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1. 发明授权

US07642318B2 Modified block copolymer 有权
标题翻译：改性嵌段共聚物
公开(公告)号：US07642318B2
公开(公告)日：2010-01-05
申请号：US11822518
申请日：2007-07-06
申请人： Nobuaki Kubo , Yasuhiro Kusanose , Shigeo Nakajima , Takaaki Matsuda , Shigeki Takayama , Toshinori Shiraki
发明人： Nobuaki Kubo , Yasuhiro Kusanose , Shigeo Nakajima , Takaaki Matsuda , Shigeki Takayama , Toshinori Shiraki
IPC分类号： C08L53/02
CPC分类号： C08F8/00 , C08F297/04 , C08L53/02 , C08L53/025 , C08L95/00 , C08L2666/02 , C09J7/22 , C09J7/38 , C09J7/387 , C09J153/02 , C09J153/025 , C09J2453/00 , C08L2666/24
摘要： A second-order modified block copolymer which can be obtained by reacting a first-order modified block copolymer with a second-order modifier, wherein the first-order modified block copolymer comprises a base block copolymer and a functional group-containing first-order modifier group bonded to the base block copolymer, wherein the base block copolymer comprises at least one polymer block comprised mainly of vinyl aromatic hydrocarbon monomer units and at least one polymer block comprised mainly of conjugated diene monomer units, and wherein the second-order modifier has a specific functional group which is reactive to the functional group of the first-order modifier group of the first-order modified block copolymer. A second-order modified block copolymer-containing polymer composition comprising the second-order modified block copolymer as well as a thermoplastic resin and/or a rubbery polymer.
摘要翻译：二级改性嵌段共聚物，其可以通过使一级改性嵌段共聚物与二级改性剂反应得到，其中一级改性嵌段共聚物包括碱嵌段共聚物和含官能团的一级改性剂基团嵌段共聚物包含至少一个主要由乙烯基芳族烃单体单元组成的聚合物嵌段和至少一个主要由共轭二烯单体单元组成的聚合物嵌段，其中二级改性剂具有与一级改性嵌段共聚物的一级改性剂基团的官能团反应的官能团。包含二级改性嵌段共聚物的二阶改性嵌段共聚物聚合物组合物以及热塑性树脂和/或橡胶状聚合物。

2. 发明授权

US07498387B2 Modified polymers and compositions containing the same 有权
标题翻译：改性聚合物和含有它们的组合物
公开(公告)号：US07498387B2
公开(公告)日：2009-03-03
申请号：US10510571
申请日：2003-04-10
申请人： Takaaki Matsuda , Shigeki Takayama , Toshinori Shiraki , Shigeo Nakajima , Yasuhiro Kusanose
发明人： Takaaki Matsuda , Shigeki Takayama , Toshinori Shiraki , Shigeo Nakajima , Yasuhiro Kusanose
IPC分类号： C08C19/02 , C08C19/22 , C08C19/25 , C08C19/28 , C08C19/30 , C08L95/00 , C08F36/04
CPC分类号： C09J151/04 , C08C19/02 , C08F8/04 , C08F297/04 , C08L51/04 , C08L53/025 , C08L2666/02 , C09J153/025 , C08L2666/24
摘要： A first-order modified, hydrogenated polymer comprising (1) a hydrogenated polymer obtained by hydrogenating at least one unhydrogenated polymer selected from the group consisting of a polymer comprising conjugated diene monomer units and a copolymer comprising conjugated diene monomer units and vinyl aromatic hydrocarbon monomer units, and (2) a functional group-containing first-order modifier group bonded to the hydrogenated polymer (1), wherein the content of the vinyl aromatic hydrocarbon monomer units, vinyl aromatic hydrocarbon block ratio, weight average molecular weight, and hydrogenation ratio (as measured with respect to the double bonds in the conjugated diene monomer units) of the first-order modified, hydrogenated polymer are, respectively, within specific ranges. A second-order modified polymer obtained by reacting a second-order modifier with a first-order modified polymer comprising (β) a base polymer and (γ) a functional group-containing first-order modifier group bonded to the base polymer (β). A composition comprising the above-mentioned first-order modified, hydrogenated polymer or second-order modified polymer and at least one functional component other than the modified polymer.
摘要翻译：一种一级改性氢化聚合物，其包含（1）氢化聚合物，其通过氢化至少一种选自包含共轭二烯单体单元的聚合物的非氢化聚合物和包含共轭二烯单体单元和乙烯基芳烃单体单元的共聚物而获得，和（2）与氢化聚合物（1）键合的含官能团的一级改性基团，其中乙烯基芳烃单体单元的含量，乙烯基芳烃嵌段比，重均分子量和氢化比（相对于共轭二烯单体单元中的双键测定的一级改性氢化聚合物分别在特定范围内。通过使二级改性剂与包含（β）基础聚合物和（γ）与基础聚合物（β）键合的含官能团的一级改性基团的一级改性聚合物反应而获得的二级改性聚合物，。包含上述一级改性氢化聚合物或二级改性聚合物和除改性聚合物以外的至少一种官能组分的组合物。

3. 发明授权

US07414093B2 Modified block copolymer 有权
标题翻译：改性嵌段共聚物
公开(公告)号：US07414093B2
公开(公告)日：2008-08-19
申请号：US11345286
申请日：2006-02-02
申请人： Nobuaki Kubo , Yasuhiro Kusanose , Shigeo Nakajima , Takaaki Matsuda , Shigeki Takayama , Toshinori Shiraki
发明人： Nobuaki Kubo , Yasuhiro Kusanose , Shigeo Nakajima , Takaaki Matsuda , Shigeki Takayama , Toshinori Shiraki
IPC分类号： C08L53/02
CPC分类号： C08F8/00 , C08F297/04 , C08L53/02 , C08L53/025 , C08L95/00 , C08L2666/02 , C09J7/22 , C09J7/38 , C09J7/387 , C09J153/02 , C09J153/025 , C09J2453/00 , C08L2666/24
摘要： A second order modified block copolymer which can be obtained by reacting a first order modified block copolymer with a second order modifier, wherein the first order modified block copolymer comprises a base block copolymer and a functional group-containing first order modifier group bonded to the base block co-polymer, wherein the base block copolymer comprises at least one polymer block comprised mainly of vinyl aromatic hydrocarbon monomer units and at least one polymer block comprised mainly of conjugated diene monomer units, and wherein the second order modifier has a specific functional group which is reactive to the functional group of the first order modifier group of the first order modified block copolymer. A second order modified block copolymer containing polymer composition comprising the second order modified block copolymer as well as a thermoplastic resin and/or a rubbery polymer.
摘要翻译：一种二阶改性嵌段共聚物，其可以通过使一级改性嵌段共聚物与二级改性剂反应而得到，其中一级改性嵌段共聚物包含与碱结合的碱嵌段共聚物和含官能团的一级改性基团嵌段共聚物，其中所述碱嵌段共聚物包含至少一种主要由乙烯基芳族烃单体单元和至少一个主要由共轭二烯单体单元组成的聚合物嵌段的聚合物嵌段，并且其中所述二级改性剂具有特定官能团，与一级改性嵌段共聚物的一级改性基团的官能团反应。含有二级改性嵌段共聚物的聚合物组合物的二阶改性嵌段共聚物以及热塑性树脂和/或橡胶状聚合物。

4. 发明授权

US07371805B2 Hydrogenated copolymer and composition thereof 有权
标题翻译：氢化共聚物及其组成
公开(公告)号：US07371805B2
公开(公告)日：2008-05-13
申请号：US10513926
申请日：2003-06-26
申请人： Masahiro Sasagawa , Toshinori Shiraki , Shigeki Takayama , Shigeru Sasaki , Katsumi Suzuki , Takahiro Hisasue , Kazuo Moritou
发明人： Masahiro Sasagawa , Toshinori Shiraki , Shigeki Takayama , Shigeru Sasaki , Katsumi Suzuki , Takahiro Hisasue , Kazuo Moritou
IPC分类号： C08F12/04 , C08F36/04
CPC分类号： C08F8/04 , C08F297/04
摘要： A hydrogenated copolymer obtained by hydrogenating an unhydrogenated copolymer comprising conjugated diene monomer units and vinyl aromatic monomer units, the hydrogenated copolymer containing at least one hydrogenated copolymer block (B) which is obtained by hydrogenating an unhydrogenated random copolymer block comprised of conjugated diene monomer units and vinyl aromatic monomer units, wherein the hydrogenated copolymer has the following characteristics: the hydrogenated copolymer has a content of the vinyl aromatic monomer units of from more than 40% by weight to less than 95% by weight; at least one peak of loss tangent (tan δ) is observed at −10 to 80° C. in a dynamic viscoelastic spectrum obtained with respect to the hydrogenated copolymer; and substantially no crystallization peak ascribed to the copolymer block (B) is observed at −20 to 80° C. in a differential scanning calorimetry (DSC) chart obtained with respect to the hydrogenated copolymer.
摘要翻译：通过氢化包含共轭二烯单体单元和乙烯基芳族单体单元的未氢化共聚物获得的氢化共聚物，所述氢化共聚物含有至少一个氢化共聚物嵌段（B），其通过氢化由共轭二烯单体单元组成的未氢化无规共聚物嵌段和乙烯基芳族单体单元，其中氢化共聚物具有以下特征：氢化共聚物的乙烯基芳族单体单元的含量大于40重量％至小于95重量％; 在相对于氢化共聚物获得的动态粘弹性光谱中，在-10〜80℃观察到损耗角正切（tanδ）的至少一个峰值。在相对于氢化共聚物获得的差示扫描量热法（DSC）图中，在-20〜80℃观察到基本上不归属于共聚物嵌段（B）的结晶峰。

5. 发明授权

US07122594B2 Modified block copolymer composition 有权
标题翻译：改性嵌段共聚物组成
公开(公告)号：US07122594B2
公开(公告)日：2006-10-17
申请号：US10480201
申请日：2002-04-24
申请人： Nobuaki Kubo , Yasuhiro Kusanose , Shigeki Takayama , Toshinori Shiraki
发明人： Nobuaki Kubo , Yasuhiro Kusanose , Shigeki Takayama , Toshinori Shiraki
IPC分类号： B60C3/04 , C08K5/5415
CPC分类号： C08K3/22 , C08F8/04 , C08F8/30 , C08F2800/20 , C08K3/01 , C08K3/36 , C08L53/005 , C08L53/025 , C08L53/02 , C08L2666/06 , C08F297/04 , C08F8/42
摘要： A modified block copolymer composition comprising (1) 100 parts by weight of a modified block copolymer consisting of vinyl aromatic hydrocarbons and conjugated dienes, containing a functional group having at least one group selected from the group consisting of a hydroxide group, an epoxy group, an amino group, a silanol group and an alkoxysilane group, or a hydrogenation product of the copolymer, and (2) 0.5 to 50 parts by weight at least one of fillers selected from the group consisting of silica-based inorganic fillers, metal oxides and metal hydroxides is disclosed. This modified block copolymer composition is excellent in heat resistance, mechanical strength, transparency, abrasion resistance, and processability.
摘要翻译：一种改性嵌段共聚物组合物，其包含（1）100重量份由乙烯基芳烃和共轭二烯构成的改性嵌段共聚物，其含有具有至少一个选自氢氧基，环氧基，氨基，硅烷醇基和烷氧基硅烷基，或该共聚物的氢化产物，和（2）0.5至50重量份的至少一种选自二氧化硅基无机填料，金属氧化物和公开了金属氢氧化物。该改性嵌段共聚物组合物的耐热性，机械强度，透明性，耐磨性和加工性优异。

6. 发明授权

US06875827B2 Hydrogenated polymer and process for producing the same 有权
标题翻译：氢化聚合物及其制备方法
公开(公告)号：US06875827B2
公开(公告)日：2005-04-05
申请号：US10297886
申请日：2002-04-05
申请人： Masahiro Sasagawa , Shinichi Nakajima , Shigeki Takayama , Takasi Sato , Toshinori Shiraki
发明人： Masahiro Sasagawa , Shinichi Nakajima , Shigeki Takayama , Takasi Sato , Toshinori Shiraki
IPC分类号： C08C19/02 , C08F8/04 , C08L9/00 , C08L15/00 , C08L21/00 , C08L23/10 , C08L23/16 , C08L53/02 , C08F136/06
CPC分类号： C08F136/06 , C08C19/02 , C08F8/04 , C08L9/00 , C08L15/005 , C08L21/00 , C08L23/10 , C08L23/16 , C08L53/025 , C08L2205/03 , C08L2666/24 , C08L2666/08 , C08L2666/02
摘要： The present invention relates to a hydrogenated polymer which is a hydrogenation product of a conjugated diene polymer having an average vinyl bond content of 20% by weight or more and less than 50% by weight and a weight average molecular weight of 60,000 to 600,000 to a degree such that 85% or more of the residual double bonds in the conjugated diene units are hydrogenated, and which has a molecular weight and a number of terminal methyl group carbons as measured by GPC/FTIR analysis satisfying relationship (1): Va−Vb≧0.03Vc (1) wherein Va, Vb and Vc represent the number of terminal methyl group carbon atoms per 1000 carbon atoms contained in a polymer whose molecular weight is twice the peak top molecular weight, half the peak top molecular weight, and the peak top molecular weight, respectively.
摘要翻译：本发明涉及一种氢化聚合物，其是平均乙烯基含量为20重量％以上且小于50重量％，重均分子量为60〜60万的共轭二烯聚合物的氢化产物，相对于使得共轭二烯单元中的残留双键的85％以上被氢化，通过GPC / FTIR分析测定的具有分子量和末端甲基碳数的满足关系式（1）：其中，Va， Vb和Vc分别表示分子量是峰顶分子量的两倍，峰顶分子量的一半和峰顶分子量的聚合物中每1000个碳原子的末端甲基碳原子数。

7. 发明授权

US06852806B2 Hydrogenated copolymer 有权
标题翻译：氢化共聚物
公开(公告)号：US06852806B2
公开(公告)日：2005-02-08
申请号：US10432194
申请日：2002-10-23
申请人： Masahiro Sasagawa , Shigeki Takayama , Shigeru Sasaki , Takahiro Hisasue , Katsumi Suzuki , Shigeo Nakajima
发明人： Masahiro Sasagawa , Shigeki Takayama , Shigeru Sasaki , Takahiro Hisasue , Katsumi Suzuki , Shigeo Nakajima
IPC分类号： C08F8/04
CPC分类号： C08F8/04 , Y10T428/31855 , C08F293/00 , C08F212/00
摘要： Disclosed is a hydrogenated copolymer obtained by hydrogenating an unhydrogenated copolymer comprising conjugated diene monomer units and vinyl aromatic monomer units, the unhydrogenated copolymer having at least one polymer block (H) of vinyl aromatic monomer units, wherein the hydrogenated copolymer has the following characteristics (1) to (5): (1) a content of the vinyl aromatic monomer units of from more than 60% by weight to less than 90% by weight, based on the weight of the hydrogenated copolymer; (2) a content of the polymer block (H) of from 1 to 40% by weight, based on the weight of the unhydrogenated copolymer; (3) a weight average molecular weight of from more than 100,000 to 1,000,000; (4) a hydrogenation ratio of 85% or more, as measured with respect to the double bonds in the conjugated diene monomer units; and (5) substantially no crystallization peak observed at −50 to 100° C. in a differential scanning calorimetry (DSC) chart obtained with respect to the hydrogenated copolymer.
摘要翻译：公开了通过氢化包含共轭二烯单体单元和乙烯基芳族单体单元的未氢化共聚物获得的氢化共聚物，所述非氢化共聚物具有至少一个乙烯基芳族单体单元的聚合物嵌段（H），其中所述氢化共聚物具有以下特征（1 ）至（5）：（1）基于氢化共聚物的重量，乙烯基芳族单体单元的含量为大于60重量％至小于90重量％（2）基于未氢化共聚物的重量，聚合物嵌段（H）的含量为1至40重量％; （3）重均分子量大于100,000至1,000,000; （4）相对于共轭二烯单体单元中的双键测定的氢化率为85％以上的氢化率; 和（5）在相对于氢化共聚物获得的差示扫描量热法（DSC）图中，在-50〜100℃观察到基本上没有结晶峰。

8. 发明授权

US5871075A Coin sorting machine 失效
标题翻译：硬币分拣机
公开(公告)号：US5871075A
公开(公告)日：1999-02-16
申请号：US591975
申请日：1996-01-29
申请人： Shigeki Takayama , Hiroshi Ohtomo
发明人： Shigeki Takayama , Hiroshi Ohtomo
IPC分类号： G07D3/14 , G07D5/08
CPC分类号： G07D5/08 , G07D3/00
摘要： A low-cost, high-performance coin sorting machine is provided by providing a plurality of coils which sense coins concurrently and using a simple oscillation circuit to provide oscillation signals at different frequencies, thereby reducing the size of the coin sorting machine. Right and left pairs of sensor coils are composed of inner and outer coils. When either of the connections between one inner coil and other inner coil, and between one outer coil and the other outer coil, is made in a cumulative mode, the other connection is made in a differential mode. The relationship between the oscillation frequencies is set so that one of the frequencies is greater than twice the other.
摘要翻译：通过提供多个同时感测硬币并使用简单的振荡电路提供不同频率的振荡信号的线圈来提供低成本，高性能的硬币分选机，从而减小硬币分选机的尺寸。传感器线圈左右对由内圈和外圈构成。当一个内部线圈和其他内部线圈之间以及一个外部线圈和另一个外部线圈之间的连接中的任一个被制成累积模式时，另一个连接是以差分模式进行的。设置振荡频率之间的关系，使得频率之一大于另一个频率的两倍。

9. 发明授权

US07256238B2 Modified block copolymer 有权
公开(公告)号：US07256238B2
公开(公告)日：2007-08-14
申请号：US10479754
申请日：2002-07-18
申请人： Nobuaki Kubo , Yasuhiro Kusanose , Shigeo Nakajima , Takaaki Matsuda , Shigeki Takayama , Toshinori Shiraki
发明人： Nobuaki Kubo , Yasuhiro Kusanose , Shigeo Nakajima , Takaaki Matsuda , Shigeki Takayama , Toshinori Shiraki
IPC分类号： C08L53/02
CPC分类号： C08F8/00 , C08F297/04 , C08L53/02 , C08L53/025 , C08L95/00 , C08L2666/02 , C09J7/22 , C09J7/38 , C09J7/387 , C09J153/02 , C09J153/025 , C09J2453/00 , C08L2666/24
摘要： A second-order modified block copolymer which can be obtained by reacting a first-order modified block copolymer with a second-order modifier, wherein the first-order modified block copolymer comprises a base block copolymer and a functional group-containing first-order modifier group bonded to the base block copolymer, wherein the base block copolymer comprises at least one polymer block comprised mainly of vinyl aromatic hydrocarbon monomer units and at least one polymer block comprised mainly of conjugated diene monomer units, and wherein the second-order modifier has a specific functional group which is reactive to the functional group of the first-order modifier group of the first-order modified block copolymer. A second-order modified block copolymer-containing polymer composition comprising the second-order modified block copolymer as well as a thermoplastic resin and/or a rubbery polymer.

10. 发明授权

US06767969B2 Hydrogenated polymer 有权
标题翻译：氢化聚合物
公开(公告)号：US06767969B2
公开(公告)日：2004-07-27
申请号：US10168613
申请日：2002-06-24
申请人： Masahiro Sasagawa , Shigeru Sasaki , Shigeki Takayama , Takashi Sato
发明人： Masahiro Sasagawa , Shigeru Sasaki , Shigeki Takayama , Takashi Sato
IPC分类号： C08F804
CPC分类号： C08F8/04 , C08C19/02
摘要： A hydrogenated polymer obtained by hydrogenating a conjugated diene polymer having an average vinyl bond content of 20% by weight or more and less than 40% by weight to a degree such that 85% or more of double bond residues in the conjugated diene unit portion are hydrogenated, wherein (1) the crystallizing peak temperature and the hydrogenated vinyl bond content satisfy the formula: −2.8V+100
摘要翻译：通过将平均乙烯基含量为20重量％以上且小于40重量％的共轭二烯聚合物氢化得到共轭二烯单元部分中85重量％以上双键残基的程度的氢化聚合物为氢化，其中（1）结晶峰温度和氢化乙烯基键含量满足下式：其中T是通过DSC测量的结晶峰温度（℃）; V为氢化乙烯基键含量（％），（2）分子量为60,000〜600,000，（3）分子量分布为1.55〜5.0。氢化聚合物的机械强度，耐热性，耐候性和加工性优异，并且当与其它热塑性树脂或橡胶状聚合物共混时，提供具有良好平衡的物理性能如耐冲击性和成型性的模塑制品。

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