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1. 发明授权

US07211238B2 Mesoporous aluminum oxide, preparation and use thereof 有权
标题翻译：介孔氧化铝，的制备和应用
公开(公告)号：US07211238B2
公开(公告)日：2007-05-01
申请号：US10795771
申请日：2004-03-08
申请人： Zhiping Shan , Jacobus Cornelius Jansen , Chuen Y. Yeh , Philip J. Angevine , Thomas Maschmeyer
发明人： Zhiping Shan , Jacobus Cornelius Jansen , Chuen Y. Yeh , Philip J. Angevine , Thomas Maschmeyer
IPC分类号： C01F7/02
CPC分类号： C01B37/00 , B01J21/04 , B01J35/10 , B01J35/1061 , B01J37/0018 , C01F7/36 , C01F7/448 , C01P2002/01 , C01P2002/72 , C01P2002/86 , C01P2006/12 , C01P2006/14 , C01P2006/16 , C01P2006/17
摘要： Mesoporous aluminum oxides with high surface areas have been synthesized using inexpensive, small organic templating agents instead of surfactants. Optionally, some of the aluminum can be framework-substituted by one or more other elements. The material has high thermal stability and possesses a three-dimensionally randomly connected mesopore network with continuously tunable pore sizes. This material can be used as catalysts for dehydration, hydrotreating, hydrogenation, catalytic reforming, steam reforming, amination, Fischer-Tropsch synthesis and Diels-Alder synthesis, etc.
摘要翻译：使用廉价的小型有机模板剂代替表面活性剂，已经合成了具有高表面积的介孔氧化铝。可选地，一些铝可以被一个或多个其它元素框架取代。该材料具有高热稳定性，并具有连续可调孔径的三维随机连接的中孔网络。该材料可用作脱水，加氢处理，氢化，催化重整，蒸汽重整，胺化，费 - 托合成和狄尔斯 - 阿尔德合成等催化剂。

2. 发明授权

US07091365B2 Process for olefin epoxidation and co-production of nylon precursor 失效
标题翻译：尼龙前体烯烃环氧化和共生产方法
公开(公告)号：US07091365B2
公开(公告)日：2006-08-15
申请号：US10795726
申请日：2004-03-08
申请人： Zhiping Shan , Chuen Y. Yeh , Philip J. Angevine , Frits M. Dautzenberg , Jacobus Cornelis Jansen
发明人： Zhiping Shan , Chuen Y. Yeh , Philip J. Angevine , Frits M. Dautzenberg , Jacobus Cornelis Jansen
IPC分类号： C07D301/16 , B01J21/12
CPC分类号： C07D301/19 , Y02P20/125
摘要： An integrated process combines olefin epoxidation with production of cyclohexanone and cyclohexanol for nylon. Cyclohexanone and cyclohexanol normally produced by the oxidation of cyclohexane, in which cyclohexyl hydroperoxide is generated and is removed or decomposed down stream. However, this invention utilizes the intermediate of cyclohexyl hydroperoxide as an oxidant for the olefin epoxidation and meanwhile generates a valuable product.
摘要翻译：一体化方法将烯烃环氧化与生产环己酮和环己醇用于尼龙。通常通过环己烷氧化生成环己酮和环己醇，其中产生环己基氢过氧化物并在流下被除去或分解。然而，本发明利用环己基氢过氧化物的中间体作为烯烃环氧化的氧化剂，同时产生有价值的产物。

3. 发明授权

US06534022B1 Conversion of nitrogen oxides in the presence of a catalyst supported on a mesh-like structure 有权
标题翻译：在负载在网状结构上的催化剂存在下氮氧化物的转化
公开(公告)号：US06534022B1
公开(公告)日：2003-03-18
申请号：US09687976
申请日：2000-10-13
申请人： Joakim A. Carlborg , Yun-Feng Chang , Lawrence L. Murrell , Robert E. Trubac , Rudolf A. Overbeek , Verena R. Schmidt , Chuen Y. Yeh , Lothar Schuh
发明人： Joakim A. Carlborg , Yun-Feng Chang , Lawrence L. Murrell , Robert E. Trubac , Rudolf A. Overbeek , Verena R. Schmidt , Chuen Y. Yeh , Lothar Schuh
IPC分类号： B01D5356
CPC分类号： B01J23/22 , B01D53/8631 , B01D53/864 , B01D53/8687 , B01D53/885 , B01D53/9431 , B01D53/9477 , B01D2257/402 , B01D2257/502 , B01D2257/702 , B01D2257/708 , B01J21/063 , B01J21/066 , B01J23/30 , B01J23/42 , B01J35/04 , B01J35/06 , B01J37/0225 , B01J37/0228 , F01N3/281 , F01N3/2814 , F01N3/2821 , F01N3/2828 , F01N3/2835 , F01N13/0097 , F01N2330/10 , F01N2330/12 , F01N2330/14 , F01N2330/38 , Y02C20/10 , Y02P20/153
摘要： An apparatus for converting at least one nitrogen oxide, such as NO, NO2, or N2O converts oxide in the presence of a catalyst supported on a metal mesh-like structure. The mesh-like structure is preferably fibrous formed of metal or ceramic fibers which may include knitted wire, sintered metal fibers and so on and has a porosity greater than about 85%. The mesh is formed into channels, preferably corrugations, and includes vortex generators, which generate turbulence to create a pressure differential across the mesh, to promote flow of fluids through the mesh pores which normally do not exhibit flow therethrough in the absence of such pressure differential. Preferred embodiments of structured packing and monoliths are disclosed each having a catalyst preferably in the mesh pores and/or coated on the fibers for converting the nitrogen oxide. In one embodiment, corrugated mesh-like sheets are arranged in series with a ceramic solid monolith structure with the corrugated sheets initially receiving the fluid with the at least one nitrogen oxide to be converted and which fluid then flows into the monolith structure to complete the conversion. In other embodiments, the mesh-like structure may have different configurations including a honeycomb arrangement and may include metal, metal and ceramic or ceramic and may be fibrous.
摘要翻译：用于转化至少一种氮氧化物如NO，NO 2或N 2 O的装置在负载在金属网状结构上的催化剂存在下转化氧化物。网状结构优选由金属或陶瓷纤维形成，其可以包括针织线，烧结金属纤维等，并且具有大于约85％的孔隙率。网格形成通道，优选波纹，并且包括涡流发生器，其产生湍流以产生横跨网孔的压力差，以促进流体流过网孔，其通常在没有这种压力差的情况下不显示流过其中。公开了优选在网孔中具有催化剂和/或涂布在纤维上用于转化氮氧化物的结构填料和整料的优选实施方案。在一个实施例中，波纹网状片材与陶瓷固体整体结构串联布置，波纹片材首先接收流体与待转化的至少一种氮氧化物，然后流体流入整料结构以完成转化。在其他实施例中，网状结构可以具有包括蜂窝结构的不同构造，并且可以包括金属，金属和陶瓷或陶瓷，并且可以是纤维状的。

4. 发明授权

US4876392A Process for preparation of keystones by oxidation of secondary alcohols using a trimetallic catalyst comprising molybdenum, rhenium and a group VIII noble metal 失效
标题翻译：通过使用包含钼，铼和VIII族贵金属的三金属催化剂氧化仲醇来制备基石的方法
公开(公告)号：US4876392A
公开(公告)日：1989-10-24
申请号：US174126
申请日：1988-03-28
申请人： Chuen Y. Yeh , Charles Savini
发明人： Chuen Y. Yeh , Charles Savini
IPC分类号： B01J23/36 , B01J23/656 , C07C45/28 , C07C45/29 , C07C45/34
CPC分类号： C07C45/34 , B01J23/36 , B01J23/6567 , C07C45/28 , C07C45/29
摘要： An improved process for preparing ketones by contacting a secondary aliphatic alcohol in the vapor phase with a trimetallic catalyst containing molybdenum, rhenium and a Group VIII noble metal.
摘要翻译：通过使气相中的仲脂族醇与含有钼，铼和VIII族贵金属的三金属催化剂接触来制备酮的改进方法。

5. 发明授权

US4088703A Recovery of phenol values from purification residues 失效
标题翻译：从净化残留物中回收苯酚值
公开(公告)号：US4088703A
公开(公告)日：1978-05-09
申请号：US407712
申请日：1973-10-18
申请人： Chuen Y. Yeh , F. Lewis Bohn , Harry E. Ulmer
发明人： Chuen Y. Yeh , F. Lewis Bohn , Harry E. Ulmer
IPC分类号： C07C29/20 , C07C35/08
CPC分类号： C07C29/20 , C07C2101/14
摘要： Processes for the recovery of phenol values as cyclohexanol from the purification residue obtained in the amine purification of phenol. The recovery of phenol values may be effected by hydrogenation in the presence of a nickel catalyst and distilling the hydrogenation product to obtain cyclohexanol. Alternatively, the purification residue may be distilled and the distillate hydrogenated to produce a hydrogenation product from which cyclohexanol may be recovered by a second distillation.
摘要翻译：从苯胺胺纯化中获得的纯化残余物中回收酚值为环己醇的方法。苯酚值的回收可以通过在镍催化剂存在下氢化并蒸馏氢化产物得到环己醇来进行。或者，可以蒸馏纯化残余物，并将馏出物氢化以产生氢化产物，通过第二次蒸馏可从中回收环己醇。

6. 发明授权

US07371910B2 Process for benzene alkylation and transalkylation of polyalkylated aromatics over improved zeolite beta catalyst 失效
标题翻译：多烷基化芳族化合物在改进的沸石β催化剂上苯烷基化和烷基转移的方法
公开(公告)号：US07371910B2
公开(公告)日：2008-05-13
申请号：US11000859
申请日：2004-12-01
申请人： Chuen Y. Yeh , Jinsuo Xu , Philip J. Angevine
发明人： Chuen Y. Yeh , Jinsuo Xu , Philip J. Angevine
IPC分类号： C07C2/64
CPC分类号： C07C2/66 , B01J29/06 , B01J29/7007 , B01J35/002 , B01J37/0009 , B01J37/08 , B01J2229/40 , B01J2229/64 , C01B37/00 , C01B39/02 , C01B39/04 , C01B39/48 , C07C2/58 , C07C6/126 , C07C2529/40 , C10G29/205 , C10G45/64 , C10G47/16 , Y02P20/52 , C07C15/073 , C07C9/21
摘要： An aromatic alkylation process includes contacting an aromatic compound with an alkylating agent in the presence of a zeolite beta in a reaction zone under alkylation reaction conditions, wherein said zeolite beta is a high performance zeolite beta possessing a ratio of strong acid sites/weak acid sites greater than 1. The high performance zeolite beta is superior to conventional zeolite beta in the aromatics alkylation reaction, such as benzene alkylation with ethylene for ethylbenzene production, and benzene alkylation with propylene for cumene production.
摘要翻译：芳族烷基化方法包括在烷基化反应条件下在反应区中在β沸石存在下使芳族化合物与烷基化剂接触，其中所述沸石β是具有强酸性位点/弱酸性位点的比例的高性能沸石β 大于1.在芳族烷基化反应中，高性能沸石β优于常规沸石β，例如用乙烯生产乙烯的苯烷基化和用丙烯生产异丙苯的苯烷基化。

7. 发明授权

US07304199B2 Solid acid catalyst and method of using same 有权
标题翻译：固体酸催化剂及其使用方法
公开(公告)号：US07304199B2
公开(公告)日：2007-12-04
申请号：US10824390
申请日：2004-04-14
申请人： Jinsuo Xu , Chuen Y. Yeh , Philip J. Angevine
发明人： Jinsuo Xu , Chuen Y. Yeh , Philip J. Angevine
IPC分类号： C07C5/22 , C07C6/08 , C07C2/58 , C01G11/00 , B01J27/053
CPC分类号： B01J23/6527 , B01J21/063 , B01J21/066 , B01J23/24 , B01J23/30 , B01J23/652 , B01J27/053 , B01J27/057 , B01J37/0009 , B01J37/08 , C07C5/2772 , C07C2523/652 , C10G45/60 , C10G45/62 , C10G47/02 , C10G49/04 , C10G2300/1081 , C10G2300/4018 , C07C9/00
摘要： A catalyst composition includes an oxygen compound of an element selected from Group IVB or Group IVA of the Periodic Table of the Elements; an oxygen compound of an element selected from Group VIB or Group VIA of the Periodic Table of the Elements; and at least about 1% by weight based upon total catalyst weight of fumed silica particles. The catalyst composition is advantageously employed in hydrocarbon conversion processes such as isomerization.
摘要翻译：催化剂组合物包括选自元素周期表的IVB族或IVA族元素的元素的氧化合物; 选自元素周期表的VIB族或VIA族的元素的氧化合物; 和基于热解二氧化硅颗粒的总催化剂重量的至少约1重量％。催化剂组合物有利地用于烃转化过程如异构化。

8. 发明授权

US06946107B2 Conversion of nitrogen oxides in the presence of a catalyst supported on a mesh-like structure 有权
标题翻译：在负载在网状结构上的催化剂存在下氮氧化物的转化
公开(公告)号：US06946107B2
公开(公告)日：2005-09-20
申请号：US10385369
申请日：2003-03-10
申请人： Joakim A. Carlborg , Yun-Feng Chang , Lawrence L. Murrell , Robert E. Trubac , Rudolf A. Overbeek , Verena R. Schmidt , Chuen Y. Yeh , Lothar Schuh
发明人： Joakim A. Carlborg , Yun-Feng Chang , Lawrence L. Murrell , Robert E. Trubac , Rudolf A. Overbeek , Verena R. Schmidt , Chuen Y. Yeh , Lothar Schuh
IPC分类号： B01D53/86 , B01D53/88 , B01D53/94 , B01J21/06 , B01J23/22 , B01J23/30 , B01J23/42 , B01J35/04 , B01J35/06 , B01J37/02 , F01N3/28 , F01N13/02 , B01J8/00 , C01B21/00
CPC分类号： B01J23/22 , B01D53/8631 , B01D53/864 , B01D53/8687 , B01D53/885 , B01D53/9431 , B01D53/9477 , B01D2257/402 , B01D2257/502 , B01D2257/702 , B01D2257/708 , B01J21/063 , B01J21/066 , B01J23/30 , B01J23/42 , B01J35/04 , B01J35/06 , B01J37/0225 , B01J37/0228 , F01N3/281 , F01N3/2814 , F01N3/2821 , F01N3/2828 , F01N3/2835 , F01N13/0097 , F01N2330/10 , F01N2330/12 , F01N2330/14 , F01N2330/38 , Y02C20/10 , Y02P20/153
摘要： An apparatus for converting at least one nitrogen oxide, such as NO, O2, or N2O converts oxide in the presence of a catalyst supported on a metal mesh-like structure. The mesh-like structure is preferably fibrous formed of metal or ceramic fibers which may include knitted wire, sintered metal fibers and so on and has a porosity greater than about 85%. The mesh is formed into channels, preferably corrugations, and includes vortex generators, which generate turbulence to create a pressure differential across the mesh, to promote flow of fluids through the mesh pores which normally do not exhibit flow therethrough in the absence of such pressure differential. Preferred embodiments of structured packing and monoliths are disclosed each having a catalyst preferably in the mesh pores and/or coated on the fibers for converting the nitrogen oxide. In one embodiment, corrugated mesh-like sheets are arranged in series with a ceramic solid monolith structure with the corrugated sheets initially receiving the fluid with the at least one nitrogen oxide to be converted and which fluid then flows into the monolith structure to complete the conversion. In other embodiments, the mesh-like structure may have different configurations including a honeycomb arrangement and may include metal, metal and ceramic or ceramic and may be fibrous.
摘要翻译：用于转化至少一种氮氧化物如NO 2 O 2或N 2 O 2的装置在负载在金属网状物上的催化剂存在下转化氧化物结构体。网状结构优选由金属或陶瓷纤维形成，其可以包括针织线，烧结金属纤维等，并且具有大于约85％的孔隙率。网格形成通道，优选波纹，并且包括涡流发生器，其产生湍流以产生横跨网孔的压力差，以促进流体流过网孔，其通常在没有这种压力差的情况下不显示流过其中。公开了优选在网孔中具有催化剂和/或涂布在纤维上用于转化氮氧化物的结构填料和整料的优选实施方案。在一个实施例中，波纹网状片材与陶瓷固体整体结构串联布置，波纹片材首先接收流体与待转化的至少一种氮氧化物，然后流体流入整料结构以完成转化。在其他实施例中，网状结构可以具有包括蜂窝结构的不同构造，并且可以包括金属，金属和陶瓷或陶瓷，并且可以是纤维状的。

9. 发明授权

US06930217B2 Catalyst containing microporous zeolite in mesoporous support and method for making same 失效
标题翻译：含有介孔载体中的微孔沸石的催化剂及其制备方法
公开(公告)号：US06930217B2
公开(公告)日：2005-08-16
申请号：US10875087
申请日：2004-06-24
申请人： Zhiping Shan , Jacobus Cornelius Jansen , Chuen Y. Yeh , Johannes Hendrik Koegler , Thomas Maschmeyer
发明人： Zhiping Shan , Jacobus Cornelius Jansen , Chuen Y. Yeh , Johannes Hendrik Koegler , Thomas Maschmeyer
IPC分类号： C01B13/14 , B01J21/06 , B01J21/12 , B01J23/26 , B01J23/38 , B01J23/44 , B01J23/50 , B01J23/52 , B01J29/00 , B01J29/03 , B01J29/04 , B01J29/08 , B01J29/40 , B01J29/70 , B01J29/80 , B01J29/87 , B01J29/88 , B01J29/89 , B01J32/00 , B01J35/00 , B01J35/10 , B01J37/00 , B01J37/03 , B01J37/08 , B01J37/10 , C01B13/32 , C01B13/36 , C01B33/113 , C01B33/12 , C01B33/26 , C01B37/00 , C01B37/02 , C01B39/00 , C07B61/00 , C07C2/66 , C07C15/073 , C07C45/46 , C07D301/06 , C07D301/10 , C10G2/00 , C10G11/04 , C10G11/05 , C10G27/04 , C10G29/20 , C10G35/095 , C10G45/00 , C10G45/04 , C10G45/12 , C10G45/60 , C10G45/62 , C10G45/64 , C10G47/14 , C10G47/16 , C10G47/20 , C10G49/08 , C10G50/00 , C07C2/58 , C07C5/22 , C10G11/00 , C10G73/02
CPC分类号： B82Y30/00 , B01J21/06 , B01J21/12 , B01J23/26 , B01J23/38 , B01J23/44 , B01J23/50 , B01J23/52 , B01J29/005 , B01J29/0308 , B01J29/04 , B01J29/041 , B01J29/084 , B01J29/40 , B01J29/70 , B01J29/7007 , B01J29/80 , B01J29/87 , B01J29/88 , B01J29/89 , B01J35/002 , B01J35/1023 , B01J35/1038 , B01J35/1047 , B01J35/1057 , B01J35/1061 , B01J35/108 , B01J35/109 , B01J37/0018 , B01J37/033 , B01J37/10 , B01J2229/32 , B01J2229/36 , B01J2229/42 , B01J2229/62 , C01B13/366 , C01B33/126 , C01B37/005 , C01B37/02 , C01P2006/12 , C01P2006/14 , C01P2006/16 , C07C2/66 , C07C45/46 , C07D301/06 , C07D301/10 , C10G2/332 , C10G11/04 , C10G11/05 , C10G27/04 , C10G29/205 , C10G45/00 , C10G45/04 , C10G45/12 , C10G45/60 , C10G45/62 , C10G45/64 , C10G47/14 , C10G49/08 , C10G50/00 , C07C15/073 , C07C49/84
摘要： A catalytic material includes a microporous zeolite supported on a mesoporous inorganic oxide support. The microporous zeolite can include zeolite beta, zeolite Y or ZSM-5. The mesoporous inorganic oxide can be, e.g., silica or alumina, and can optionally include other metals. Methods for making and using the catalytic material are described herein.
摘要翻译：催化材料包括负载在介孔无机氧化物载体上的微孔沸石。微孔沸石可以包括沸石β，沸石Y或ZSM-5。介孔无机氧化物可以是例如二氧化硅或氧化铝，并且可以任选地包括其它金属。本文描述了制备和使用催化材料的方法。

10. 发明授权

US06350429B1 Method for making molecular sieves and novel molecular sieve compositions 有权
标题翻译：制备分子筛和新型分子筛组合物的方法
公开(公告)号：US06350429B1
公开(公告)日：2002-02-26
申请号：US09465029
申请日：1999-12-16
申请人： Lawrence L. Murrell , Rudolf A. Overbeek , Yun-feng Chang , Nelleke Van Der Puil , Chuen Y. Yeh
发明人： Lawrence L. Murrell , Rudolf A. Overbeek , Yun-feng Chang , Nelleke Van Der Puil , Chuen Y. Yeh
IPC分类号： C01B3704
CPC分类号： B01J29/035 , B01J29/084 , B01J29/40 , B01J29/7007 , B01J2229/60 , B01J2229/64 , C01B37/00 , C01B37/02 , C01B39/00 , C01B39/24 , C01B39/38 , C01B39/46 , Y10S423/21 , Y10S423/22 , Y10S423/27 , Y10S423/30
摘要： This invention relates to the synthesis of large pore composite molecular sieves and to the synthetic large pore composite molecular sieves so produced. The molecular sieves of the invention have the same general utilities of the comparable molecular sieves of the prior art but have been found to be superior catalysts and absorbents. This invention relates to a hydrothermal synthesis of large pore molecular sieves from nutrients, at least one of which contains an amorphous framework-structure, and which framework-structure is essentially retained in the synthetic molecular sieve. This invention stems from a discovery that the intrinsic porosity characteristics of a nutrient that possesses an amorphous cation oxide-framework can be substantially retained in the final molecular sieve containing product formed by a hydrothermal process by carefully controlling the conditions under which the hydrothermal process is conducted. For example, the invention contemplates retention of the particle size in a final molecular sieve-containing product that corresponds with that of an amorphous cation oxide-framework nutrient used in its manufacture. This invention drives the selection of process conditions to achieve one or more of macro and meso porosity (“large pore composite porosity”) in the final molecular sieve product as a direct product of the hydrothermal reaction producing the molecular sieve. The invention allows the production of a molecular sieve that is in situ incorporated in the framework morphology of a solid cation oxide-framework used in the molecular sieve's manufacture.
摘要翻译：本发明涉及大孔复合分子筛的合成以及如此生产的合成大孔复合分子筛。本发明的分子筛具有与现有技术相当的分子筛相同的通用效用，但已被发现是优异的催化剂和吸收剂。本发明涉及从营养物质中大量分子筛的水热合成，其中至少一种含有无定形骨架结构，其中骨架结构基本上保留在合成分子筛中。本发明源自一个发现，即通过仔细控制进行水热处理的条件，具有无定形阳离子氧化物 - 框架的营养物质的固有孔隙特性可以基本上保留在通过水热法形成的含最终分子筛的产品中。例如，本发明考虑到在与其制造中使用的无定形阳离子氧化物 - 骨架营养物相当的最终的含分子筛的产品中保留粒度。本发明驱动工艺条件的选择，以实现最终分子筛产物中作为产生分子筛的水热反应的直接产物的宏观和中孔多孔性（“大孔复合孔隙率”）中的一种或多种。本发明允许生产分子筛，其原位掺入分子筛制造中使用的固体阳离子氧化物框架的骨架形态。

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