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1. 发明授权

US06576120B1 Catalytic dewaxing process 有权
标题翻译：催化脱蜡工艺
公开(公告)号：US06576120B1
公开(公告)日：2003-06-10
申请号：US09856038
申请日：2001-05-16
申请人： Carolus Maria Van Ballegoy , Edward Julius Creyghton , Jean-Paul Darnanville , Eric Duprey , Laurent Georges Huve , Carolus Matthias Anna Maria Mesters , Thomas Joris Remans , Maria Barbara Hendrica Crijnen-Van Beers
发明人： Carolus Maria Van Ballegoy , Edward Julius Creyghton , Jean-Paul Darnanville , Eric Duprey , Laurent Georges Huve , Carolus Matthias Anna Maria Mesters , Thomas Joris Remans , Maria Barbara Hendrica Crijnen-Van Beers
IPC分类号： C10G1105
CPC分类号： C10G45/64 , B01J29/06 , B01J29/40 , B01J2229/16 , B01J2229/32 , B01J2229/42
摘要： The invention relates to a process for the catalytic dewaxing of a hydrocarbon feed containing waxy molecules by contacting the hydrocarbon feed under catalytic dewaxing conditions with a catalyst composition having metallosilicate crystallites, a binder and a hydrogenation component, wherein the weight ratio of the metallosilicate crystallites and the binder is between 5:95 and 35:65. The invention also relates to a catalyst composition having at least a low acidity refractory oxide binder, which binder is essentially free of aluminum, metallosilicate crystallites and a hydrogenation component, wherein the weight ratio of the metallosilicate crystallites and the binder is between 5:95 and 35:65.
摘要翻译：本发明涉及一种通过在催化脱蜡条件下使烃进料与具有金属硅酸盐微晶的催化剂组合物，粘合剂和氢化组分接触使含有蜡质分子的烃进料进行催化脱蜡的方法，其中金属硅酸盐微晶和粘合剂介于5:95至35:65之间。本发明还涉及至少具有低酸度难熔氧化物粘合剂的催化剂组合物，该粘合剂基本上不含铝，金属硅酸盐微晶和氢化组分，其中金属硅酸盐微晶和粘合剂的重量比为5:95至 35:65。

2. 发明授权

US06709570B1 Method for preparing a catalyst 有权
标题翻译：催化剂的制备方法
公开(公告)号：US06709570B1
公开(公告)日：2004-03-23
申请号：US09664293
申请日：2000-09-18
申请人： Maria Barbara Hendrica Van Crijnen-Beers , Jean-Paul Darnanville , Carolus Matthias Anna Maria Mesters , Thomas Joris Remans
发明人： Maria Barbara Hendrica Van Crijnen-Beers , Jean-Paul Darnanville , Carolus Matthias Anna Maria Mesters , Thomas Joris Remans
IPC分类号： C10G4700
CPC分类号： B01J29/40 , B01J29/06 , B01J37/0018 , C10G45/64 , Y10S502/514
摘要： A method for preparing a catalyst comprising a zeolite and a low acidity refractory oxide binder which is essentially free of alumina which method comprises: (a) preparing an extrudable mass comprising a substantially homogenous mixture of zeolite, water, a source of the low acidity refractory oxide binder present which comprises an acid sol, and an amine compound, (b) extruding the extrudable mass resulting from step (a), (c) drying the extrudate resulting from step (b); and, (d) calcining the dried extrudate resulting from step (c).
摘要翻译：一种制备催化剂的方法，所述催化剂包含基本上不含氧化铝的沸石和低酸度难熔氧化物粘合剂，所述方法包括：（a）制备包含沸石，水，低酸耐火材料源的基本上均匀的混合物的可挤出物料含有酸溶胶和胺化合物的氧化物粘合剂，（b）挤出步骤（a）得到的可挤出物料，（c）干燥由步骤（b）得到的挤出物; 和（d）煅烧由步骤（c）得到的干燥的挤出物。

3. 发明授权

US08455556B2 Fischer-Tropsch catalyst 有权
标题翻译：费 - 托催化剂
公开(公告)号：US08455556B2
公开(公告)日：2013-06-04
申请号：US12373464
申请日：2007-07-12
申请人： Ralph Haswell , Carolus Matthias Anna Maria Mesters , Heiko Oosterbeek , Thomas Joris Remans , Marinus Johannes Reynhout
发明人： Ralph Haswell , Carolus Matthias Anna Maria Mesters , Heiko Oosterbeek , Thomas Joris Remans , Marinus Johannes Reynhout
IPC分类号： C07C27/00 , C07C27/06
CPC分类号： B01J23/8472 , B01J23/75 , B01J23/8892 , B01J35/0006 , B01J35/0073 , B01J37/0238 , B01J37/0244 , B01J37/18 , C10G2/332
摘要： A process for the preparation of a packed bed comprising an iron enriched cobalt catalyst for use in a Fischer-Tropsch reaction, the process comprising the steps of: (a) providing a packed bed with one or more catalyst particles comprising metallic cobalt; (b) contacting a part of the catalyst particle(s) in the packed bed with an iron containing compound. The process is preferably conducted in situ which conveniently results in an iron containing cobalt catalyst with a higher C5+ selectivity. In certain preferred embodiments the concentration of iron increases towards the surface of the resulting catalyst particles whereas the cobalt concentration is constant which further increases the selectivity of the catalyst to producing C5+ hydrocarbons.
摘要翻译：一种用于制备包含用于费 - 托反应的富铁钴催化剂的填充床的方法，所述方法包括以下步骤：（a）向填充床提供一种或多种包含金属钴的催化剂颗粒; （b）使填充床中的一部分催化剂颗粒与含铁化合物接触。该方法优选原位进行，其方便地得到具有较高C5 +选择性的含铁钴催化剂。在某些优选实施方案中，铁的浓度朝向所得催化剂颗粒的表面增加，而钴浓度是恒定的，这进一步提高了催化剂生产C5 +烃的选择性。

4. 发明申请

US20100004346A1 FISCHER-TROPSCH CATALYST 有权
标题翻译： FISCHER-TROPSCH催化剂
公开(公告)号：US20100004346A1
公开(公告)日：2010-01-07
申请号：US12373464
申请日：2007-07-12
申请人： Ralph Haswell , Carolus Matthias Anna Maria Mesters , Heiko Oosterbeek , Thomas Joris Remans , Marinus Johannes Reynhout
发明人： Ralph Haswell , Carolus Matthias Anna Maria Mesters , Heiko Oosterbeek , Thomas Joris Remans , Marinus Johannes Reynhout
IPC分类号： C07C27/06 , B01J31/12 , B01J23/75 , B01J8/02
CPC分类号： B01J23/8472 , B01J23/75 , B01J23/8892 , B01J35/0006 , B01J35/0073 , B01J37/0238 , B01J37/0244 , B01J37/18 , C10G2/332
摘要： A process for the preparation of a packed bed comprising an iron enriched cobalt catalyst for use in a Fischer-Tropsch reaction, the process comprising the steps of: (a) providing a packed bed with one or more catalyst particles comprising metallic cobalt; (b) contacting a part of the catalyst particle(s) in the packed bed with an iron containing compound. The process is preferably conducted in situ which conveniently results in an iron containing cobalt catalyst with a higher C5+ selectivity. In certain preferred embodiments the concentration of iron increases towards the surface of the resulting catalyst particles whereas the cobalt concentration is constant which further increases the selectivity of the catalyst to producing C5+ hydrocarbons.
摘要翻译：一种用于制备包含用于费 - 托反应的富铁钴催化剂的填充床的方法，所述方法包括以下步骤：（a）向填充床提供一种或多种包含金属钴的催化剂颗粒; （b）使填充床中的一部分催化剂颗粒与含铁化合物接触。该方法优选原位进行，其方便地得到具有较高C5 +选择性的含铁钴催化剂。在某些优选实施方案中，铁的浓度朝向所得催化剂颗粒的表面增加，而钴浓度是恒定的，这进一步提高了催化剂生产C5 +烃的选择性。

5. 发明授权

US08933136B2 High-speed stop in Fischer-Tropsch process 有权
标题翻译：在费 - 托过程中高速停止
公开(公告)号：US08933136B2
公开(公告)日：2015-01-13
申请号：US12638647
申请日：2009-12-15
申请人： Gerrit Leendert Bezemer , Carolus Matthias Anna Maria Mesters , Thomas Joris Remans , Johannes Theodorus Maria Smits
发明人： Gerrit Leendert Bezemer , Carolus Matthias Anna Maria Mesters , Thomas Joris Remans , Johannes Theodorus Maria Smits
IPC分类号： C07C27/00 , B01J35/02 , B01J8/22 , C10G2/00 , B01J23/75 , B01J23/847 , B01J23/889
CPC分类号： B01J35/023 , B01J8/22 , B01J23/75 , B01J23/8472 , B01J23/8892 , B01J2208/00637 , C10G2/341
摘要： The present invention pertains to a process for carrying out a high-speed stop in a Fischer-Tropsch process which comprises providing a feed to a fixed bed reactor comprising a Fischer-Tropsch catalyst, the reactor being at reaction temperature and pressure, and withdrawing an effluent from the reactor, wherein the high-speed stop is effected by blocking provision of feed to the reactor and simultaneously blocking the withdrawal of effluent from the reactor.
摘要翻译：本发明涉及在费 - 托方法中进行高速停止的方法，该方法包括向包含费 - 托催化剂的固定床反应器提供进料，反应器处于反应温度和压力下，来自反应器的流出物，其中高速停止通过阻止向反应器提供进料并同时阻止流出物从反应器中排出来实现。

6. 发明授权

US07855236B2 Method to start a process for producing hydrocarbons from synthesis gas 有权
标题翻译：从合成气开始生产烃的方法
公开(公告)号：US07855236B2
公开(公告)日：2010-12-21
申请号：US12096412
申请日：2006-12-06
申请人： Robert Martijn Van Hardeveld , Hans Michiel Huisman , Lip Piang Kueh , Thomas Joris Remans
发明人： Robert Martijn Van Hardeveld , Hans Michiel Huisman , Lip Piang Kueh , Thomas Joris Remans
IPC分类号： C07C27/00
CPC分类号： C10G2/32 , C10G2300/1022 , C10G2300/4081
摘要： Method to start a steady state process for producing normally gaseous, normally liquid and optionally normally solid hydrocarbons from synthesis gas, which process comprises the steps of: (i) providing the synthesis gas; and (ii) catalytically converting the synthesis gas at an elevated temperature and a steady state total reactor pressure to obtain the normally gaseous, normally liquid and optionally normally solid hydrocarbons; the method comprising admixing the synthesis gas of step (i) with one or more inert gases to form an admixture stream prior to catalytically converting the synthesis gas in step (ii) at the steady state total reactor pressure and wherein as the activity of the catalyst converting the synthesis gas proceeds towards a steady state, the amount of inert gas(es) in the admixture stream is reduced.
摘要翻译：开始用于从合成气中产生通常为气态，通常为液态和任选通常为固体烃的稳态过程的方法，该方法包括以下步骤：（i）提供合成气; 和（ii）在升高的温度和稳态的总反应器压力下催化转化合成气以获得通常为气态的，通常为液体的和任选的通常为固体的烃; 该方法包括将步骤（i）的合成气与一种或多种惰性气体混合以在稳定状态的总反应器压力下催化转化步骤（ii）中的合成气之前形成混合物流，并且其中作为催化剂的活性合成气转化为稳定状态，混合物流中的惰性气体的量减少。

7. 发明申请

US20080275144A1 Method to Start a Process for Producing Hydrocarbons from Synthesis Gas 有权
标题翻译：从合成气体开始生产碳氢化合物的方法
公开(公告)号：US20080275144A1
公开(公告)日：2008-11-06
申请号：US12096412
申请日：2006-12-06
申请人： Robert Martijn Van Hardeveld , Hans Michiel Huisman , Lip Piang Kueh , Thomas Joris Remans
发明人： Robert Martijn Van Hardeveld , Hans Michiel Huisman , Lip Piang Kueh , Thomas Joris Remans
IPC分类号： C07C1/04
CPC分类号： C10G2/32 , C10G2300/1022 , C10G2300/4081
摘要： Method to start a steady state process for producing normally gaseous, normally liquid and optionally normally solid hydrocarbons from synthesis gas, which process comprises the steps of: (i) providing the synthesis gas; and (ii) catalytically converting the synthesis gas at an elevated temperature and a steady state total reactor pressure to obtain the normally gaseous, normally liquid and optionally normally solid hydrocarbons; the method comprising admixing the synthesis gas of step (i) with one or more inert gases to form an admixture stream prior to catalytically converting the synthesis gas in step (ii) at the steady state total reactor pressure and wherein as the activity of the catalyst converting the synthesis gas proceeds towards a steady state, the amount of inert gas(es) in the admixture stream is reduced.
摘要翻译：开始用于从合成气中产生通常为气态，通常为液态和任选通常为固体烃的稳态过程的方法，该方法包括以下步骤：（i）提供合成气; 和（ii）在升高的温度和稳态的总反应器压力下催化转化合成气以获得通常为气态的，通常为液体的和任选的通常为固体的烃; 该方法包括将步骤（i）的合成气与一种或多种惰性气体混合以在稳定状态的总反应器压力下催化转化步骤（ii）中的合成气之前形成混合物流，并且其中作为催化剂的活性合成气转化为稳定状态，混合物流中的惰性气体的量减少。

8. 发明申请

US20110160318A1 STACKED CATALYST BED FOR FISCHER-TROPSCH 有权
标题翻译：用于FISCHER-TROPSCH的堆叠催化剂床
公开(公告)号：US20110160318A1
公开(公告)日：2011-06-30
申请号：US12969158
申请日：2010-12-15
申请人： Alouisius Nicolaas Renée BOS , Peter John Van Den Brink , Thomas Joris Remans , Erwin Roderick Stobbe , Dominik Johannes Michael Unruh , Ronald Vladimir Wisman
发明人： Alouisius Nicolaas Renée BOS , Peter John Van Den Brink , Thomas Joris Remans , Erwin Roderick Stobbe , Dominik Johannes Michael Unruh , Ronald Vladimir Wisman
IPC分类号： C07C27/00 , B01J19/00
CPC分类号： B01J8/06 , B01J2208/00017 , B01J2208/00663 , B01J2208/00672 , B01J2208/00681 , B01J2208/025 , C10G2/341
摘要： The present invention pertains to a reactor tube comprising a fixed bed of Fischer-Tropsch catalyst particles, wherein the catalyst particles in 5% to 40% of the fixed bed volume at the upstream end have an average outer surface to volume ratio (S/V) in the range of between 3.0 to 4.5 mm−1, and the catalyst particles in the remaining fixed bed volume have an average outer surface to volume ratio (S/V) in the range of between 4.5 to 8.0 mm−1, and wherein the difference between the average S/V of the particles at the upstream end and the average S/V of the particles in the remaining fixed bed volume is at least 0.5 mm−1.
摘要翻译：本发明涉及一种包含费 - 托催化剂颗粒的固定床的反应器管，其中在上游端固定床体积的5％至40％的催化剂颗粒具有平均的外表面与体积比（S / V ）在3.0至4.5mm -1的范围内，剩余固定床体积中的催化剂颗粒的平均外表面与体积比（S / V）在4.5至8.0mm -1的范围内，其中在上游端的颗粒的平均S / V与剩余固定床体积中的颗粒的平均S / V之间的差为至少0.5mm-1。

9. 发明授权

US09005538B2 Stacked catalyst bed for Fischer-Tropsch 有权
标题翻译：堆叠的费 - 托催化剂床
公开(公告)号：US09005538B2
公开(公告)日：2015-04-14
申请号：US13535040
申请日：2012-06-27
申请人： Robert Martijn Van Hardeveld , Thomas Joris Remans , Erwin Roderick Stobbe
发明人： Robert Martijn Van Hardeveld , Thomas Joris Remans , Erwin Roderick Stobbe
IPC分类号： B01J8/06 , B01J8/04 , C10G2/00 , B01J35/02 , B01J8/02 , B01J35/00 , B01J23/75
CPC分类号： C10G2/00 , B01J8/025 , B01J8/06 , B01J8/067 , B01J23/75 , B01J35/0006 , B01J35/026 , B01J2208/00672 , B01J2208/025 , B01J2219/00038 , B01J2219/0004
摘要： The invention pertains to a reactor tube comprising a fixed bed of Fischer-Tropsch catalyst particles, wherein the catalyst particles in 5%-40% of the fixed bed volume at the upstream end have an average outer surface to volume ratio (S/V) of between 3.0 to 4.5 mm-1, and the remaining catalyst particles have an average S/V of between 4.5 to 8.0 mm-1, and wherein the difference between the average S/V of the particles at the upstream end and the remaining fixed bed volume is at least 0.5 mm-1. Additionally the fixed bed volume at the upstream end shows a full-bed apparent catalytic activity per volume unit lower than the full-bed apparent catalytic activity per volume unit in the remaining fixed bed volume and/or the weight of catalytically active metal per weight unit at the upstream end is more than 70% lower than in the remaining fixed bed volume.
摘要翻译：本发明涉及一种包含费 - 托催化剂颗粒固定床的反应器管，其中上游端固定床体积的5％-40％的催化剂颗粒具有平均的外表面与体积比（S / V）为3.0〜4.5mm -1，剩余的催化剂粒子的平均S / V为4.5〜8.0mm -1，上游侧的粒子的平均S / V与剩余的固定床体积至少为0.5mm-1。此外，上游端的固定床体积显示出比在剩余固定床体积中每单位体积单体的全床视在催化活性和/或每重量单位的催化活性金属重量的每体积单位的全床表观催化活性在上游端比剩下的固定床体积低70％以上。

10. 发明申请

US20100184873A1 MULTI STAGE PROCESS FOR PRODUCING HYDROCARBONS FROM SYNGAS 审中-公开
标题翻译：从SYNGAS生产石油烃的多阶段工艺
公开(公告)号：US20100184873A1
公开(公告)日：2010-07-22
申请号：US12640298
申请日：2009-12-17
申请人： Maarten Bracht , Maarten Hesselink , Christiaan Nijst , Thomas Joris Remans
发明人： Maarten Bracht , Maarten Hesselink , Christiaan Nijst , Thomas Joris Remans
IPC分类号： C07C27/06
CPC分类号： C10G2/30 , C10K3/06
摘要： The invention pertains to a multi-stage process for the production of hydrocarbons from syngas comprising hydrogen and carbon monoxide, which comprises the steps of: a) providing a fresh syngas feed to a first stage Fischer-Tropsch reactor and allowing CO and hydrogen to convert into hydrocarbon products at a temperature in the range from 125 to 400° C. and a pressure in the range from 5 to 150 bar absolute, and a gaseous hourly space velocity in the range from 500 to 10000 Nl/l/h; b) feeding the effluent from the first stage reactor to a separation unit; c) removing a gasous effluent stream comprising hydrogen and CO from the separation unit; d) removing one or more other streams comprising hydrocarbon and/or water from the separation unit; e) conveying a first portion of the gaseous effluent stream to a second stage Fischer-Tropsch reactor and allowing CO and hydrogen to convert into hydrocarbon products in the second stage Fischer-Tropsch reactor at a temperature in the range from 125 to 400° C. and a pressure in the range from 5 to 150 bar absolute, and a gaseous hourly space velocity in the range from 500 to 10000 Nl/l/h, whereby the first stage Fischer-Tropsch reactor and the second stage Fischer-Tropsch reactor are separate reactors; f) feeding the effluent from the second stage Fischer-Tropsch reactor to the separation unit; g) removing a second portion of the gaseous effluent stream as off-gas.
摘要翻译：本发明涉及用于从包含氢气和一氧化碳的合成气生产碳氢化合物的多级方法，其包括以下步骤：a）向新的第一阶段费 - 托反应器提供新的合成气进料并允许CO和氢转化在125至400℃的温度和5至150巴绝对压力的范围内的气体产物，并且气时空速在500至10000Nl / l / h的范围内; b）将来自第一级反应器的流出物供给到分离单元; c）从分离单元中除去包含氢和CO的气体流出物流; d）从分离单元去除包含烃和/或水的一种或多种其它流; e）将第一部分气态流出物流输送到第二级费 - 托反应器，并允许CO和氢在第二级费 - 托反应器中在125-400℃的温度下转化成烃产物。压力范围为5至150巴绝对压力，气时空速为500至10000Nl / l / h，其中第一级费 - 托反应器和第二级费 - 托反应器是分开的反应堆 f）将来自第二级费 - 托反应器的流出物供给到分离单元; g）除去作为废气的气态流出物流的第二部分。

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