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1. 发明授权

US08343657B2 Negative electrode for lithium secondary battery, method of manufacturing the electrode, and lithium secondary battery 失效
标题翻译：锂二次电池用负极，电极的制造方法以及锂二次电池
公开(公告)号：US08343657B2
公开(公告)日：2013-01-01
申请号：US11657092
申请日：2007-01-24
申请人： Hiroshi Minami , Atsushi Fukui , Yasuyuki Kusumoto
发明人： Hiroshi Minami , Atsushi Fukui , Yasuyuki Kusumoto
IPC分类号： H01M4/58
CPC分类号： H01M4/0435 , H01M4/0471 , H01M4/134 , H01M4/1395 , H01M4/621 , H01M4/625 , H01M4/661
摘要： In a lithium secondary battery using a negative electrode having a negative electrode mixture layer formed on a surface of a negative electrode current collector, the mixture layer made of a binder and negative electrode active material particles of silicon and/or a silicon alloy, charge-discharge cycle performance is improved without degrading the capacity per unit volume, by making the negative electrode mixture layer sufficiently adhere to the negative electrode current collector. The negative electrode has a negative electrode mixture layer composed of a binder and negative electrode active material particles of silicon and/or a silicon alloy. The negative electrode mixture layer is formed on a surface of the negative electrode current collector by sintering. Negative electrode active material particles are partially embedded in the negative electrode current collector.
摘要翻译：在使用在负极集电体的表面形成有负极混合层的负极的锂二次电池中，由粘合剂构成的混合层和硅和/或硅合金的负极活性物质粒子，通过使负极混合物层充分地粘附到负极集电体，可以提高放电循环性能，而不降低单位体积的容量。负极具有由粘合剂和硅和/或硅合金的负极活性物质粒子构成的负极混合层。通过烧结在负极集电体的表面上形成负极合剂层。负极活性物质粒子部分嵌入负极集电体。

2. 发明授权

US08338022B2 Lithium secondary battery and method for manufacturing the same 有权
标题翻译：锂二次电池及其制造方法
公开(公告)号：US08338022B2
公开(公告)日：2012-12-25
申请号：US11001192
申请日：2004-12-02
申请人： Atsushi Fukui , Hiroshi Minami , Shoichiro Sawa , Mariko Torimae , Yasuyuki Kusumoto , Maruo Kamino
发明人： Atsushi Fukui , Hiroshi Minami , Shoichiro Sawa , Mariko Torimae , Yasuyuki Kusumoto , Maruo Kamino
IPC分类号： H01M2/02
CPC分类号： H01M10/052 , H01M4/0471 , H01M4/131 , H01M4/134 , H01M4/386 , H01M4/525 , H01M4/622 , H01M4/661 , H01M4/70 , H01M10/0587 , H01M2004/021 , Y10T29/49108
摘要： A lithium secondary battery of the present invention comprises a positive electrode formed by disposing a positive-electrode mixture layer containing a positive-electrode active material and a positive-electrode binder, on a surface of a positive-electrode current collector; a negative electrode formed by sintering a negative-electrode mixture layer containing a negative-electrode binder and a negative-electrode active material containing silicon and/or a silicon alloy, disposed on a surface of a negative-electrode current collector; a separator disposed between the positive electrode and the negative electrode; and a nonaqueous electrolyte; wherein an electrode unit obtained by setting the positive electrode and the negative electrode opposed to each other through the separator and rolling them in spirally rolled state is placed in a cylindrical battery container and wherein a curvature radius of the negative-electrode mixture layer opposed to the positive-electrode mixture layer through the separator in the spirally rolled state is 1.5 mm or larger.
摘要翻译：本发明的锂二次电池包括在正极集电体的表面上设置含有正极活性物质和正极粘合剂的正极合剂层而形成的正极，通过在负极集电体的表面上烧结含有负极粘合剂的负极混合层和含有硅和/或硅合金的负极活性物质而形成的负极，设置在所述正极和所述负极之间的隔膜; 和非水电解质; 其特征在于，将通过隔板相对的正极和负极通过将螺旋卷绕状态进行轧制而得到的电极单元配置在圆筒状的电池容器中，其中与负极混合层相对的曲率半径螺旋状卷取状态的正极混合层通过隔膜的厚度为1.5mm以上。

3. 发明授权

US07316717B2 Method of manufacturing an electrode active material particle for a rechargeable battery 有权
标题翻译：制造可充电电池用电极活性物质粒子的方法
公开(公告)号：US07316717B2
公开(公告)日：2008-01-08
申请号：US10239745
申请日：2001-03-15
申请人： Masahisa Fujimoto , Yasuyuki Kusumoto , Masahide Miyake , Hiroaki Ikeda , Shin Fujitani
发明人： Masahisa Fujimoto , Yasuyuki Kusumoto , Masahide Miyake , Hiroaki Ikeda , Shin Fujitani
IPC分类号： H01M4/00 , H01M4/40
CPC分类号： H01M4/134 , H01M4/364 , H01M4/38 , H01M4/386 , H01M4/387 , H01M4/626 , H01M10/052 , Y10T29/49115
摘要： A rechargeable battery includes electrodes containing particles of an active material capable of being alloyed with Li. A metallic element that is not alloyed with Li is distributed by its diffusion in particles of the active material.
摘要翻译：可再充电电池包括含有能够与Li合金化的活性物质颗粒的电极。与Li不合金的金属元素通过其在活性物质的颗粒中的扩散而分布。

4. 发明申请

US20070072077A1 Lithium secondary battery, negative electrode therefor, and method of their manufacture 审中-公开
标题翻译：锂二次电池及其负极及其制造方法
公开(公告)号：US20070072077A1
公开(公告)日：2007-03-29
申请号：US11527713
申请日：2006-09-27
申请人： Yasuyuki Kusumoto , Nobuhiro Sakitani
发明人： Yasuyuki Kusumoto , Nobuhiro Sakitani
IPC分类号： H01M4/38 , H01M4/62
CPC分类号： H01M10/052 , H01M4/136 , H01M4/621 , H01M4/623 , Y02T10/7011 , Y10T29/49108
摘要： A practical lithium secondary battery is provided having a greater battery capacity than in the case of using particulate graphite as its negative electrode active material but a less electrical resistance of its negative electrode mixture layer than in the case of using particulate Si as the negative electrode active material. The lithium secondary battery also exhibits good charge-discharge cycle performance. The lithium secondary battery is furnished with a negative electrode having negative electrode current collector and a negative electrode mixture layer that contains a Sn-based particulate negative electrode active material and a negative electrode binder. The negative electrode binder is melt-bonded to the Sn-based particulate negative electrode active material and/or the negative electrode current collector, and the Sn-based particulate negative electrode active material is made of an intermetallic compound represented as SnXM1-X, where 1>X≧1/2 and M is Mn, Fe, Co, or Ni.
摘要翻译：提供了一种实用的锂二次电池，其具有比在使用颗粒状石墨作为其负极活性物质时更大的电池容量，但是与使用颗粒状Si作为负极活性物质相比，其负极混合物层的电阻较小材料。锂二次电池也具有良好的充放电循环性能。锂二次电池配备有负极集电体和含有Sn系粒子状负极活性物质和负极活性物质的负极混合层的负极。负极粘合剂与Sn系粒子状负极活性物质和/或负极集电体熔融结合，Sn系粒子状负极活性物质由Sn X系金属间化合物 M 1-X 1，其中1> X> = 1/2，M是Mn，Fe，Co或Ni。

5. 发明授权

US07192673B1 Electrode for rechargeable lithium battery and rechargeable lithium battery 失效
标题翻译：可充电锂电池和可充电锂电池电极
公开(公告)号：US07192673B1
公开(公告)日：2007-03-20
申请号：US10111074
申请日：2000-10-20
申请人： Hiroaki Ikeda , Masahisa Fujimoto , Shin Fujitani , Masaki Shima , Hiromasa Yagi , Hisaki Tarui , Hiroshi Kurokawa , Kenji Asaoka , Shigeki Matsuta , Yoichi Domoto , Ryuji Ohshita , Yoshio Kato , Hiroshi Nakajima , Yasuyuki Kusumoto
发明人： Hiroaki Ikeda , Masahisa Fujimoto , Shin Fujitani , Masaki Shima , Hiromasa Yagi , Hisaki Tarui , Hiroshi Kurokawa , Kenji Asaoka , Shigeki Matsuta , Yoichi Domoto , Ryuji Ohshita , Yoshio Kato , Hiroshi Nakajima , Yasuyuki Kusumoto
IPC分类号： H01M4/02 , H01M4/38 , H01M4/70
CPC分类号： H01M4/13 , H01M2/0207 , H01M4/04 , H01M4/131 , H01M4/134 , H01M4/1395 , H01M4/366 , H01M4/38 , H01M4/386 , H01M4/387 , H01M4/40 , H01M4/405 , H01M4/485 , H01M4/525 , H01M4/661 , H01M4/667 , H01M4/70 , H01M6/40 , H01M10/052 , H01M10/0587 , H01M10/44 , H01M2010/4292
摘要： An electrode for a rechargeable lithium battery which includes a thin film composed of active material that expands and shrinks as it stores and releases lithium, e.g., a microcrystalline or amorphous silicon thin film, deposited on a current collector, characterized in that said current collector exhibits a tensile strength (=tensile strength (N/mm2) per sectional area of the current collector material×thickness (mm) of the current collector) of not less than 3.82 N/mm.
摘要翻译：一种用于可再充电锂电池的电极，其包括由活性材料构成的薄膜，所述活性材料在其存储和释放锂时膨胀和收缩，例如沉积在集电器上的微晶或非晶硅薄膜，其特征在于，所述集电器显示集电体材料厚度（mm）的每个截面积的拉伸强度（=拉伸强度（N / mm 2））不小于3.82N / mm。

6. 发明申请

US20060159997A1 Electrode for lithium secondary battery and lithium secondary battery 有权
标题翻译：锂二次电池和锂二次电池用电极
公开(公告)号：US20060159997A1
公开(公告)日：2006-07-20
申请号：US11108831
申请日：2005-04-19
申请人： Takuya Sunagawa , Yasuyuki Kusumoto , Shin Fujitani , Kensuke Nakatani , Muneto Kobayashi
发明人： Takuya Sunagawa , Yasuyuki Kusumoto , Shin Fujitani , Kensuke Nakatani , Muneto Kobayashi
IPC分类号： H01M4/70 , H01M4/58 , H01M4/66
CPC分类号： H01M4/0404 , H01M4/02 , H01M4/13 , H01M4/134 , H01M4/364 , H01M4/366 , H01M4/661 , H01M10/052 , H01M10/0525 , H01M2004/021
摘要： There is provided an electrode for a lithium secondary battery where particles, composed of an active material capable of occluding and releasing lithium, are arranged on a current collector, the active material particle being directly bonded to the surface of the current collector in a state where the bottom of the active material particle is imbedded in a concave portion formed on the surface of the current collector. A second particle layer may be provided on a first particle layer comprising the active material particles directly bonded to the surface of the current collector.
摘要翻译：提供了一种用于锂二次电池的电极，其中由能够吸收和释放锂的活性材料构成的颗粒被布置在集电器上，活性材料颗粒直接结合到集电器的表面，活性物质颗粒的底部嵌入形成在集电体表面上的凹部中。第二粒子层可以设置在包含与集电体的表面直接接合的活性物质粒子的第一粒子层上。

7. 发明申请

US20060003226A1 Lithium secondary battery and method for producing same 有权
标题翻译：锂二次电池及其制造方法
公开(公告)号：US20060003226A1
公开(公告)日：2006-01-05
申请号：US10531047
申请日：2004-06-04
申请人： Shouichirou Sawa , Hiroshi Minami , Mariko Torimae , Atsushi Fukui , Yasuyuki Kusumoto , Katsunobu Sayama , Maruo Kamino
发明人： Shouichirou Sawa , Hiroshi Minami , Mariko Torimae , Atsushi Fukui , Yasuyuki Kusumoto , Katsunobu Sayama , Maruo Kamino
IPC分类号： H01M4/58 , H01M10/40 , H01M4/66
CPC分类号： H01M10/052 , H01M4/0471 , H01M4/134 , H01M4/386 , H01M4/405 , H01M10/0567 , H01M10/058 , H01M2004/027 , Y10T29/49108
摘要： A rechargeable lithium battery including a negative electrode made by sintering, on a surface of a conductive metal foil as a current collector, a layer of a mixture of active material particles containing silicon and/or a silicon alloy and a binder, a positive electrode and a nonaqueous electrolyte, characterized in that the nonaqueous electrolyte contains carbon dioxide dissolved therein.
摘要翻译：一种可再充电锂电池，包括通过烧结制成的负极，作为集电体的导电金属箔的表面，含有硅和/或硅合金和粘合剂的活性物质颗粒的混合物层，正极和非水电解质，其特征在于，所述非水电解质含有溶解在其中的二氧化碳。

8. 发明授权

US06979516B2 Lithium secondary battery and positive electrode for lithium secondary battery 失效
标题翻译：锂二次电池和锂二次电池正极
公开(公告)号：US06979516B2
公开(公告)日：2005-12-27
申请号：US10056209
申请日：2002-01-28
申请人： Yasuyuki Kusumoto , Masahisa Fujimoto , Shin Fujitani , Yoichi Domoto , Daizo Jito , Hisaki Tarui
发明人： Yasuyuki Kusumoto , Masahisa Fujimoto , Shin Fujitani , Yoichi Domoto , Daizo Jito , Hisaki Tarui
IPC分类号： H01M4/66 , H01M4/13 , H01M4/131 , H01M4/139 , H01M4/1391 , H01M4/52 , H01M10/05 , H01M10/052 , H01M10/0566 , H01M4/36 , H01M4/58 , C23C14/00 , C23C14/32
CPC分类号： H01M4/525 , H01M4/04 , H01M4/485 , H01M4/661 , H01M10/052 , H01M10/0525 , H01M2004/028
摘要： A lithium secondary battery comprises a negative electrode containing lithium metal or a material previously storing lithium as an active material, a positive electrode containing a positive active material, and an electrolyte containing a non-aqueous electrolyte solution. The positive active material is a thin film formed by depositing on a substrate from vapor phase or liquid phase and including an oxide containing at least iron as a main constituent by a sputtering method, a reactive deposition method, a vacuum deposition method, a chemical vapor deposition method, a spraying method, a plating method, or a method in combination of these methods.
摘要翻译：锂二次电池包括含有锂金属的负极或预先存储锂作为活性材料的材料，含有正极活性物质的正极和含有非水电解质溶液的电解质。正极活性物质是通过溅射法，反应性沉积法，真空沉积法，化学蒸气法，从气相或液相沉积在基底上而形成的薄膜，包括至少含有铁作为主要成分的氧化物沉积法，喷涂法，电镀法或这些方法的组合方法。

9. 发明申请

US20050244711A1 Negative electrode for lithium secondary cell and lithium secondary cell 有权
标题翻译：锂二次电池和锂二次电池用负极
公开(公告)号：US20050244711A1
公开(公告)日：2005-11-03
申请号：US10519073
申请日：2003-06-25
申请人： Atsushi Fukui , Yasuyuki Kusumoto , MAriko Torimae , Hiroshi Nakamura
发明人： Atsushi Fukui , Yasuyuki Kusumoto , MAriko Torimae , Hiroshi Nakamura
IPC分类号： H01M4/134 , H01M4/38 , H01M4/40 , H01M4/62 , H01M4/66 , H01M10/052 , H01M10/36 , H01M4/58
CPC分类号： H01M4/134 , H01M4/386 , H01M4/405 , H01M4/621 , H01M4/661 , H01M10/052
摘要： A negative electrode for a lithium secondary cell having a collector composed of an electroconductive metal foil and, provided on the surface thereof, an active material layer containing active material particles containing silicon and/or a silicon alloy and a binder, characterized in that the binder has mechanical characteristics of a tensile strength of 50 N/mm2 or more, an elongation at break of 10% or more, a strain energy density of 2.5×10−3 J/mm3 or more and a coefficient of elasticity of 10000 N/mm2 or less, and preferably characterized in that the collector has mechanical characteristics of a tensile strength of 80 N/mm2 or more, a proportional limit 30 N/mm2 or more, an elongation at break of 1.0% or more and an elastic elongation limit of 0.03% or more.
摘要翻译：一种锂二次电池用负极，其具有由导电性金属箔构成的集电体，在其表面上设有包含含有硅和/或硅合金的活性物质粒子和粘合剂的活性物质层，其特征在于，所述粘合剂具有拉伸强度为50N / mm 2以上的机械特性，断裂伸长率为10％以上，应变能密度为2.5×10 -3 J / mm 3以上，弹性系数为10000N / mm 2以下，其特征在于，集电体具有抗拉强度为80N的机械特性 / mm 2以上，比例范围为30N / mm 2以上，断裂伸长率为1.0％以上，弹性伸长极限为0.03％以上。

10. 发明申请

US20050233066A1 Manufacturing method of chemical battery electrode and battery 审中-公开
标题翻译：化学电池电极和电池的制造方法
公开(公告)号：US20050233066A1
公开(公告)日：2005-10-20
申请号：US11108846
申请日：2005-04-19
申请人： Takuya Sunagawa , Yasuyuki Kusumoto , Shin Fujitani , Kensuke Nakatani
发明人： Takuya Sunagawa , Yasuyuki Kusumoto , Shin Fujitani , Kensuke Nakatani
IPC分类号： H01M4/66 , B05D1/02 , B05D5/12 , B05D7/00 , C23C24/04 , H01M4/139 , H01M4/1395 , H01M4/26 , H01M4/36 , H01M4/38 , H01M4/62 , H01M4/70 , H01M10/05 , H01M4/48 , H01M4/58
CPC分类号： H01M4/38 , C23C24/04 , H01M4/02 , H01M4/0404 , H01M4/0419 , H01M4/134 , H01M4/139 , H01M4/1395 , H01M4/364 , H01M4/386 , H01M4/387 , H01M4/62 , H01M4/661 , H01M4/662 , H01M4/70 , H01M10/0525 , H01M2004/021
摘要： A method of manufacturing a chemical battery electrode characterized in that active material particles are attached on a current collector comprising a step of dispersing active material particles in gas flow without melting nor evaporating it, a step of spraying the gas flow to the current collector so that the active material particles collide with the current collector, and a step of bonding the active material particles onto a surface of the current collector by the impact force.
摘要翻译：一种制造化学电池电极的方法，其特征在于，活性物质颗粒附着在集电器上，包括将活性物质颗粒分散在气流中而不熔化或蒸发的步骤，将气流喷射到集电体，使得活性物质粒子与集电体碰撞，通过冲击力将活性物质粒子接合到集电体的表面上。

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