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1. 发明授权

US5241109A Asymmetrical oxalic acid diarylamide 失效
标题翻译：不对称氧化二乙酰胺
公开(公告)号：US5241109A
公开(公告)日：1993-08-31
申请号：US858913
申请日：1992-03-27
申请人： Jurgen Kaschig , Gerhard Reinert , Georges Metzger
发明人： Jurgen Kaschig , Gerhard Reinert , Georges Metzger
IPC分类号： D06P1/645 , C07C309/11 , C07C309/51 , D06M13/02 , D06M13/322 , D06M13/402 , D06M101/00 , D06M101/12 , D06M101/16 , D06M101/30 , D06M101/34 , D06P1/649 , D06P3/24 , D06P5/00 , D06P5/06
CPC分类号： C07C309/11 , C07C309/51 , D06P1/6495
摘要： There is disclosed a water-soluble, asymmetrical oxalic acid diarylamide of general formula ##STR1## wherein the substituents R.sub.1 are each independently of the other unsubstituted or hydroxy- or alkoxy-substituted C.sub.1 -C.sub.5 alkyl, unsubstituted or C.sub.1 -C.sub.5 alkyl-substituted benzyl,R.sub.2 is hydrogen, halogen, C.sub.1 -C.sub.12 alkyl or phenyl-C.sub.1 -C.sub.5 alkyl,R.sub.3 is hydrogen, halogen, C.sub.1 -C.sub.12 alkyl, phenyl-C.sub.1 -C.sub.5 alkyl or C.sub.1 -C.sub.5 alkoxy,A is a direct bond or a divalent radical of formula --O--Q--, whereinQ is unsubstituted or hydroxy-substituted C.sub.1 -C.sub.6 alkylene,M is hydrogen or alkali metal, andr is 2, 1 or 0.The novel water-soluble compound having fiber affinity is suitable for the photochemical and thermal stabilisation of polyamide fiber materials and the dyeings produced thereon.
摘要翻译：公开了通式为（1）的水溶性不对称草酸二芳基酰胺，其中取代基R 1各自独立地为其它未取代的或羟基或烷氧基取代的C 1 -C 5烷基，未取代的或C 1 -C 5烷基取代的苄基，R 2是氢，卤素，C 1 -C 12烷基或苯基-C 1 -C 5烷基，R 3是氢，卤素，C 1 -C 12烷基，苯基-C 1 -C 5烷基或C 1 -C 5烷氧基，A是直接键或式 - OQ-，其中Q为未取代的或羟基取代的C 1 -C 6亚烷基，M为氢或碱金属，r为2或1。具有纤维亲和性的新型水溶性化合物适用于聚酰胺的光化学和热稳定性纤维材料和其上产生的染色。

2. 发明申请

US20050019281A1 Biphenyl-substituted triazines 失效
标题翻译：联苯取代三嗪
公开(公告)号：US20050019281A1
公开(公告)日：2005-01-27
申请号：US10921282
申请日：2004-08-18
申请人： Ian Fletcher , Jurgen Kaschig , Georges Metzger , Dieter Reinehr , Pascal Hayoz
发明人： Ian Fletcher , Jurgen Kaschig , Georges Metzger , Dieter Reinehr , Pascal Hayoz
IPC分类号： C07D251/10 , C07D251/24 , C07D405/04 , C08K5/3435 , C08K5/3475 , C08K5/3492 , A61K7/42 , C07D413/14
CPC分类号： C07D405/04 , A61K8/4966 , A61Q17/04 , C07D251/10 , C07D251/24 , C08K5/3435 , C08K5/3475 , C08K5/3492
摘要： Biphenyl-substituted triazines of the formulae which are notable for high thermal stability, are used as stabilizers for organic polymers to counter damage thereto caused by light, oxygen and heat, as light stabilizers for textile fiber materials and as sunscreens for the human skin.
摘要翻译：用于高热稳定性的配方的联苯取代三嗪作为有机聚合物的稳定剂用作抗光，氧和热引起的损伤，作为纺织纤维材料的光稳定剂和用于人体皮肤的防晒剂。

3. 发明申请

US20070274933A1 Amino- and hydroxysubstituted triphenyl-S-triazines as stabilizers 失效
公开(公告)号：US20070274933A1
公开(公告)日：2007-11-29
申请号：US11891554
申请日：2007-08-10
申请人： Dieter Reinehr , Georges Metzger , Peter Michaelis , Helmut Luther
发明人： Dieter Reinehr , Georges Metzger , Peter Michaelis , Helmut Luther
IPC分类号： A61K31/785 , A61K47/22 , A61K8/00 , A61Q17/04
CPC分类号： A61K8/4966 , A61K31/785 , A61K2800/52 , A61Q17/04 , C07D251/24 , C07D265/22 , Y10S514/972
摘要： The present invention provides compounds having the formula: in which R is hydrogen, hydroxy, halogen, C1-C20-alkyl, C4-C12cycloalkyl, C2-C20alkenyl, C2-C20alkynyl, C1-C20-alkoxy, C4-C12cycloalkoxy, C2-C20alkenoxy, C2-C20alkynoxy or C7-C13aralkyl; R1 and R2, independently, are hydrogen, C1-C20alkyl, C4-C12cycloalkyl, C7-C13 aralkyl, —C(═O)—R4 (in which R4 is C1-C20alkyl, C2-C20alkyl interrupted by 1 to 6 oxygen atoms, hetero-substituted C1-C20alkyl, C4-C12cycloalkyl, C2-C20alkenyl, C2-C20alkynyl, C1-C20-alkoxy, C4-C12cycloalkoxy, C2-C20alkenoxy, C2-C20alkynoxy, C6-C12 aryl, C6-C12 aryloxy or C7-C13 aralkyl), or —C(═O)—NH—R1 in which R1 has its previous significance; and R3 is hydrogen, halogen, hydroxy, C1-C20alkyl, C4-C12cycloalkyl, C2-C20alkenyl, C2-C20alkynyl, C1-C20-alkoxy, C4-C12cycloalkoxy, C2-C20alkenoxy, C2-C20alkynoxy, phenyl, C7-C13 aralkyl or —N(R1)(R2) in which R1 and R2 have their previous significance, or R1 and R2 together form a C4-C12 membered ring. The new triphenyltriazine compounds have improved absorption spectrum characteristics and superior resistance to exposure to UV light, relative to known triphenyltriazine compounds.

4. 发明授权

US07087753B2 Naphthyltriazines as stabilizers for organic material 有权
标题翻译：萘基三嗪作为有机材料的稳定剂
公开(公告)号：US07087753B2
公开(公告)日：2006-08-08
申请号：US11098640
申请日：2005-04-04
申请人： Vien Van Toan , Georges Metzger , Thomas Schäfer , Stéphane Biry , Christophe Bulliard , Dieter Reinehr , Peter Michaelis
发明人： Vien Van Toan , Georges Metzger , Thomas Schäfer , Stéphane Biry , Christophe Bulliard , Dieter Reinehr , Peter Michaelis
IPC分类号： C07D251/24 , A61K7/42 , G03C1/005
CPC分类号： C07D251/24
摘要： Novel compounds of formula I are described wherein E corresponds to the formula or to the formula and the radicals R1, R2, R11, R22, R′22, R′33 and R′33 are as defined in claim 1. Compounds of formula I are suitable for stabilizing organic material, especially plastics materials, surface-coatings, cosmetic preparations, sun protection agents or photographic material, against damage by light, oxygen and/or heat.
摘要翻译：描述了新的式I化合物，其中E对应于式或式，基团R 1，R 2，R 11， R 22，R 22，R 33和R 33如权利要求1中所定义。式I化合物适用于稳定有机材料，特别是塑料材料，表面涂层，化妆品制剂，防晒剂或照相材料，以防止光，氧和/或热的损害。

5. 发明授权

US06919454B2 Biphenyl-substituted triazines 失效
标题翻译：联苯取代三嗪
公开(公告)号：US06919454B2
公开(公告)日：2005-07-19
申请号：US10921282
申请日：2004-08-18
申请人： Ian John Fletcher , Jürgen Kaschig , Georges Metzger , Dieter Reinehr , Pascal Hayoz
发明人： Ian John Fletcher , Jürgen Kaschig , Georges Metzger , Dieter Reinehr , Pascal Hayoz
IPC分类号： C07D251/10 , C07D251/24 , C07D405/04 , C08K5/3435 , C08K5/3475 , C08K5/3492 , C08K5/34
CPC分类号： C07D405/04 , A61K8/4966 , A61Q17/04 , C07D251/10 , C07D251/24 , C08K5/3435 , C08K5/3475 , C08K5/3492
摘要： Biphenyl-substituted triazines of the formula which are notable for high thermal stability, are used as stabilizers for organic polymers to counter damage thereto caused by light, oxygen and heat, as light stabilizers for textile fiber materials and as sunscreens for the human skin.
摘要翻译：用于高热稳定性的联苯取代三嗪作为有机聚合物的稳定剂用作抗光，氧和热引起的损伤，作为纺织纤维材料的光稳定剂和用作人体皮肤的防晒剂。

6. 发明授权

US06841670B2 Biphenyl-substituted triazines 失效
标题翻译：联苯取代三嗪
公开(公告)号：US06841670B2
公开(公告)日：2005-01-11
申请号：US10209440
申请日：2002-07-31
申请人： Ian John Fletcher , Jürgen Kaschig , Georges Metzger , Dieter Reinehr
发明人： Ian John Fletcher , Jürgen Kaschig , Georges Metzger , Dieter Reinehr
IPC分类号： C07D251/10 , C07D251/24 , C07D405/04 , C08K5/3435 , C08K5/3475 , C08K5/3492
CPC分类号： C07D405/04 , A61K8/4966 , A61Q17/04 , C07D251/10 , C07D251/24 , C08K5/3435 , C08K5/3475 , C08K5/3492
摘要： Biphenyl-substituted triazines of the formulae which are notable for high thermal stability, are used as stabilizers for organic polymers to counter damage thereto caused by light, oxygen and heat, as light stabilizers for textile fiber materials and as sunscreens for the human skin.
摘要翻译：用于高热稳定性的配方的联苯取代三嗪作为有机聚合物的稳定剂用作抗光，氧和热引起的损伤，作为纺织纤维材料的光稳定剂和用作人体皮肤的防晒剂。

7. 发明授权

US06210449B1 Fluorescent whitening agents 失效
标题翻译：荧光增白剂
公开(公告)号：US06210449B1
公开(公告)日：2001-04-03
申请号：US09381468
申请日：1999-09-20
申请人： Peter Rohringer , Georges Metzger , Dieter Reinehr
发明人： Peter Rohringer , Georges Metzger , Dieter Reinehr
IPC分类号： C07D25100
CPC分类号： C09B23/148 , C07D251/68 , C11D3/42 , D06L4/621 , D06L4/657 , D06L4/75 , D06M13/07 , D06M13/358 , D06P1/6426 , D21H21/30 , Y10S8/919
摘要： The present invention provides new compounds having formula (1), in which X is 0 or, preferably, NH; M is hydrogen, an alkali metal atom, ammonium or a cation formed from an amine; each R1, independently, is an aminoacid residue from which a hydrogen atom on the amino group has been removed; n is 1 or 2; and each R2, independently, is hydrogen, C1-C3alkyl, halogen, cyano, COOR in which R is hydrogen or C1-C3alkyl, CONH—R in which R has its previous significance, SO2NH—R in which R has its previous significance, NH—COR in which R has its previous significance, SO3M in which M has its previous significance or, when n is 1, R2 can also be CO—R3 in which R3 is C1-C3alkyl or phenyl; provided that those compounds are excluded in which a) X is NH, n is 1 and R2 is SO3M in which M has its previous significance; or b) X is NH, n is 2 and one R2 is SO3M in which M has its previous significance, and the other R2 is hydrogen, methyl or halogen; or c) X is NH, n is 1, R1 is glycine and R2 is H or CO2H; or d) X is NH, n is 2, each R2 is SO3M in which M has its previous significance and the SO3M groups are in 2,5-positions in the phenyl ring and R1 is D,L-alanine, L-valine, L-leucine; L-isoleucine, L-threonine, L-aspartic acid, L-glutamic acid, L-phenylalanine, L-proline, D,L-methionine or glycine. Most of the new class of 4,4′-diaminostilbene-2,2′-disulfonic acid compounds are useful as fluorescent whitening agents, especially for paper.
摘要翻译：本发明提供具有式（1）的新化合物，其中X为0或优选为NH; M是氢，碱金属原子，铵或由胺形成的阳离子; 每个R 1独立地是氨基酸被除去的氨基酸残基; n为1或2; 并且每个R 2独立地是氢，C 1 -C 3烷基，卤素，氰基，其中R是氢或C 1 -C 3烷基的COOR，其中R具有其先前含义的CONH-R，其中R具有其先前含义的SO 2 NH- 其中R具有其先前含义的NH-COR，其中M具有其先前含义的SO 3 M，或当n为1时，R 2也可以是其中R 3为C 1 -C 3烷基或苯基的CO-R 3; 条件是排除这些化合物，其中a）X是NH，n是1，R2是其中M具有其先前意义的SO 3 M; 或b）X是NH，n是2，一个R2是SO3M，其中M具有其先前的含义，另一个R 2是氢，甲基或卤素; 或c）X是NH，n是1，R1是甘氨酸，R2是H或CO2H; 或d）X是NH，n是2，每个R2是SO3M，其中M具有其先前的意义，SO 3 M基团在苯环中是2.5位，R 1是D，L-丙氨酸，L-缬氨酸， L-亮氨酸 L-异亮氨酸，L-苏氨酸，L-天冬氨酸，L-谷氨酸，L-苯丙氨酸，L-脯氨酸，D，L-甲硫氨酸或甘氨酸。大多数新类的4,4'-二氨基芪-2,2'-二磺酸化合物可用作荧光增白剂，特别是用于纸。

8. 发明授权

US5939379A Triazine derivatives and their use 失效
标题翻译：三嗪衍生物及其用途
公开(公告)号：US5939379A
公开(公告)日：1999-08-17
申请号：US867110
申请日：1997-06-02
申请人： Claude Eckhardt , Dieter Reinehr , Georges Metzger , Hanspeter Sauter
发明人： Claude Eckhardt , Dieter Reinehr , Georges Metzger , Hanspeter Sauter
IPC分类号： C07D251/52 , C07D251/54 , C07D251/68 , C09B62/04 , C09K3/00 , C11D3/395 , C11D3/42 , D06L3/12 , D06M13/02 , D06M13/248 , D06M13/256 , D06M13/322 , D06M13/35 , D06M13/355 , D06M13/358 , D06M13/402 , D06M13/415 , D06M13/463 , D06P1/642 , D21H21/28 , D21H27/00 , C11D3/34 , C11D7/54
CPC分类号： C09B23/148 , C07D251/52 , C07D251/68 , C11D3/42 , D06L3/1214 , D06L3/1257 , D06M13/358 , D06P1/6426
摘要： The present invention relates to new compounds which are useful as ultraviolet absorbing agents (UVAs) and as fluorescent whitening agents (FWAs), and to a method of improving the sun protection factor (SPF) of textile fibre material, especially cotton, polyamide and wool, treated with the new compounds.
摘要翻译：本发明涉及可用作紫外线吸收剂（UVA）和荧光增白剂（FWA）的新化合物，以及改善纺织纤维材料，特别是棉花，聚酰胺和羊毛的防晒因子（SPF）的方法，用新化合物处理。

9. 发明授权

US07476699B2 Amino- and hydroxysubstituted triphenyl-s-triazines as stabilizers 失效
标题翻译：氨基和羟基取代的三苯基-s-三嗪作为稳定剂
公开(公告)号：US07476699B2
公开(公告)日：2009-01-13
申请号：US11891554
申请日：2007-08-10
申请人： Dieter Reinehr , Georges Metzger , Peter Michaelis , Helmut Luther
发明人： Dieter Reinehr , Georges Metzger , Peter Michaelis , Helmut Luther
IPC分类号： C08K5/3492
CPC分类号： A61K8/4966 , A61K31/785 , A61K2800/52 , A61Q17/04 , C07D251/24 , C07D265/22 , Y10S514/972
摘要： The present invention provides compounds having the formula: in which R is hydrogen, hydroxy, halogen, C1-C20-alkyl, C4-C12cycloalkyl, C2-C20alkenyl, C2-C20alkynyl, C1-C20-alkoxy, C4-C12cycloalkoxy, C2-C20alkenoxy, C2-C20alkynoxy or C7-C13aralkyl; R1 and R2, independently, are hydrogen, C1-C20alkyl, C4-C12cycloalkyl, C7-C13 aralkyl, —C(═O)—R4 (in which R4 is C1-C20alkyl, C2-C20alkyl interrupted by 1 to 6 oxygen atoms, hetero-substituted C1-C20alkyl, C4-C12cycloalkyl, C2-C20alkenyl, C2-C20alkynyl, C1-C20-alkoxy, C4-C12cycloalkoxy, C2-C20alkenoxy, C2-C20alkynoxy, C6-C12 aryl, C6-C12 aryloxy or C7-C13 aralkyl), or —C(═O)—NH—R1 in which R1 has its previous significance; and R3 is hydrogen, halogen, hydroxy, C1-C20alkyl, C4-C12cycloalkyl, C2-C20alkenyl, C2-C20alkynyl, C1-C20-alkoxy, C4-C12cycloalkoxy, C2-C20alkenoxy, C2-C20alkynoxy, phenyl, C7-C13 aralkyl or —N(R1)(R2) in which R1 and R2 have their previous significance, or R1 and R2 together form a C4-C12 membered ring. The new triphenyltriazine compounds have improved absorption spectrum characteristics and superior resistance to exposure to UV light, relative to known triphenyltriazine compounds.
摘要翻译：本发明提供具有下式的化合物：其中R是氢，羟基，卤素，C 1 -C 20烷基，C 4 -C 12环烷基，C 2 -C 20烯基，C 2 -C 20炔基，C 1 -C 20烷氧基，C 4 -C 12环烷氧基，C 2 -C 20链烯氧基，C 2 -C 20炔氧基或C 7 -C 13芳烷基; R 1和R 2独立地是氢，C 1 -C 20烷基，C 4 -C 12环烷基，C 7 -C 13芳烷基，-C（-O）-R 4（其中R 4是C 1 -C 20烷基，被1至6个氧原子间断的C 2 -C 20烷基， C 1 -C 20烷基，C 2 -C 20炔基，C 1 -C 20烷氧基，C 4 -C 12环烷氧基，C 2 -C 20烯烃氧基，C 2 -C 20炔氧基，C 6 -C 12芳基，C 6 -C 12芳氧基或C 7 -C 13 芳烷基）或-C（-O）-NH-R 1，其中R 1具有其先前的含义; 并且R 3是氢，卤素，羟基，C 1 -C 20烷基，C 4 -C 12环烷基，C 2 -C 20烯基，C 2 -C 20炔基，C 1 -C 20烷氧基，C 4 -C 12环烷氧基，C 2 -C 20链烯氧基，C 2 -C 20炔氧基，苯基，C 7 -C 13芳烷基或 -N（R 1）（R 2），其中R 1和R 2具有其先前的含义，或者R 1和R 2一起形成C 4 -C 12元环。相对于已知的三苯基三嗪化合物，新的三苯基三嗪化合物具有改善的吸收光谱特性和对UV光的暴露性优异的抗性。

10. 发明授权

US07425222B2 Process for improving the sun protection factor of cellulosic fibre material 失效
标题翻译：改善纤维素纤维材料防晒系数的方法
公开(公告)号：US07425222B2
公开(公告)日：2008-09-16
申请号：US10504945
申请日：2002-02-11
申请人： Georges Metzger , Jean-Jacques Donzé , Hans Kramer , Serge Hauger , Volker Papendick , Michael Milde , Ted Deisenroth , Rainer Hans Traber , Ullrich Menge , Hauke Rohwer
发明人： Georges Metzger , Jean-Jacques Donzé , Hans Kramer , Serge Hauger , Volker Papendick , Michael Milde , Ted Deisenroth , Rainer Hans Traber , Ullrich Menge , Hauke Rohwer
IPC分类号： D06L3/12
CPC分类号： D06M13/358 , C07D251/68 , D06M2200/25
摘要： A process for improving the sun protection factor (SPF) of cellulosic fibre materials and blends thereof, which comprises contacting said materials with at least one compound of the formula (1) in which M is hydrogen, an alkali metal atom, ammonium or a cation formed from an amine; R1 and R1′ independently of each other are hydrogen, hydroxy, optionally substituted alkyl, 4-morpholinyl, —NH—R3, —N(R3)2 or —O—R3, wherein R3is optionally substituted alkyl or optionally substituted aryl, R2 is a group of formula (2) wherein X is —O— or —NH— and R4 is C1-C4-alkyl which carries at least one hydrophilic substituent and R2′ has the meaning of R1 or R2.
摘要翻译：一种用于改善纤维素纤维材料及其共混物的防晒因子（SPF）的方法，其包括使所述材料与至少一种其中M为氢的式（1）化合物，碱金属原子，铵或阳离子由胺形成; R 1和R 2彼此独立地是氢，羟基，任选取代的烷基，4-吗啉基，-NH-R 3， -N（R 3 3）2或-OR 3，其中R 3是任选取代的烷基或任选取代的芳基，R 2是式（2）的基团，其中X是-O-或-NH-，R 4是C 1 - 携带至少一个亲水取代基的C 4 - 烷基和R 2'具有R 1或R 2的含义， SUB>。

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