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1. 发明授权

US08097383B2 Electrolyte material for polymer electrolyte fuel cells, electrolyte membrane and membrane/electrode assembly 有权
标题翻译：用于聚合物电解质燃料电池，电解质膜和膜/电极组件的电解质材料
公开(公告)号：US08097383B2
公开(公告)日：2012-01-17
申请号：US12010589
申请日：2008-01-28
申请人： Isamu Kaneko , Tetsuji Shimohira , Atsushi Watakabe , Seigo Kotera , Satoru Hommura , Koichi Murata , Jyunichi Tayanagi , Susumu Saito
发明人： Isamu Kaneko , Tetsuji Shimohira , Atsushi Watakabe , Seigo Kotera , Satoru Hommura , Koichi Murata , Jyunichi Tayanagi , Susumu Saito
IPC分类号： H01M8/10
CPC分类号： C08J5/225 , C08J2327/12 , H01M8/1004 , H01M8/1023 , H01M8/1039 , H01M2300/0082
摘要： To provide a polymer electrolyte material for polymer electrolyte fuel cells, which is an electrolyte material having a high ion exchange capacity and a low resistance, and which has a higher softening temperature than a conventional electrolyte material.An electrolyte material for polymer electrolyte fuel cells, which is made of a polymer containing repeating units based on a fluoromonomer having a radical polymerization reactivity, wherein the repeating units contain, in their side chains, a structure having ionic groups represented in the following formula (α) (provided that in the formula, each of Q1 and Q2 which are independent of each other, is a single bond or a perfluoroalkylene group that may have an etheric oxygen atom, provided that they are not single bonds at the same time, Rf1 is a perfluoroalkyl group which may have an etheric oxygen atom, and X is an oxygen atom, a nitrogen atom or a carbon atom, provided that when X is an oxygen atom, a=0, when X is a nitrogen atom, a=1, and when X is a carbon atom, a=2, and Y is a fluorine atom or a monovalent perfluoro organic group).
摘要翻译：本发明提供一种高分子电解质燃料电池用聚合物电解质材料，该高分子电解质材料是具有高离子交换能力和低电阻的电解质材料，其软化温度高于常规电解质材料。一种用于聚合物电解质燃料电池的电解质材料，其由含有具有自由基聚合反应性的含氟单体的重复单元的聚合物制成，其中重复单元在其侧链中包含具有下式表示的离子基团的结构（ α）（条件是在式中，Q1和Q2各自独立地为可以具有醚性氧原子的单键或全氟亚烷基，条件是它们不同时为单键，Rf1 是可以具有醚性氧原子的全氟烷基，X是氧原子，氮原子或碳原子，条件是当X是氧原子时a = 0，当X是氮原子时，a = 1 ，当X为碳原子时，a = 2，Y为氟原子或1价全氟有机基团）。

2. 发明申请

US20080138685A1 Electrolyte material for polymer electrolyte fuel cells, electrolyte membrane and membrane/electrode assembly 有权
标题翻译：用于聚合物电解质燃料电池，电解质膜和膜/电极组件的电解质材料
公开(公告)号：US20080138685A1
公开(公告)日：2008-06-12
申请号：US12010589
申请日：2008-01-28
申请人： Isamu Kaneko , Tetsuji Shimohira , Atsushi Watakabe , Seigo Kotera , Satoru Hommura , Koichi Murata , Jyunichi Tayanagi , Susumu Saito
发明人： Isamu Kaneko , Tetsuji Shimohira , Atsushi Watakabe , Seigo Kotera , Satoru Hommura , Koichi Murata , Jyunichi Tayanagi , Susumu Saito
IPC分类号： H01M8/10 , C08J5/20
CPC分类号： C08J5/225 , C08J2327/12 , H01M8/1004 , H01M8/1023 , H01M8/1039 , H01M2300/0082
摘要： To provide a polymer electrolyte material for polymer electrolyte fuel cells, which is an electrolyte material having a high ion exchange capacity and a low resistance, and which has a higher softening temperature than a conventional electrolyte material.An electrolyte material for polymer electrolyte fuel cells, which is made of a polymer containing repeating units based on a fluoromonomer having a radical polymerization reactivity, wherein the repeating units contain, in their side chains, a structure having ionic groups represented in the following formula (α) (provided that in the formula, each of Q1 and Q2 which are independent of each other, is a single bond or a perfluoroalkylene group that may have an etheric oxygen atom, provided that they are not single bonds at the same time, Rf1 is a perfluoroalkyl group which may have an etheric oxygen atom, and X is an oxygen atom, a nitrogen atom or a carbon atom, provided that when X is an oxygen atom, a=0, when X is a nitrogen atom, a=1, and when X is a carbon atom, a=2, and Y is a fluorine atom or a monovalent perfluoro organic group).
摘要翻译：本发明提供一种高分子电解质燃料电池用聚合物电解质材料，该高分子电解质材料是具有高离子交换能力和低电阻的电解质材料，其软化温度高于常规电解质材料。一种用于聚合物电解质燃料电池的电解质材料，其由含有具有自由基聚合反应性的含氟单体的重复单元的聚合物制成，其中重复单元在其侧链中包含具有下式表示的离子基团的结构（ α）（条件是在该式中，彼此独立的Q 1和Q 2各自是单键或可具有醚的全氟亚烷基氧原子，条件是它们不是同时是单键，R f1是可以具有醚性氧原子的全氟烷基，X是氧原子，氮原子或碳原子条件是当X是氧原子时，a = 0，当X为氮原子时a = 1，当X为碳原子时a = 2，Y为氟原子或1价全氟有机基团）。

3. 发明申请

US20090110967A1 ELECTROLYTE MEMBRANE FOR POLYMER ELECTROLYTE FUEL CELL, PROCESS FOR ITS PRODUCTION, MEMBRANE/ELECTRODE ASSEMBLY FOR POLYMER ELECTROLYTE FUEL CELL AND METHOD OF OPERATING POLYMER ELECTROLYTE FUEL CELL 审中-公开
标题翻译：聚合物电解质燃料电池用电解质膜及其制造方法，聚合物电解质燃料电池用膜/电极组件及聚合物电解质燃料电池的运行方法
公开(公告)号：US20090110967A1
公开(公告)日：2009-04-30
申请号：US11931934
申请日：2007-10-31
申请人： Satoru Hommura , Atsushi Watakabe , Jyunichi Tayanagi , Susumu Saito , Tetsuji Shimohira , Eiji Endoh
发明人： Satoru Hommura , Atsushi Watakabe , Jyunichi Tayanagi , Susumu Saito , Tetsuji Shimohira , Eiji Endoh
IPC分类号： H01M8/10
CPC分类号： C08J5/2237 , C08J5/225 , C08J2327/18 , H01B1/122 , H01M8/1023 , H01M8/1039 , H01M8/1051 , H01M8/1083 , H01M8/1088 , H01M2008/1095 , H01M2300/0082 , Y02P70/56
摘要： An electrolyte membrane for a polymer electrolyte fuel cell, which comprises an ion exchange membrane made of a fluoropolymer having a softening temperature of at least 90° C. and having acidic groups, and contains cerium atoms.
摘要翻译：一种用于固体高分子型燃料电池的电解质膜，其包含由软化温度为90℃以上且具有酸性基团的含氟聚合物构成的离子交换膜，并含有铈原子。

4. 发明申请

US20090004527A1 POLYMER, POLYMER ELECTROLYTE MEMBRANE FOR POLYMER ELECTROLYTE FUEL CELL, AND MEMBRANE/ELECTRODE ASSEMBLY 有权
标题翻译：聚合物聚合物电解质膜聚合物电解质膜和膜/电极组件
公开(公告)号：US20090004527A1
公开(公告)日：2009-01-01
申请号：US12019355
申请日：2008-01-24
申请人： Tetsuji Shimohira , Kazuo Hamazaki , Susumu Saito , Satoru Hommura , Seigo Kotera
发明人： Tetsuji Shimohira , Kazuo Hamazaki , Susumu Saito , Satoru Hommura , Seigo Kotera
IPC分类号： H01M8/10 , C08G75/20
CPC分类号： H01B1/122 , C08F20/22 , C08F20/38 , C08F214/18 , C08J5/2237 , C08J2327/12 , H01M8/1023 , H01M8/1039 , H01M2300/0082
摘要： A polymer electrolyte membrane made of a polymer has a low electrical resistance, high heat resistance and is strong against repeats of swelling and shrinkage. Thus, a membrane/electrode assembly for polymer electrolyte fuel cells having high power generation performance and excellent in durability can be provided.For a polymer electrolyte membrane 15 or for a catalyst layer 11 constituting electrodes 13 and 14, a polymer comprising units (U1) and units (U2) is used: Q1, Q2, Q3: a perfluoroalkylene group which may have —O— or the like; Rf1, Rf2: a perfluoroalkyl group which may have —O—; X1, X2: an oxygen atom or the like; a, b: 0 or the like; Y1, Y2: a fluorine atom or a monovalent perfluoroorganic group; and s, t: 0 to 1.
摘要翻译：由聚合物制成的聚合物电解质膜具有低电阻，高耐热性，并且强烈地反映了膨胀和收缩的重复。因此，可以提供具有高发电性能和优异的耐久性的用于聚合物电解质燃料电池的膜/电极组件。对于构成电极13和14的高分子电解质膜15或催化剂层11，使用包含单元（U1）和单元（U2）的聚合物：Q1，Q2，Q3：可具有-O-或喜欢; Rf1，Rf2：可具有-O-的全氟烷基; X1，X2：氧原子等; a，b：0等; Y1，Y2：氟原子或一价全氟有机基团; 和s，t：0到1。

5. 发明申请

US20090291345A1 MEMBRANE/ELECTRODE ASSEMBLY FOR POLYMER ELECTROLYTE FUEL CELLS, POLYMER ELECTROLYTE FUEL CELL, AND PROCESSES FOR THEIR PRODUCTION 有权
标题翻译：聚合物电解质燃料电池的膜/电极组件，聚合物电解质燃料电池及其生产方法
公开(公告)号：US20090291345A1
公开(公告)日：2009-11-26
申请号：US12533667
申请日：2009-07-31
申请人： Satoru Hommura , Shinji Kinoshita , Hiroshi Shimoda , Susumu Saito , Seigo Kotera , Tetsuji Shimohira , Hideki Nakagawa
发明人： Satoru Hommura , Shinji Kinoshita , Hiroshi Shimoda , Susumu Saito , Seigo Kotera , Tetsuji Shimohira , Hideki Nakagawa
IPC分类号： H01M8/10 , H01M4/82
CPC分类号： H01M8/1004 , H01M4/8605 , H01M4/8642 , H01M4/8657 , H01M4/8807 , H01M4/881 , H01M4/8828 , H01M4/926 , H01M8/1023 , H01M8/1039 , H01M2004/8689 , H01M2008/1095 , H01M2300/0082 , Y02P70/56 , Y10T29/49114 , Y10T29/49115
摘要： To provide a membrane/electrode assembly for polymer electrolyte fuel cells, a polymer electrolyte fuel cell and processes for their production, which make it possible to stably exhibit a high power generation performance in various environments. A membrane/electrode assembly for polymer electrolyte fuel cells, which comprises a first electrode having a first catalyst layer and a first gas diffusion layer, a second electrode having a second catalyst layer and a second gas diffusion layer, and a polymer electrolyte membrane disposed between the first electrode and the second electrode, wherein the 90° peel strength at least one of the interface between the first electrode and the polymer electrolyte membrane and the interface between the second electrode and the polymer electrolyte membrane is at least 0.03 N/cm.
摘要翻译：为了提供用于聚合物电解质燃料电池的膜/电极组件，聚合物电解质燃料电池及其生产方法，这使得可以在各种环境中稳定地显示高发电性能。一种用于聚合物电解质燃料电池的膜/电极组件，其包括具有第一催化剂层和第一气体扩散层的第一电极，具有第二催化剂层和第二气体扩散层的第二电极，以及设置在第一电极和第二电极，其中第一电极和聚合物电解质膜之间的界面中的至少一个与第二电极和聚合物电解质膜之间的界面的90°剥离强度为至少0.03N / cm。

6. 发明授权

US08017257B2 Polymer, polymer electrolyte membrane for polymer electrolyte fuel cell, and membrane/electrode assembly 有权
标题翻译：用于聚合物电解质燃料电池的聚合物，聚合物电解质膜和膜/电极组件
公开(公告)号：US08017257B2
公开(公告)日：2011-09-13
申请号：US12019355
申请日：2008-01-24
申请人： Tetsuji Shimohira , Kazuo Hamazaki , Susumu Saito , Satoru Hommura , Seigo Kotera
发明人： Tetsuji Shimohira , Kazuo Hamazaki , Susumu Saito , Satoru Hommura , Seigo Kotera
IPC分类号： H01M8/10
CPC分类号： H01B1/122 , C08F20/22 , C08F20/38 , C08F214/18 , C08J5/2237 , C08J2327/12 , H01M8/1023 , H01M8/1039 , H01M2300/0082
摘要： A polymer electrolyte membrane made of a polymer having a low electrical resistance, high heat resistance and is strong against repeats of swelling and shrinkage. Thus, a membrane/electrode assembly for polymer electrolyte fuel cells having high power generation performance and excellent in durability can be provided. The polymer has repeating units represented by the following formula (U1 ) and repeating units represented by the following formula (U2):
摘要翻译：由聚合物制成的聚合物电解质膜，具有低电阻，高耐热性，并且强烈地反映了膨胀和收缩的重复。因此，可以提供具有高发电性能和优异的耐久性的用于聚合物电解质燃料电池的膜/电极组件。聚合物具有由下式（U1）表示的重复单元和由下式（U2）表示的重复单元：

7. 发明授权

US08673517B2 Polymer electrolyte membrane composed of a fluorinated proton conductive polymer and a fluorinated reinforcing material 有权
标题翻译：由氟化质子导电聚合物和氟化增强材料构成的聚合物电解质膜
公开(公告)号：US08673517B2
公开(公告)日：2014-03-18
申请号：US12483315
申请日：2009-06-12
申请人： Seigo Kotera , Tetsuji Shimohira , Satoru Hommura , Susumu Saito
发明人： Seigo Kotera , Tetsuji Shimohira , Satoru Hommura , Susumu Saito
IPC分类号： H01M8/10
CPC分类号： H01B1/122 , H01M8/1023 , H01M8/1039 , H01M8/106 , H01M8/1067
摘要： To provide a polymer electrolyte membrane for polymer electrolyte fuel cells having high mechanical strength and excellent dimensional stability when it contains water even when it is made thin and the concentration of ionic groups is increased so as to reduce the electrical resistance, and a membrane/electrode assembly providing high output and having excellent durability.
摘要翻译：为了提供具有高机械强度和优异的尺寸稳定性的高分子电解质膜的高分子电解质膜，即使在含有水的情况下也含有水分，并且提高离子基团的浓度以降低电阻，并且提供膜/电极组装提供高输出并具有优异的耐久性。

8. 发明申请

US20100009236A1 POLYMER ELECTROLYTE MEMBRANE FOR POLYMER ELECTROLYTE FUEL CELLS, AND MEMBRANE/ELECTRODE ASSEMBLY 有权
标题翻译：用于聚合物电解质燃料电池的聚合物电解质膜和膜/电极组件
公开(公告)号：US20100009236A1
公开(公告)日：2010-01-14
申请号：US12483315
申请日：2009-06-12
申请人： Seigo Kotera , Tetsuji Shimohira , Satoru Hommura , Susumu Saito
发明人： Seigo Kotera , Tetsuji Shimohira , Satoru Hommura , Susumu Saito
IPC分类号： H01M8/10
CPC分类号： H01B1/122 , H01M8/1023 , H01M8/1039 , H01M8/106 , H01M8/1067
摘要： To provide a polymer electrolyte membrane for polymer electrolyte fuel cells having high mechanical strength and excellent dimensional stability when it contains water even when it is made thin and the concentration of ionic groups is increased so as to reduce the electrical resistance, and a membrane/electrode assembly providing high output and having excellent durability.A polymer electrolyte membrane 15, which comprises a fluorinated proton conductive polymer (i) having a proton conductivity of at least 0.06 S/cm in an atmosphere at a temperature of 80° C. under a relative humidity of 50%, and (ii) having repeating units based on a vinyl ether type monomer with a mass (equivalent weight) of at most 400 per 1 mol of ionic groups and repeating units based on a perfluoromonomer (except for the above vinyl ether type monomer) and a fluorinated reinforcing material; and a membrane/electrode assembly 10 comprising the polymer electrolyte membrane 15 interposed between an anode 13 and a cathode 14.
摘要翻译：为了提供具有高机械强度和优异的尺寸稳定性的高分子电解质膜的高分子电解质膜，即使在含有水的情况下也含有水分，并且提高离子基团的浓度以降低电阻，并且提供膜/电极组装提供高输出并具有优异的耐久性。在相对湿度为50％的温度为80℃的气氛中，包含质子传导率为0.06S / cm以上的质子传导性聚合物（i）的高分子电解质膜15，（ii）具有基于每1mol离子基质量（当量）至多400个/基于全氟单体（除上述乙烯基醚型单体除外）和氟化增强材料的重复单元）的乙烯基醚型单体的重复单元; 以及包含介于阳极13和阴极14之间的聚合物电解质膜15的膜/电极组件10。

9. 发明申请

US20080193821A1 POLYMER, POLYMER ELECTROLYTE MEMBRANE FOR POLYMER ELECTROLYTE FUEL CELL, AND MEMBRANE/ELECTRODE ASSEMBLY 有权
标题翻译：聚合物聚合物电解质膜聚合物电解质膜和膜/电极组件
公开(公告)号：US20080193821A1
公开(公告)日：2008-08-14
申请号：US11771414
申请日：2007-06-29
申请人： Tetsuji Shimohira , Kazuo Hamazaki , Susumu Saito , Satoru Hommura , Seigo Kotera
发明人： Tetsuji Shimohira , Kazuo Hamazaki , Susumu Saito , Satoru Hommura , Seigo Kotera
IPC分类号： H01M8/10 , C08F12/30 , C08J5/22
CPC分类号： C08J5/225 , C08J2327/12 , H01M8/1007 , H01M8/1023 , H01M8/1039 , H01M8/1067 , H01M2300/0082
摘要： A polymer electrolyte membrane made of a polymer has a low electrical resistance, high heat resistance and is strong against repeats of swelling and shrinkage. Thus, a membrane/electrode assembly for polymer electrolyte fuel cells having high power generation performance and excellent in durability can be provided.For a polymer electrolyte membrane 15 or for a catalyst layer 11 constituting electrodes 13 and 14, a polymer comprising units (U1) and units (U2) is used: Q1, Q2: a perfluoroalkylene group which may have —O— or the like; Rf1, Rf2: a perfluoroalkyl group which may have —O—; X: an oxygen atom or the like; a: 0 or the like; Y, Z: a fluorine atom, or a monovalent perfluoroorganic group such as —CF3; S: 0 to 1; and t: 0 to 3.
摘要翻译：由聚合物制成的聚合物电解质膜具有低电阻，高耐热性，并且强烈地反映了膨胀和收缩的重复。因此，可以提供具有高发电性能和优异的耐久性的用于聚合物电解质燃料电池的膜/电极组件。对于构成电极13和14的聚合物电解质膜15或催化剂层11，使用包含单元（U1）和单元（U2）的聚合物：Q 1，Q 2， SUP>：可具有-O-等的全氟亚烷基; R f2，R f2，可以具有-O-的全氟烷基; X：氧原子等; a：0等; Y，Z：氟原子，或一价全氟有机基团如-CF 3 O; S：0到1; 和t：0到3。

10. 发明授权

US08124295B2 Polymer, polymer electrolyte membrane for polymer electrolyte fuel cell, and membrane/electrode assembly 有权
标题翻译：用于聚合物电解质燃料电池的聚合物，聚合物电解质膜和膜/电极组件
公开(公告)号：US08124295B2
公开(公告)日：2012-02-28
申请号：US11771414
申请日：2007-06-29
申请人： Tetsuji Shimohira , Kazuo Hamazaki , Susumu Saito , Satoru Hommura , Seigo Kotera
发明人： Tetsuji Shimohira , Kazuo Hamazaki , Susumu Saito , Satoru Hommura , Seigo Kotera
IPC分类号： H01M8/10
CPC分类号： C08J5/225 , C08J2327/12 , H01M8/1007 , H01M8/1023 , H01M8/1039 , H01M8/1067 , H01M2300/0082
摘要： A polymer electrolyte membrane made of a polymer has a low electrical resistance, high heat resistance and is strong against repeats of swelling and shrinkage. Thus, a membrane/electrode assembly for polymer electrolyte fuel cells having high power generation performance and excellent in durability can be provided.For a polymer electrolyte membrane 15 or for a catalyst layer 11 constituting electrodes 13 and 14, a polymer comprising units (U1) and units (U2) is used: Q1, Q2: a perfluoroalkylene group which may have —O— or the like; Rf1, Rf2: a perfluoroalkyl group which may have —O—; X: an oxygen atom or the like; a: 0 or the like; Y, Z: a fluorine atom, or a monovalent perfluoroorganic group such as —CF3; S: 0 to 1; and t: 0 to 3.
摘要翻译：由聚合物制成的聚合物电解质膜具有低电阻，高耐热性，并且强烈地反映了膨胀和收缩的重复。因此，可以提供具有高发电性能和优异的耐久性的用于聚合物电解质燃料电池的膜/电极组件。对于构成电极13和14的高分子电解质膜15或催化剂层11，使用包含单元（U1）和单元（U2）的聚合物：Q1，Q2：可具有-O-等的全氟亚烷基; Rf1，Rf2：可具有-O-的全氟烷基; X：氧原子等; a：0等; Y，Z：氟原子，或一价全氟有机基团如-CF 3; S：0到1; 和t：0到3。

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