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1. 发明授权

US5506302A Organopolysiloxane composition and rubber substrate having a coating thereof 失效
标题翻译：有机聚硅氧烷组合物和具有其涂层的橡胶基材
公开(公告)号：US5506302A
公开(公告)日：1996-04-09
申请号：US493154
申请日：1995-06-21
申请人： Mikio Shiono , Kazumi Okada , Hironao Fujiki
发明人： Mikio Shiono , Kazumi Okada , Hironao Fujiki
IPC分类号： C08K7/16 , C08K13/02 , C09D183/04 , C08K5/54
CPC分类号： C08K13/02 , C08K7/16 , C09D183/04
摘要： An organopolysiloxane composition contains (A) a both end hydroxyl-blocked diorganopoly-siloxane, (B) a hydroxyl-free diorganopoly-siloxane having a degree of polymerization equal to or greater than that of (A), (C) an organo-hydrogenpolysiloxane having at least three hydrogen atoms in a molecule, (D) an organosilane containing at least two alkoxy groups and an amino group attached to a silicon atom through an alkylene group in a molecule and/or a partial hydrolyzate thereof, (E) a fatty acid metal salt, (F) polycarbonate powder having a mean particle size of up to 50 .mu.m, and optionally (G) an organo-silane containing at least two alkoxy groups and a mercapto group attached to a silicon atom through an alkylene group in a molecule and/or a partial hydrolyzate thereof. It is applied to a rubber substrate to form a wear resistance coating thereon.
摘要翻译：有机聚硅氧烷组合物含有（A）双端羟基封端的二有机硅氧烷，（B）聚合度等于或大于（A）的聚合度的无羟基的二有机聚硅氧烷，（C）有机氢聚硅氧烷在分子中具有至少三个氢原子，（D）含有至少两个烷氧基的有机硅烷和通过分子中的亚烷基与硅原子连接的氨基和/或其部分水解产物，（E）脂肪酸性金属盐，（F）平均粒径达50μm的聚碳酸酯粉末，以及任选地（G）含有至少两个烷氧基的有机硅烷和通过亚烷基连接到硅原子上的巯基，分子和/或部分水解产物。将其施加到橡胶基材上以在其上形成耐磨性涂层。

2. 发明授权

US5064891A Curable silicone compositions 失效
标题翻译：可固化硅胶组合物
公开(公告)号：US5064891A
公开(公告)日：1991-11-12
申请号：US525047
申请日：1990-05-18
申请人： Hironao Fujiki , Mikio Shiono , Toshiaki Takahashi
发明人： Hironao Fujiki , Mikio Shiono , Toshiaki Takahashi
IPC分类号： A61K6/10 , C08L83/04 , C08L83/07 , G02B1/04
CPC分类号： A61K6/10 , C08L83/04 , G02B1/043 , C08G77/12 , C08G77/20 , C08G77/46 , Y10S524/912
摘要： A curable silicone composition comprising:(A) an organopolysiloxane having at least two silicon-bonded aliphatic unsaturated hydrocarbon radicals in its molecule;(B) an organohydrogenpolysiloxane having at least three silicon-bonded hydrogen atoms in its molecule;(C) a platinum family metal catalyst; and(D) a nonionic surface active agent having a hydrophobic silicone portion and at least one hydrophilic polyol portion in its molecule. The curable silicone composition gives cured products having good hydrophilic properties and dimensional stability, and are especially suitable for use as a dental impression material.

3. 发明授权

US5120810A Adhesive composition 失效
标题翻译：粘合剂组合物
公开(公告)号：US5120810A
公开(公告)日：1992-06-09
申请号：US522013
申请日：1990-05-11
申请人： Hironao Fujiki , Mikio Shiono , Toshiaki Takahashi
发明人： Hironao Fujiki , Mikio Shiono , Toshiaki Takahashi
IPC分类号： C08G77/14 , C08K3/10 , C08K5/5435 , C08K5/549 , C08L83/05 , C08L83/07 , C09D183/04 , C09D183/05 , C09D183/07 , C09J183/00 , C09J183/04 , C09J183/05 , C09J183/07
CPC分类号： C09J183/04
摘要： This invention discloses an adhesive organopolysiloxane compositions which cure in the presence of addition reaction catalysts and adhere firmly to various materials when they harden comprising;(1) 100 parts by weight of an organopolysiloxane containing at least alkenyl groups bonded to silicon atoms in 1 molecule,(2) an organohydrogenpolysiloxane containing at least 3 hydrogen atoms bonded to silicon atoms in 1 molecule, in sufficient quantity to donate 0.5-10 hydrogen atoms bonded to silicon atoms to 1 alkenyl group in said 1st constituent,(3) 0.1-20 parts by weight of an organosilicone compound containing at least 1 hydrogen atom bonded to silicon atoms, at least 1 fluoroalkyl group or fluoroalkylether group bonded to silicon atoms via carbon atoms and at least 1 epoxy group and/or trialkoxysilyl group bonded to silicon atoms via carbon atoms in 1 molecule, and(4) platinum or a platinum compound in suitable quantity to act as a catalyst.
摘要翻译：本发明公开了一种粘合剂有机聚硅氧烷组合物，其在加成反应催化剂存在下固化，并且在硬化时牢固地粘附到各种材料上，（1）100重量份在1分子中至少含有与硅原子键合的烯基的有机聚硅氧烷，（2）在1分子中含有至少3个与硅原子键合的氢原子的有机氢聚硅氧烷，以足够的量配合0.5-10 所述第一成分中与硅原子键合至1个烯基的氢原子，（3）0.1-20重量份含有至少1个与硅原子键合的氢原子的有机硅化合物，至少1个氟烷基或与硅键合的氟烷基通过碳原子和至少1个环氧基和/或通过1分子中的碳原子键合到硅原子上的三烷氧基甲硅烷基，和（4）铂或铂化合物以合适的量作为催化剂。

4. 发明授权

US5854344A Organopolysiloxane composition for electrical insulation 失效
标题翻译：电绝缘用有机聚硅氧烷组合物
公开(公告)号：US5854344A
公开(公告)日：1998-12-29
申请号：US704866
申请日：1996-08-30
申请人： Mikio Shiono , Mitsuaki Igarashi , Hironao Fujiki
发明人： Mikio Shiono , Mitsuaki Igarashi , Hironao Fujiki
IPC分类号： C08L83/04 , C08L83/07 , C08L83/05 , C08G77/08 , C08K3/36
CPC分类号： C08L83/04 , C08G77/12 , C08G77/16 , C08G77/20 , C08G77/24 , C08G77/70
摘要： There is provided an organopolysiloxane composition for electrical insulation wherein the fluidity is good and an inorganic filler deposited on the bottom of a vessel during the storage can be easily and simply redispersed. The unfoamable organopolysiloxane composition for electrical insulation comprises (A) an organopolysiloxane containing at least two alkenyl groups each bonded to a silicon atom in the molecule, (B) an organohydrogenpolysiloxane containing at least two hydrogen atoms each bonded to a silicon atom in the molecule, (C) an organopolysiloxane containing at least one hydroxyl group bonded to a silicon atom in the molecule, (D) an inorganic filler having an average particle diameter of 1 to 50 .mu.m, and (E) platinum or a platinum compound.
摘要翻译：提供了一种用于电绝缘的有机基聚硅氧烷组合物，其中流动性良好，并且在储存期间沉积在容器底部的无机填料可以容易且简单地再分散。用于电绝缘的不可发射的有机基聚硅氧烷组合物包含（A）含有至少两个各自键合到分子中的硅原子的烯基的有机聚硅氧烷，（B）含有至少两个分别键合到硅原子上的氢原子的有机氢聚硅氧烷，（C）分子中含有与硅原子键合的至少一个羟基的有机聚硅氧烷，（D）平均粒径为1〜50μm的无机填料，（E）铂或铂化合物。

5. 发明授权

US5661198A Ablator compositions 失效
标题翻译：消音器组成
公开(公告)号：US5661198A
公开(公告)日：1997-08-26
申请号：US312734
申请日：1994-09-27
申请人： Yoshifumi Inatani , Kazunori Kawasaki , Tadashi Harada , Hironao Fujiki , Mikio Shiono
发明人： Yoshifumi Inatani , Kazunori Kawasaki , Tadashi Harada , Hironao Fujiki , Mikio Shiono
IPC分类号： C08K7/14 , C08K7/22 , C08L83/04 , C08L83/07 , C09K21/14 , C08G77/06
CPC分类号： C09K21/14 , B64G1/58 , B64G1/62 , C08K7/14 , C08K7/22 , C08L83/04 , C08G77/12 , C08G77/20 , C08G77/70
摘要： The invention relates to an ablator composition for providing ablation protection. The ablator composition comprises 100 parts by weight of a mixture of vinyl-containing organopolysiloxanes, the mixture containing 50-80 wt. % of a diorganopolysiloxane which contains vinyl groups and 20-50 wt. % of a silicone resin which contains vinyl groups; an organohydrogenpolysiloxane containing in one molecule thereof at least three hydrogen atoms which are directly bonded to silicon atoms thereof; a catalyst which is at least one selected from the group consisting of metallic platinum and platinum compounds; up to 150 parts by weight of silica microballoons; and at least one selected from the group consisting of up to 15 parts by weight of quartz glass fibers and up to 15 parts by weight of carbon fibers. An ablator material prepared by curing the ablator composition has a low surface recession rate even under a condition of a high heating rate such as about 4 MW/m.sup.2 and a high pressure such as about one atmospheric pressure.
摘要翻译：本发明涉及一种用于提供消融保护的消融器组合物。消融器组合物包含100重量份的含乙烯基的有机聚硅氧烷的混合物，该混合物含有50-80wt。％的含有乙烯基的二有机聚硅氧烷和20-50wt。含有乙烯基的硅树脂的％在一个分子中含有至少三个与其硅原子键合的氢原子的有机氢聚硅氧烷; 选自金属铂和铂化合物中的至少一种的催化剂; 最多150重量份的二氧化硅微球; 和至少一种选自由至多15重量份的石英玻璃纤维和至多15重量份的碳纤维组成的组。即使在高加热速度如约4MW / m 2和高压例如约一个大气压的条件下，通过固化消融器组合物制备的消融器材料也具有低表面凹陷率。

6. 发明授权

US5438094A Adhesive silicone compositions 失效
标题翻译：粘合硅胶组合物
公开(公告)号：US5438094A
公开(公告)日：1995-08-01
申请号：US266336
申请日：1994-07-01
申请人： Hironao Fujiki , Hiroyasu Hara , Mikio Shiono , Masayuki Ikeno
发明人： Hironao Fujiki , Hiroyasu Hara , Mikio Shiono , Masayuki Ikeno
IPC分类号： C08L83/04 , C09J183/04 , C09J183/07 , C08K5/54
CPC分类号： C08L83/04 , C09J183/04 , C08G77/12 , C08G77/20 , C08G77/24 , C08G77/70
摘要： An adhesive silicone composition comprising (A) an alkenyl group-containing organopolysiloxane, (B) an organohydrogen-polysiloxane having at least three hydrogen atoms each directly bonded to a silicon atom in a molecule, (C) a compound having at least one aliphatic unsaturated group and at least two phenyl skeletons in a molecule, and (D) a platinum catalyst is well adhesive to both metals and reins, and even to difficult-to-adhere resins such as nylon, polycarbonate and acryl resins.
摘要翻译：一种粘合性硅氧烷组合物，其包含（A）含链烯基的有机聚硅氧烷，（B）具有至少三个氢原子的有机氢 - 聚硅氧烷，每个氢原子分别直接键合到硅原子上，（C）具有至少一个脂族不饱和基团的化合物基团和至少两个苯基骨架，以及（D）铂催化剂对金属和筘具有良好的粘合性，并且甚至难以粘附的树脂如尼龙，聚碳酸酯和丙烯酸树脂。

7. 发明授权

US5525660A Organopolysiloxane compositions and rubber articles 失效
标题翻译：有机聚硅氧烷组合物和橡胶制品
公开(公告)号：US5525660A
公开(公告)日：1996-06-11
申请号：US354064
申请日：1994-12-06
申请人： Mikio Shiono , Kazumi Okada
发明人： Mikio Shiono , Kazumi Okada
IPC分类号： C08L83/04 , C09D183/04 , C08K5/54
CPC分类号： C09D183/04 , C08L83/04 , C08G77/04 , C08G77/16
摘要： An organopolysiloxane composition contains (A) a both end hydroxyl-blocked diorganopolysiloxane, (B) an inert diorganopolysiloxane, (C) a silane or siloxane having at least three hydrolyzable functional groups, (D) an organosilane having at least two alkoxy groups each attached to a silicon atom and one mercapto group separated from a silicon atom by an alkylene group or a partial hydrolyzate thereof, (E) an organosilane having at least two alkoxy groups each attached to a silicon atom and one amino group separated from a silicon atom by an alkylene group or a partial hydrolyzate thereof, (F) a condensation catalyst, and (G) a fine powder, typically of polycarbonate, having a mean particle size of 0.1-50 .mu.m. The composition is useful as a surface treating agent for cured rubber moldings for imparting non-tackiness, water repellency and lubricity to the rubber surface and forming a long-lasting abrasion resistant coating.
摘要翻译：有机聚硅氧烷组合物含有（A）两末端羟基封端的二有机聚硅氧烷，（B）惰性二有机聚硅氧烷，（C）具有至少三个可水解官能团的硅烷或硅氧烷，（D）具有至少两个烷氧基的有机硅烷，通过亚烷基或其部分水解物与硅原子分离的硅原子和一个巯基，（E）具有至少两个烷氧基的有机硅烷各自连接到硅原子上，一个氨基与硅原子分开，通过（F）缩合催化剂，（G）通常为聚碳酸酯的平均粒径为0.1-50μm的细粉末。该组合物可用作固化橡胶模制品的表面处理剂，用于赋予橡胶表面非粘性，防水性和润滑性并形成持久的耐磨涂层。

8. 发明授权

US08299196B2 Adhesive composition 有权
标题翻译：粘合剂组合物
公开(公告)号：US08299196B2
公开(公告)日：2012-10-30
申请号：US13085510
申请日：2011-04-13
申请人： Mikio Shiono , Noriyuki Koike
发明人： Mikio Shiono , Noriyuki Koike
IPC分类号： C08G77/08
CPC分类号： C09D183/08 , C08G77/24 , C08L71/02
摘要： An adhesive composition is provided comprising (A) a fluorinated amide compound containing at least two vinyl groups and having a polyfluoro structure, (B) a fluorinated organosilicon compound containing a fluorinated organic group, at least two SiH groups, and an alkyl, aryl or aralkyl group, and (C) a platinum catalyst, and (D) an organosiloxane containing a SiH group and an epoxy and/or trialkoxysilyl group. The composition is cured on brief heating into a product which achieves adhesion to various substrates and has solvent resistance, chemical resistance, heat resistance, low-temperature properties, low moisture permeability, electric insulation, and acid resistance.
摘要翻译：提供一种粘合剂组合物，其包含（A）含有至少两个乙烯基并具有多氟结构的氟化酰胺化合物，（B）含氟化有机基团的氟化有机硅化合物，至少两个SiH基团和烷基，芳基或芳族烷基，（C）铂催化剂，（D）含有SiH基和环氧基和/或三烷氧基甲硅烷基的有机硅氧烷。该组合物在短暂加热下固化成实现对各种基材的粘合性的产品，并具有耐溶剂性，耐化学性，耐热性，低温性，低透湿性，电绝缘性和耐酸性。

9. 发明授权

US08110065B2 Heat-curable fluoropolyether adhesive composition and bonding method 有权
标题翻译：可热固化的氟聚醚粘合剂组合物和粘合方法
公开(公告)号：US08110065B2
公开(公告)日：2012-02-07
申请号：US12124556
申请日：2008-05-21
申请人： Hidenori Koshikawa , Mikio Shiono , Hiroyasu Hara , Takashi Aketa
发明人： Hidenori Koshikawa , Mikio Shiono , Hiroyasu Hara , Takashi Aketa
IPC分类号： C04B37/00 , C09J7/02 , C08F283/00 , C08F283/12 , C08G77/00 , C08G77/38 , C08L83/00
CPC分类号： C08G65/007 , C08G2650/48 , C08K5/0025 , C08L83/00 , C08L83/08 , C08L2666/34 , C09J171/02
摘要： A heat-curable fluoropolyether adhesive composition comprising (A) a linear polyfluoro compound having at least two alkenyl groups and a perfluoropolyether structure, (B) a fluorinated organohydrogensiloxane having at least two SiH groups, (C) a platinum group metal catalyst, (D) an organosiloxane having at least one SiH group and at least one epoxy and/or trialkoxysilyl group, and (E) a compound having at least two allyloxycarbonyl groups can be cured to metal and plastic substrates by heating at a temperature from 20° C. to less than 100° C.
摘要翻译：一种可热固化的氟聚醚粘合剂组合物，其包含（A）具有至少两个烯基和全氟聚醚结构的线性多氟化合物，（B）具有至少两个SiH基团的氟化有机氢硅氧烷，（C）铂族金属催化剂，（D ）具有至少一个SiH基团和至少一个环氧基和/或三烷氧基甲硅烷基的有机硅氧烷，和（E）具有至少两个烯丙氧基羰基的化合物可以通过在20℃的温度下加热固化到金属和塑料基材上。至小于100℃

10. 发明授权

US07851066B2 Curable fluoropolyether composition and integral molded resin/rubber articles 有权
标题翻译：可固化的氟聚醚组合物和整体模塑树脂/橡胶制品
公开(公告)号：US07851066B2
公开(公告)日：2010-12-14
申请号：US12124436
申请日：2008-05-21
申请人： Hiromasa Yamaguchi , Mikio Shiono
发明人： Hiromasa Yamaguchi , Mikio Shiono
IPC分类号： B32B9/04
CPC分类号： C08G65/007 , C08G65/336 , C08G77/12 , C08G77/24 , C08G2650/48 , C08L71/02 , C08L83/04 , C08L2205/02 , Y10T428/31663 , Y10T428/31786 , C08L83/00
摘要： Curable fluoropolyether compositions comprising (a) a polyfluorodialkenyl compound, (b) a fluorinated organohydrogenpolysiloxane, (c) a platinum catalyst, (d) hydrophobic silica powder, (e) a tackifier in the form of a specific silicon compound, and (f) an organosiloxane having a SiH group, an epoxy and/or trialkoxysilyl group, and a perfluoroalkyl or perfluoropolyether group cure to thermoplastic resins to form a durable tight bond at a low temperature within a short time and are readily releasable from metal molds.
摘要翻译：固化氟聚醚组合物，其包含（a）多氟二烯基化合物，（b）氟化有机氢聚硅氧烷，（c）铂催化剂，（d）疏水性二氧化硅粉末，（e）特定硅化合物形式的增粘剂，和（f）具有SiH基团，环氧基和/或三烷氧基甲硅烷基的有机硅氧烷和全氟烷基或全氟聚醚基固化成热塑性树脂，以在短时间内在低温下形成耐久的紧密结合，并且容易从金属模上释放。

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