请

US20140157987A1 Fe(II)-SUBSTITUTED BETA TYPE ZEOLITE, GAS ADSORBENT CONTAINING SAME AND METHOD FOR PRODUCING SAME, AND METHOD FOR REMOVING NITROGEN MONOXIDE AND HYDROCARBON 有权
标题翻译： Fe（II） - 沸石型沸石，含有它们的气体吸附剂及其生产方法，以及除去一氧化氮和氢氧化碳的方法
公开(公告)号：US20140157987A1
公开(公告)日：2014-06-12
申请号：US13979670
申请日：2012-01-17
申请人： Masaru Ogura , Keiji Itabashi , Tatsuya Okubo , Shanmugam Palani Elangovan
发明人： Masaru Ogura , Keiji Itabashi , Tatsuya Okubo , Shanmugam Palani Elangovan
IPC分类号： B01J20/30 , B01J20/28 , B01D53/02
CPC分类号： B01J20/3085 , B01D53/02 , B01D2253/108 , B01D2253/1085 , B01D2253/306 , B01D2253/311 , B01D2257/404 , B01D2257/702 , B01D2258/01 , B01J20/28061 , B01J20/28071 , C01B39/065 , C01B39/46 , C01P2006/12 , C01P2006/14 , F01N3/0835 , F01N3/0842
摘要： To provide an Fe(II)-substituted beta type zeolite which has been ion-exchanged with Fe(II) ions and can effectively adsorb and remove nitrogen monoxide or hydrocarbon contained in gas to be cleaned, even if oxygen is present in the gas at a high concentration or the temperature of the gas is low. In the Fe(II)-substituted beta type zeolite, a ratio of SiO2/Al2O3 is preferably 10 to 18, a BET specific surface area is preferably 400 m2/g to 700 m2/g, a micropore specific surface area is preferably 290 m2/g to 500 m2/g, and a micropore volume is preferably 0.15 cm3/g to 0.25 cm3/g. The amount of Fe(II) supported is preferably 0.01% by mass to 6.5% by mass based on the Fe(II)-substituted beta type zeolite.
摘要翻译：为了提供与Fe（II）离子进行离子交换的Fe（II） - 取代的β型沸石，并且即使在气体中存在氧气也可以有效地吸附和去除待清洁的气体中所含的一氧化氮或烃。高浓度或气体的温度低。在Fe（II）取代的β型沸石中，SiO 2 / Al 2 O 3的比例优选为10〜18，BET比表面积优选为400m 2 / g〜700m 2 / g，微孔比表面积优选为290m 2 g〜500m 2 / g，微孔体积优选为0.15cm 3 / g〜0.25cm 3 / g。相对于Fe（II）取代的β型沸石，Fe（II）的量优选为0.01质量％〜6.5质量％。

7. 发明授权

US08212028B2 Method for producing ε-caprolactam and method for producing pentasil type zeolite 失效
标题翻译：生产ε-己内酰胺的方法和生产pentasil型沸石的方法
公开(公告)号：US08212028B2
公开(公告)日：2012-07-03
申请号：US12543022
申请日：2009-08-18
申请人： Tatsuya Okubo , Yuki Suzuki , Tsuyoshi Matsushita , Tatsuya Suzuki
发明人： Tatsuya Okubo , Yuki Suzuki , Tsuyoshi Matsushita , Tatsuya Suzuki
IPC分类号： C07D201/04
CPC分类号： C07D201/04 , C01B37/02 , C01B39/36 , C01B39/40 , Y02P20/52
摘要： The present invention provides a method which can produce ε-caprolactam with a good selectivity by reacting cyclohexanone oxime with a good conversion in a vapor phase Beckmann rearrangement reaction. Disclosed is a method for producing ε-caprolactam, which comprises performing a vapor phase Beckmann rearrangement reaction of cyclohexanone oxime in the presence of a pentasil type zeolite, wherein the pentasil type zeolite is a zeolite obtained by subjecting a mixture containing a silicon compound, water, and a compound represented by formula (I): [(R1)3N+—(CH2)m—N+(R1)2—(CH2)m—N+(R1)3]·3/n(A) (I) wherein R1 represents an alkyl group having 1 to 4 carbon atoms, A represents an n-valent anion, m represents an integer of 5 to 7, and n represents an integer of 1 to 3, to a hydrothermal synthesis reaction.
摘要翻译：本发明提供了一种通过在气相贝克曼重排反应中使环己酮肟与良好的转化率反应，能够以良好的选择性生产“己内酰胺”的方法。公开了一种生产ε-己内酰胺的方法，其包括在pentasil型沸石存在下进行环己酮肟的气相Beckmann重排反应，其中pentasil型沸石是通过使含有硅化合物的混合物，水和由式（I）表示的化合物：[（R1）3N + - （CH2）m-N +（R1）2-（CH2）m-N +（R1）3]·3 / n（A）其中，R1表示碳原子数1〜4的烷基，A表示n价阴离子，m表示5〜7的整数，n表示1〜3的整数。

8. 发明申请

US20060083674A1 Method for forming catalyst metal particles for production of single-walled carbon nanotube 审中-公开
标题翻译：用于形成用于制备单壁碳纳米管的催化剂金属颗粒的方法
公开(公告)号：US20060083674A1
公开(公告)日：2006-04-20
申请号：US10545298
申请日：2004-02-16
申请人： Shigeo Maruyama , Yoichi Murakami , Tatsuya Okubo , Shigehrio Yamakita
发明人： Shigeo Maruyama , Yoichi Murakami , Tatsuya Okubo , Shigehrio Yamakita
IPC分类号： D01F9/12 , B01J23/00 , B05D3/04 , B05D3/02
CPC分类号： B82Y30/00 , B01J23/88 , B01J37/0203 , B01J37/12 , B82Y40/00 , C01B32/162 , C01B2202/02
摘要： Provided is a process for forming catalyst metal fine particles for synthesizing a single-walled carbon nanotube by a CCVD process on a substrate, wherein a solution is prepared by dispersing or dissolving a catalyst metal salt of an organic compound or an inorganic compound in a solvent; the solution is coated on the substrate and dried; then, the substrate is heated in an oxidative atmosphere to thereby remove the solvent component remaining on the substrate by oxidative decomposition, and fine particles of an oxide of the catalyst metal are formed on the substrate; and then, the oxide of the catalyst metal is reduced in an atmosphere of an inert gas or a gas having reducing action to fix the catalyst metal fine particles on the substrate.
摘要翻译：本发明提供一种通过CCVD法在基材上形成用于合成单层碳纳米管的催化剂金属微粒的方法，其中通过将有机化合物或无机化合物的催化剂金属盐分散或溶解在溶剂中制备溶液 ; 将溶液涂布在基材上并干燥; 然后在氧化气氛中加热基板，通过氧化分解除去留在基板上的溶剂成分，在基板上形成催化剂金属的氧化物微粒; 然后在惰性气体气氛中还原催化剂金属的氧化物或具有还原作用的气体，以将催化剂金属微粒固定在基材上。

9. 发明授权

US06801640B1 Gate control device 失效
标题翻译：门控装置
公开(公告)号：US06801640B1
公开(公告)日：2004-10-05
申请号：US09586978
申请日：2000-06-05
申请人： Tatsuya Okubo , Shigeo Atarashi
发明人： Tatsuya Okubo , Shigeo Atarashi
IPC分类号： G06K900
CPC分类号： G07C9/025 , G06K9/00221 , G07C9/00 , G07C9/00158
摘要： The present invention discloses a gate control device which controls the passage (e.g., entry, exit, etc.) through a passageway of both authorized persons and unauthorized companions of authorized persons into a protected room. The device may be configured such that the unauthorized companions may be permitted or denied passage if the unauthorized companions are with an authorized person. For example, the device may be configured to allow an entire group of persons to enter a room if only one authorized person is present. In another example, the device may deny passage to the entire group if it contains even one unauthorized person.
摘要翻译：本发明公开了一种门控制装置，其通过授权人员的通道和授权人员的未经授权的同伴进入受保护的房间来控制通道（例如进入，离开等）。该设备可以被配置为使得如果未授权的同伴与授权的人在一起，则允许或拒绝未经授权的同伴通过。例如，如果只有一个授权人存在，则该设备可以被配置为允许整个人员组进入房间。在另一个示例中，如果设备甚至包含一个未授权的人，则设备可以拒绝通过整个组。

10. 发明授权

US09333495B2 Method for producing MTW-type zeolite 有权
标题翻译：生产MTW型沸石的方法
公开(公告)号：US09333495B2
公开(公告)日：2016-05-10
申请号：US13509677
申请日：2010-11-19
申请人： Keiji Itabashi , Tatsuya Okubo , Kenta Iyoki
发明人： Keiji Itabashi , Tatsuya Okubo , Kenta Iyoki
IPC分类号： C01B39/42 , B01J29/70 , B01J20/30
CPC分类号： C01B39/42 , B01J20/3078 , B01J29/7034
摘要： A method for producing an MTW-type zeolite, comprising (1) mixing an alumina source, an alkali source, a lithium source, and water so as to obtain a reaction mixture (2) Adding a seed crystal of an MTW-type zeolite before or while a silica source is added to the reaction mixture in a proportion of 0.1 to 20% by weight relative to the silica component in the reaction mixture. Mixing and stirring the reaction mixture. Wherein the MTW-type zeolite of the seed crystal has a SiO2/Al2O3 ratio of 10 to 500 and does not contain an organic compound. The reaction mixture has a composition represented by the following molar ratios: SiO2/Al2O3=12 to 200, Na2O/SiO2=0.1 to 0.3, Li2O/(Na2O+Li2O)=0.05 to 0.5 and H2O/SiO2=10 to 50. (3) Air tightly heating the reaction mixture, to which the seed crystal of the MTW type zeolite has been added, at 100 to 200° C.
摘要翻译：一种生产MTW型沸石的方法，包括（1）将氧化铝源，碱源，锂源和水混合以获得反应混合物（2）在MTW型沸石之前加入MTW型沸石的晶种或者相对于反应混合物中的二氧化硅组分，以0.1至20重量％的比例将二氧化硅源加入到反应混合物中。混合搅拌反应混合物。其中晶种的MTW型沸石的SiO 2 / Al 2 O 3比例为10〜500，不含有机化合物。反应混合物具有以下摩尔比表示的组成：SiO 2 / Al 2 O 3 = 12〜200，Na 2 O / SiO 2 = 0.1〜0.3，Li 2 O /（Na 2 O + Li 2 O）= 0.05〜0.5，H 2 O / SiO 2 = 10〜50 3）在100〜200℃下，将加入MTW型沸石的晶种的反应混合物气密加热

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