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1. 发明授权

US4870152A Process for the production of compounds containing isocyanurate groups and olefinic double bonds and their use as binders 失效
标题翻译：用于生产含有异氰脲酸酯基和烯属双键的化合物的方法及其作为粘合剂的用途
公开(公告)号：US4870152A
公开(公告)日：1989-09-26
申请号：US262623
申请日：1988-10-26
申请人： Jurgen Meixner , Manfred Bock , Josef Pedain , Manfred Schonfelder
发明人： Jurgen Meixner , Manfred Bock , Josef Pedain , Manfred Schonfelder
IPC分类号： C07D251/34 , C08G18/42 , C08G18/67 , C08G18/72 , C08G18/79 , C08G18/81 , C09D175/00 , C09D175/14
CPC分类号： C08G18/672 , C07D251/34 , C08G18/4216 , C08G18/4238 , C08G18/792 , C08G18/8175
摘要： Binders which are hardenable by radiation or peroxides and are useful in coating compositions are compounds containing isocyanurate groups and olefinic double bonds produced by the reaction of components (a), (b) and (c) wherein(a) is a polyisocyanate component containing isocyanurate polyisocyanates which is(i) N,N',N"-tris-(isocyanatohexyl)-isocyanurate alone or in admixture with its higher homologs containing more than one isocyanurate ring or(ii) mixtures of the polyisocyanates (i) with up to 40 NCO-equivalent-%, based on the total component (a), of other polyisocyanates containing aliphatically or cycloaliphatically bound isocyanate groups;(b) is an olefinically unsaturated alcohol component comprising at least one hydroxyalkyl ester of acrylic acid or methacrylic acid; and(c) is a polyol component consisting essentially of a polyester polyol having an OH value of 80 to 350 based on (i) an acid component, of which at least 80 carboxyl equivalent-% is adipic acid, isophthalic acid or a mixture of both and (ii) a polyhydroxy component of which at least 70 hydroxyl equivalent-% is hexane-1, 6-diol;wherein component (c) amounts to 20 to 150% by weight, based on the weight of component (b), and the reaction is carried out at with an NCO:OH equivalent ratio maintained at 0.9:1 to 1.1:1, and wherein components (b) and (c) are reacted with the polyisocyanate component in any order or in admixture.
摘要翻译：通过辐射或过氧化物可硬化并且可用于涂料组合物的粘合剂是含有通过组分（a），（b）和（c）反应生成的异氰脲酸酯基团和烯属双键的化合物，其中（a）是含有异氰脲酸酯的多异氰酸酯组分多异氰酸酯，其是单独的或与其含有多于一个异氰脲酸酯环的较高同系物混合的（i）N，N'，N“ - 三 - （异氰酸根合己基） - 异氰脲酸酯的多异氰酸酯，或（ii）多异氰酸酯（i）基于总组分（a），含有脂族或环脂族结合的异氰酸酯基团的其它多异氰酸酯的40NCO当量％; （b）是包含至少一种丙烯酸或甲基丙烯酸的羟烷基酯的烯属不饱和醇组分; 和（c）是基于（i）酸组分的羟值为80至350的聚酯多元醇组成的多元醇组分，其中至少80羧基当量 - ％是己二酸，间苯二甲酸或两者和（ii）多羟基组分，其中至少70个羟基当量 - ％是己烷-1,6-二醇; 其中组分（c）基于组分（b）的重量计为20至150重量％，并且以保持在0.9:1至1.1:1的NCO:OH当量比进行反应，其中组分（b）和（c）以多异氰酸酯组分的任何顺序或混合物反应。

2. 发明授权

US5902897A Polyamines and their use in coating compositions 失效
标题翻译：多胺及其在涂料组合物中的用途
公开(公告)号：US5902897A
公开(公告)日：1999-05-11
申请号：US684355
申请日：1996-07-19
申请人： Christian Wamprecht , Theodor Engbert , Holger Casselmann , Josef Pedain , Jurgen Meixner
发明人： Christian Wamprecht , Theodor Engbert , Holger Casselmann , Josef Pedain , Jurgen Meixner
IPC分类号： C07C211/13 , C08G18/40 , C08G18/46 , C08G18/64 , C08G18/80 , C08G73/02 , C08L79/02 , C09D175/00 , C09D175/04 , C09D179/02 , C07C229/26
CPC分类号： C08G18/6415 , C08G18/4669 , C08G73/02 , C08G73/028 , C08L79/02 , C09D179/02
摘要： The present invention relates to polyamines which are prepared by reactinga) unsaturated oligoesters having an average of 2 to 4 double bonds per molecule andb) optionally other unsaturated compounds suitable as Michael addition acceptors and having an average of 1 to 4 double bonds per molecule withc) (cyclo)aliphatic diamines having two primary amino groups andd) optionally other amino-functional compounds suitable as Michael addition donors.The present invention also relates to the use of these polyamines as a binder component in lacquers and coating compositions, particularly as reactants for blocked polyisocyanates in one-component stoving lacquers.
摘要翻译：本发明涉及多胺，其通过使a）每分子平均具有2至4个双键的不饱和低聚酯和b）任选的适合作为迈克尔加成受体并且每分子平均具有1至4个双键的其它不饱和化合物与c）具有两个伯氨基的（环）脂族二胺和d）任选的其它适用作迈克尔加成供体的氨基官能化合物。本发明还涉及这些多胺作为粘合剂组分在漆和涂料组合物中的用途，特别是作为单组分烘烤漆中封端多异氰酸酯的反应物。

3. 发明授权

US5252648A Compositions containing octadienyl ethers as reactive thinners 失效
标题翻译：含有辛二烯基醚作为反应性稀释剂的组合物
公开(公告)号：US5252648A
公开(公告)日：1993-10-12
申请号：US985977
申请日：1992-12-04
申请人： Peter Hohlein , Jurgen Meixner , Josef Pedain
发明人： Peter Hohlein , Jurgen Meixner , Josef Pedain
IPC分类号： C09K3/10 , C09D5/34 , C09D7/00 , C09D7/12 , C08L75/04
CPC分类号： C09D7/001 , C09D5/34
摘要： The present invention relates to a composition which is suitable for the preparation of coatings, sealants and/or fillers and contains one or more binder components and as reactive thinner an octadienyl ether which may contain ester groups and which has a viscosity at 23.degree. C. of at most 5,000 mPas and a content of 1 to 80% by weight of octadienyl groups, --C.sub.8 H.sub.13, 0 to 35% by weight of hydroxyl groups and 0 to 30% by weight of carboxyl groups.
摘要翻译：本发明涉及一种适用于制备涂料，密封剂和/或填料并且含有一种或多种粘合剂组分的组合物，并且作为活性稀释剂可以含有酯基并且在23℃下具有粘度的辛二烯基醚。至多5,000mPas，含量为1至80％（重量）的辛二烯基，-C 8 H 13 0至35％（重量）的羟基和0至30％（重量）的羧基。

4. 发明授权

US5128432A Aliphatic polyurethanes containing acryloyl groups and a process for their preparation 失效
标题翻译：含有丙烯酸酯的聚氨酯和其制备方法
公开(公告)号：US5128432A
公开(公告)日：1992-07-07
申请号：US749235
申请日：1991-08-23
申请人： Jurgen Meixner , Wolfgang Fischer , Josef Pedain
发明人： Jurgen Meixner , Wolfgang Fischer , Josef Pedain
IPC分类号： C08F299/06 , C08G18/28 , C08G18/32 , C08G18/48 , C08G18/67 , C08G18/73 , C09D175/14 , C09D175/16
CPC分类号： C08G18/4887 , C08G18/284 , C08G18/3221 , C08G18/672 , C08G18/673 , C08G18/73 , C09D175/16
摘要： The present invention relates to aliphatic polyurethanes which contain acryloyl groups and are based on the reaction product (at an NCO/OH equivalent ratio of 0.5:1 to 1:1) ofa) 1.0 mole of a diisocyanate component containing at least 50 equivalent percent, based on NCO equivalents, of hexamethylene diisocyanate withb) 0.5 to 0.85 moles of at least one monohydric alcohol having a molecular weight of 116 to 144 and containing acryloyl groups.c) 0.15 to 0.5 moles of a monohydric alcohol having a molecular weight of 154 to 2000 and containing ester groups or a mixture of alcohols having an average molecular weight of 154 to 2000 and an average hydroxyl functionality of 0.8 to 1.5 and containing ester groups andd) 0.3 to 0.5 moles of at least one polyhydric alcohol having a molecular weight of 62 to 2000.The present invention also relates to a process for the preparation of these polyurethanes.
摘要翻译：本发明涉及含有丙烯酰基并基于反应产物（以NCO / OH当量比为0.5:1至1:1）的a）1.0摩尔含至少50当量％的二异氰酸酯组分的脂族聚氨酯基于NCO当量，六亚甲基二异氰酸酯与b）0.5至0.85摩尔的至少一种分子量为116至144的一元醇并含有丙烯酰基。 c）0.15至0.5摩尔分子量为154至2000的一元醇，并且含有酯基或平均分子量为154至2000的醇和0.8至1.5的平均羟基官能度的混合物，并且含有酯基和 d）0.3至0.5摩尔的至少一种分子量为62至2000的多元醇。本发明还涉及制备这些聚氨酯的方法。

5. 发明授权

US5126393A Water-dispersible binder composition, a process for the production of a stoving filler and a coating prepared therefrom 失效
标题翻译：水分散性组合物，生产填充填料的方法及其制备的涂料
公开(公告)号：US5126393A
公开(公告)日：1992-06-30
申请号：US602595
申请日：1990-10-24
申请人： Harald Blum , Jurgen Meixner , Josef Pedain , Hans-Heribert Burgdorfer
发明人： Harald Blum , Jurgen Meixner , Josef Pedain , Hans-Heribert Burgdorfer
IPC分类号： C08G18/00 , B01F17/42 , C08G18/08 , C08G18/10 , C08G18/12 , C08G18/42 , C08G18/66 , C08G18/75 , C09D161/20 , C09D175/06
CPC分类号： C08G18/12 , C08G18/0823 , C08G18/423 , C08G18/4288 , C08G18/6659 , C08G18/75 , C09D175/06
摘要： The present invention relates to a water-dispersible binder composition which is suitable for the production of a stoving filler to be processed from the aqueous phase and which containsa) 65 to 95% by weight of a urethane-modified polyester resin containing carboxyl groups,b) 5 to 35% by weight of a crosslinker resin andc) 0 to 2% by weight of an emulsifier,wherein the percentages are based on the total weight of components a) to c), characterized in that component a) has an acid value of 15 to 36, a hydroxyl value of at least 40 and a molecular weight (M.sub.w) of 5,000 to 50,000 and has been obtained by reactinga1) 72 to 80% by weight of a polyester polyol having a hydroxyl value of 130 to 200 and an acid value of 1 to 5 anda2) 4 to 7% by weight of a 2,2-bis-(hydroxymethyl)-alkane carboxylic acid or a quantity corresponding to this quantity of acid of a tertiary amine salt of such an acid witha3) 15 to 24% by weight of at least one cycloaliphatic diisocyanate having a molecular weight of 166 to 294,wherein the percentages are based on the total weight of components a1) to a3).The present invention also relates to a process for the production of an aqueous stoving filler which is suitable for the production of chip resistant coatings and to the chip resistant coatings produced therefrom.
摘要翻译：本发明涉及一种水分散性粘合剂组合物，其适用于从水相制备待加工的烘干填料，其含有a）65至95重量％的含有羧基的氨基甲酸酯改性的聚酯树脂， b）5〜35重量％的交联剂树脂和c）0〜2重量％的乳化剂，其中所述百分比基于组分a）至c）的总重量，其特征在于组分a）具有酸值为15〜36，羟基值为40以上，分子量（Mw）为5,000〜50,000，通过使a1〜72〜80重量％的羟基值为130的聚酯多元醇与 200，酸值1〜5，a2）4〜7重量％的2,2-双 - （羟甲基） - 烷烃羧酸，或相当于该量的这种叔胺盐的酸量酸与a3）15至24重量％的至少一种具有分子的脂环族二异氰酸酯 166至294的百分比，其中百分比基于组分a1）至a3）的总重量。本发明还涉及一种用于生产水性烘干填料的方法，该方法适用于生产耐屑涂层和由其制备的耐芯片涂层。

6. 发明授权

US5095066A Hydrophilic polyurethanes containing (meth)acryloyl groups, their use as reactive emulsifiers for radically curable synthetic resins, water-dispersible mixture of radically curable synthetic resins and an aqueous coating composition based on this mixture 失效
标题翻译：含有（甲基）丙烯酸基团的亲水性聚氨酯，它们作为无机可固化合成树脂的反应性乳化剂，可溶性合成树脂的水分散混合物和基于该混合物的水性涂料组合物
公开(公告)号：US5095066A
公开(公告)日：1992-03-10
申请号：US456539
申请日：1989-12-26
申请人： Jurgen Meixner , Josef Pedain , Wolfgang Fischer
发明人： Jurgen Meixner , Josef Pedain , Wolfgang Fischer
IPC分类号： C08F299/06 , B01F17/52 , C08F290/00 , C08G18/48 , C08G18/67 , C08G18/81 , C09D175/00 , C09D175/14 , C09D175/16
CPC分类号： C08G18/8175 , C08G18/4833 , C09D175/16
摘要： A polyurethane is disclosed having improved properties as a reactive emulsifier for radically-curable synthetic resins. The polyurethane is obtained by the reaction of a) a polyisocyanate component; b) an alcohol component; and c) a polyethylene glycol component. The reactive emulsifiers are useful in aqueous coating compositions.
摘要翻译：公开了具有改进的性质的聚氨酯作为用于可自由基固化的合成树脂的反应性乳化剂。聚氨酯通过a）多异氰酸酯组分的反应获得; b）醇组分; 和c）聚乙二醇组分。反应性乳化剂可用于水性涂料组合物。

7. 发明授权

US5925711A Polyamines and their use in aqueous coating compositions 失效
标题翻译：多胺及其在水性涂料组合物中的用途
公开(公告)号：US5925711A
公开(公告)日：1999-07-20
申请号：US882852
申请日：1997-06-26
申请人： Christian Wamprecht , Hans-Josef Laas , Jurgen Meixner , Josef Pedain
发明人： Christian Wamprecht , Hans-Josef Laas , Jurgen Meixner , Josef Pedain
IPC分类号： C08G18/32 , C08G18/46 , C08G18/64 , C08G18/70 , C08G73/00 , C08G73/02 , C08L79/08 , C09D5/00 , C09D175/04 , C09D179/08 , C09J179/02 , C07C209/16
CPC分类号： C08G18/6415 , C08G18/4669 , C08G18/706 , C08G73/02 , C08G73/028 , C08L79/08 , C09D179/08 , C09J179/02 , C08G2261/135 , C08G2261/334 , C08G2261/76
摘要： The present invention relates to polyamines which are the reaction products ofa) unsaturated oligoesters containing an average of 2 to 4 double bonds per molecule andb) optionally other unsaturated compounds which are suitable as Michael addition acceptors and which contain an average of 1 to 4 double bonds per molecule, withc) (cyclo)aliphatic diamines which contain two primary amino groups, andd) optionally other amino-functional compounds which are suitable as Michael addition donors.The present invention also relates to aqueous, two-component coating compositions containing as binderA) the polyamines according to the invention andB) water dispersible polyisocyanates, andto coatings obtained from these coating compositions.
摘要翻译：本发明涉及多胺，其为a）每分子平均含有2〜4个双键的不饱和低聚酯的反应产物，以及b）任选的其它适合作为迈克尔加成受体的不饱和化合物，其平均含有1至4个每个分子具有双键，c）（环）脂族二胺，其含有两个伯氨基，以及d）任选的其它适合作为迈克尔加成供体的氨基官能化合物。本发明还涉及包含作为粘合剂A）本发明的多胺和B）水分散性多异氰酸酯的水性双组分涂料组合物以及由这些涂料组合物获得的涂料。

8. 发明授权

US4748269A Process for the preparation of (meth)acrylic acid esters and their use 失效
标题翻译：制备（甲基）丙烯酸酯的方法及其用途
公开(公告)号：US4748269A
公开(公告)日：1988-05-31
申请号：US851742
申请日：1986-04-14
申请人： Jurgen Meixner , Josef Pedain , Peter Hohlein , Dieter Margotte
发明人： Jurgen Meixner , Josef Pedain , Peter Hohlein , Dieter Margotte
IPC分类号： C07C69/54 , C08F2/46 , C08F220/36 , C07C69/52
CPC分类号： C07C69/54 , C07C67/08 , C07C67/60
摘要： (Meth)acrylic acid esters can be prepared by acid-catalyzed reaction of (meth)acrylic acid with alcohols in a water-immiscible solvent. After the esterification, the reaction mixture is washed with aqueous solutions having an alkaline reaction and then reacted at elevated temperature with carbodiimides. Acid numbers below 0.5 (mg of KOH/g of substance) are obtained in this way. (Meth)acrylic acid esters are used, for example, as reactive diluents or as comonomers.
摘要翻译：（甲基）丙烯酸酯可以通过（甲基）丙烯酸与醇在水不混溶溶剂中的酸催化反应来制备。酯化后，反应混合物用碱性反应的水溶液洗涤，然后在高温下与碳二亚胺反应。以这种方式获得酸值低于0.5（KOH / g的物质）。（甲基）丙烯酸酯用作例如作为反应性稀释剂或共聚单体。

9. 发明授权

US5068305A Powder coating compositions containing polyurethanes having (meth)acryloyl groups as binders 失效
标题翻译：含有（甲基）丙烯酰基作为粘合剂的聚氨酯的粉末涂料组合物
公开(公告)号：US5068305A
公开(公告)日：1991-11-26
申请号：US556223
申请日：1990-07-20
申请人： Jurgen Meixner , Josef Pedain , Peter Hohlein , Hans-Joachim Kreuder
发明人： Jurgen Meixner , Josef Pedain , Peter Hohlein , Hans-Joachim Kreuder
IPC分类号： C08F299/00 , C08F290/00 , C08F299/06 , C08G18/67 , C08G18/81 , C09D5/03 , C09D5/46 , C09D175/14 , C09D175/16
CPC分类号： C09D175/16 , C08F299/06 , C08G18/8175 , C08G2150/20
摘要： The present invention relates to powder coating compositions which can be cured in the presence of heat and/or high energy radiation and contain polyurethanes which melt at temperatures of 50.degree. to 180.degree. C., have 3 to 10% by weight of olefinic double bonds in the form of (meth)acryloyl groups (calculated as .dbd.C.dbd.C.dbd., molecular weight=24) and are based on the reaction product ofA) 40 to 80 parts by weight of one or more organic polyisocyanates withB) 15 to 50 parts of weight of one or more monohydric alcohols containing (meth)acryloyl groups andC) 2 to 20 parts by weight one or more compounds which are free from (meth)acryloyl groups and contain isocyanate reactive groups.
摘要翻译：本发明涉及粉末涂料组合物，其可以在热和/或高能量辐射的存在下固化，并且包含在50-180℃的温度下熔化的聚氨酯，具有3至10重量％的烯属双键以（甲基）丙烯酰基的形式（以C = C =分子量= 24计算），并且基于A）的反应产物：40至80重量份的一种或多种有机多异氰酸酯与B）15至 50重量份的一种或多种含（甲基）丙烯酰基的一元醇和C）2至20重量份的一种或多种不含（甲基）丙烯酰基并含有异氰酸酯反应性基团的化合物。

10. 发明授权

US5208291A Powder coating compositions, a process for their production and their use for coating heat-resistant substrates 失效
标题翻译：粉末涂料组合物，其制备方法及其用于涂覆耐热基材的方法
公开(公告)号：US5208291A
公开(公告)日：1993-05-04
申请号：US941498
申请日：1992-09-08
申请人： Christian Wamprecht , Reinhard Halpaap , Hans-Joachim Kreuder , Manfred Bock , Jurgen Meixner , Rainer Rettig , Wolfgang Schultz
发明人： Christian Wamprecht , Reinhard Halpaap , Hans-Joachim Kreuder , Manfred Bock , Jurgen Meixner , Rainer Rettig , Wolfgang Schultz
IPC分类号： B05D7/24 , C08G18/62 , C08G18/78 , C08G18/79 , C08G18/80 , C08J3/12 , C09D5/03 , C09D5/46 , C09D175/00 , C09D175/04
CPC分类号： C08G18/6229 , C08G18/6254 , C08G18/78 , C08G18/7831 , C08G18/792 , C08G18/8077 , C08G2150/20 , Y10S524/904
摘要： The present invention relates to a process for the production of powder coating compositions having a glass transition temperature of 20.degree. to 80.degree. C. bya) homogeneously dissolving in an inert solvent or solvent mixture having a boiling point or range between 50.degree. and 150.degree. C.A) a polyol component having a hydroxyl value of 30 to 155 and a glass transition temperature of 30.degree. to 120.degree. C. and containing at least one hydroxy-functional copolymer of olefinically unsaturated monomers,B) a polyisocyanate component containing blocked isocyanate groups, having a glass transition temperature of -45.degree. to +45.degree. C. and containing at least one ketoxime-blocked polyisocyanate andC) a catalyst component containing at least one catalyst for the reaction between blocked isocyanate groups and hydroxyl groups components, wherein components A) and B) are present in an amount which is sufficient to provide an equivalent ratio of blocked isocyanate groups to hydroxyl groups of 0.5:1 to 1.5:1,b) freeing the resulting solution from the solvent andc) simultaneously and/or subsequently converting the solid obtained into powder form.The present invention also relates to the powder coating compositions obtained by this process and their use for the production of coatings of heat-resistant substrates.
摘要翻译：本发明涉及通过以下方法生产具有玻璃化转变温度为20-80℃的粉末涂料组合物的方法：a）均匀溶于沸点或范围为50至150℃的惰性溶剂或溶剂混合物中 A）多元醇组分，其羟基值为30至155，玻璃化转变温度为30至120℃，并含有至少一种烯属不饱和单体的羟基官能共聚物，B）含有封端的多异氰酸酯组分异氰酸酯基团，玻璃化转变温度为-45℃至+ 45℃，并含有至少一种酮肟封端的多异氰酸酯和C）含有至少一种用于封端异氰酸酯基团和羟基组分之间反应的催化剂的催化剂组分，其中组分A）和B）以足以提供封端异氰酸酯基与羟基的当量比为0.5:1至1的量存在 b）将所得溶液从溶剂中释放，以及c）同时和/或随后将获得的固体转化为粉末形式。本发明还涉及通过该方法获得的粉末涂料组合物及其用于生产耐热基材的涂层的用途。

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