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1. 发明授权

US6096843A Process for making high stereoregular polypropylenes 失效
标题翻译：制备高立体规则聚丙烯的方法
公开(公告)号：US6096843A
公开(公告)日：2000-08-01
申请号：US858498
申请日：1997-05-19
申请人： Jun Saito , Naoshi Kawamoto , Akiko Kageyama , Yoshiyuki Oogi , Kouichi Hatada
发明人： Jun Saito , Naoshi Kawamoto , Akiko Kageyama , Yoshiyuki Oogi , Kouichi Hatada
IPC分类号： C08F4/642 , C08F4/44 , C08F4/60 , C08F4/659 , C08F4/6592 , C08F8/00 , C08F10/06 , C08F110/06
CPC分类号： C08F110/06 , C08F4/65904 , C08F4/65912 , C08F4/65927 , Y10S526/943
摘要： A process for the production of a high stereoregular polypropylene wherein(a) an isotactic pentad (m m m m) is 0.950 to 0.995,(b) a syndiotactic pentad (r r r r) is 0 to 0.01,(c) a different bond due to 2,1- and 1,3-insertions of propylene monomer is 0 to 0.3 mol %,(d) an absence of a terminal double bond is confirmed,(e) a weight average molecular weight (Mw) is 50,000 to 1,000,000 and(f) a ratio (Mw/Mn) of the weight average molecular weight (Mw) to a number average molecular weight (Mn) is 1.5 to 3.8, (a) to (d) being determined from .sup.13 C NMR spectra, comprising polymerizing propylene in the presence of hydrogen using a catalyst comprising a chiral transition metal compound and an aluminoxane, the transition metal compound being represented by the formula of Q(C.sub.5 H.sub.4-m R.sup.1.sub.m) (C.sub.5 H.sub.4-n R.sup.2.sub.n)MXY wherein (C.sub.5 H.sub.4-m R.sup.1.sub.m) and (C.sub.5 H.sub.4-n R.sup.2.sub.n) represent a substituted cyclopentadienyl group; m and n are an integer of 1 to 3; R.sup.1 and R.sup.2 may be the same or different and each represents an alkyl group of 1 to 20 carbons; Q is a group capable of crosslinking (C.sub.5 H.sub.4-m R.sup.1.sub.m) and (C.sub.5 H.sub.4-n R.sup.2.sub.n) and represents a divalent, hydrocarbyl radical, an unsubstituted silylene group or a hydrocarbyl-substituted silylene group; M represents a transition metal selected from the group consisting of titanium, zirconium, and hafnium; X and Y may be the same or different and each represents a hydrogen, a halogen or a hydrocarbyl radical, and wherein said polymerization is performed by a slurry polymerization using an aliphatic hydrocarbon as a solvent or by a bulk polymerization using propylene as a solvent.
摘要翻译：一种制备高立构规则聚丙烯的方法，其中（a）全同立构五单元组（mmmm）为0.950-0.995，（b）间同立构五单元组（rrrr）为0至0.01，（c）由于2,1 - 和丙烯单体的1,3-插入为0〜0.3摩尔％，（d）不存在末端双键，（e）重均分子量（Mw）为50,000〜1,000,000，（f）a 重均分子量（Mw）与数均分子量（Mn）之比（Mw / Mn）为1.5至3.8，（a）至（d）由13 C NMR谱确定，包括在存在下聚合丙烯使用包含手性过渡金属化合物和铝氧烷的催化剂的氢，所述过渡金属化合物由下式Q（C5H4-mR1m）（C5H4-nR2n）MXY表示，其中（C5H4-mR1m）和（C5H4-nR2n）表示取代的环戊二烯基; m和n为1〜3的整数， R 1和R 2可以相同或不同，各自表示1〜20个碳的烷基; Q是能够交联的基团（C5H4-mR1m）和（C5H4-nR2n），代表二价烃基，未取代的亚甲硅烷基或烃基取代的亚甲硅烷基; M表示选自钛，锆和铪的过渡金属; X和Y可以相同或不同，各自表示氢，卤素或烃基，并且其中所述聚合通过使用脂族烃作为溶剂的淤浆聚合或通过使用丙烯作为溶剂的本体聚合进行。

2. 发明授权

US6156856A Propylene-ethylene copolymers processes for the production thereof and molded articles made therefrom 失效
标题翻译：丙烯 - 乙烯共聚物的制备方法和由其制成的模塑制品
公开(公告)号：US6156856A
公开(公告)日：2000-12-05
申请号：US142033
申请日：1998-09-01
申请人： Jun Saito , Naoshi Kawamoto , Akiko Kageyama , Kouichi Hatada , Yoshiyuki Oogi
发明人： Jun Saito , Naoshi Kawamoto , Akiko Kageyama , Kouichi Hatada , Yoshiyuki Oogi
IPC分类号： C08F4/642 , C08F4/659 , C08F210/06 , C08F210/16 , C08F4/06
CPC分类号： C08F210/16 , C08F210/06 , C08F4/65912
摘要： There are provided propylene-ethylene copolymers from which there are made molded articles having excellent heat resistance and films having both low temperature heat-sealing characteristics and stiffness, processes for the production thereof and molded articles. The propylene-ethylene copolymers contain 0.01-15 mol % of an ethylene unit and are characterized by that in the chain structure determined by NMR, triad (PEP), triad (EEE) and a ratio (N.sub..alpha..beta.) of all .alpha., .beta.-methylene carbons to all propylene units are in the specified range, a weight average molecular weight is 50,000-1,500,000 and a molecular weight distribution (Mw/Mn) is 1.2-3.8. The copolymers can be produced by copolymerizing ethylene and propylene in the presence of a catalyst in which the specified chiral transition metal compound (metallocene) and aluminoxane are combined.
摘要翻译： PCT No.PCT / JP97 / 00038 Sec。 371日期：1998年9月1日 102（e）1998年9月1日PCT PCT 1997年1月10日PCT公布。出版物WO98 / 30614 PCT 日期1998年7月16日提供丙烯 - 乙烯共聚物，其中制备具有优异耐热性的模制品和具有低温热封特性和刚度的薄膜，其制备方法和模塑制品。丙烯 - 乙烯共聚物含有0.01-15mol％的乙烯单元，其特征在于在通过NMR，三单元组（PEP），三单元组（EEE）和所有α，β的比率（Nαβ）测定的链结构中所有丙烯单元的亚甲基碳数均在规定范围内，重均分子量为50,000-1,500,000，分子量分布（Mw / Mn）为1.2-3.8。共聚物可以通过在其中组合指定的手性过渡金属化合物（金属茂）和铝氧烷的催化剂存在下共聚合乙烯和丙烯来制备。

3. 发明授权

US5874505A Polypropylene composition 失效
标题翻译：聚丙烯组成
公开(公告)号：US5874505A
公开(公告)日：1999-02-23
申请号：US980421
申请日：1997-11-28
申请人： Jun Saito , Naoshi Kawamoto , Akiko Kageyama , Kouichi Hatada , Yoshiyuki Oogi , Tsutomu Ushioda
发明人： Jun Saito , Naoshi Kawamoto , Akiko Kageyama , Kouichi Hatada , Yoshiyuki Oogi , Tsutomu Ushioda
IPC分类号： C08F4/58 , C08F4/64 , C08F110/06 , C08L23/10 , C08L23/16 , C08L23/12
CPC分类号： C08L23/10 , C08F110/06 , C08L23/16 , Y10S526/943
摘要： A polypropylene composition comprising 20 to 95% by weight of a stereoregular polypropylene characterized by the specified physical properties determined from .sup.13 C NMR spectra and 5 to 80% by weight of an .alpha.-olefin copolymer comprising 10 to 90% by weight of an .alpha.-olefin and 10 to 90% by weight of at least one of other .alpha.-olefins. The polypropylene composition demonstrates good balance of rigidity and impact resistance, high heat resistance and high toughness, when used as molding materials.
摘要翻译：一种聚丙烯组合物，其包含20至95重量％的立构规整聚丙烯，其特征在于由13 C NMR谱确定的特定物理性质和5至80重量％的包含10至90重量％的α-烯烃的α-烯烃共聚物和10至90重量％的至少一种其它α-烯烃。当用作成型材料时，聚丙烯组合物表现出良好的刚性和耐冲击性的平衡，高耐热性和高韧性。

4. 发明授权

US6153710A Preactivated catalyst for olefin (CO)polymer, catalyst for olefin (CO)polymerization, olefin (CO)polymer composition, and process for producing the same 失效
标题翻译：烯烃（CO）聚合物预活化催化剂，烯烃（CO）聚合催化剂，烯烃（CO））聚合物组合物及其制备方法
公开(公告)号：US6153710A
公开(公告)日：2000-11-28
申请号：US155189
申请日：1998-09-22
申请人： Jun Saito , Shingo Kikukawa , Tsutomu Ushioda , Akiko Kageyama , Mototake Tsutsui
发明人： Jun Saito , Shingo Kikukawa , Tsutomu Ushioda , Akiko Kageyama , Mototake Tsutsui
IPC分类号： C08F2/00 , C08F4/619 , C08F4/642 , C08F4/651 , C08F4/655 , C08F10/00 , C08F110/06 , C08F210/06 , C08L23/04 , C08L23/08 , C08L23/10 , C08L23/16 , B01J31/06
CPC分类号： C08F10/00 , C08L23/10 , C08F110/06 , C08F210/06 , C08F4/61904 , C08L23/04 , C08L23/0815 , C08L2314/06 , Y10S526/904 , Y10S526/943
摘要： An olefin (co)polymer composition comprising, as major components, (a) 0.01 to 5 parts by weight of an olefin (co)polymer having an intrinsic viscosity [.eta..sub.a ] as measured in 135.degree. C. tetralin of 15 to 100 dl/g and (b) 100 parts by weight of an olefin (co)polymer obtained by using a metallocene catalyst and having an intrinsic viscosity [.eta..sub.b ] as measured in 135.degree. C. tetralin of 0.2 to 10 dl/g. When polyethylene having a high degree of polymerization is produced before a so-called metallocene catalyst is used to polymerize, e.g., propylene in the presence of the polyethylene as a component of a catalyst composition, a polypropylene composition having a high melt tension and a high crystallization temperature is produced.
摘要翻译： PCT No.PCT / JP98 / 00534 Sec。 371日期：1998年9月22日 102（e）1998年9月22日日期PCT提交1998年2月9日PCT公布。第WO98 / 35997号公报日期1998年8月20日一种烯烃（共）聚合物组合物，其包含作为主要组分的（a）在135℃下测定的具有特性粘度[η]的烯属（共）聚合物0.01至5重量份的四氢化萘为15〜100dl / g，（b）100重量份通过使用金属茂催化剂得到的烯烃（共）聚合物，其在135℃四氢萘中的特性粘度为0.2〜10dl /G。在聚乙烯作为催化剂组合物的组分存在下，使用所谓的茂金属催化剂聚合例如丙烯之前，生产具有高聚合度的聚乙烯时，具有高熔体张力和高的聚丙烯组合物产生结晶温度。

5. 发明申请

US20080160347A1 Benzofluorene compound, emission materials and organic electroluminescent device 审中-公开
标题翻译：苯并芴化合物，发射材料和有机电致发光器件
公开(公告)号：US20080160347A1
公开(公告)日：2008-07-03
申请号：US11905737
申请日：2007-10-03
申请人： Guofang Wang , Akiko Kageyama , Toshihiro Koike , Manabu Uchida
发明人： Guofang Wang , Akiko Kageyama , Toshihiro Koike , Manabu Uchida
IPC分类号： C07C211/54 , C07C25/18 , H01J1/63 , B32B11/04 , C07C13/66
CPC分类号： H01L51/0039 , C07C13/66 , C07C2601/14 , C07C2603/26 , C07C2603/40 , C09K11/06 , C09K2211/1007 , C09K2211/1011 , H01L51/0054 , H01L51/0058 , H01L51/006 , H01L51/0071 , H01L51/0072 , H01L51/0081 , H01L51/0094 , H05B33/14 , Y10T428/31504
摘要： Provided is a benzofluorene compound which exhibits excellent performances when applied to an organic electroluminescent device.In the benzofluorene compound, a central five-membered ring in a benzofluorene skeleton is substituted with aryl, and a benzene ring condensed to the five-membered ring is substituted with aryl, diarylamino and the like.
摘要翻译：提供了当应用于有机电致发光器件时表现出优异性能的苯并芴化合物。在苯并芴化合物中，苯并芴骨架中的中心五元环被芳基取代，并且被五元环稠合的苯环被芳基，二芳基氨基等取代。

6. 发明申请

US20060110622A1 Organic electroluminescent device 审中-公开
标题翻译：有机电致发光器件
公开(公告)号：US20060110622A1
公开(公告)日：2006-05-25
申请号：US11196741
申请日：2005-08-04
申请人： Manabu Uchida , Guofang Wang , Akiko Kageyama , Kyung Hoon Lee , Jae Man Lee , Chun Gun Park
发明人： Manabu Uchida , Guofang Wang , Akiko Kageyama , Kyung Hoon Lee , Jae Man Lee , Chun Gun Park
IPC分类号： H01L51/54 , H05B33/12
CPC分类号： H01L51/0052 , H01L51/0058 , H01L51/0067 , H01L51/007 , H01L51/0072 , H01L51/0074 , H01L51/0081 , H01L51/0085 , H01L51/5096 , H01L2251/308
摘要： A phosphorescent device with high brightness and a long usable life including at least an emitting layer situated between a pair of electrodes and at least one hole blocking layer in direct contact with the emitting layer, wherein the phosphorescent device employs as the hole blocking layer, a compound which can be used as a blue luminescent host material.
摘要翻译：一种具有高亮度和长使用寿命的磷光装置，其包括位于一对电极之间的至少一个发光层和与发光层直接接触的至少一个空穴阻挡层，其中磷光装置用作空穴阻挡层，可用作蓝色发光主体材料的化合物。

7. 发明申请

US20110215310A1 ELECTRON TRANSPORT MATERIAL AND ORGANIC ELECTROLUMINESCENT DEVICE USING THE SAME 有权
标题翻译：电子运输材料和有机电致发光器件
公开(公告)号：US20110215310A1
公开(公告)日：2011-09-08
申请号：US13107105
申请日：2011-05-13
申请人： Youhei Ono , Hiroshi Yamada , Akiko Kageyama , Manabu Uchida
发明人： Youhei Ono , Hiroshi Yamada , Akiko Kageyama , Manabu Uchida
IPC分类号： H01L51/54 , C07D401/14 , C07D417/14 , C07D413/14
CPC分类号： H01L51/5048 , C07D213/22 , C07D213/53 , C07D401/14 , C07D413/14 , C07D417/14 , C09K11/06 , C09K2211/1029 , H01L51/0067 , H01L51/0069 , H01L51/0071 , H05B33/14 , Y10S428/917
摘要： A compound represented by the following Formula (1) is useful as an electron transport material of an organic EL device, and an organic EL device comprising the compound in the electron transport layer is long in life, and low in drive voltage: wherein G is an n-valent link, n is an integer of 2 to 4; R1 to R4 are each independently hydrogen, a monovalent group, or a free valency bonded with G, and R5 to R8 are each independently hydrogen or a monovalent group, and one of R1 to R4 is a free valency bonded with G; and n groups of 2,3′-bipyridyl may be the same or different with each other.
摘要翻译：由下式（1）表示的化合物可用作有机EL器件的电子传输材料，并且包含电子传输层中的化合物的有机EL器件寿命长，驱动电压低：其中G为 n价连接，n为2〜4的整数， R 1〜R 4各自独立地为氢，一价基团或与G键合的自由价，R 5〜R 8各自独立地为氢或一价基团，R 1〜R 4中的一个为与G键合的自由价; 并且n个2,3'-联吡啶基可以彼此相同或不同。

8. 发明授权

US07964293B2 Electron transport material and organic electroluminescent device using the same 有权
标题翻译：电子传输材料和使用其的有机电致发光器件
公开(公告)号：US07964293B2
公开(公告)日：2011-06-21
申请号：US11991454
申请日：2006-09-05
申请人： Youhei Ono , Hiroshi Yamada , Akiko Kageyama , Manabu Uchida
发明人： Youhei Ono , Hiroshi Yamada , Akiko Kageyama , Manabu Uchida
IPC分类号： H01J1/63
CPC分类号： H01L51/5048 , C07D213/22 , C07D213/53 , C07D401/14 , C07D413/14 , C07D417/14 , C09K11/06 , C09K2211/1029 , H01L51/0067 , H01L51/0069 , H01L51/0071 , H05B33/14 , Y10S428/917
摘要： A compound represented by the following Formula (1) is useful as an electron transport material of an organic EL device, and an organic EL device comprising the compound in the electron transport layer is long in life, and low in drive voltage: wherein G is an n-valent link, n is an integer of 2 to 4; R1 to R4 are each independently hydrogen, a monovalent group, or a free valency bonded with G, and R5 to R8 are each independently hydrogen or a monovalent group, and one of R1 to R4 is a free valency bonded with G; and n groups of 2,3′-bipyridyl may be the same or different with each other.
摘要翻译：由下式（1）表示的化合物可用作有机EL器件的电子传输材料，并且包含电子传输层中的化合物的有机EL器件寿命长，驱动电压低：其中G为 n价连接，n为2〜4的整数， R 1〜R 4各自独立地为氢，一价基团或与G键合的自由价，R 5〜R 8各自独立地为氢或一价基团，R 1〜R 4中的一个为与G键合的自由价; 并且n个2,3'-联吡啶基可以彼此相同或不同。

9. 发明授权

US08202633B2 Electron transport material and organic electroluminescent device using the same 有权
标题翻译：电子传输材料和使用其的有机电致发光器件
公开(公告)号：US08202633B2
公开(公告)日：2012-06-19
申请号：US13107105
申请日：2011-05-13
申请人： Youhei Ono , Hiroshi Yamada , Akiko Kageyama , Manabu Uchida
发明人： Youhei Ono , Hiroshi Yamada , Akiko Kageyama , Manabu Uchida
IPC分类号： H01L51/54
CPC分类号： H01L51/5048 , C07D213/22 , C07D213/53 , C07D401/14 , C07D413/14 , C07D417/14 , C09K11/06 , C09K2211/1029 , H01L51/0067 , H01L51/0069 , H01L51/0071 , H05B33/14 , Y10S428/917
摘要： A compound represented by the following Formula (1) is useful as an electron transport material of an organic EL device, and an organic EL device comprising the compound in the electron transport layer is long in life, and low in drive voltage: wherein G is an n-valent link, n is an integer of 2 to 4; R1 to R4 are each independently hydrogen, a monovalent group, or a free valency bonded with G, and R5 to R8 are each independently hydrogen or a monovalent group, and one of R1 to R4 is a free valency bonded with G; and n groups of 2,3′-bipyridyl may be the same or different with each other.
摘要翻译：由下式（1）表示的化合物可用作有机EL器件的电子传输材料，并且包含电子传输层中的化合物的有机EL器件寿命长，驱动电压低：其中G为 n价连接，n为2〜4的整数， R 1〜R 4各自独立地为氢，一价基团或与G键合的自由价，R 5〜R 8各自独立地为氢或一价基团，R 1〜R 4中的一个为与G键合的自由价; 并且n个2,3'-联吡啶基可以彼此相同或不同。

10. 发明申请

US20090134780A1 Electron transport material and organic electroluminescent device using the same 有权
标题翻译：电子传输材料和使用其的有机电致发光器件
公开(公告)号：US20090134780A1
公开(公告)日：2009-05-28
申请号：US11991454
申请日：2006-09-05
申请人： Youhei Ono , Hiroshi Yamada , Akiko Kageyama , Manabu Uchida
发明人： Youhei Ono , Hiroshi Yamada , Akiko Kageyama , Manabu Uchida
IPC分类号： H01J1/63 , C07D401/04 , C07D401/14
CPC分类号： H01L51/5048 , C07D213/22 , C07D213/53 , C07D401/14 , C07D413/14 , C07D417/14 , C09K11/06 , C09K2211/1029 , H01L51/0067 , H01L51/0069 , H01L51/0071 , H05B33/14 , Y10S428/917
摘要： A compound represented by the following Formula (1) is useful as an electron transport material of an organic EL device, and an organic EL device comprising the compound in the electron transport layer is long in life, and low in drive voltage: wherein G is an n-valent link, n is an integer of 2 to 4; R1 to R4 are each independently hydrogen, a monovalent group, or a free valency bonded with G, and R5 to R8 are each independently hydrogen or a monovalent group, and one of R1 to R4 is a free valency bonded with G; and n groups of 2,3′-bipyridyl may be the same or different with each other.
摘要翻译：由下式（1）表示的化合物可用作有机EL器件的电子传输材料，并且包含电子传输层中的化合物的有机EL器件寿命长，驱动电压低：其中G为 n价连接，n为2〜4的整数， R 1〜R 4各自独立地为氢，一价基团或与G键合的自由价，R 5〜R 8各自独立地为氢或一价基团，R 1〜R 4中的一个为与G键合的自由价; 并且n个2,3'-联吡啶基可以彼此相同或不同。

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