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1. 发明授权

US5336753A Polycondensation and/or addition product containing carboxyl groups and tertiary amino groups, coating agents based thereon, and the use thereof 失效
标题翻译：包含羧基和叔氨基的缩聚和/或加成产物，基于其的包衣剂及其用途
公开(公告)号：US5336753A
公开(公告)日：1994-08-09
申请号：US2291
申请日：1993-01-08
申请人： Werner A. Jung , Udo Vorbeck , Arno Schmitz , Wilhelm Heise , Lutz-Werner Gross
发明人： Werner A. Jung , Udo Vorbeck , Arno Schmitz , Wilhelm Heise , Lutz-Werner Gross
IPC分类号： C08G63/685 , C09D167/00 , C08G69/26
CPC分类号： C09D167/00 , C08G63/685
摘要： The present invention relates to a polycondensation and/or addition product containing carboxyl groups and amino groups. This can be obtained by reactinga) polycarboxylic acids or anhydrides thereof, if appropriate together with monocarboxylic acids,b) polyols, if appropriate together with monools, and, if appropriatec) further modifying components, and, if appropriate,d) a component which is capable of reacting with the reaction product from a), b) and, if appropriate, c), with the proviso that the final product contains tertiary amino groups which originate from components a) and/or b) and/or d), and the reaction product from a), b), if appropriate c) and if appropriate d) has an acid number from 5 to 200, preferably 10 to 130, and an amine number from 3 to 150, preferably 10 to 100.The invention also relates to a process for the preparation of the polycondensation and/or addition product, and to coating agents based on the polycondensation and/or addition product, a process for the preparation of the coating agents, and the use thereof for automobile refinishing of automobile bodies and as a topcoat, filler, varnish, primer or undercoat.
摘要翻译：本发明涉及含有羧基和氨基的缩聚和/或加成产物。这可以通过使a）多元羧酸或其酸酐与适宜的一元羧酸反应获得，b）多元醇，如果适用，与一元醇一起，以及如果合适的话c）进一步修饰组分，如果合适，d）组分其能够与a），b）和（如果合适的话）c）的反应产物反应，条件是最终产物含有源自组分a）和/或b）和/或d）的叔氨基，，和a），b）的反应产物，如果合适c），如果合适，d）的酸值为5至200，优选10至130，胺数为3至150，优选10至100。本发明还涉及一种制备缩聚和/或加成产物的方法，以及基于缩聚和/或加成产物的涂布剂，制备涂料的方法及其用于汽车修补的用途汽车车身和顶棚燕麦，填料，清漆，底漆或底漆。

2. 发明授权

US5331052A Curable composition based on branched acrylates with carboxyl groups and/or branched acrylates with epoxide groups and aminoplast resins 失效
标题翻译：基于具有羧基和/或具有环氧基和氨基塑料树脂的支链丙烯酸酯的支化丙烯酸酯的可固化组合物
公开(公告)号：US5331052A
公开(公告)日：1994-07-19
申请号：US411525
申请日：1989-09-29
申请人： Werner A. Jung
发明人： Werner A. Jung
IPC分类号： C08L33/02 , C08F220/06 , C08F220/10 , C08G59/40 , C08G59/42 , C08G59/50 , C08L33/00 , C08L33/04 , C08L33/06 , C08L33/14 , C08L61/20 , C08L63/00 , C09D133/02 , C09D133/04 , C09D133/14 , C09D163/00 , C08L61/26 , C08L61/24
CPC分类号： C09D133/04 , C08L33/02 , C08L33/14 , C09D133/02 , C09D133/14 , C08L33/06 , C08L33/064 , C08L33/068 , C08L61/20 , C08L63/00
摘要： Curable composition based on branched acrylates with COOH groups and/or branched acrylates with epoxide groups, and aminoplast resins.The present invention relates to a curable composition consisting ofA) a polymer with at least 2 COOH groups,B) a polymer with at least 2 epoxide groups andC) an aminoplast resin.At least one of components A) or B) is based on a branched soluble acrylate copolymer, more than 3 to 30% by weight, based on the total weight of the monomers, of a monomer with at least two polymerizable, olefinically unsaturated double bonds being used in the preparation of these branched acrylate copolymers and the proportions of the individual components relative to one another being chosen so that a molar ratio of 3:1 to 1:3 prevails between the carboxyl groups of component A) and the epoxide groups of component B) and a weight ratio of 65:35% by weight to 98:2% by weight prevails between the epoxy resin component and the aminoplast resin component.The invention also relates to coating agents based on the curable composition.
摘要翻译： PCT No.PCT / EP88 / 00249 Sec。 371日期：1989年9月29日 102（e）日期1989年9月29日PCT提交1988年3月25日PCT Pub。出版物WO88 / 07565 日本1988年10月6日。具有COOH基和/或具有环氧基的支链丙烯酸酯的支化丙烯酸酯和氨基塑料树脂的可固化组合物。本发明涉及由A）具有至少2个COOH基团的聚合物组成的可固化组合物，B）具有至少2个环氧基团的聚合物，和C）氨基塑料树脂。组分A）或B）中的至少一种是基于支链可溶性丙烯酸酯共聚物，基于单体总重量大于3至30重量％的具有至少两个可聚合的烯属不饱和双键的单体用于制备这些支化丙烯酸酯共聚物，并且各组分相对于彼此的比例被选择为使得组分A）的羧基与环氧化物基团之间的摩尔比为3:1至1:3。组分B），并且环氧树脂组分和氨基塑料树脂组分之间的重量比为65:35重量％至98:2重量％。本发明还涉及基于可固化组合物的包衣剂。

3. 发明授权

US5276104A Copolymers containing carboxyl groups and, if appropriate, tertiary amino groups, a process for their preparation and their use in coating materials 失效
标题翻译：含羧基的共聚物，如果合适的话，叔氨基，它们的制备方法及其在涂料中的应用
公开(公告)号：US5276104A
公开(公告)日：1994-01-04
申请号：US778118
申请日：1991-12-05
申请人： Peter Hoffmann , Werner A. Jung
发明人： Peter Hoffmann , Werner A. Jung
IPC分类号： C08F212/04 , C08F2/00 , C08F2/04 , C08F2/06 , C08F8/00 , C08F8/46 , C08F18/02 , C08F20/26 , C08F212/00 , C08F218/10 , C08F220/04 , C08F220/06 , C08F220/28 , C08L63/00 , C09D131/02 , C09D133/06 , C08F220/40
CPC分类号： C08F8/46 , C08F212/04 , C08F8/00 , C09D133/066 , C08L63/00
摘要： The invention relates to copolymers containing carboxyl groups and having an acid number of 20 to 150 mg of KOH/g and a number average molecular weight of 2000 to 8000, which can preferably be prepared from copolymers containing hydroxyl groups by reaction with carboxylic anhydrides, to a process for their preparation and their use in coating agents. The copolymers contain a vinyl ester, a vinyl aromatic, a hydroxyalkyl ester of an .alpha.,.beta.-unsaturated carboxylic acid, and optionally other monomers that may contain acid groups. The vinyl ester is taken initially and the other monomers are metered during the course of a monomer addition time of equal length for all monomers, in the following manner:1) the amount of the hydroxyalkyl ester added per time unit remains constant, and2) the amount of the vinyl aromatic added within the first third of the monomer addition time is 15 to 30% by weight, that added within the second third is 25 to 40% by weight, and that added within the last third is 35 to 60% by weight, in each case relative to the total amount of vinyl aromatic.
摘要翻译： PCT No.PCT / EP90 / 00878 Sec。 371 1991年12月5日第 102（e）日期1991年12月5日PCT Filed 1990年6月2日PCT公布。 WO90 / 15086 PCT出版物日本1990年12月13日。本发明涉及含有羧基，酸值为20〜150mg KOH / g，数均分子量为2000〜8000的共聚物，其优选可由含有羟基的共聚物通过与羧酸酐的反应，制备它们及其在包衣剂中的用途。共聚物含有乙烯基酯，乙烯基芳族化合物，（α），（β-）不饱和羧酸的羟烷基酯，以及任选的可含有酸基团的其它单体。首先采用乙烯基酯，并且在所有单体的相同长度的单体添加时间期间，以下列方式计量其它单体：1）每时间单元添加的羟烷基酯的量保持恒定，和2）在单体添加时间的第一三分之内添加的乙烯基芳族化合物的量为15〜30重量％，第二次添加量为25〜40重量％，最后三分之一为35〜60重量％在每种情况下相对于乙烯基芳族化合物的总量。

4. 发明授权

US5179191A Polycondensation and/or addition product containing carboxyl groups and tertiary amino groups, coating agents based thereon, and the use thereof 失效
标题翻译：含有羧基和仲胺基团的聚合和/或添加产品，基于其的涂料代理及其使用
公开(公告)号：US5179191A
公开(公告)日：1993-01-12
申请号：US328583
申请日：1989-02-27
申请人： Werner A. Jung , Udo Vorbeck , Arno Schmitz , Wilhelm Heise , Lutz-Werner Gross
发明人： Werner A. Jung , Udo Vorbeck , Arno Schmitz , Wilhelm Heise , Lutz-Werner Gross
IPC分类号： C08G63/685 , C09D167/00
CPC分类号： C09D167/00 , C08G63/685
摘要： A polycondensation and/or addition product containing carboxyl groups and tertiary amino groups, coating agents based on the latter, and the use thereof.The present invention relates to a polycondensation and/or addition product containing carboxyl groups and amino groups. This can be obtained by reactinga) polycarboxylic acids or anhydrides thereof, if appropriate together with monocarboxylic acids,b) polyols, if appropriate together with monools, and, if appropriatec) further modifying components, and, if appropriate,d) a component which is capable of reacting with the reaction product from a), b) and, if appropriate, c), with the proviso that the final product contains tertiary amino groups which originate from components a) and/or b) and/or d), and the reaction product from a), b), if appropriate c) and if appropriate d) and an acid number from 5 to 200, preferably 10 to 130, and an amine number from 3 to 150, preferably 10 to 300.The invention also relates to a process for the preparation of the polycondensation and/or process product, and to coating agents based on the polycondensation and/or addition product, a process for the preparation of the coating agents, and the use thereof for automobile refinishing of automobile bodies and as a topcoat, filler, varnish, primer or undercoat.
摘要翻译： PCT No.PCT / EP87 / 00429 Sec。 371日期1989年2月27日 102（e）日期1989年2月27日PCT PCT 1987年8月6日PCT公布。第WO88 / 01629号公报日期：1988年3月10日。含有羧基和叔氨基的缩聚和/或加成产物，基于后者的涂布剂及其用途。本发明涉及含有羧基和氨基的缩聚和/或加成产物。这可以通过使a）多元羧酸或其酸酐与适宜的一元羧酸反应获得，b）多元醇，如果适用，与一元醇一起，以及如果合适的话c）进一步修饰组分，如果合适，d）组分其能够与a），b）和（如果合适的话）c）的反应产物反应，条件是最终产物含有源自组分a）和/或b）和/或d）的叔氨基，，和a），b）的反应产物，如果合适的话c），如果合适的话d）和酸值为5-200，优选10-130，胺值为3- 150，优选为10-300。本发明还涉及一种制备缩聚和/或加工产品的方法，以及基于缩聚和/或加成产物的涂布剂，制备涂料的方法及其用于汽车修补的用途汽车车身和topco 在，填料，清漆，底漆或底漆。

5. 发明授权

US5322897A Copolymers containing hydroxyl groups, based on vinyl ester monomers, vinylaromatic monomers and hydroxylalkyl ester monomers, process for the preparation thereof and use thereof in coating compositions 失效
标题翻译：基于乙烯基酯单体，乙烯基芳族单体和羟烷基酯单体的含羟基的共聚物，其制备方法及其在涂料组合物中的用途
公开(公告)号：US5322897A
公开(公告)日：1994-06-21
申请号：US634175
申请日：1990-12-19
申请人： Werner A. Jung , Udo Vorbeck
发明人： Werner A. Jung , Udo Vorbeck
IPC分类号： C08F212/04 , C08F220/28 , C08G18/62 , C08F8/32
CPC分类号： C08G18/6229 , C08F212/04 , C08F220/28 , C08G18/6254
摘要： The invention relates to copolymers containing hydroxyl groups having a hydroxyl value of 50 to 200 mg of KOH/g and an average molecular weight (number average) of 1500 to 6000, which can be prepared by free-radical solution polymerization at temperatures of 130.degree. to 200.degree. C. of 5 to 25% by weight of vinyl ester monomers, 10 to 50% by weight of vinylaromatic monomers, 10 to 50% by weight of hydroxyalkyl ester monomers and, if desired, other monomers, in which the vinyl ester is initially used and the remaining monomers are added over a monomer addition period which is the same for all monomers as follows:i) The amount of the acrylate monomer added per unit time remains constant.ii) The amount of the vinylaromatic hydrocarbon added over the first third of the monomer addition period is 15 to 30% by weight, preferably 18 to 26% by weight, that added over the second third is 25 to 40% by weight, preferably 30 to 38% by weight, and that added over the last third is 35 to 60% by weight preferably 40 to 50% by weight, of the total amount of the vinylaromatic hydrocarbon.The subject-matter of the invention is also a process for the preparation of the copolymers as well as their use in coating compositions.
摘要翻译： PCT No.PCT / EP89 / 00688 Sec。 371 1990年12月19日第 102（e）1990年12月19日的PCT PCT 1989年6月19日PCT公布。出版物WO90 / 00570 日本1990年1月25日。本发明涉及羟基值为50〜200mg KOH / g，平均分子量（数均）为1500〜6000的羟基的共聚物，其可以通过自由基在130至200℃的温度下溶液聚合为5至25重量％的乙烯酯单体，10至50重量％的乙烯基芳族单体，10至50重量％的羟烷基酯单体，如果需要，其它单体，其中最初使用乙烯基酯，并且在单体添加周期中加入剩余的单体，对于所有单体，相同的单体添加时间如下：i）每单位时间添加的丙烯酸酯单体的量保持恒定。 ii）在单体添加期的第一三分之一中加入的乙烯基芳族烃的量为15〜30重量％，优选为18〜26重量％，第二次添加量为25〜40重量％，优选为30重量％至38重量％，并且在最后三分之一中加入的是乙烯基芳烃的总量的35至60重量％，优选40至50重量％。本发明的主题也是制备共聚物的方法及其在涂料组合物中的用途。

6. 发明授权

US5300571A Hardenable composition based on a Michael addition product, process for its preparation and its use 失效
标题翻译：基于迈克尔加成产物的可硬化组合物，其制备方法及其用途
公开(公告)号：US5300571A
公开(公告)日：1994-04-05
申请号：US663826
申请日：1991-03-26
申请人： Werner A. Jung , Peter Hoffmann
发明人： Werner A. Jung , Peter Hoffmann
IPC分类号： C08L33/00 , C08F20060101 , C08F8/32 , C08F290/12 , C08F299/00 , C08G18/62 , C08G73/00 , C08G73/02 , C08G73/12 , C08G81/02 , C08L33/04 , C09D133/00 , C09D133/04 , C08L61/00
CPC分类号： C08F299/00 , C08F290/12 , C08F8/30
摘要： The invention relates to a hardenable composition containingA) compounds having at least two activated double bonds (I) based on .alpha.,.beta.-unsaturated carbonyl compounds, .alpha.,.beta.-unsaturated carboxylic acid esters or .alpha.,.beta.-unsaturated nitrile groups,B) compounds containing either at least one primary amino group which is blocked by an aldehyde or ketone having not more than 10 C atoms or at least 2 groups which can be hydrolyzed to NH groups, andC) customary additives, if appropriate catalysts, if appropriate pigments and organic solvents.Either component A or component B or components A and B are based on a branched soluble acrylate copolymer P, which is obtainable by copolymerization ofa) 5 to 30% by weight of monomers having at least two ethylenically unsaturated polymerizable double bonds,b) 5 to 60% by weight of monomers having a functional group andc) 5 to 90% by weight of other ethylenically unsaturated monomers,the sum of a, b and c being 100% by weight.The invention also relates to processes for the preparation of the hardenable composition and its use.
摘要翻译： PCT No.PCT / EP89 / 00950 Sec。 371日期1991年3月26日 102（e）1991年3月26日PCT PCT 1989年8月11日PCT公布。出版物WO90 / 03404 本发明涉及一种可硬化组合物，其含有A）具有至少两种基于（α），（β-）不饱和羰基化合物，（α），（β） - 不饱和羧酸酯或（α），（β） - 不饱和腈基，B）含有至少一个被不多于10个碳原子或至少2个基团的醛或酮封闭的伯氨基的化合物，被水解成NH基，C）常规添加剂，如果合适的话，适当的催化剂，如果合适的颜料和有机溶剂。组分A或组分B或组分A和B基于支化可溶性丙烯酸酯共聚物P，其可通过a）5至30重量％的具有至少两个烯属不饱和可聚合双键的单体的共聚获得，b）5 至60重量％的具有官能团的单体和c）5-90重量％的其它烯属不饱和单体，a，b和c的总和为100重量％。本发明还涉及制备可硬化组合物的方法及其用途。

7. 发明授权

US5283290A Coating agents of acrylic copolymer and polyester with tertiary amino groups and epoxy resin 失效
标题翻译：丙烯酸共聚物和聚酯与叔氨基和环氧树脂的涂层剂
公开(公告)号：US5283290A
公开(公告)日：1994-02-01
申请号：US573037
申请日：1990-08-31
申请人： Werner A. Jung , Udo Vorbeck
发明人： Werner A. Jung , Udo Vorbeck
IPC分类号： C08L63/00 , C09D133/06 , C09D163/00 , C09D167/00 , C08L33/14 , C08L63/02 , C08L67/02
CPC分类号： C09D133/066 , C09D163/00 , C09D167/00 , C08L63/00
摘要： The present invention relates to a coating agent containing A) a component containing carboxyl and tertiary amino groups and a polyepoxy resin B). A) consists of 10 to 90% by weight of a carboxyl- and amino-containing polyacrylate (A1) having an acid number from 20 to 140 and an amine number from 5 to 60 and 90 to 10% by weight of a carboxyl- and amino-containing polyester (A2) having an acid number from 10 to 160 and an amine number from 3 to 90.(A2) is obtainable by reaction ofa) polycarboxylic acids or anhydrides thereof, if desired together with monocarboxylic acids,b) polyols, if desired together with monools, andc) further modifying components and, if desired,d) a component which reacts with the reaction product from a), b) and possibly c),with the proviso that the final product contains tertiary amino groups originating from component a) and/or b) and/or d), the sum of components (A1) to (A2) being 100% by weight.
摘要翻译：本发明涉及含有A）含有羧基和叔氨基的成分和聚环氧树脂B）的包衣剂。 A）由10至90重量％的含羧基和氨基的聚丙烯酸酯（A1），其酸值为20至140，胺数为5至60，和90至10重量％的羧基和含氨基的聚酯（A2），其酸值为10至160，胺数为3-90。（A2）可通过a）多元羧酸或其酸酐与一元羧酸一起反应而获得; b）多元醇如果需要，与单醇一起，和c）进一步改性组分，如果需要，d）与a），b）和可能的c）反应产物反应的组分，条件是最终产物含有叔氨基源自组分a）和/或b）和/或d），组分（A1）至（A2）的总和为100重量％。

8. 发明授权

US5229467A Copolymers containing amino groups, process for their preparation and their use in coating agents 失效
标题翻译：含有氨基团的共聚物，其制备方法及其在涂料中的用途
公开(公告)号：US5229467A
公开(公告)日：1993-07-20
申请号：US640399
申请日：1991-01-22
申请人： Werner A. Jung
发明人： Werner A. Jung
IPC分类号： C08F2/06 , C08F8/32
CPC分类号： C08F8/32
摘要： The invention relates to copolymers containing amino groups and having an amine number of 30 to 150 mg of KOH/g and a number-average molecular weight of 1,500 to 8,000, which can be prepared from copolymers containing alkyl ester groups by aminolysis with polyamines, processes for their preparation and their use in coating agents.
摘要翻译： PCT No.PCT / EP89 / 00850 Sec。 371日期1991年1月22日 102（e）日期1991年1月22日PCT提交1989年7月20日PCT公布。出版物WO90 / 01502 日本1990年2月22日。本发明涉及含有氨基并且胺值为30〜150mg KOH / g，数均分子量为1500〜8,000的共聚物，其可以由含有烷基酯的共聚物基团通过用多胺进行氨解，其制备方法及其在包衣剂中的用途。

9. 发明授权

US5319044A Branched polymer containing silyl groups, a process for the preparation thereof, coating agents based on the polymer, and the use thereof 失效
标题翻译：含有甲硅烷基的支链聚合物，其制备方法，基于聚合物的包衣剂及其用途
公开(公告)号：US5319044A
公开(公告)日：1994-06-07
申请号：US850648
申请日：1992-03-13
申请人： Werner A. Jung , Arno Schmitz
发明人： Werner A. Jung , Arno Schmitz
IPC分类号： C08F230/08 , C09D143/04
CPC分类号： C08F230/08 , C09D143/04
摘要： A branched polymer containing silyl groups, a process for the preparation thereof, coating agents based on the polymer, and the use thereof.The invention relates to polymers containing silyl groups, the silyl groups being introduced into the polymer through ethylenically unsaturated monomers of the general formula ##STR1## wherein R.sup.1 =alkyl, aryl, acyl or aralkyl having 1 to 10 carbon atoms,R.sup.2 =an organic radical having a polymerizable double bond,X=a hydrolyzable group, andn=1, 2 or 3.The polymers can be obtained by copolymerization ofa) 0.1 to 40% by weight of the silane monomers (a),b) 5 to 30% by weight, preferably 8 to 25% by weight, of monomers containing at least 2 polymerizable, ethylenically unsaturated double bonds, andc) 30 to 90% by weight of ethylenically unsaturated monomers without groups containing active hydrogen.The invention also relates to moisture-hardening coating agents based on the polymers containing silyl groups. The coating agents are suitable, in particular, for automobile repair paintwork.
摘要翻译：含有甲硅烷基的支链聚合物，其制备方法，基于聚合物的涂布剂及其用途。本发明涉及含有甲硅烷基的聚合物，该甲硅烷基通过通式（a）的烯属不饱和单体引入聚合物中，其中R1 =具有1-10个碳原子的烷基，芳基，酰基或芳烷基，R2 = 具有可聚合双键的有机基团，X =可水解基团，n = 1,2或3.可以通过以下步骤获得聚合物：a）0.1至40重量％的硅烷单体（a），b） 5至30重量％，优选8至25重量％的含有至少2个可聚合的烯属不饱和双键的单体，和c）30至90重量％的不含活性氢的基团的烯属不饱和单体。本发明还涉及基于含有甲硅烷基的聚合物的湿润硬化涂层剂。涂层剂特别适用于汽车修补漆。

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