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31. 发明授权

US6013848A Conversion of heavy polyalkylaromatic compounds 失效
标题翻译：重质聚烷基芳族化合物的转化
公开(公告)号：US6013848A
公开(公告)日：2000-01-11
申请号：US889729
申请日：1997-07-08
申请人： Jamin Chen , Chuen Y. Yeh
发明人： Jamin Chen , Chuen Y. Yeh
IPC分类号： C07C6/12 , C07C15/02 , C07C15/073 , C07C15/085 , C07C1/00 , C07C2/64 , C07C2/68 , C07C5/22
CPC分类号： C07C15/085 , C07C15/02 , C07C15/073 , C07C6/126 , C07C2529/08 , Y02P20/127
摘要： A process for the conversion of heavy bottoms from aromatic alkylation known as "flux oil" and containing heavier polyalkylaromatic compounds, in which the heavier polyalkylates are fed along with aromatic to a reactor containing an acidic zeolite catalyst for conversion to light mono-, and poly alkylaromatic compounds. The light polyalkylates may then be transalkylated with benzene to form additional monoalkylate.
摘要翻译：将重质底部物质从称为“助熔剂油”并含有较重的多烷基芳族化合物的芳族烷基化转化的方法，其中较重的多烷基化物与芳族化合物一起进料到含有酸性沸石催化剂的反应器中以转化为光单 - 和聚烷基芳族化合物。然后轻的聚烷基化物可以与苯进行烷基交换以形成另外的单烷基化。

32. 发明授权

US6004527A Method for making molecular sieves and novel molecular sieve compositions 失效
标题翻译：制备分子筛和新型分子筛组合物的方法
公开(公告)号：US6004527A
公开(公告)日：1999-12-21
申请号：US939271
申请日：1997-09-29
申请人： Lawrence L. Murrell , Rudolf A. Overbeek , Yun-feng Chang , Nelleke Van der Puil , Chuen Y. Yeh
发明人： Lawrence L. Murrell , Rudolf A. Overbeek , Yun-feng Chang , Nelleke Van der Puil , Chuen Y. Yeh
IPC分类号： C01B37/00 , C01B37/02 , C01B39/00 , C01B39/24 , C01B39/38 , C01B39/46 , C01B39/02 , C01B39/20
CPC分类号： B01J29/035 , B01J29/084 , B01J29/40 , B01J29/7007 , C01B37/00 , C01B37/02 , C01B39/00 , C01B39/24 , C01B39/38 , C01B39/46 , B01J2229/60 , B01J2229/64 , Y10S423/21 , Y10S423/22 , Y10S423/27 , Y10S423/30
摘要： This invention relates to the synthesis of large pore composite molecular sieves and to the synthetic large pore composite molecular sieves so produced. The molecular sieves of the invention have the same general utilties of the comparable molecular sieves of the prior art but have been found to be superior catalysts and absorbents. This invention relates to a hydrothermal synthesis of large pore molecular sieves from nutrients, at least one of which contains an amorphous framework-structure, and which framework-structure is essentially retained in the synthetic molecular sieve. This invention stems from a discovery that the intrinsic porosity characteristics of a nutrient that possesses an amorphous cation oxide-framework can be substantially retained in the final molecular sieve containing product formed by a hydrothermal process by carefully controlling the conditions under which the hydrothermal process is conducted. For example, the invention contemplates retention of the particle size in a final molecular sieve-containing product that corresponds with that of an amorphous cation oxide-framework nutrient used in its manufacture. This invention drives the selection of process conditions to achieve one or more of macro and meso porosity ("large pore composite porosity") in the final molecular sieve product as a direct product of the hydrothermal reaction producing the molecular sieve. The invention allows the production of a molecular sieve that is in situ incorporated in the framework morphology of a solid cation oxide-framework used in the molecular sieve's manufacture.
摘要翻译：本发明涉及大孔复合分子筛的合成以及如此生产的合成大孔复合分子筛。本发明的分子筛具有与现有技术相当的分子筛相同的一般用途，但已被发现是优异的催化剂和吸收剂。本发明涉及从营养物质中大量分子筛的水热合成，其中至少一种含有无定形骨架结构，其中骨架结构基本上保留在合成分子筛中。本发明源自一个发现，即通过仔细控制进行水热处理的条件，具有无定形阳离子氧化物 - 框架的营养物质的固有孔隙特性可以基本上保留在通过水热法形成的含最终分子筛的产品中。例如，本发明考虑到在与其制造中使用的无定形阳离子氧化物 - 骨架营养物相当的最终的含分子筛的产品中保留粒度。本发明驱动工艺条件的选择，以实现最终分子筛产物中作为产生分子筛的水热反应的直接产物的宏观和中孔多孔性（“大孔复合孔隙率”）中的一种或多种。本发明允许生产分子筛，其原位掺入分子筛制造中使用的固体阳离子氧化物框架的骨架形态。

33. 发明授权

US4649223A Catalysts and process for the conversion of olefins to ketones 失效
标题翻译：用于将烯烃转化为酮的催化剂和方法
公开(公告)号：US4649223A
公开(公告)日：1987-03-10
申请号：US776790
申请日：1985-09-16
申请人： Chuen Y. Yeh , Charles Savini
发明人： Chuen Y. Yeh , Charles Savini
IPC分类号： B01J23/36 , B01J23/656 , C07C45/28 , C07C45/29 , C07C45/34 , C07C45/00
CPC分类号： C07C45/34 , B01J23/36 , B01J23/6567 , C07C45/28 , C07C45/29
摘要： An improved process is provided for forming ketones from the corresponding olefins in the vapor phase in the presence of water vapor employing a heterogeneous catalyst comprising rhenium compounds and complexes, optionally containing at least one metal compound or complex selected from the group consisting of Group VIB metals and Group VIII noble metals, and mixtures thereof. It has been surprisingly found that these catalysts effect the formation of ketones in high selectivities with minimal selectivities to the undesirable carbon dioxide and carbon monoxide by-products.
摘要翻译：提供了一种改进的方法，用于在水蒸气存在下，使用包含铼化合物和配合物的非均相催化剂，任选地含有至少一种金属化合物或选自由VIB族金属组成的组的复合物，在蒸气相中形成酮和VIII族贵金属及其混合物。已经令人惊奇地发现，这些催化剂以高选择性的方式影响酮的形成，对不期望的二氧化碳和一氧化碳副产物的选择性最小。

34. 发明授权

US4560805A Catalysts and process for the conversion of olefins to ketones 失效
公开(公告)号：US4560805A
公开(公告)日：1985-12-24
申请号：US516902
申请日：1983-07-25
申请人： Chuen Y. Yeh , Charles Savini
发明人： Chuen Y. Yeh , Charles Savini
IPC分类号： B01J23/36 , B01J23/656 , C07C45/28 , C07C45/29 , C07C45/34 , C07C45/42
CPC分类号： C07C45/34 , B01J23/36 , B01J23/6567 , C07C45/28 , C07C45/29
摘要： An improved process is provided for forming ketones from the corresponding olefins in the vapor phase in the presence of water vapor employing a heterogeneous catalyst comprising rhenium compounds and complexes, optionally containing at least one metal compound or complex selected from the group consisting of Group VIB metals and Group VIII noble metals, and mixtures thereof. It has been surprisingly found that these catalysts effect the formation of ketones in high selectivities with minimal selectivities to the undesirable carbon dioxide and carbon monoxide by-products.

35. 发明授权

US5252197A Process for upgrading gasolines and other hydrocarbon mixtures 失效
标题翻译：汽油和其他烃类混合物的升级方法
公开(公告)号：US5252197A
公开(公告)日：1993-10-12
申请号：US952352
申请日：1992-09-28
申请人： Anatoly Alexander , Chuen Y. Yeh , George D. Suciu
发明人： Anatoly Alexander , Chuen Y. Yeh , George D. Suciu
IPC分类号： C10G35/095 , C10G35/04
CPC分类号： C10G35/095
摘要： A process for upgrading gasolines and other hydrocarbon mixtures. The hydrocarbon mixture is contacted with a large pore zeolite catalyst in order to crack n-paraffins to form olefins and lower molecular weight n-paraffins, to cause the olefins to react with benzene in order to form alkylbenzenes, and to catalyze the isomerization of the n-paraffins to form i-paraffins. Preferably, all of the above reactions occur in a single reactant mixture in the presence of a zeolite catalyst having ten and/or twelve membered ring-type structures. The process of the invention reduces the benzene quantity of the hydrocarbon mixture and increases its octane number.
摘要翻译：汽油和其他烃混合物的升级方法。将烃混合物与大孔沸石催化剂接触以裂解正链烷烃以形成烯烃和较低分子量的正链烷烃，以使烯烃与苯反应以形成烷基苯，并催化异构化正链烷烃形成正链烷烃。优选地，在具有十个和/或十二元环型结构的沸石催化剂的存在下，所有上述反应都发生在单一反应物混合物中。本发明的方法降低烃混合物的苯量并增加其辛烷值。

36. 发明授权

US4737482A Catalysts for oxidation of olefins to ketones 失效
标题翻译：用于将烯烃氧化成酮的催化剂
公开(公告)号：US4737482A
公开(公告)日：1988-04-12
申请号：US776228
申请日：1985-09-16
申请人： Chuen Y. Yeh , Charles Savini
发明人： Chuen Y. Yeh , Charles Savini
IPC分类号： B01J23/36 , B01J23/656 , C07C45/28 , C07C45/29 , C07C45/34 , B01J27/051 , B01J27/045 , B01J27/047 , B01J27/049
CPC分类号： C07C45/29 , B01J23/36 , B01J23/6567 , C07C45/28 , C07C45/34
摘要： An improved process is provided for forming ketones from the corresponding olefins by vapor phase oxidiation of the olefin in the presence of molecular oxygen and water vapor employing a heterogeneous catalyst comprising rhenium compounds and complexes, optionally containing at least one metal compound or complex selected from the group consisting of Group VIB metals and Group VIII noble metals, and mixtures thereof. It has been surprisingly found that these catalysts effect the formation of ketones in high selectivities with minimal selectivities to the undesirable carbon dioxide and carbon monoxide by-products.
摘要翻译：提供了一种改进的方法，用于在分子氧和水蒸汽的存在下，使用包含铼化合物和络合物的非均相催化剂，任选地含有至少一种选自以下的金属化合物或络合物的复合物，通过气相氧化烯烃从相应的烯烃形成酮：由VIB族金属和VIII族贵金属组成的组，及其混合物。已经令人惊奇地发现，这些催化剂以高选择性的方式影响酮的形成，对不期望的二氧化碳和一氧化碳副产物的选择性最小。

37. 发明授权

US4560804A Catalytic process for the manufacture of ketones 失效
标题翻译：用于制造酮的催化方法
公开(公告)号：US4560804A
公开(公告)日：1985-12-24
申请号：US516537
申请日：1983-07-25
申请人： Chuen Y. Yeh , Charles Savini
发明人： Chuen Y. Yeh , Charles Savini
IPC分类号： B01J27/04 , C07C45/28 , C07C45/34 , C07C45/42
CPC分类号： B01J27/04 , C07C45/28 , C07C45/34
摘要： An improved process is provided for forming ketones from the corresponding olefins by vapor phase oxidation of the olefin in the presence of water vapor, and optionally in the additional presence of molecular oxygen employing a heterogeneous catalyst comprising at least one member selected from the group consisting of Ce, Nd and La and compounds and complexes thereof, optionally containing at least one metal compound or complex selected from the group consisting of Group VIB metals and Group VIII noble metals, and mixtures thereof. It has been surprisingly found that these catalysts effect the formation of ketones in high selectivities with minimal selectivities to the undesirable carbon dioxide and carbon monoxide by-products.
摘要翻译：提供了一种改进的方法，用于在水蒸气存在下通过气相氧化烯烃从相应的烯烃形成酮，并且任选地在额外存在分子氧的情况下，使用包含至少一种选自以下的组分的多相催化剂： Ce，Nd和La及其化合物和络合物，任选地含有至少一种选自VIB族金属和VIII族贵金属的金属化合物或络合物，及其混合物。已经令人惊奇地发现，这些催化剂以高选择性的方式影响酮的形成，对不期望的二氧化碳和一氧化碳副产物的选择性最小。

38. 发明授权

US4560803A Catalysts and process for oxidation of olefins to ketones 失效
标题翻译：将烯烃氧化成酮的催化剂和方法
公开(公告)号：US4560803A
公开(公告)日：1985-12-24
申请号：US516901
申请日：1983-07-25
申请人： Chuen Y. Yeh , Charles Savini
发明人： Chuen Y. Yeh , Charles Savini
IPC分类号： B01J23/36 , B01J23/656 , C07C45/28 , C07C45/29 , C07C45/34 , C07C45/39
CPC分类号： C07C45/34 , B01J23/36 , B01J23/6567 , C07C45/28 , C07C45/29
摘要： An improved process is provided for forming ketones from the corresponding olefins by vapor phase oxidation of the olefin in the presence of molecular oxygen and water vapor employing a heterogeneous catalyst comprising rhenium compounds and complexes, optionally containing at least one metal compound or complex selected from the group consisting of Group VIB metals and Group VIII noble metals, and mixtures thereof. It has been surprisingly found that these catalysts effect the formation of ketones in high selectivities with minimal selectivities to the undesirable carbon dioxide and carbon monoxide by-products.
摘要翻译：提供了一种改进的方法，用于通过使用包含铼化合物和络合物的非均相催化剂在分子氧和水蒸汽存在下气相氧化烯烃来形成酮，任选地含有至少一种选自以下的金属化合物或络合物：由VIB族金属和VIII族贵金属组成的组，及其混合物。已经令人惊奇地发现，这些催化剂以高选择性的方式影响酮的形成，对不期望的二氧化碳和一氧化碳副产物的选择性最小。

39. 发明授权

US4203923A Method for promotion of phenol hydrogenation 失效
标题翻译：苯酚氢化促进方法
公开(公告)号：US4203923A
公开(公告)日：1980-05-20
申请号：US667760
申请日：1976-03-17
申请人： Chuen Y. Yeh , Harry E. Ulmer
发明人： Chuen Y. Yeh , Harry E. Ulmer
IPC分类号： C07C29/20 , C07C45/00 , C07C41/00
CPC分类号： C07C29/20 , C07C45/006 , C07C2101/14
摘要： A method for promoting the hydrogenation of phenol to cyclohexanone in the presence of a non-promoted palladium catalyst which comprises effecting the hydrogenation reaction in the presence of an in situ promoter selected from the group consisting of alkalie metal and alkaline earth metal chlorides, fluorides, bicarbonates, carbonates, hydroxides and nitrates, ammonia, ammonium hydroxide, secondary amines and mixtures thereof.
摘要翻译：一种在非促进的钯催化剂存在下促进苯酚氢化成环己酮的方法，该方法包括在存在选自碱金属和碱土金属氯化物，氟化物的原位促进剂的情况下进行氢化反应，碳酸氢盐，碳酸盐，氢氧化物和硝酸盐，氨，氢氧化铵，仲胺及其混合物。

40. 发明授权

US4014867A Production of hexamethyleneimine from caprolactam 失效
标题翻译：由己内酰胺生产六亚甲基亚胺
公开(公告)号：US4014867A
公开(公告)日：1977-03-29
申请号：US616105
申请日：1975-09-23
申请人： Chuen Y. Yeh , Harry E. Ulmer
发明人： Chuen Y. Yeh , Harry E. Ulmer
IPC分类号： C07D295/023 , C07D295/02
CPC分类号： C07D295/023
摘要： A method of preparing hexamethyleneimine which comprises the steps of:A. forming a solution of .epsilon.-caprolactam in a solvent selected from the group consisting of linear and cyclic ethers and polyethers having a boiling point of at least about 100.degree. C, said solution having a concentration of about 1 to 40 percent by weight;B. contacting said solution with gaseous hydrogen in the presence of a catalyst comprising copper chromite and at a temperature of about 150 to 300.degree. C. and a pressure of at least about 1,000 psig, whereby a solution containing hexamethyleneimine is formed; andC. recovering hexamethyleneimine from said hexamethyleneimine-containing solution.
摘要翻译：一种制备六亚甲基亚胺的方法，包括以下步骤：

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