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1. 发明申请

WO2013087185A2 A CATALYST SYSTEM FOR THE PRODUCTION OF ULTRA-HIGH MOLECULAR WEIGHT POLYETHYLENE 审中-公开
标题翻译：用于生产超高分子量聚乙烯的催化剂体系
公开(公告)号：WO2013087185A2
公开(公告)日：2013-06-20
申请号：PCT/EP2012/005089
申请日：2012-12-10
申请人： SAUDI BASIC INDUSTRIES CORPORATION (SABIC) , BATINAS-GEURTS, Aurora Alexandra , FRIEDERICHS, Nicolaas Hendrika , SCHOFFELEN, Tom , ZUIDEMA, Erik
发明人： BATINAS-GEURTS, Aurora Alexandra , FRIEDERICHS, Nicolaas Hendrika , SCHOFFELEN, Tom , ZUIDEMA, Erik
IPC分类号： C08F4/651 , C08F4/649 , C08F4/656 , C08F110/02
CPC分类号： C08F110/02 , C08F4/651 , C08F4/6494 , C08F4/6567 , C08F2500/01 , C08F2500/18 , C08F2500/24
摘要： The invention relates to a catalyst system for the production of ultrahigh molecular weight polyethylene comprising I. a solid reaction product obtained by reaction of: (a) a hydrocarbon solution comprising (1) an organic oxygen containing magnesium compound or a halogen containing magnesium compound and (2) an organic oxygen containing titanium compound and (b) a mixture comprising a metal compound having the formula MeR n X 3-n wherein X is a halogenide, Me is a metal of Group III of Mendeleev's Periodic System of Chemical Elements, R is a hydrocarbon radical containing 1 - 10 carbon atoms and 0 ≤ n ≤ 3 and a silicon compound of formula R m SiCI 4.m wherein 0 ≤ m ≤ 2 and R is a hydrocarbon radical containing 1 - 10 carbon atoms wherein the molar ratio of metal from (b): titanium from (a) is lower than 1:1 II. an organo aluminium compound having the formula AIR 3 in which R is a hydrocarbon radical containing 1 - 10 carbon atoms and III. an external electron donor selected from the group of 1,2- dialkoxyalkanes, 1,2-dialkoxyalkenes or an external polymeric electron donor.
摘要翻译：本发明涉及一种用于生产超高分子量聚乙烯的催化剂体系，其包括I.通过以下反应获得的固体反应产物：（a）烃溶液，其包含（1）含有机氧的镁化合物或含卤素的镁化合物和（2）含有机氧的钛化合物和（b）包含具有式MeRnX3-n的金属化合物的混合物，其中X是卤化物，Me是Mendeleev的化学元素周期系统的III族金属，R是烃含有1-10个碳原子且0 <= n <3的基团和式RmSiCl 4 m的硅化合物，其中0≤m≤2且R是含有1-10个碳原子的烃基，其中金属的摩尔比来自（b）：（a）的钛低于1:1。具有式AIR3的有机铝化合物，其中R是含有1-10个碳原子的烃基和III。选自1,2-二烷氧基烷烃，1,2-二烷氧基羰基或外部聚合电子给体的外部电子给体。

2. 发明申请

WO2013087167A3 A PROCESS FOR THE PRODUCTION OF BIMODAL POLYETHYLENE IN THE PRESENCE OF THIS CATALYST SYSTEM 审中-公开
公开(公告)号：WO2013087167A3
公开(公告)日：2013-06-20
申请号：PCT/EP2012/005031
申请日：2012-12-06
申请人： SAUDI BASIC INDUSTRIES CORPORATION , BATINAS-GEURTS, Aurora Alexandra , FRIEDERICHS, Nicolaas Hendrika , SCHOFFELEN, Tom , ZUIDEMA, Erik , GARG, Priya
发明人： BATINAS-GEURTS, Aurora Alexandra , FRIEDERICHS, Nicolaas Hendrika , SCHOFFELEN, Tom , ZUIDEMA, Erik , GARG, Priya
IPC分类号： C08F210/16 , C08F2/00 , C08F4/651 , C08F4/649 , C08F4/655
摘要： The invention relates to a process for the production of bimodal polyethylene in a two-step polymerisation process in the presence of a catalyst system comprising: (I) the solid reaction product obtained by reacting of: a) a hydrocarbon solution containing 1) an organic oxygen containing magnesium compound or a halogen containing magnesium compound and 2) an organic oxygen containing titanium compound and b) an aluminium halogenide having the formula AIR n X 3-n in which R is a hydrocarbon radical containing 1 − 10 carbon atoms, X is halogen and 0 3 in which R is a hydrocarbon radical containing 1 − 10 carbon atom and (III) an electron donor selected from the group of 1,2-dialkoxyalkanes and 1,2- dialkoxyalkenes wherein in the first step a low molecular weight polyethylene is produced which has a MFI 190/1,2 is between 1 and 200 dg/min, and in the second step a high molecular weight ethylene copolymer is produced in which the MFI 190/5 of the total product is between 0.1 and 5 dg/min, and the weight fraction of the material produced in the first step is between 40 wt% and 60 wt% of the total product.

3. 发明授权

EP2791182B1 A CATALYST SYSTEM AND A PROCESS FOR THE PRODUCTION OF ULTRA HIGH MOLECULAR WEIGHT POLYETHYLENE IN PRESENCE OF THIS CATALYST SYSTEM 有权
标题翻译：该催化剂体系存在下催化剂体系和生产超高分子量聚乙烯的方法
公开(公告)号：EP2791182B1
公开(公告)日：2017-08-30
申请号：EP12798618.0
申请日：2012-12-10
申请人： SAUDI BASIC INDUSTRIES CORPORATION (SABIC)
发明人： BATINAS-GEURTS, Aurora Alexandra , FRIEDERICHS, Nicolaas Henrika , SCHOFFELEN, Tom , ZUIDEMA, Erik
IPC分类号： C08F4/649 , C08F4/656 , C08F110/02
CPC分类号： C08F110/02 , C08F4/651 , C08F4/6494 , C08F4/6567 , C08F2500/01 , C08F2500/18 , C08F2500/24

4. 发明公开

EP2791182A2 A CATALYST SYSTEM FOR THE PRODUCTION OF ULTRA-HIGH MOLECULAR WEIGHT POLYETHYLENE 有权
标题翻译： KATALYSATORSYSTEM ZUR HERSTELLUNG VON聚乙烯麻醉药超声乳化液
公开(公告)号：EP2791182A2
公开(公告)日：2014-10-22
申请号：EP12798618.0
申请日：2012-12-10
申请人： SAUDI BASIC INDUSTRIES CORPORATION (SABIC)
发明人： BATINAS-GEURTS, Aurora Alexandra , FRIEDERICHS, Nicolaas Henrika , SCHOFFELEN, Tom , ZUIDEMA, Erik
IPC分类号： C08F4/651 , C08F4/649 , C08F4/656 , C08F110/02
CPC分类号： C08F110/02 , C08F4/651 , C08F4/6494 , C08F4/6567 , C08F2500/01 , C08F2500/18 , C08F2500/24
摘要： The invention relates to a catalyst system for the production of ultrahigh molecular weight polyethylene comprising I. a solid reaction product obtained by reaction of: (a) a hydrocarbon solution comprising (1) an organic oxygen containing magnesium compound or a halogen containing magnesium compound and (2) an organic oxygen containing titanium compound and (b) a mixture comprising a metal compound having the formula MeR
n X
3-n wherein X is a halogenide, Me is a metal of Group III of Mendeleev's Periodic System of Chemical Elements, R is a hydrocarbon radical containing 1 - 10 carbon atoms and 0 ≤ n ≤ 3 and a silicon compound of formula R
m SiCI
4.m wherein 0 ≤ m ≤ 2 and R is a hydrocarbon radical containing 1 - 10 carbon atoms wherein the molar ratio of metal from (b): titanium from (a) is lower than 1:1 II. an organo aluminium compound having the formula AIR
3 in which R is a hydrocarbon radical containing 1 - 10 carbon atoms and III. an external electron donor selected from the group of 1,2- dialkoxyalkanes, 1,2-dialkoxyalkenes or an external polymeric electron donor.
摘要翻译：本发明涉及一种用于生产超高分子量聚乙烯的催化剂体系，其包含I.通过以下反应获得的固体反应产物：（a）烃溶液，其包含（1）含有机氧的镁化合物或含卤素的镁化合物和（2）含有机氧的钛化合物和（b）包含具有式MeRnX3-n的金属化合物的混合物，其中X是卤化物，Me是Mendeleev的化学元素周期系统的III族金属，R是烃含有1-10个碳原子和0≤n≤3的基团和式RmSiCl4m的硅化合物，其中0≤m≤2且R是含有1-10个碳原子的烃基，其中来自（b）的金属的摩尔比：（a）的钛低于1：1 II。具有式AIR3的有机铝化合物，其中R是含有1-10个碳原子的烃基和III。选自1,2-二烷氧基烷烃，1,2-二烷氧基羰基或外部聚合电子给体的外部电子给体。

5. 发明申请

WO2015091966A1 CATALYST SYSTEM FOR POLYMERIZATION OF AN OLEFIN 审中-公开
标题翻译：用于烯烃聚合的催化剂体系
公开(公告)号：WO2015091966A1
公开(公告)日：2015-06-25
申请号：PCT/EP2014/078773
申请日：2014-12-19
申请人： SAUDI BASIC INDUSTRIES CORPORATION , SABIC GLOBAL TECHNOLOGIES B.V. , ZUIDEVELD, Martin Alexander , ZUIDEMA, Erik
发明人： ZUIDEVELD, Martin Alexander , ZUIDEMA, Erik
IPC分类号： C08F210/16 , C08F4/656 , C08F4/646 , C08F4/649
CPC分类号： C08F10/06 , C08F110/02 , C08F110/06 , C08F210/16 , C08F2410/00 , C08F2500/15 , C08F2500/12 , C08F4/6565 , C08F4/6465 , C08F4/6495 , C08F210/06
摘要： The present invention relates to a catalyst system comprising a procatalyst, a co-catalyst and an external electron donor, wherein the external electron donor comprises a compound having the structure according to Formula I': Si (L) n (OR 11 ) 4-n-m (R 12 ) m wherein, Si is a silicon atom with valency 4+; O is an oxygen atom with valency 2- and O is bonded to Si via a silicon-oxygen bond; n is 1, 2, 3 or 4; m is 0, 1, 2 or 3 n+m≤4 each R 11 group is independently selected from the group consisting of linear, branched and cyclic alkyl having at most 20 carbon atoms and aromatic substituted and unsubstituted hydrocarbyl having 6 to 20 carbon atoms; each R 12 group is independently selected from the group consisting of linear, branched and cyclic alkyl having at most 20 carbon atoms and aromatic substituted and unsubstituted hydrocarbyl having 6 to 20 carbon atoms; each L group is independently a group represented by the following structure, Formula II, wherein, L is bonded to the silicon atom via the nitrogen-silicon bond; L has a single substituent on the nitrogen atom, where this single substituent is an imine carbon atom; and X and Y are independently selected from the group consisting of a hydrogen atom; a heteroatom selected from group 13, 14, 15, 16 or 17 of the lUPAC Periodic Table of the Elements; a linear, branched and cyclic alkyl having at most 20 carbon atoms, optionally containing a heteroatom selected from group 13, 14, 15, 16 or 17 of the lUPAC Periodic Table of the Elements and an aromatic substituted and unsubstituted hydrocarbyl having 6 to 20 carbon atoms, optionally containing a heteroatom selected from group 13, 14, 15, 16 or 17 of the lUPAC Periodic Table of the Elements.
摘要翻译：本发明涉及包含前催化剂，助催化剂和外电子给体的催化剂体系，其中外电子给体包括具有式I'结构的化合物：Si（L）n（OR 11）4-nm （R 12）m，其中Si是4价的硅原子; O是具有2-价的氧原子，O经由硅 - 氧键与Si键合; n为1,2,3或4; m为0,1,2或3 n +m≤4，每个R 11基团独立地选自具有至多20个碳原子的直链，支链和环状烷基和具有6至20个碳原子的芳族取代和未取代的烃基; 每个R 12基团独立地选自具有至多20个碳原子的直链，支链和环状烷基和具有6至20个碳原子的芳族取代和未取代的烃基; 每个L基团独立地是由以下结构表示的基团，式II，其中L经由氮 - 硅键与硅原子键合; L在氮原子上具有单个取代基，其中该单取代基是亚胺碳原子; X和Y独立地选自氢原子; 选自元素周期表的第14,14,15,16或17号的杂原子; 含有至多20个碳原子的直链，支链和环状烷基，任选地含有选自元素周期表的LUPAC元素周期表第13,14,15,16或17族的杂原子和具有6至20个碳原子的芳族取代和未取代的烃基原子，任选地含有选自元素周期表的LUPAC元素的第13,14,15,16或17族的杂原子。

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