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1. 发明授权

US4847227A Solid catalyst component for olefin polymerization catalysts 失效
标题翻译：烯烃聚合催化剂的固体催化剂组分
公开(公告)号：US4847227A
公开(公告)日：1989-07-11
申请号：US105586
申请日：1987-10-08
申请人： Atsushi Murai , Minoru Terano , Kohei Kimura , Masuo Inoue , Katsuyoshi Miyoshi
发明人： Atsushi Murai , Minoru Terano , Kohei Kimura , Masuo Inoue , Katsuyoshi Miyoshi
IPC分类号： C08F4/60 , C08F4/64 , C08F4/658 , C08F10/00
CPC分类号： C08F10/00
摘要： A solid catalyst component for olefin polymerization catalysts prepared by suspending diethoxymagnesium (a) in an aromatic hydrocarbon (b) which is liquid at normal temperature and bringing the suspension into a first contact with titanium tetrachloride (c) to form a product and bringing it into a second contact with tianium tetrachloride (c) in such manner that a diester (d) of an aromatic dicarboxylic acid and calcium chloride (e) are allowed to coexist at any stage of the above suspending and/or contacts, the calcium chloride (e) being used in an amount of 1-2 grams per gram of the diethoxymagnesium (a). This solid catalyst component exhibits, when applied to the polymerization of olefins, a surprisingly enhanced polymerization activity per titanium atom and a high stereospecific performance and scarcely necessitates any deashing treatment, thus affording a great economical advantage.
摘要翻译：一种用于烯烃聚合催化剂的固体催化剂组分，其通过将二乙氧基镁（a）悬浮在常温下为液体的芳族烃（b）中并使悬浮液与四氯化钛（c）首次接触形成产物并使其进入与四氯化钛（c）的第二次接触，使得芳族二羧酸和氯化钙（e）的二酯（d）在上述悬浮和/或接触的任何阶段共存，氯化钙（e ）的用量为每克二乙氧基镁（a）1-2克。当用于烯烃聚合时，该固体催化剂组分表现出惊人的增加的每个钛原子的聚合活性和高立体特异性性能，并且几乎不需要任何脱屑处理，从而提供了巨大的经济优势。

2. 发明授权

US4839321A Solid catalyst component for olefin polymerization catalysts 失效
标题翻译：用于烯烃聚合催化剂的固体催化剂组分
公开(公告)号：US4839321A
公开(公告)日：1989-06-13
申请号：US141523
申请日：1988-01-07
申请人： Atsushi Murai , Minoru Terano , Kohei Kimura , Masuo Inoue
发明人： Atsushi Murai , Minoru Terano , Kohei Kimura , Masuo Inoue
IPC分类号： C08F4/60 , C08F4/64 , C08F4/658 , C08F10/00
CPC分类号： C08F10/00
摘要： A solid catalyst component for olefin polymerization catalysts prepared by subjecting diethoxymagnesium (a), calcium chloride (b) and a silicon compound (c) of the general formula: Si(OR).sub.4 (wherein R is an alkyl or aryl group) together to a contact treatment in the presence of an organic solvent (d), suspending the treated composition in an aromatic hydrocarbon (e) which is liquid at normal temperature and bringing the suspension into a first contact with titanium tetrachloride (f) to form a product and bringing it to a second contact with titanium tetrachloride (f) in such manner that a diester (g) of an aromatic dicarboxylic acid is allowed to coexist at any stage of the above suspending and/or contacts with the exception of the contact treatment, the calcium chloride (b) being used in an amount of 1-2 g per gram of the diethoxymagnesium (a). This solid catalyst component exhibits, when applied to the polymerization of olefins, a surprisingly enhanced polymerization activity per titanium atom and a high stereospecific performance and scarcely necessitates any deashing treatment, thus affording a great economical advantage.
摘要翻译：将通式为Si（OR）4（其中R为烷基或芳基）的二乙氧基镁（a），氯化钙（b）和硅化合物（c））（其中R为烷基或芳基）一起制备的烯烃聚合催化剂固体催化剂组分在有机溶剂（d）的存在下进行接触处理，将经处理的组合物悬浮在常温下为液态的芳烃（e）中，并使悬浮液与四氯化钛（f）进行第一次接触以形成产物，使其与四氯化钛（f）进行第二次接触，使得除了接触处理之外，在上述悬浮和/或接触的任何阶段允许芳族二羧酸的二酯（g）共存，氯化钙（b）的用量为每克二乙氧基镁（a）1-2克。当用于烯烃聚合时，该固体催化剂组分表现出惊人的增加的每个钛原子的聚合活性和高立体特异性性能，并且几乎不需要任何脱屑处理，从而提供了巨大的经济优势。

3. 发明授权

US4829037A Catalyst for polymerization of olefins 失效
标题翻译：烯烃聚合催化剂
公开(公告)号：US4829037A
公开(公告)日：1989-05-09
申请号：US150650
申请日：1988-01-05
申请人： Minoru Terano , Hirokazu Soga , Kohei Kimura
发明人： Minoru Terano , Hirokazu Soga , Kohei Kimura
IPC分类号： C08F4/64 , C08F10/00
CPC分类号： C08F10/00 , Y10S526/903
摘要： A catalyst for the polymerization of olefins which exhibits a high catalytic activity and is capable of producing a stereoregular polymer in a high yield. The catalyst includes a catalyst component for the polymerization of olefins prepared by subjecting a solid composition obtained by a process comprising contacting dialkoxymagnesium, diester of aromatic dicarboxylic acid, aromatic hydrocarbon and titanium halide to a heat treatment in the presence or absence of a solvent; a silicon compound; and an organic aluminum compound.
摘要翻译： PCT No.PCT / JP87 / 00278 Sec。 371日期1988年1月5日第 102（e）日期1988年1月5日PCT提交1987年5月6日PCT公布。第WO87 / 06945号公报日期：1987年11月19日。用于烯烃聚合的催化剂，其表现出高催化活性并且能够以高产率制备立体有规聚合物。催化剂包括用于烯烃聚合的催化剂组分，其通过使含有二烷氧基镁，芳族二羧酸二酯，芳族烃和卤化钛的方法得到的固体组合物在溶剂存在或不存在下进行热处理而制备。硅化合物; 和有机铝化合物。

4. 发明申请

US20120053310A1 Aminosilane Compounds, Catalyst Components and Catalysts for Olefin Polymerization, and Process for Production of Olefin Polymers with the Same 有权
标题翻译：用于烯烃聚合的氨基硅烷化合物，催化剂组分和催化剂及其生产烯烃聚合物的方法
公开(公告)号：US20120053310A1
公开(公告)日：2012-03-01
申请号：US13289728
申请日：2011-11-04
申请人： Motoki Hosaka , Takefumi Yano , Maki Sato , Kohei Kimura
发明人： Motoki Hosaka , Takefumi Yano , Maki Sato , Kohei Kimura
IPC分类号： C08F4/52 , C07F7/10 , C08F4/72
CPC分类号： C07F7/10 , C08F10/00 , C08F110/06 , C08F4/6492 , C08F4/6495 , C08F4/65927 , C08F2500/18 , C08F2500/12 , C08F2500/04 , C08F4/6465 , C08F4/6548 , C08F4/6565
摘要： A catalyst for polymerization of olefins formed from (A) a solid catalyst component containing magnesium, titanium, halogen, and an electron donor compound, (B) an organoaluminum compound shown by the formula, R6pAlQ3-p, and (C) an aminosilane compound shown by the formula, R3nSi(NR4R5)4-n; and a process for producing a catalyst for polymerization of olefins in the presence of the catalyst are provided. A novel aminosilane compound, a catalyst component for polymerization of olefins having a high catalytic activity, capable of producing polymers with high stereoregularity in a high yield, and exhibiting an excellent hydrogen response, a catalyst, and a process for producing olefin polymers using the catalyst are provided.
摘要翻译：由（A）含有镁，钛，卤素和电子给体化合物的固体催化剂组分形成的烯烃聚合催化剂，（B）由式R6pAlQ3-p表示的有机铝化合物和（C）氨基硅烷化合物如下式所示：R3nSi（NR4R5）4-n; 提供了在催化剂存在下制备烯烃聚合催化剂的方法。一种新型氨基硅烷化合物，具有高催化活性的烯烃聚合催化剂组分，能够以高产率制备具有高立构规整性的聚合物，并表现出优异的氢响应，催化剂和使用该催化剂生产烯烃聚合物的方法被提供。

5. 发明申请

US20100190942A1 AMINOSILANE COMPOUNDS, CATALYST COMPONENTS AND CATALYSTS FOR OLEFIN POLYMERIZATION, AND PROCESS FOR PRODUCTION OF OLEFIN POLYMERS WITH THE SAME 审中-公开
标题翻译：用于烯烃聚合的氨基甲酸酯化合物，催化剂组分和催化剂以及用于生产烯烃聚合物的方法
公开(公告)号：US20100190942A1
公开(公告)日：2010-07-29
申请号：US11916039
申请日：2006-05-26
申请人： Motoki Hosaka , Takefumi Yano , Maki Sato , Kohei Kimura
发明人： Motoki Hosaka , Takefumi Yano , Maki Sato , Kohei Kimura
IPC分类号： C08F2/00 , C07F7/10 , C08F4/602
CPC分类号： C07F7/10 , C08F10/00 , C08F110/06 , C08F4/6492 , C08F4/6495 , C08F4/65927 , C08F2500/18 , C08F2500/12 , C08F2500/04 , C08F4/6465 , C08F4/6548 , C08F4/6565
摘要： A catalyst for polymerization of olefins formed from (A) a solid catalyst component containing magnesium, titanium, halogen, and an electron donor compound, (B) an organoaluminum compound shown by the formula, R6pAlQ3-p, and (C) an aminosilane compound shown by the formula, R3nSi(NR4R5)4-n; and a process for producing a catalyst for polymerization of olefins in the presence of the catalyst are provided. A novel aminosilane compound, a catalyst component for polymerization of olefins having a high catalytic activity, capable of producing polymers with high stereoregularity in a high yield, and exhibiting an excellent hydrogen response, a catalyst, and a process for producing olefin polymers using the catalyst are provided.
摘要翻译：由（A）含有镁，钛，卤素和电子给体化合物的固体催化剂组分形成的烯烃聚合催化剂，（B）由式R6pAlQ3-p表示的有机铝化合物和（C）氨基硅烷化合物如下式所示：R3nSi（NR4R5）4-n; 提供了在催化剂存在下制备烯烃聚合催化剂的方法。一种新型氨基硅烷化合物，具有高催化活性的烯烃聚合催化剂组分，能够以高产率制备具有高立构规整性的聚合物，并表现出优异的氢响应，催化剂和使用该催化剂生产烯烃聚合物的方法被提供。

6. 发明授权

US08247504B2 Catalyst component, catalyst for olefin polymerization, and process for producing olefin polymer using catalyst 有权
标题翻译：催化剂组分，烯烃聚合催化剂和使用催化剂生产烯烃聚合物的方法
公开(公告)号：US08247504B2
公开(公告)日：2012-08-21
申请号：US11997924
申请日：2006-08-04
申请人： Takefumi Yano , Motoki Hosaka , Maki Sato , Kohei Kimura
发明人： Takefumi Yano , Motoki Hosaka , Maki Sato , Kohei Kimura
IPC分类号： C08F4/44 , C07F7/02 , B01J31/00 , B01J37/00 , C08K3/34
CPC分类号： C08F10/00 , C07F7/1804 , C08F110/06 , C08F4/6465 , C08F2500/12 , C08F2500/18 , C08F2500/04
摘要： A polymer having high catalyst activity, excellent hydrogen response, high stereoregularity and high yield can be obtained by polymerizing olefins in the presence of a catalyst for olefin polymerization comprising (A) a solid catalyst component containing magnesium, titanium, a halogen, and an electron donor compound, (B) an organoaluminum compound shown by the formula R6pAlQ3-p(R1R2N)m, and (C) an aminosilane compound shown by the formula (R3HN)nR4pSi(OR5)q.
摘要翻译：通过在烯烃聚合催化剂存在下聚合烯烃，可以获得具有高催化剂活性，优异的氢响应，高立构规整性和高收率的聚合物，其包含（A）含有镁，钛，卤素和电子的固体催化剂组分供体化合物，（B）式R6pAlQ3-p（R1R2N）m所示的有机铝化合物，（C）由式（R3HN）nR4pSi（OR5）q表示的氨基硅烷化合物。

7. 发明授权

US08648001B2 Aminosilane compounds, catalyst components and catalysts for olefin polymerization, and process for production of olefin polymers with the same 有权
标题翻译：用于烯烃聚合的氨基硅烷化合物，催化剂组分和催化剂，以及用于生产烯烃聚合物的方法
公开(公告)号：US08648001B2
公开(公告)日：2014-02-11
申请号：US13289728
申请日：2011-11-04
申请人： Motoki Hosaka , Takefumi Yano , Maki Sato , Kohei Kimura
发明人： Motoki Hosaka , Takefumi Yano , Maki Sato , Kohei Kimura
IPC分类号： B01J31/00 , B01J21/00 , C08F4/44 , C08F4/42 , C08F4/06 , C08F2/00 , C08F4/00
CPC分类号： C07F7/10 , C08F10/00 , C08F110/06 , C08F4/6492 , C08F4/6495 , C08F4/65927 , C08F2500/18 , C08F2500/12 , C08F2500/04 , C08F4/6465 , C08F4/6548 , C08F4/6565
摘要： A catalyst for polymerization of olefins formed from (A) a solid catalyst component containing magnesium, titanium, halogen, and an electron donor compound, (B) an organoaluminum compound shown by the formula, R6pAlQ3-p, and (C) an aminosilane compound shown by the formula, R3nSi(NR4R5)4-n; and a process for producing a catalyst for polymerization of olefins in the presence of the catalyst are provided. A novel aminosilane compound, a catalyst component for polymerization of olefins having a high catalytic activity, capable of producing polymers with high stereoregularity in a high yield, and exhibiting an excellent hydrogen response, a catalyst, and a process for producing olefin polymers using the catalyst are provided.
摘要翻译：由（A）含有镁，钛，卤素和电子给体化合物的固体催化剂组分形成的烯烃聚合催化剂，（B）由式R6pAlQ3-p表示的有机铝化合物和（C）氨基硅烷化合物如下式所示：R3nSi（NR4R5）4-n; 提供了在催化剂存在下制备烯烃聚合催化剂的方法。一种新型氨基硅烷化合物，具有高催化活性的烯烃聚合催化剂组分，能够以高产率制备具有高立构规整性的聚合物，并表现出优异的氢响应，催化剂和使用该催化剂生产烯烃聚合物的方法被提供。

8. 发明申请

US20100190938A1 CATALYST COMPONENT, CATALYST FOR OLEFIN POLYMERIZATION, AND PROCESS FOR PRODUCING OLEFIN POLYMER USING CATALYST 有权
标题翻译：催化剂组分，烯烃聚合催化剂和使用催化剂生产烯烃聚合物的方法
公开(公告)号：US20100190938A1
公开(公告)日：2010-07-29
申请号：US11997924
申请日：2006-08-04
申请人： Takefumi Yano , Motoki Hosaka , Maki Sato , Kohei Kimura
发明人： Takefumi Yano , Motoki Hosaka , Maki Sato , Kohei Kimura
IPC分类号： B01J31/18 , C08F4/602
CPC分类号： C08F10/00 , C07F7/1804 , C08F110/06 , C08F4/6465 , C08F2500/12 , C08F2500/18 , C08F2500/04
摘要： A polymer exhibiting high catalytic activity, good hydrogen response and high three-dimensional regularity can be obtained with high yield by polymerizing an olefin in the presence of a catalyst for olefin polymerization which is composed of a solid catalyst component (A) containing magnesium, titanium, a halogen and an electron-donating compound, an organic aluminum compound (B) represented by the following general formula: R6pAlQ3-p, and an aminosilane compound (C) represented by the following general formula: (R1R2N)m(R3HN)nR4pSi(OR5)q.
摘要翻译：通过在烯烃聚合催化剂存在下聚合烯烃，可以高收率地获得表现出高催化活性，良好的氢响应和高三维规则性的聚合物，该催化剂由含镁的固体催化剂组分（A），钛，卤素和给电子化合物，由以下通式表示的有机铝化合物（B）：R6pAlQ3-p和由以下通式表示的氨基硅烷化合物（C）：（R1R2N）m（R3HN）nR4pSi （OR5）q。

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