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1. 发明授权

US08173041B2 Method for intercalating chromophores into zeolite-L nanochannels and products thereof 失效
标题翻译：将发色团插入沸石-L纳米通道及其产物的方法
公开(公告)号：US08173041B2
公开(公告)日：2012-05-08
申请号：US12361616
申请日：2009-01-29
申请人： Gion Calzaferri , Luisa De Cola , Michael Busby , Christian Blum , Vinod Subramaniam
发明人： Gion Calzaferri , Luisa De Cola , Michael Busby , Christian Blum , Vinod Subramaniam
IPC分类号： C09K11/06 , H01L31/00
CPC分类号： C01B39/026
摘要： The present invention discloses a method for the intercalation of a chromophore within channels of a zeolite L crystal. The intercalated chromophores exhibit J type aggregation of the chromophores within the channels of the zeolite L crystals. The invention discloses method parameters which lead to the J type aggregation of the chromophores within the channels of the zeolite L crystals. The J type aggregation of the chromophores affords unique florescent properties rendering the intercalated zeolite L crystals as a material for use in novel optoelectronic devices.
摘要翻译：本发明公开了一种在沸石L晶体的通道内插入发色团的方法。插层发色团在沸石L晶体的通道内显示发色团的J型聚集体。本发明公开了导致沸石L晶体通道内发色团的J型聚集的方法参数。发色团的J型聚集提供了独特的荧光性质，使嵌入的沸石L晶体作为用于新型光电子器件的材料。

2. 发明申请

US20110287408A1 Preparation of Micro-Porous Crystals and Conjugates Thereof 失效
标题翻译：微孔多晶体及其结合体的制备
公开(公告)号：US20110287408A1
公开(公告)日：2011-11-24
申请号：US13099577
申请日：2011-05-03
申请人： Zoran Popovic , Manuel Matthias Tsotsalas , Michael Busby , Luisa De Cola , Gion Calzaferri , Hans-Peter Josel
发明人： Zoran Popovic , Manuel Matthias Tsotsalas , Michael Busby , Luisa De Cola , Gion Calzaferri , Hans-Peter Josel
IPC分类号： C12Q1/70 , C07F19/00 , C12Q1/02
CPC分类号： G01N33/533 , G01N33/582
摘要： A conjugate comprising a dye-labeled microporous crystal, a stop-cock moiety, and covalently bound thereto an affinity binding agent is disclosed. The dye-labeled microporous crystal is a zeolite crystal, such as a zeolite L crystal, having a large number of channels in its interior into which the dye is loaded. The stop-cock moiety can be functionalized with an amino group to which a carboxyester group can be attached. The affinity binding agent allows for the binding to a biological moiety. The conjugate of the moiety can be used in in-vivo and/or in-vitro imaging applications.
摘要翻译：公开了包含染料标记的微孔结晶，停止旋塞部分并与其共价结合的亲和力结合剂的缀合物。染料标记的微孔结晶是沸石晶体，例如沸石L晶体，其内部具有大量通道，染料加载到其中。停止旋塞部分可以与可以连接羧基酯基团的氨基官能化。亲和力结合剂允许结合生物部分。该部分的缀合物可用于体内和/或体外成像应用。

3. 发明授权

US08445214B2 Preparation of micro-porous crystals and conjugates thereof 失效
标题翻译：微孔结晶及其共轭物的制备
公开(公告)号：US08445214B2
公开(公告)日：2013-05-21
申请号：US13099577
申请日：2011-05-03
申请人： Zoran Popovic , Manuel Matthias Tsotsalas , Michael Busby , Luisa De Cola , Gion Calzaferri , Hans-Peter Josel
发明人： Zoran Popovic , Manuel Matthias Tsotsalas , Michael Busby , Luisa De Cola , Gion Calzaferri , Hans-Peter Josel
IPC分类号： G01N33/53
CPC分类号： G01N33/533 , G01N33/582
摘要： A conjugate comprising a dye-labeled microporous crystal, a stop-cock moiety, and covalently bound thereto an affinity binding agent is disclosed. The dye-labeled microporous crystal is a zeolite crystal, such as a zeolite L crystal, having a large number of channels in its interior into which the dye is loaded. The stop-cock moiety can be functionalized with an amino group to which a carboxyester group can be attached. The affinity binding agent allows for the binding to a biological moiety. The conjugate of the moiety can be used in in-vivo and/or in-vitro imaging applications.
摘要翻译：公开了包含染料标记的微孔结晶，停止旋塞部分并与其共价结合的亲和力结合剂的缀合物。染料标记的微孔结晶是沸石晶体，例如沸石L晶体，其内部具有大量通道，染料加载到其中。停止旋塞部分可以与可以连接羧基酯基团的氨基官能化。亲和力结合剂允许结合生物部分。该部分的缀合物可用于体内和/或体外成像应用。

4. 发明授权

US07960124B2 Preparation of micro-porous crystals and conjugates thereof 有权
标题翻译：微孔结晶及其结合物的制备
公开(公告)号：US07960124B2
公开(公告)日：2011-06-14
申请号：US11824416
申请日：2007-06-29
申请人： Zoran Popovic , Manuel Matthias Tsotsalas , Michael Busby , Luisa De Cola , Gion Calzaferri , Hans-Peter Josel
发明人： Zoran Popovic , Manuel Matthias Tsotsalas , Michael Busby , Luisa De Cola , Gion Calzaferri , Hans-Peter Josel
IPC分类号： G01N33/53
CPC分类号： G01N33/533 , G01N33/582
摘要： A conjugate comprising a dye-labeled microporous crystal, a stop-cock moiety, and covalently bound thereto an affinity binding agent is disclosed. The dye-labeled microporous crystal is a zeolite crystal, such as a zeolite L crystal, having a large number of channels in its interior into which the dye is loaded. The stop-cock moiety can be functionalized with an amino group to which a carboxyester group can be attached. The affinity binding agent allows for the binding to a biological moiety. The conjugate of the moiety can be used in in-vivo and/or in-vitro imaging applications.
摘要翻译：公开了包含染料标记的微孔结晶，停止旋塞部分并与其共价结合的亲和力结合剂的缀合物。染料标记的微孔结晶是沸石晶体，例如沸石L晶体，其内部具有大量通道，染料加载到其中。停止旋塞部分可以与可以连接羧基酯基团的氨基官能化。亲和力结合剂允许结合生物部分。该部分的缀合物可用于体内和/或体外成像应用。

5. 发明申请

US20080138914A1 Preparation of micro-porous crystals and conjugates thereof 有权
标题翻译：微孔结晶及其结合物的制备
公开(公告)号：US20080138914A1
公开(公告)日：2008-06-12
申请号：US11824416
申请日：2007-06-29
申请人： Zoran Popovic , Manuel Matthias Tsotsalas , Michael Busby , Luisa De Cola , Gion Calzaferri , Hans-Peter Josel
发明人： Zoran Popovic , Manuel Matthias Tsotsalas , Michael Busby , Luisa De Cola , Gion Calzaferri , Hans-Peter Josel
IPC分类号： G01N33/536 , C01B39/02 , C07F7/02 , C07H21/00 , C07K16/00 , C07K14/42 , C07K2/00
CPC分类号： G01N33/533 , G01N33/582
摘要： A conjugate comprising a dye-labeled microporous crystal, a stop-cock moiety, and covalently bound thereto an affinity binding agent is disclosed. The dye-labeled microporous crystal is a zeolite crystal, such as a zeolite L crystal, having a large number of channels in its interior into which the dye is loaded. The stop-cock moiety can be functionalized with an amino group to which a carboxyester group can be attached. The affinity binding agent allows for the binding to a biological moiety. The conjugate of the moiety can be used in in-vivo and/or in-vitro imaging applications.
摘要翻译：公开了包含染料标记的微孔结晶，停止旋塞部分并与其共价结合的亲和力结合剂的缀合物。染料标记的微孔结晶是沸石晶体，例如沸石L晶体，其内部具有大量通道，染料加载到其中。停止旋塞部分可以与可以连接羧基酯基团的氨基官能化。亲和力结合剂允许结合生物部分。该部分的缀合物可用于体内和/或体外成像应用。

6. 发明申请

US20140328761A1 Local J-Coupling Dye-Zeolite Antenna Composite Materials 有权
标题翻译：局部J-偶联染料 - 沸石天线复合材料
公开(公告)号：US20140328761A1
公开(公告)日：2014-11-06
申请号：US14360877
申请日：2012-12-10
申请人： Gion Calzaferri , Andreas Kunzmann , Universität Zürick
发明人： Gion Calzaferri , Andreas Kunzmann , Dominik Bruehwiler
IPC分类号： A61K49/00 , C09K11/06 , C12Q1/70 , H05B33/20 , H01G9/20 , H01L51/00 , H05B33/14 , C09C1/40 , C12Q1/02
CPC分类号： A61K49/0013 , C01B37/04 , C01B39/02 , C09C1/40 , C09K11/06 , C09K2211/1007 , C09K2211/1011 , C09K2211/1018 , C09K2211/1022 , C09K2211/1029 , C09K2211/1033 , C09K2211/1037 , C09K2211/1044 , C09K2211/1088 , C09K2211/1092 , C12Q1/02 , C12Q1/70 , H01G9/2063 , H01L51/0072 , H01L51/5012 , H05B33/14 , H05B33/20
摘要： A dye loaded zeolite composite material comprises a plurality of zeolite crystals each having a plurality of straight through uniform channels extending between the proximal face and the distal face and having a channel axis parallel to and a channel width transverse to a longitudinal crystal axis A. Each channel contains a substantially linear arrangement of dye molecules comprising first and second dye molecules having an elongated shape with a longitudinal extension exceeding said channel width and a lateral extension not exceeding said channel width. Each dye molecule consists of a chromophore moiety arranged between a pair of terminal moieties, wherein: the chromophore moieties of the first and second dye molecules are substantially identical, the terminal moieties of the first dye molecules have a lateral extension larger than half of the channel width, the terminal moieties of the second dye molecules have a lateral extension smaller than half of the channel width, the linear arrangement of dye molecules comprises at least one pair of second dye molecules adjacent each other.
摘要翻译：染料负载的沸石复合材料包括多个沸石晶体，每个沸石晶体具有在近端面和远端面之间延伸的多个直通的均匀通道，并且具有平行于纵向晶轴A的横向轴线和横向宽度的通道宽度。每个通道包含染料分子的基本线性排列，其包含具有细长形状的第一和第二染料分子，其纵向延伸超过所述通道宽度，横向延伸不超过所述通道宽度。每个染料分子由布置在一对末端部分之间的发色团部分组成，其中：第一和第二染料分子的发色团部分基本相同，第一染料分子的末端部分具有大于通道一半的横向延伸第二染料分子的末端部分具有小于沟道宽度的一半的横向延伸，染料分子的线性排列包括彼此相邻的至少一对第二染料分子。

7. 发明授权

US07372012B2 Dye loaded zeolite material containing devices 失效
标题翻译：含染料负载沸石材料的装置
公开(公告)号：US07372012B2
公开(公告)日：2008-05-13
申请号：US11173163
申请日：2005-07-05
申请人： Gion Calzaferri
发明人： Gion Calzaferri
IPC分类号： H01J40/14 , C09K11/06 , C01B39/32 , H01L31/06
CPC分类号： C09K11/06 , B01J20/3204 , B01J39/14 , B82Y15/00 , H01L51/005 , H01L51/0064 , H01L51/0069 , H01L51/0071 , H01L51/008 , H01L51/447 , Y02E10/549
摘要： The present invention provides a dye loaded zeolite material comprising: a) at least one zeolite crystal having straight through uniform channels each having a channel axis parallel to, and a channel width transverse to, a c-axis of crystal unit cells; b) closure molecules having an elongated shape and consisting of a head moiety and a tail moiety, the tail moiety having a longitudinal extension of more than a dimension of the crystal unit cells along the c-axis and the head moiety having a lateral extension that is larger than said channel width and will prevent said head moiety from penetrating into a channel; c) a channel being terminated, in generally plug-like manner, at least at one end thereof located at a surface of the zeolite crystal by a closure molecule hose tail moiety penetrates into said channel and whose head moiety substantially occludes said channel end while projecting over said surface; and d) an essentially linear arrangement of luminescent dye molecules enclosed within a terminated channel adjacent to at least one closure molecule and exhibiting properties related to supramolecular organization.
摘要翻译：本发明提供一种负载染料的沸石材料，包括：a）至少一种具有直通均匀通道的沸石晶体，每个通道均具有平行于晶体单元晶胞的c轴的沟道轴线和沟槽宽度; b）具有细长形状并由头部部分和尾部部分组成的封闭分子，所述尾部部分具有比c轴更多的晶体单位细胞尺寸的纵向延伸，并且头部部分具有侧向延伸，大于所述通道宽度，并且将防止所述头部部分穿透通道; c）通常通过塞子状方式终止位于沸石晶体表面的通道，封闭分子软管尾部穿透入所述通道，并且其头部基本封闭所述通道端，同时突出在所述表面上; 以及d）包封在与至少一个封闭分子相邻的封端通道中并且显示与超分子组织相关的性质的发光染料分子的基本线性排列。

8. 发明授权

US08917969B2 Luminescence concentrators and luminescence dispersers on the basis of oriented dye zeolite antennas 有权
标题翻译：基于定向染料沸石天线的发光聚光器和发光分散器
公开(公告)号：US08917969B2
公开(公告)日：2014-12-23
申请号：US12999013
申请日：2009-03-31
申请人： Gion Calzaferri , Andreas Kunzmann , Dominik Brühwiler , Christophe Bauer
发明人： Gion Calzaferri , Andreas Kunzmann , Dominik Brühwiler , Christophe Bauer
IPC分类号： G02B6/00 , C09K11/06 , H01L31/0232 , H01L51/44 , H01L31/055 , F24J2/06
CPC分类号： C09K11/06 , F24S23/11 , H01L31/02322 , H01L31/055 , H01L51/447 , Y02E10/52 , Y02E10/549 , Y02P70/521
摘要： A luminescence concentrator (LK) may concentrate both incident direct and diffuse light by way of frequency shift and total internal reflection. It differs fundamentally from geometric concentrators. With sufficient geometric expansion of the collector plate, nearly arbitrarily high concentration can be achieved in the LK. A luminescence disperser is an apparatus which holds both directional and nondirectional incident light captive in a transparent body by way of frequency shift and total internal reflection and emits it diffusely or directionally uniformly distributed across an area by way of luminescence emission. The object of the invention is a method for the technical implementation of the LK and luminescence disperser, using zeolite crystals having a nanotube structure, into which the luminescent dyes are embedded such that they have antenna properties. Using the resulting novel structures, problems can be solved which made the technical use of LK impossible or at least considerably limited it. This results in completely novel usage possibilities for collecting and concentrating sun light and feeding it into photovoltaic systems, for converting it into electric and thermal energy in combined photovoltaic/hot water apparatuses, and for feeding it into fiber optic apparatuses.
摘要翻译：发光集中器（LK）可以通过频移和全内反射集中入射直射光和漫射光。它与几何集中器的根本不同。在集电板的几何膨胀充分的情况下，LK可实现几乎任意高的浓度。发光分散器是通过频移和全内反射来保持透明体中的定向和非定向入射光的装置，并通过发光发射漫射或均匀分布在区域上。本发明的目的是使用具有纳米管结构的沸石晶体技术实现LK和发光分散器的方法，其中嵌入发光染料，使得它们具有天线性质。使用所得到的新颖结构，可以解决使得LK的技术使用不可能或至少大大限制的问题。这导致了用于收集和集中太阳光并将其馈送到光伏系统中的完全新颖的使用可能性，以将其转换为组合的光伏/热水设备中的电能和热能，并将其馈送到光纤设备中。

9. 发明授权

US08222592B2 Dye loaded zeolite material 失效
标题翻译：染料负载的沸石材料
公开(公告)号：US08222592B2
公开(公告)日：2012-07-17
申请号：US13030207
申请日：2011-02-18
申请人： Gion Calzaferri
发明人： Gion Calzaferri
IPC分类号： H01J40/14 , H01L31/06
CPC分类号： C09K11/06 , B01J20/3204 , B01J39/14 , B82Y15/00 , H01L51/005 , H01L51/0064 , H01L51/0069 , H01L51/0071 , H01L51/008 , H01L51/447 , Y02E10/549
摘要： The present invention provides a dye loaded zeolite material comprising: a) at least one zeolite crystal having straight through uniform channels each having a channel axis parallel to, and a channel width transverse to, a c-axis of crystal unit cells; b) closure molecules having an elongated shape and consisting of a head moiety and a tail moiety, the tail moiety having a longitudinal extension of more than a dimension of the crystal unit cells along the c-axis and the head moiety having a lateral extension that is larger than said channel width and will prevent said head moiety from penetrating into a channel; c) a channel being terminated, in generally plug-like manner, at least at one end thereof located at a surface of the zeolite crystal by a closure molecule hose tail moiety penetrates into said channel and whose head moiety substantially occludes said channel end while projecting over said surface; and d) an essentially linear arrangement of luminescent dye molecules enclosed within a terminated channel adjacent to at least one closure molecule and exhibiting properties related to supramolecular organization.
摘要翻译：本发明提供一种负载染料的沸石材料，包括：a）至少一种具有直通均匀通道的沸石晶体，每个通道均具有平行于晶体单元晶胞的c轴的沟道轴线和沟槽宽度; b）具有细长形状并由头部部分和尾部部分组成的封闭分子，所述尾部部分具有比c轴更多的晶体单位细胞尺寸的纵向延伸，并且头部部分具有侧向延伸，大于所述通道宽度，并且将防止所述头部部分穿透通道; c）以通常塞状方式至少在其一端处被定位在沸石晶体的表面处的通道通过闭合分子软管尾部穿透入所述通道并且其头部部分基本上封闭所述通道端而突出在所述表面上; 以及d）包封在与至少一个封闭分子相邻的封端通道中并且显示与超分子组织相关的性质的发光染料分子的基本线性排列。

10. 发明申请

US20110094566A1 Luminescence Concentrators and Luminescence Dispersers on the Basis of Oriented Dye Zeolite Antennas 有权
标题翻译：发光浓缩器和发光分散器在定向染料沸石天线的基础上
公开(公告)号：US20110094566A1
公开(公告)日：2011-04-28
申请号：US12999013
申请日：2009-03-31
申请人： Gion Calzaferri , Andreas Kunzmann , Dominik Brühwiler , Christophe Bauer
发明人： Gion Calzaferri , Andreas Kunzmann , Dominik Brühwiler , Christophe Bauer
IPC分类号： H01L31/052 , G02B6/00 , B05D5/06 , F24J2/08
CPC分类号： C09K11/06 , F24S23/11 , H01L31/02322 , H01L31/055 , H01L51/447 , Y02E10/52 , Y02E10/549 , Y02P70/521
摘要： A luminescence concentrator (LK) may concentrate both incident direct and diffuse light by way of frequency shift and total internal reflection. It differs fundamentally from geometric concentrators. With sufficient geometric expansion of the collector plate, nearly arbitrarily high concentration can be achieved in the LK. A luminescence disperser is an apparatus which holds both directional and nondirectional incident light captive in a transparent body by way of frequency shift and total internal reflection and emits it diffusely or directionally uniformly distributed across an area by way of luminescence emission. The object of the invention is a method for the technical implementation of the LK and luminescence disperser, using zeolite crystals having a nanotube structure, into which the luminescent dyes are embedded such that they have antenna properties. Using the resulting novel structures, problems can be solved which made the technical use of LK impossible or at least considerably limited it. This results in completely novel usage possibilities for collecting and concentrating sun light and feeding it into photovoltaic systems, for converting it into electric and thermal energy in combined photovoltaic/hot water apparatuses, and for feeding it into fiber optic apparatuses.
摘要翻译：发光集中器（LK）可以通过频移和全内反射集中入射直射光和漫射光。它与几何集中器的根本不同。在集电板的几何膨胀充分的情况下，LK可实现几乎任意高的浓度。发光分散器是通过频移和全内反射来保持透明体中的定向和非定向入射光的装置，并通过发光发射漫射或均匀分布在区域上。本发明的目的是使用具有纳米管结构的沸石晶体技术实现LK和发光分散器的方法，其中嵌入发光染料，使得它们具有天线性质。使用所得到的新颖结构，可以解决使得LK的技术使用不可能或至少大大限制的问题。这导致了用于收集和集中太阳光并将其馈送到光伏系统中的完全新颖的使用可能性，以将其转换为组合的光伏/热水设备中的电能和热能，并将其馈送到光纤设备中。

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