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1. 发明授权

US5998530A Flowability of mineral oils and mineral oil distillates using alkylphenol-aldehyde resins 失效
标题翻译：使用烷基酚 - 醛树脂的矿物油和矿物油馏出物的流动性
公开(公告)号：US5998530A
公开(公告)日：1999-12-07
申请号：US002614
申请日：1998-01-05
申请人： Matthias Krull , Michael Feustel , Werner Reimann , Ulrike Tepper
发明人： Matthias Krull , Michael Feustel , Werner Reimann , Ulrike Tepper
IPC分类号： C10L1/16 , C10L1/14 , C10L1/18 , C10L1/182 , C10L1/192 , C10L1/197 , C10L1/198 , C10L1/22 , C10L10/18 , C08K5/01 , C10L1/04 , C10L1/10
CPC分类号： C10L10/14 , C10L1/143 , C10L1/18 , C10L1/1608 , C10L1/1616 , C10L1/1824 , C10L1/1881 , C10L1/19 , C10L1/1966 , C10L1/1973 , C10L1/1981 , C10L1/1985 , C10L1/221 , C10L1/2222 , C10L1/2225 , C10L1/224 , C10L1/2364 , C10L1/2368 , C10L1/238
摘要： Improving the flowability of mineral oils and mineral oil distillates using alkylphenol-aldehyde resinsThe invention relates to a process for improving the flowability of paraffin-containing mineral oils and mineral oil distillates by adding flow improvers based on ethylene/vinyl ester co- and terpolymers, alkylphenol-aldehyde resins and, if appropriate, other paraffin dispersants, mixtures of these different flow improvers and mineral oils and mineral oil distillates which comprise these flow improvers.
摘要翻译：使用烷基酚醛树脂提高矿物油和矿物油馏出物的流动性本发明涉及一种通过加入基于乙烯/乙烯基酯共聚物和三元共聚物的流动改进剂来改进含石蜡矿物油和矿物油馏出物的流动性的方法，烷基酚醛树脂，以及如果合适的话，其它石蜡分散剂，这些不同流动改进剂的混合物和矿物油以及包含这些流动改进剂的矿物油馏分。

2. 发明授权

US5439981A Graft polymers, their preparation and use as pour point depressants and flow improvers for crude oils, residual oils and middle distillates 失效
标题翻译：接枝聚合物，它们的制备和用作倾点下降剂和用于原油，残油和中间馏分的流动改进剂
公开(公告)号：US5439981A
公开(公告)日：1995-08-08
申请号：US163085
申请日：1993-12-07
申请人： Juliane Balzer , Michael Feustel , Matthias Krull , Werner Reimann
发明人： Juliane Balzer , Michael Feustel , Matthias Krull , Werner Reimann
IPC分类号： C08F8/30 , C08F255/00 , C08F255/02 , C10L1/14 , C10L1/16 , C10L1/22 , C10L1/236 , C10M149/06 , C10M143/02
CPC分类号： C10M149/06 , C08F255/026 , C08F8/30 , C10L1/143 , C10L1/2364 , C10L1/1616 , C10M2205/00 , C10M2205/02 , C10M2209/062 , C10M2217/024 , C10M2217/06
摘要： Graft polymers which comprise 20 to 99.9% by weight of an ethylene copolymer (base polymer) and 0.1 to 80% by weight of a graft component. The base polymer includes 30% to 95% by weight of ethylene and (1) 5% to 70% by weight of vinyl esters of saturated aliphatic C.sub.2 - to C.sub.18 -monocarboxylic acids or (2) 4% to 50% by weight of vinyl esters of saturated aliphatic C.sub.2 - to C.sub.18 -monocarboxylic acids and 1% to 20% by weight of linear or branched C.sub.3 - to C.sub.18 -monoolefins. Graft components are N-substituted alpha,beta-unsaturated dicarboxylic acid imides, dicarboxylic acid amides, dicarboxylic acid half-amides, or ammonium salts of the half-amides. The graft polymers are employed for improving the flow properties of paraffin-containing mineral oils, mineral oil distillates, and middle distillates.
摘要翻译：包含20至99.9重量％的乙烯共聚物（基础聚合物）和0.1至80重量％的接枝组分的接枝聚合物。基础聚合物包括30重量％至95重量％的乙烯和（1）5重量％至70重量％的饱和脂族C 2 -C 18单羧酸的乙烯基酯或（2）4重量％至50重量％饱和脂肪族C 2 -C 18单羧酸酯和1％-20％重量的直链或支链C 3 -C 18单烯烃。接枝组分是N-取代的α，β-不饱和二羧酸酰亚胺，二羧酸酰胺，二羧酸半酰胺或半酰胺的铵盐。接枝聚合物用于改进含石蜡矿物油，矿物油馏分和中间馏分的流动性能。

3. 发明授权

US08293690B2 Dispersions of polymer oil additives 有权
标题翻译：聚合物油添加剂的分散体
公开(公告)号：US08293690B2
公开(公告)日：2012-10-23
申请号：US12520358
申请日：2007-06-28
申请人： Michael Feustel , Matthias Krull , Christoph Kayser , Mario Loew
发明人： Michael Feustel , Matthias Krull , Christoph Kayser , Mario Loew
IPC分类号： C10M173/00 , C10M161/00
CPC分类号： C10L1/10 , C10L1/125 , C10L1/1608 , C10L1/1616 , C10L1/1641 , C10L1/1824 , C10L1/1826 , C10L1/1855 , C10L1/1857 , C10L1/1885 , C10L1/1886 , C10L1/1888 , C10L1/19 , C10L1/1963 , C10L1/1966 , C10L1/1973 , C10L1/198 , C10L1/1981 , C10L1/1985 , C10L1/2225 , C10L1/2335 , C10L10/16 , C10M169/044 , C10M173/02 , C10M2205/02 , C10M2205/022 , C10M2205/028 , C10M2207/021 , C10M2207/022 , C10M2207/08 , C10M2207/16 , C10M2207/18 , C10M2207/20 , C10M2207/281 , C10M2209/101 , C10M2209/103 , C10N2220/023 , C10N2230/04 , C10N2230/08 , C10N2250/12 , C10M2209/062 , C10M2209/084 , C10M2209/08
摘要： The invention relates to dispersions comprising I) at least one polymer that is effective for mineral oils as a cold extrusion improver and is soluble in oil, II) at least one organic solvent that cannot be mixed with water, III) water, IV) at least one alkanolamine salt of a polycyclic carboxylic acid as a dispersing agent, and V) possibly at least one organic solvent that can be mixed with water.
摘要翻译：本发明涉及分散体，其包括I）至少一种对矿物油作为冷挤出改进剂有效并且可溶于油的聚合物，II）至少一种不能与水混合的有机溶剂，III）水，IV）在作为分散剂的多环羧酸的至少一种链烷醇胺盐，以及V）可能与水混合的至少一种有机溶剂。

4. 发明授权

US08123930B2 Additives for crude oils 失效
标题翻译：原油添加剂
公开(公告)号：US08123930B2
公开(公告)日：2012-02-28
申请号：US11525881
申请日：2006-09-22
申请人： Carsten Cohrs , Matthias Krull , Michael Feustel , Heidi Rausch
发明人： Carsten Cohrs , Matthias Krull , Michael Feustel , Heidi Rausch
IPC分类号： C10G71/00
CPC分类号： C10L1/1985 , B01D17/047 , C09K8/524 , C10L1/1981 , C10L10/16 , C10L10/18 , C10M2209/101 , C10N2230/04 , C10N2230/08 , C10N2230/24
摘要： The invention thus provides crude oils and products which have been produced therefrom and comprise distillation residues, comprising at least one alkylphenol-aldehyde resin having a repeat structural unit of the formula where R1 is a branched alkyl or alkenyl radical which has from 10 to 40 carbon atoms and bears at least one carboxyl, carboxylate and/or ester group, R2 is hydrogen or R1 R3 is hydrogen or an alkoxy group of the formula -(A-O)m—H, A is a C2- to C4-alkylene group, m is from 1 to 100, R4 is hydrogen, a C1- to C11-alkyl radical or a carboxyl group, R5 is C1-C200-alkyl or -alkenyl, O—R6 or O—C(O)—R6, R6 is C1-C200-alkyl or -alkenyl, n is from 1 to 100 and k is 1 or 2, the use of the alkylphenol-aldehyde resin for splitting emulsions of water and crude oils or products derived therefrom, the use of the alkylphenol-aldehyde resin for improving the cold flowability of crude oils and products derived therefrom, and the use of the alkylphenol-aldehyde resin as an asphaltene dispersant in crude oils and products derived therefrom.
摘要翻译：因此，本发明提供了由其生产并包含蒸馏残余物的原油和产品，其包含至少一种具有下式重复结构单元的烷基酚醛树脂，其中R 1是具有10至40个碳原子的支链烷基或烯基原子并具有至少一个羧基，羧酸酯和/或酯基团，R 2是氢或R 1 R 3是氢或式 - （AO）m -H的烷氧基，A是C 2 -C 4亚烷基，m 为1〜100，R 4为氢，C 1至C 11 - 烷基或羧基，R 5为C 1 -C 20 - 烷基或 - 烯基，O-R 6或O-C（O）-R 6，R 6为C 1 -C 200 - 烷基或 - 烯基，n为1〜100，k为1或2，使用烷基酚 - 醛树脂分解水和原油或其衍生产物的乳液，使用烷基酚醛树脂用于改善原油及其衍生物的冷流动性，以及使用烷基苯酚 - 醛树脂作为沥青原油中的分散剂和由其衍生的产物。

5. 发明授权

US06821933B2 Additives for improving the cold flow properties and the storage stability of crude oil 失效
标题翻译：用于改善冷流特性和原油储存稳定性的添加剂
公开(公告)号：US06821933B2
公开(公告)日：2004-11-23
申请号：US10311057
申请日：2002-12-13
申请人： Michael Feustel , Matthias Krull , Hans-Jörg Oschmann
发明人： Michael Feustel , Matthias Krull , Hans-Jörg Oschmann
IPC分类号： C10M15700
CPC分类号： C10L1/143 , C10L1/1641 , C10L1/1963 , C10L1/1966 , C10L1/1973 , C10L1/1981 , C10L1/2437
摘要： The invention relates to additives for improving the flowability of mineral oils, containing: A) 1-40 wt. % of at least one copolymer, which is oil-soluble and improves the cold flow properties of mineral oil, selected from A1) copolymers consisting of 80 to 96.5 mol % ethylene and 3.5-20 mol % vinyl esters of carboxylic acids with 1-20 C atoms and/or (meth)acrylic acid esters of alcohols with 1-8 C atoms, and A2) homopolymers or copolymers of esters, containing C10-C30 alkyl radicals, of ethylenically unsaturated carboxylic acids with up to 20 mol % of other olefinically unsaturated compounds, B) 20-80 wt. % of at least one poly-alpha-olefin with a molecular weight of 250-5000, derived from monoolefins with 3-5 C atoms, and C) 5-70 wt. % of at least one organic acid selected from C1) alkylphenol-aldehyde resins of formula (1), wherein R1 and R2 independently designate H or alkyl radicals with 1-30 C atoms, but both radicals do not at the same time signify H, n represents an integer of 3-50, and R3 represents H or an alkyl radical with 1-4 C atoms, and C2) aliphatic and/or aromatic sulfonic acids of formula R18—SO3H, wherein R18 stands for C6-C40-alkyl, C6-C40-alkenyl, or an alk(en)yl aryl radical which has 1, 2, 3 or 4 aromatic rings and 1, 2, 3 or 4 alkyl or aryl radicals with respectively 6-40 C-atoms.
摘要翻译：本发明涉及用于改善矿物油的流动性的添加剂，其含有：A）1-40wt。％的至少一种共聚物，其是油溶性的并且改善矿物油的冷流动性质，选自A1）由80至96.5mol％乙烯和3.5-20mol％羧酸乙烯基酯与1-20 C原子和/或具有1-8个C原子的醇的（甲基）丙烯酸酯，和A2）烯键式不饱和羧酸与含有至多20摩尔％其它烯属不饱和羧酸的C 10 -C 30烷基酯的均聚物或共聚物不饱和化合物，B）20-80wt。％的至少一种分子量为250-5000的聚-α-烯烃，衍生自具有3-5个C原子的单烯烃，和C）5-70wt。％的至少一种选自式（1）的C1）烷基酚醛树脂的有机酸，其中R 1和R 2独立地表示H或具有1-30个C原子的烷基，但两个基团不在同时表示H，n表示3-50的整数，R 3表示H或具有1-4个C原子的烷基，以及C2）式R 18的脂族和/或芳族磺酸 - SO 3 H，其中R 18代表C 6 -C 40 - 烷基，C 6 -C 40 - 烯基或具有1,2,3或4个芳环和1,2,3或4个烷基的烷基（烯）基芳基，或具有6-40个C原子的芳基。

6. 发明申请

US20070221539A1 Additives for crude oils 失效
标题翻译：原油添加剂
公开(公告)号：US20070221539A1
公开(公告)日：2007-09-27
申请号：US11525881
申请日：2006-09-22
申请人： Carsten Cohrs , Matthias Krull , Michael Feustel , Heidi Rausch
发明人： Carsten Cohrs , Matthias Krull , Michael Feustel , Heidi Rausch
IPC分类号： C10G71/00
CPC分类号： C10L1/1985 , B01D17/047 , C09K8/524 , C10L1/1981 , C10L10/16 , C10L10/18 , C10M2209/101 , C10N2230/04 , C10N2230/08 , C10N2230/24
摘要： The invention thus provides crude oils and products which have been produced therefrom and comprise distillation residues, comprising at least one alkylphenol-aldehyde resin having a repeat structural unit of the formula where R1 is a branched alkyl or alkenyl radical which has from 10 to 40 carbon atoms and bears at least one carboxyl, carboxylate and/or ester group, R2 is hydrogen or R1 R3 is hydrogen or an alkoxy group of the formula -(A-O)m—H, A is a C2- to C4-alkylene group, m is from 1 to 100, R4 is hydrogen, a C1- to C11-alkyl radical or a carboxyl group, R5 is C1-C200-alkyl or -alkenyl, O—R6 or O—C(O)—R6, R6 is C1-C200-alkyl or -alkenyl, n is from 1 to 100 and k is 1 or 2, the use of the alkylphenol-aldehyde resin for splitting emulsions of water and crude oils or products derived therefrom, the use of the alkylphenol-aldehyde resin for improving the cold flowability of crude oils and products derived therefrom, and the use of the alkylphenol-aldehyde resin as an asphaltene dispersant in crude oils and products derived therefrom.
摘要翻译：因此，本发明提供由其制备的原油和产品，其包含蒸馏残余物，其包含至少一种具有下式重复结构单元的烷基酚醛树脂：其中R 1是支链烷基或链烯基具有10至40个碳原子并具有至少一个羧基，羧酸酯和/或酯基团的基团，R 2是氢或R 1，R 3， / SUP>是氢或式的烷氧基<？in-line-formula description =“In-line Formulas”end =“lead”→>（AO）？in-line-formula description =“In-line Formulas”end =“tail”？> A是C 4 - 亚烷基，m是 1至100，R 4是氢，C 1至C 11 - 烷基或羧基，R 11， 5是C 1 -C 20 - 烷基或 - 烯基，或6或OC（O）-R 6，R 6为C 1 -C 20 - 烷基或 - 烯基，n为1至100，并且 k为1或2，使用烷基苯酚醛树脂来分解水和原油或其衍生产物的乳液，使用烷基苯酚醛树脂来改善原油及其衍生产物的冷流动性，以及在原油中使用烷基酚醛树脂作为沥青质分散剂和由其衍生的产品。

7. 发明申请

US20140004611A1 METHOD FOR DETERMINING THE CONTENT OF HYDROGEN SULFIDE IN CRUDE AND RESIDUAL OILS 有权
标题翻译：测定硫化氢在残留油中的含量的方法
公开(公告)号：US20140004611A1
公开(公告)日：2014-01-02
申请号：US14001325
申请日：2012-02-14
申请人： Michael Feustel , Michael Brauchle , Dominko Andrin , Matthias Krull
发明人： Michael Feustel , Michael Brauchle , Dominko Andrin , Matthias Krull
IPC分类号： G01N33/28
CPC分类号： G01N33/287 , C10G21/14 , C10G2300/1033 , C10G2300/1048 , C10G2300/202 , C10G2300/207 , C10G2300/4006 , C10G2300/44 , G01N33/28 , Y10T436/182 , Y10T436/184
摘要： The subject of the invention is a method for determining the H2S content arising during the warm storage of sulfur-containing crude and residual oils and mineral distillates containing sulfur-containing crude and/or residual oils, in which a sample of the sulfur-containing mineral oil is dissolved in a solvent or solvent mixture that boils at more than 200° C. and a carrier gas is caused to flow through the solution of the sulfur-containing mineral oil at temperatures above 80° C., and the quantity of hydrogen sulfide carried out with the carrier gas is analyzed quantitatively.
摘要翻译：本发明的主题是确定在含硫含粗油和/或残余油的含硫原油和残余油和矿物馏出物的热储存期间产生的H 2 S含量的方法，其中含硫矿物样品油溶解在沸点高于200℃的溶剂或溶剂混合物中，并使载气在高于80℃的温度下流过含硫矿物油的溶液，并且硫化氢的量对载气进行定量分析。

8. 发明申请

US20100025290A1 Dispersions Of Polymer Oil Additives 有权
标题翻译：聚合物油添加剂的分散体
公开(公告)号：US20100025290A1
公开(公告)日：2010-02-04
申请号：US12520358
申请日：2007-06-28
申请人： Michael Feustel , Matthias Krull , Christoph Kayser , Mario Loew
发明人： Michael Feustel , Matthias Krull , Christoph Kayser , Mario Loew
IPC分类号： C10L1/234 , C08K5/17
CPC分类号： C10L1/10 , C10L1/125 , C10L1/1608 , C10L1/1616 , C10L1/1641 , C10L1/1824 , C10L1/1826 , C10L1/1855 , C10L1/1857 , C10L1/1885 , C10L1/1886 , C10L1/1888 , C10L1/19 , C10L1/1963 , C10L1/1966 , C10L1/1973 , C10L1/198 , C10L1/1981 , C10L1/1985 , C10L1/2225 , C10L1/2335 , C10L10/16 , C10M169/044 , C10M173/02 , C10M2205/02 , C10M2205/022 , C10M2205/028 , C10M2207/021 , C10M2207/022 , C10M2207/08 , C10M2207/16 , C10M2207/18 , C10M2207/20 , C10M2207/281 , C10M2209/101 , C10M2209/103 , C10N2220/023 , C10N2230/04 , C10N2230/08 , C10N2250/12 , C10M2209/062 , C10M2209/084 , C10M2209/08
摘要： The invention relates to dispersions comprising I) at least one polymer that is effective for mineral oils as a cold extrusion improver and is soluble in oil, II) at least one organic solvent that cannot be mixed with water, III) water, IV) at least one alkanolamine salt of a polycyclic carboxylic acid as a dispersing agent, and V) possibly at least one organic solvent that can be mixed with water.
摘要翻译：本发明涉及分散体，其包括I）至少一种对矿物油作为冷挤出改进剂有效并且可溶于油的聚合物，II）至少一种不能与水混合的有机溶剂，III）水，IV）在作为分散剂的多环羧酸的至少一种链烷醇胺盐，以及V）可能与水混合的至少一种有机溶剂。

9. 发明授权

US5391632A Terpolymers based on .alpha.,.beta.-unsaturated dicarboxylic anhydrides, .alpha.,.beta.-unsaturated compounds and polyoxyalkylene ethers of lower unsaturated alcohols 失效
标题翻译：基于α，β-不饱和二羧酸酐，α，β-不饱和化合物和低级不饱和醇的聚氧化烯醚的三元共聚物
公开(公告)号：US5391632A
公开(公告)日：1995-02-21
申请号：US177906
申请日：1994-01-06
申请人： Matthias Krull , Michael Feustel
发明人： Matthias Krull , Michael Feustel
IPC分类号： C08F222/04 , C08F8/32 , C08F20/10 , C08F20/52 , C08F210/14 , C08F216/14 , C08F220/04 , C08F222/00 , C08F222/10 , C08F222/38 , C08F222/40 , C08L23/08 , C08L35/00 , C08L67/00 , C10L1/14 , C10L1/18 , C10L1/196 , C10L1/197 , C10L1/198 , C10L1/22 , C10L1/236 , C10M145/10 , C10M145/16 , C10M149/06 , C10M157/00 , C10M157/04
CPC分类号： C10M157/04 , C08F222/00 , C08F8/32 , C08L23/0853 , C10L1/143 , C10L1/146 , C10L1/1966 , C10L1/1973 , C10L1/1985 , C10L1/2364 , C10M145/16 , C10M149/06 , C10M157/00 , C08L67/00 , C10L1/192 , C10L1/195 , C10L1/1963 , C10L1/2222 , C10L1/2225 , C10L1/238 , C10L1/2387 , C10M2209/04 , C10M2209/06 , C10M2209/062 , C10M2209/086 , C10M2217/024 , C10M2217/06
摘要： Terpolymers based on .alpha.,.beta.-unsaturated dicarboxylic anhydrides, .alpha.,.beta.-unsaturated compounds and polyoxyalkylene ethers of lower unsaturated alcohols.The present invention relates to terpolymers based on .alpha.,.beta.-unsaturated dicarboxylic anhydrides, .alpha.,.beta.-unsaturated compounds and polyoxyalkylene ethers as defined in claim 1, and also a process for preparing the same as defined in claim 5.The invention likewise relates to a mixture of at least one terpolymer as defined in claim 1 and at least one ethylene-vinyl ester copolymer.The terpolymers of the invention, and mixtures thereof, are used as paraffin inhibitors in crude oils and petroleum products.
摘要翻译：基于α，β-不饱和二羧酸酐，α，β-不饱和化合物和低级不饱和醇的聚氧化烯醚的三元共聚物。本发明涉及基于如权利要求1所定义的α，β-不饱和二羧酸酐，α，β-不饱和化合物和聚氧化烯醚的三元共聚物，以及其权利要求5中定义的制备方法。本发明同样涉及如权利要求1所述的至少一种三元共聚物和至少一种乙烯 - 乙烯基酯共聚物的混合物。本发明的三元共聚物及其混合物用作原油和石油产品中的石蜡抑制剂。

10. 发明授权

US09029160B2 Method for determining the content of hydrogen sulfide in crude and residual oils 有权
标题翻译：测定原油和残余油中硫化氢含量的方法
公开(公告)号：US09029160B2
公开(公告)日：2015-05-12
申请号：US14001325
申请日：2012-02-14
申请人： Michael Feustel , Michael Brauchle , Dominko Andrin , Matthias Krull
发明人： Michael Feustel , Michael Brauchle , Dominko Andrin , Matthias Krull
IPC分类号： G01N33/28 , C10G21/14
CPC分类号： G01N33/287 , C10G21/14 , C10G2300/1033 , C10G2300/1048 , C10G2300/202 , C10G2300/207 , C10G2300/4006 , C10G2300/44 , G01N33/28 , Y10T436/182 , Y10T436/184
摘要： The subject of the invention is a method for determining the H2S content arising during the warm storage of sulfur-containing crude and residual oils and mineral distillates containing sulfur-containing crude and/or residual oils, in which a sample of the sulfur-containing mineral oil is dissolved in a solvent or solvent mixture that boils at more than 200° C. and a carrier gas is caused to flow through the solution of the sulfur-containing mineral oil at temperatures above 80° C., and the quantity of hydrogen sulfide carried out with the carrier gas is analyzed quantitatively.
摘要翻译：本发明的主题是确定在含硫含粗油和/或残余油的含硫原油和残余油和矿物馏出物的热储存期间产生的H 2 S含量的方法，其中含硫矿物样品油溶解在沸点高于200℃的溶剂或溶剂混合物中，并使载气在高于80℃的温度下流过含硫矿物油的溶液，并且硫化氢的量对载气进行定量分析。

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