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1. 发明申请

WO2006130280A3 SUPPORTS AND CATALYSTS COMPRISING RARE EARTH ALUMINATES, AND THEIR USE IN PARTIAL OXIDATION 审中-公开
标题翻译：包含稀土铝的支持和催化剂及其在部分氧化中的应用
公开(公告)号：WO2006130280A3
公开(公告)日：2007-11-15
申请号：PCT/US2006015952
申请日：2006-04-26
申请人： CONOCOPHILLIPS CO , ERCAN CEMAL , XIE SHUIBO , WRIGHT HAROLD A , JIN YAMING , WANG DAXIANG , FJARE KRISTI A , MINAHAN DAVID M , ORTEGO BEATRICE C , SIMON DAVID E
发明人： ERCAN CEMAL , XIE SHUIBO , WRIGHT HAROLD A , JIN YAMING , WANG DAXIANG , FJARE KRISTI A , MINAHAN DAVID M , ORTEGO BEATRICE C , SIMON DAVID E
IPC分类号： C01B3/26 , B01J21/04 , B01J21/10 , B01J21/12 , B01J23/00 , B01J23/63 , B01J23/75 , B01J23/89 , B01J37/06 , B01J37/08 , C01B3/38 , C01B3/40
CPC分类号： C01B3/386 , B01J21/04 , B01J21/10 , B01J21/12 , B01J23/002 , B01J23/10 , B01J23/40 , B01J23/464 , B01J23/63 , B01J23/75 , B01J23/8913 , B01J35/002 , B01J35/0053 , B01J35/0066 , B01J35/08 , B01J35/1009 , B01J35/1038 , B01J35/1061 , B01J37/0207 , B01J37/0244 , B01J37/06 , B01J37/08 , B01J37/18 , B01J2523/00 , C01B3/40 , C01B2203/0261 , C01B2203/062 , C01B2203/1011 , C01B2203/1041 , C01B2203/1047 , C01B2203/1064 , C01B2203/1082 , C01B2203/1094 , C01B2203/1241 , C01B2203/1247 , Y02P20/52 , B01J2523/31 , B01J2523/3706 , B01J2523/3737 , B01J2523/822
摘要： The present invention relates to thermally stable supports and catalysts for use in high temperature operation, and methods of preparing such supports and catalysts, which includes adding a rare earth metal to an aluminum-containing precursor prior to calcining. The present invention can be more specifically seen as a support, process and catalyst wherein the thermally stable support comprises two rare earth aluminates of different molar ratios of aluminum to rare earth metal, and optionally, alumina and/or a rare earth oxide. More particularly, the invention relates to the use of noble metal catalysts comprising the thermally stable support for synthesis gas production via partial oxidation of light hydrocarbon (e.g., methane) with minimal deactivation over long-term operations and further relates to gas-to-liquids conversion processes.
摘要翻译：本发明涉及用于高温操作的热稳定性载体和催化剂，以及制备这种载体和催化剂的方法，其包括在煅烧之前向含铝前体中加入稀土金属。本发明可以更具体地看作是一种载体，方法和催化剂，其中热稳定载体包括两种不同摩尔比的铝与稀土金属的稀土铝酸盐，以及任选的氧化铝和/或稀土氧化物。更具体地说，本发明涉及贵金属催化剂的用途，所述催化剂包括热稳定性载体，用于通过在长期操作下具有最小失活的轻质烃（例如甲烷）的部分氧化产生合成气，并且还涉及气体 - 液体转换过程。

2. 发明申请

WO9617940A2 METHOD OF DESULFURIZATION OF FOSSIL FUEL WITH FLAVOPROTEIN 审中-公开
标题翻译： FASIL燃料与FLAVOPROTEIN的脱硫方法
公开(公告)号：WO9617940A2
公开(公告)日：1996-06-13
申请号：PCT/US9515865
申请日：1995-12-05
申请人： ENERGY BIOSYSTEMS CORP , SQUIRES CHARLES H , JI WAN , XI LEI , ORTEGO BEATRICE C , POGREBINSKY OLGA S , GRAY KEVIN A , CHILDS JOHN D
发明人： SQUIRES CHARLES H , JI WAN , XI LEI , ORTEGO BEATRICE C , POGREBINSKY OLGA S , GRAY KEVIN A , CHILDS JOHN D
IPC分类号： C12N15/09 , C10G32/00 , C10L1/04 , C12N1/21 , C12N9/02 , C12N15/00 , C12N15/53 , C12P1/00 , C12R1/01 , C12R1/19 , C12S1/02 , C12N15/52
CPC分类号： C12N9/0036 , C10G32/00 , C12P1/00 , C12R1/01
摘要： The invention relates to the discovery that the rate of reaction of the desulfurization of fossil fuels is enhanced by the addition of a flavoprotein to the biocatalyst. The invention is drawn to a method for enhancing the rate of desulfurizing a fossil fuel containing organic sulfur compounds, comprising the steps of: a) contacting the fossil fuel with an aqueous phase containing a biocatalyst capable of cleaving carbon-sulfur bonds and a rate-enhancing amount of a flavoprotein, thereby forming a fossil fuel and aqueous phase mixture; b) maintaining the mixture of step (a) under conditions sufficient for cleavage of the carbon-sulfur bonds of the organic sulfur molecules by the biocatalyst, thereby resulting in a fossil fuel having a reduced organic sulfur content; and c) separating the fossil fuel having a reduced organic sulfur content from the resulting aqueous phase. The invention also relates to a recombinant microorganism containing one or more recombinant DNA molecules which encode a biocatalyst capable of desulfurizing a fossil fuel containing organic sulfur molecules and which encode a flavoprotein. The invention also relates to a composition comprising (a) a biocatalyst capable of desulfurizing a fossil fuel containing organic sulfur molecules and (b) a flavoprotein.
摘要翻译：本发明涉及通过向生物催化剂中加入黄素蛋白来提高化石燃料脱硫反应速率的发现。本发明涉及提高含有机硫化合物的化石燃料脱硫速率的方法，包括以下步骤：a）使化石燃料与含有能够裂解碳 - 硫键的生物催化剂的水相接触，增加量的黄素蛋白，从而形成化石燃料和水相混合物; b）将步骤（a）的混合物保持在足以通过生物催化剂裂解有机硫分子的碳 - 硫键的条件下，从而导致具有降低的有机硫含量的化石燃料; 和c）从所得水相中分离具有降低的有机硫含量的化石燃料。本发明还涉及含有一种或多种重组DNA分子的重组微生物，所述重组DNA分子编码能够脱硫含有有机硫分子的化石燃料并且编码黄素蛋白的生物催化剂。本发明还涉及包含（a）能够使含有有机硫分子的化石燃料脱硫的生物催化剂和（b）黄素蛋白的组合物。

3. 发明申请

WO2004007406A3 METHOD FOR REDUCING THE MAXIMUM WATER CONCENTRATION IN A MULTI-PHASE COLUMN REACTOR 审中-公开
标题翻译：减少多相柱反应器中最大水分浓度的方法
公开(公告)号：WO2004007406A3
公开(公告)日：2005-06-30
申请号：PCT/US0321560
申请日：2003-07-10
申请人： CONOCOPHILLIPS CO
发明人： ZHANG JIANPING , ESPINOZA RAFAEL L , MOHEDAS SERGIO R , ORTEGO BEATRICE C
IPC分类号： B01D12/00 , B01D17/12 , B01D21/00 , B01F13/02 , B01J8/22 , C07C27/00 , C07C27/06 , C07C27/26 , C10G2/00 , B01D3/14 , B01D3/34 , B01D3/42 , B01D11/00 , B01D15/00 , B01D21/26 , B01D37/00 , B01D63/00
CPC分类号： C10G2/342 , B01F13/0255 , B01J8/22
摘要： The present invention relates to a method and apparatus for reducing the maximum water concentration in multi-phase reactors operating at Fischer-Tropsch conditions. In a preferred embodiment of the present invention, a method of reducing the maximum concentration of water in a multi-phase reactor containing an expanded slurry bed and a water-rich slurry region for Fisher-Tropsch synthesis includes changing the flow structure of a predetermined region in the reactor. The flow structure may be changed by introducing a mixing enhancing fluid into the predetermined region, installing baffles into the predetermined region, or by other methods known in the art. Preferably the predetermined region is located between 1/2 H and H and between 1/2 R and R, where H is the height of the expanded slurry bed and R is the radius of the reactor.
摘要翻译：本发明涉及用于降低在费 - 托条件下操作的多相反应器中的最大水浓度的方法和装置。在本发明的一个优选实施方案中，一种减少含有膨胀浆料床和用于费 - 托合成的富水浆料区域的多相反应器中的水的最大浓度的方法包括改变预定区域的流动结构在反应堆。可以通过将混合增强流体引入预定区域，将挡板安装到预定区域中，或通过本领域已知的其它方法来改变流动结构。优选地，预定区域位于1/2H和H之间以及1/2R和R之间，其中H是发泡浆料床的高度，R是反应器的半径。

4. 发明申请

WO2004035511A3 FISCHER-TROPSCH PROCESSES AND CATALYSTS USING STABILIZED SUPPORTS 审中-公开
标题翻译： FISCHER-TROPSCH工艺和使用稳定支撑的催化剂
公开(公告)号：WO2004035511A3
公开(公告)日：2004-08-05
申请号：PCT/US0332798
申请日：2003-10-16
申请人： CONOCOPHILLIPS CO
发明人： ORTEGO JAMES DALE , JOTHIMURUGESAN KANDASWAMY , ESPINOZA RAFAEL L , COY KEVIN L , ORTEGO BEATRICE C
IPC分类号： B01J31/10 , B01J21/00 , B01J21/04 , B01J21/06 , B01J21/12 , B01J23/74 , B01J23/89 , B01J31/00 , B01J32/00 , B01J35/10 , B01J37/02 , C10G2/00 , B01J23/00 , B01J23/40 , B01J23/58 , C07C27/00
CPC分类号： B01J37/0207 , B01J21/005 , B01J21/04 , B01J21/06 , B01J21/12 , B01J23/74 , B01J23/8913 , B01J35/1014 , B01J35/1038 , B01J35/1061 , B01J37/0205 , C10G2/332
摘要： A catalyst and method for producing hydrocarbons using a catalyst support having an improved hydrothermal stability, such as under Fischer-Tropsch synthesis conditions. The stabilized support is made by a method comprising treating a boehmite material in contact with at least one structural stabilizer. Contacting the boehmite with at least one structural stabilizer can include forming a mixture comprising the boehmite material and at the least one structural stabilizer. The mixture can be a sol or a slurry. The treating preferably includes drying or spray drying the mixture, and calcining in an oxidizing atmosphere to obtain the stabilized support. Preferred structural stabilizers can include an element, such as cobalt, magnesium, zirconium, boron, aluminum, barium, silicon, lanthanum, oxides thereof, or combinations thereof; or can include precipitated oxides, such as a co-precipitated silica-alumina.
摘要翻译：使用具有改进的水热稳定性的催化剂载体，例如在费 - 托合成条件下生产烃的催化剂和方法。稳定的载体通过包括处理与至少一种结构稳定剂接触的勃姆石材料的方法制备。使勃姆石与至少一种结构稳定剂接触可以包括形成包含勃姆石材料和至少一种结构稳定剂的混合物。该混合物可以是溶胶或浆液。处理优选包括干燥或喷雾干燥混合物，并在氧化气氛中煅烧以获得稳定的载体。优选的结构稳定剂可以包括元素，例如钴，镁，锆，硼，铝，钡，硅，镧，其氧化物或其组合; 或者可以包括沉淀氧化物，例如共沉淀二氧化硅 - 氧化铝。

5. 发明专利

ZA200707949B Stabilized boehmite-derived catalyst supports, catalysts, methods of making and using 未知
公开(公告)号：ZA200707949B
公开(公告)日：2008-12-31
申请号：ZA200707949
申请日：2006-03-27
申请人： CONOCOPHILLIPS CO
发明人： ESPINOZA RAFAEL L , KANDASWAMY JOTHIMURUGESAN , YAMING JIN , DALE ORTEGO JR J , FJARE KRISTI A , ORTEGO BEATRICE C
IPC分类号： B01J20090101 , B01J21/04 , B01J23/89 , B01J32/00 , B01J35/02 , B01J35/10 , B01J37/00 , C07C20090101 , C07C27/06 , C10G2/00
摘要： A stabilized catalyst support having improved hydrothermal stability, catalyst made therefrom, and method for producing hydrocarbons from synthesis gas using said catalyst. The stabilized support is made by a method comprising treating a crystalline hydrous alumina precursor in contact with at least one structural stabilizer or compound thereof. The crystalline hydrous alumina precursor preferably includes an average crystallite size selected from an optimum range delimited by desired hydrothermal resistance and desired porosity. The crystalline hydrous alumina precursor preferably includes an alumina hydroxide, such as crystalline boehmite, crystalline bayerite, or a plurality thereof differing in average crystallite sizes by at least about 1 nm. The crystalline hydrous alumina precursor may be shaped before or after contact with the structural stabilizer or compound thereof. The treating includes calcining at 450° C. or more. Preferred structural stabilizers can include cobalt, magnesium, manganese, manganese, zirconium, boron, aluminum, barium, silicon, lanthanum, oxides thereof, or combinations thereof.

6. 发明专利

AU2003277409A1 FISCHER-TROPSCH PROCESSES AND CATALYSTS USING STABILIZED SUPPORTS 未知
公开(公告)号：AU2003277409A1
公开(公告)日：2004-05-04
申请号：AU2003277409
申请日：2003-10-16
申请人： CONOCOPHILLIPS CO
发明人： ORTEGO JAMES DALE , ORTEGO BEATRICE C , JOTHIMURUGESAN KANDASWAMY , ESPINOZA RAFAEL L , COY KEVIN L
IPC分类号： B01J31/10 , B01J21/00 , B01J21/04 , B01J21/06 , B01J21/12 , B01J23/74 , B01J23/89 , B01J31/00 , B01J32/00 , B01J35/10 , B01J37/02 , C10G2/00

7. 发明公开

EP1569880A4 FISCHER-TROPSCH PROCESSES AND CATALYSTS USING STABILIZED SUPPORTS 审中-公开
标题翻译：费 - 托工艺和具有稳定承运人催化剂
公开(公告)号：EP1569880A4
公开(公告)日：2008-04-09
申请号：EP03809064
申请日：2003-10-16
申请人： CONOCOPHILLIPS CO
发明人： ORTEGO JAMES DALE , JOTHIMURUGESAN KANDASWAMY , ESPINOZA RAFAEL L , COY KEVIN L , ORTEGO BEATRICE C
IPC分类号： B01J31/10 , B01J21/00 , B01J21/04 , B01J21/06 , B01J21/12 , B01J23/74 , B01J23/89 , B01J31/00 , B01J32/00 , B01J35/10 , B01J37/02 , C10G2/00
CPC分类号： B01J37/0207 , B01J21/005 , B01J21/04 , B01J21/06 , B01J21/12 , B01J23/74 , B01J23/8913 , B01J35/1014 , B01J35/1038 , B01J35/1061 , B01J37/0205 , C10G2/332
摘要： A catalyst and method for producing hydrocarbons using a catalyst support having an improved hydrothermal stability, such as under Fischer-Tropsch synthesis conditions. The stabilized support is made by a method comprising treating a boehmite material in contact with at least one structural stabilizer. Contacting the boehmite with at least one structural stabilizer can include forming a mixture comprising the boehmite material and at the least one structural stabilizer. The mixture can be a sol or a slurry. The treating preferably includes drying or spray drying the mixture, and calcining in an oxidizing atmosphere to obtain the stabilized support. Preferred structural stabilizers can include an element, such as cobalt, magnesium, zirconium, boron, aluminum, barium, silicon, lanthanum, oxides thereof, or combinations thereof; or can include precipitated oxides, such as a co-precipitated silica-alumina.

8. 发明公开

EP1569869A4 STABILIZED ALUMINA SUPPORTS, CATALYSTS MADE THEREFROM, AND THEIR USE IN PARTIAL OXIDATION 审中-公开
标题翻译：稳定的氧化铝载体，催化剂由其制得和他们的部分氧化VERWENUDNG
公开(公告)号：EP1569869A4
公开(公告)日：2008-11-19
申请号：EP03786654
申请日：2003-11-12
申请人： CONOCOPHILLIPS CO
发明人： RAPIER CHARLES R , XIE SHUIBO , HU BAILI , ORTEGO BEATRICE C , SIMON DAVID E , MINAHAN DAVID M , ERCAN CEMAL
IPC分类号： B01J21/04 , B01J21/10 , B01J21/12 , B01J23/00 , B01J23/10 , B01J23/40 , B01J23/46 , B01J23/56 , B01J23/63 , B01J23/656 , B01J23/75 , B01J23/89 , B01J35/00 , B01J35/10 , B01J37/02 , B01J37/06 , B01J37/08 , C01B3/26 , C01B3/38 , C01B3/40 , C07C27/06 , C10G2/00 , C01B3/42 , C01B3/56
CPC分类号： C01B3/40 , B01J21/04 , B01J21/10 , B01J21/12 , B01J23/002 , B01J23/10 , B01J23/40 , B01J23/464 , B01J23/468 , B01J23/56 , B01J23/63 , B01J23/6567 , B01J23/75 , B01J23/8913 , B01J35/002 , B01J35/0026 , B01J35/0053 , B01J35/1014 , B01J35/1019 , B01J37/0201 , B01J37/06 , B01J37/08 , B01J2523/00 , C01B3/386 , C01B2203/0261 , C01B2203/062 , C01B2203/1011 , C01B2203/1017 , C01B2203/1041 , C01B2203/1047 , C01B2203/1052 , C01B2203/1064 , C01B2203/1082 , C01B2203/1094 , C01B2203/1241 , C01B2203/1633 , C10G2/30 , Y02P20/52 , B01J2523/31 , B01J2523/3706 , B01J2523/22 , B01J2523/3737 , B01J2523/822 , B01J2523/821 , B01J2523/845 , B01J2523/41
摘要： The present invention relates to stabilized supports stable at temperatures above 800 °C, and method of preparing such supports, which includes adding a rare earth metal to an aluminum-containing precursor prior to calcining. The present invention can be more specifically seen as a support, process and catalyst wherein the stabilized alumina catalyst support comprises a rare earth aluminate with a molar ratio of aluminum to rare earth metal greater than 5:1 and, optionally, an aluminum oxide. More particularly, the invention relates to the use of catalysts comprising rhodium, ruthenium, iridium, or combinations thereof, loaded onto said stabilized supports for the synthesis gas production via partial oxidation of light hydrocarbons, and further relates to gas-to-liquids conversion processes.

9. 发明专利

NO20052349L 未知
公开(公告)号：NO20052349L
公开(公告)日：2005-08-10
申请号：NO20052349
申请日：2005-05-12
申请人： CONOCOPHILLIPS CO
发明人： RAPIER CHARLES R , XIE SHUIBO , HU BAILI , ORTEGO BEATRICE C , SIMON DAVID E , MINAHAN DAVID M
IPC分类号： B01J21/04 , B01J21/10 , B01J21/12 , B01J23/00 , B01J23/10 , B01J23/40 , B01J23/46 , B01J23/56 , B01J23/63 , B01J23/656 , B01J23/75 , B01J23/89 , B01J35/00 , B01J35/10 , B01J37/02 , B01J37/06 , B01J37/08 , C01B3/26 , C01B3/38 , C01B3/40 , C07C27/06 , C10G2/00
摘要： The present invention relates to stabilized supports stable at temperatures above 800° C., and method of preparing such supports, which includes adding a rare earth metal to an aluminum-containing precursor prior to calcining. The present invention can be more specifically seen as a support, process and catalyst wherein the stabilized alumina catalyst support comprises a rare earth aluminate with a molar ratio of aluminum to rare earth metal greater than 5:1 and, optionally, an aluminum oxide. More particularly, the invention relates to the use of catalysts comprising rhodium, ruthenium, iridium, or combinations thereof, loaded onto said stabilized supports for the synthesis gas production via partial oxidation of light hydrocarbons, and further relates to gas-to-liquids conversion processes.

10. 发明专利

NO20052349D0 未知
公开(公告)号：NO20052349D0
公开(公告)日：2005-05-12
申请号：NO20052349
申请日：2005-05-12
申请人： CONOCOPHILLIPS CO
发明人： RAPIER CHARLES R , XIE SHUIBO , HU BAILI , ORTEGO BEATRICE C , SIMON DAVID E , MINAHAN DAVID M
IPC分类号： B01J21/04 , B01J21/10 , B01J21/12 , B01J23/00 , B01J23/10 , B01J23/40 , B01J23/46 , B01J23/56 , B01J23/63 , B01J23/656 , B01J23/75 , B01J23/89 , B01J35/00 , B01J35/10 , B01J37/02 , B01J37/06 , B01J37/08 , C01B3/26 , C01B3/38 , C01B3/40 , C07C27/06 , C10G2/00 , C01B
摘要： The present invention relates to stabilized supports stable at temperatures above 800° C., and method of preparing such supports, which includes adding a rare earth metal to an aluminum-containing precursor prior to calcining. The present invention can be more specifically seen as a support, process and catalyst wherein the stabilized alumina catalyst support comprises a rare earth aluminate with a molar ratio of aluminum to rare earth metal greater than 5:1 and, optionally, an aluminum oxide. More particularly, the invention relates to the use of catalysts comprising rhodium, ruthenium, iridium, or combinations thereof, loaded onto said stabilized supports for the synthesis gas production via partial oxidation of light hydrocarbons, and further relates to gas-to-liquids conversion processes.

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