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1. 发明授权

US5089565A Process for the preparation of curable binder combinations, the combinations obtainable by this process and the use thereof 失效
标题翻译：制备可固化粘合剂组合的方法，本方法可获得的组合及其用途
公开(公告)号：US5089565A
公开(公告)日：1992-02-18
申请号：US358448
申请日：1989-05-30
申请人： Harald Blum , Christian Wamprecht , Josef Pedain , Michael Sonntag
发明人： Harald Blum , Christian Wamprecht , Josef Pedain , Michael Sonntag
IPC分类号： C08L35/00 , C08F20/02 , C08F22/06 , C08K5/35 , C09D133/02 , C09D135/00
CPC分类号： C09D135/00 , C08K5/35
摘要： A moisture-curing binder composition useful in paints and other coating compositions is prepared by mixing or mixing with spontaneous reaction in the absence of moistureA) 30 to 99 parts by weight of at least one compound containing at least two intramolecular carboxylic anhydride groups andB) 1 to 70 parts by weight of organic compounds having blocked amino groups, wherein B)comprises organic compounds containing hydrogen atoms which are reactive to acid anhydride groups and containing bicyclic amide acetal or bicyclic amide groups or both, wherein the ratios of the amounts of the individual components are chosen such that, by taking into account the addition reaction which occurs spontaneously between components A) and B) in the absence of moisture, in the resulting mixture 0.25 to 50 anhydride groups are present per bicyclic amide acetal and bicyclic amide aminal group.
摘要翻译：用于油漆和其他涂料组合物的湿固化粘合剂组合物通过在不存在水分的情况下与自发反应混合或混合制备A）30至99重量份的至少一种含有至少两个分子内羧酸酐基团的化合物和B ）1至70重量份具有封闭氨基的有机化合物，其中B）包含含有与酸酐基团反应并含有双环酰胺缩醛或双环酰胺基团或两者的氢原子的有机化合物，其中，选择各个组分使得通过考虑到在不存在水分的情况下在组分A）和B）之间自发发生的加成反应，在所得混合物中，每双酰胺缩醛和双环酰胺缩醛存在0.25至50个酸酐基团组。

2. 发明授权

US4975493A Process for the production of moisture-hardening binder compositions and their use 失效
标题翻译：湿固化粘合剂组合物的生产方法及其用途
公开(公告)号：US4975493A
公开(公告)日：1990-12-04
申请号：US223803
申请日：1988-07-25
申请人： Harald Blum , Josef Pedain , Christian Wamprecht , Michael Sonntag
发明人： Harald Blum , Josef Pedain , Christian Wamprecht , Michael Sonntag
IPC分类号： C08L23/00 , C08F8/32 , C08K5/35 , C09D133/04 , C09D135/00
CPC分类号： C08K5/35 , C08F8/32 , C09D135/00 , C08F2800/20
摘要： A moisture-hardening binder composition for lacquer of coating compositions is prepared by mixing(A) 50 to 97 parts by weight of copolymers of maleic anhydride with olefinically unsaturated monomers, said copolymers containing succinic anhydride units and having molecular weights Mw of 1,500 to 75,000 with(B) 3 to 50 parts by weight oxazolanes having a molecular weight Mw of 87 to 10,000,the quantitative ratios of (A) to (B) being such that the composition contains 0.25 to 10 anhydride groups for every oxazolane group,wherein component (A) consists essentially of copolymers of(a) 4.5 to 45 parts by weight of maleic anhydride,(b) 5 to 80 parts by weight of monomers of the formulae ##STR1## or both, and (c) 15 to 92 parts by weight of monomers of the formula ##STR2## wherein, R.sub.1 and R.sub.4 is each, independent of the other, an aliphatic or cycloaliphatic C.sub.1 -C.sub.12 hydrocarbon radical with or without oxygen, sulfur or nitrogen as a heteratom, R.sub.2 is hydrogen, methyl, ethyl, chlorine or fluorine,R.sub.3 is a C.sub.2 -C.sub.15 aliphatic hydrocarbon radical, a C.sub.5 -C.sub.10 cycloaliphatic hydrocarbon radical, a C.sub.7 -C.sub.18 araliphatic hydrocarbon radical, a C.sub.6 -C.sub.12 aromatic hydrocarbon radical, chlorine, fluorine, nitrile or a C.sub.2 -C.sub.18 hydrocarbon radical containing one or more heteroatoms selected from the group consisting of oxygen, sulfur and nitrogen in the form of ether, ester, amide, urethane, urea, thioester, oxirane, ketone, lactam or lactone groups.
摘要翻译：通过混合（A）50至97重量份的马来酸酐与烯属不饱和单体的共聚物，所述共聚物含有琥珀酸酐单元并具有1500至75,000的分子量Mw，制备用于涂料组合物漆的湿润硬化粘合剂组合物，（B）3〜50重量份的分子量Mw为87〜10,000的恶唑烷，（A）〜（B）的定量比为每个恶唑烷基组成含有0.25〜10个酸酐基，其中组分（ A）基本上由（a）4.5至45重量份马来酸酐的共聚物组成，（b）5-80重量份式（IMAGE）或两者的单体，和（c）15至92重量份具有下式的单体：其中，R 1和R 4各自独立地为具有或不具有氧，硫或氮作为杂原子的脂族或脂环族C 1 -C 12烃基，R 2为氢，甲基，乙基，氯或氟 ne，R 3是C 2 -C 15脂族烃基，C 5 -C 10脂环族烃基，C 7 -C 18芳脂族烃基，C 6 -C 12芳烃基，氯，氟，腈或含有一个的C 2 -C 18烃基或更多选自醚，酯，酰胺，氨基甲酸酯，脲，硫酯，环氧乙烷，酮，内酰胺或内酯基团的氧，硫和氮的杂原子。

3. 发明授权

US4945137A Binder combinations and a process for the production of flat materials 失效
标题翻译：粘合剂组合和生产平板材料的工艺
公开(公告)号：US4945137A
公开(公告)日：1990-07-31
申请号：US415863
申请日：1989-10-02
申请人： Walter Schafer , Hans Rudolph , Rolf Dhein , Hanns-Peter Muller , Michael Sonntag , Christian Wamprecht , Harald Blum , Walter Krauss
发明人： Walter Schafer , Hans Rudolph , Rolf Dhein , Hanns-Peter Muller , Michael Sonntag , Christian Wamprecht , Harald Blum , Walter Krauss
IPC分类号： C08L33/06 , C03C25/10 , C08F8/32 , C08K3/28 , C08K5/17 , C08K5/353 , C08K13/02 , C08L33/04 , C08L35/00 , C08L101/00 , C08L101/08 , C09D7/12 , C09D201/08
CPC分类号： C08K5/17 , C08F8/32 , C08K3/28 , C08K5/353
摘要： A binder for a coating composition is a combination of(a) polymers containing intramolecular carboxylic anhydride groups and having an average molecular weight of from 500 to 25,000 and(b) organic compounds containing 4,5-dihydrooxazole groups in a quantity corresponding to an equivalent ratio of carboxylic anhydride groups to 4,5-dihydrooxazole groups of from 0.5:1 to 2:1, and contains from 0.005 to 5% by weight, based on the weight of components (a) and (b), of ammonia, a primary amine or secondary amine.
摘要翻译：用于涂料组合物的粘合剂是（a）含有分子内羧酸酐基团并且平均分子量为500至25,000的聚合物和（b）含有相当于当量的4,5-二氢恶唑基团的有机化合物的组合羧酸酐基团与4,5-二氢恶唑基团的比例为0.5:1至2:1，并且基于组分（a）和（b）的重量，含有0.005至5重量％的氨，伯胺或仲胺。

4. 发明授权

US4727128A Diisocyanates containing urethane groups, a process for their preparation and their use as binders or binder component in polyurethane lacquers 失效
标题翻译：含有氨基甲酸酯基团的二异氰酸酯，其制备方法以及它们在聚氨酯漆中作为粘合剂或粘合剂组分的用途
公开(公告)号：US4727128A
公开(公告)日：1988-02-23
申请号：US820057
申请日：1986-01-21
申请人： Josef Pedain , Bernd Riberi , Michael Sonntag , Klaus Konig , Jurg Frohlich
发明人： Josef Pedain , Bernd Riberi , Michael Sonntag , Klaus Konig , Jurg Frohlich
IPC分类号： C08G18/00 , C07C67/00 , C07C239/00 , C07C269/02 , C07C271/06 , C07C271/20 , C08G18/10 , C08G18/32 , C08G18/73 , C08G18/80 , C09D175/00 , C09D175/04 , C07C125/07 , C08G18/78
CPC分类号： C08G18/8009
摘要： The present invention is directed to a process for the preparation of a diisocyanate by reacting a diisocyanate with 2,2,4-trimethyl-pentanediol-(1,3) or reaction products of this diol which contain either ether or ester groups and optionally other diols or triols. The present invention is additionally directed to the diisocyanates produced by this process and to their use in one-component and two-component coating compositions.
摘要翻译：本发明涉及通过使二异氰酸酯与2,2,4-三甲基戊二醇 - （1,3）或该二醇的含有醚基或酯基的任意其它的二醇的反应产物进行反应来制备二异氰酸酯的方法二醇或三醇。本发明另外涉及通过该方法制备的二异氰酸酯及其在单组分和双组分涂料组合物中的用途。

5. 发明授权

US06423816B1 Polyester polyols and their use as a binder component in two-component polyurethane coating compositions 失效
标题翻译：聚酯多元醇及其在双组分聚氨酯涂料组合物中作为粘合剂组分的用途
公开(公告)号：US06423816B1
公开(公告)日：2002-07-23
申请号：US08583167
申请日：1996-01-04
申请人： Christian Wamprecht , Michael Sonntag
发明人： Christian Wamprecht , Michael Sonntag
IPC分类号： C08G6312
CPC分类号： C09D175/14 , C08G18/68 , C08G63/52 , C09D167/06 , C08L2666/36
摘要： The present invention relates to polyester polyols having a hydroxyl number of 60 to 400, which are esterification products of a) an alcohol component containing one or more aliphatic or cycloaliphatic alcohols having at least 3 hydroxyl groups and 3 to 8 carbon atoms with b) a carboxylic acid component containing itaconic acid, maleic acid, their anhydrides and/or fumaric acid, provided that at least 10 mole % of either component a) or component b) is an aliphatic or cycloaliphatic, saturated or unsaturated monoalcohol or monocarboxylic acid having 1 to 18 carbon atoms. The present invention also relates to two-component polyurethane coating compositions containing these polyester polyols and lacquer polyisocyanates as the binder and to their use for coating substrates, in particular automotive substrates.
摘要翻译：本发明涉及羟基数为60〜400的聚酯多元醇，它们是a）含有一个或多个具有至少3个羟基和3至8个碳原子的脂族或脂环族醇的醇组分与b）羧酸的酯化产物含有衣康酸的组分，马来酸，它们的酸酐和/或富马酸，条件是至少10摩尔％的组分a）或组分b）是具有1至18个碳原子的脂族或脂环族饱和或不饱和的一元醇或一元羧酸原子本发明还涉及含有这些聚酯多元醇和漆多异氰酸酯作为粘合剂的双组分聚氨酯涂料组合物，以及它们用于涂覆基材，特别是汽车基材的用途。

6. 发明授权

US4801675A Process for the preparation of prepolymers containing isocyanate groups, the prepolymers obtainable by this process and their use as binders in one-component lacquers 失效
标题翻译：用于制备含异氰酸酯基团的预聚物的方法，可通过该方法获得的预聚物及其作为单组分漆中的粘合剂的用途
公开(公告)号：US4801675A
公开(公告)日：1989-01-31
申请号：US60782
申请日：1987-06-10
申请人： Josef Pedain , Michael Sonntag , Klaus Konig
发明人： Josef Pedain , Michael Sonntag , Klaus Konig
IPC分类号： C08G18/10 , C08G18/42 , C08G18/44 , C08G18/66 , C08G18/79 , C09D175/00 , C09D175/04 , C08G18/28 , C08G18/70 , C08G18/77
CPC分类号： C08G18/792 , C08G18/10 , C08G18/42 , C08G18/423 , C08G18/44 , C08G18/664
摘要： The invention is directed to a process for the preparation of prepolymers containing free isocyanate groups and having an isocyanate content of 1 to 16% by weight by the reaction of(a) a polyisocyanate component with(b) a polyhydroxyl component based on (i) at least one polyester polyol having a hydroxyl functionality (average) of about 1.8 to 5 and a hydroxyl number (average) of from 15 to 300 or (ii) mixtures of polyester polyols of the type mentioned under (i) with up to about 10% by weight, based on the weight of the mixture, of (cyclo)alkane polyols having a hydroxyl number above about 300 and optionally containing ester groupsat an NCO/OH equivalent ratio above 2:1, characterized in that the compounds used as component (a) contain triisocyanato-isocyanurates having aliphatically or cycloaliphatically bound isocyanate groups. The present invention also relates to the prepolymers with free isocyanate groups obtainable by this process and their use as binders for moisture hardening one-component lacquers.
摘要翻译：本发明涉及通过（a）多异氰酸酯组分与（b）多羟基组分的反应制备含有游离异氰酸酯基团和异氰酸酯含量为1至16重量％的预聚物的方法，其基于（i）至少一种具有羟基官能度（平均值）为约1.8至5，羟值（平均）为15至300）的聚酯多元醇或（ii）（i）所述类型的聚酯多元醇与高达约10 重量％，基于混合物的重量，羟基数大于约300的（环）烷烃多元醇和任选地含有高于2:1的NCO / OH当量比的酯基，其特征在于用作组分的化合物（a）含有具有脂族或环脂键结合的异氰酸酯基团的三异氰酸酯 - 异氰脲酸酯。本发明还涉及可通过该方法获得的具有游离异氰酸酯基团的预聚物及其作为湿润硬化单组分漆的粘合剂的用途。

7. 发明授权

US4737566A Process for the preparation of oligourethanes containing free isocyanate groups, the oligourethanes obtainable by this process and their use as binders or binder components in moisture hardening one-component lacquers 失效
标题翻译：制备含有游离异氰酸酯基团的低聚氨酯的方法，可通过该方法获得的低聚氨酯和它们作为湿润硬化单组分漆中的粘合剂或粘合剂组分的用途
公开(公告)号：US4737566A
公开(公告)日：1988-04-12
申请号：US34175
申请日：1987-04-02
申请人： Josef Pedain , Michael Sonntag
发明人： Josef Pedain , Michael Sonntag
IPC分类号： C08G18/65 , C08G18/32 , C08G18/66 , C09D175/04 , C09D175/08
CPC分类号： C08G18/3206 , C08G18/6607 , C08G18/6611
摘要： The present invention is directed to a process for the preparation of an oligourethane and free isocyanate groups which soluble in aromatic solvents and suitable as a lacquer binder by reacting an organic diisocyanate with a high molecular polyol and a low molecular weight polyol which contains 2,2,4-trimethylpentane-1,3-diol, its ethoxylation and/or propoxylation products or addition products of this low molecular weight diol with .epsilon.-caprolactone. The present invention is also directed to oligourethanes produced by this process and to their use as the binder or binder component in moisture hardening one-component lacquers.
摘要翻译：本发明涉及通过使有机二异氰酸酯与高分子多元醇和低分子量多元醇反应制备可溶于芳族溶剂并适合作为漆粘合剂的低聚氨酯和游离异氰酸酯基团的方法，所述低分子量多元醇含有2,2 ，4-三甲基戊烷-1,3-二醇，其乙氧基化和/或丙氧基化产物或该低分子量二醇与ε-己内酯的加成产物。本发明还涉及通过该方法制备的低聚氨酯，以及它们在湿润硬化单组分漆中作为粘合剂或粘合剂组分的用途。

8. 发明授权

US4639499A Cross-linkable polymer resins and use thereof as binders for coating agents 失效
标题翻译：可交联聚合物树脂及其作为涂布剂的粘合剂的用途
公开(公告)号：US4639499A
公开(公告)日：1987-01-27
申请号：US756483
申请日：1985-07-18
申请人： Peter Hohlein , Manfred Schmidt , Josef Pedain , Bernd Riberi , Michael Sonntag
发明人： Peter Hohlein , Manfred Schmidt , Josef Pedain , Bernd Riberi , Michael Sonntag
IPC分类号： C09D201/06 , C08F216/00 , C08F246/00 , C09D133/04 , C09D157/04 , C09D175/00 , C08F238/00 , C08F220/04
CPC分类号： C08F246/00 , C08F216/00 , C09D157/04
摘要： The present invention is directed to cross-linkable, hydroxyl group-containing polymer resins which are obtained by copolymerizing olefinically-unsaturated monomers and are suitable as binder components for lacquers, the polymer resins having a hydroxyl number of about 20 to 400, an average osmometrically-determined molecular weight of about 500 to 30,000 and a molecular inhomogeneity U of about 0.5 to 15, characterized in that they contain about 0.2 to 80% by weight, preferably about 10 to 70% by weight, based on the total weight of the copolymers, of incorporated monomers selected from olefinically- and acetylenically-unsaturated aliphatic diols having 4 carbon atoms, the ether group-containing alkoxylation products thereof with a hydroxyl number of about 50 to 900, the reaction products of these diols with .epsilon.-caprolactone in a mol ratio of diol:-caprolactone of about 1:0.2 to 1:10 and any mixtures of these components.The present invention is also directed to the use of the above polymer resins as binders for coating compositions.
摘要翻译：本发明涉及可交联的含羟基的聚合物树脂，其通过使烯属不饱和单体共聚合而获得，并且适合作为漆的粘合剂组分，聚合物树脂的羟值为约20至400，平均渗透压约500至30,000的测定分子量和约0.5至15的分子不均匀性U，其特征在于它们含有约0.2至80重量％，优选约10至70重量％，基于共聚物的总重量包含选自具有4个碳原子的烯属和炔属不饱和脂族二醇的单体，其含醚基的烷氧基化产物的羟值为约50至900，这些二醇与ε-己内酯的摩尔比为摩尔二醇：己内酯的比例为约1:0.2至1:10，以及这些组分的任何混合物。本发明还涉及上述聚合物树脂作为涂料组合物的粘合剂的用途。

9. 发明授权

US06458898B1 Two-component polyurethane coating compositions containing polyester polyols as a binder component 失效
标题翻译：含有聚酯多元醇作为粘合剂组分的双组分聚氨酯涂料组合物
公开(公告)号：US06458898B1
公开(公告)日：2002-10-01
申请号：US08329109
申请日：1994-10-25
申请人： Christian Wamprecht , Michael Sonntag
发明人： Christian Wamprecht , Michael Sonntag
IPC分类号： B32B2740
CPC分类号： C09D175/14 , C08G18/68 , C08G18/686 , Y10T428/31551 , Y10T428/31605
摘要： Two-component polyurethane coating compositions containing wherein the binder contains polyisocyanates and certain polyester polyols having hydroxyl numbers of 80 to 250 prepared from a) polyol mixtures and b) aliphatic unsaturated dicarboxylic acids and, optionally, aliphatic saturated dicarboxylic acids, and their use for the production of coatings on plastic moldings such as those used in automobile construction.
摘要翻译：双组分聚氨酯涂料组合物，其中粘合剂含有多异氰酸酯和由a）多元醇混合物和b）脂族不饱和二羧酸和任选的脂族饱和二羧酸制备的羟基数为80至250的某些聚酯多元醇及其用于在塑料模制品上生产涂料，如汽车制造中使用的涂料。

10. 发明授权

US06380308B1 High-solids binder compositions and their use 有权
标题翻译：高固体粘合剂组合物及其用途
公开(公告)号：US06380308B1
公开(公告)日：2002-04-30
申请号：US09711743
申请日：2000-11-13
申请人： Christian Wamprecht , Michael Sonntag , Holger Mundstock
发明人： Christian Wamprecht , Michael Sonntag , Holger Mundstock
IPC分类号： C08G1863
CPC分类号： C08L51/04 , C08F279/02 , C08G18/635 , C09D151/04 , C09D175/04 , Y10T428/31551
摘要： The invention relates to a binder composition containing A) 50-90 parts by wt. of OH-functional graft copolymer resins prepared from a) 0.1 to 10 parts by wt. of polybutadiene, b) 5 to 60 parts by wt. of an unsaturated aromatic monomer, c) 10 to 50 parts by wt. of a hydroxyalkyl ester of (meth)acrylic acid, d) 5 to 70 parts by wt. of a cycloaliphatic ester of (meth)acrylic acid, e) 5 to 50 parts by wt. of an aliphatic ester of (meth)acrylic acid, f) 0.1 to 5 parts by wt. of a mono-olifinically unsaturated mono- or dicarboxylic acid and/or maleic or fumaric acid half esters, B) 0.1 to 5 parts by wt. of a polyfunctional crosslinking agent.
摘要翻译：本发明涉及一种粘合剂组合物，其包含A）50-90重量份由以下制备的OH官能接枝共聚物树脂：0.1〜10重量份的聚丁二烯，b）5〜60重量份。的不饱和芳族单体，c）10至50重量份。的（甲基）丙烯酸的羟烷基酯，d）5〜70重量份。的（甲基）丙烯酸的脂环族酯，e）5〜50重量份的（甲基）丙烯酸的脂肪族酯，f）0.1〜5重量份。的单烯烃不饱和单羧酸和/或马来酸或富马酸半酯，B）0.1至5重量份。的多官能交联剂。

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