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1. 发明申请

WO2017066586A1 BLOCK COPOLYMERS HAVING AMINE OR PHOSPHINE FUNCTIONALIZED END BLOCKS 审中-公开
标题翻译：具有胺或膦官能化封端的嵌段共聚物
公开(公告)号：WO2017066586A1
公开(公告)日：2017-04-20
申请号：PCT/US2016/057066
申请日：2016-10-14
申请人： KRATON POLYMERS U.S. LLC
发明人： VAN DER HUIZEN, Adrie, A. , WILLIS, Carl, L. , STOL, Marianne , MUYLDERMANS, Xavier, D.
IPC分类号： B01D71/82 , B01D61/44 , B01D65/10
CPC分类号： C08G81/022 , C08F297/04 , C08J5/18 , C08J2353/00
摘要： Disclosed herein is a functionalized block copolymer comprising (a) at least one end block D comprising on average at least one amino- or phosphino- functionalized polymer unit of formula (I) and one or more additional blocks selected from the group consisting of (b) one or more A blocks substantially free of amino- or phosphino- functional groups and having a number average molecular weight of from about 1,000 to about 60,000, and has a high service temperature, and (c) one or more B blocks, wherein each block B is essentially non-functionalized, has a number average molecular weight of from about 1,000 to about 1,000,000, and has a glass transition temperature of at most about 20°C, and (d) mixtures of one or more A blocks and one or more B blocks; wherein Z is nitrogen or phosphorus; R 1 is hydrogen or alkyl; R 2 is hydrogen or is tertiary alkyl; R each independently, is alkyl or phenyl optionally substituted by a moiety -(A 1 - NR a ) x R b or -(A 1 -OR a )xR b ; or two R groups, together with the Z to which they are bonded, form an optionally substituted ring; x is 1, 2 or 3; A 1 is straight chain alkylene optionally substituted by one or more methyl and/or ethyl groups; and R a and R b , each independently, is hydrogen or alkyl; or a corresponding onium salt.
摘要翻译：本文公开了一种官能化嵌段共聚物，其包含（a）至少一个末端嵌段D，其平均包含至少一个式（I）的氨基 - 或膦基 - 官能化聚合物单元和一个或多个另外的嵌段（b）基本上不含氨基或膦基官能团且数均分子量为约1,000至约60,000且具有高使用温度的一个或多个A嵌段，和（c）一个或多个B嵌段，其中每个嵌段B基本上未官能化，数均分子量为约1,000至约1,000,000，并且具有至多约20℃的玻璃化转变温度，和（d）一个或多个A块和一个或多个B块; 其中Z是氮或磷; R 1是氢或烷基; R 2是氢或是叔烷基; R各自独立地为烷基或苯基，所述苯基任选地被部分 - （A 1-NR 2）a -XR b -X- 或 - （A <1> -OR ）xR ; 或两个R基团与它们所键合的Z一起形成任选取代的环; x是1,2或3; A 1是任选被一个或多个甲基和/或乙基取代的直链亚烷基; 和R a和R b各自独立地是氢或烷基; 或相应的鎓盐。

2. 发明申请

WO2015153747A1 BLOCK COPOLYMERS CONTAINING A COPOLYMER MYRCENE BLOCK 审中-公开
标题翻译：包含共聚物MYRCENE块的嵌段共聚物
公开(公告)号：WO2015153747A1
公开(公告)日：2015-10-08
申请号：PCT/US2015/023857
申请日：2015-04-01
申请人： KRATON POLYMERS U.S. LLC
发明人： STOL, Marianne , DUPONT, Martine
IPC分类号： C08F297/04 , C09J153/02
CPC分类号： C09J153/02 , C08F297/02 , C08F301/00 , C08K11/00 , C09J153/00
摘要： A block copolymer comprising: at least one monoalkenyl arene monomer polymer block (A) and copolymer block (B) containing myrcene, said copolymer block B also including: a) at least one conjugated diene monomer having a lower molecular weight than myrcene, or b) at least one monoalkenyl arene monomer, or c) a mixture of a) and b). The polymer block A may be a copolymer block. When the polymer block A is a copolymer block, both block A and the copolymer myrcene block copolymer B can have a random, tapered or a controlled distribution configuration of comonomers. The block copolymer can be selectively or exhaustively hydrogenated. The block copolymer may be used in making adhesives and vibration damping compositions.
摘要翻译：一种嵌段共聚物，其包含：至少一种含有月桂烯的单烯基芳烃单体聚合物嵌段（A）和共聚物嵌段（B），所述共聚物嵌段B还包括：a）至少一种具有低于分子量的共轭二烯单体，）至少一种单烯基芳烃单体，或c）a）和b）的混合物。聚合物嵌段A可以是共聚物嵌段。当聚合物嵌段A是共聚物嵌段时，嵌段A和共聚物月桂烯嵌段共聚物B都可以具有共聚单体的随机的，锥形的或受控的分布构型。嵌段共聚物可以选择性地或穷尽地氢化。嵌段共聚物可用于制备粘合剂和减振组合物。

3. 发明申请

WO2015153736A1 ADHESIVE COMPOSITIONS CONTAINING A BLOCK COPOLYMER WITH POLYMYRCENE 审中-公开
标题翻译：含有嵌段共聚物的胶粘组合物与聚苯乙烯
公开(公告)号：WO2015153736A1
公开(公告)日：2015-10-08
申请号：PCT/US2015/023842
申请日：2015-04-01
申请人： KRATON POLYMERS U.S. LLC
发明人： DUPONT, Martine , STOL, Marianne
IPC分类号： C08L9/00
CPC分类号： C09J153/02 , C08F236/22 , C08F293/00 , C08F297/023 , C09J153/00
摘要： The invention relates to a novel block copolymer comprising at least one polymeric monoalkenyl arene block and at least one polymeric myrcene block having a low and stable viscosity and having good adhesive properties when used in an adhesive composition or as a damping material. An adhesive composition is also described, preferably containing an SMS triblock optionally mixed with an SM diblock. The adhesive composition comprises: 1) a block copolymer having at least one polymeric monoalkenyl arene block and at least one polymeric myrcene block; 2) a tackifier; 3) optional plasticizer; and 4) optionally a stabilizer. Compared with adhesive compositions comprising SIS block copolymers, those comprising SMS block copolymers have lower and more stable viscosity.
摘要翻译：本发明涉及包含至少一种聚合单烯基芳烃嵌段和至少一种聚合月桂烯嵌段的新型嵌段共聚物，其具有低且稳定的粘度并且当用于粘合剂组合物或作为阻尼材料时具有良好的粘合性能。还描述了粘合剂组合物，优选含有任选与SM二嵌段混合的SMS三嵌段。粘合剂组合物包括：1）具有至少一个聚合单烯基芳烃嵌段和至少一个聚合月桂烯嵌段的嵌段共聚物; 2）增粘剂; 3）任选的增塑剂; 和4）任选的稳定剂。与包含SIS嵌段共聚物的粘合剂组合物相比，包含SMS嵌段共聚物的粘合剂组合物具有更低和更稳定的粘度。

4. 发明申请

WO2011092071A1 THERMOFUSIBLE COMPOSITION FOR SLUSH MOULDING 审中-公开
标题翻译：用于SLUSH模制的可热成分组合物
公开(公告)号：WO2011092071A1
公开(公告)日：2011-08-04
申请号：PCT/EP2011/050538
申请日：2011-01-17
申请人： SO.F.TER.SPA , BELLOMO, Leonardo , CARFIGNINI, Alessandro , STOL, Marianne , VERVOORT, Freddy M.A. , KRATON POLYMERS U.S. LLC
发明人： BELLOMO, Leonardo , CARFIGNINI, Alessandro , STOL, Marianne , VERVOORT, Freddy M.A.
IPC分类号： C08L53/02 , B29C41/04 , B60K37/00
CPC分类号： C08L53/025 , B29C41/003 , B29C41/18 , B29K2105/0085 , C08L23/10 , C08L23/20 , Y10T428/2982 , C08L2666/02 , C08L2666/06
摘要： A thermofusible composition in the form of pellets and/or powder, with a particle size of 1400 μm or less comprising from about 40 to about 70 weight percent of a selectively hydrogenated styrenic block copolymer (HSBC), and from about 1 to about 30 weight percent of a butylene homopolymer, a butylene copolymer, or a combination of the butylene homopolymer and the copolymer, wherein the HSBC (i) is a linear or branched hydrogenated block copolymer having the general configuration A-B-A, (A-B) n , (A-B-A) n , (A-B-A) n X, (A-B) n X or mixtures thereof, where n is an integer from 2 to about 30, and X is coupling agent residue and wherein: a. prior to hydrogenation each A block is a mono alkenyl arene polymer block and each B block is a controlled distribution copolymer block of at least one conjugated diene and at least one mono alkenyl arene; b. subsequent to hydrogenation about 0-10% of the arene double bonds have been reduced, and at least about 90% of the conjugated diene double bonds have been reduced; c. each A block has a number average molecular weight from about 5.0 to about 7.5 kg/mol and, wherein the linear HSBC has a total number average molecular weight from about 70 to about 150 kg/mol and the branched HSBC has a total apparent number average molecular weight from about 35 to about 75 kg/mol per arm d. each B block comprises terminal regions adjacent to the A blocks that are rich in conjugated diene units and one or more regions not adjacent to the A blocks that are rich in mono alkenyl arene units; e. the total amount of mono alkenyl arene in the hydrogenated block copolymer is from about 20 to about 45 weight percent; f. the weight percent of mono alkenyl arene in each B block is from about 10 to about 40 weight percent; g. each B block has a styrene blockiness index of less than 10 percent; and h. the weight percent of vinyl in each B block is at least about 40 weight percent.
摘要翻译：粒径为1400μm或更小的颗粒和/或粉末形式的热熔组合物，包含约40至约70重量％的选择性氢化苯乙烯嵌段共聚物（HSBC）和约1至约30重量％丁烯均聚物，丁烯共聚物或丁烯均聚物和共聚物的组合的百分比，其中HSBC（i）是具有通式ABA，（AB）n，（ABA）n的直链或支链氢化嵌段共聚物，（ABA）nX，（AB）nX或其混合物，其中n为2至约30的整数，X为偶联剂残基，其中：a。在氢化之前，每个A嵌段是单烯基芳烃聚合物嵌段，并且每个B嵌段是至少一种共轭二烯和至少一个单烯基芳烃的受控分布共聚物嵌段; 湾在氢化后约0-10％的芳烃双键已经被还原，并且至少约90％的共轭二烯双键已经被还原; C。每个A嵌段具有约5.0至约7.5kg / mol的数均分子量，并且其中线性HSBC具有约70至约150kg / mol的总数均分子量，并且分支HSBC具有总表观数均分子量每臂约35至约75kg / mol的分子量d。每个B嵌段包括与富含共轭二烯单元的A嵌段相邻的末端区域和不与A链段相邻且富含单烯基芳烃单元的一个或多个区域; 即氢化嵌段共聚物中单烯基芳烃的总量为约20至约45重量％; F。每个B嵌段中单烯基芳烃的重量百分比为约10至约40重量％; G。每个B嵌段的苯乙烯嵌段指数小于10％; 和h。每个B嵌段中乙烯基的重量百分比为至少约40重量％。

5. 发明公开

EP3362169A1 BLOCK COPOLYMERS HAVING AMINE OR PHOSPHINE FUNCTIONALIZED END BLOCKS 审中-实审
公开(公告)号：EP3362169A1
公开(公告)日：2018-08-22
申请号：EP16856287.4
申请日：2016-10-14
申请人： Kraton Polymers U.S. LLC
发明人： VAN DER HUIZEN, Adrie A. , WILLIS, Carl L. , STOL, Marianne , MUYLDERMANS, Xavier D.
IPC分类号： B01D71/82 , B01D61/44 , B01D65/10
CPC分类号： C08G81/022 , C08J5/18 , C08J2353/00 , C08F8/32 , C08F297/04 , C08F8/40
摘要： Disclosed herein is a functionalized block copolymer comprising (a) at least one end block D comprising on average at least one amino- or phosphino- functionalized polymer unit of formula (I) and one or more additional blocks selected from the group consisting of (b) one or more A blocks substantially free of amino- or phosphino- functional groups and having a number average molecular weight of from about 1,000 to about 60,000, and has a high service temperature, and (c) one or more B blocks, wherein each block B is essentially non-functionalized, has a number average molecular weight of from about 1,000 to about 1,000,000, and has a glass transition temperature of at most about 20°C, and (d) mixtures of one or more A blocks and one or more B blocks; wherein Z is nitrogen or phosphorus; R1 is hydrogen or alkyl; R2 is hydrogen or is tertiary alkyl; R each independently, is alkyl or phenyl optionally substituted by a moiety -(A1- NRa)xRb or -(A1-ORa)xRb; or two R groups, together with the Z to which they are bonded, form an optionally substituted ring; x is 1, 2 or 3; A1 is straight chain alkylene optionally substituted by one or more methyl and/or ethyl groups; and Ra and Rb, each independently, is hydrogen or alkyl; or a corresponding onium salt.

6. 发明公开

EP3126422A1 BLOCK COPOLYMERS CONTAINING A COPOLYMER MYRCENE BLOCK 有权
标题翻译：麻醉剂麻醉剂EINEM COPOLYMER-MYRCEN-BLOCK
公开(公告)号：EP3126422A1
公开(公告)日：2017-02-08
申请号：EP15773576.2
申请日：2015-04-01
申请人： Kraton Polymers U.S. LLC
发明人： STOL, Marianne , DUPONT, Martine
IPC分类号： C08F297/04 , C09J153/02
CPC分类号： C09J153/02 , C08F297/02 , C08F301/00 , C08K11/00 , C09J153/00
摘要： A block copolymer comprising: at least one monoalkenyl arene monomer polymer block (A) and copolymer block (B) containing myrcene, said copolymer block B also including: a) at least one conjugated diene monomer having a lower molecular weight than myrcene, or b) at least one monoalkenyl arene monomer, or c) a mixture of a) and b). The polymer block A may be a copolymer block. When the polymer block A is a copolymer block, both block A and the copolymer myrcene block copolymer B can have a random, tapered or a controlled distribution configuration of comonomers. The block copolymer can be selectively or exhaustively hydrogenated. The block copolymer may be used in making adhesives and vibration damping compositions.
摘要翻译：一种嵌段共聚物，其包含：至少一种单烯基芳烃单体聚合物嵌段（A）和含有月桂烯的共聚物嵌段（B），所述共聚物嵌段B还包括：a）至少一种具有低于分子量的共轭二烯单体，）至少一种单烯基芳烃单体，或c）a）和b）的混合物。聚合物嵌段A可以是共聚物嵌段。当聚合物嵌段A是共聚物嵌段时，嵌段A和共聚物月桂烯嵌段共聚物B都可以具有共聚单体的随机的，锥形的或受控的分布构型。嵌段共聚物可以选择性地或穷尽地氢化。嵌段共聚物可用于制备粘合剂和减振组合物。

7. 发明公开

EP3126441A1 ADHESIVE COMPOSITIONS CONTAINING A BLOCK COPOLYMER WITH POLYMYRCENE 有权
标题翻译： KLEBSTOFFZUSAMMENSETZUNGEN MIT EINEM BLOCKCOPOLYMER MIT POLYMYRCEN
公开(公告)号：EP3126441A1
公开(公告)日：2017-02-08
申请号：EP15774136.4
申请日：2015-04-01
申请人： Kraton Polymers U.S. LLC
发明人： DUPONT, Martine , STOL, Marianne
IPC分类号： C08L9/00
CPC分类号： C09J153/02 , C08F236/22 , C08F293/00 , C08F297/023 , C09J153/00
摘要： The invention relates to a novel block copolymer comprising at least one polymeric monoalkenyl arene block and at least one polymeric myrcene block having a low and stable viscosity and having good adhesive properties when used in an adhesive composition or as a damping material. An adhesive composition is also described, preferably containing an SMS triblock optionally mixed with an SM diblock. The adhesive composition comprises: 1) a block copolymer having at least one polymeric monoalkenyl arene block and at least one polymeric myrcene block; 2) a tackifier; 3) optional plasticizer; and 4) optionally a stabilizer. Compared with adhesive compositions comprising SIS block copolymers, those comprising SMS block copolymers have lower and more stable viscosity.
摘要翻译：本发明涉及一种新颖的嵌段共聚物，其包含至少一种聚合单烯基芳烃嵌段和至少一种聚合月桂烯嵌段，其具有低且稳定的粘度并且当用于粘合剂组合物或作为阻尼材料时具有良好的粘合性能。还描述了粘合剂组合物，优选含有任选与SM二嵌段混合的SMS三嵌段。粘合剂组合物包括：1）具有至少一个聚合单烯基芳烃嵌段和至少一个聚合月桂烯嵌段的嵌段共聚物; 2）增粘剂; 3）任选的增塑剂; 和4）任选的稳定剂。与包含SIS嵌段共聚物的粘合剂组合物相比，包含SMS嵌段共聚物的粘合剂组合物具有更低和更稳定的粘

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