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1. 发明授权

US07145022B2 Catalyst for the carbonylation of oxiranes 有权
标题翻译：环氧乙烷羰基化催化剂
公开(公告)号：US07145022B2
公开(公告)日：2006-12-05
申请号：US10523264
申请日：2003-07-31
申请人： Gerrit Luinstra , Bernhard Rieger , Markus Allmendinger
发明人： Gerrit Luinstra , Bernhard Rieger , Markus Allmendinger
IPC分类号： C07D305/12
CPC分类号： C07D315/00 , B01J23/26 , B01J31/1805 , B01J31/20 , B01J31/2243 , B01J2231/34 , B01J2531/0208 , B01J2531/0252 , B01J2531/62 , B01J2531/845
摘要： Lactones are prepared by catalytic carbonylation of oxiranes using a catalyst system comprising a) at least one carbonylation catalyst A comprising uncharged or anionic transition metal complexes of metals of groups 5 to 11 of the Periodic Table of the Elements and b) at least one chiral Lewis acid B, with the exception of [(salph)Al(THF)2][Co(CO)4], as catalyst.
摘要翻译：内酯通过使用催化剂体系的催化体系催化羰基化制备，所述催化剂体系包含a）至少一种羰基化催化剂A，其包含元素周期表第5至11族金属的不带电荷或阴离子过渡金属络合物，和b）至少一种手性路易斯酸性B，但[（salph）Al（THF）2] [Co（CO）4]]除外。

2. 发明申请

US20050256320A1 Catalyst and method for the carbonylation of oxiranes 失效
标题翻译：催化剂和环氧乙烷羰基化方法
公开(公告)号：US20050256320A1
公开(公告)日：2005-11-17
申请号：US10523263
申请日：2003-07-31
申请人： Gerrit Luinstra , Ferenc Molnar , Bernhard Rieger , Markus Allmendinger
发明人： Gerrit Luinstra , Ferenc Molnar , Bernhard Rieger , Markus Allmendinger
IPC分类号： B01J31/12 , B01J31/14 , B01J31/20 , C07D303/04 , C07D305/12
CPC分类号： C07D305/12 , B01J31/122 , B01J31/143 , B01J31/20 , B01J2231/34 , B01J2531/845 , C07D303/04
摘要： Lactones are prepared by catalytic carbonylation of oxiranes using a catalyst system comprising a) at least one cobalt compound as component A and b) at least one metal compound of the formula (I) as component B, MXxRn-x (I) where M is an alkaline earth metal or a metal of group 3, 4 or preferably 12 or 13 of the Periodic Table of the Elements, R is hydrogen or a hydrocarbon radical which may be substituted on the carbon atoms other than the carbon atom bound to M, X is an anion, n is a number corresponding to the valence of M and x is in the range from 0 to n, with n and x being selected so that the compound is uncharged, as catalyst.
摘要翻译：内酯通过使用包含a）至少一种钴化合物作为组分A和b）至少一种式（I）的金属化合物作为组分B的催化剂体系制备，所述催化剂体系包括：a）至少一种钴化合物作为组分A， “在线公式”end =“lead”？> MX R （I）<？in-line-formula description =“In-line Formulas”end =“尾”→其中M是元素周期表中的3,4或优选12或13的碱土金属或金属，R是氢或可以在碳原子上被取代的烃基除了与M结合的碳原子之外，X是阴离子，n是对应于M的化合价的数，x在0至n的范围内，选择n和x，以使化合物不带电作为催化剂。

3. 发明授权

US07420064B2 Catalyst and method for the carbonylation of oxiranes 失效
标题翻译：催化剂和环氧乙烷羰基化方法
公开(公告)号：US07420064B2
公开(公告)日：2008-09-02
申请号：US10523263
申请日：2003-07-31
申请人： Gerrit Luinstra , Ferenc Molnar , Bernhard Rieger , Markus Allmendinger
发明人： Gerrit Luinstra , Ferenc Molnar , Bernhard Rieger , Markus Allmendinger
IPC分类号： C07D305/12 , B01J31/00
CPC分类号： C07D305/12 , B01J31/122 , B01J31/143 , B01J31/20 , B01J2231/34 , B01J2531/845 , C07D303/04
摘要： Lactones are prepared by catalytic carbonylation of oxiranes using a catalyst system comprising a) at least one cobalt compound as component A and b) at least one metal compound of the formula (I) as component B, MXxRn-x (I) where M is an alkaline earth metal or a metal of group 3, 4 or preferably 12 or 13 of the Periodic Table of the Elements, R is hydrogen or a hydrocarbon radical which may be substituted on the carbon atoms other than the carbon atom bound to M, X is an anion, n is a number corresponding to the valence of M and x is in the range from 0 to n, with n and x being selected so that the compound is uncharged, as catalyst.
摘要翻译：内酯通过使用包含a）至少一种钴化合物作为组分A和b）至少一种式（I）的金属化合物作为组分B的催化剂体系制备，所述催化剂体系包括：a）至少一种钴化合物作为组分A， “在线公式”end =“lead”？> MX R （I）<？in-line-formula description =“In-line Formulas”end =“尾”→其中M是元素周期表中的3,4或优选12或13的碱土金属或金属，R是氢或可以在碳原子上被取代的烃基除了与M结合的碳原子之外，X是阴离子，n是对应于M的化合价的数，x在0至n的范围内，选择n和x，以使化合物不带电作为催化剂。

4. 发明授权

US07019107B2 Method for the production of poly(3-hydroxyalkanoates) in the presence of a nucleophile 失效
标题翻译：在亲核试剂存在下生产聚（3-羟基链烷酸酯）的方法
公开(公告)号：US07019107B2
公开(公告)日：2006-03-28
申请号：US10505707
申请日：2003-02-26
申请人： Gerrit Luinstra , Markus Allmendinger , Bernhard Rieger
发明人： Gerrit Luinstra , Markus Allmendinger , Bernhard Rieger
IPC分类号： C08G59/68 , C08G65/10
CPC分类号： C08G63/823 , C08G63/08
摘要： The invention relates to a catalytical process for preparing poly(3-hydroxyalkanoates) by copolymerizing an oxirane compound with carbon monoxide in the presence of a) at least one single- or multicenter neutral transition metal complex (A) based on a metal of groups 5 to 11 of the Periodic Table of the Elements, in which the metal center(s) is/are present in the formal oxidation state 0, and/or b) at least one single- or multicenter anionic transition metal complex (B) based on a metal of groups 5 to 11 of the Periodic Table of the Elements, where multicenter transition metal complexes have metal centers which, without exception, are of the same transition metal, which comprises carrying out the copolymerization in the presence of at least one nucleophile other than hydroxy-substituted pyridine compounds.
摘要翻译：本发明涉及通过在a）至少一种基于5族金属的单中心或多中心中性过渡金属络合物（A）的存在下将环氧乙烷化合物与一氧化碳共聚来制备聚（3-羟基链烷酸酯）的催化方法至元素周期表中的11个，其中金属中心以形式氧化态0存在，和/或b）至少一种单或多中心阴离子过渡金属络合物（B），基于元素周期表第5至11组的金属，其中多中心过渡金属络合物具有金属中心，无一例外是相同的过渡金属，其包括在存在至少一种亲核试剂的情况下进行共聚比羟基取代的吡啶化合物。

5. 发明申请

US20050240032A1 Catalyst for the carbonylation of oxiranes 有权
标题翻译：环氧乙烷羰基化催化剂
公开(公告)号：US20050240032A1
公开(公告)日：2005-10-27
申请号：US10523264
申请日：2003-07-31
申请人： Gerrit Luinstra , Bernhard Rieger , Markus Allmendinger
发明人： Gerrit Luinstra , Bernhard Rieger , Markus Allmendinger
IPC分类号： B01J23/26 , B01J31/12 , B01J31/18 , B01J31/20 , C07D315/00 , C07D305/12
CPC分类号： C07D315/00 , B01J23/26 , B01J31/1805 , B01J31/20 , B01J31/2243 , B01J2231/34 , B01J2531/0208 , B01J2531/0252 , B01J2531/62 , B01J2531/845
摘要： Lactones are prepared by catalytic carbonylation of oxiranes using a catalyst system comprising a) at least one carbonylation catalyst A comprising uncharged or anionic transition metal complexes of metals of groups 5 to 11 of the Periodic Table of the Elements and b) at least one chiral Lewis acid B, with the exception of [(salph)Al(THF)2][Co(CO)4], as catalyst.
摘要翻译：内酯通过使用催化剂体系的催化体系催化羰基化制备，所述催化剂体系包含a）至少一种羰基化催化剂A，其包含元素周期表第5至11族金属的不带电荷或阴离子过渡金属络合物，和b）至少一种手性路易斯酸性B，但[（salph）Al（THF）2] [Co（CO）4]]除外，作为催化剂。

6. 发明申请

US20050107573A1 Method for the production of poly(3-hydroxyalkanoates) in the presence of a nucleophile 失效
标题翻译：在亲核试剂存在下生产聚（3-羟基链烷酸酯）的方法
公开(公告)号：US20050107573A1
公开(公告)日：2005-05-19
申请号：US10505707
申请日：2003-02-26
申请人： Gerrit Lunistra , Markus Allmendinger , Bernhard Rieger
发明人： Gerrit Lunistra , Markus Allmendinger , Bernhard Rieger
IPC分类号： C08G63/85 , C08G63/08 , C08G63/42 , C08G63/82 , C08L101/16 , C08G63/02
CPC分类号： C08G63/823 , C08G63/08
摘要： The invention relates to a catalytical process for preparing poly(3-hydroxyalkanoates) by copolymerizing an oxirane compound with carbon monoxide in the presence of a) at least one single- or multicenter neutral transition metal complex (A) based on a metal of groups 5 to 11 of the Periodic Table of the Elements, in which the metal center(s) is/are present in the formal oxidation state 0, and/or b) at least one single- or multicenter anionic transition metal complex (B) based on a metal of groups 5 to 11 of the Periodic Table of the Elements, where multicenter transition metal complexes have metal centers which, without exception, are of the same transition metal, which comprises carrying out the copolymerization in the presence of at least one nucleophile other than hydroxy-substituted pyridine compounds.
摘要翻译：本发明涉及通过在a）至少一种基于5族金属的单中心或多中心中性过渡金属络合物（A）的存在下将环氧乙烷化合物与一氧化碳共聚来制备聚（3-羟基链烷酸酯）的催化方法至元素周期表中的11个，其中金属中心以形式氧化态0存在，和/或b）至少一种单或多中心阴离子过渡金属络合物（B），基于元素周期表第5至11组的金属，其中多中心过渡金属络合物具有金属中心，无一例外是相同的过渡金属，其包括在存在至少一种亲核试剂的情况下进行共聚比羟基取代的吡啶化合物。

7. 发明申请

US20090039537A1 Method for the Production of Expandable Styrol Polymers Having Improved Expandability 审中-公开
标题翻译：具有改进的膨胀性的可膨胀型苯乙烯聚合物的生产方法
公开(公告)号：US20090039537A1
公开(公告)日：2009-02-12
申请号：US11632354
申请日：2005-07-08
申请人： Klaus Hahn , Gerd Ehrmann , Joachim Ruch , Markus Allmendinger , Bernhard Schmied , Jan Holoch
发明人： Klaus Hahn , Gerd Ehrmann , Joachim Ruch , Markus Allmendinger , Bernhard Schmied , Jan Holoch
IPC分类号： B29B9/10
CPC分类号： C08J9/16 , C08J2325/06
摘要： A process for producing expandable styrene polymers (EPS) having improved expandability, wherein from 0.1 to 1% by weight, based on the styrene polymer, of a free-radical former is metered into a styrene polymer melt containing blowing agent at a melt temperature in the range from 150 to 220° C. and the melt is extruded through a die plate with subsequent underwater pelletization.
摘要翻译：一种制备具有改进的可膨胀性的可发性苯乙烯聚合物（EPS）的方法，其中基于苯乙烯聚合物的0.1-1％重量的自由基形成剂在熔融温度下计量加入含有发泡剂的苯乙烯聚合物熔体中在150至220℃的范围内，熔体通过模板挤出，随后进行水下造粒。

8. 发明申请

US20080096988A1 Expandable Styrene Polymers With Halogen-Free Flame Retardancy 审中-公开
标题翻译：可扩展的苯乙烯聚合物与无卤阻燃
公开(公告)号：US20080096988A1
公开(公告)日：2008-04-24
申请号：US11720563
申请日：2005-12-01
申请人： Klaus Hahn , Gerd Ehrmann , Joachim Ruch , Markus Allmendinger , Bernhard Schmied
发明人： Klaus Hahn , Gerd Ehrmann , Joachim Ruch , Markus Allmendinger , Bernhard Schmied
IPC分类号： C08J9/16 , C08J9/228
CPC分类号： C08J9/0066 , C08J9/16 , C08J2203/12 , C08J2203/14 , C08J2325/06
摘要： Expandable styrene polymer granules with halogen-free flame retardancy, comprising a) from 5 to 50% by weight of a filler selected from pulverulent inorganic substances such as talc, chalk, kaolin, aluminum hydroxide, aluminum nitrite, aluminum silicate, barium sulfate, calcium carbonate, titanium dioxide, calcium sulfate, silica, quartz flour, aerosil, alumina or wollastonite, and b) from 2 to 40% by weight of expandable graphite having a mean particle size in the range from 10 to 1000 μm, c) from 0 to 20% by weight of red phosphorus or an organic or inorganic phosphate, phosphite or phosphonate, d) from 0 to 10% by weight of carbon black or graphite, and processes for their preparation and use for preparing self-extinguishing polystyrene particle foams.
摘要翻译：含有无卤阻燃性的可发性苯乙烯聚合物颗粒，其包含a）5至50重量％的填料，其选自粉末状无机物质如滑石粉，白垩，高岭土，氢氧化铝，亚硝酸铝，硅酸铝，硫酸钡，钙碳酸盐，二氧化钛，硫酸钙，二氧化硅，石英粉，气溶胶，氧化铝或硅灰石，和b）2〜40重量％的平均粒径在10〜1000μm的可膨胀石墨，c）0 至20重量％的红磷或有机或无机磷酸盐，亚磷酸盐或膦酸盐，d）0至10重量％的炭黑或石墨，以及其制备和用于制备自熄性聚苯乙烯颗粒泡沫体的方法。

9. 发明申请

US20050156344A1 Method for producing expandable polystyrene 有权
标题翻译：生产可发性聚苯乙烯的方法
公开(公告)号：US20050156344A1
公开(公告)日：2005-07-21
申请号：US10516921
申请日：2003-06-06
申请人： Franz-Josef Dietzen , Gerd Ehrmann , Bernhard Schmied , Martin Laun , Klaus Hahn , Joachim Ruch , Markus Allmendinger , Jan Holoch , Achim Datko
发明人： Franz-Josef Dietzen , Gerd Ehrmann , Bernhard Schmied , Martin Laun , Klaus Hahn , Joachim Ruch , Markus Allmendinger , Jan Holoch , Achim Datko
IPC分类号： C08J9/00 , B29B9/10 , B29B11/10 , B29C44/34 , B29K25/00 , B29K105/04 , C08J9/16 , B29C44/00
CPC分类号： C08J9/16 , B29C44/3461 , C08J2325/04
摘要： A process for the preparation of expandable styrene polymers having a molecular weight Mw of greater than 170,000 g/mol, which comprises conveying a blowing agent-containing styrene polymer melt having a temperature of at least 120° C. through a die plate with holes whose diameter at the die exit is at most 1.5 mm, and subsequently granulating the extrudate, and expandable styrene polymers (EPS) having a molecular weight Mw of more than 170,000 g/mol with 0.05 to 1.5% by weight of internal water.
摘要翻译：一种制备分子量大于170,000g / mol的可发性苯乙烯聚合物的方法，其包括输送温度至少为120℃的含发泡剂的苯乙烯聚合物熔体通过具有在模具出口处的直径为至多1.5mm的孔的模具板，然后将挤出物造粒，并且具有大于170,000g的分子量M w的可膨胀的苯乙烯聚合物（EPS） /摩尔，含有0.05〜1.5重量％的内部水。

10. 发明授权

US08222307B2 Flameproof expandable styrene polymers, and method for the production thereof 有权
标题翻译：隔爆性可发性苯乙烯聚合物及其制造方法
公开(公告)号：US08222307B2
公开(公告)日：2012-07-17
申请号：US12743755
申请日：2008-11-20
申请人： Markus Allmendinger , Bernhard Schmied , Joachim Ruch , Konrad Knoll , Michael Riethues , Klaus Hahn , Carsten Schips , Jessica Rylander
发明人： Markus Allmendinger , Bernhard Schmied , Joachim Ruch , Konrad Knoll , Michael Riethues , Klaus Hahn , Carsten Schips , Jessica Rylander
IPC分类号： C08J9/16 , C08J9/14 , C08F290/06 , C08K5/02
CPC分类号： C08K5/0066 , C08J9/0019 , C08J9/0023 , C08J9/16 , C08J2201/03 , C08J2325/06 , C08K5/02 , C08K5/14 , C08L25/06
摘要： Expandable styrene polymers (EPS) comprising, in each case based on the styrene polymer, a) from 0.05 to 5% by weight of an organic bromine compound whose bromine content is at least 50% by weight, as flame retardant, b) from 0.05 to 2% by weight of a flame retardant synergist, c) from 0.1 to 5% by weight of a metal salt as acid scavenger, and process for their production.
摘要翻译：包括在每种情况下基于苯乙烯聚合物的可发射苯乙烯聚合物（a）a）0.05至5重量％的溴含量为至少50重量％的有机溴化合物作为阻燃剂，b）0.05 至2重量％的阻燃增效剂，c）0.1至5重量％的作为酸清除剂的金属盐及其制备方法。

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