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1. 发明申请

US20090134066A1 Method for producing alkyl-aromatic compounds by direct alkylation of aromatic hydrocarbons with alkanes 审中-公开
标题翻译：通过芳族烃与烷烃直接烷基化生产烷基芳族化合物的方法
公开(公告)号：US20090134066A1
公开(公告)日：2009-05-28
申请号：US11659422
申请日：2005-08-04
申请人： Nils Bottke , Michael Triller , Ulrich Muller , Rolf Pinkos , Thomas Heidemann
发明人： Nils Bottke , Michael Triller , Ulrich Muller , Rolf Pinkos , Thomas Heidemann
IPC分类号： C10G35/06 , C07C2/58
CPC分类号： C07C303/06 , C07C2/76 , C07C15/02 , C07C309/31
摘要： The present invention relates to a process for preparing alkylaromatics by reacting aromatic compounds with C1-C14-alkanes in the presence of a heterogeneous catalyst, which comprises using as the catalyst a crystalline, micro- and/or mesoporous solid comprising silicon and at least one father element selected from the group consisting of the transition metals and the main group elements gallium and tin, and activating said catalysts by a reducing pretreatment. Furthermore, the present invention relates to a process for preparing alkylarylsulfonates by sulfonating and neutralizing the alkyl aromatic compounds.
摘要翻译：本发明涉及在非均相催化剂存在下使芳族化合物与C 1 -C 14烷烃反应制备烷基芳族化合物的方法，该方法包括使用包含硅和至少一种以上的硅的结晶，微孔和/或介孔固体作为催化剂父元素选自过渡金属和主要元素镓和锡，并通过还原预处理活化所述催化剂。此外，本发明涉及通过磺化和中和烷基芳族化合物来制备烷基芳基磺酸盐的方法。

2. 发明申请

US20070142258A1 Method for producing alkylaryl compounds 审中-公开
标题翻译：烷基芳基化合物的制备方法
公开(公告)号：US20070142258A1
公开(公告)日：2007-06-21
申请号：US10583140
申请日：2004-12-17
申请人： Ulrich Steinbrenner , Thomas Heidemann , Michael Roper , Jurgen Stephan , Thomas Narbeshuber , Jurgen Tropsch , Nils Bottke , Regina Benfer
发明人： Ulrich Steinbrenner , Thomas Heidemann , Michael Roper , Jurgen Stephan , Thomas Narbeshuber , Jurgen Tropsch , Nils Bottke , Regina Benfer
IPC分类号： C09D9/00
CPC分类号： C07C6/04 , C07C2/08 , C07C2/66 , C07C5/2506 , C07C303/06 , C11D1/22 , C11D11/04 , C07C309/31 , C07C11/02 , C07C11/10 , C07C15/107
摘要： The preparation of alkylaryl compounds takes place by a) reaction of a C4/C5-olefin mixture over a metathesis catalyst to prepare a C4-8-olefin mixture comprising 2-pentene, and optional removal of the C4-8-olefin mixture, b) removal of from 5 to 100% of the 2-pentene present in stage a) and subsequent reaction over an isomerization catalyst to give a mixture of 2-pentene and 1-pentene which is returned to stage a), c) dimerization of the C4-8-olefin mixture obtained in stage b) following removal in the presence of a dimerization catalyst to give a mixture containing C8-16-olefins, removal of these C8-16-olefins and optional removal of a partial stream thereof, d) reaction of the c8-16-olefin mixtures obtained in stage c) or of the partial stream with an aromatic hydrocarbon in the presence of an alkylation catalyst to form alkyl aromatic compounds where, prior to the reaction, 0 to 60% by weight, based on the c8-16-olefin mixtures obtained in stage c), of linear olefins may additionally be added, e) optional sulfonation of the alkyl aromatic compounds obtained in stage d) and neutralization to give alkylarylsulfonates, where, prior to the sulfonation, 0 to 60% by weight, based on the alkyl aromatic compounds obtained in stage d), of linear alkylbenzenes may additionally be added if no admixing has taken place in stage d), f) optional mixing of the alkylarylsulfonates obtained in stage e) with 0 to 60% by weight, based on the alkylarylsulfonates obtained in stage e), of linear alkylarylsulfonate, if no admixing has taken place in stages d) and e).
摘要翻译：烷基芳基化合物的制备通过以下步骤进行：a）在复分解催化剂上使C 4-14 C 5 -C 5 - 烯烃混合物反应以制备C 4-8 - 其包含2-戊烯，任选地除去C 4-18α-烯烃混合物，b）除去在步骤a）中存在的5-100％的2-戊烯，并随后在异构化催化剂上反应，得到2-戊烯和1-戊烯的混合物，将其返回到a）步骤，c）在步骤b中获得的C 4-18α-烯烃混合物的二聚反应），在二聚催化剂存在下除去，得到含有C 8-16 - 烯烃的混合物，除去这些C 8-16 - 烯烃并任选地除去其部分流，d）在烷基化催化剂存在下，将阶段c）或部分流中获得的C 8-16 - α-烯烃混合物与芳族烃反应，形成烷基芳族化合物，其中在反应之前，0至60重量％，b 在阶段c）中得到的C 8-16α-烯烃混合物中，可以另外加入线性烯烃，e）任选的在步骤d）中获得的烷基芳族化合物磺化，中和得到烷基芳基磺酸盐，其中在磺化之前，如果在步骤d）中没有混合，则可以另外加入基于直链烷基苯中得到的直链烷基苯0至60重量％，f）任选混合如果在阶段d）和e）中没有混合，则在阶段e）中获得的烷基芳基磺酸盐以0至60重量％的量计，基于阶段e）中得到的烷基芳基磺酸盐，为直链烷基芳基磺酸盐。

3. 发明申请

US20090312583A1 PROCESS FOR CODIMERIZING OLEFINS 有权
标题翻译：用于编织烯烃的方法
公开(公告)号：US20090312583A1
公开(公告)日：2009-12-17
申请号：US12303527
申请日：2007-06-06
申请人： Marcus Sigl , Michael Triller , Thomas Heidemann
发明人： Marcus Sigl , Michael Triller , Thomas Heidemann
IPC分类号： C07C29/50 , C07C2/08 , C07C11/00
CPC分类号： C07C2/12 , C07C29/141 , C07C45/50 , C07C2529/06 , C12C11/02 , Y02P20/582 , C07C31/125 , C07C47/02
摘要： The present invention relates to a process for preparing olefin codimers, the olefin codimers which can be obtained by this process, a process for preparing alcohols in which such olefin codimers are subjected to hydroformylation and subsequent hydrogenation, the alcohol mixtures which can be obtained in this way and their use.
摘要翻译：本发明涉及一种制备烯烃共聚物的方法，可通过该方法获得的烯烃共聚物，一种制备醇的方法，其中这种烯烃共聚物经受加氢甲酰化和随后的氢化，可以在此获得的醇混合物方式和使用。

4. 发明授权

US08129572B2 Process for codimerizing olefins 有权
标题翻译：烯烃共聚方法
公开(公告)号：US08129572B2
公开(公告)日：2012-03-06
申请号：US12303527
申请日：2007-06-06
申请人： Marcus Sigl , Michael Triller , Thomas Heidemann
发明人： Marcus Sigl , Michael Triller , Thomas Heidemann
IPC分类号： C07C29/50 , C07C2/08
CPC分类号： C07C2/12 , C07C29/141 , C07C45/50 , C07C2529/06 , C12C11/02 , Y02P20/582 , C07C31/125 , C07C47/02
摘要： The present invention relates to a process for preparing olefin codimers, the olefin codimers which can be obtained by this process, a process for preparing alcohols in which such olefin codimers are subjected to hydroformylation and subsequent hydrogenation, the alcohol mixtures which can be obtained in this way and their use.
摘要翻译：本发明涉及一种制备烯烃共聚物的方法，可通过该方法获得的烯烃共聚物，一种制备醇的方法，其中这种烯烃共聚物经受加氢甲酰化和随后的氢化，可以在此获得的醇混合物方式和使用。

5. 发明申请

US20080176782A1 Production of (Co)Surfactants by Reacting Polyols With Olefins 有权
标题翻译：通过与烯烃反应多元醇制备（Co）表面活性剂
公开(公告)号：US20080176782A1
公开(公告)日：2008-07-24
申请号：US11911028
申请日：2006-04-05
申请人： Jurgen Stephan , Michael Roper , Thomas Heidemann , Michael Triller , Jurgen Tropsch
发明人： Jurgen Stephan , Michael Roper , Thomas Heidemann , Michael Triller , Jurgen Tropsch
IPC分类号： C11D1/66 , C07C41/06 , C07C43/13
CPC分类号： C07C41/06 , C07C43/135 , C08G65/329 , C11D1/72 , C11D1/721 , C11D3/3707 , Y02P20/582
摘要： The present invention relates to a process for preparing polyol alkyl ethers by reacting compounds comprising at least three hydroxyl functionalities with olefins in the presence of acidic catalysts at temperatures of from 20 to 250° C. and pressures of from 0.5 to 10 bar, wherein the olefins correspond to the general formula (I) in which R1 is hydrogen and R2 is a linear or branched carbon radical having from 7 to 28 carbon atoms, or R1 and R2 are each linear or branched carbon radicals having from 1 to 27 carbon atoms, the sum of the carbon number of R1 and R2 being at most 28, to polyol alkyl ethers derived from compounds having at least three hydroxyl functionalities, not more than all but one hydroxyl functionality being replaced by a moiety of the general formula (VIII) to the use of these polyol alkyl ethers as surfactants and to laundry detergents and cleaning compositions comprising these polyol alkyl ethers.
摘要翻译：本发明涉及一种制备多元醇烷基醚的方法，该方法是在20至250℃的温度和0.5至10巴的压力下，在酸性催化剂存在下，使包含至少三个羟基官能团的化合物与烯烃反应，烯烃对应于其中R 1为氢且R 2为具有7至28个碳原子的直链或支链碳基团的通式（I），或R' SUP 1和R 2各自为具有1至27个碳原子的直链或支链碳原子，R 1和R 2的碳数之和至少28个的多元醇烷基醚衍生自具有至少三个羟基官能团的化合物，不超过一个羟基官能团，除了一个羟基官能团被通式（VIII）的部分替代为使用的这些多元醇烷基醚作为表面活性剂和洗涤剂和包含这些多元醇烷基醚的清洁组合物。

6. 发明授权

US07807615B2 Production of (co)surfactants by reacting polyols with olefins 有权
标题翻译：通过使多元醇与烯烃反应制备（共）表面活性剂
公开(公告)号：US07807615B2
公开(公告)日：2010-10-05
申请号：US11911028
申请日：2006-04-05
申请人： Juergen Stephan , Michael Roeper , Thomas Heidemann , Michael Triller , Juergen Tropsch
发明人： Juergen Stephan , Michael Roeper , Thomas Heidemann , Michael Triller , Juergen Tropsch
IPC分类号： C11D1/66
CPC分类号： C07C41/06 , C07C43/135 , C08G65/329 , C11D1/72 , C11D1/721 , C11D3/3707 , Y02P20/582
摘要： The present invention relates to a process for preparing polyol alkyl ethers by reacting compounds comprising at least three hydroxyl functionalities with olefins in the presence of acidic catalysts at temperatures of from 20 to 250° C. and pressures of from 0.5 to 10 bar, wherein the olefins correspond to the general formula (I) in which R1 is hydrogen and R2 is a linear or branched carbon radical having from 7 to 28 carbon atoms, or R1 and R2 are each linear or branched carbon radicals having from 1 to 27 carbon atoms, the sum of the carbon number of R1 and R2 being at most 28, to polyol alkyl ethers derived from compounds having at least three hydroxyl functionalities, not more than all but one hydroxyl functionality being replaced by a moiety of the general formula (VIII) to the use of these polyol alkyl ethers as surfactants and to laundry detergents and cleaning compositions comprising these polyol alkyl ethers.
摘要翻译：本发明涉及一种制备多元醇烷基醚的方法，该方法是在20至250℃的温度和0.5至10巴的压力下，在酸性催化剂存在下，使包含至少三个羟基官能团的化合物与烯烃反应，烯烃对应于其中R 1为氢且R 2为具有7至28个碳原子的直链或支链碳原子的通式（I），或R 1和R 2为具有1至27个碳原子的直链或支链碳原子， R 1和R 2的碳数最多为28的多元醇烷基醚衍生自具有至少三个羟基官能团的化合物的多元醇烷基醚，不超过一个羟基官能团，除了一个羟基官能团被通式（Ⅷ）的部分替代为使用这些多元醇烷基醚作为表面活性剂和洗衣洗涤剂以及包含这些多元醇烷基醚的清洁组合物。

7. 发明授权

US08809588B2 Method for producing aromatic amines 有权
标题翻译：生产芳香胺的方法
公开(公告)号：US08809588B2
公开(公告)日：2014-08-19
申请号：US13320384
申请日：2010-05-05
申请人： Lucia Konigsmann , Ekkehard Schwab , Michael Hesse , Christian Schneider , Thomas Heidemann , Celine Liekens , Jutta Bickelhaupt , Dirk Theis
发明人： Lucia Konigsmann , Ekkehard Schwab , Michael Hesse , Christian Schneider , Thomas Heidemann , Celine Liekens , Jutta Bickelhaupt , Dirk Theis
IPC分类号： C07C209/00
CPC分类号： C07C209/36 , C07C211/46
摘要： The invention relates to a process for preparing aromatic amines by catalytically hydrogenating the corresponding aromatic nitro compound, which comprises using a copper catalyst with a support comprising SiO2, the SiO2 having been prepared by wet grinding and subsequent spray drying.
摘要翻译：本发明涉及通过催化氢化相应的芳族硝基化合物来制备芳族胺的方法，其包括使用具有包含SiO 2的载体的铜催化剂，通过湿法研磨和随后的喷雾干燥制备的SiO 2。

8. 发明授权

US08729331B2 Method for electrochemically removing hydrogen from a reaction mixture 有权
标题翻译：从反应混合物中电化学除去氢的方法
公开(公告)号：US08729331B2
公开(公告)日：2014-05-20
申请号：US13259863
申请日：2010-03-29
申请人： Joana Coelho Tsou , Alexander Panchenko , Annebart Engbert Wentink , Sebastian Ahrens , Thomas Heidemann , Guenther Huber , Albena Kostova
发明人： Joana Coelho Tsou , Alexander Panchenko , Annebart Engbert Wentink , Sebastian Ahrens , Thomas Heidemann , Guenther Huber , Albena Kostova
IPC分类号： C07C7/144
CPC分类号： H01M8/0656 , C01B3/505 , C01B2203/041 , C01B2203/048 , H01M4/92 , H01M4/921 , H01M8/0625 , H01M8/1213 , H01M2008/1095 , H01M2008/1293
摘要： The invention relates to a process for the electrochemical separation of hydrogen from a hydrogen-comprising reaction mixture R by means of a gastight membrane-electrode assembly comprising at least one selectively proton-conducting membrane and at least one electrode catalyst on each side of the membrane, where at least part of the hydrogen present in the reaction mixture R is oxidized to protons over the anode catalyst on the retentate side of the membrane and the protons are, after passing through the membrane to the permeate side, I reduced to hydrogen over the cathode catalyst and/or II reacted with oxygen over the cathode catalyst to form water, with the oxygen originating from an oxygen-comprising stream O which is brought into contact with the permeate side of the membrane, and also a reactor equipped with at least one membrane-electrode assembly.
摘要翻译：本发明涉及通过包含至少一个选择性质子传导膜和至少一个电极催化剂的气密膜 - 电极组件从含氢的反应混合物R电化学分离氢的方法其中存在于反应混合物R中的至少一部分氢被氧化成在膜的滞留侧上的阳极催化剂上的质子，质子在通过膜到达渗透侧之后被还原成氢阴极催化剂和/或II在阴极催化剂上与氧反应形成水，其中氧源源于与膜的渗透侧接触的含氧物流O，以及装有至少一个膜 - 电极组件。

9. 发明授权

US08529869B2 Catalysts and method for the hydroamination of olefins 有权
标题翻译：烯烃水解催化剂和方法
公开(公告)号：US08529869B2
公开(公告)日：2013-09-10
申请号：US13265457
申请日：2010-04-19
申请人： Thomas Heidemann , Jens Kehrer
发明人： Thomas Heidemann , Jens Kehrer
IPC分类号： C01B39/46 , C07C209/60
CPC分类号： B01J29/7057 , B01J29/7007 , B01J37/0201 , B01J2229/186 , C07C209/60 , C07C211/07
摘要： The present invention relates to a hydroamination catalyst comprising boron beta zeolites, wherein the hydroamination catalyst is doped with lithium, and also a process for producing it. The present patent application further relates to a process for preparing amines by reaction of ammonia or primary or secondary amines with olefins at elevated temperatures and pressures in the presence of the hydroamination catalyst of the invention.
摘要翻译：本发明涉及包含硼沸石的水解催化剂，其中所述水化催化剂掺杂有锂，并且还涉及其生产方法。本专利申请还涉及在本发明的水解催化剂存在下，在升高的温度和压力下，通过氨或伯胺或仲胺与烯烃的反应来制备胺的方法。

10. 发明申请

US20120111732A1 METHOD FOR DIRECT AMINATION OF HYDROCARBONS TO FORM AMINO HYDROCARBONS WITH THE ELECTROCHEMICAL SEPARATION OF HYDROCARBON 有权
标题翻译：碳氢化合物的电化学分离直接氨化到氨基碳氢化合物的方法
公开(公告)号：US20120111732A1
公开(公告)日：2012-05-10
申请号：US13383321
申请日：2010-07-08
申请人： Petr Kubanek , Alexander Panchenko , Andreas Fischer , Thomas Heidemann
发明人： Petr Kubanek , Alexander Panchenko , Andreas Fischer , Thomas Heidemann
IPC分类号： C25B1/02 , H01M8/06
CPC分类号： C07C209/02 , C25B3/00 , Y02P20/582 , C07C211/46
摘要： Process for the direct amination of hydrocarbons to aminohydrocarbons, which comprises the steps: a) reaction of a feed stream E comprising at least one hydrocarbon and at least one aminating reagent to form a reaction mixture R comprising aminohydrocarbons and hydrogen and b) electrochemical separation of at least part of the hydrogen formed in the reaction from the reaction mixture R by means of a gastight membrane-electrode assembly having at least one selectively proton-conducting membrane and at least one electrode catalyst on each side of the membrane, where at least part of the hydrogen is oxidized to protons over the anode catalyst on the retentate side of the membrane and the protons are, after passing through the membrane, b1) reduced to hydrogen and/or b2) reacted with oxygen from an oxygen-comprising stream O which is brought into contact with the permeate side of the membrane to form water over the cathode catalyst on the permeate side.
摘要翻译：用于将烃直接胺化成氨基烃的方法，其包括以下步骤：a）包含至少一种烃和至少一种氨化试剂的进料流E的反应以形成包含氨基烃和氢的反应混合物R和b）电化学分离通过具有至少一个选择性质子传导膜和在膜的每一侧上的至少一个电极催化剂的气密膜 - 电极组件在反应混合物R的反应中形成的至少一部分氢，其中至少部分的氢被氧化成在膜的滞留侧上的阳极催化剂上的质子，并且质子在通过膜之后，b1）还原为氢和/或b2）与来自含氧流O的氧反应，其中与膜的渗透侧接触以在渗透侧的阴极催化剂上形成水。

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