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1. 发明授权

US08389670B2 Dithienobenzo-thieno[3,2-B]thiophene-copolymer and its use as high performance solution processable semiconducting polymer 有权
公开(公告)号：US08389670B2
公开(公告)日：2013-03-05
申请号：US13511890
申请日：2010-11-29
申请人： Marcel Kastler , Silke Annika Koehler , Klaus Muellen , Ralph Rieger
发明人： Marcel Kastler , Silke Annika Koehler , Klaus Muellen , Ralph Rieger
IPC分类号： C08G75/00
CPC分类号： H01L51/0043 , C08G61/126 , C08G2261/124 , C08G2261/3223 , C08G2261/3243 , C08G2261/414 , C08G2261/92 , H01L51/0036 , H01L51/0558 , Y02E10/549
摘要： Dithienobenzo-thieno[3,2-b]thiophene-copolymers of the formula (I) wherein: pi is a monocyclic or polycyclic moiety optionally substituted with 1-4 Ra groups, wherein Ra, at each occurrence, is independently hydrogen or a) a halogen, b) —(CN, c) —NO2, d) oxo, e) —OH, f) ═C(Rb)2; g) a C1-20 alkyl group, h) a C2-20 alkenyl group, i) a C2-20 alkynyl group, j) a C1-20 alkoxy group, k) a C1-20 alkylthio group, l) a C1-20 haloalkyl group, m) a —Y—C3-10 cycloalkyl group, n) a —Y—C6-14 aryl group, o) a —Y-3-12 membered cycloheteroalkyl group, or p) a —Y-5-14 membered heteroaryl group, wherein each of the C1-20 alkyl group, the C2-20 alkenyl group, the C2-20 alkynyl group, the C3-10 cycloalkyl group, the C6-14 aryl or haloaryl group, the 3-12 membered cycloheteroalkyl group, and the 5-14 membered heteroaryl group is optionally substituted with 1-4 Rb groups; Y, at each occurrence, is independently a divalent C1-6 alkyl group, a divalent C1-6 haloalkyl group, or a covalent bond; and R1, R2, R3, at each occurrence, are independently H, a halogen, CN, a C1-30 alkyl group, a C2-30 alkenyl group, a C1-30 haloalkyl group, a C2-30 alkynyl group, a C1-30 alkoxy group, a C(O)—C1-20 alkyl group, a C(O)—OC1-20 alkyl group, a Y—C3-10 cycloalkyl group, a —Y-3-12 membered cycloheteroalkyl group, each optionally substituted with 1-5 substituents selected from a halogen, —CN, a C1-6 alkyl group, a C1-6 alkoxy group, and a C1-6 haloalkyl group, -L-Ar1, -L-Ar1—Ar1, -L-Ar1—R4, or -L-Ar1—Ar1—R4 and Y, at each occurrence, is independently a divalent C1-6 alkyl group, a divalent C1-6 haloalkyl group, or a covalent bond; n=0, 1, 2; and o=1-1000.

2. 发明申请

US20120289672A1 DITHIENOBENZO-THIENO[3,2-B]THIOPHENE-COPOLYMER AND ITS USE AS HIGH PERFORMANCE SOLUTION PROCESSABLE SEMICONDUCTING POLYMER 有权
公开(公告)号：US20120289672A1
公开(公告)日：2012-11-15
申请号：US13511890
申请日：2010-11-29
申请人： Marcel Kastler , Silke Annika Koehler , Klaus Muellen , Ralph Rieger
发明人： Marcel Kastler , Silke Annika Koehler , Klaus Muellen , Ralph Rieger
IPC分类号： C08G75/00 , H01L51/40 , H01B1/12
CPC分类号： H01L51/0043 , C08G61/126 , C08G2261/124 , C08G2261/3223 , C08G2261/3243 , C08G2261/414 , C08G2261/92 , H01L51/0036 , H01L51/0558 , Y02E10/549
摘要： Dithienobenzo-thieno[3,2-b]thiophene-copolymers of the formula (I) wherein: pi is a monocyclic or polycyclic moiety optionally substituted with 1-4 Ra groups, wherein Ra, at each occurrence, is independently hydrogen or a) a halogen, b) —(CN, c) —NO2, d) oxo, e) —OH, f) ═C(Rb)2; g) a C1-20 alkyl group, h) a C2-20 alkenyl group, i) a C2-20 alkynyl group, j) a C1-20 alkoxy group, k) a C1-20 alkylthio group, l) a C1-20 haloalkyl group, m) a —Y—C3-10 cycloalkyl group, n) a —Y—C6-14 aryl group, o) a —Y-3-12 membered cycloheteroalkyl group, or p) a —Y-5-14 membered heteroaryl group, wherein each of the C1-20 alkyl group, the C2-20 alkenyl group, the C2-20 alkynyl group, the C3-10 cycloalkyl group, the C6-14 aryl or haloaryl group, the 3-12 membered cycloheteroalkyl group, and the 5-14 membered heteroaryl group is optionally substituted with 1-4 Rb groups; Y, at each occurrence, is independently a divalent C1-6 alkyl group, a divalent C1-6 haloalkyl group, or a covalent bond; and R1, R2, R3, at each occurrence, are independently H, a halogen, CN, a C1-30 alkyl group, a C2-30 alkenyl group, a C1-30 haloalkyl group, a C2-30 alkynyl group, a C1-30 alkoxy group, a C(O)—C1-20 alkyl group, a C(O)—OC1-20 alkyl group, a Y—C3-10 cycloalkyl group, a —Y-3-12 membered cycloheteroalkyl group, each optionally substituted with 1-5 substituents selected from a halogen, —CN, a C1-6 alkyl group, a C1-6 alkoxy group, and a C1-6 haloalkyl group, -L-Ar1, -L-Ar1-—Ar1, -L-Ar1—R4, or -L-Ar1—Ar1—R4 and Y, at each occurrence, is independently a divalent C1-6 alkyl group, a divalent C1-6 haloalkyl group, or a covalent bond; n=0, 1, 2; and o=1-1000.

3. 发明申请

US20110168264A1 POLY(5,5'-BIS(THIOPHEN-2-YL)-BENZO[2,1-B;3,4-B']DITHIOPHENE) AND ITS USE AS HIGH PERFORMANCE SOLUTION PROCESSABLE SEMICONDUCTING POLYMER 有权
标题翻译： POLY（5,5'-双（噻吩-2-基） - 苯并[2,1-B; 3,4-B']二苯基），并且可用作高性能溶液可处理的半导体聚合物
公开(公告)号：US20110168264A1
公开(公告)日：2011-07-14
申请号：US13002392
申请日：2009-06-25
申请人： Marcel Kastler , Silke Koehler , Klaus Muellen , Miaoyin Liu , Dirk Beckmann , Ralph Rieger
发明人： Marcel Kastler , Silke Koehler , Klaus Muellen , Miaoyin Liu , Dirk Beckmann , Ralph Rieger
IPC分类号： H01L51/46 , H01L51/30 , H01L51/54 , C08G75/06 , C08L81/02
CPC分类号： H01L51/0036 , C07D495/04 , C08G61/126 , H01B1/127 , H01L51/0043 , H01L51/0074 , H01L51/0541 , H01L51/0545 , Y02E10/549
摘要： Poly(5,5′-bis(thiophen-2-yl)-benzo[2,1-b;3,4-b′]dithiophene) comprising as repeating units the group of the formula (I) wherein R is independently selected from a) a C1-2O alkyl group, b) a C2-20 alkenyl group, c) a C2-20 alkynyl group, d) a C1-20 alkoxy group, e) a —Y—C3-10 cycloalkyl group, f) a —Y—C6-14 aryl group, g) a —Y-3-12 membered cycloheteroalkyl group, or h) a —Y-5-14 membered het-eroaryl group, wherein each of the C1-20 alkyl group, the C2-20 alkenyl group, the C2-20 alkynyl group, the C3-10 cycloalkyl group, the C6-14 aryl group, the 3-12 membered cycloheteroalkyl group, and the 5-14 membered heteroaryl group is optionally substituted with 1-4 R1 groups, R1 is independently selected from a) a S(O)m—C1-20 alkyl group, b) a S(O)m—OC1-20 alkyl group, c) a S(O)m—OC6-14 aryl group, d) a C(O)—OC1-20 alkyl group, e) a C(O)—OC6-14 aryl group, f) a C1-20 alkyl group, g) a C2-20 alkenyl group, h) a C2-20 alkynyl group, i) a C1-20 alkoxy group, j) a C3-10 cycloalkyl group, k) a C6-14 aryl group, I) a 3-12 membered cycloheteroalkyl group, or m) a 5-14 membered heteroaryl group, Y is independently selected from a divalent C1-6 alkyl group, or a covalent bond; and m is independently selected from 0, 1, or 2, and having a number average molecular weight Mn in the range of from 5,000 to 200,000 g/mol.
摘要翻译：包括作为重复单元的式（I）基团，其中R独立地被选择的聚（5,5'-双（噻吩-2-基） - 苯并[2,1-b; 3,4-b']二噻吩）从a）C1-2O烷基，b）C2-20烯基，c）C2-20炔基，d）C1-20烷氧基，e）-Y-C3-10环烷基，f ）a -Y-C 6-14芳基，g）-Y-3-12元环杂烷基，或h）-Y-5-14元环芳基，其中每个C 1-20烷基， C2-20烯基，C2-20炔基，C3-10环烷基，C6-14芳基，3-12元环杂烷基和5-14元杂芳基任选被1- 4个R 1基团，R 1独立地选自a）S（O）m -C 1-20烷基，b）S（O）m OC 1-7-20烷基，c）S（O）m OC 1-6 - 14芳基，d）C（O）-OC1-20烷基，e）C（O）-OC6-14芳基，f）C1-20烷基，g）C2-20烯基， h）C 20-20炔基，i）C 1-20烷氧基，j）C 3-10环烷基烷叉基，k）C 6-14芳基，I）3-12元环杂烷基或m）5-14元杂芳基，Y独立地选自二价C 1-6烷基或共价键 ; m独立地选自0,1或2，数均分子量Mn在5,000至200,000g / mol的范围内。

4. 发明授权

US08598304B2 Poly(5,5′bis(thiophen-2-yl)-benzo[2,1-b;3,4-b′]dithiophene) and its use as high performance solution processable semiconducting polymer 有权
标题翻译：聚（5,5'-双（噻吩-2-基） - 苯并[2,1-b; 3,4-b']二噻吩）及其作为高性能溶液可加工半导体聚合物
公开(公告)号：US08598304B2
公开(公告)日：2013-12-03
申请号：US13002392
申请日：2009-06-25
申请人： Marcel Kastler , Silke Koehler , Klaus Muellen , Miaoyin Liu , Dirk Beckmann , Ralph Rieger
发明人： Marcel Kastler , Silke Koehler , Klaus Muellen , Miaoyin Liu , Dirk Beckmann , Ralph Rieger
IPC分类号： C08G75/00
CPC分类号： H01L51/0036 , C07D495/04 , C08G61/126 , H01B1/127 , H01L51/0043 , H01L51/0074 , H01L51/0541 , H01L51/0545 , Y02E10/549
摘要： Poly(5,5′-bis(thiophen-2-yl)-benzo[2,1-b;3,4-b′]dithiophene) comprising as repeating units the group of the formula (I) wherein R is independently selected from a) a C1-20 alkyl group, b) a C2-20 alkenyl group, c) a C2-20 alkynyl group, d) a C1-20 alkoxy group, e) a —Y—C3-10 cycloalkyl group, f) a —Y—C6-14 aryl group, g) a —Y-3-12 membered cycloheteroalkyl group, or h) a —Y-5-14 membered heteroaryl group, wherein each of the C1-20 alkyl group, the C2-20 alkenyl group, the C2-20 alkynyl group, the C3-10 cycloalkyl group, the C6-14 aryl group, the 3-12 membered cycloheteroalkyl group, and the 5-14 membered heteroaryl group is optionally substituted with 1-4 R1 groups, R1 is independently selected from a) a S(O)m—C1-20 alkyl group, b) a S(O)m—OC1-20 alkyl group, c) a S(O)m—OC6-14 aryl group, d) a C(O)—OC1-20 alkyl group, e) a C(O)—OC6-14 aryl group, f) a C1-20 alkyl group, g) a C2-20 alkenyl group, h) a C2-20 alkynyl group, i) a C1-20 alkoxy group, j) a C3-10 cycloalkyl group, k) a C6-14 aryl group, l) a 3-12 membered cycloheteroalkyl group, or m) a 5-14 membered heteroaryl group, Y is independently selected from a divalent C1-6 alkyl group, or a covalent bond; and m is independently selected from 0, 1, or 2, and having a number average molecular weight Mn in the range of from 5,000 to 200,000 g/mol.
摘要翻译：包括作为重复单元的式（I）基团，其中R独立地被选择的聚（5,5'-双（噻吩-2-基） - 苯并[2,1-b; 3,4-b']二噻吩）从a）C 1-20烷基，b）C 2-20烯基，c）C 2-20炔基，d）C 1-20烷氧基，e）-Y-C 3-10环烷基，f ）-Y-C 6-14芳基，g）a -Y-3-12元环杂烷基，或h）-Y-5-14元杂芳基，其中C 1-20烷基，C 2 -20链烯基，C2-20炔基，C3-10环烷基，C6-14芳基，3-12元环杂烷基和5-14元杂芳基任选被1-4个R1 基团，R 1独立地选自a）S（O）m -C 1-20烷基，b）S（O）m OC 1-7-20烷基，c）S（O）m -C 0-6-14芳基基团，d）C（O）-OC 1-20烷基，e）C（O）-OC 6-14芳基，f）C 1-20烷基，g）C 2-20烯基，h） C 20-20炔基，i）C 1-20烷氧基，j）C 3-10环烷基，k）C 6-14 芳基，l）3-12元环杂烷基，或m）5-14元杂芳基，Y独立地选自二价C 1-6烷基或共价键; m独立地选自0,1或2，数均分子量Mn在5,000至200,000g / mol的范围内。

5. 发明授权

US08853820B2 Crosslinkable dielectrics and methods of preparation and use thereof 有权
标题翻译：可交联电介质及其制备方法及用途
公开(公告)号：US08853820B2
公开(公告)日：2014-10-07
申请号：US13322252
申请日：2010-05-20
申请人： Marcel Kastler , Silke Annika Koehler
发明人： Marcel Kastler , Silke Annika Koehler
IPC分类号： H01L29/78 , H01L51/30 , H01L51/05 , H01L23/498 , H01G4/18 , H01G4/33
CPC分类号： H01L51/052 , H01G4/18 , H01G4/33 , H01L23/49894 , H01L51/0043 , H01L51/0545 , H01L2251/308 , H01L2924/0002 , H01L2924/00
摘要： The present invention relates to an electronic device comprising at least one dielectric layer, said dielectric layer comprising a crosslinked organic compound based on at least one compound which is radically crosslinkable and a method of making the electronic device.
摘要翻译：本发明涉及包含至少一个电介质层的电子器件，所述电介质层包含基于至少一种可自由交联的化合物的交联有机化合物和制备该电子器件的方法。

6. 发明授权

US08404844B2 Perylene semiconductors and methods of preparation and use thereof 有权
标题翻译：苝半导体及其制备方法及用途
公开(公告)号：US08404844B2
公开(公告)日：2013-03-26
申请号：US12866331
申请日：2009-02-05
申请人： Marcel Kastler , Subramanian Vaidyanathan , Florian Doetz , Silke Annika Koehler , He Yan , Antonio Facchetti , Shaofeng Lu , Yan Zheng
发明人： Marcel Kastler , Subramanian Vaidyanathan , Florian Doetz , Silke Annika Koehler , He Yan , Antonio Facchetti , Shaofeng Lu , Yan Zheng
IPC分类号： C07D471/08 , H01L51/50 , H01L29/02
CPC分类号： C07D471/06 , C09B5/62 , H01L51/0053 , H01L51/0541 , H01L51/0545 , H01L51/42 , Y02E10/549 , Y02P70/521
摘要： The present invention relates to semiconducting compounds, materials prepared from such compounds, methods of preparing such compounds and semiconductor materials, as well as various compositions, composites, and devices that incorporate the compounds and semiconductor materials. The semiconducting compounds can have higher electron-transport efficiency and higher solubility in common solvents compared to related representative compounds.
摘要翻译：本发明涉及半导体化合物，由这些化合物制备的材料，制备这种化合物和半导体材料的方法，以及掺入化合物和半导体材料的各种组合物，复合材料和器件。与相关的代表性化合物相比，半导体化合物可以具有较高的电子传输效率和较高的溶解度。

7. 发明授权

US09219233B2 Semiconductor materials prepared from rylene-(π-acceptor)copolymers 有权
标题翻译：由Rylene - （＆amp;受体）共聚物制备的半导体材料
公开(公告)号：US09219233B2
公开(公告)日：2015-12-22
申请号：US12865031
申请日：2009-02-05
申请人： Antonio Facchetti , Zhihua Chen , He Yan , Shaofeng Lu , Tobin J. Marks , Yan Zheng , Marcel Kastler , Subramanian Vaidyanathan , Florian Doetz , Silke Annika Koehler
发明人： Antonio Facchetti , Zhihua Chen , He Yan , Shaofeng Lu , Tobin J. Marks , Yan Zheng , Marcel Kastler , Subramanian Vaidyanathan , Florian Doetz , Silke Annika Koehler
IPC分类号： H01L51/46 , H01B1/12 , C08G61/12 , C08G61/10 , H05B33/14 , C09K11/06 , H01L51/00 , H01L51/05
CPC分类号： H01L51/0043 , C08G61/10 , C08G61/12 , C09B5/62 , C09B69/102 , C09B69/105 , C09B69/106 , C09K11/06 , C09K2211/1458 , C09K2211/1483 , H01B1/127 , H01L51/0036 , H01L51/0053 , H01L51/0094 , H01L51/0541 , H01L51/0545 , H05B33/14 , Y02E10/549 , Y02P70/521
摘要： Disclosed are new semiconductor materials prepared from rylene-(π-acceptor) copolymers. Such copolymers can exhibit high n-type carrier mobility and/or good current modulation characteristics. In addition, the polymers of the present teachings can possess certain processing advantages such as solution-processability and/or good stability at ambient conditions.
摘要翻译：公开了由二烯 - （＆amp;受体）共聚物制备的新的半导体材料。这种共聚物可表现出高的n型载流子迁移率和/或良好的电流调制特性。此外，本教导的聚合物可以具有某些加工优点，例如在环境条件下的溶液加工性和/或良好的稳定性。

8. 发明申请

US20120068314A1 CROSSLINKABLE DIELECTRICS AND METHODS OF PREPARATION AND USE THEREOF 有权
标题翻译：可交换电介质及其制备和使用方法
公开(公告)号：US20120068314A1
公开(公告)日：2012-03-22
申请号：US13322252
申请日：2010-05-20
申请人： Marcel Kastler , Silke Annika Koehler
发明人： Marcel Kastler , Silke Annika Koehler
IPC分类号： H01L29/00 , C08F222/20 , C08F222/22 , C08F230/08 , C08F220/40 , C08L67/08 , C08G63/91 , C08F299/00 , C08L53/00 , C08L43/04 , C08L35/02 , C08L33/06 , C08F222/14 , C08F236/10
CPC分类号： H01L51/052 , H01G4/18 , H01G4/33 , H01L23/49894 , H01L51/0043 , H01L51/0545 , H01L2251/308 , H01L2924/0002 , H01L2924/00
摘要： The present invention relates to an electronic device comprising at least one dielectric layer, said dielectric layer comprising a crosslinked organic compound based on at least one compound which is radically crosslinkable and a method of making the electronic device.
摘要翻译：本发明涉及包含至少一个电介质层的电子器件，所述电介质层包含基于至少一种可自由交联的化合物的交联有机化合物和制备该电子器件的方法。

9. 发明申请

US20110120558A1 SEMICONDUCTOR MATERIALS PREPARED FROM RYLENE-(PI-ACCEPTOR)COPOLYMERS 有权
标题翻译：由RYLENE（PI-ACCEPTOR）共聚物制备的半导体材料
公开(公告)号：US20110120558A1
公开(公告)日：2011-05-26
申请号：US12865031
申请日：2009-02-05
申请人： Antonio Facchetti , Zhihua Chen , He Yan , Shaofeng Lu , Tobin J. Marks , Yan Zheng , Marcel Kastler , Subramanian Vaidyanathan , Florian Doetz , Silke Annika Koehler
发明人： Antonio Facchetti , Zhihua Chen , He Yan , Shaofeng Lu , Tobin J. Marks , Yan Zheng , Marcel Kastler , Subramanian Vaidyanathan , Florian Doetz , Silke Annika Koehler
IPC分类号： H01L51/46 , C08F228/06 , H01B1/12 , C08F26/06 , H01L51/30 , H01L51/54 , H01L51/40 , H01L51/48 , H01L51/56
CPC分类号： H01L51/0043 , C08G61/10 , C08G61/12 , C09B5/62 , C09B69/102 , C09B69/105 , C09B69/106 , C09K11/06 , C09K2211/1458 , C09K2211/1483 , H01B1/127 , H01L51/0036 , H01L51/0053 , H01L51/0094 , H01L51/0541 , H01L51/0545 , H05B33/14 , Y02E10/549 , Y02P70/521
摘要： Disclosed are new semiconductor materials prepared from rylene-(π-acceptor) copolymers. Such copolymers can exhibit high n-type carrier mobility and/or good current modulation characteristics. In addition, the polymers of the present teachings can possess certain processing advantages such as solution-processability and/or good stability at ambient conditions.
摘要翻译：公开了由二烯 - （＆amp;受体）共聚物制备的新的半导体材料。这种共聚物可表现出高的n型载流子迁移率和/或良好的电流调制特性。此外，本教导的聚合物可以具有某些加工优点，例如在环境条件下的溶液加工性和/或良好的稳定性。

10. 发明申请

US20100319778A1 PERYLENE SEMICONDUCTORS AND METHODS OF PREPARATION AND USE THEREOF 有权
标题翻译： PERYLENE SEMICONDUCTORS及其制备和使用方法
公开(公告)号：US20100319778A1
公开(公告)日：2010-12-23
申请号：US12866331
申请日：2009-02-05
申请人： Marcel Kastler , Subramanian Vaidyanathan , Florian Doetz , Silke Annika Koehler , He Yan , Antonio Facchetti , Shaofeng Lu , Yan Zheng
发明人： Marcel Kastler , Subramanian Vaidyanathan , Florian Doetz , Silke Annika Koehler , He Yan , Antonio Facchetti , Shaofeng Lu , Yan Zheng
IPC分类号： H01L51/46 , C07D471/06 , H01L51/30 , H01L51/40
CPC分类号： C07D471/06 , C09B5/62 , H01L51/0053 , H01L51/0541 , H01L51/0545 , H01L51/42 , Y02E10/549 , Y02P70/521
摘要： The present teachings provide semiconducting compounds, materials prepared from such compounds, methods of preparing such compounds and semiconductor materials, as well as various compositions, composites, and devices that incorporate the compounds and semiconductor materials. Specifically, compounds of the present teachings can have higher electron-transport efficiency and higher solubility in common solvents compared to related representative compounds.
摘要翻译：本发明提供半导体化合物，由这些化合物制备的材料，制备这种化合物和半导体材料的方法，以及掺入化合物和半导体材料的各种组合物，复合材料和器件。具体而言，与相关的代表性化合物相比，本发明的化合物可具有较高的电子传输效率和较高的溶解度。

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