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1. 发明申请

US20100121009A1 CATALYST SYSTEM FOR OLEFIN POLYMERIZATION PROCESS FOR PRODUCING IT AND A PROCESS FOR THE POLYMERIZATION OF ALPHA-OLEFINS USING THE CATALYST SYSTEM 审中-公开
标题翻译：用于生产烯烃聚合方法的催化剂体系和使用催化剂体系合成α-烯烃的方法
公开(公告)号：US20100121009A1
公开(公告)日：2010-05-13
申请号：US12451207
申请日：2008-05-05
申请人： Marc Oliver Kristen , Rolf Mülhaupt , Gil Scheuermann , Alexander Kurek
发明人： Marc Oliver Kristen , Rolf Mülhaupt , Gil Scheuermann , Alexander Kurek
IPC分类号： C08F4/12 , B01J37/30
CPC分类号： C08F10/00 , C08F110/02 , C08F4/7006 , C08F4/69034 , C08F4/025 , C08F2500/20 , C08F2500/04 , C08F4/69224
摘要： The invention relates to a catalyst system comprising a support in which transition metal cations or uncharged transition metal atoms are distributed. The system further comprises one or more separately added ligands which are capable of forming a coordinate or covalent bond with the transition metals. The catalyst system is produced by replacing metal ions present in a support by transition metal ions. The transition metal ions can optionally be reduced. One or more ligands which are capable of forming a coordinate or covalent bond with the transition metal or metals are subsequently added. The catalyst is used for the polymerization of olefins.
摘要翻译：本发明涉及一种催化剂体系，其包括其中分布有过渡金属阳离子或不带电过渡金属原子的载体。该体系还包含一个或多个单独添加的能够与过渡金属形成配位或共价键的配体。通过用过渡金属离子代替载体中存在的金属离子来制备催化剂体系。可以任选地还原过渡金属离子。随后加入能够与过渡金属或金属形成配位或共价键的一个或多个配位体。该催化剂用于烯烃的聚合。

2. 发明申请

US20100190931A1 CATALYST SYSTEM FOR POLYMERIZATION OF OLEFINIC MONOMERS, PROCESS FOR PREPARING POLYMERS, AND POLYMERS PREPARED BY THE PROCESS 失效
标题翻译：烯烃单体聚合催化剂体系，制备聚合物的方法和工艺制备的聚合物
公开(公告)号：US20100190931A1
公开(公告)日：2010-07-29
申请号：US12452713
申请日：2008-07-22
申请人： Marc Oliver Kristen , Rolf Mülhaupt , Georg Müller
发明人： Marc Oliver Kristen , Rolf Mülhaupt , Georg Müller
IPC分类号： C08F4/64 , C08L23/06 , B32B5/02 , B01J32/00 , B01J31/14 , B01J31/06
CPC分类号： C08F10/00 , C08F4/65925 , Y10S526/943 , Y10T428/249924 , C08F4/027
摘要： The present invention relates to new catalyst supports comprising nanofibers, a catalyst system comprising these supports as well as a process for preparing nanocomposites and the nanocomposites prepared. The invention especially concerns a supported catalyst system for polymerization of olefins, comprising a support made of fibers or a fleece of fibers, wherein the mean fiber diameter is less than 1000 nm, preferably less than 500 nm and the mean fiber length is more than 200,000 nm, preferably more than 500,000 nm and especially preferred more than 1,000,000 nm as well as a process for polymerizing olefinic systems in the presence of these catalyst systems and the resulting nanocomposites.
摘要翻译：本发明涉及包含纳米纤维的新催化剂载体，包含这些载体的催化剂体系以及制备纳米复合材料的方法和制备的纳米复合材料。本发明特别涉及用于烯烃聚合的负载型催化剂体系，其包括由纤维制成的载体或纤维的绒毛，其中平均纤维直径小于1000nm，优选小于500nm，平均纤维长度大于20万 nm，优选大于500,000nm，特别优选大于1,000,000nm，以及在这些催化剂体系存在下聚合烯属体系的方法和所得的纳米复合材料。

3. 发明申请

US20120328502A1 Preparation of Metal Oxide Nanotubes 审中-公开
标题翻译：金属氧化物纳米管的制备
公开(公告)号：US20120328502A1
公开(公告)日：2012-12-27
申请号：US13516693
申请日：2010-12-16
申请人： Georg Müller , Rolf Mülhaupt , Marc Oliver Kristen
发明人： Georg Müller , Rolf Mülhaupt , Marc Oliver Kristen
IPC分类号： C01B33/12 , C08F16/06 , B82Y40/00 , B82Y30/00
CPC分类号： D01F9/10 , B01J21/08 , B01J35/06 , B01J37/0018 , B82Y30/00 , B82Y40/00 , C01B33/18 , C04B35/62807 , C04B35/63416 , C04B2235/3418 , C04B2235/444 , C04B2235/5264 , C04B2235/5284 , C04B2235/5409 , C04B2235/6028 , D01D5/24
摘要： The present invention relates to a preparation process for metal oxide nanotubes, the SiO2 nanotubes prepared by this process and the use of these nanotubes as catalyst supports. The invention especially concerns a supported catalyst system for polymerization of olefins, comprising a support made of fibers or a fleece of fibers.
摘要翻译：本发明涉及金属氧化物纳米管的制备方法，通过该方法制备的SiO 2纳米管和这些纳米管作为催化剂载体的用途。本发明特别涉及用于烯烃聚合的负载催化剂体系，其包括由纤维制成的载体或纤维的绒毛。

4. 发明授权

US08133832B2 Catalyst system for polymerization of olefinic monomers, process for preparing polymers, and polymers prepared by the process 失效
标题翻译：用于聚合烯烃单体的催化剂体系，制备聚合物的方法和通过该方法制备的聚合物
公开(公告)号：US08133832B2
公开(公告)日：2012-03-13
申请号：US12452713
申请日：2008-07-22
申请人： Marc Oliver Kristen , Rolf Mülhaupt , Georg Müller
发明人： Marc Oliver Kristen , Rolf Mülhaupt , Georg Müller
IPC分类号： C08F4/02 , C08F4/642 , C08F4/6592
CPC分类号： C08F10/00 , C08F4/65925 , Y10S526/943 , Y10T428/249924 , C08F4/027
摘要： The present invention relates to new catalyst supports comprising nanofibers, a catalyst system comprising these supports as well as a process for preparing nanocomposites and the nanocomposites prepared. The invention especially concerns a supported catalyst system for polymerization of olefins, comprising a support made of fibers or a fleece of fibers, wherein the mean fiber diameter is less than 1000 nm, preferably less than 500 nm and the mean fiber length is more than 200,000 nm, preferably more than 500,000 nm and especially preferred more than 1,000,000 nm as well as a process for polymerizing olefinic systems in the presence of these catalyst systems and the resulting nanocomposites.
摘要翻译：本发明涉及包含纳米纤维的新催化剂载体，包含这些载体的催化剂体系以及制备纳米复合材料的方法和制备的纳米复合材料。本发明特别涉及用于烯烃聚合的负载型催化剂体系，其包括由纤维制成的载体或纤维的绒毛，其中平均纤维直径小于1000nm，优选小于500nm，平均纤维长度大于20万 nm，优选大于500,000nm，特别优选大于1,000,000nm，以及在这些催化剂体系存在下聚合烯属体系的方法和所得的纳米复合材料。

5. 发明授权

US07129292B1 Method for the emulsion polymerization of olefins 失效
标题翻译：烯烃乳液聚合方法
公开(公告)号：US07129292B1
公开(公告)日：2006-10-31
申请号：US10168113
申请日：2000-10-18
申请人： Marc Oliver Kristen , Lambertus Manders , Stefan Mecking , Florian M. Bauers , Rolf Mülhaupt
发明人： Marc Oliver Kristen , Lambertus Manders , Stefan Mecking , Florian M. Bauers , Rolf Mülhaupt
IPC分类号： C08F2/16
CPC分类号： C08F10/02 , C08F10/00 , C08F2/22 , C08F4/80 , C08F4/7006 , C08F4/7031 , C08F4/7022 , C08F4/7027 , C08F4/7019
摘要： A process for emulsion polymerizing one or more olefins involves reacting it/them with at least one complex compound of the formula Ia or b where M is a transition metal from groups 7 to 10 of the Periodic Table of the Elements and is preferably Ni in aqueous dispersion and at least one radical R1 to R3 and optionally one radical R4 to R9 contains a hydrophilic group X, selection being made from —SO3−, —O—PO32−, NH(R15)2+, N(R15)3+ or —(OCH2CH2)nOH, where n is an integer between 1 and 15. For the process of the invention it is optional to use an activator such as, for example, olefin complexes of rhodium or of nickel. This invention further relates to dispersions of polyolefins such as polyethylene and ethylene copolymers in water, for example, and to the use of the aqueous dispersions of the invention for paper applications such as paper coating or surface sizing, paints, adhesive base materials, molded foams such as mattresses, textile and leather applications, carpet back coatings, or pharmaceutical applications.
摘要翻译：用于将一种或多种烯烃乳液聚合的方法涉及使其与至少一种式Ia或b的络合物反应，其中M是元素周期表第7至10族的过渡金属，并且优选为Ni 分散体和至少一个R 1至R 3基团和任选的一个基团R 4至R 9包含一个亲水基团X，选自-SO 3 - ， - O-PO 3 - ， - NH 2， - NH （R 15）2 N 2 O 3 N（R 15）3 或+ - 或 - （OCH 2 CH 2）n OH，其中n是1和15之间的整数。对于本发明的方法任选使用活化剂，例如铑或镍的烯烃络合物。本发明还涉及聚烯烃如聚乙烯和乙烯共聚物在水中的分散体，以及本发明的水性分散体用于纸张涂布或表面施胶，涂料，粘合剂基材，模塑泡沫例如床垫，纺织和皮革应用，地毯背部涂层或药物应用。

6. 发明授权

US06998269B2 Determination of the quality of polymerization catalysts 失效
标题翻译：聚合催化剂质量的测定
公开(公告)号：US06998269B2
公开(公告)日：2006-02-14
申请号：US10359239
申请日：2003-02-06
申请人： Marc Oliver Kristen , Peter Eibeck , Heike Gregorius , Dieter Lilge
发明人： Marc Oliver Kristen , Peter Eibeck , Heike Gregorius , Dieter Lilge
IPC分类号： G01N31/00
CPC分类号： C08F10/06 , B01J19/0046 , B01J2219/00722 , B01J2219/00738 , C08F4/65912 , C08F4/65916 , C08F110/06 , C40B40/14 , C08F4/65927
摘要： A method of determining the quality of polymerization catalysts comprises a) provision of the catalysts, b) polymerization of a monomer using these catalysts, c) isolation of the polymers obtained in b), d) characterization of the polymers, wherein the method is carried out in an assembly of n vessels in an essentially automated fashion, where the steps a) to d) are all carried out in parallel or are all carried out sequentially or some of the steps a) to d) are carried out in parallel and the remainder are carried out sequentially and n is a natural number greater than or equal to 2.
摘要翻译：确定聚合催化剂质量的方法

7. 发明授权

US06683018B1 Method for producing a supported catalyst system 失效
标题翻译：负载催化剂体系的制备方法
公开(公告)号：US06683018B1
公开(公告)日：2004-01-27
申请号：US09622211
申请日：2000-08-14
申请人： Marc Oliver Kristen , Laurent Deloux , Peter Kölle , Ulrich Moll , Ursula Rief
发明人： Marc Oliver Kristen , Laurent Deloux , Peter Kölle , Ulrich Moll , Ursula Rief
IPC分类号： B01J3100
CPC分类号： B01J31/1616 , B01J31/2295 , B01J37/0203 , B01J2531/48 , C08F4/61908 , C08F4/61912 , C08F10/00 , C08F210/16 , C08F4/61916 , C08F210/14 , C08F2500/17
摘要： A process for the preparation of a supported catalyst system, an inorganic carrier material being reacted with a metal compound of the formula M1(R1)r(R2)5(R3)t(R4)u I in the presence of an inert solvent in a first step and, in a subsequent step, the suspension thus obtained being reacted with a metallocene complex and a compound forming metallocenium ions, in which process the solvent is not removed after the first step and the subsequent step is carried out without isolation of the pretreated carrier material thus obtained.
摘要翻译：一种制备负载型催化剂体系的方法，无机载体材料与第一步惰性溶剂的存在下的金属化合物反应，在随后的步骤中，将由此获得的悬浮液与茂金属络合物和形成金属茂离子的化合物，其中在第一步骤之后不除去溶剂，并且在不分离由此获得的预处理载体材料的情况下进行随后的步骤。

8. 发明授权

US06359086B1 Non self-igniting solid 失效
标题翻译：非自燃固体
公开(公告)号：US06359086B1
公开(公告)日：2002-03-19
申请号：US09341517
申请日：1999-07-13
申请人： Marc Oliver Kristen , Patrik Müller , Ulrich Moll , Peter Kölle
发明人： Marc Oliver Kristen , Patrik Müller , Ulrich Moll , Peter Kölle
IPC分类号： C08F442
CPC分类号： B01J31/143 , B01D53/28 , B01J31/12 , B01J31/1616 , B01J31/165 , B01J31/2295 , B01J2531/48 , C08F4/65912 , C08F4/6592 , C08F10/00 , C08F110/02 , Y10S526/943 , C08F4/61916 , C08F2500/17
摘要： A free-flowing solid which does not self-ignite, comprising: a) at least one support component, b) at least one chemical compound which per se is self-igniting, c) at least one inert liquid and d) further components.
摘要翻译：一种不自燃的自由流动的固体，包括：a）至少一种载体组分，b）至少一种本身是自燃的化合物，c）至少一种惰性液体，和d）其它组分。

9. 发明授权

US06946568B2 Complexed compounds and use thereof for the polymerization of olefins 失效
标题翻译：复合化合物及其用于烯烃聚合的用途
公开(公告)号：US06946568B2
公开(公告)日：2005-09-20
申请号：US10467169
申请日：2002-02-06
申请人： Marc Oliver Kristen , Benno Bildstein , Alexander Krajete
发明人： Marc Oliver Kristen , Benno Bildstein , Alexander Krajete
IPC分类号： C07D215/14 , C07C251/24 , C07D207/335 , C07D213/30 , C07F7/00 , C07F9/00 , C08F4/62 , C08F4/625 , C08F4/76 , C08F10/00 , C08F10/02 , C08F110/02 , C08F210/16 , B01J31/00 , C08F4/44
CPC分类号： C08F10/02 , C07F7/003 , C07F9/005 , C08F10/00 , C08F110/02 , C08F210/16 , C08F2500/17 , C08F210/14 , C08F4/64048 , C08F4/6812
摘要： Complexes of the formulae Ia and Ib where M=Ti, Zr, Hf, V, Nb or Ta, can be used for the polymerization and copolymerization of olefins, for example in suspension polymerization processes, gas-phase polymerization processes and bulk polymerization processes.
摘要翻译：其中M = Ti，Zr，Hf，V，Nb或Ta的式Ia和Ib的络合物可用于烯烃的聚合和共聚，例如在悬浮聚合方法，气相聚合方法和本体聚合方法中。

10. 发明授权

US06812306B2 Metallic compounds and the use thereof in the polymerization of olefins 失效
标题翻译：金属化合物及其在烯烃聚合中的应用
公开(公告)号：US06812306B2
公开(公告)日：2004-11-02
申请号：US10312880
申请日：2003-01-02
申请人： Marc Oliver Kristen , Peter Hofmann , Frank Eisenträger
发明人： Marc Oliver Kristen , Peter Hofmann , Frank Eisenträger
IPC分类号： C08F480
CPC分类号： C08F110/02 , C07F15/006 , C07F15/04 , C08F10/00 , C08F4/80 , C08F2500/03 , C08F4/7016
摘要： Metal compounds of the formula I, where M is selected from among Ni and Pd in the oxidation state +II can be used for the polymerization or copolymerization of olefins. Supported catalysts for the polymerization and copolymerization of olefins can be obtained by application of one or more of the above-described ionic metal compounds to a support.
摘要翻译：式I的金属化合物，其中M选自氧化态+ II的Ni和Pd可用于烯烃的聚合或共聚。用于烯烃聚合和共聚的载体催化剂可以通过将一种或多种上述离子金属化合物应用于载体来获得。

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